Various aspects relate to binder compositions including a bio-based component and pre-blends for forming the same. A binder composition includes an oligomerized biorenewable oil that is at least 10 wt % of the binder composition. The binder composition also includes an Asphaltene Additive comprising at least 20 wt % to 100 wt % asphaltenes, wherein the Asphaltene Additive is at least 8 wt % of the binder composition.

Devices and systems for collapsible engagement mechanisms are described herein. In some examples, one or more embodiments include a front panel, a first side panel connected to the front panel, a second side panel connected to the front panel, and a collapsible portion connected to at least one of the first side panel and the second side panel, where the collapsible portion is collapsible about a hinge.

Devices and systems for collapsible engagement mechanisms are described herein. In some examples, one or more embodiments include a front panel, a first side panel connected to the front panel, a second side panel connected to the front panel, and a collapsible portion connected to at least one of the first side panel and the second side panel, where the collapsible portion is collapsible about a hinge.

Methods of preparing graphene/graphene oxide particulates under mild conditions, comprising reacting pristine graphene with hydrogen peroxide and a source of iron to oxidize the outer surface of the pristine graphene particulates in solution and yield graphene/graphene oxide particulates. Methods and articles incorporating the same are also disclosed.

Methods of preparing engineered cementitious composite precursors include carbonating a fly ash comprising >about 25% by weight of calcium oxide (CaO) and having a water content of >about 12% to <about 18% by weight of water by exposing the fly ash to a first gas stream comprising carbon dioxide to form a carbonated fly ash. A steel slag is also carbonated that comprises>about 40% by weight of calcium oxide (CaO) and having a water content of >about 12% to <about 18% by weight of water by exposing the steel slag to a second gas stream comprising carbon dioxide to form a carbonated steel slag. The carbonated fly ash and the carbonated steel slag are suitable for use as engineered cementitious composite precursors in a bendable engineered cementitious composite composition that further comprises Portland cement, a polymeric fiber, and a superplasticizer.

Methods of preparing engineered cementitious composite precursors include carbonating a fly ash comprising >about 25% by weight of calcium oxide (CaO) and having a water content of >about 12% to <about 18% by weight of water by exposing the fly ash to a first gas stream comprising carbon dioxide to form a carbonated fly ash. A steel slag is also carbonated that comprises>about 40% by weight of calcium oxide (CaO) and having a water content of >about 12% to <about 18% by weight of water by exposing the steel slag to a second gas stream comprising carbon dioxide to form a carbonated steel slag. The carbonated fly ash and the carbonated steel slag are suitable for use as engineered cementitious composite precursors in a bendable engineered cementitious composite composition that further comprises Portland cement, a polymeric fiber, and a superplasticizer.

A method of reducing sulfur concentration in fly ash, flue gas desulfurization (FGD) ash, and mixtures thereof by contacting the fly ash, FGD ash, or mixtures thereof with an aqueous acidic solution, for a time, at a temperature, and at a liquid-to-solid ratio wherein the sulfur concentration within the fly ash, FGD ash, or mixture thereof is reduced to no more than 5 wt % SO.sub.3 based on the total weight of dry fly ash, FGD ash, or mixture thereof so treated.

A method of reducing sulfur concentration in fly ash, flue gas desulfurization (FGD) ash, and mixtures thereof by contacting the fly ash, FGD ash, or mixtures thereof with an aqueous acidic solution, for a time, at a temperature, and at a liquid-to-solid ratio wherein the sulfur concentration within the fly ash, FGD ash, or mixture thereof is reduced to no more than 5 wt % SO.sub.3 based on the total weight of dry fly ash, FGD ash, or mixture thereof so treated.

A method of forming a concrete product includes directly capturing CO.sub.2 from a gas source, the capturing comprising contacting the gas source with an absorption solution having a solvent and a solute, wherein the solvent and/or the solute are capable of reacting with CO.sub.2 to form an anionic compound, adjusting the pH of the absorption solution electrochemically to less than about 7 to release the CO.sub.2 as a concentrated vapor containing CO.sub.2, collecting the concentrated vapor containing CO.sub.2, regenerating the solvent and/or the solute, and optionally collecting the regenerated solvent and/or solute; flowing the concentrated vapor containing CO.sub.2 through a gas processing unit to adjust at least one of a temperature, a relative humidity, or a flow rate of the concentrated vapor containing CO.sub.2; and contacting the concentrated vapor containing CO.sub.2 with a concrete component.

A method of forming a concrete product includes directly capturing CO.sub.2 from a gas source, the capturing comprising contacting the gas source with an absorption solution having a solvent and a solute, wherein the solvent and/or the solute are capable of reacting with CO.sub.2 to form an anionic compound, adjusting the pH of the absorption solution electrochemically to less than about 7 to release the CO.sub.2 as a concentrated vapor containing CO.sub.2, collecting the concentrated vapor containing CO.sub.2, regenerating the solvent and/or the solute, and optionally collecting the regenerated solvent and/or solute; flowing the concentrated vapor containing CO.sub.2 through a gas processing unit to adjust at least one of a temperature, a relative humidity, or a flow rate of the concentrated vapor containing CO.sub.2; and contacting the concentrated vapor containing CO.sub.2 with a concrete component.