The present invention relates to a method of preparing an MFI zeolite with a microporous and mesoporous hierarchical structure in which a non-benzene-based first structure-directing agent, which provides ordered microporous pore sizes and a framework of MFI zeolite seed crystals, and a second structure-directing agent containing one benzene ring and an ammonium ion, which functions as a mesopore-directing agent without interfering with the function of the first structure-directing agent, are simultaneously used; an MFI zeolite with a microporous and mesoporous hierarchical structure, which is prepared by the method, and a catalyst use thereof for a reaction of converting acetylene into an aromatic compound; and a method of preparing an aromatic compound from acetylene using the catalyst.

The present invention relates to a method of preparing an MFI zeolite with a microporous and mesoporous hierarchical structure in which a non-benzene-based first structure-directing agent, which provides ordered microporous pore sizes and a framework of MFI zeolite seed crystals, and a second structure-directing agent containing one benzene ring and an ammonium ion, which functions as a mesopore-directing agent without interfering with the function of the first structure-directing agent, are simultaneously used; an MFI zeolite with a microporous and mesoporous hierarchical structure, which is prepared by the method, and a catalyst use thereof for a reaction of converting acetylene into an aromatic compound; and a method of preparing an aromatic compound from acetylene using the catalyst.

The present invention relates to a method of preparing an MFI zeolite with a microporous and mesoporous hierarchical structure in which a non-benzene-based first structure-directing agent, which provides ordered microporous pore sizes and a framework of MFI zeolite seed crystals, and a second structure-directing agent containing one benzene ring and an ammonium ion, which functions as a mesopore-directing agent without interfering with the function of the first structure-directing agent, are simultaneously used; an MFI zeolite with a microporous and mesoporous hierarchical structure, which is prepared by the method, and a catalyst use thereof for a reaction of converting acetylene into an aromatic compound; and a method of preparing an aromatic compound from acetylene using the catalyst.

The present invention relates to a method of preparing an aromatic compound from acetylene, which includes synthesizing an aromatic compound from an acetylene-containing reactant gas in the presence of a zeolite catalyst for the aromatization of acetylene, and subjecting the zeolite catalyst deactivated by the coke formed in the aromatization of acetylene, to plasma treatment at ambient temperature and pressure so as to selectively remove the external cokes and partial internal coke, thereby regenerating the zeolite catalyst; a method of regenerating the zeolite catalyst used in the aromatization of acetylene by plasma treatment; and a regenerated zeolite catalyst for the aromatization of acetylene, prepared thereof.

The present invention relates to a method of preparing an aromatic compound from acetylene, which includes synthesizing an aromatic compound from an acetylene-containing reactant gas in the presence of a zeolite catalyst for the aromatization of acetylene, and subjecting the zeolite catalyst deactivated by the coke formed in the aromatization of acetylene, to plasma treatment at ambient temperature and pressure so as to selectively remove the external cokes and partial internal coke, thereby regenerating the zeolite catalyst; a method of regenerating the zeolite catalyst used in the aromatization of acetylene by plasma treatment; and a regenerated zeolite catalyst for the aromatization of acetylene, prepared thereof.

The present invention relates to a method of preparing an aromatic compound from acetylene, which includes synthesizing an aromatic compound from an acetylene-containing reactant gas in the presence of a zeolite catalyst for the aromatization of acetylene, and subjecting the zeolite catalyst deactivated by the coke formed in the aromatization of acetylene, to plasma treatment at ambient temperature and pressure so as to selectively remove the external cokes and partial internal coke, thereby regenerating the zeolite catalyst; a method of regenerating the zeolite catalyst used in the aromatization of acetylene by plasma treatment; and a regenerated zeolite catalyst for the aromatization of acetylene, prepared thereof.

A process for the upgrading of hydrocarbon streams, i.e., processing any hydrocarbon feed streams rich in benzene and sulphur compounds. The process for simultaneous hydrodesulfurization and benzene conversion to higher alkylated aromatic molecules (C.sub.7 to C.sub.10 aromatics), without need of prior treatment like distillation, or sulfur removal. The hydrocarbon feed streams are processed over sulfided metal catalyst impregnated on acid support simultaneously desulfurizes and alkylates the benzene molecules.

A process for the upgrading of hydrocarbon streams, i.e., processing any hydrocarbon feed streams rich in benzene and sulphur compounds. The process for simultaneous hydrodesulfurization and benzene conversion to higher alkylated aromatic molecules (C.sub.7 to C.sub.10 aromatics), without need of prior treatment like distillation, or sulfur removal. The hydrocarbon feed streams are processed over sulfided metal catalyst impregnated on acid support simultaneously desulfurizes and alkylates the benzene molecules.