A method for making sulfur charged carbon nanotubes, the structure of the sulfur charged carbon nanotubes, and a cathode including the sulfur charged carbon nanotubes are described herein. The method comprises dissolving sublimed sulfur in a solvent to create a solution. The method further comprises adding carbon nanotubes to the solution. The method further comprises adding a polar protic solvent to the solution. The method further comprises removing the solvent from the solution.

A method of forming an electrode material includes: (1) loading an electrochemically active material onto graphene sheets; (2) combining the electrochemically active material-loaded graphene sheets with holey graphene oxide sheets to form a mixture; and (3) treating the mixture under reducing conditions to form a composite including a graphene framework loaded with the electrochemically active material.