MULTI-MODE CAVITIES FOR HIGH-EFFICIENCY NONLINEAR WAVELENGTH CONVERSION FORMED WITH OVERLAP OPTIMIZATION
20170248831 · 2017-08-31
Assignee
- The Trustees Of Princeton University (Princeton, NJ)
- President And Fellows Of Harvard College (Cambridge, MA)
- Massachusetts Institute Of Technology (Cambridge, MA)
Inventors
- Alejandro Rodriguez (Princeton, NJ)
- Zin Lin (Somerville, MA)
- Steven G. Johnson (Arlington, MA)
- Marko Loncar (Belmont, MA)
- Xiangdong Liang (Arlington, MA)
Cpc classification
G02F1/3501
PHYSICS
G02F1/3548
PHYSICS
G02F1/3503
PHYSICS
G02F1/353
PHYSICS
International classification
Abstract
A dual frequency optical resonator configured for optical coupling to light having a first frequency ω1. The dual frequency optical resonator includes a plurality of alternating layer pairs stacked in a post configuration, each layer pair having a first layer formed of a first material and a second layer formed of a second material, the first material and second materials being different materials. The first layer has a first thickness and the second layer has a second thickness, the thicknesses of the first and second layer being selected to create optical resonances at the first frequency ω1 and a second frequency ω2 which is a harmonic of ω1 and the thicknesses of the first and second layer also being selected to enhance nonlinear coupling between the first frequency ω1 and a second frequency ω2.
Claims
1. A dual frequency optical resonator configured for optical coupling to light having a first frequency ω.sub.1, the dual frequency optical resonator comprising: a plurality of alternating layer pairs stacked in a post configuration, each layer pair having a first layer formed of a first material and a second layer formed of a second material, the first material and second materials being different materials, the first layer having a first thickness and the second layer having a second thickness, the thicknesses of the first and second layer being selected to create optical resonances at the first frequency ω.sub.1 and a second frequency ω.sub.2 which is a harmonic of ω.sub.1 and the thicknesses of the first and second layer also being selected to enhance nonlinear coupling between the first frequency ω.sub.1 and a second frequency ω.sub.2.
2. The dual frequency optical resonator of claim 1 wherein ω.sub.2 is a second harmonic of ω.sub.1.
3. The dual frequency optical resonator of claim 1 wherein ω.sub.2 is a third harmonic of ω.sub.1.
4. The dual frequency optical resonator of claim 1 wherein the thicknesses of the first and second layer are selected to maximize the nonlinear coupling between the first frequency ω.sub.1 and a second frequency ω.sub.2.
5. The dual frequency optical resonator of claim 1 wherein the first material is AlGaAs and the second material is Al.sub.2O.sub.3.
6. The dual frequency optical resonator of claim 1 wherein the first and second layer are formed in a deposition process.
7. A dual frequency optical resonator configured for optical coupling to light having a first frequency ω.sub.1, the dual frequency optical resonator comprising: a plurality of alternating layers pairs configured in a grating configuration, each layer pair having a first layer formed of a first material and a second layer formed of a second material, the first material and second materials being different materials, the first layer having a first thickness and the second layer having a second thickness, the thicknesses of the first and second layer being selected to create optical resonances at the first frequency ω.sub.1 and a second frequency ω.sub.2 which is a harmonic of ω.sub.1 and the thicknesses of the first and second layer also being selected to enhance nonlinear coupling between the first frequency ω.sub.1 and a second frequency ω.sub.2.
8. The dual frequency optical resonator of claim 7 wherein ω.sub.2 is a second harmonic of ω.sub.1.
9. The dual frequency optical resonator of claim 7 wherein ω.sub.2 is a third harmonic of ω.sub.1.
10. The dual frequency optical resonator of claim 7 wherein the thicknesses of the first and second layer are selected to maximize the nonlinear coupling between the first frequency ω.sub.1 and a second frequency ω.sub.2.
11. The dual frequency optical resonator of claim 7 wherein the first material is AlGaAs and the second material is Al.sub.2O.sub.3.
12. The dual frequency optical resonator of claim 7 wherein the first material is GaAs and the second material is SiO.sub.2.
13. The dual frequency optical resonator of claim 7 wherein the first material is LN and the second material is air.
14. The dual frequency optical resonator of claim 7 wherein the first and second layer are formed in an etching process.
15. A dual frequency optical resonator configured for optical coupling to light having a first frequency ω.sub.1, the dual frequency optical resonator comprising: a plurality of pixels configured in an X-Y plane, each pixel being formed of either a first material or a second material, the first material and second materials being different materials, the material for each pixel is selected such that the plurality of pixels create optical resonances at the first frequency ω.sub.1 and a second frequency ω.sub.2 which is a harmonic of ω.sub.1 and the material for each pixel is also selected such that the plurality of pixels enhance nonlinear coupling between the first frequency ω.sub.1 and a second frequency ω.sub.2.
16. The dual frequency optical resonator of claim 15 wherein ω.sub.2 is a second harmonic of ω.sub.1.
17. The dual frequency optical resonator of claim 15 wherein ω.sub.2 is a third harmonic of ω.sub.1.
18. The dual frequency optical resonator of claim 15 wherein the material for each pixel is selected such that the plurality of pixels maximize the nonlinear coupling between the first frequency ω.sub.1 and a second frequency ω.sub.2.
19. The dual frequency optical resonator of claim 15 wherein the first material is GaAs gratings and the second material is air.
20. The dual frequency optical resonator of claim 15 wherein the first material is LN and the second material is air.
Description
BRIEF DESCRIPTION OF THE FIGURES
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DETAILED DESCRIPTION
[0027] Nonlinear optical processes mediated by second-order (χ.sup.(2)) nonlinearities play a crucial role in many photonic applications, including ultra-short pulse shaping, spectroscopy, generation of novel frequencies and states of light and quantum information processing. Because nonlinearities are generally weak in bulk media, a well-known approach for lowering the power requirements of devices is to enhance nonlinear interactions by employing optical resonators that confine light for long times (dimensionless lifetimes Q) in small volumes V. Microcavity resonators designed for on-chip, infrared applications offer some of the smallest confinement factors available, but their implementation in practical devices has been largely hampered by the difficult task of identifying wavelength-scale (V˜λ.sup.3) structures supporting long-lived, resonant modes at widely separated wavelengths and satisfying rigid frequency-matching and mode-overlap constraints.
[0028] This disclosure is directed to scalable topology optimization of microcavities, where every pixel of the geometry is a degree of freedom and to the problem of designing wavelength-scale photonic structures for second harmonic generation (SHG). This approach is applied to obtain novel micropost, and grating microcavity designs supporting strongly coupled fundamental and harmonic modes at infrared and visible wavelengths with relatively large lifetimes Q.sub.1, Q.sub.2>10.sup.4. In contrast to recently proposed designs based on known, linear cavity structures hand-tailored to maximize the Purcell factors or mode volumes of individual resonances, e.g. ring resonators and nanobeam cavities, the disclosed designs ensure frequency matching and small confinement factors while also simultaneously maximizing the SHG enhancement factor Q.sup.2 Q.sub.2|
TABLE-US-00001 TABLE I SHG figures of merit for topology-optimized micropost and grating cavities of different material systems. Structure h.sub.x × h.sub.y × h.sub.z (λ.sub.1.sup.3) λ (μm) (Q.sub.1, Q.sub.2) (Q.sub.1.sup.rad, Q.sub.2.sup.rad)
[0029] Most experimental demonstrations of SHG in chip-based photonic systems operate in the so-called small-signal regime of weak nonlinearities, where the lack of pump depletion leads to the well-known quadratic scaling of harmonic output power with incident power. In situations involving all-resonant conversion, where confinement and long interaction times lead to strong nonlinearities and non-negligible down conversion, the maximum achievable conversion efficiency
[0030] occurs at a critical input power,
[0031] where X.sub.eff.sup.(2) is the effective nonlinear susceptibility of the medium [SM],
is the dimensionless quality factor (ignoring material absorption) incorporating radiative decay
and coupling to an input/output channel
The dimensionless coupling coefficient
[0032] Where
[0033] where FOM.sub.1 represents the efficiency per power, often quoted in the so-called undepleted regime of low-power conversion, and FOM.sub.2 represents limits to power enhancement. Note that for a given radiative loss rate, FOM.sub.1 is maximized when the modes are critically coupled,
with the absolute maximum occurring in the absence of radiative losses, Q.sup.rad.fwdarw.∞, or equivalently, when FOM.sub.2 is maximized. From either FOM, it is clear that apart from frequency matching and lifetime engineering, the design of optimal SHG cavities rests on achieving a large nonlinear coupling
[0034] Optimal Designs.—
[0035] Table I characterizes the FOMs of some of our newly discovered microcavity designs, involving simple micropost and gratings structures of various χ.sup.(2) materials, including GaAs, AlGaAs and LiNbO.sub.3. The low-index material layers of the microposts consist of alumina (Al.sub.2O.sub.3), while gratings are embedded in either silica or air (see supplement for detailed specifications). Note that in addition to their performance characteristics, these structures are also significantly different from those obtained by conventional methods in that traditional designs often involve rings, periodic structures or tapered defects, which tend to ignore or sacrifice
[0036]
[0037] It should be understood that other structures having a single dimension of freedom or multiple dimensions of freedom may be used without departing from the scope of this disclosure. For example,
[0038] To understand the mechanism of improvement in
[0039] Based on the tabulated FOMs (Table I), the efficiencies and power requirements of realistic devices can be directly calculated. For example, assuming x.sub.eff.sup.2 (AlGaAs)˜100 pm/V, the AlGaAs/Al.sub.2O.sub.3 micropost cavity (
in the undepleted regime when the modes are critically coupled,
For larger operational bandwidths, e.g. Q.sub.1=5000 and Q.sub.2=1000, we find that
When the system is in the depleted regime and critically coupled, we find that a maximum efficiency of 25% can be achieved at P.sub.1.sup.crit≈0.15 mW whereas assuming smaller Q.sub.1=5000 and Q.sub.2=1000, a maximum efficiency of 96% can be achieved at P.sub.1.sup.crit≈0.96 W.
[0040] Comparison against previous designs.—Table II summarizes various performance characteristics, including the aforementioned FOM, for a handful of previously studied geometries with length-scales spanning from mm to a few wavelengths (microns).
[0041] Comparing Tables I and II, one observes that for a comparable Q, the topology-optimized structures perform significantly better in both FOM.sub.1 and FOM2 than any conventional geometry, with the exception of the LN gratings, whose low Q.sup.rad lead to slightly lower FOM2. Generally, the optimized microposts and gratings perform better by virtue of a large and robust
[0042] Optimization Formulation:
[0043] Optimization techniques have been regularly employed by the photonic device community, primarily for fine-tuning the characteristics of a pre-determined geometry; the majority of these techniques involve probabilistic Monte-Carlo algorithms such as particle swarms, simulated annealing and genetic algorithms. While some of these gradient-free methods have been used to uncover a few unexpected results out of a limited number of degrees of freedom (DOF), gradient-based topology optimization methods efficiently handle a far larger design space, typically considering every pixel or voxel as a DOF in an extensive 2D or 3D computational domain, giving rise to novel topologies and geometries that might have been difficult to conceive from conventional intuition alone. The early applications of topology optimization were primarily focused on mechanical problems and only recently have they been expanded to consider photonic systems, though largely limited to linear device designs.
TABLE-US-00002 TABLE II Structure λ (μm) (Q.sub.1, Q.sub.2) (Q.sub.1.sup.rad, Q.sub.2.sup.rad)
[0044] Table II includes SHG figures of merit, including the frequencies λ, overall and radiative quality factors Q, Q.sup.rad and nonlinear coupling
[0045] A high level example of a suitable computation system generally proceeds as follows:
[0046] 1(a) define a grid of degrees of freedom (DOF). 1(b) assign permittivity (material property) to each DOF. 2(a) place a dipole current source J.sub.1 at ω.sub.1 in the domain and compute a relative electric field E.sub.1 by solving Maxwell's equations. 2(b) compute the derivative of E.sub.1 with respect to each DOF. 3(a) using E.sub.1 at ω1, compute the work done by the electric field on the current source (P=E.sub.1.Math.J.sub.1). 3b) compute the field E.sub.2 due to current source J2 at ω.sub.2 (e.g., 2 ω.sub.1 for the 2.sup.nd harmonic) by solving Maxwell's equations. 3(c) compute the work done by the electric field on the current source (P=E.sub.2.Math.J.sub.2). 4 maximize 3(c) and 3(a). In this example
[0047] In what follows, we describe a system for gradient-based topology optimization of nonlinear wavelength-scale frequency converters. Previous approaches exploited the equivalency between LDOS and the power radiated by a point dipole in order to reduce Purcell-factor maximization problems to a series of small scattering calculations. Defining the objective max.sub.(iΔx, jΔy, kΔz)}. An important realization is that instead of maximizing the LDOS at a single discrete frequency ω, a better-posed problem is that of maximizing the frequency-averaged ƒ in the vicinity of ω, denoted by (ƒ)=∫dω′W(ω′;ω,Γ)ƒ(ω′), where W is a weight function defined over some specified bandwidth Γ. Using contour integration techniques, the frequency integral can be conveniently replaced by a single evaluation of ƒ at a complex frequency ω+iΓ. For a fixed Γ, the frequency average effectively shifts the algorithm in favor of minimizing V over maximizing Q; the latter can be enhanced over the course of the optimization by gradually winding down the averaging bandwidth Γ. A major merit of the frequency-averaged LDOS formulation is that it features a mathematically well-posed objective as opposed to a direct maximization of the cavity Purcell factor Q, allowing for rapid convergence of the optimization algorithm into an extremal solution.
[0048] An extension of the optimization problem from single to multimode cavities maximizes the minimum of a collection of LDOS at different frequencies. Applying such an approach to the problem of SHG, the optimization objective becomes: max.sub.
[0049] where
[0050] and where ∈.sub.d denotes the dielectric contrast of the nonlinear medium and ∈.sub.m is that of the surrounding linear medium. Note that
[0051]
[0052] For computational convenience, the optimization is carried out using a 2D computational cell (in the xz-plane), though the resulting optimized structures are given a finite transverse extension h.sub.y (along the y direction) to make realistic 3D devices (see e.g.,
creating a kind of metamaterial in the optimization direction; these arise during the optimization process regardless of starting conditions due to the low-dimensionality of the problem. We find that these features are not easily removable as their absence greatly perturbs the quality factors and frequency matching.
[0053] The computational framework discussed above is based on largescale topology-optimization (TO) techniques that enable automatic discovery of multilayer and grating structures exhibiting some of the largest SHG figures of merit ever predicted. It is also possible to extend the TO formulation to allow the possibility of more sophisticated nonlinear processes and apply it to the problem of designing rotationally symmetric and slab microresonators that exhibit high-efficiency second harmonic generation (SHG) and sum/difference frequency generation (SFG/DFG). In particular, disclosed herein are multi-track ring resonators and proof-of-principle two-dimensional slab cavities supporting multiple, resonant modes (even several octaves apart) that would be impossible to design “by hand”. The disclosed designs ensure frequency matching, long radiative lifetimes, and small (wavelength-scale) modal confinement while also simultaneously maximizing the nonlinear modal overlap (or “phase matching”) necessary for efficient NFC. For instance, disclosed herein are topology-optimized concentric ring cavities exhibiting SHG efficiencies as high as P.sub.2/P.sub.1.sup.2=1.3×10.sup.25 (x.sup.(2)).sup.2[W.sup.−1] even with low operational Q˜10.sup.4, a performance that is on a par with recently fabricated 60 μm-diameter, ultrahigh Q˜10.sup.6 AIN microring resonators (P.sub.2/P.sub.1.sup.2=1.13×10.sup.24 (x.sup.(2)).sup.2[W.sup.−1]); essentially, our topology-optimized cavities not only possess the smallest possible modal volumes ˜(λ/n).sup.3, but can also operate over wider bandwidths by virtue of their increased nonlinear modal overlap.
[0054] A typical topology optimization problem seeks to maximize or minimize an objective function ƒ, subject to certain constraints g, over a set of free variables or degrees of freedom (DOF):
max/min ƒ(
g(
0≦
[0055] where the DOFs are the normalized dielectric constants.
[0056]
[0057] describing the steady-state E(r; ω) in response to incident currents J(r, θ) at frequency ω. While solution of (4) is straightforward and commonplace, an important aspect to making optimization problems tractable is to obtain a fast-converging and computationally efficient adjoint formulation of the problem. Within the scope of TO, this requires efficient calculations of the derivatives
[0058] at every pixel α, which we perform by exploiting the adjoint-variable method (AVM).
[0059] Any NFC process can be viewed as a frequency mixing scheme in which two or more constituent photons at a set of frequencies {ω.sub.n} interact to produce an output photon at frequency Ω=Σ.sub.nc.sub.nw.sub.n, where {c.sub.n} can be either negative or positive, depending on whether the corresponding photons are created or destroyed in the process. Given an appropriate nonlinear tensor component X.sub.ijk . . . , with i, j, k, . . . ∈{x, y, z}, mediating an interaction between the polarization components E.sub.i(Ω) and E.sub.1j, E.sub.2k, . . . , we begin with a collection of point dipole currents, each at the constituent frequency ω.sub.n, n∈{1, 2, . . . } and positioned at the center of the computational cell r′, such that J.sub.n=ê.sub.nvδ (r−r′), where ê.sub.nv ∈{ê.sub.1j, ê.sub.2k, . . . } is a polarization vector chosen so as to excite the desired electric field polarization components (v) of the corresponding mode. Given the choice of incident currents Jn, we solve Maxwell's equations to obtain the corresponding constituent electric-field response E.sub.n, from which one can construct a nonlinear polarization current J(Ω)=
[0060] Writing down the objective function in terms of the nonlinear polarization currents, it follows that solution of (5), obtained by employing any mathematical programming technique that makes use of gradient information, e.g. the adjoint variable method maximizes the nonlinear coefficient (mode overlap) associated with the aforementioned nonlinear optical process.
[0061] Multi-track ring resonators—NLTO formulations may be applied to the design of rotationally symmetric cavities for SHG. A material platform may include gallium arsenide (GaAs) thin films cladded in silica.
TABLE-US-00003 TABLE III (m.sub.1, m.sub.2) Polari- zation Q.sub.1 Q.sub.2
[0062] Table III shows the SHG figures of merit, including azithmuthal numbers m.sub.1,2, field polarizations, lifetimes Q.sub.1,2, and nonlinear coupling
TABLE-US-00004 TABLE IV ω.sub.1:ω.sub.2:ω.sub.3 (m.sub.1, m.sub.2, m.sub.3) Polarization (Q.sub.1, Q.sub.2, Q.sub.3)
[0063] Table IV shows Similar figures of merit as in Table III, but for multi-track rings designed to enhance a SFG process involving light at ω.sub.1=ω.sub.3−ω.sub.2, ω.sub.2=1.2ω.sub.1, and ω.sub.3=2.2ω.sub.1, with
[0064]
[0065] In Table. IV, we also consider resonators optimized to enhance a SFG process involving three resonant modes, ω.sub.1=ω.sub.3−ω.sub.2, with ω.sub.2=1.2ω.sub.1 and ω.sub.3=2.2ω.sub.1. Note that two of these modes are more than an octave apart.
[0066] The resulting structures and figures of merit suggest the possibility of orders of magnitude improvements. In particular, we find that the largest overlap factors
[0067] Slab Microcavities—
[0068] We now consider a different class of structure and NFC process, namely DFG in slab microcavities. In particular, we consider a χ.sup.(3) nonlinear process satisfying the frequency relation ω.sub.s=ω.sub.0−2ω.sub.b, with ω.sub.s, ω.sub.0, and ω.sub.b denoting the frequencies of signal, emitted, and pump photons (see
[0069]
[0070] Note that the lifetimes of these 2D modes are bounded only by the finite size of our computational cell (and hence are ignored in our discussion), whereas in realistic 3D microcavities, they will be limited by vertical radiation losses. Despite the two-dimensional aspect of this slab design, and in contrast to the fully 3D multitrack ring resonators above, these results provide proof of the existence of wavelength-scale photonic structures that can greatly enhance challenging NFC processes. One example is the NV problem described above, which is particularly challenging if a monolithic all-diamond approach is desired, in which case both single-photon emission and wavelength conversion are to be seamlessly realized in the same diamond cavity. A viable solution that was recently proposed is the use of four-wave mixing Bragg scattering (FWM-BS) by way of whispering gallery modes, which are relatively easy to phase-match but suffer from large mode volumes. Furthermore, FWM-BS requires two pump lasers, at least one of which has a shorter wavelength than the converted signal photon, which could lead to spontaneous down-conversion and undesirable noise, degrading quantum fidelity, in contrast to the DFG scheme above, based on a long-wavelength pump.
[0071]
[0072] Further disclosure is contained in U.S. provisional application 62/300,516, filed Feb. 26, 2016, which is incorporated herein in its entirety. All references that are cited in U.S. provisional application 62/300,516 and the appendix are also incorporated herein in their entirety. Further disclosure is also provided in Lin et al. “Topology optimization of multi-track ring resonators and 2D microcavities for nonlinear frequency conversion”, Physics—Optics, January 2017 which is also incorporated herein in its entirety. It should be understood that many variations are possible based on the disclosure herein. Although features and elements are described above in particular combinations, each feature or element can be used alone without the other features and elements or in various combinations with or without other features and elements. The digital processing techniques disclosed herein may be partially implemented in a computer program, software, or firmware incorporated in a computer-readable (non-transitory) storage medium for execution by a general-purpose computer or a processor. Examples of computer-readable storage mediums include a read only memory (ROM), a random access memory (RAM), a register, cache memory, semiconductor memory devices, magnetic media such as internal hard disks and removable disks, magneto-optical media, and optical media such as CD-ROM disks, and digital versatile disks (DVDs).
[0073] Suitable processors include, by way of example, a general-purpose processor, a special purpose processor, a conventional processor, a digital signal processor (DSP), a plurality of microprocessors, one or more microprocessors in association with a DSP core, a controller, a microcontroller, Application-Specific Integrated Circuits (ASICs), Field-Programmable Gate Arrays (FPGAs) circuits, any other type of integrated circuit (IC), and/or a state machine.