A curable composition includes an olefin-aromatic vinyl compound-aromatic polyene copolymer satisfying conditions (1) to (4) and an additive resin, which is at least one of a hydrocarbon-based elastomer, polyphenylene ether, olefin-aromatic vinyl compound-aromatic polyene copolymerized oligomer, and aromatic polyene-based resin. (1) The number average molecular weight of the copolymer is 5000 to 100000. (2) The aromatic vinyl compound monomer has 8 to 20 carbon atoms, and the content of the unit of the monomer is 0 to 70 mass %. (3) The aromatic polyene is selected from polyenes having 5 to 20 carbon atoms and a plurality of vinyl and/or vinylene groups in the molecule, and the content of the groups is 1.5 to 20 pieces per number average molecular weight. (4) The olefin is selected from olefins having 2 to 20 carbon atoms, and the total monomer units of the olefin, aromatic vinyl compound, and aromatic polyene is 100 mass %.

A curable composition includes an olefin-aromatic vinyl compound-aromatic polyene copolymer satisfying conditions (1) to (4) and an additive resin, which is at least one of a hydrocarbon-based elastomer, polyphenylene ether, olefin-aromatic vinyl compound-aromatic polyene copolymerized oligomer, and aromatic polyene-based resin. (1) The number average molecular weight of the copolymer is 5000 to 100000. (2) The aromatic vinyl compound monomer has 8 to 20 carbon atoms, and the content of the unit of the monomer is 0 to 70 mass %. (3) The aromatic polyene is selected from polyenes having 5 to 20 carbon atoms and a plurality of vinyl and/or vinylene groups in the molecule, and the content of the groups is 1.5 to 20 pieces per number average molecular weight. (4) The olefin is selected from olefins having 2 to 20 carbon atoms, and the total monomer units of the olefin, aromatic vinyl compound, and aromatic polyene is 100 mass %.

A borate compound-containing composition soluble in hydrocarbon solvents. A composition containing base A, or a compound having a total carbon number of not less than 8 and represented by the formula (5):

##STR00001##

wherein R and R′ are each independently an optionally substituted C.sub.1-30 alkyl group, an optionally substituted C.sub.3-15 cycloalkyl group, or an optionally substituted C.sub.6-14 aryl group; and
a borate compound represented by the following formula (1):

##STR00002##

wherein R.sup.1, R.sup.2, R.sup.3 and R.sup.4 are each independently a C.sub.6-14 aryl group substituted by one or more fluorine atoms or fluoro C.sub.1-4 alkyl groups; and
[A-H].sup.+ is a base A-derived cation. A method for producing a polymer, by polymerizing at least one kind of monomer selected from the group consisting of olefins and dienes by using the composition A as a cocatalyst.

A borate compound-containing composition soluble in hydrocarbon solvents. A composition containing base A, or a compound having a total carbon number of not less than 8 and represented by the formula (5):

##STR00001##

wherein R and R′ are each independently an optionally substituted C.sub.1-30 alkyl group, an optionally substituted C.sub.3-15 cycloalkyl group, or an optionally substituted C.sub.6-14 aryl group; and
a borate compound represented by the following formula (1):

##STR00002##

wherein R.sup.1, R.sup.2, R.sup.3 and R.sup.4 are each independently a C.sub.6-14 aryl group substituted by one or more fluorine atoms or fluoro C.sub.1-4 alkyl groups; and
[A-H].sup.+ is a base A-derived cation. A method for producing a polymer, by polymerizing at least one kind of monomer selected from the group consisting of olefins and dienes by using the composition A as a cocatalyst.

This invention relates to a biaxially-oriented polyethylene film comprising polyethylene having: (A) a melt index, I.sub.2, of 1.0 g/10 min or greater; (B) a density of 0.925 g/cm.sup.3 to 0.945 g/cm.sup.3; (C) a g′.sub.vis of less than 0.8; (D) an Mz of 1,000,000 g/mol or more; (E) an Mw/Mn of 5 or more; (F) an Mw of 100,000 g/mol or more; (G) a ratio of the g′.sub.LCB to the g′.sub.Zave is greater than 1.0; and (H) a Strain Hardening Ratio of 4 or more, where the film has a 1% secant in the transverse direction of 60,000 psi or more, a Dart Drop of 250 g/mil or more, and a ratio of 1% secant MD/1% secant TD is 0.65 or more.

This invention relates to a biaxially-oriented polyethylene film comprising polyethylene having: (A) a melt index, I.sub.2, of 1.0 g/10 min or greater; (B) a density of 0.925 g/cm.sup.3 to 0.945 g/cm.sup.3; (C) a g′.sub.vis of less than 0.8; (D) an Mz of 1,000,000 g/mol or more; (E) an Mw/Mn of 5 or more; (F) an Mw of 100,000 g/mol or more; (G) a ratio of the g′.sub.LCB to the g′.sub.Zave is greater than 1.0; and (H) a Strain Hardening Ratio of 4 or more, where the film has a 1% secant in the transverse direction of 60,000 psi or more, a Dart Drop of 250 g/mil or more, and a ratio of 1% secant MD/1% secant TD is 0.65 or more.

The present invention relates to a new multimodal ethylene copolymer (P), to the use of the copolymer in film applications and to a film comprising the copolymer of the invention.

The present invention relates to a new multimodal ethylene copolymer (P), to the use of the copolymer in film applications and to a film comprising the copolymer of the invention.

Catalyst system, the catalyst system comprising (i) at least one metallocene complex of formula (I) wherein Mt1 is Hf, X is a sigma-donor ligand, R.sup.1, R.sup.2, R.sup.3 are the same or different from each other and can be hydrogen or a saturated linear or branched C.sub.1-C.sub.10 alkyl, whereby the alkyl group can optionally contain up to 2 heteroatoms belonging to groups 14-16 of the periodic table, or R.sup.1 and R.sup.2 or R.sup.2 and R.sup.3 can form a ring having 4 to 6 C-atoms and 1 to 3 double bonds, R.sup.4 and R.sup.5 are the same or different from each other and can be saturated linear or branched C.sub.1-C.sub.10 alkyl, C.sub.5-C.sub.10 aryl, C.sub.6-C.sub.20 alkylaryl or C.sub.6-C.sub.20 arylalkyl groups, which can optionally contain up to 2 heteroatoms belonging to groups 14-16 of the periodic table, n can be 1 to 5, Ar is a C.sub.6-C.sub.20-aryl or -heteroaryl group, which can be unsubstituted or substituted by 1 to 5 linear or branched C.sub.1-C.sub.10 alkyl group(s), and (ii) an aluminoxane cocatalyst and (iii) optionally an aluminium alkyl compound AI(R.sup.7).sub.3, with R.sup.7 being a linear or branched C.sub.2-C.sub.8-alkyl group. ##STR00001##

Catalyst system, the catalyst system comprising (i) at least one metallocene complex of formula (I) wherein Mt1 is Hf, X is a sigma-donor ligand, R.sup.1, R.sup.2, R.sup.3 are the same or different from each other and can be hydrogen or a saturated linear or branched C.sub.1-C.sub.10 alkyl, whereby the alkyl group can optionally contain up to 2 heteroatoms belonging to groups 14-16 of the periodic table, or R.sup.1 and R.sup.2 or R.sup.2 and R.sup.3 can form a ring having 4 to 6 C-atoms and 1 to 3 double bonds, R.sup.4 and R.sup.5 are the same or different from each other and can be saturated linear or branched C.sub.1-C.sub.10 alkyl, C.sub.5-C.sub.10 aryl, C.sub.6-C.sub.20 alkylaryl or C.sub.6-C.sub.20 arylalkyl groups, which can optionally contain up to 2 heteroatoms belonging to groups 14-16 of the periodic table, n can be 1 to 5, Ar is a C.sub.6-C.sub.20-aryl or -heteroaryl group, which can be unsubstituted or substituted by 1 to 5 linear or branched C.sub.1-C.sub.10 alkyl group(s), and (ii) an aluminoxane cocatalyst and (iii) optionally an aluminium alkyl compound AI(R.sup.7).sub.3, with R.sup.7 being a linear or branched C.sub.2-C.sub.8-alkyl group. ##STR00001##