One variation of a method includes: ingesting an air sample captured during an air capture period at a target location for collection of a first mixture including carbon dioxide and a first concentration of impurities; conveying the first mixture through a liquefaction unit to generate a second mixture including carbon dioxide and a second concentration of impurities less than the first concentration of impurities; in a methanation reactor, mixing the second mixture with hydrogen to generate a first hydrocarbon mixture comprising a third concentration of impurities comprising nitrogen, carbon dioxide, and hydrogen; conveying the first hydrocarbon mixture through a separation unit configured to remove impurities from the first hydrocarbon mixture to generate a second hydrocarbon a fourth concentration of impurities less than the third concentration of impurities; and depositing the second hydrocarbon mixture in a diamond reactor containing a set of diamond seeds to generate a first set of diamonds.

Disclosed are a high-entropy nitride ceramic fiber, and a preparation method and use thereof. The high-entropy ceramic fiber comprises Ti, Hf, Ta, Nb, and Mo; the high-entropy nitride ceramic fiber presents single crystal phase, and each of the elements are uniformly distributed at molecular level. The preparation method of the high-entropy ceramic fiber comprises: mixing a high-entropy ceramic precursor comprising the target metal elements, a spinning aid, and a solvent uniformly to prepare a precursor spinning solution, followed by working procedures of spinning, pyrolyzation, and nitriding to prepare the high-entropy nitride ceramic fiber. The high-entropy nitride ceramic fiber can be used in photocatalysis process of carbon dioxide to prepare methane.

Disclosed are a high-entropy nitride ceramic fiber, and a preparation method and use thereof. The high-entropy ceramic fiber comprises Ti, Hf, Ta, Nb, and Mo; the high-entropy nitride ceramic fiber presents single crystal phase, and each of the elements are uniformly distributed at molecular level. The preparation method of the high-entropy ceramic fiber comprises: mixing a high-entropy ceramic precursor comprising the target metal elements, a spinning aid, and a solvent uniformly to prepare a precursor spinning solution, followed by working procedures of spinning, pyrolyzation, and nitriding to prepare the high-entropy nitride ceramic fiber. The high-entropy nitride ceramic fiber can be used in photocatalysis process of carbon dioxide to prepare methane.

Disclosed are a high-entropy nitride ceramic fiber, and a preparation method and use thereof. The high-entropy ceramic fiber comprises Ti, Hf, Ta, Nb, and Mo; the high-entropy nitride ceramic fiber presents single crystal phase, and each of the elements are uniformly distributed at molecular level. The preparation method of the high-entropy ceramic fiber comprises: mixing a high-entropy ceramic precursor comprising the target metal elements, a spinning aid, and a solvent uniformly to prepare a precursor spinning solution, followed by working procedures of spinning, pyrolyzation, and nitriding to prepare the high-entropy nitride ceramic fiber. The high-entropy nitride ceramic fiber can be used in photocatalysis process of carbon dioxide to prepare methane.

One variation of a method includes: ingesting an air sample captured during an air capture period at a target location for collection of a first mixture including carbon dioxide and a first concentration of impurities; conveying the first mixture through a liquefaction unit to generate a second mixture including carbon dioxide and a second concentration of impurities less than the first concentration of impurities; in a methanation reactor, mixing the second mixture with hydrogen to generate a first hydrocarbon mixture comprising a third concentration of impurities comprising nitrogen, carbon dioxide, and hydrogen; conveying the first hydrocarbon mixture through a separation unit configured to remove impurities from the first hydrocarbon mixture to generate a second hydrocarbon a fourth concentration of impurities less than the third concentration of impurities; and depositing the second hydrocarbon mixture in a diamond reactor containing a set of diamond seeds to generate a first set of diamonds.

One variation of a method includes: ingesting an air sample captured during an air capture period at a target location for collection of a first mixture including carbon dioxide and a first concentration of impurities; conveying the first mixture through a liquefaction unit to generate a second mixture including carbon dioxide and a second concentration of impurities less than the first concentration of impurities; in a methanation reactor, mixing the second mixture with hydrogen to generate a first hydrocarbon mixture comprising a third concentration of impurities comprising nitrogen, carbon dioxide, and hydrogen; conveying the first hydrocarbon mixture through a separation unit configured to remove impurities from the first hydrocarbon mixture to generate a second hydrocarbon a fourth concentration of impurities less than the third concentration of impurities; and depositing the second hydrocarbon mixture in a diamond reactor containing a set of diamond seeds to generate a first set of diamonds.

The present invention relates to a dielectric barrier discharge (DBD) plasma reactor comprising a catalyst bed for CO.sub.X hydrogenation in a discharge region; and a method to produce light hydrocarbons from a CO.sub.X-containing gas mixture in the DBD plasma reactor. In the DBD plasma reactor for a CO.sub.X hydrogenation reaction, the catalyst for CO.sub.X hydrogenation comprises a catalytically active component on a mesoporous support that is a dielectric. When the DBD plasma reactor for a CO.sub.X hydrogenation reaction according to the present invention is used, it is possible to convert by-product gases or waste gases into higher-value-added chemical products without additional heat supply from the outside.

The present invention relates to a dielectric barrier discharge (DBD) plasma reactor comprising a catalyst bed for CO.sub.X hydrogenation in a discharge region; and a method to produce light hydrocarbons from a CO.sub.X-containing gas mixture in the DBD plasma reactor. In the DBD plasma reactor for a CO.sub.X hydrogenation reaction, the catalyst for CO.sub.X hydrogenation comprises a catalytically active component on a mesoporous support that is a dielectric. When the DBD plasma reactor for a CO.sub.X hydrogenation reaction according to the present invention is used, it is possible to convert by-product gases or waste gases into higher-value-added chemical products without additional heat supply from the outside.

The present invention relates to a dielectric barrier discharge (DBD) plasma reactor comprising a catalyst bed for CO.sub.X hydrogenation in a discharge region; and a method to produce light hydrocarbons from a CO.sub.X-containing gas mixture in the DBD plasma reactor. In the DBD plasma reactor for a CO.sub.X hydrogenation reaction, the catalyst for CO.sub.X hydrogenation comprises a catalytically active component on a mesoporous support that is a dielectric. When the DBD plasma reactor for a CO.sub.X hydrogenation reaction according to the present invention is used, it is possible to convert by-product gases or waste gases into higher-value-added chemical products without additional heat supply from the outside.

Methods and systems for making calcium oxide (CaO), carbon dioxide (CO.sub.2) and/or calcium hydroxide (Ca(OH).sub.2) from aragonite, for example, oolitic aragonite, are provided. The method can include applying solar energy, for example, by focusing one or more mirrors in one or more heliostats, to heat a reactant mixture in a vessel. The reactant mixture includes oolitic aragonite and can be heated to a temperature from 500° C. to 950° C. The system can include a vessel and a means for applying solar energy to heat a supply of oolitic aragonite disposed inside the vessel. Methods of converting the CO.sub.2 to ethanol, ethylene, graphene, and/or methane are also provided.