A method of producing a multi-layered functionalised graphene oxide paper, comprises the steps of providing an aqueous suspension of oxidised graphene oxide flakes, size reducing the oxidised graphene oxide flakes in the suspension to provide an aqueous suspension of particulate oxidised graphene oxide having an average particle size of less than 1 μm and drying the aqueous suspension in a vessel to provide a multi-layered graphene oxide material. The multi-layered graphene oxide material is annealed to provide a multi-layered reduced graphene oxide material, before surface grafting functional groups to the surface of the multi-layered reduced graphene oxide material by reacting the material with a functional group precursor in the presence of plasma. The use of a graphene oxide material to treat bone defects, and as an energy storage device, is also described.

Some implementations of the disclosure are directed to a method, comprising: receiving a sheet of graphite comprising a first surface and a second surface opposite the first surface; and perforating the sheet in a first plurality of locations from the first surface through the second surface to form a first plurality of perforations through the sheet and a first plurality of protrusions of the graphite oriented outward from the second surface, the first plurality of protrusions configured to conduct heat away from a plane of the sheet. Further implementations comprise perforating the sheet in a second plurality of locations from the second surface through the first surface to form a second plurality of perforations through the sheet and a second plurality of protrusions of graphite material oriented outward from the first surface, wherein the second plurality of protrusions are configured to conduct heat away from the plane of the sheet.

Some implementations of the disclosure are directed to a method, comprising: receiving a sheet of graphite comprising a first surface and a second surface opposite the first surface; and perforating the sheet in a first plurality of locations from the first surface through the second surface to form a first plurality of perforations through the sheet and a first plurality of protrusions of the graphite oriented outward from the second surface, the first plurality of protrusions configured to conduct heat away from a plane of the sheet. Further implementations comprise perforating the sheet in a second plurality of locations from the second surface through the first surface to form a second plurality of perforations through the sheet and a second plurality of protrusions of graphite material oriented outward from the first surface, wherein the second plurality of protrusions are configured to conduct heat away from the plane of the sheet.

Provided is a sulfur-carbon material composite body which, when used for an electrode of a secondary battery, is unlikely to degrade cycle characteristics at the time of charging and discharging of the secondary battery. Disclosed is a sulfur-carbon material composite body including a first carbon material having a graphene layered structure; a spacer at least partially disposed between graphene layers of the first carbon material or at an end of the first carbon material; and sulfur or a sulfur-containing compound at least partially disposed between the graphene layers of the first carbon material or at the end of the first carbon material.

Provided is a sulfur-carbon material composite body which, when used for an electrode of a secondary battery, is unlikely to degrade cycle characteristics at the time of charging and discharging of the secondary battery. Disclosed is a sulfur-carbon material composite body including a first carbon material having a graphene layered structure; a spacer at least partially disposed between graphene layers of the first carbon material or at an end of the first carbon material; and sulfur or a sulfur-containing compound at least partially disposed between the graphene layers of the first carbon material or at the end of the first carbon material.

Provided is a carbon material that can improve characteristics such as electrostatic capacitance and rate characteristics of the power storage device. A carbon material used for an electrode material of a power storage device, the carbon material having a graphene layered structure, and in a small-angle X-ray scattering spectrum of the carbon material, a slope of a straight line connecting a point indicating a scattering intensity when a natural logarithm LN (q) of a scattering vector is −1.5 and a point indicating a natural logarithm of a scattering intensity when the natural logarithm LN (q) of the scattering vector is 1.4 being −1.5 or less.

A coating layer for a substrate includes a coating material. The coating material includes graphene and/or graphene derivatives that reflect and/or absorb an electromagnetic (EM) wave having a frequency of above 20 GHz. The coating layer is deposited on a surface of the substrate.

Described herein are methods for continuous production of an exfoliated two-dimensional (2D) material comprising passing a 2D material mixture through a convergent-divergent nozzle, the 2D material mixture comprising a 2D layered material and a compressible fluid. The method of the present disclosure employs physical compression and expansion of a flow of high-pressure gases, leaving the 2D layered material largely defect free to produce an exfoliated 2D layered in a simple, continuous, and environmentally friendly manner.

Described herein are methods for continuous production of an exfoliated two-dimensional (2D) material comprising passing a 2D material mixture through a convergent-divergent nozzle, the 2D material mixture comprising a 2D layered material and a compressible fluid. The method of the present disclosure employs physical compression and expansion of a flow of high-pressure gases, leaving the 2D layered material largely defect free to produce an exfoliated 2D layered in a simple, continuous, and environmentally friendly manner.

A solution is prepared that contains (A) a polymer compound that includes at least one of a hydrolyzable polymer compound or a thermally-decomposable polymer compound, (B) an oxoacid-based compound that includes at least one of a phosphate-based compound, a sulfate-based compound, a sulfonate-based compound, or a perchlorate-based compound, and (C) a laminate of layered substances, and the solution is irradiated with at least one of sonic waves or radio waves, or the solution is heated.