A compound is represented by Formula (1) below,

##STR00001##

in Formula (1) above, R.sup.1 to R.sup.22 each independently contain at least one atom selected from the group consisting of H, B, C, N, O, F, Si, P, S, Cl, I, and Br, and L.sup.1 and L.sup.2 each independently represent a single bond or CC.

A compound is represented by Formula (1) below,

##STR00001##

in Formula (1) above, R.sup.1 to R.sup.22 each independently contain at least one atom selected from the group consisting of H, B, C, N, O, F, Si, P, S, Cl, I, and Br, and L.sup.1 and L.sup.2 each independently represent a single bond or CC.

Organic dyes that are covalently bonded multimers or higher order symmetrical structures where one or more dye units may optionally contain deuterium substitutions are disclosed. The disclosed dyes are particularly useful for optical coatings, new optical nanomaterials, high density storage devices. The structural and optical characteristics of the disclosed dyes provide avenues for increased information-content through surface-enhanced Raman resonance spectroscopy.

Organic dyes that are covalently bonded multimers or higher order symmetrical structures where one or more dye units may optionally contain deuterium substitutions are disclosed. The disclosed dyes are particularly useful for optical coatings, new optical nanomaterials, high density storage devices. The structural and optical characteristics of the disclosed dyes provide avenues for increased information-content through surface-enhanced Raman resonance spectroscopy.

Method for manufacturing an optical information recording medium includes: preparing a substrate material where a first guide groove has been formed on a first side of the substrate material; forming a second guide groove by applying an energy-curable resin material between a second side of the substrate material opposite to the first side and a stamper and subsequently curing the energy-curable resin material to form a substrate; providing at least one recording layer and a cover layer on a first side of the substrate where the first guide groove has been formed, while holding the substrate with the stamper left unremoved from the substrate to protect the second guide groove; and exposing the second guide groove by removing the stamper and providing at least one recording layer and a cover layer on a second side of the substrate where the second guide groove has been formed.

Method for manufacturing an optical information recording medium includes: preparing a substrate material where a first guide groove has been formed on a first side of the substrate material; forming a second guide groove by applying an energy-curable resin material between a second side of the substrate material opposite to the first side and a stamper and subsequently curing the energy-curable resin material to form a substrate; providing at least one recording layer and a cover layer on a first side of the substrate where the first guide groove has been formed, while holding the substrate with the stamper left unremoved from the substrate to protect the second guide groove; and exposing the second guide groove by removing the stamper and providing at least one recording layer and a cover layer on a second side of the substrate where the second guide groove has been formed.

A nonlinear optical dye includes a compound represented by the general formula (1) below. ##STR00001## In the above general formula (1), each of X.sup.1, X.sup.2, X.sup.3 and X.sup.4 independently represents a hydrogen atom, an alkyl group having a carbon number of 1 to 6, a halogen atom, a hydroxyl group, a nitro group, a cyano group, or a methylsulfonyl group. In the present invention, it is preferred that each of X.sup.1, X.sup.2, X.sup.3 and X.sup.4 independently represents a hydrogen atom, an alkyl group having a carbon number of 1 to 6, or a halogen atom. In the present invention, it is also preferred that the nonlinear optical dye has a dipole moment of 2.1 D or less and a maximum absorption wavelength within a range of 315 to 360 nm.

A nonlinear optical dye includes a compound represented by the general formula (1) below. ##STR00001## In the above general formula (1), each of X.sup.1, X.sup.2, X.sup.3 and X.sup.4 independently represents a hydrogen atom, an alkyl group having a carbon number of 1 to 6, a halogen atom, a hydroxyl group, a nitro group, a cyano group, or a methylsulfonyl group. In the present invention, it is preferred that each of X.sup.1, X.sup.2, X.sup.3 and X.sup.4 independently represents a hydrogen atom, an alkyl group having a carbon number of 1 to 6, or a halogen atom. In the present invention, it is also preferred that the nonlinear optical dye has a dipole moment of 2.1 D or less and a maximum absorption wavelength within a range of 315 to 360 nm.

Provided is a photopolymer composition that may exhibit low volume shrinkage during holographic recording and may prevent a photosensitive dye from remaining unbleached after holographic recording.

A multilayer optical information recording disk comprising a plurality of recording layers and intermediate layers provided between the plurality of recording layers, and a method for manufacturing the same are provided. At least one of two intermediate layers disposed adjacent to respective sides of one recording layer is made of adhesive. Each of the recording layers includes a polymer binder and a dye dispersed in the polymer binder or includes a polymer to which a dye is bonded. Each recording layer is configured such that the dye absorbs a recording beam and generates heat which deforms the recording layer, causing an interface between the recording layer and the intermediate layer made of adhesive to have a protrusive shape protruding into the intermediate layer, thereby recording information thereat. The interface between the recording layer and the recording layer made of adhesive has a groove for track-following servo control.