It remains a challenge to generate coherent radiation in the spectral range of 0.1-10 THz (“the THz gap”), a band for applications ranging from spectroscopy to security and high-speed wireless communications. Here, we disclose how to produce coherent radiation spanning the THz gap using efficient second-harmonic generation (SHG) in low-loss dielectric structures, starting from an electronic oscillator (EO) that generates coherent radiation at frequencies of about 100 GHz. The EO is coupled to cascaded, hybrid THz-band dielectric cavities that combine (1) extreme field concentration in high-quality-factor resonators with (2) nonlinear materials enhanced by phonon resonances. These cavities convert the input radiation into higher-frequency coherent radiation at conversion efficiencies of >10.sup.3%/W, making it possible to bridge the THz gap with 1 W of input power. This approach enables efficient, cascaded parametric frequency converters, representing a new generation of light sources extensible into the mid-IR spectrum and beyond.

It remains a challenge to generate coherent radiation in the spectral range of 0.1-10 THz (“the THz gap”), a band for applications ranging from spectroscopy to security and high-speed wireless communications. Here, we disclose how to produce coherent radiation spanning the THz gap using efficient second-harmonic generation (SHG) in low-loss dielectric structures, starting from an electronic oscillator (EO) that generates coherent radiation at frequencies of about 100 GHz. The EO is coupled to cascaded, hybrid THz-band dielectric cavities that combine (1) extreme field concentration in high-quality-factor resonators with (2) nonlinear materials enhanced by phonon resonances. These cavities convert the input radiation into higher-frequency coherent radiation at conversion efficiencies of >10.sup.3%/W, making it possible to bridge the THz gap with 1 W of input power. This approach enables efficient, cascaded parametric frequency converters, representing a new generation of light sources extensible into the mid-IR spectrum and beyond.

Apparatus and methods for producing ultrashort optical pulses are described. A high-power, solid-state, passively mode-locked laser can be manufactured in a compact module that can be incorporated into a portable instrument. The mode-locked laser can produce sub-50-ps optical pulses at a repetition rates between 200 MHz and 50 MHz, rates suitable for massively parallel data-acquisition. The optical pulses can be used to generate a reference clock signal for synchronizing data-acquisition and signal-processing electronics of the portable instrument.

Apparatus and methods for producing ultrashort optical pulses are described. A high-power, solid-state, passively mode-locked laser can be manufactured in a compact module that can be incorporated into a portable instrument. The mode-locked laser can produce sub-50-ps optical pulses at a repetition rates between 200 MHz and 50 MHz, rates suitable for massively parallel data-acquisition. The optical pulses can be used to generate a reference clock signal for synchronizing data-acquisition and signal-processing electronics of the portable instrument.

Methods and systems are provided for separating polarized UV light. In one example, a method may include passing polarized source light through a group of at least four prisms to collimate and separate a second-harmonic generation (SHG) beam from a pump beam. The separated SHG beam may then be further passed through a spatial filter to reduce spatial distribution.

Methods and systems are provided for separating polarized UV light. In one example, a method may include passing polarized source light through a group of at least four prisms to collimate and separate a second-harmonic generation (SHG) beam from a pump beam. The separated SHG beam may then be further passed through a spatial filter to reduce spatial distribution.

Single crystals of a new noncentrosymmetric polar oxysulfide SrZn.sub.2S.sub.2O (s.g. Pmn2.sub.1) grown in a eutectic KF-KCl flux with unusual wurtzite-like slabs consisting of close-packed corrugated double layers of ZnS.sub.3O tetrahedra vertically separated from each other by Sr atoms and methods of making same.

A pulsed third-harmonic laser system includes a pulsed laser, an extra-cavity nonlinear crystal, and an intracavity nonlinear crystal. The pulsed laser generates fundamental laser pulses and couples out a portion of each fundamental laser pulse out of the laser resonator to undergo second-harmonic-generation in the extra-cavity nonlinear crystal. Resulting second-harmonic laser pulses are directed back into the laser resonator and mixes with the fundamental laser pulses in the intracavity nonlinear crystal to generate third-harmonic laser pulses. The pulsed third-harmonic laser system thus maintains a non-zero output coupling efficiency regardless of the efficiency of the second-harmonic-generation stage, while the third-harmonic-generation stage benefits from the intracavity power of the fundamental laser pulses.

A pulsed third-harmonic laser system includes a pulsed laser, an extra-cavity nonlinear crystal, and an intracavity nonlinear crystal. The pulsed laser generates fundamental laser pulses and couples out a portion of each fundamental laser pulse out of the laser resonator to undergo second-harmonic-generation in the extra-cavity nonlinear crystal. Resulting second-harmonic laser pulses are directed back into the laser resonator and mixes with the fundamental laser pulses in the intracavity nonlinear crystal to generate third-harmonic laser pulses. The pulsed third-harmonic laser system thus maintains a non-zero output coupling efficiency regardless of the efficiency of the second-harmonic-generation stage, while the third-harmonic-generation stage benefits from the intracavity power of the fundamental laser pulses.

A system for nonlinear frequency conversion includes an acousto-optic modulator for diffracting a portion of an input laser beam as a first-order beam and transmitting a non-diffracted portion of the input laser beam as a zeroth-order beam. The system also includes a nonlinear crystal arranged to receive and frequency convert each of the zeroth-order and first-order beams to generate two respective frequency-converted laser beams, whereby, when the acousto-optic modulator changes the average-power ratio between the zeroth-order and first-order beams, variations of the heat load in the nonlinear crystal are minimized. Either one of the two frequency-converted laser beams may be used as an output laser beam of the system, while the other one of the two frequency-converted laser beams serves to stabilize the heat load in the nonlinear crystal when the acousto-optic modulator is operated to change the average power in the output laser beam.