1-(PYRIDYL)-5-AZINYLPYRAZOLE DERIVATIVES, AND THEIR USE FOR CONTROL OF UNDESIRED PLANT GROWTH
20240041042 · 2024-02-08
Inventors
- Estella BUSCATO (Sant Cugat del Valles, ES)
- Michael Gerhard HOFFMANN (Konstanz, DE)
- Harald Jakobi (Frankfurt, DE)
- Thomas MÜLLER (Frankfurt, DE)
- Birgit BOLLENBACH-WAHL (Weiler/Bingen, DE)
- Jan Dittgen (Frankfurt, DE)
- Elmar Gatzweiler (Bad Nauheim, DE)
- Anna Maria REINGRUBER (Heppenheim, DE)
Cpc classification
A01N43/66
HUMAN NECESSITIES
International classification
A01N43/66
HUMAN NECESSITIES
Abstract
The present invention relates to novel herbicidally active substituted 1-pyridyl-5-azinylpyrazolyl-3-oxyalkyl acids, 1-pyridyl-5-azinylpyrazolyl-3-sulfanylalkyl acids, 1-pyridyl-5-azinylpyrazolyl-3-sulfinylalkyl acids and 1-pyridyl-5-azinylpyrazolyl-3-sulfonylalkyl acids, and to the derivatives thereof according to the general formula (I) or agrochemically acceptable salts thereof. The present invention further relates to processes for preparing these compounds and to the use thereof for controlling broad-leaved weeds and weed grasses.
Claims
1. Compounds of general formula (I) and agrochemically compatible salts, N-oxides, hydrates, and hydrates of the salts and N-oxides thereof, ##STR00091## where A is selected from the group consisting of A1-A15: ##STR00092## ##STR00093## Q is selected from the group consisting of Q1-Q3: ##STR00094## R.sup.1 is OR.sup.1a, NR.sup.9R.sup.10 or O(CH.sub.2).sub.xO(CH.sub.2).sub.yO(CH.sub.2).sub.z H; R.sup.1a is hydrogen or is (C.sub.1-C.sub.6)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, each of which is unsubstituted or substituted by one or more substituents selected from the group consisting of halogen, (C.sub.1-C.sub.6)-alkyl, (C.sub.1-C.sub.6)-haloalkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.1-C.sub.6)-alkoxy, (C.sub.1-C.sub.2)-haloalkoxy, (C.sub.1-C.sub.6)-alkoxycarbonyl, cyano and nitro or is (C.sub.2-C.sub.4)-alkenyl, CH.sub.2C(COOMe)=CH.sub.2, (C.sub.2-C.sub.4)-alkynyl or is (C.sub.1-C.sub.6)-alkyl-S(C.sub.1-C.sub.6)-alkyl-, (C.sub.1-C.sub.6)-alkyl-SO(C.sub.1-C.sub.6)-alkyl-, (C.sub.1-C.sub.6)-alkyl-SO.sub.2(C.sub.1-C.sub.6)-alkyl- or is N(C.sub.3-C.sub.6)-cycloalkyl, NC(CH.sub.3).sub.2 or is heterocyclyl, heteroaryl, aryl or is heterocyclyl-(C.sub.1-C.sub.4)-alkyl-, heteroaryl-(C.sub.1-C.sub.4)-alkyl-, aryl-(C.sub.1-C.sub.4)-alkyl-, each of which is unsubstituted or substituted by one or more substituents selected from the group consisting of halogen, (C.sub.1-C.sub.6)-alkyl, (C.sub.1-C.sub.6)-haloalkyl; R.sup.9 is hydrogen, (C.sub.1-C.sub.12)-alkyl; R.sup.10 is hydrogen, aryl, heteroaryl, heterocyclyl, (C.sub.1-C.sub.12)-alkyl, (C.sub.3-C.sub.8)-cycloalkyl, (C.sub.3-C.sub.8)-cycloalkyl-(C.sub.1-C.sub.7)-alkyl-, (C.sub.2-C.sub.12)-alkenyl, (C.sub.5-C.sub.7)-cycloalkenyl, (C.sub.2-C.sub.12)-alkynyl, S(O).sub.nR.sup.5, cyano, nitro, OR.sup.5, SO.sub.2NR.sup.6R.sup.7, CO.sub.2R.sup.8, COR.sup.8, NR.sup.6R.sup.8, NR.sup.6COR.sup.8, NR.sup.6CO.sub.2R.sup.8, NR.sup.6SO.sub.2R.sup.8, where the abovementioned alkyl, cycloalkyl, alkenyl, cycloalkenyl and alkynyl radicals are unsubstituted or each independently substituted by m radicals selected from the group consisting of hydrogen, optionally mono- or polysubstituted aryl, halogen, cyano, nitro, OR.sup.5, S(O).sub.nR.sup.5, SO.sub.2NR.sup.6R.sup.7, CO.sub.2R.sup.8, CONR.sup.6R.sup.8, COR.sup.6, NR.sup.6R.sup.8, NR.sup.6COR.sup.8, NR.sup.6CONR.sup.8R.sup.8, NR.sup.6CO.sub.2R.sup.8, NR.sup.6SO.sub.2R.sup.8, NR.sup.6SO.sub.2NR.sup.6R.sup.8, C(R.sup.6)NOR.sup.8; or R.sup.9 and R.sup.10 together with the nitrogen atom to which they are bonded form a saturated or partly or fully unsaturated five-, six- or seven-membered ring which is optionally mono- to hexasubstituted by the following radicals from the group consisting of halogen, (C.sub.1-C.sub.6)-alkyl, (C.sub.1-C.sub.6)-haloalkyl, OR.sup.5, S(O).sub.nRS, CO.sub.2R.sup.8, CONR.sup.6R.sup.8, COR.sup.6 and C(R.sup.6)NOR.sup.8 and which, in addition to this nitrogen atom, contains r carbon atoms, o oxygen atoms, p sulfur atoms and q elements from the group consisting of NR.sup.7, CO and NCOR.sup.7 as ring atoms; R.sup.5 is (C.sub.1-C.sub.6)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.1-C.sub.6)-haloalkyl, aryl; R.sup.6 is hydrogen, (C.sub.1-C.sub.6)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.1-C.sub.6)-haloalkyl, aryl; R.sup.7 is hydrogen, (C.sub.1-C.sub.6)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.3-C.sub.4)-alkenyl, (C.sub.3-C.sub.4)-alkynyl, CH.sub.2C(O)O(C.sub.1-C.sub.2)-alkyl; R.sup.8 is hydrogen, (C.sub.1-C.sub.6)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.3-C.sub.4)-alkenyl, (C.sub.1-C.sub.6)-alkyl-C(O)O(C.sub.1-C.sub.2)-alkyl or (C.sub.3-C.sub.4)-alkynyl; R.sup.2 is hydrogen, cyano, (C.sub.1-C.sub.6)-alkyl, (C.sub.1-C.sub.6)-alkoxy-(C.sub.1-C.sub.6)-alkyl-, (C.sub.1-C.sub.6)-haloalkyl, (C.sub.1-C.sub.6)-alkoxy, (C.sub.2-C.sub.6)-alkenyl, (C.sub.2-C.sub.6)-haloalkenyl, (C.sub.2-C.sub.6)-alkynyl, (C.sub.2-C.sub.6)-haloalkynyl, (C.sub.3-C.sub.6)-cycloalkyl; R.sup.3 is halogen, cyano, isocyano, NO.sub.2, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.1-C.sub.6)-alkyl, (C.sub.3-C.sub.6)-halocycloalkyl, (C.sub.1-C.sub.6)-haloalkyl, (C.sub.1-C.sub.6)-alkylcarbonyl-, (C.sub.1-C.sub.6)-haloalkylcarbonyl-, (C.sub.1-C.sub.6)-alkyloxycarbonyl-, (C.sub.2-C.sub.3)-alkenyl, (C.sub.2-C.sub.3)-haloalkenyl, (C.sub.2-C.sub.3)-alkynyl, (C.sub.2-C.sub.3)-haloalkynyl, (C.sub.1-C.sub.6)-alkyl-S(O).sub.n and (C.sub.1-C.sub.6)-haloalkyl-S(O).sub.n, CHO, NH.sub.2; R.sup.12 is halogen, cyano, isocyano, NO.sub.2, (C.sub.1-C.sub.6)-alkyl, (C.sub.1-C.sub.6)-haloalkyl, (C.sub.1-C.sub.6)-alkylcarbonyl, (C.sub.1-C.sub.6)-haloalkylcarbonyl, (C.sub.1-C.sub.6)-alkyloxycarbonyl, (C.sub.1-C.sub.6)-alkoxy, (C.sub.1-C.sub.6)-haloalkoxy, (C.sub.1-C.sub.6)-alkyl-, S(O).sub.n, (C.sub.2-C.sub.3)-alkenyl, (C.sub.2-C.sub.3)-haloalkenyl, (C.sub.2-C.sub.3)-alkynyl, (C.sub.2-C.sub.3)-haloalkynyl, NH.sub.2; R.sup.13 is halogen, cyano, isocyano, NO.sub.2, (C.sub.1-C.sub.6)-alkyl, (C.sub.1-C.sub.6)-haloalkyl, (C.sub.1-C.sub.6)-alkylcarbonyl, (C.sub.1-C.sub.6)-haloalkylcarbonyl, (C.sub.1-C.sub.6)-alkyloxycarbonyl, (C.sub.1-C.sub.6)-alkoxy, (C.sub.1-C.sub.6)-haloalkoxy, (C.sub.1-C.sub.6)-alkyl-S(O).sub.n, (C.sub.2-C.sub.3)-alkenyl, (C.sub.2-C.sub.3)-haloalkenyl; (C.sub.2-C.sub.3)-alkynyl, (C.sub.2-C.sub.3)-haloalkynyl, NH.sub.2; Y is oxygen, S(O).sub.n; m is 0, 1 or 2; n is 0, 1 or 2; o is 0, 1 or 2; p is 0 or 1; q is 0 or 1; r is 3, 4, 5 or 6; s is 0, 1, 2, 3 or 4; x is 2, 3; y is 2, 3; z is 1, 2.
2. The compounds of the formula (I) according to claim 1 and their agrochemically compatible salts, N-oxides, hydrates, and hydrates of the salts and N-oxides, where A is selected from the group consisting of A1-A4, A6, A8, A9, A12, A15 ##STR00095## Q is selected from the group consisting of Q1-Q3: ##STR00096## R.sup.1 is OR.sup.1a, NR.sup.9R.sup.10 or O(CH.sub.2).sub.xO(CH.sub.2).sub.yO(CH.sub.2).sub.zH; R.sup.1a is hydrogen or is (C.sub.1-C.sub.3)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, each of which is unsubstituted or substituted by one or more substituents selected from the group consisting of halogen, (C.sub.1-C.sub.4)-alkyl, (C.sub.1-C.sub.4)-haloalkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.1-C.sub.4)-alkoxy, (C.sub.1-C.sub.4)-alkoxycarbonyl, cyano, or is (C.sub.2-C.sub.4)-alkenyl, (C.sub.2-C.sub.4)-alkynyl, or is (C.sub.2-C.sub.3)-alkyl-SMe-, (C.sub.2-C.sub.3)-alkyl-SOMe-, (C.sub.2-C.sub.3)-alkyl-SO.sub.2Me-, or is NC(CH.sub.3).sub.2 or is heterocyclyl, or is heterocyclyl-(C.sub.1-C.sub.2)-alkyl-, heteroaryl-(C.sub.1-C.sub.2)-alkyl-, aryl-(C.sub.1-C.sub.2)-alkyl-, each of which is unsubstituted or substituted by one or more substituents selected from the group consisting of halogen, (C.sub.1-C.sub.2)-alkyl, (C.sub.1-C.sub.2)-haloalkyl; R.sup.9 is hydrogen, (C.sub.1-C.sub.4)-alkyl; R.sup.10 is (C.sub.1-C.sub.4)-alkyl, (C.sub.2-C.sub.4)-alkenyl, (C.sub.2-C.sub.4)-alkynyl, S(O).sub.nR.sup.5, SO.sub.2NR.sup.6R.sup.7, where the abovementioned alkyl, alkenyl and alkynyl radicals are unsubstituted or each independently substituted by m radicals selected from the group consisting of halogen, cyano, S(O).sub.nRS, SO.sub.2NR.sup.6R.sup.7, CO.sub.2R.sup.8, CONR.sup.6R.sup.8, or R.sup.9 and R.sup.10 together with the nitrogen atom to which they are bonded form a saturated or partly or fully unsaturated five-, six- or seven-membered ring which is optionally mono- or disubstituted by the following radicals from the group consisting of (C.sub.1-C.sub.4)-alkyl, (C.sub.1-C.sub.4)-haloalkyl, CO.sub.2R.sup.8 and CONR.sup.6R.sup.8; R.sup.5 is (C.sub.1-C.sub.4)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.1-C.sub.4)-haloalkyl, phenyl; R.sup.6 is hydrogen, (C.sub.1-C.sub.4)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.1-C.sub.4)-haloalkyl, phenyl; R.sup.7 is hydrogen, (C.sub.1-C.sub.4)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.3-C.sub.4)-alkenyl, (C.sub.3-C.sub.4)-alkynyl; R.sup.8 is hydrogen, (C.sub.1-C.sub.4)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.3-C.sub.4)-alkenyl, (C.sub.1-C.sub.4)-alkyl-C(O)O(C.sub.1-C.sub.2)-alkyl or (C.sub.3-C.sub.4)-alkynyl; R.sup.2 is hydrogen, (C.sub.1-C.sub.3)-alkyl, (C.sub.1-C.sub.3)-alkoxy, (C.sub.2-C.sub.3)-alkenyl, (C.sub.2-C.sub.3)-alkynyl, (C.sub.3-C.sub.6)-cycloalkyl; R.sup.3 is halogen, cyano, isocyano, NO.sub.2, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.1-C.sub.4)-alkyl, (C.sub.3-C.sub.6)-halocycloalkyl, (C.sub.1-C.sub.4)-haloalkyl, (C.sub.1-C.sub.4)-alkylcarbonyl-, (C.sub.1-C.sub.4)-haloalkylcarbonyl-, (C.sub.1-C.sub.4)-alkyloxycarbonyl-, (C.sub.2-C.sub.3)-alkenyl, (C.sub.2-C.sub.3)-haloalkenyl, (C.sub.2-C.sub.3)-alkynyl, (C.sub.2-C.sub.3)-haloalkynyl, CHO; R.sup.12 is halogen, cyano, NO.sub.2, (C.sub.1-C.sub.4)-alkyl, (C.sub.1-C.sub.4)-haloalkyl, (C.sub.1-C.sub.4)-alkylcarbonyl, (C.sub.1-C.sub.4)-haloalkylcarbonyl, (C.sub.1-C.sub.4)-alkyloxycarbonyl, (C.sub.1-C.sub.4)-alkoxy, (C.sub.1-C.sub.4)-haloalkoxy, (C.sub.2-C.sub.3)-alkenyl, (C.sub.2-C.sub.3)-haloalkenyl, (C.sub.2-C.sub.3)-alkynyl, (C.sub.2-C.sub.3)-haloalkynyl, NH.sub.2; R.sup.13 is halogen, cyano, NO.sub.2, (C.sub.1-C.sub.4)-alkyl, (C.sub.1-C.sub.4)-haloalkyl, (C.sub.1-C.sub.4)-alkylcarbonyl, (C.sub.1-C.sub.4)-haloalkylcarbonyl, (C.sub.1-C.sub.4)-alkyloxycarbonyl, (C.sub.1-C.sub.4)-alkoxy, (C.sub.1-C.sub.4)-haloalkoxy, (C.sub.2-C.sub.3)-alkenyl, (C.sub.2-C.sub.3)-haloalkenyl; (C.sub.2-C.sub.3)-alkynyl, (C.sub.2-C.sub.3)-haloalkynyl, NH.sub.2; Y is oxygen, S(O).sub.n; m is 0 or 1; n is 0, 1 or 2; s is 0, 1, 2 or 3; x is 2; y is 2; z is 1.
3. The compounds of the formula (I) according to claim 1 and their agrochemically compatible salts, N-oxides, hydrates, and hydrates of the salts and N-oxides, where A is selected from the group consisting of A2, A3, A6 and A8 ##STR00097## Q is selected from the group consisting of Q1-Q3: ##STR00098## R.sup.1 is OR.sup.1a, NR.sup.9R.sup.10 or O(CH.sub.2).sub.2O(CH.sub.2).sub.2OCH.sub.3; R.sup.1a is hydrogen or is (C.sub.1-C.sub.3)-alkyl which is unsubstituted or substituted by a substituent selected from the group consisting of C(O)OMe, cyclopropyl, cyclopentyl, methoxy, cyano, trifluoromethyl or is (C.sub.3-C.sub.6)-cycloalkyl or is NC(CH.sub.3).sub.2 or is prop-2-ynyl or is oxetan-3-yl-(C.sub.1-C.sub.2)-alkyl-, tetrahydrofuran-2-yl-(C.sub.1-C.sub.2)-alkyl-, tetrahydrofuran-3-yl-(C.sub.1-C.sub.2)-alkyl-, pyridin-2-yl-(C.sub.1-C.sub.2)-alkyl-, pyridin-3-yl-(C.sub.1-C.sub.2)-alkyl-, pyridin-4-yl-(C.sub.1-C.sub.2)-alkyl-, phenyl-(C.sub.1-C.sub.2)-alkyl-; R.sup.9 is hydrogen; R.sup.10 is (C.sub.1-C.sub.4)-alkyl where the alkyl radical is unsubstituted or monosubstituted by CO.sub.2R.sup.8, S(O).sub.2R.sup.5 or SO.sub.2NR.sup.6R.sup.7; or R.sup.9 and R.sup.10 together with the nitrogen atom to which they are bonded form a saturated five- or seven-membered ring monosubstituted by CO.sub.2R.sup.8; R.sup.5 is methyl, ethyl or CH.sub.2CF.sub.3; R.sup.6 is hydrogen or methyl; R.sup.7 is methyl or ethyl; R.sup.8 is hydrogen, methyl or ethyl; R.sup.2 is hydrogen, methyl or ethyl; R.sup.3 is halogen, cyano, NO.sub.2, (C.sub.3-C.sub.5)-cycloalkyl, (C.sub.3-C.sub.5)-halocycloalkyl, (C.sub.1-C.sub.2)-alkyl, (C.sub.1-C.sub.2)-haloalkyl; R.sup.12 is fluorine or chlorine; R.sup.13 is fluorine, chlorine, methyl, ethyl, methoxy, trifluoromethyl; Y is oxygen; s is 0, 1, 2.
4. The compounds of the formula (I) according to claim 1 and their agrochemically compatible salts, N-oxides, hydrates, and hydrates of the salts and N-oxides, where A is selected from the group consisting of A2, A3 and A6 ##STR00099## Q is selected from the group consisting of Q1-Q3: ##STR00100## R.sup.1 is OR.sup.1a or NR.sup.9R.sup.10, R.sup.1a is hydrogen or methyl, ethyl, each of which is unsubstituted or substituted by a substituent selected from the group consisting of C(O)OMe, cyclopropyl, cyclopentyl, methoxy, cyano, trifluoromethyl or is NC(CH.sub.3).sub.2 or is prop-2-ynyl or CH.sub.2-tetrahydrofuran-2-yl, CH.sub.2-tetrahydrofuran-3-yl, CH.sub.2-oxetan-3-yl, CH.sub.2-pyridyl-2-yl, CH.sub.2-pyridin-3-yl, CH.sub.2-pyridin-4-yl, CH.sub.2-phenyl, R.sup.9 is hydrogen; R.sup.10 methyl or ethyl, where the radicals are monosubstituted by CO.sub.2R.sup.8, or R.sup.9 and R.sup.10 together with the nitrogen atom to which they are bonded form a cyclopentyl or cyclohexyl radical monosubstituted by CO.sub.2R.sup.8; R.sup.8 is methyl or ethyl; R.sup.2 is hydrogen or methyl; R.sup.3 is halogen, cyano, NO.sub.2, cyclopropyl, cyclobutyl, 2,2-difluorocyclopropyl, trifluoromethyl; R.sup.12 is fluorine; R.sup.13 is fluorine, chlorine, methyl, trifluoromethyl; Y is oxygen; s is 0, 1, 2.
5. The compounds of the formula (I) according to claim 1 and their agrochemically compatible salts, N-oxides, hydrates, and hydrates of the salts and N-oxides, where A is selected from the group consisting of A2, A3 and A6 ##STR00101## Q is selected from the group consisting of Q1-Q3: ##STR00102## R.sup.1 is OR.sup.1a; R.sup.1a is hydrogen, methyl, ethyl; R.sup.2 is hydrogen or methyl; R.sup.3 is fluorine, chlorine, bromine, cyano, NO.sub.2, cyclopropyl, trifluoromethyl; R.sup.12 is fluorine; R.sup.13 is fluorine, chlorine, trifluoromethyl; Y is oxygen; s is 0, 1, 2.
6. Compounds of formula (Z) with Q=Q1, R.sup.1=OR.sup.1a and YO and their agrochemically compatible salts, N-oxides, hydrates, and hydrates of the salts and N-oxides, where ##STR00103## substituents are as set forth in claim 1.
7. Compounds of formula (Y) with Q=Q1, YO and A=A2 and their agrochemically compatible salts, N-oxides, hydrates, and hydrates of the salts and N-oxides, where ##STR00104## substituents are as set forth in claim 1.
8. A process for preparing compounds of formula (Ic) or an agrochemically acceptable salt thereof according to claim 1 by converting compounds of general formulae (III) and (IV) ##STR00105## in which R.sup.2, R.sup.1a, R.sup.3, A, Q and Y are as set forth in claim 1 and X is chlorine, bromine or iodine, in the presence of a sulfurizing reagent.
9. A process for preparing compounds of formula (Ia) or an agrochemically acceptable salt thereof according to claim 1 by converting, via an ester cleavage reaction, a compound of general formula (Ic) ##STR00106## in which R.sup.2, R.sup.1a, R.sup.3, A, Q and Y are as set forth in claim 1, in the presence of a base or a Lewis acid.
10. A process for preparing compounds of formula (Ib) or an agrochemically acceptable salt thereof according to claim 1 by converting compounds of general formulae (Ia) and (II) ##STR00107## in which R.sup.9, R.sup.10, R.sup.2, R.sup.1a, R.sup.3, A, Q and Y are as set forth in claim 1, in the presence of an amide coupling reagent.
11. An agrochemical composition comprising at least one compound of the formula (I) or an agrochemically acceptable salt thereof as set forth in claim 1.
12. An agrochemical composition comprising: a) at least one compound of the formula (I) or an agrochemically acceptable salt thereof as set forth in claim 1; and b) one or more active agrochemical ingredients other than component a).
13. A method of controlling unwanted plants or for regulating the growth of plants, wherein at least one compound of the formula (I) or an agrochemically acceptable salt thereof, as set forth in claim 1, is applied to the plants, a seed or an area in which the plants grow.
14. A method of inhibiting plant growth, the method comprising use of compounds of the formula (I) or an agrochemically acceptable salt thereof, as set forth in claim 1, as herbicides or plant growth regulators.
15. The method according to claim 14, wherein the compounds of the formula (I) or an agrochemically acceptable salt thereof are used for controlling harmful plants or for regulating growth in crop plants.
16. The method according to claim 15, wherein the crop plants are transgenic or nontransgenic crop plants.
17. The compounds according to claim 1, comprising 1-Pyridyl-5-azinylpyrazolyl-3-oxyalkyl acids, 1-pyridyl-5-azinylpyrazolyl-3-sulfanylalkyl acids, 1-pyridyl-5-azinylpyrazolyl-3-sulfinylalkyl acids, 1-pyridyl-5-azinylpyrazolyl-3-sulfonylalkyl acids, or combinations thereof.
18. The process according to claim 8, wherein the sulfurizing reagent is one of phosphorus pentasulfide and Lawesson's reagent.
Description
EXAMPLES
[0493] The present invention is illustrated in detail by the examples which follow, but these examples do not restrict the invention in any way.
A. Synthesis Examples
Methyl (2R)-2-{[4-bromo-1-(3-fluoropyridin-2-yl)-5-(6-fluoropyridin-3-yl)-1H-pyrazol-3-yl]oxy}propanoate (I-05)
N-(3-Fluoropyridin-2-yl)-3-(6-methylpyridin-3-yl)prop-2-yne hydrazide
[0494] To a solution of 1.27 g (6.92 mmol) of 3-(6-fluoropyridin-3-yl)prop-2-ynoic acid, 1.32 g (10.38 mmol) of 2-fluoro-6-hydrazinopyridine and 3.5 g (34.61 mmol) of triethylamine in 72 ml of THF is added dropwise 6.6 g (10.38 mmol) of a 50% propanephosphonic anhydride solution in THF, and this mixture is stirred at room temperature for one hour. For workup, H.sub.2O is added, the organic phase is removed, and the aqueous phase is extracted repeatedly with CH.sub.2Cl.sub.2. The combined organic phase is dried over Na.sub.2SO.sub.4 and concentrated. 2.25 g (95%) of crude product is obtained, which is used without further purification for the next reaction stage.
1-(3-Fluoropyridin-2-yl)-5-(6-fluoropyridin-3-yl)-1H-pyrazol-3-ol
[0495] To a solution of 2.23 g (6.50 mmol) of N-(3-fluoropyridin-2-yl)-3-(6-methylpyridin-3-yl)prop-2-yne hydrazide in 10 ml of CH.sub.2Cl.sub.2 and 3 ml of DMF is added 99 mg (0.52 mmol) of CuI, and the mixture is stirred at 80 C. for one hour. This is followed by removal by filtration and concentration, and purification of the crude product by column chromatography using silica gel with heptane/ethyl acetate (3:7). In this way, 0.95 g (53%) of product is obtained in solid form.
[0496] .sup.1H-NMR (400 MHz, DMSO-d.sub.6): 6.25 (bs, 1H), 7.15 (d, 1H), 7.50 (bs, 1H), 7.78 (m, 1H), 7.95 (m, 1H), 8.10 (s, 1H), 8.20 (bs, 1H).
Methyl (2R)-2-{[1-(3-fluoropyridin-2-yl)-5-(6-fluoropyridin-3-yl)-1H-pyrazol-3-yl]oxy}propanoate
[0497] To a solution of 0.34 g (1.25 mmol) of 1-(3-fluoropyridin-2-yl)-5-(6-fluoropyridin-3-yl)-1H-pyrazol-3-ol in 10 ml of DMF are successively added 0.61 g (1.87 mmol) of Cs.sub.2CO.sub.3 and 0.18 g (1.50 mmol) of methyl (2S)-2-chloropropanoate, and then the mixture is stirred at 80 C. for 1 hour. Thereafter, the reaction mixture is concentrated to dryness, taken up in H.sub.2O and extracted repeatedly with CH.sub.2Cl.sub.2. The organic phase is dried over Na.sub.2SO.sub.4 and then concentrated. Purification by column chromatography on silica gel using heptane/ethyl acetate (8.2) gives 0.4 g (87%) of product as a colourless oil.
[0498] .sup.1H-NMR (400 MHz, CDCl.sub.3): 1.65 (d, 3H), 3.79 (s, 3H), 5.25 (q, 1H), 6.14 (s, 1H), 6.89 (m, 1H), 7.35 (m, 1H), 7.50 (m, 1H), 7.68 (m, 1H), 8.10 (s, 1H), 8.25 (d, 1H).
Methyl (2R)-2-{[4-bromo-1-(3-fluoropyridin-2-yl)-5-(6-fluoropyridin-3-yl)-1H-pyrazol-3-yl]oxy}propanoate
[0499] To a solution of 0.38 g (1.05 mmol) of methyl (2R)-2-{[1-(3-fluoropyridin-2-yl)-5-(6-fluoropyridin-3-yl)-1H-pyrazol-3-yl]oxy}propanoate in 4 ml of DMF is added 0.22 g (1.26 mmol) of N-bromosuccinimide, and the mixture is stirred at 65 C. for 1 hour. The reaction mixture is then added to H.sub.2O and extracted repeatedly with CH.sub.2Cl.sub.2. The organic phase is dried over Na.sub.2SO.sub.4 and concentrated, and the crude product thus obtained is purified by column chromatography using silica gel with heptane/ethyl acetate (8:2). In this way, 0.45 g (95%) of product is obtained in solid form.
[0500] .sup.1H-NMR (400 MHz, CDCl.sub.3): 1.70 (d, 3H), 3.78 (s, 3H), 5.70 (q, 1H), 6.95 (m, 1H), 7.30 (m, 1H), 7.50 (m, 1H), 7.84 (m, 1H), 8.12 S, 1H), 8.20 (d, 1H).
Methyl (2R)-2-{[4-cyano-1-(3-fluoropyridin-2-yl)-5-(6-fluoropyridin-3-yl)-1H-pyrazol-3-yl]oxy}propanoate (I-06)
[0501] Under argon, a baked-out MW vial is charged with a mixture of 0.17 g (0.40 mmol) of methyl (2R)-2-{[4-bromo-1-(3-fluoropyridin-2-yl)-5-(6-fluoropyridin-3-yl)-1H-pyrazol-3-yl]oxy}propanoate, 0.045 g (0.38 mmol) of Zn(CN).sub.2 and 0.046 g (0.040 mmol) of tetrakis(triphenylphosphine)palladium, and 5 ml of N,N-dimethylacetamide is added. The vessel is degassed and blanketed with argon, and the reaction mixture is stirred in a microwave at 180 C. for 40 minutes. The reaction mixture is then concentrated, taken up in H.sub.2O and extracted repeatedly with CH.sub.2Cl.sub.2. The organic phase is dried over Na.sub.2SO.sub.4 and concentrated, and the crude product thus obtained is purified by column chromatography using silica gel with heptane/ethyl acetate (8:2). In this way, 0.082 g (52%) of product is obtained in solid form.
[0502] .sup.1H-NMR (400 MHz, CDCl.sub.3): 1.70 (d, 3H), 3.79 (s, 3H), 5.77 (q, 1H), 7.00 (m, 1H), 7.45 (m, 1H), 7.68 (m, 1H), 7.92 (m, 1H), 8.12 (s, 1H), 8.29 (d, 1H).
Methyl (2R)-2-{[4-chloro-5-(2-fluoropyridin-4-yl)-1-(pyridin-2-yl)-1H-pyrazol-3-yl]oxy}propanoate (..) and (2R)-2-{[4-chloro-5-(2-fluoropyridin-4-yl)-1-(pyridin-2-yl)-1H-pyrazol-3-yl]oxy}propanoic acid (..)
5-amino-4-chloro-1-(pyridin-2-yl)-1H-pyrazol-3-ol
[0503] To a solution of 2 g (11.35 mmol) of 5-amino-1-(pyridin-2-yl)-1H-pyrazol-3-ol in 80 ml of DMF is added, in portions, 1.10 g (12.48 mmol) of N-chlorosuccinimide. The reaction mixture is stirred at 50 C. for 5 hours and then left to stand at room temperature for 12 hours. After addition of 80 ml of H.sub.2O and 60 ml of CH.sub.2Cl.sub.2, the product precipitates out in solid form. Filtration and drying under reduced pressure gives 1.43 g (60%) of product in solid form.
[0504] .sup.1H-NMR (400 MHz, DMSO-d.sub.6): 7.10 (bs, 2H, NH2), 7.20 (dd, 1H), 7.55 (d, 1H), 7.90 (dd, 1H), 8.46 (d, 1H).
Methyl (2R)-2-{[5-amino-4-chloro-1-(pyridin-2-yl)-1H-pyrazol-3-yl]oxy}propanoate
[0505] To a solution of 1.4 g (6.64 mmol) of 5-amino-4-chloro-1-(pyridin-2-yl)-1H-pyrazol-3-ol is added 3.25 g (9.98 mmol) of Cs.sub.2CO.sub.3, and this mixture is stirred at room temperature for 10 minutes. After addition of 1.20 g (7.97 mmol) of methyl (2S)-2-chloropropanoate, the reaction mixture is stirred at room temperature for 12 hours. After filtration, the reaction solution is added to H.sub.2O and extracted repeatedly with CH.sub.2Cl.sub.2. The organic phase is dried over Na.sub.2SO.sub.4 and concentrated. 1.56 g (75%) of product is obtained in solid form.
[0506] .sup.1H-NMR (400 MHz, CDCl.sub.3): 1.65 (d, 3H), 3.75 (s, 3H), 5.18 (q, 1H), 6.00 (bs, 2H, NH2), 7.04 (dd, 1H), 7.63 (d, 1H), 7.72 (dd, 1H), 8.26 (d, 2H).
Methyl (2R)-2-{[4-chloro-5-iodo-1-(pyridin-2-yl)-1H-pyrazol-3-yl]oxy}propanoate
[0507] To a solution of 0.30 g (1.01 mmol) of methyl (2R)-2-{[5-amino-4-chloro-1-(pyridin-2-yl)-1H-pyrazol-3-yl]oxy}propanoate in 6 ml of acetonitrile are successively added 1.08 g (4.04 mmol) of diiodomethane and 0.23 g (2.02 mmol) of isopentyl nitrite, and the mixture is then stirred at 50 C. for 1 hour. Thereafter, the reaction mixture is added to H.sub.2O and extracted repeatedly with CH.sub.2Cl.sub.2. The organic phase is dried over Na.sub.2SO.sub.4 and concentrated, and the crude product is purified by column chromatography on silica gel using heptane/ethyl acetate (1:1). In this way, 0.24 g (55%) of product is obtained as an oil.
[0508] .sup.1H-NMR (400 MHz, CDCl.sub.3): 1.68 (d, 3H), 3.75 (s, 3H), 5.20 (q, 1H), 7.21 (dd, 1H), 7.60 (d, 1H), 7.70 (dd, 1H), 8.45 (d, 1H).
(2R)-2-{[4-Chloro-5-(2-fluoropyridin-4-yl)-1-(pyridin-2-yl)-1H-pyrazol-3-yl]oxy}propanoic acid (I-21)
[0509] Under argon, a mixture of 0.18 g (0.45 mmol) of methyl (2R)-2-{[4-chloro-5-iodo-1-(pyridin-2-yl)-1H-pyrazol-3-yl]oxy}propanoate, 0.16 g (1.13 mmol) of (2-fluoropyridin-4-yl)boronic acid, 0.055 g (0.067 mmol) of PdCl.sub.2dppf, DCM complex, and 0.44 g (1.35 mmol) of Cs.sub.2CO.sub.3 in 3 ml of 1,4-dioxane and 0.9 ml of H.sub.2O is stirred in a microwave at 130 C. for 3.5 hours. Thereafter, the reaction mixture is added to a saturated aqueous NH.sub.4Cl solution and extracted repeatedly with CH.sub.2Cl.sub.2. The organic phase is dried over Na.sub.2SO.sub.4 and concentrated, and the crude product thus obtained is purified by column chromatography using silica gel with heptane/ethyl acetate (1:1). In this way, 38 mg (21%) of the methyl ester was obtained. Concentrating the water phase and subsequent purification by column chromatography using silica gel with heptane/ethyl acetate (3:7) gives 67 mg (33%) of the carboxylic acid.
[0510] .sup.1H-NMR (400 MHz, DMSO-d.sub.6): 1.55 (d, 3H), 5.10 (q, 1H), 7.26 (m, 2H) 7.65 (d, 1H), 7.96 (m, 2H), 8.10 (d, 1H), 8.20 (s, 1H).
Ethyl {[4-bromo-5-(2-fluoropyridin-4-yl)-1-(pyridin-2-yl)-1H-pyrazol-3-yl]oxy}acetate (I-01)
2-[3-(Benzyloxy)-1H-pyrazol-1-yl]pyridine
[0511] A mixture consisting of 5 g (28.70 mmol) of 3-(benzyloxy)-1H-pyrazole, 6.80 g (43.05 mmol) of 2-bromopyridine, 0.77 g (4.02 mmol) of CuI and 13.09 g (40.18 mmol) of Cs.sub.2CO.sub.3 in 40 ml of DMF is stirred under argon at 100 C. for 5 hours. Thereafter, the reaction mixture is filtered through kieselguhr, added to H.sub.2O and extracted repeatedly with CH.sub.2Cl.sub.2. The organic phase is dried over Na.sub.2SO.sub.4 and concentrated, and the crude product is purified by column chromatography on silica gel using heptane/ethyl acetate (1:1). In this way, 6.65 g (92%) of product is obtained in solid form.
[0512] .sup.1H-NMR (400 MHz, CDCl.sub.3): 5.31 (s, 2H), 5.95 (s, 1H), 7.10 (dd, 1H), 7.35 (m, 3H), 7.50 (m, 2H), 7.75 (m, 1H), 7.80 (d, 1H), 8.35 (d, 1H), 8.40 (s, 1H).
2-[3-(Benzyloxy)-5-iodo-1H-pyrazol-1-yl]pyridine
[0513] To a solution of 31.80 mmol of LDA in 140 ml of THF is added dropwise, at 78 C. under argon, a solution of 4.70 g (18.70 mmol) of 2-[3-(benzyloxy)-1H-pyrazol-1-yl]pyridine in 130 ml THF, and this mixture is stirred at 78 C. for a further 1.5 hours. A solution of 7.6 g (30.00 mmol) of iodine in 130 ml THF is then added dropwise to the reaction mixture, and the reaction mixture is stirred for a further 2 hours at 78 C., before being allowed to come to room temperature. The reaction mixture is then added to H.sub.2O and extracted repeatedly with CH.sub.2Cl.sub.2. The organic phase is dried over Na.sub.2SO.sub.4 and concentrated, and the crude product is purified by column chromatography on silica gel using heptane/ethyl acetate (8:2). In this way, 3.83 g (54%) of product is obtained as an oil.
[0514] .sup.1H-NMR (400 MHz, CDCl.sub.3): 5.29 (s, 2H), 6.20 (s, 1H), 7.25 (m, 1H), 7.24 (m, 1H), 7.38 (m, 2H), 7.45 (m, 1H), 7.73 (d, 1H), 8.50 (s, 1H).
4-[3-(Benzyloxy)-1-(pyridin-2-yl)-1H-pyrazol-5-yl]-2-fluoropyridine
[0515] To a solution of 0.50 g (1.32 mmol) of 2-[3-(benzyloxy)-5-iodo-1H-pyrazol-1-yl]pyridine in 8 ml of 1,4-dioxane are added successively under argon 0.65 g (2.91 mmol) of 2-fluoro-4-(4,4,5,5-tetramethyl-1,3,2-dioxaborolan-2-yl)pyridine, 0.86 g (2.65 mmol) of Cs.sub.2CO.sub.3, 13 mg (0.066 mmol) of CuI, 1 ml of H.sub.2O and 77 mg (0.066 mmol) of tetrakis(triphenylphosphine)palladium(0), and this mixture is stirred at 70 C. for 3.5 hours and then left to stand overnight. After filtration, the reaction solution is concentrated and the crude mixture is purified by column chromatography using silica gel with heptane/ethyl acetate (7:3). In this way, 0.32 g (69%) of product is obtained in solid form.
[0516] 1-H-NMR (400 MHz, CDCl3) 5.35 (s, 1H), 6.10 (s, 1H), 6.85 (s, 1H), 7.08 (d, 1H), 7.20 (m, 1H), 7.40 (m, 3H) 7.50 (m, 2H), 7.70 (d, 1H), 7.82, (m, 1H), 8.20 (m, 2H), 8.40 (d, 1H).
5-(2-Fluoropyridin-4-yl)-1-(pyridin-2-yl)-1H-pyrazol-3-ol
[0517] To a solution of 0.44 g (0.63 mmol) of 5-(2-fluoropyridin-4-yl)-1-(pyridin-2-yl)-1H-pyrazol-3-ol in 18 ml of toluene is added 37 g (324.5 mmol) of trifluoroacetic acid (dried over molecular sieve), and then the mixture is stirred at 50 C. for 3.5 hours and left to stand at room temperature overnight. Thereafter, another 3 ml of trifluoroacetic acid is added and the mixture is stirred at 50 C. for a further 3.5 hours. After filtration, the reaction solution is concentrated and the crude product is purified by column chromatography using silica gel with heptane/ethyl acetate (1:1). The mixture thus obtained contains 50% product and is used in the next reaction step without further purification.
Ethyl {[5-(2-fluoropyridin-4-yl)-1-(pyridin-2-yl)-1H-pyrazol-3-yl]oxy}acetate
[0518] To a solution of 0.07 g (0.273 mmol) of 5-(2-fluoropyridin-4-yl)-1-(pyridin-2-yl)-1H-pyrazol-3-ol in 5.5 ml of acetonitrile is added 0.23 g (1.64 mmol) of K.sub.2CO.sub.3, and the mixture is stirred at room temperature for 10 minutes. After addition of 0.091 g (0.55 mmol) of ethyl bromoacetate, the reaction mixture is stirred under reflux for 5 hours and then left to stand at room temperature overnight. For workup, the mixture is concentrated to dryness, and the residue is taken up in H.sub.2O and extracted repeatedly with CH.sub.2Cl.sub.2. The organic phase is dried over Na.sub.2SO.sub.4 and concentrated, and the crude product is purified by column chromatography on silica gel using heptane/ethyl acetate (7:3). 0.036 g (38%) of product is obtained in solid form.
[0519] .sup.1H-NMR (400 MHz, CDCl.sub.3): 1.32 (t, 3h), 4.30 (q, 2H), 4.90 (s, 2H), 6.15 (s, 1H), 6.85 (s, 1H), 7.08 (s, 1H), 7.08 (m, 1H), 7.15 (dd, 1H), 7.65 (d, 1H), 7.80 dd, 1H), 8.15 (m, 2H).
Ethyl {[4-bromo-5-(2-fluoropyridin-4-yl)-1-(pyridin-2-yl)-1H-pyrazol-3-yl]oxy}acetate
[0520] To a solution of 0.036 g (0.105 mmol) of ethyl {[5-(2-fluoropyridin-4-yl)-1-(pyridin-2-yl)-1H-pyrazol-3-yl]oxy}acetate in 0.6 ml of CH.sub.2Cl.sub.2 is added 0.021 g (0.116 mmol) of N-bromosuccinimide, and the mixture is stirred at room temperature for 12 hours. This is followed by concentration to dryness, extraction of the residue by stirring with diethyl ether, and removal by filtration. The ether phase is concentrated, and the crude product thus obtained is purified using silica gel with heptane/ethyl acetate (1.1). In this way, 0.021 g (47%) of product is obtained in solid form.
[0521] .sup.1H-NMR (400 MHz, CDCl.sub.3): 1.30 (t, 3H), 4.70 (q, 2H), 4.95 (s, 2H), 6.93 (6.93 (s, 1H), 7.12 (m, 2H), 7.62 (d, 1H), 7.69 (m, 1H), 8.08 (m, 1H), 8.25 (s, 1H).
[0522] NMR Data of Selected Examples:
[0523] The .sup.1H NMR data of selected examples of compounds of the general formula (I) are stated in two different ways, namely (a) conventional NMR evaluation and interpretation or (b) in the form of .sup.1H NMR peak lists according to the method described below.
[0524] a) Conventional NMR Interpretation
Example I-144
[0525] .sup.1H-NMR (400 MHz, CDCl.sub.3, , ppm): 8.40 (m, 1H), 8.30 (m, 1H), 8.16-8.15 (m, 1H), 7.48-7.39 (m, 2H), 7.26-7.23 (m, 1H), 5.25 (q, 1H), 3.75 (s, 3H), 1.63-1.57 (m, 4H), 0.84-0.77 (m, 4H).
Example I-166
[0526] .sup.1H-NMR (400 MHz, CDCl.sub.3, , ppm): 8.43 (m, 1H), 8.32 (s, 1H), 8.20-8.19 (m, 1H), 7.47-7.41 (m, 2H), 7.28-7.24 (m, 1H), 5.29 (q, 1H), 1.67 (d, 3H), 1.62-1.55 (m, 1H), 0.81-0.75 (m, 4H).
Example I-172
[0527] .sup.1H-NMR (400 MHz, CDCl.sub.3, , ppm): 8.39 (m, 1H), 8.31 (s, 1H), 8.16-8.15 (m, 1H), 7.48-7.39 (m, 2H), 7.26-7.22 (m, 1H), 5.24 (q, 1H), 4.21 (q, 2H), 1.62 (d, 3H), 1.61-1.57 (m, 1H), 1.25 (t, 3H), 0.86-0.76 (m, 4H).
[0528] b) NMR Peak List Method
[0529] The 1H NMR data of selected examples are noted in the form of 1H NMR peak lists. For each signal peak, first the value in ppm and then the signal intensity in round brackets are listed. The valuesignal intensity number pairs for different signal peaks are listed with separation from one another by semicolons.
[0530] The peak list for one example therefore takes the form of: [0531] .sub.1 (intensity.sub.1); .sub.2 (intensity.sub.2); . . . ; .sub.i (intensity.sub.i); . . . ; .sub.n (intensity.sub.n)
[0532] The intensity of sharp signals correlates with the height of the signals in a printed example of an NMR spectrum in cm and shows the true ratios of the signal intensities. In the case of broad signals, several peaks or the middle of the signal and the relative intensity thereof may be shown in comparison to the most intense signal in the spectrum.
[0533] For calibration of the chemical shift of 1H NMR spectra we use tetramethylsilane and/or the chemical shift of the solvent, particularly in the case of spectra measured in DMSO. Therefore, the tetramethylsilane peak may but need not occur in NMR peak lists.
[0534] The lists of the 1H NMR peaks are similar to the conventional 1H NMR printouts and thus usually contain all peaks listed in a conventional NMR interpretation.
[0535] In addition, like conventional 1H NMR printouts, they may show solvent signals, signals of stereoisomers of the target compounds, which likewise form part of the subject matter of the invention, and/or peaks of impurities.
[0536] In the reporting of compound signals in the delta range of solvents and/or water, our lists of 1H NMR peaks show the usual solvent peaks, for example peaks of DMSO in DMSO-D.sub.6 and the peak of water, which usually have a high intensity on average.
[0537] The peaks of stereoisomers of the target compounds and/or peaks of impurities usually have a lower intensity on average than the peaks of the target compounds (for example with a purity of >90%).
[0538] Such stereoisomers and/or impurities may be typical of the particular preparation process. Their peaks can thus help in identifying reproduction of our preparation process with reference to by-product fingerprints.
[0539] An expert calculating the peaks of the target compounds by known methods (MestreC, ACD simulation, but also with empirically evaluated expected values) can, if required, isolate the peaks of the target compounds, optionally using additional intensity filters. This isolation would be similar to the relevant peak picking in conventional 1H NMR interpretation.
[0540] Further details of 1H NMR peak lists can be found in the Research Disclosure Database Number 564025.
TABLE-US-00004 I-01: .sup.1H-NMR(599.6 MHz, CDCl3): = 8.5362 (1.8); 8.5343 (1.9); 8.5284 (1.9); 8.5262 (1.8); 8.4282 (0.4); 8.2542 (11.2); 8.2456 (11.3); 8.0981 (6.6); 8.0963 (6.6); 8.0901 (6.7); 8.0883 (6.4); 7.8572 (1.2); 7.8543 (1.2); 7.8442 (2.0); 7.8416 (2.0); 7.8312 (1.4); 7.8281 (1.3); 7.7984 (3.7); 7.7954 (3.6); 7.7846 (6.5); 7.7828 (6.3); 7.7723 (4.6); 7.7693 (4.2); 7.7612 (0.3); 7.6572 (0.3); 7.6435 (0.4); 7.6225 (10.6); 7.6088 (9.0); 7.3077 (1.6); 7.2995 (1.7); 7.2954 (1.7); 7.2872 (1.6); 7.2656 (10.5); 7.1614 (5.6); 7.1532 (6.0); 7.1522 (5.9); 7.1475 (8.9); 7.1446 (8.8); 7.1416 (8.7); 7.1394 (7.9); 7.1360 (7.9); 6.9597 (13.5); 5.0092 (0.4); 4.9453 (50.0); 4.9007 (1.0); 4.8887 (15.3); 4.8780 (1.6); 4.3122 (6.6); 4.3003 (19.7); 4.2884 (19.8); 4.2765 (8.7); 4.2646 (6.3); 4.2527 (6.3); 4.2408 (2.1); 1.3248 (21.4); 1.3129 (41.8); 1.3010 (21.0); 1.2948 (7.2); 1.2829 (13.2); 1.2711 (6.6); 1.2556 (0.6); 0.0001 (10.6); 0.0054 (0.4) I-02: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2031 (2.1); 8.2010 (1.6); 8.1989 (1.7); 8.1970 (2.1); 8.0734 (1.3); 8.0714 (1.4); 8.0688 (1.5); 8.0667 (1.3); 8.0613 (1.4); 8.0593 (1.4); 8.0567 (1.4); 8.0546 (1.3); 7.8629 (1.1); 7.8567 (1.1); 7.8440 (1.3); 7.8418 (1.4); 7.8378 (1.3); 7.8356 (1.3); 7.8229 (1.2); 7.8167 (1.2); 7.7707 (1.1); 7.7660 (1.1); 7.7523 (1.3); 7.7501 (1.6); 7.7476 (1.3); 7.7454 (1.6); 7.7317 (1.6); 7.7270 (1.6); 7.6445 (1.8); 7.6422 (3.0); 7.6399 (1.8); 7.6238 (1.3); 7.6215 (2.2); 7.6192 (1.2); 7.2610 (26.3); 7.1176 (1.4); 7.1151 (1.4); 7.1055 (1.4); 7.1029 (1.4); 7.0993 (1.4); 7.0967 (1.3); 7.0871 (1.4); 7.0845 (1.2); 6.9975 (1.6); 6.9963 (1.5); 6.9902 (1.5); 6.9888 (1.4); 6.9764 (1.4); 6.9750 (1.4); 6.9691 (1.5); 6.9677 (1.4); 4.9460 (15.8); 4.3229 (2.0); 4.3051 (6.2); 4.2873 (6.3); 4.2695 (2.0); 3.4880 (1.1); 3.4705 (1.1); 1.5506 (7.4); 1.3334 (7.7); 1.3157 (16.0); 1.2978 (7.6); 1.2263 (1.2); 1.2088 (2.4); 1.1912 (1.2); 0.0080 (1.0); 0.0002 (34.1); 0.0085 (1.0) I-03: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.5762 (1.6); 8.5671 (1.5); 8.5643 (1.6); 8.4971 (2.3); 8.4934 (2.3); 8.2124 (1.7); 8.2010 (1.7); 7.7525 (1.3); 7.7325 (1.4); 7.4880 (0.8); 7.4674 (1.6); 7.4444 (1.0); 7.3219 (1.8); 7.3110 (1.8); 7.3023 (2.4); 7.2903 (1.7); 7.2819 (0.7); 7.2620 (9.2); 5.3215 (0.6); 5.3040 (1.8); 5.2866 (1.8); 5.2691 (0.6); 3.7703 (16.0); 2.7737 (1.9); 1.7011 (7.5); 1.6837 (7.4); 0.0002 (10.4) I-04: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.6474 (1.0); 8.6434 (1.1); 8.6352 (1.1); 8.6312 (1.1); 8.4585 (1.4); 8.4539 (1.4); 8.2784 (1.0); 8.2689 (1.0); 7.8547 (0.7); 7.8503 (0.9); 7.8448 (0.7); 7.8347 (0.8); 7.8301 (1.0); 7.8248 (0.7); 7.5667 (0.6); 7.5630 (0.6); 7.5456 (1.0); 7.5422 (1.0); 7.5232 (0.8); 7.5196 (0.8); 7.4361 (0.8); 7.4268 (0.9); 7.4246 (0.8); 7.4153 (1.3); 7.4060 (0.6); 7.4038 (0.6); 7.3945 (0.6); 7.3885 (0.8); 7.3761 (0.8); 7.3685 (0.8); 7.3564 (0.8); 7.2617 (9.5); 5.2775 (1.7); 5.2600 (1.7); 3.7702 (16.0); 2.1270 (0.5); 2.0913 (0.9); 1.7023 (6.6); 1.6848 (6.5); 0.0002 (14.9) I-05: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2168 (0.7); 8.2151 (0.8); 8.2132 (0.8); 8.2115 (0.8); 8.2052 (0.7); 8.2034 (0.8); 8.2016 (0.8); 8.1999 (0.8); 8.1359 (1.1); 8.1340 (0.8); 8.1318 (0.8); 8.1297 (1.1); 7.8634 (0.6); 7.8572 (0.6); 7.8447 (0.7); 7.8423 (0.7); 7.8384 (0.7); 7.8360 (0.7); 7.8235 (0.6); 7.8172 (0.6); 7.5130 (0.6); 7.5093 (0.6); 7.4923 (0.8); 7.4888 (1.0); 7.4860 (0.7); 7.4690 (0.8); 7.4653 (0.8); 7.3390 (0.8); 7.3300 (0.8); 7.3274 (0.8); 7.3183 (1.3); 7.3094 (0.6); 7.3067 (0.6); 7.2977 (0.6); 7.2621 (21.6); 6.9586 (0.7); 6.9572 (0.8); 6.9512 (0.8); 6.9497 (0.8); 6.9374 (0.7); 6.9359 (0.8); 6.9300 (0.8); 6.9285 (0.8); 5.2887 (1.6); 5.2713 (1.6); 3.7688 (16.0); 2.0454 (0.5); 1.6986 (6.5); 1.6812 (6.5); 1.5647 (2.2); 1.2596 (0.5); 0.8818 (0.7); 0.0002 (13.4) I-08: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.0716 (0.6); 8.2690 (2.0); 8.2666 (2.7); 8.2656 (2.6); 8.2635 (2.2); 8.2573 (2.3); 8.2551 (2.9); 8.2541 (2.6); 8.2518 (2.2); 8.2214 (3.2); 8.2151 (3.5); 7.9863 (3.0); 7.9826 (2.2); 7.9804 (1.8); 7.9653 (4.1); 7.9613 (4.9); 7.9589 (2.9); 7.9578 (2.8); 7.9461 (1.8); 7.9401 (3.4); 7.9367 (2.2); 7.6052 (2.0); 7.5958 (2.4); 7.5936 (2.1); 7.5843 (3.7); 7.5750 (1.8); 7.5727 (1.9); 7.5634 (1.7); 7.2910 (2.0); 7.2897 (2.1); 7.2841 (2.2); 7.2828 (2.1); 7.2697 (2.0); 7.2684 (2.1); 7.2628 (2.1); 7.2614 (2.0); 5.7569 (1.2); 4.8568 (16.0); 3.3362 (17.9); 2.6709 (0.6); 2.5247 (1.5); 2.5200 (2.0); 2.5112 (28.2); 2.5067 (62.8); 2.5021 (89.3); 2.4975 (63.5); 2.4929 (30.3); 2.4693 (1.1); 2.3291 (0.6); 1.2472 (1.0); 0.8749 (0.5); 0.8581 (2.1); 0.8404 (0.7); 0.0080 (1.6); 0.0056 (0.5); 0.0047 (0.6); 0.0002 (52.2); 0.0050 (1.0); 0.0058 (0.9); 0.0067 (0.8); 0.0085 (1.7) I-10: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2697 (2.5); 8.2677 (2.6); 8.2595 (2.4); 8.2580 (2.7); 8.2560 (2.7); 8.1330 (3.5); 8.1268 (3.9); 7.8671 (1.6); 7.8608 (1.6); 7.8484 (1.9); 7.8458 (2.1); 7.8421 (2.0); 7.8397 (2.1); 7.8272 (1.8); 7.8210 (1.8); 7.5068 (1.6); 7.5031 (1.7); 7.4860 (2.3); 7.4827 (2.9); 7.4801 (2.1); 7.4630 (2.2); 7.4593 (2.2); 7.3572 (2.1); 7.3481 (2.5); 7.3455 (2.3); 7.3364 (3.7); 7.3274 (1.8); 7.3248 (1.8); 7.3158 (1.6); 7.2610 (26.2); 6.9684 (2.4); 6.9623 (2.4); 6.9611 (2.4); 6.9471 (2.4); 6.9410 (2.4); 6.9399 (2.3); 5.3734 (1.2); 5.3560 (4.6); 5.3385 (4.7); 5.3210 (1.3); 1.7447 (15.9); 1.7272 (16.0); 1.7147 (0.8); 0.8819 (0.7); 0.0079 (1.2); 0.0002 (40.7); 0.0085 (1.6) I-11: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.1907 (1.2); 8.1888 (1.0); 8.1865 (1.0); 8.1845 (1.2); 7.8990 (1.7); 7.8916 (1.7); 7.8418 (0.6); 7.8356 (0.6); 7.8229 (0.7); 7.8207 (0.8); 7.8167 (0.7); 7.8145 (0.7); 7.8018 (0.6); 7.7956 (0.6); 7.6469 (0.7); 7.6459 (0.7); 7.6372 (0.8); 7.6362 (0.8); 7.6243 (1.0); 7.6233 (1.0); 7.6147 (1.0); 7.6138 (1.0); 7.4984 (0.8); 7.4910 (0.7); 7.4796 (0.8); 7.4759 (0.6); 7.4722 (0.8); 7.4685 (0.6); 7.4571 (0.6); 7.4497 (0.6); 7.2629 (7.7); 7.0011 (0.8); 6.9998 (0.8); 6.9937 (0.8); 6.9925 (0.8); 6.9800 (0.8); 6.9787 (0.8); 6.9726 (0.8); 6.9712 (0.8); 5.2486 (1.6); 5.2312 (1.6); 3.7972 (16.0); 2.0449 (0.7); 1.7171 (6.3); 1.6996 (6.3); 1.5757 (0.7); 1.2641 (0.8); 1.2594 (0.9); 0.8816 (1.5); 0.8638 (0.6); 0.0002 (5.4) I-13: .sup.1H-NMR(599.6 MHz, CDCl3): = 8.1922 (12.8); 8.1884 (13.0); 7.9613 (0.4); 7.9565 (0.4); 7.9151 (14.6); 7.9102 (14.9); 7.8328 (4.0); 7.8288 (4.0); 7.8189 (6.7); 7.8161 (6.5); 7.8063 (4.3); 7.8022 (4.1); 7.6173 (6.5); 7.6110 (6.7); 7.6022 (7.7); 7.5959 (7.6); 7.5375 (0.4); 7.5334 (0.5); 7.4536 (4.7); 7.4487 (4.7); 7.4410 (5.6); 7.4386 (5.7); 7.4363 (6.0); 7.4339 (5.0); 7.4262 (4.2); 7.4212 (3.8); 7.4115 (0.4); 7.2607 (34.4); 7.0003 (7.3); 6.9959 (7.4); 6.9862 (7.2); 6.9818 (7.2); 6.6449 (0.4); 6.6292 (0.4); 5.3183 (3.0); 5.3067 (9.8); 5.2950 (9.9); 5.2833 (3.1); 5.2697 (0.4); 5.2580 (0.3); 3.9749 (0.7); 2.2711 (1.2); 1.7606 (39.1); 1.7489 (38.9); 1.7322 (1.3); 1.4320 (8.8); 1.2550 (2.8); 0.8797 (0.4); 0.0701 (0.6); 0.0052 (2.2); 0.0001 (50.0); 0.0056 (1.8) I-14: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): = 13.1318 (0.6); 8.2740 (3.6); 8.2679 (3.6); 8.1682 (4.9); 8.1607 (5.2); 8.0299 (1.4); 8.0237 (1.4); 8.0090 (2.2); 8.0028 (2.1); 7.9891 (1.5); 7.9829 (1.5); 7.9601 (1.7); 7.9526 (1.5); 7.9395 (2.0); 7.9377 (2.3); 7.9301 (2.2); 7.9171 (2.0); 7.9095 (1.8); 7.7365 (2.8); 7.7268 (2.9); 7.7138 (2.4); 7.7042 (2.3); 7.3072 (2.3); 7.3009 (2.3); 7.2859 (2.2); 7.2797 (2.1); 4.9188 (16.0); 3.3231 (1.2); 2.5249 (0.8); 2.5202 (1.0); 2.5114 (16.8); 2.5069 (36.9); 2.5023 (51.5); 2.4978 (36.1); 2.4932 (16.1); 2.1834 (0.6); 1.3559 (4.6); 0.0080 (1.0); 0.0002 (37.2); 0.0085 (1.1) I-15: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4443 (1.3); 8.4376 (1.4); 8.2932 (1.5); 8.2037 (0.8); 8.2020 (0.9); 8.2002 (0.9); 8.1921 (0.9); 8.1904 (1.0); 8.1885 (1.0); 7.5266 (1.0); 7.5239 (0.9); 7.5221 (0.9); 7.5197 (1.0); 7.5152 (0.7); 7.5070 (1.0); 7.5040 (1.8); 7.5003 (1.2); 7.4973 (0.9); 7.4929 (0.7); 7.4838 (0.8); 7.4801 (0.8); 7.3419 (0.7); 7.3329 (0.8); 7.3303 (0.8); 7.3213 (1.3); 7.3123 (0.6); 7.3096 (0.7); 7.3007 (0.6); 7.2614 (30.4); 5.2864 (1.6); 5.2690 (1.6); 3.7710 (16.0); 2.0454 (0.6); 1.7015 (6.6); 1.6841 (6.6); 1.5664 (1.7); 1.2596 (0.6); 0.8820 (0.6); 0.0080 (0.6); 0.0002 (18.4); 0.0084 (0.7) I-16: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4532 (1.8); 8.4463 (1.9); 8.3017 (1.0); 8.2979 (1.8); 8.2940 (1.0); 8.2515 (0.8); 8.2497 (0.9); 8.2479 (0.9); 8.2461 (0.8); 8.2399 (0.8); 8.2381 (0.9); 8.2362 (0.9); 8.2345 (0.8); 7.5285 (0.8); 7.5261 (0.8); 7.5241 (0.9); 7.5219 (1.2); 7.5172 (0.8); 7.5057 (1.3); 7.5019 (1.9); 7.4994 (1.6); 7.4950 (0.8); 7.4823 (0.9); 7.4786 (0.9); 7.3640 (0.9); 7.3550 (1.0); 7.3524 (0.9); 7.3434 (1.5); 7.3343 (0.7); 7.3317 (0.7); 7.3227 (0.6); 7.2617 (36.6); 4.9588 (8.4); 3.8031 (16.0); 2.9631 (1.0); 2.7750 (0.6); 2.0454 (0.5); 1.5596 (5.9); 0.0080 (0.6); 0.0002 (21.9); 0.0084 (0.7) I-17: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.0844 (1.7); 8.6499 (5.8); 8.6430 (5.8); 8.3670 (3.0); 8.3628 (5.8); 8.3589 (2.9); 8.2464 (2.1); 8.2440 (2.8); 8.2430 (2.8); 8.2409 (2.4); 8.2348 (2.4); 8.2325 (3.0); 8.2294 (2.3); 7.9959 (1.8); 7.9924 (1.8); 7.9750 (2.1); 7.9710 (3.2); 7.9672 (2.0); 7.9498 (2.1); 7.9463 (2.0); 7.8424 (2.0); 7.8381 (2.1); 7.8355 (2.1); 7.8311 (1.9); 7.8188 (2.2); 7.8144 (2.3); 7.8119 (2.0); 7.8075 (1.9); 7.6006 (2.1); 7.5913 (2.4); 7.5890 (2.2); 7.5797 (3.8); 7.5704 (1.8); 7.5682 (2.0); 7.5588 (1.7); 5.7568 (4.2); 4.8604 (16.0); 3.3190 (34.6); 2.6745 (1.0); 2.6698 (1.5); 2.6652 (1.1); 2.6607 (0.5); 2.5405 (1.2); 2.5237 (3.1); 2.5190 (4.7); 2.5102 (79.1); 2.5056 (175.0); 2.5011 (247.3); 2.4965 (172.8); 2.4919 (78.5); 2.4742 (3.7); 2.4703 (3.4); 2.3328 (1.0); 2.3281 (1.5); 2.3235 (1.1); 0.1457 (0.7); 0.0079 (6.6); 0.0055 (1.5); 0.0002 (243.0); 0.0068 (2.5); 0.0085 (7.4); 0.0139 (0.9); 0.0155 (0.8); 0.0187 (0.6); 0.0211 (0.6); 0.0226 (0.7); 0.0258 (0.5); 0.0275 (0.9); 0.0313 (0.9); 0.0322 (0.8); 0.0344 (0.5); 0.1495 (0.7) I-18: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4613 (3.2); 8.4547 (3.3); 8.3036 (3.5); 8.2283 (2.4); 8.2263 (2.5); 8.2183 (2.2); 8.2166 (2.5); 8.2147 (2.4); 7.5540 (1.6); 7.5496 (1.7); 7.5471 (1.8); 7.5427 (1.6); 7.5319 (1.7); 7.5275 (1.9); 7.5250 (1.8); 7.5190 (2.2); 7.5142 (1.7); 7.4972 (2.2); 7.4939 (2.7); 7.4911 (1.9); 7.4740 (2.1); 7.4703 (2.0); 7.3554 (2.0); 7.3463 (2.3); 7.3438 (2.1); 7.3347 (3.5); 7.3257 (1.6); 7.3230 (1.7); 7.3141 (1.6); 7.2704 (1.0); 7.2697 (1.0); 7.2680 (1.1); 7.2672 (1.3); 7.2664 (1.6); 7.2606 (212.2); 7.2494 (0.5); 6.9970 (1.1); 5.3576 (1.2); 5.3401 (4.7); 5.3226 (4.8); 5.3052 (1.2); 5.3002 (0.9); 2.7754 (0.7); 1.7488 (16.0); 1.7313 (15.9); 1.7142 (0.6); 1.2425 (1.2); 1.2390 (1.2); 1.2222 (0.5); 0.0080 (3.7); 0.0056 (1.1); 0.0047 (1.5); 0.0002 (126.8); 0.0058 (1.4); 0.0066 (1.2); 0.0084 (3.3); 0.0115 (0.5) I-100: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2102 (2.1); 8.2062 (1.7); 8.2040 (2.2); 8.0824 (1.2); 8.0804 (1.4); 8.0778 (1.4); 8.0757 (1.4); 8.0703 (1.3); 8.0683 (1.4); 8.0656 (1.4); 8.0636 (1.3); 7.8669 (1.2); 7.8607 (1.1); 7.8480 (1.3); 7.8458 (1.4); 7.8419 (1.3); 7.8396 (1.4); 7.8269 (1.2); 7.8207 (1.2); 7.7753 (1.1); 7.7705 (1.1); 7.7568 (1.3); 7.7546 (1.7); 7.7521 (1.4); 7.7499 (1.6); 7.7362 (1.6); 7.7315 (1.6); 7.6443 (1.7); 7.6420 (3.0); 7.6397 (1.8); 7.6236 (1.2); 7.6213 (2.1); 7.6191 (1.3); 7.2606 (32.0); 7.1228 (1.4); 7.1203 (1.4); 7.1107 (1.3); 7.1081 (1.4); 7.1045 (1.4); 7.1019 (1.3); 7.0923 (1.3); 7.0897 (1.3); 6.9995 (1.5); 6.9981 (1.6); 6.9921 (1.5); 6.9907 (1.5); 6.9784 (1.4); 6.9770 (1.5); 6.9710 (1.4); 6.9696 (1.5); 4.9473 (16.0); 4.3249 (2.0); 4.3071 (6.3); 4.2893 (6.4); 4.2715 (2.1); 1.5495 (3.4); 1.3346 (7.8); 1.3168 (16.0); 1.2989 (7.6); 0.0080 (1.3); 0.0002 (47.6); 0.0085 (1.4) I-101: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.1754 (2.3); 8.1693 (2.3); 8.0295 (1.4); 8.0275 (1.5); 8.0249 (1.6); 8.0229 (1.4); 8.0174 (1.4); 8.0154 (1.5); 8.0127 (1.5); 8.0107 (1.4); 7.8344 (1.2); 7.8282 (1.1); 7.8153 (1.4); 7.8134 (1.5); 7.8091 (1.4); 7.8072 (1.4); 7.7943 (1.2); 7.7881 (1.2); 7.7470 (1.1); 7.7422 (1.0); 7.7285 (1.2); 7.7262 (1.7); 7.7239 (1.3); 7.7215 (1.6); 7.7079 (1.7); 7.7031 (1.6); 7.6383 (1.8); 7.6361 (3.3); 7.6339 (2.0); 7.6177 (1.3); 7.6154 (2.2); 7.6131 (1.2); 7.2615 (16.8); 7.0810 (1.4); 7.0785 (1.5); 7.0689 (1.4); 7.0663 (1.5); 7.0628 (1.5); 7.0601 (1.4); 7.0506 (1.4); 7.0480 (1.3); 6.9933 (1.6); 6.9871 (1.6); 6.9721 (1.6); 6.9660 (1.5); 5.2437 (0.9); 5.2262 (3.1); 5.2088 (3.2); 5.1914 (0.9); 4.2901 (1.0); 4.2831 (1.1); 4.2722 (3.1); 4.2654 (3.2); 4.2544 (3.2); 4.2477 (3.1); 4.2366 (1.1); 4.2300 (1.0); 1.7114 (11.9); 1.6939 (11.9); 1.5609 (8.8); 1.3049 (7.9); 1.2871 (16.0); 1.2692 (8.6); 0.8987 (1.0); 0.8818 (3.6); 0.8641 (1.4); 0.0079 (0.5); 0.0002 (19.0); 0.0085 (0.6) I-102: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1982 (2.3); 8.1921 (2.4); 8.0465 (1.4); 8.0445 (1.5); 8.0419 (1.6); 8.0399 (1.5); 8.0344 (1.5); 8.0324 (1.6); 8.0298 (1.6); 8.0277 (1.5); 7.8583 (1.2); 7.8521 (1.2); 7.8393 (1.4); 7.8372 (1.5); 7.8332 (1.4); 7.8311 (1.4); 7.8183 (1.3); 7.8121 (1.2); 7.7579 (1.1); 7.7531 (1.1); 7.7395 (1.3); 7.7372 (1.8); 7.7348 (1.4); 7.7325 (1.7); 7.7189 (1.7); 7.7141 (1.7); 7.6375 (1.8); 7.6354 (3.1); 7.6332 (1.9); 7.6169 (1.3); 7.6147 (2.2); 7.6125 (1.2); 7.2626 (23.6); 7.0980 (1.5); 7.0954 (1.5); 7.0859 (1.5); 7.0833 (1.6); 7.0797 (1.6); 7.0771 (1.5); 7.0675 (1.5); 7.0650 (1.4); 6.9934 (1.6); 6.9920 (1.6); 6.9861 (1.6); 6.9847 (1.6); 6.9722 (1.5); 6.9709 (1.6); 6.9650 (1.6); 6.9636 (1.5); 5.2555 (0.9); 5.2381 (3.2); 5.2207 (3.3); 5.2033 (0.9); 4.2935 (1.0); 4.2864 (1.1); 4.2757 (3.1); 4.2687 (3.1); 4.2578 (3.2); 4.2510 (3.1); 4.2401 (1.1); 4.2333 (1.0); 3.5060 (1.9); 3.4885 (6.0); 3.4710 (6.1); 3.4535 (2.0); 1.7152 (12.3); 1.6978 (12.2); 1.5835 (6.5); 1.3055 (7.7); 1.2877 (16.0); 1.2699 (7.7); 1.2263 (6.4); 1.2088 (12.8); 1.1912 (6.2); 0.8820 (0.5); 0.0002 (11.4) I-103: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 8.2163 (3.4); 8.2101 (3.6); 8.0964 (2.2); 8.0944 (2.4); 8.0917 (2.7); 8.0897 (2.5); 8.0843 (2.4); 8.0823 (2.6); 8.0796 (2.7); 8.0776 (2.4); 7.9897 (1.6); 7.9834 (1.6); 7.9723 (2.5); 7.9680 (3.6); 7.9637 (2.2); 7.9624 (2.3); 7.9538 (2.6); 7.9518 (2.9); 7.9491 (4.0); 7.9472 (3.0); 7.9427 (1.8); 7.9333 (2.6); 7.9285 (2.4); 7.6686 (2.6); 7.6664 (4.8); 7.6642 (2.8); 7.6480 (2.4); 7.6459 (4.3); 7.6436 (2.4); 7.2933 (2.3); 7.2876 (2.3); 7.2719 (2.4); 7.2693 (3.1); 7.2667 (4.5); 7.2572 (2.3); 7.2547 (2.5); 7.2508 (2.5); 7.2484 (2.2); 7.2387 (2.3); 7.2362 (2.3); 4.8941 (16.0); 4.0382 (0.8); 4.0204 (0.8); 3.3370 (9.0); 2.5256 (0.8); 2.5209 (1.1); 2.5122 (15.4); 2.5076 (34.1); 2.5030 (48.2); 2.4984 (34.1); 2.4939 (15.6); 1.9891 (3.6); 1.9100 (4.0); 1.3559 (1.3); 1.1924 (1.0); 1.1747 (2.2); 1.1569 (1.0) I-104: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5475 (2.6); 8.5406 (2.6); 8.3448 (1.5); 8.3411 (2.6); 8.3375 (1.5); 8.1952 (1.2); 8.1930 (1.3); 8.1907 (1.4); 8.1885 (1.3); 8.1831 (1.2); 8.1807 (1.4); 8.1788 (1.4); 8.1764 (1.3); 7.9271 (0.7); 7.9225 (0.7); 7.9096 (0.6); 7.9066 (1.9); 7.9021 (1.9); 7.8892 (2.3); 7.8848 (2.3); 7.8811 (2.1); 7.8788 (2.4); 7.8774 (2.7); 7.8749 (2.4); 7.8606 (0.8); 7.8584 (0.9); 7.8570 (0.6); 7.5385 (1.2); 7.5341 (1.3); 7.5316 (1.3); 7.5272 (1.2); 7.5167 (1.3); 7.5123 (1.4); 7.5098 (1.3); 7.5054 (1.2); 7.3327 (1.4); 7.3289 (1.4); 7.3206 (1.4); 7.3166 (1.5); 7.3153 (1.6); 7.3115 (1.3); 7.3033 (1.4); 7.2993 (1.3); 7.2647 (10.0); 5.3012 (13.1); 4.4380 (15.8); 4.2762 (2.1); 4.2583 (6.8); 4.2405 (6.8); 4.2226 (2.2); 1.6028 (2.1); 1.2834 (7.6); 1.2656 (16.0); 1.2592 (0.6); 1.2568 (0.6); 1.2551 (0.6); 1.2477 (7.4); 0.0705 (3.1); 0.0002 (10.6) I-105: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.1519 (2.3); 8.1459 (2.3); 8.0663 (1.6); 8.0636 (1.6); 8.0543 (1.6); 8.0514 (1.6); 7.8464 (0.9); 7.8403 (0.8); 7.8259 (1.3); 7.8202 (1.2); 7.8067 (0.9); 7.8006 (0.9); 7.7838 (1.1); 7.7790 (1.2); 7.7633 (1.8); 7.7586 (1.7); 7.7446 (1.6); 7.7399 (1.5); 7.6305 (3.0); 7.6099 (2.3); 7.2608 (31.2); 7.1562 (1.4); 7.1537 (1.4); 7.1440 (1.5); 7.1416 (1.5); 7.1377 (1.5); 7.1351 (1.4); 7.1255 (1.4); 7.1230 (1.3); 6.9861 (1.7); 6.9788 (1.7); 6.9659 (1.7); 6.9579 (1.6); 5.2999 (5.7); 4.9538 (16.0); 4.9476 (1.4); 4.7851 (0.6); 4.3166 (2.1); 4.2987 (6.4); 4.2808 (6.6); 4.2686 (0.7); 4.2630 (2.2); 3.9012 (0.8); 1.5454 (11.2); 1.3279 (7.7); 1.3204 (1.2); 1.3101 (15.6); 1.3025 (1.0); 1.2991 (1.2); 1.2923 (7.6); 1.2812 (0.6); 1.2552 (0.8); 0.0080 (1.3); 0.0002 (42.0); 0.0085 (1.4) I-106: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5338 (3.0); 8.5269 (3.1); 8.3349 (1.6); 8.3312 (3.0); 8.3276 (1.6); 8.1816 (1.2); 8.1794 (1.3); 8.1771 (1.4); 8.1749 (1.3); 8.1695 (1.3); 8.1672 (1.4); 8.1651 (1.4); 8.1628 (1.3); 7.9156 (0.8); 7.9110 (0.8); 7.8979 (0.7); 7.8951 (1.9); 7.8906 (1.8); 7.8775 (2.2); 7.8731 (2.2); 7.8668 (2.0); 7.8645 (2.4); 7.8633 (2.7); 7.8609 (2.3); 7.8463 (0.9); 7.8440 (1.0); 7.8428 (0.8); 7.8404 (0.6); 7.5133 (1.3); 7.5089 (1.3); 7.5064 (1.4); 7.5020 (1.2); 7.4913 (1.3); 7.4869 (1.4); 7.4845 (1.3); 7.4801 (1.3); 7.3059 (1.4); 7.3022 (1.4); 7.2937 (1.3); 7.2900 (1.4); 7.2883 (1.6); 7.2846 (1.3); 7.2762 (1.4); 7.2725 (1.4); 7.2626 (22.8); 5.3006 (9.1); 4.4170 (16.0); 4.2811 (1.7); 4.2633 (5.5); 4.2455 (5.8); 4.2277 (1.9); 1.5794 (5.8); 1.2966 (7.4); 1.2788 (15.6); 1.2609 (7.4); 0.0696 (3.7); 0.0080 (0.6); 0.0002 (24.8); 0.0085 (0.7) I-107: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.1455 (1.9); 8.1395 (1.9); 8.0421 (1.2); 8.0403 (1.3); 8.0376 (1.4); 8.0356 (1.2); 8.0301 (1.3); 8.0281 (1.4); 8.0254 (1.4); 8.0235 (1.3); 7.8393 (0.8); 7.8333 (0.7); 7.8187 (1.1); 7.8131 (1.1); 7.7993 (0.8); 7.7934 (0.8); 7.7702 (1.0); 7.7654 (1.0); 7.7516 (1.2); 7.7497 (1.5); 7.7469 (1.3); 7.7450 (1.4); 7.7311 (1.4); 7.7263 (1.4); 7.6239 (1.6); 7.6217 (2.8); 7.6011 (2.0); 7.2609 (25.4); 7.1369 (1.3); 7.1345 (1.3); 7.1248 (1.3); 7.1223 (1.3); 7.1184 (1.2); 7.1159 (1.1); 7.1063 (1.2); 7.1038 (1.2); 6.9814 (1.4); 6.9741 (1.4); 6.9603 (1.4); 6.9542 (1.3); 5.2716 (0.7); 5.2543 (2.5); 5.2369 (2.6); 5.2195 (0.8); 4.2856 (1.0); 4.2817 (1.0); 4.2678 (3.0); 4.2639 (3.0); 4.2499 (3.1); 4.2462 (2.9); 4.2320 (1.0); 4.2284 (1.0); 1.7113 (0.6); 1.6999 (10.5); 1.6942 (1.0); 1.6825 (10.3); 1.5508 (16.0); 1.3047 (0.6); 1.2986 (6.5); 1.2870 (1.4); 1.2808 (13.5); 1.2693 (1.3); 1.2630 (6.8); 0.8819 (0.6); 0.0080 (0.8); 0.0002 (28.3); 0.0085 (0.8) I-108: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2005 (1.1); 8.1943 (1.2); 8.0860 (0.6); 8.0750 (0.6); 7.8559 (0.6); 7.8496 (0.6); 7.8369 (0.7); 7.8348 (0.8); 7.8308 (0.7); 7.8286 (0.7); 7.8158 (0.6); 7.8097 (0.6); 7.7536 (0.6); 7.2606 (39.7); 6.9925 (0.7); 6.9853 (0.7); 6.9715 (0.7); 6.9642 (0.7); 5.3003 (5.3); 5.1175 (1.3); 5.0434 (0.9); 3.7107 (2.3); 3.6798 (1.6); 3.1571 (0.6); 2.0455 (1.2); 1.5446 (16.0); 1.2596 (0.9); 0.0080 (1.6); 0.0058 (0.5); 0.0050 (0.5); 0.0002 (64.7); 0.0085 (2.0) I-109: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2018 (2.0); 8.2000 (2.1); 8.1978 (1.9); 8.1958 (2.2); 8.0848 (1.5); 8.0828 (1.6); 8.0801 (1.7); 8.0781 (1.5); 8.0726 (1.6); 8.0707 (1.6); 8.0680 (1.7); 8.0660 (1.4); 7.8572 (0.6); 7.8540 (0.7); 7.8510 (0.7); 7.8479 (0.7); 7.8381 (0.8); 7.8356 (1.2); 7.8326 (1.3); 7.8296 (1.2); 7.8268 (0.8); 7.8172 (0.7); 7.8140 (0.7); 7.8110 (0.7); 7.8079 (0.7); 7.7792 (0.8); 7.7745 (0.8); 7.7588 (1.5); 7.7574 (1.4); 7.7541 (1.4); 7.7401 (1.2); 7.7353 (1.2); 7.6558 (1.0); 7.6536 (1.6); 7.6513 (1.0); 7.6418 (1.1); 7.6396 (1.7); 7.6373 (1.1); 7.6353 (0.9); 7.6330 (1.2); 7.6307 (0.7); 7.6212 (0.8); 7.6190 (1.2); 7.6167 (0.7); 7.2620 (23.2); 7.1218 (1.6); 7.1192 (1.6); 7.1096 (1.6); 7.1070 (1.6); 7.1034 (1.6); 7.1008 (1.4); 7.0913 (1.5); 7.0887 (1.4); 6.9927 (1.6); 6.9853 (1.7); 6.9715 (1.6); 6.9642 (1.6); 5.3004 (13.5); 4.9833 (5.7); 4.9754 (3.7); 4.9721 (3.3); 3.8745 (1.3); 3.8643 (1.2); 3.8569 (1.3); 3.8449 (1.7); 3.8291 (1.1); 3.8229 (1.3); 3.8130 (1.2); 3.7606 (0.6); 3.7543 (0.9); 3.7428 (15.2); 3.7298 (0.6); 3.7195 (16.0); 3.6631 (0.7); 3.6381 (0.5); 3.5889 (0.7); 3.5588 (0.5); 3.2273 (0.6); 3.2088 (0.9); 3.1904 (0.6); 3.1157 (0.6); 3.0984 (0.8); 3.0796 (0.6); 2.3251 (0.8); 2.3073 (1.0); 2.2893 (0.9); 2.2743 (0.7); 2.2219 (0.6); 2.2033 (1.1); 2.1895 (0.7); 2.1842 (1.3); 2.1646 (1.0); 1.5761 (7.2); 0.0079 (1.0); 0.0002 (36.5); 0.0085 (1.0) I-110: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2024 (1.8); 8.1966 (2.2); 8.0706 (1.5); 8.0588 (1.5); 7.8533 (0.7); 7.8472 (0.8); 7.8324 (1.2); 7.8281 (1.3); 7.8133 (0.8); 7.8072 (0.9); 7.7781 (0.7); 7.7736 (0.7); 7.7573 (1.5); 7.7530 (1.4); 7.7394 (1.3); 7.7349 (1.3); 7.7063 (2.2); 7.6858 (1.1); 7.6621 (0.5); 7.2627 (8.3); 7.1150 (1.0); 7.1124 (1.0); 7.1027 (1.2); 7.1000 (1.3); 7.0973 (1.2); 7.0944 (1.0); 7.0850 (0.9); 7.0822 (0.8); 6.9884 (1.3); 6.9817 (1.3); 6.9675 (1.3); 6.9606 (1.2); 5.3005 (6.3); 5.0258 (8.2); 4.9364 (0.9); 4.9231 (0.8); 4.6059 (0.8); 4.5970 (1.0); 4.5859 (0.9); 4.5759 (0.9); 3.7904 (0.9); 3.7779 (0.8); 3.7717 (0.8); 3.7582 (4.0); 3.7168 (16.0); 3.7011 (1.2); 3.6833 (1.2); 3.6659 (0.6); 3.6588 (0.8); 2.2218 (0.6); 2.2096 (0.7); 2.1958 (0.6); 2.1891 (0.6); 2.1786 (0.7); 2.1666 (0.5); 2.1511 (0.6); 2.1353 (0.6); 2.0640 (0.9); 2.0453 (2.7); 2.0332 (1.1); 2.0200 (0.8); 1.5923 (3.1); 1.2773 (0.6); 1.2594 (1.4); 1.2416 (0.6); 0.0002 (12.8) I-111: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 8.2464 (2.3); 8.2421 (2.0); 8.2403 (2.3); 8.1035 (1.2); 8.1015 (1.4); 8.0988 (1.8); 8.0968 (1.8); 8.0943 (0.7); 8.0915 (1.5); 8.0894 (1.5); 8.0867 (1.8); 8.0847 (1.8); 8.0183 (0.9); 8.0122 (0.9); 7.9972 (1.5); 7.9924 (1.2); 7.9910 (1.2); 7.9777 (1.1); 7.9731 (1.5); 7.9716 (1.2); 7.9685 (1.1); 7.9584 (0.5); 7.9546 (1.6); 7.9526 (1.6); 7.9499 (1.3); 7.9479 (1.4); 7.9341 (1.5); 7.9293 (1.3); 7.7515 (1.4); 7.7492 (2.6); 7.7470 (1.6); 7.7309 (1.3); 7.7287 (2.3); 7.7264 (1.3); 7.7059 (0.8); 7.6853 (0.7); 7.3033 (1.6); 7.2975 (1.6); 7.2836 (2.7); 7.2814 (2.8); 7.2764 (1.7); 7.2717 (1.4); 7.2691 (1.6); 7.2654 (1.6); 7.2627 (1.5); 7.2596 (0.5); 7.2532 (1.3); 7.2505 (1.5); 5.0709 (4.1); 5.0654 (3.6); 5.0352 (0.7); 4.8073 (0.6); 4.7709 (0.5); 4.3088 (1.0); 4.2987 (1.2); 4.2870 (1.2); 4.2770 (1.0); 4.0557 (1.1); 4.0379 (3.3); 4.0202 (3.4); 4.0024 (1.1); 3.6395 (0.7); 3.6239 (1.3); 3.6074 (0.9); 3.6012 (1.8); 3.5842 (0.8); 3.5771 (0.6); 3.3227 (5.1); 2.5411 (1.3); 2.5243 (0.8); 2.5197 (1.1); 2.5109 (17.0); 2.5063 (37.8); 2.5017 (53.3); 2.4972 (37.4); 2.4926 (16.9); 2.1946 (0.5); 2.1835 (0.8); 2.1731 (0.8); 2.1634 (0.8); 2.1532 (0.5); 2.1445 (0.7); 1.9888 (16.0); 1.9679 (1.7); 1.9506 (1.2); 1.9334 (0.5); 1.9090 (1.0); 1.9045 (0.6); 1.8858 (0.6); 1.8753 (0.6); 1.8717 (0.5); 1.7593 (0.6); 1.3555 (3.5); 1.2352 (1.2); 1.1922 (4.6); 1.1745 (9.3); 1.1567 (4.4); 0.0080 (1.0); 0.0002 (35.3); 0.0085 (1.0) I-112: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2026 (1.9); 8.2004 (1.5); 8.1984 (1.6); 8.1964 (2.0); 8.1944 (1.4); 8.0863 (1.2); 8.0843 (1.4); 8.0816 (1.5); 8.0795 (1.4); 8.0742 (1.4); 8.0721 (1.5); 8.0695 (1.5); 8.0674 (1.4); 7.8561 (1.1); 7.8499 (1.1); 7.8372 (1.3); 7.8350 (1.4); 7.8310 (1.3); 7.8288 (1.3); 7.8161 (1.2); 7.8099 (1.2); 7.7840 (1.1); 7.7792 (1.1); 7.7655 (1.3); 7.7634 (1.6); 7.7608 (1.3); 7.7586 (1.6); 7.7449 (1.7); 7.7402 (1.6); 7.6485 (1.6); 7.6462 (3.0); 7.6439 (1.8); 7.6279 (1.3); 7.6256 (2.2); 7.6232 (1.2); 7.2623 (19.3); 7.1215 (1.4); 7.1189 (1.4); 7.1093 (1.4); 7.1068 (1.5); 7.1031 (1.5); 7.1005 (1.4); 7.0909 (1.4); 7.0883 (1.3); 6.9928 (1.4); 6.9913 (1.4); 6.9855 (1.4); 6.9839 (1.4); 6.9717 (1.4); 6.9701 (1.4); 6.9643 (1.4); 6.9628 (1.4); 5.3003 (14.6); 5.0555 (2.9); 5.0406 (3.0); 4.1890 (2.0); 4.1712 (6.4); 4.1533 (6.5); 4.1355 (2.0); 3.2242 (0.5); 2.9432 (0.5); 2.5978 (0.6); 2.5876 (1.1); 2.5775 (0.6); 2.5612 (0.6); 2.0453 (1.0); 1.9937 (0.8); 1.9686 (0.5); 1.5773 (3.7); 1.2823 (7.4); 1.2774 (0.6); 1.2645 (16.0); 1.2596 (1.3); 1.2467 (7.2); 1.2418 (0.6); 0.0079 (0.8); 0.0002 (30.9); 0.0028 (1.8); 0.0043 (0.9); 0.0052 (0.7); 0.0060 (0.6); 0.0085 (1.0) I-113: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3320 (2.4); 8.3303 (2.5); 8.3259 (2.5); 8.3242 (2.4); 8.1160 (1.1); 8.1138 (1.2); 8.1116 (1.4); 8.1093 (1.2); 8.1039 (1.2); 8.1012 (1.4); 8.0999 (1.5); 8.0972 (1.2); 7.8253 (0.6); 7.8208 (0.5); 7.8047 (1.9); 7.8002 (1.8); 7.7879 (2.3); 7.7834 (4.0); 7.7811 (2.7); 7.7785 (2.3); 7.7647 (0.7); 7.7625 (0.7); 7.7028 (2.4); 7.6967 (2.3); 7.6822 (2.7); 7.6761 (2.6); 7.3929 (3.0); 7.3912 (3.0); 7.3723 (2.6); 7.3706 (2.6); 7.2633 (6.3); 7.1806 (1.2); 7.1763 (1.2); 7.1685 (1.2); 7.1639 (2.3); 7.1595 (1.2); 7.1520 (1.2); 7.1474 (1.1); 5.3001 (3.1); 4.2643 (2.0); 4.2465 (6.2); 4.2287 (6.2); 4.2109 (2.0); 3.9398 (16.0); 1.5827 (5.8); 1.3003 (7.2); 1.2824 (14.6); 1.2646 (7.0); 0.0705 (1.7); 0.0002 (8.3) I-114: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2039 (1.4); 8.2017 (1.3); 8.1979 (1.8); 8.0764 (1.2); 8.0743 (1.3); 8.0717 (1.4); 8.0697 (1.3); 8.0643 (1.3); 8.0622 (1.4); 8.0596 (1.4); 8.0575 (1.3); 7.8566 (0.7); 7.8503 (0.8); 7.8375 (0.9); 7.8355 (0.9); 7.8312 (1.0); 7.8294 (1.1); 7.8166 (0.8); 7.8103 (0.9); 7.7791 (0.6); 7.7745 (0.6); 7.7610 (1.0); 7.7585 (1.4); 7.7539 (1.1); 7.7405 (1.3); 7.7358 (1.2); 7.7068 (1.2); 7.7045 (2.0); 7.7021 (1.4); 7.6863 (0.8); 7.6840 (1.1); 7.6813 (0.9); 7.6785 (0.6); 7.2619 (16.5); 7.1151 (0.9); 7.1121 (0.9); 7.1029 (1.1); 7.1000 (1.1); 7.0970 (1.0); 7.0941 (0.9); 7.0849 (0.9); 7.0820 (0.8); 6.9900 (1.2); 6.9827 (1.2); 6.9688 (1.2); 6.9615 (1.2); 5.3003 (8.7); 5.1281 (8.8); 5.0156 (1.9); 4.2225 (1.8); 4.1929 (7.5); 3.7930 (3.6); 3.7375 (16.0); 3.1866 (15.4); 3.0605 (3.1); 2.0453 (2.0); 1.5735 (5.7); 1.2773 (0.6); 1.2594 (1.4); 1.2562 (0.6); 1.2416 (0.6); 0.0079 (0.7); 0.0002 (25.4); 0.0085 (0.9) I-115: .sup.1H-NMR(400.0 MHz, CDCl3): = 9.2263 (4.1); 8.8053 (0.6); 8.7652 (10.3); 8.0695 (0.9); 8.0576 (0.9); 7.8596 (0.6); 7.8423 (1.4); 7.8397 (1.8); 7.8366 (1.4); 7.8280 (1.3); 7.8235 (1.1); 7.8104 (1.1); 7.8059 (1.0); 7.2603 (68.5); 7.1733 (0.8); 7.1697 (0.8); 7.1612 (0.8); 7.1577 (0.9); 7.1523 (0.7); 7.1435 (0.8); 7.1401 (0.7); 4.2757 (1.2); 4.2579 (3.9); 4.2400 (3.8); 4.2222 (1.3); 3.9539 (9.9); 1.7397 (2.8); 1.5435 (16.0); 1.3115 (4.6); 1.2936 (9.2); 1.2758 (4.4); 1.2557 (1.0); 0.0080 (2.6); 0.0002 (93.7); 0.0085 (2.6) I-116: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2102 (1.2); 8.2081 (0.9); 8.2041 (1.2); 8.0726 (0.7); 8.0706 (0.8); 8.0679 (0.8); 8.0659 (0.8); 8.0605 (0.8); 8.0585 (0.8); 8.0558 (0.9); 8.0538 (0.8); 7.8670 (0.6); 7.8608 (0.6); 7.8480 (0.7); 7.8459 (0.8); 7.8418 (0.8); 7.8397 (0.8); 7.8270 (0.7); 7.8208 (0.7); 7.7845 (0.6); 7.7797 (0.6); 7.7660 (0.7); 7.7638 (0.9); 7.7613 (0.8); 7.7591 (0.9); 7.7455 (0.9); 7.7407 (0.9); 7.6608 (1.0); 7.6586 (1.7); 7.6563 (1.0); 7.6402 (0.7); 7.6380 (1.2); 7.6357 (0.7); 7.2622 (6.1); 7.1220 (0.8); 7.1194 (0.8); 7.1099 (0.8); 7.1073 (0.8); 7.1036 (0.8); 7.1011 (0.8); 7.0915 (0.8); 7.0889 (0.7); 6.9978 (0.9); 6.9965 (0.8); 6.9904 (0.9); 6.9892 (0.8); 6.9766 (0.8); 6.9754 (0.8); 6.9693 (0.9); 6.9680 (0.8); 4.9481 (8.5); 4.5227 (2.0); 4.5070 (4.3); 4.4913 (2.2); 3.6845 (16.0); 2.7182 (2.0); 2.7026 (4.1); 2.6869 (2.0); 1.5648 (1.0); 0.0002 (9.7) I-117: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2124 (1.4); 8.2063 (1.4); 8.0812 (0.9); 8.0784 (1.0); 8.0691 (1.0); 8.0663 (1.0); 7.8607 (0.6); 7.8545 (0.6); 7.8416 (0.8); 7.8396 (0.9); 7.8355 (0.8); 7.8335 (0.8); 7.8207 (0.7); 7.8146 (0.7); 7.8064 (0.6); 7.8017 (0.6); 7.7858 (1.0); 7.7833 (0.9); 7.7812 (1.0); 7.7674 (1.0); 7.7627 (0.9); 7.6988 (1.9); 7.6782 (1.2); 7.2612 (15.7); 7.1464 (0.8); 7.1440 (0.8); 7.1343 (0.8); 7.1318 (0.9); 7.1282 (0.9); 7.1257 (0.8); 7.1160 (0.9); 7.1135 (0.9); 7.0077 (1.0); 7.0005 (1.0); 6.9867 (1.0); 6.9794 (1.0); 4.8751 (8.4); 3.6809 (16.0); 3.6684 (2.4); 3.6532 (2.4); 3.6378 (1.0); 2.6295 (1.9); 2.6142 (3.0); 2.5992 (1.9); 1.5551 (6.5); 1.2556 (0.7); 0.0078 (0.9); 0.0002 (25.1); 0.0085 (1.0) I-118: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.6501 (1.0); 8.4673 (1.2); 8.4527 (2.6); 8.4379 (1.2); 8.2656 (3.8); 8.2614 (3.0); 8.2594 (3.9); 8.1151 (2.5); 8.1131 (2.8); 8.1105 (3.2); 8.1084 (2.9); 8.1031 (2.7); 8.1010 (3.1); 8.0984 (3.1); 8.0963 (2.8); 8.0331 (1.8); 8.0269 (1.8); 8.0135 (2.3); 8.0119 (2.5); 8.0073 (2.2); 8.0057 (2.4); 7.9924 (2.0); 7.9861 (2.0); 7.9818 (2.4); 7.9770 (2.2); 7.9633 (2.7); 7.9611 (3.0); 7.9586 (2.5); 7.9564 (2.9); 7.9427 (3.1); 7.9379 (2.9); 7.7796 (3.1); 7.7773 (5.7); 7.7750 (3.2); 7.7589 (2.7); 7.7567 (4.8); 7.7544 (2.6); 7.3128 (2.4); 7.3115 (2.6); 7.3059 (2.6); 7.3046 (2.5); 7.2988 (3.0); 7.2963 (3.0); 7.2916 (2.5); 7.2902 (2.8); 7.2866 (3.3); 7.2843 (5.1); 7.2804 (3.1); 7.2779 (2.6); 7.2683 (2.8); 7.2657 (2.7); 4.8733 (16.0); 3.8544 (7.9); 3.8396 (7.9); 3.6217 (0.8); 3.6177 (4.3); 3.6155 (2.4); 3.6115 (2.2); 3.6093 (1.7); 3.6074 (3.0); 3.6029 (3.2); 3.6011 (9.9); 3.5989 (3.4); 3.5950 (3.1); 3.5931 (1.7); 3.5908 (2.1); 3.5867 (2.2); 3.5845 (4.4); 3.5806 (0.7); 3.3225 (12.0); 3.2025 (1.2); 2.6706 (0.6); 2.5244 (1.9); 2.5197 (2.6); 2.5110 (34.2); 2.5064 (74.6); 2.5018 (104.1); 2.4972 (71.1); 2.4926 (30.7); 2.3289 (0.6); 2.1831 (0.8); 1.9950 (1.0); 1.9090 (0.8); 1.7808 (0.7); 1.7761 (4.3); 1.7744 (1.9); 1.7684 (3.4); 1.7641 (2.1); 1.7595 (12.5); 1.7548 (2.2); 1.7505 (3.4); 1.7429 (4.3); 1.7383 (0.6); 1.3555 (7.5); 1.2390 (0.8); 1.0897 (0.5); 1.0744 (0.5); 0.0079 (1.6); 0.0038 (0.7); 0.0002 (63.1); 0.0027 (2.6); 0.0043 (0.9); 0.0052 (0.6); 0.0060 (0.5); 0.0085 (1.8) I-119: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 8.2715 (1.8); 8.2653 (1.8); 8.1037 (1.1); 8.1017 (1.2); 8.0991 (1.4); 8.0971 (1.2); 8.0916 (1.2); 8.0896 (1.3); 8.0870 (1.3); 8.0849 (1.2); 8.0400 (0.8); 8.0338 (0.8); 8.0203 (1.1); 8.0189 (1.1); 8.0141 (1.0); 8.0127 (1.1); 7.9993 (0.9); 7.9930 (0.8); 7.9721 (1.0); 7.9675 (1.0); 7.9536 (1.2); 7.9515 (1.3); 7.9489 (1.2); 7.9468 (1.2); 7.9330 (1.3); 7.9283 (1.2); 7.6904 (1.3); 7.6883 (2.3); 7.6862 (1.3); 7.6698 (1.2); 7.6677 (2.0); 7.6655 (1.1); 7.3036 (1.2); 7.2980 (1.2); 7.2840 (2.2); 7.2819 (2.3); 7.2767 (1.2); 7.2753 (1.2); 7.2721 (1.2); 7.2696 (1.2); 7.2657 (1.2); 7.2633 (1.1); 7.2536 (1.1); 7.2511 (1.1); 5.7566 (16.0); 4.8364 (3.2); 4.4534 (0.6); 4.4280 (0.6); 4.0379 (1.4); 4.0201 (1.4); 3.3455 (0.5); 2.6703 (0.5); 2.5241 (1.3); 2.5194 (1.7); 2.5107 (26.6); 2.5061 (58.5); 2.5015 (82.1); 2.4969 (56.8); 2.4924 (25.0); 2.3286 (0.5); 1.9886 (6.7); 1.2355 (1.4); 1.1923 (2.0); 1.1745 (3.9); 1.1568 (1.8); 0.0080 (1.3); 0.0002 (50.4); 0.0051 (0.8); 0.0059 (0.6); 0.0067 (0.6); 0.0085 (1.5) I-120: .sup.1H-NMR(400.6 MHz, CDCl3): = 9.2075 (1.2); 8.2087 (1.6); 8.2067 (1.3); 8.2045 (1.3); 8.2024 (1.7); 8.0973 (1.0); 8.0953 (1.1); 8.0927 (1.2); 8.0906 (1.0); 8.0852 (1.1); 8.0832 (1.1); 8.0805 (1.1); 8.0785 (1.0); 7.8592 (0.9); 7.8530 (0.9); 7.8404 (1.1); 7.8381 (1.1); 7.8342 (1.0); 7.8318 (1.0); 7.8193 (1.0); 7.8160 (1.0); 7.8130 (1.1); 7.8114 (1.0); 7.7975 (1.0); 7.7954 (1.3); 7.7928 (1.0); 7.7907 (1.2); 7.7769 (1.2); 7.7722 (1.2); 7.6945 (1.3); 7.6923 (2.3); 7.6900 (1.3); 7.6739 (1.0); 7.6717 (1.6); 7.6694 (0.9); 7.2617 (18.1); 7.1651 (1.2); 7.1625 (1.2); 7.1529 (1.1); 7.1504 (1.2); 7.1467 (1.2); 7.1441 (1.1); 7.1345 (1.1); 7.1319 (1.0); 7.0147 (1.2); 7.0132 (1.2); 7.0073 (1.2); 7.0058 (1.1); 6.9936 (1.1); 6.9920 (1.1); 6.9862 (1.2); 6.9847 (1.1); 5.3005 (6.0); 4.9417 (11.9); 4.2445 (1.4); 4.2267 (4.5); 4.2088 (4.6); 4.1910 (1.6); 4.1802 (7.9); 4.1309 (0.6); 4.1131 (0.6); 3.0727 (16.0); 2.0455 (2.8); 1.5653 (1.8); 1.3064 (0.6); 1.3005 (5.8); 1.2827 (12.1); 1.2774 (1.2); 1.2648 (5.8); 1.2595 (2.1); 1.2417 (0.8); 0.0080 (0.8); 0.0002 (29.2); 0.0085 (0.8) I-122: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): = 8.3153 (3.4); 8.3024 (3.5); 8.1155 (1.8); 8.1128 (1.9); 8.1110 (1.8); 8.1033 (1.9); 8.1006 (1.9); 8.0989 (1.8); 8.0130 (1.3); 8.0084 (1.2); 7.9926 (1.9); 7.9881 (1.8); 7.9738 (1.5); 7.9692 (1.4); 7.6986 (3.3); 7.6780 (3.0); 7.3172 (3.0); 7.3149 (3.1); 7.3051 (3.2); 7.3025 (3.1); 7.2985 (1.8); 7.2962 (1.7); 7.2862 (1.5); 7.2840 (1.6); 7.2533 (3.8); 4.9274 (12.7); 3.3292 (16.0); 2.5245 (0.7); 2.5199 (1.0); 2.5110 (17.2); 2.5066 (37.9); 2.5021 (53.1); 2.4975 (38.0); 2.4930 (17.4); 2.0742 (2.6); 1.2344 (0.7) I-123: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.6124 (0.7); 8.6062 (0.6); 8.5847 (3.8); 8.5788 (3.7); 8.3972 (3.8); 8.3926 (3.7); 8.3737 (0.6); 8.3690 (0.6); 8.1031 (1.4); 8.0988 (1.6); 8.0910 (1.4); 8.0877 (2.1); 8.0843 (1.2); 7.8538 (0.6); 7.8333 (0.8); 7.8289 (0.6); 7.8127 (2.2); 7.8083 (2.3); 7.8006 (2.7); 7.7975 (4.1); 7.7952 (3.7); 7.7930 (4.4); 7.7776 (0.9); 7.7719 (0.7); 7.7666 (0.5); 7.7490 (2.7); 7.7438 (3.8); 7.7385 (2.4); 7.2616 (45.4); 7.1818 (1.4); 7.1762 (1.3); 7.1696 (1.4); 7.1663 (1.4); 7.1636 (1.4); 7.1607 (1.4); 7.1547 (1.2); 7.1485 (1.2); 4.2681 (2.0); 4.2502 (6.2); 4.2324 (6.3); 4.2145 (2.1); 3.9438 (16.0); 1.6012 (0.9); 1.5160 (1.3); 1.4928 (0.8); 1.3029 (7.0); 1.2851 (14.1); 1.2672 (6.9); 0.0080 (1.0); 0.0002 (28.8); 0.0085 (1.3) I-124: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5780 (5.7); 8.5722 (5.7); 8.3895 (5.4); 8.3849 (5.6); 8.1785 (1.9); 8.1764 (2.1); 8.1739 (2.3); 8.1718 (2.1); 8.1664 (2.1); 8.1642 (2.2); 8.1618 (2.3); 8.1596 (2.1); 7.8614 (1.7); 7.8567 (1.7); 7.8433 (1.7); 7.8409 (3.2); 7.8388 (1.9); 7.8363 (3.2); 7.8228 (3.5); 7.8182 (3.6); 7.8068 (16.0); 7.7943 (3.4); 7.7917 (5.1); 7.7891 (3.7); 7.7738 (1.7); 7.7713 (2.3); 7.7686 (1.6); 7.7619 (5.0); 7.7571 (5.6); 7.7562 (5.9); 7.7514 (5.0); 7.2634 (11.6); 7.2335 (0.5); 7.2307 (3.1); 7.2277 (3.0); 7.2186 (2.6); 7.2155 (2.7); 7.2126 (2.8); 7.2095 (2.7); 7.2005 (2.4); 7.1974 (2.3); 5.2990 (10.0); 4.8158 (0.6); 4.5075 (0.6); 4.4897 (0.6); 4.4572 (0.6); 4.4393 (0.6); 4.2500 (0.5); 4.2457 (0.6); 4.2319 (0.5); 4.2278 (1.7); 4.2159 (0.5); 4.2100 (1.8); 4.1981 (0.5); 4.1921 (0.6); 3.9441 (0.9); 3.6124 (0.6); 3.6040 (0.6); 3.5829 (3.5); 1.6631 (1.2); 1.5532 (4.0); 1.5514 (4.0); 1.5261 (0.7); 1.4527 (0.8); 1.4511 (1.0); 1.4349 (1.4); 1.4170 (0.7); 1.4059 (0.7); 1.3881 (1.6); 1.3702 (1.0); 1.3423 (0.6); 1.3245 (1.2); 1.3195 (1.6); 1.3174 (0.8); 1.3148 (0.8); 1.3066 (0.8); 1.3017 (3.5); 1.2996 (1.7); 1.2970 (1.4); 1.2872 (0.9); 1.2840 (2.2); 1.2818 (1.0); 1.2792 (0.8); 1.2694 (0.6); 1.2668 (0.8); 1.2540 (1.4); 0.0002 (16.3) I-125: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 8.6638 (3.2); 8.6567 (3.2); 8.4120 (1.6); 8.4085 (2.9); 8.4078 (3.1); 8.4043 (1.6); 8.1420 (1.2); 8.1400 (1.3); 8.1374 (1.6); 8.1353 (1.4); 8.1299 (1.3); 8.1278 (1.6); 8.1253 (1.5); 8.1232 (1.4); 8.0530 (1.2); 8.0484 (1.2); 8.0344 (1.4); 8.0325 (1.5); 8.0298 (1.3); 8.0278 (1.5); 8.0139 (1.6); 8.0092 (1.4); 7.8793 (1.2); 7.8750 (1.3); 7.8723 (1.3); 7.8680 (1.2); 7.8552 (1.3); 7.8509 (1.4); 7.8482 (1.2); 7.8440 (1.2); 7.7843 (1.5); 7.7820 (2.8); 7.7797 (1.6); 7.7637 (1.3); 7.7615 (2.5); 7.7591 (1.4); 7.3589 (1.4); 7.3564 (1.5); 7.3468 (1.3); 7.3443 (1.4); 7.3403 (1.4); 7.3378 (1.3); 7.3282 (1.4); 7.3257 (1.4); 4.1727 (1.8); 4.1550 (6.2); 4.1372 (6.3); 4.1195 (1.9); 4.0828 (11.0); 3.3234 (122.3); 2.5244 (1.1); 2.5197 (1.5); 2.5109 (20.7); 2.5063 (46.0); 2.5017 (65.0); 2.4972 (45.4); 2.4926 (20.5); 1.5915 (1.0); 1.2011 (7.2); 1.1834 (16.0); 1.1657 (7.1); 0.0080 (1.2); 0.0030 (0.8); 0.0023 (1.5); 0.0002 (44.9); 0.0027 (2.4); 0.0034 (1.7); 0.0043 (1.1); 0.0051 (0.9); 0.0059 (0.8); 0.0067 (0.6); 0.0085 (1.5) I-126: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.6098 (3.6); 8.6040 (3.7); 8.4036 (3.6); 8.3990 (3.7); 8.1282 (1.4); 8.1255 (1.5); 8.1180 (1.4); 8.1161 (1.5); 8.1134 (1.5); 7.8357 (1.0); 7.8310 (1.0); 7.8170 (1.4); 7.8151 (1.7); 7.8125 (1.4); 7.8104 (1.6); 7.7967 (1.7); 7.7920 (1.7); 7.7548 (2.9); 7.7498 (4.0); 7.7443 (2.8); 7.7239 (3.1); 7.7219 (1.9); 7.7034 (2.1); 7.2613 (65.4); 7.2064 (1.3); 7.2039 (1.3); 7.1943 (1.3); 7.1917 (1.4); 7.1880 (1.4); 7.1855 (1.3); 7.1758 (1.3); 7.1733 (1.2); 5.3003 (1.6); 3.9602 (16.0); 2.1038 (12.7); 1.2595 (0.6); 1.2556 (0.6); 0.0079 (1.2); 0.0002 (48.8); 0.0085 (1.6) I-19: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2083 (1.0); 8.2062 (0.8); 8.2043 (0.8); 8.2022 (1.1); 8.2002 (0.8); 8.0601 (0.7); 8.0580 (0.7); 8.0553 (0.8); 8.0533 (0.7); 8.0479 (0.7); 8.0458 (0.8); 8.0432 (0.7); 8.0411 (0.7); 7.8628 (0.6); 7.8567 (0.6); 7.8439 (0.7); 7.8417 (0.8); 7.8378 (0.7); 7.8355 (0.7); 7.8228 (0.7); 7.8166 (0.6); 7.7692 (0.6); 7.7645 (0.6); 7.7508 (0.7); 7.7486 (0.9); 7.7461 (0.7); 7.7438 (0.8); 7.7302 (0.8); 7.7254 (0.8); 7.6275 (0.9); 7.6252 (1.6); 7.6228 (1.0); 7.6068 (0.7); 7.6045 (1.2); 7.6022 (0.7); 7.2606 (22.4); 7.1083 (0.8); 7.1058 (0.8); 7.0962 (0.8); 7.0936 (0.8); 7.0900 (0.8); 7.0874 (0.7); 7.0778 (0.8); 7.0752 (0.7); 6.9955 (0.8); 6.9939 (0.8); 6.9881 (0.8); 6.9865 (0.8); 6.9743 (0.8); 6.9727 (0.8); 6.9669 (0.8); 6.9654 (0.8); 5.2765 (1.5); 5.2591 (1.5); 3.8013 (16.0); 3.7263 (0.8); 3.7238 (0.7); 1.7211 (6.1); 1.7037 (6.0); 1.5462 (6.7); 1.2648 (0.6); 1.2596 (0.6); 0.8820 (1.4); 0.8643 (0.5); 0.0080 (0.9); 0.0002 (30.8); 0.0085 (0.8) I-20: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): = 8.6435 (2.7); 8.6360 (0.8); 8.4120 (0.7); 8.3999 (0.8); 8.2493 (3.0); 8.2431 (3.3); 8.0967 (2.5); 8.0844 (2.4); 8.0166 (1.1); 8.0105 (1.2); 7.9964 (1.8); 7.9899 (2.0); 7.9743 (2.5); 7.9695 (2.9); 7.9537 (3.0); 7.9349 (2.2); 7.9302 (2.1); 7.6619 (4.0); 7.6411 (3.8); 7.6169 (0.9); 7.4066 (0.5); 7.3000 (2.5); 7.2935 (2.8); 7.2778 (4.1); 7.2634 (2.2); 7.2591 (2.0); 7.2448 (1.9); 6.3103 (0.5); 5.7568 (16.0); 5.1154 (0.7); 5.0981 (2.5); 5.0807 (2.8); 5.0641 (1.5); 5.0461 (0.8); 4.0379 (1.0); 4.0202 (1.0); 3.3894 (3.8); 3.3388 (6.7); 2.6714 (1.0); 2.5415 (3.2); 2.5247 (2.1); 2.5112 (51.6); 2.5067 (112.5); 2.5021 (157.4); 2.4975 (111.9); 2.4931 (50.8); 2.3332 (0.7); 2.3289 (0.9); 2.1174 (0.6); 1.9888 (4.3); 1.9063 (1.1); 1.5668 (9.4); 1.5494 (9.8); 1.5257 (3.2); 1.3380 (1.5); 1.2977 (0.8); 1.2816 (0.6); 1.2585 (0.9); 1.2348 (5.4); 1.1924 (1.2); 1.1746 (2.3); 1.1567 (1.2); 1.1403 (1.4); 0.8722 (0.6); 0.8537 (1.0); 0.0080 (2.8); 0.0002 (95.8); 0.0085 (3.0) I-21: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 8.6673 (2.8); 8.4204 (0.7); 8.4107 (0.7); 8.4084 (0.7); 8.3131 (5.6); 8.3002 (5.8); 8.1181 (2.9); 8.1161 (3.2); 8.1135 (3.6); 8.1115 (3.2); 8.1060 (3.2); 8.1040 (3.5); 8.1014 (3.5); 8.0994 (3.1); 8.0111 (2.5); 8.0064 (2.3); 7.9925 (3.5); 7.9905 (3.7); 7.9880 (3.5); 7.9859 (3.2); 7.9720 (3.2); 7.9673 (3.2); 7.9496 (0.7); 7.9451 (0.6); 7.6732 (6.0); 7.6548 (3.8); 7.6527 (5.4); 7.6388 (1.4); 7.6181 (1.1); 7.4282 (0.6); 7.4228 (0.7); 7.4119 (0.7); 7.4063 (1.0); 7.3997 (0.8); 7.3889 (0.7); 7.3834 (0.8); 7.3548 (0.8); 7.3479 (0.7); 7.3385 (0.9); 7.3136 (6.3); 7.3012 (6.5); 7.2993 (6.6); 7.2954 (5.3); 7.2830 (3.2); 7.2806 (2.9); 7.2438 (5.5); 6.3099 (1.0); 6.2869 (1.0); 6.1606 (0.5); 6.1577 (0.5); 6.1444 (1.0); 6.1416 (0.9); 5.7569 (12.6); 5.1530 (1.1); 5.1358 (3.8); 5.1184 (4.0); 5.0995 (1.6); 5.0816 (0.9); 4.0557 (0.8); 4.0378 (2.5); 4.0200 (2.5); 4.0022 (0.9); 3.3889 (2.1); 3.3268 (7.8); 2.6754 (0.9); 2.6708 (1.3); 2.6661 (0.9); 2.5412 (1.4); 2.5346 (1.6); 2.5301 (2.4); 2.5246 (4.6); 2.5197 (6.4); 2.5110 (71.1); 2.5065 (148.2); 2.5019 (202.3); 2.4973 (146.2); 2.4928 (72.4); 2.4720 (5.0); 2.4673 (4.4); 2.3335 (1.3); 2.3290 (1.6); 2.3245 (1.3); 2.1172 (1.5); 1.9888 (11.1); 1.9079 (2.2); 1.7542 (0.5); 1.5867 (15.4); 1.5693 (16.0); 1.5641 (6.1); 1.5465 (3.8); 1.5201 (0.7); 1.4509 (0.6); 1.2983 (1.3); 1.2585 (2.1); 1.2355 (6.4); 1.1923 (3.6); 1.1745 (6.7); 1.1567 (3.4); 1.1404 (4.1); 1.1067 (1.6); 1.0573 (1.2); 1.0419 (1.2); 1.0223 (0.8); 1.0133 (0.7); 1.0066 (0.9); 0.9997 (0.6); 0.8884 (0.7); 0.8726 (1.3); 0.8537 (1.5); 0.8363 (0.7); 0.1457 (0.5); 0.0279 (1.3); 0.0080 (5.6); 0.0002 (170.9); 0.0085 (8.4); 0.0344 (1.1); 0.0377 (1.0); 0.1494 (0.7) I-22: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): = 9.2496 (7.1); 8.8883 (13.9); 8.6788 (2.0); 8.0732 (1.5); 8.0610 (1.5); 8.0130 (1.1); 8.0084 (1.0); 7.9923 (1.8); 7.9738 (1.5); 7.9691 (1.2); 7.7084 (2.9); 7.6877 (2.6); 7.6393 (1.0); 7.6184 (0.9); 7.3226 (0.7); 7.3055 (0.7); 7.2939 (1.8); 7.2793 (1.5); 7.2753 (1.4); 7.2608 (1.4); 5.7568 (5.4); 5.1972 (0.7); 5.1797 (2.3); 5.1622 (2.2); 5.1451 (0.6); 5.1159 (0.6); 5.0986 (0.8); 3.3203 (16.0); 2.6702 (1.0); 2.5239 (2.8); 2.5192 (4.0); 2.5104 (53.4); 2.5059 (115.4); 2.5013 (161.0); 2.4968 (114.4); 2.4923 (52.1); 2.3328 (0.9); 2.3284 (1.2); 2.1168 (0.7); 1.6108 (7.8); 1.5935 (7.6); 1.5741 (2.4); 1.5566 (2.4); 1.5279 (0.6); 1.4686 (0.8); 1.4513 (1.5); 1.2983 (1.6); 1.2583 (2.4); 1.2346 (7.0); 1.1404 (1.9); 1.1068 (1.1); 1.0571 (0.9); 1.0418 (0.9); 1.0135 (2.6); 0.9998 (0.8); 0.8888 (0.5); 0.8720 (1.0); 0.8615 (0.9); 0.8535 (1.4); 0.8363 (0.7); 0.1460 (0.6); 0.0080 (4.0); 0.0002 (142.7); 0.0085 (4.7); 0.1496 (0.6) I-23: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3881 (2.3); 8.3841 (2.4); 8.3764 (2.4); 8.3724 (2.4); 8.1389 (2.2); 8.1327 (2.4); 7.8626 (1.1); 7.8564 (1.0); 7.8438 (1.2); 7.8414 (1.3); 7.8376 (1.2); 7.8352 (1.3); 7.8227 (1.2); 7.8164 (1.1); 7.8012 (2.4); 7.7972 (2.4); 7.7811 (2.6); 7.7771 (2.6); 7.3335 (2.5); 7.3219 (2.5); 7.3135 (2.4); 7.3018 (2.3); 7.2617 (11.3); 6.9351 (1.5); 6.9280 (1.6); 6.9138 (1.5); 6.9067 (1.5); 4.9187 (16.0); 4.2820 (1.9); 4.2642 (6.0); 4.2464 (6.1); 4.2286 (2.0); 2.0453 (1.3); 1.5616 (5.4); 1.3002 (7.2); 1.2824 (14.6); 1.2646 (7.6); 1.2599 (1.5); 0.8821 (1.3); 0.8644 (0.5); 0.0002 (16.8); 0.0085 (0.6) I-24: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3500 (1.3); 8.3460 (1.4); 8.3384 (1.4); 8.3343 (1.4); 8.1353 (1.0); 8.1332 (0.8); 8.1311 (0.9); 8.1291 (1.1); 7.8576 (0.6); 7.8513 (0.6); 7.8388 (0.7); 7.8364 (0.7); 7.8325 (0.7); 7.8301 (0.7); 7.8176 (0.6); 7.8114 (0.6); 7.8028 (1.4); 7.7988 (1.4); 7.7827 (1.5); 7.7787 (1.5); 7.3170 (1.5); 7.3053 (1.5); 7.2969 (1.4); 7.2852 (1.4); 7.2619 (7.1); 6.9300 (0.7); 6.9286 (0.8); 6.9226 (0.8); 6.9211 (0.8); 6.9088 (0.8); 6.9073 (0.8); 6.9013 (0.8); 6.8998 (0.7); 5.2593 (1.5); 5.2419 (1.5); 4.1309 (0.6); 4.1130 (0.6); 3.7563 (16.0); 2.0453 (2.8); 1.6961 (6.3); 1.6787 (6.3); 1.5609 (3.4); 1.2773 (1.0); 1.2645 (0.8); 1.2595 (2.1); 1.2416 (0.9); 0.8818 (1.5); 0.8641 (0.6); 0.0002 (11.2) I-25: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3707 (3.6); 8.3667 (3.8); 8.3590 (3.8); 8.3550 (3.8); 8.1350 (3.4); 8.1287 (3.5); 7.8620 (1.7); 7.8557 (1.6); 7.8433 (2.0); 7.8408 (2.1); 7.8371 (2.0); 7.8346 (1.9); 7.8221 (1.8); 7.8158 (1.8); 7.8111 (3.8); 7.8071 (3.8); 7.7910 (4.1); 7.7870 (4.0); 7.3331 (4.0); 7.3214 (4.0); 7.3130 (3.8); 7.3012 (3.6); 7.2606 (50.9); 6.9398 (2.3); 6.9325 (2.4); 6.9186 (2.2); 6.9112 (2.2); 5.3337 (1.2); 5.3162 (4.6); 5.2988 (4.7); 5.2814 (1.3); 1.7459 (16.0); 1.7284 (15.9); 1.2644 (2.1); 0.8990 (1.1); 0.8821 (3.8); 0.8644 (1.5); 0.0080 (2.4); 0.0002 (81.0); 0.0086 (2.8) I-26: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3888 (3.3); 8.3872 (3.5); 8.3849 (3.6); 8.3771 (3.5); 8.3756 (3.7); 8.3732 (3.6); 8.1350 (4.4); 8.1291 (4.6); 7.8596 (1.8); 7.8534 (1.8); 7.8387 (2.6); 7.8327 (2.5); 7.8197 (2.0); 7.8135 (2.0); 7.8030 (4.1); 7.7990 (4.3); 7.7830 (4.6); 7.7790 (4.6); 7.3362 (4.0); 7.3245 (4.0); 7.3161 (3.9); 7.3044 (3.9); 7.2668 (73.3); 6.9349 (3.2); 6.9275 (3.3); 6.9137 (3.2); 6.9063 (3.2); 5.3020 (1.2); 4.9259 (16.0); 4.9220 (14.5); 4.0916 (0.8); 4.0876 (0.8); 2.5953 (1.2); 2.0982 (1.2); 1.2637 (2.1); 0.8983 (1.0); 0.8819 (2.9); 0.8641 (1.3); 0.0079 (2.0); 0.0002 (84.1); 0.0084 (4.0); 0.0266 (0.8) I-27: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3542 (2.5); 8.3502 (2.7); 8.3425 (2.7); 8.3385 (2.8); 8.1323 (2.4); 8.1261 (2.6); 7.8582 (1.2); 7.8520 (1.2); 7.8394 (1.4); 7.8371 (1.5); 7.8332 (1.4); 7.8309 (1.5); 7.8183 (1.3); 7.8120 (1.3); 7.7986 (2.6); 7.7946 (2.7); 7.7786 (2.9); 7.7745 (2.9); 7.3154 (2.8); 7.3038 (2.8); 7.2954 (2.7); 7.2837 (2.6); 7.2613 (17.2); 6.9288 (1.8); 6.9215 (1.8); 6.9076 (1.7); 6.9003 (1.7); 5.3002 (1.7); 5.2577 (0.9); 5.2403 (3.3); 5.2230 (3.4); 5.2056 (1.0); 4.2408 (1.8); 4.2230 (5.9); 4.2052 (6.2); 4.1875 (2.1); 2.1730 (1.1); 1.6909 (13.0); 1.6735 (13.0); 1.2677 (7.8); 1.2499 (16.0); 1.2321 (7.8); 0.0079 (0.8); 0.0002 (26.7); 0.0084 (1.2) I-28: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3882 (1.4); 8.3842 (1.5); 8.3765 (1.5); 8.3725 (1.5); 8.1409 (1.3); 8.1390 (1.0); 8.1367 (1.0); 8.1346 (1.3); 7.8628 (0.6); 7.8565 (0.6); 7.8441 (0.7); 7.8416 (0.8); 7.8378 (0.7); 7.8353 (0.8); 7.8229 (0.7); 7.8166 (0.7); 7.8043 (1.5); 7.8003 (1.5); 7.7842 (1.7); 7.7802 (1.6); 7.3365 (1.6); 7.3248 (1.6); 7.3164 (1.5); 7.3047 (1.5); 7.2618 (9.0); 6.9370 (0.8); 6.9358 (0.9); 6.9297 (0.8); 6.9283 (0.9); 6.9159 (0.8); 6.9145 (0.8); 6.9084 (0.8); 6.9070 (0.8); 4.9368 (8.7); 3.7924 (16.0); 1.5637 (6.8); 0.0002 (12.8) I-29: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2558 (0.6); 8.2541 (0.7); 8.2522 (0.7); 8.2505 (0.6); 8.2442 (0.6); 8.2424 (0.7); 8.2406 (0.7); 8.2389 (0.7); 8.1338 (0.9); 8.1318 (0.7); 8.1296 (0.8); 8.1276 (1.0); 7.8457 (0.6); 7.8432 (0.6); 7.8395 (0.6); 7.8370 (0.6); 7.8245 (0.6); 7.8183 (0.5); 7.5051 (0.5); 7.4881 (0.7); 7.4845 (0.8); 7.4820 (0.6); 7.4650 (0.7); 7.4613 (0.7); 7.3557 (0.6); 7.3467 (0.7); 7.3441 (0.7); 7.3351 (1.1); 7.3260 (0.5); 7.3234 (0.6); 7.2612 (21.3); 6.9646 (0.6); 6.9631 (0.7); 6.9571 (0.7); 6.9556 (0.7); 6.9434 (0.6); 6.9418 (0.7); 6.9359 (0.6); 6.9344 (0.6); 4.9905 (6.9); 4.3640 (1.6); 4.3556 (0.9); 4.3523 (1.7); 4.3486 (0.9); 4.3404 (1.8); 3.6273 (2.0); 3.6190 (0.9); 3.6154 (1.8); 3.6121 (1.0); 3.6037 (1.9); 3.3659 (16.0); 1.5532 (10.3); 0.0079 (0.6); 0.0002 (24.7); 0.0085 (0.9) I-30: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2583 (1.2); 8.2564 (1.3); 8.2466 (1.3); 8.2448 (1.3); 8.1494 (1.7); 8.1431 (1.8); 7.8692 (0.9); 7.8629 (0.9); 7.8505 (1.0); 7.8480 (1.1); 7.8443 (1.0); 7.8418 (1.1); 7.8293 (1.0); 7.8231 (1.0); 7.5260 (0.9); 7.5223 (0.9); 7.5190 (0.6); 7.5053 (1.2); 7.5019 (1.5); 7.4993 (1.0); 7.4823 (1.2); 7.4785 (1.2); 7.3724 (1.2); 7.3633 (1.3); 7.3608 (1.2); 7.3517 (2.0); 7.3426 (0.9); 7.3401 (0.9); 7.3310 (0.9); 7.2606 (84.6); 6.9705 (1.2); 6.9644 (1.2); 6.9492 (1.2); 6.9431 (1.2); 5.0371 (13.7); 4.8404 (16.0); 1.5427 (8.1); 0.0081 (2.8); 0.0002 (97.2); 0.0085 (3.3) I-31: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2951 (1.6); 8.2934 (1.9); 8.2915 (1.9); 8.2898 (1.8); 8.2835 (1.8); 8.2818 (2.0); 8.2799 (2.0); 8.2782 (1.8); 8.1602 (2.5); 8.1582 (1.9); 8.1559 (2.0); 8.1539 (2.7); 7.8498 (1.4); 7.8435 (1.4); 7.8312 (1.5); 7.8286 (1.7); 7.8249 (1.6); 7.8224 (1.6); 7.8100 (1.5); 7.8037 (1.5); 7.5386 (1.3); 7.5349 (1.4); 7.5179 (1.9); 7.5156 (1.9); 7.5143 (2.1); 7.5121 (1.6); 7.4950 (1.8); 7.4913 (1.8); 7.3980 (1.8); 7.3888 (2.0); 7.3864 (1.9); 7.3773 (3.2); 7.3681 (1.4); 7.3657 (1.5); 7.3566 (1.3); 7.2627 (20.5); 6.9737 (1.8); 6.9723 (1.8); 6.9663 (1.9); 6.9648 (1.8); 6.9526 (1.7); 6.9510 (1.8); 6.9451 (1.8); 6.9436 (1.8); 6.6525 (0.6); 5.9488 (0.6); 5.9350 (1.3); 5.9230 (0.8); 5.9214 (0.7); 5.9093 (1.4); 5.9060 (0.8); 5.8956 (0.7); 5.8922 (1.6); 5.8801 (0.9); 5.8786 (0.9); 5.8665 (1.6); 5.8528 (0.8); 5.2850 (0.8); 5.2808 (2.0); 5.2776 (2.2); 5.2734 (1.0); 5.2422 (0.7); 5.2379 (1.8); 5.2347 (1.9); 5.2305 (0.9); 5.1997 (0.9); 5.1961 (2.3); 5.1928 (2.3); 5.1893 (0.9); 5.1740 (0.8); 5.1704 (2.2); 5.1671 (2.2); 5.1636 (0.9); 4.8925 (16.0); 4.0378 (1.1); 4.0338 (2.1); 4.0299 (1.3); 4.0233 (2.2); 4.0196 (3.8); 4.0158 (2.3); 4.0093 (1.4); 4.0053 (2.2); 4.0013 (1.3); 2.0454 (0.7); 1.5810 (5.4); 1.2595 (0.7); 1.2558 (0.5); 0.0002 (19.4); 0.0085 (0.7) I-32: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2221 (1.4); 8.2204 (1.6); 8.2185 (1.6); 8.2169 (1.5); 8.2105 (1.5); 8.2087 (1.7); 8.2069 (1.6); 8.2053 (1.4); 8.1253 (2.2); 8.1233 (1.7); 8.1191 (2.2); 7.8566 (1.2); 7.8504 (1.1); 7.8379 (1.3); 7.8354 (1.4); 7.8317 (1.3); 7.8292 (1.3); 7.8167 (1.2); 7.8105 (1.2); 7.5154 (1.2); 7.5117 (1.2); 7.4947 (1.6); 7.4914 (2.0); 7.4884 (1.3); 7.4715 (1.5); 7.4678 (1.4); 7.3408 (1.4); 7.3318 (1.6); 7.3291 (1.5); 7.3201 (2.5); 7.3111 (1.2); 7.3085 (1.2); 7.2996 (1.1); 7.2610 (31.5); 6.9621 (1.5); 6.9607 (1.5); 6.9546 (1.6); 6.9532 (1.5); 6.9409 (1.5); 6.9394 (1.5); 6.9334 (1.5); 6.9320 (1.4); 5.2849 (0.9); 5.2675 (3.2); 5.2501 (3.2); 5.2328 (0.9); 4.2553 (1.3); 4.2386 (4.2); 4.2377 (4.2); 4.2206 (4.4); 4.2027 (1.5); 1.6951 (12.4); 1.6777 (12.4); 1.5489 (11.6); 1.2730 (7.7); 1.2552 (16.0); 1.2374 (7.5); 0.0080 (1.3); 0.0002 (47.7); 0.0085 (1.4) I-33: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.2157 (1.3); 8.2139 (1.3); 8.2040 (1.3); 8.2023 (1.3); 8.1334 (1.7); 8.1272 (1.8); 7.8631 (0.8); 7.8569 (0.8); 7.8443 (1.0); 7.8419 (1.0); 7.8381 (1.0); 7.8357 (1.0); 7.8231 (0.9); 7.8168 (0.8); 7.5072 (0.8); 7.5035 (0.8); 7.4865 (1.1); 7.4831 (1.4); 7.4803 (1.0); 7.4633 (1.0); 7.4596 (1.0); 7.3355 (1.0); 7.3265 (1.2); 7.3239 (1.1); 7.3149 (1.8); 7.3058 (0.9); 7.3032 (0.9); 7.2942 (0.8); 7.2615 (20.5); 6.9557 (1.2); 6.9495 (1.2); 6.9344 (1.1); 6.9283 (1.1); 5.2825 (0.6); 5.2651 (2.3); 5.2477 (2.3); 5.2303 (0.6); 4.2531 (1.0); 4.2369 (2.9); 4.2354 (3.0); 4.2190 (3.1); 4.2176 (3.0); 4.2011 (1.1); 2.0453 (0.6); 1.6936 (8.8); 1.6762 (8.7); 1.5569 (16.0); 1.2719 (5.6); 1.2594 (1.2); 1.2541 (11.3); 1.2363 (5.3); 0.8819 (1.1); 0.0079 (0.6); 0.0002 (20.9); 0.0085 (0.6) I-34: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2178 (0.5); 8.2160 (0.6); 8.2141 (0.7); 8.2061 (0.6); 8.2043 (0.7); 8.2025 (0.7); 8.2008 (0.7); 8.1303 (0.8); 8.1240 (0.9); 7.8394 (0.5); 7.8369 (0.6); 7.8332 (0.6); 7.8308 (0.6); 7.8120 (0.5); 7.5048 (0.5); 7.4878 (0.6); 7.4843 (0.8); 7.4816 (0.6); 7.4646 (0.6); 7.4609 (0.6); 7.3389 (0.6); 7.3299 (0.7); 7.3273 (0.6); 7.3183 (1.1); 7.3092 (0.5); 7.3067 (0.5); 7.2603 (61.6); 6.9554 (0.6); 6.9496 (0.6); 6.9480 (0.6); 6.9358 (0.6); 6.9343 (0.6); 6.9284 (0.6); 6.9268 (0.6); 5.3051 (1.3); 5.2877 (1.3); 4.3625 (0.5); 4.3511 (0.8); 4.3490 (0.7); 4.3374 (0.6); 4.3325 (0.6); 4.3214 (0.7); 4.3193 (0.8); 4.3083 (0.6); 3.7113 (0.8); 3.7077 (0.8); 3.7005 (0.9); 3.6963 (1.2); 3.6942 (1.1); 3.6866 (0.7); 3.6830 (0.8); 3.6120 (0.8); 3.6077 (0.8); 3.6013 (1.8); 3.5967 (1.0); 3.5939 (1.3); 3.5879 (1.3); 3.5857 (1.4); 3.5109 (2.0); 3.5054 (0.5); 3.5022 (0.9); 3.4982 (1.8); 3.4876 (1.0); 3.3605 (16.0); 3.3156 (0.6); 1.7081 (4.8); 1.6907 (4.8); 1.6255 (0.6); 0.0079 (2.5); 0.0002 (95.6); 0.0085 (2.9) I-35: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2149 (0.6); 8.2130 (0.7); 8.2112 (0.7); 8.2095 (0.7); 8.2032 (0.6); 8.2015 (0.7); 8.1996 (0.7); 8.1979 (0.7); 8.1293 (0.9); 8.1231 (1.0); 7.8593 (0.5); 7.8406 (0.6); 7.8381 (0.6); 7.8343 (0.6); 7.8319 (0.6); 7.8194 (0.5); 7.8131 (0.5); 7.5075 (0.5); 7.5038 (0.5); 7.4869 (0.7); 7.4834 (0.9); 7.4806 (0.6); 7.4636 (0.6); 7.4599 (0.6); 7.3355 (0.7); 7.3266 (0.7); 7.3239 (0.7); 7.3149 (1.2); 7.3059 (0.5); 7.3033 (0.5); 7.2607 (20.0); 6.9575 (0.6); 6.9560 (0.7); 6.9500 (0.7); 6.9486 (0.7); 6.9362 (0.6); 6.9347 (0.7); 6.9288 (0.6); 6.9273 (0.6); 5.3137 (1.4); 5.2963 (1.4); 4.3344 (0.8); 4.3281 (0.9); 4.3247 (0.9); 4.3213 (1.1); 4.3171 (1.1); 4.3138 (1.0); 4.3100 (1.0); 4.3045 (0.9); 3.6013 (1.0); 3.5973 (1.0); 3.5886 (1.7); 3.5860 (1.8); 3.5772 (0.9); 3.5733 (1.0); 3.3304 (16.0); 1.7120 (5.3); 1.6946 (5.2); 1.5480 (12.0); 0.0080 (0.8); 0.0002 (30.1); 0.0085 (0.9) I-36: .sup.1H-NMR(599.6 MHz, CDCl3): = 8.6302 (2.0); 8.2879 (2.2); 8.2811 (2.2); 8.1464 (3.1); 7.8591 (0.9); 7.8452 (1.7); 7.8326 (1.0); 7.5382 (1.0); 7.5230 (2.1); 7.5091 (1.2); 7.4030 (0.9); 7.3962 (1.5); 7.3894 (1.6); 7.3829 (1.2); 7.2602 (32.6); 6.9805 (1.7); 6.9665 (1.7); 4.9133 (10.7); 4.1279 (0.6); 4.1159 (0.6); 2.9962 (33.0); 2.0444 (2.6); 1.5479 (41.5); 1.2710 (1.1); 1.2592 (2.1); 1.2474 (0.9); 0.8933 (0.4); 0.8821 (0.9); 0.8702 (0.4); 0.0001 (50.0) I-37: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.2569 (0.9); 8.2435 (1.0); 8.1350 (1.2); 8.1285 (1.2); 7.8644 (0.5); 7.8580 (0.5); 7.8432 (0.7); 7.8395 (0.7); 7.8244 (0.6); 7.8184 (0.6); 7.5196 (0.6); 7.5095 (0.5); 7.5059 (0.5); 7.4862 (1.0); 7.4657 (0.7); 7.4618 (0.7); 7.3581 (0.8); 7.3487 (0.9); 7.3373 (1.1); 7.3282 (0.6); 7.2606 (108.8); 6.9966 (0.6); 6.9641 (0.8); 6.9565 (0.9); 6.9427 (0.8); 6.9351 (0.8); 4.9798 (7.6); 4.3788 (1.7); 4.3668 (1.9); 4.3546 (1.9); 3.7371 (2.0); 3.7287 (1.2); 3.7250 (2.0); 3.7130 (1.8); 3.6403 (1.4); 3.6293 (1.9); 3.6241 (1.5); 3.6172 (2.6); 3.5369 (2.5); 3.5300 (1.4); 3.5249 (1.9); 3.5137 (1.4); 3.3724 (16.0); 1.5424 (12.2); 0.0080 (1.6); 0.0002 (66.1); 0.0085 (2.1) I-38: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.2633 (1.7); 8.2517 (1.7); 8.1287 (2.3); 8.1225 (2.3); 7.8610 (1.1); 7.8546 (1.1); 7.8422 (1.3); 7.8397 (1.3); 7.8359 (1.3); 7.8335 (1.2); 7.8210 (1.2); 7.8147 (1.1); 7.5198 (0.5); 7.5167 (1.1); 7.5130 (1.1); 7.4959 (1.5); 7.4925 (1.9); 7.4900 (1.2); 7.4728 (1.4); 7.4691 (1.3); 7.3620 (1.3); 7.3529 (1.6); 7.3504 (1.4); 7.3413 (2.3); 7.3322 (1.1); 7.3297 (1.1); 7.3206 (1.0); 7.2610 (70.8); 6.9676 (1.5); 6.9614 (1.5); 6.9476 (1.5); 6.9401 (1.4); 4.9380 (16.0); 4.2936 (1.9); 4.2757 (6.1); 4.2578 (6.2); 4.2400 (2.0); 1.5488 (5.2); 1.3054 (7.3); 1.2875 (15.0); 1.2697 (7.2); 0.0079 (1.2); 0.0002 (42.2); 0.0085 (1.2) I-39: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.2585 (1.8); 8.2567 (1.7); 8.2468 (1.8); 8.2450 (1.7); 8.1373 (2.3); 8.1311 (2.3); 7.8676 (1.1); 7.8613 (1.1); 7.8488 (1.3); 7.8463 (1.4); 7.8426 (1.3); 7.8401 (1.3); 7.8276 (1.2); 7.8214 (1.1); 7.5198 (0.5); 7.5087 (1.1); 7.5049 (1.1); 7.4879 (1.6); 7.4845 (1.8); 7.4649 (1.4); 7.4611 (1.4); 7.3565 (1.4); 7.3474 (1.7); 7.3449 (1.4); 7.3358 (2.4); 7.3268 (1.2); 7.3242 (1.2); 7.3151 (1.0); 7.2609 (90.8); 6.9629 (1.6); 6.9567 (1.6); 6.9430 (1.5); 6.9356 (1.6); 4.9367 (16.0); 4.2909 (2.0); 4.2730 (6.1); 4.2552 (6.2); 4.2373 (2.0); 1.5461 (10.5); 1.3038 (7.5); 1.2859 (15.3); 1.2680 (7.3); 0.0079 (1.6); 0.0002 (53.6); 0.0085 (1.6) I-40: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2292 (1.4); 8.2273 (1.6); 8.2257 (1.7); 8.2238 (1.6); 8.2176 (1.4); 8.2157 (1.7); 8.2140 (1.7); 8.2122 (1.5); 8.1361 (2.3); 8.1299 (2.4); 7.7748 (1.1); 7.7686 (1.1); 7.7557 (1.3); 7.7538 (1.4); 7.7495 (1.3); 7.7476 (1.4); 7.7347 (1.1); 7.7285 (1.1); 7.4624 (1.1); 7.4587 (1.2); 7.4418 (1.4); 7.4383 (2.1); 7.4353 (1.4); 7.4184 (1.4); 7.4147 (1.4); 7.2867 (1.4); 7.2778 (1.6); 7.2751 (1.6); 7.2661 (2.6); 7.2619 (16.9); 7.2573 (1.7); 7.2545 (1.4); 7.2456 (1.0); 6.9180 (1.6); 6.9119 (1.5); 6.9106 (1.6); 6.8969 (1.5); 6.8895 (1.5); 4.8875 (16.0); 4.2745 (2.0); 4.2567 (6.1); 4.2389 (6.2); 4.2210 (2.0); 1.6146 (0.6); 1.5998 (0.8); 1.5948 (1.0); 1.5875 (0.8); 1.5806 (2.4); 1.5729 (1.3); 1.5655 (1.6); 1.5610 (1.6); 1.5464 (0.7); 1.3010 (7.6); 1.2832 (15.3); 1.2653 (7.2); 0.7978 (1.5); 0.7927 (4.1); 0.7902 (3.5); 0.7842 (5.6); 0.7792 (5.1); 0.7752 (2.6); 0.7678 (2.4); 0.7637 (3.7); 0.7609 (1.9); 0.7582 (1.7); 0.0079 (0.8); 0.0002 (24.0); 0.0085 (0.8) I-41: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2220 (0.7); 8.2202 (0.8); 8.2183 (0.8); 8.2166 (0.7); 8.2103 (0.8); 8.2085 (0.8); 8.2067 (0.8); 8.2051 (0.7); 8.1279 (1.1); 8.1258 (0.8); 8.1236 (0.9); 8.1218 (1.1); 7.8570 (0.6); 7.8507 (0.6); 7.8382 (0.7); 7.8357 (0.7); 7.8320 (0.7); 7.8295 (0.7); 7.8170 (0.6); 7.8108 (0.6); 7.5206 (0.7); 7.5169 (0.6); 7.5000 (0.8); 7.4970 (1.0); 7.4936 (0.7); 7.4767 (0.8); 7.4730 (0.7); 7.3441 (0.7); 7.3351 (0.8); 7.3325 (0.8); 7.3234 (1.3); 7.3145 (0.6); 7.3118 (0.6); 7.3028 (0.5); 7.2611 (44.6); 6.9634 (0.8); 6.9619 (0.8); 6.9559 (0.8); 6.9544 (0.8); 6.9421 (0.8); 6.9406 (0.8); 6.9347 (0.8); 6.9331 (0.7); 5.2926 (1.5); 5.2752 (1.5); 3.7708 (16.0); 1.7001 (6.4); 1.6828 (6.4); 1.5547 (1.0); 0.0080 (0.8); 0.0002 (27.8); 0.0085 (0.8) I-42: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2315 (0.7); 8.2296 (0.9); 8.2279 (0.9); 8.2261 (0.8); 8.2198 (0.8); 8.2179 (0.9); 8.2162 (0.9); 8.2144 (0.8); 8.1366 (1.2); 8.1303 (1.2); 7.7747 (0.6); 7.7685 (0.6); 7.7557 (0.7); 7.7536 (0.8); 7.7495 (0.7); 7.7474 (0.8); 7.7346 (0.7); 7.7284 (0.7); 7.5191 (0.6); 7.4641 (0.6); 7.4604 (0.7); 7.4436 (0.8); 7.4401 (1.2); 7.4370 (0.7); 7.4201 (0.8); 7.4164 (0.8); 7.2895 (0.7); 7.2805 (0.9); 7.2778 (0.9); 7.2689 (1.8); 7.2607 (110.2); 7.2509 (0.7); 7.2484 (1.0); 6.9970 (0.6); 6.9201 (0.8); 6.9186 (0.9); 6.9126 (0.9); 6.9111 (0.9); 6.8990 (0.8); 6.8975 (0.8); 6.8915 (0.8); 6.8900 (0.8); 4.9056 (8.5); 3.7858 (16.0); 1.5980 (0.8); 1.5811 (1.2); 1.5639 (1.2); 1.5473 (3.0); 0.7823 (10.1); 0.7652 (6.5); 0.0079 (1.9); 0.0002 (66.1); 0.0085 (2.0) I-43: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2723 (1.8); 8.2623 (1.8); 8.2607 (1.8); 8.1385 (2.7); 8.1324 (2.8); 7.7709 (1.1); 7.7647 (1.1); 7.7519 (1.4); 7.7499 (1.5); 7.7457 (1.4); 7.7437 (1.5); 7.7309 (1.2); 7.7247 (1.2); 7.4642 (1.1); 7.4607 (1.1); 7.4435 (1.6); 7.4404 (2.2); 7.4375 (1.4); 7.4203 (1.4); 7.4168 (1.4); 7.3098 (1.2); 7.3007 (1.5); 7.2984 (1.4); 7.2892 (2.1); 7.2801 (1.1); 7.2778 (1.2); 7.2686 (1.0); 7.2626 (34.1); 6.9256 (1.7); 6.9193 (1.7); 6.9044 (1.7); 6.8982 (1.6); 5.3001 (1.1); 4.9419 (16.0); 1.6072 (0.5); 1.5933 (1.0); 1.5867 (1.1); 1.5809 (0.7); 1.5731 (2.0); 1.5669 (0.8); 1.5590 (1.0); 1.5526 (1.1); 1.5389 (0.6); 1.4320 (1.2); 1.2644 (1.6); 0.8986 (0.9); 0.8817 (3.3); 0.8640 (1.2); 0.7961 (0.6); 0.7808 (1.8); 0.7762 (3.1); 0.7734 (2.1); 0.7697 (2.5); 0.7601 (2.0); 0.7574 (2.2); 0.7532 (4.2); 0.7495 (4.2); 0.7462 (3.1); 0.7386 (3.0); 0.7341 (3.6); 0.7312 (2.2); 0.7282 (2.1); 0.0079 (0.5); 0.0002 (20.9); 0.0085 (0.7) I-44: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2886 (0.9); 8.2869 (1.0); 8.2850 (1.1); 8.2834 (1.0); 8.2770 (1.0); 8.2753 (1.1); 8.2734 (1.1); 8.2718 (1.0); 8.1543 (1.4); 8.1480 (1.5); 7.8684 (0.7); 7.8622 (0.7); 7.8499 (0.8); 7.8472 (0.9); 7.8437 (0.8); 7.8410 (0.9); 7.8287 (0.8); 7.8224 (0.8); 7.5556 (0.7); 7.5519 (0.8); 7.5348 (1.0); 7.5312 (1.2); 7.5290 (0.9); 7.5119 (1.0); 7.5082 (1.0); 7.4147 (1.0); 7.4055 (1.1); 7.4031 (1.0); 7.3940 (1.7); 7.3848 (0.8); 7.3824 (0.8); 7.3732 (0.7); 7.2618 (17.1); 6.9914 (0.9); 6.9900 (1.0); 6.9840 (1.0); 6.9825 (1.0); 6.9702 (0.9); 6.9687 (1.0); 6.9627 (1.0); 6.9613 (1.0); 4.9522 (11.5); 3.3771 (16.0); 3.3705 (0.8); 2.1725 (3.9); 0.8819 (0.7); 0.0080 (0.6); 0.0002 (21.4); 0.0085 (0.7) I-45: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2753 (0.8); 8.2734 (0.8); 8.2637 (0.8); 8.2618 (0.8); 8.1311 (1.1); 8.1249 (1.2); 7.8640 (0.5); 7.8578 (0.5); 7.8452 (0.6); 7.8428 (0.7); 7.8390 (0.6); 7.8366 (0.6); 7.8241 (0.6); 7.8179 (0.6); 7.5011 (0.5); 7.4975 (0.5); 7.4804 (0.8); 7.4773 (0.9); 7.4747 (0.6); 7.4575 (0.7); 7.4538 (0.7); 7.3653 (0.7); 7.3562 (0.8); 7.3538 (0.7); 7.3446 (1.2); 7.3355 (0.6); 7.3331 (0.6); 7.2609 (29.4); 6.9670 (0.8); 6.9604 (0.8); 6.9466 (0.7); 6.9392 (0.7); 5.1198 (8.6); 2.0433 (14.2); 1.9725 (15.2); 1.5477 (16.0); 1.2599 (0.7); 0.0081 (1.0); 0.0002 (34.2); 0.0085 (1.2) I-46: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5752 (1.4); 8.5650 (1.4); 8.5631 (1.4); 8.2657 (1.6); 8.2639 (1.7); 8.2542 (1.7); 8.2523 (1.7); 8.1326 (2.2); 8.1263 (2.4); 7.8629 (1.1); 7.8567 (1.1); 7.8441 (1.3); 7.8418 (1.4); 7.8379 (1.3); 7.8355 (1.3); 7.8230 (1.2); 7.8168 (1.2); 7.6351 (1.0); 7.6306 (1.0); 7.6158 (2.0); 7.6114 (2.0); 7.5966 (1.2); 7.5921 (1.2); 7.5121 (1.0); 7.5084 (1.1); 7.4913 (1.6); 7.4882 (1.8); 7.4854 (1.2); 7.4684 (1.4); 7.4647 (1.4); 7.3682 (1.5); 7.3592 (3.6); 7.3570 (2.7); 7.3475 (2.6); 7.3387 (2.6); 7.3269 (1.1); 7.2609 (39.1); 7.2238 (1.1); 7.2115 (1.1); 7.2049 (1.1); 7.1927 (1.0); 6.9673 (1.6); 6.9599 (1.6); 6.9461 (1.5); 6.9387 (1.6); 5.3574 (11.4); 5.0698 (16.0); 2.1719 (0.9); 1.5601 (2.8); 1.2597 (0.6); 0.8819 (0.9); 0.0078 (1.5); 0.0053 (0.6); 0.0002 (53.1); 0.0085 (1.9) I-47: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2893 (1.8); 8.2875 (1.8); 8.2778 (1.8); 8.2759 (1.8); 8.1551 (2.4); 8.1488 (2.6); 7.8508 (1.1); 7.8446 (1.1); 7.8321 (1.3); 7.8297 (1.4); 7.8259 (1.4); 7.8235 (1.4); 7.8110 (1.2); 7.8048 (1.2); 7.5321 (1.1); 7.5285 (1.1); 7.5113 (1.6); 7.5085 (1.9); 7.4886 (1.5); 7.4849 (1.5); 7.3914 (1.4); 7.3822 (1.6); 7.3798 (1.5); 7.3707 (2.5); 7.3615 (1.2); 7.3591 (1.2); 7.3500 (1.0); 7.2631 (14.3); 7.1166 (0.8); 6.9713 (1.7); 6.9640 (1.8); 6.9502 (1.7); 6.9428 (1.7); 4.8520 (15.0); 4.2002 (2.2); 4.1824 (6.8); 4.1646 (6.9); 4.1468 (2.3); 3.6798 (1.4); 3.6644 (3.8); 3.6492 (4.0); 3.6337 (1.6); 2.6179 (3.4); 2.6025 (5.4); 2.5874 (3.3); 1.5857 (5.6); 1.2918 (7.8); 1.2740 (16.0); 1.2562 (8.0); 0.0080 (0.6); 0.0002 (20.9); 0.0085 (0.8) I-48: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2969 (1.4); 8.2953 (1.6); 8.2934 (1.7); 8.2853 (1.6); 8.2837 (1.8); 8.2818 (1.7); 8.1577 (2.2); 8.1514 (2.4); 7.8583 (1.1); 7.8520 (1.1); 7.8396 (1.3); 7.8371 (1.4); 7.8334 (1.3); 7.8308 (1.3); 7.8184 (1.2); 7.8122 (1.2); 7.5328 (1.0); 7.5291 (1.1); 7.5120 (1.6); 7.5086 (1.8); 7.5064 (1.3); 7.4892 (1.5); 7.4855 (1.4); 7.3936 (1.4); 7.3844 (1.6); 7.3820 (1.5); 7.3729 (2.4); 7.3637 (1.1); 7.3613 (1.2); 7.3522 (1.0); 7.2631 (13.4); 7.1160 (0.8); 6.9741 (1.6); 6.9730 (1.6); 6.9667 (1.6); 6.9530 (1.6); 6.9518 (1.5); 6.9455 (1.6); 4.9173 (13.2); 4.2839 (2.0); 4.2661 (6.3); 4.2482 (6.4); 4.2304 (2.1); 4.1605 (6.3); 4.1474 (6.4); 4.1309 (0.9); 4.1131 (0.8); 2.0454 (3.7); 1.5810 (4.7); 1.3269 (7.8); 1.3091 (16.0); 1.2913 (7.9); 1.2774 (1.3); 1.2596 (2.6); 1.2417 (1.1); 0.8819 (1.2); 0.8642 (0.5); 0.0080 (0.5); 0.0002 (19.8); 0.0085 (0.7) I-49: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3109 (0.7); 8.3091 (0.8); 8.3072 (0.8); 8.3056 (0.7); 8.2992 (0.7); 8.2976 (0.8); 8.2956 (0.8); 8.2941 (0.7); 8.1055 (1.3); 8.1038 (1.3); 8.0994 (1.4); 8.0977 (1.3); 7.5663 (1.3); 7.5602 (1.2); 7.5448 (1.3); 7.5386 (1.3); 7.4810 (0.5); 7.4772 (0.5); 7.4603 (0.8); 7.4581 (0.7); 7.4567 (0.8); 7.4546 (0.6); 7.4376 (0.7); 7.4338 (0.7); 7.3518 (0.7); 7.3427 (0.8); 7.3402 (0.8); 7.3311 (1.2); 7.3220 (0.5); 7.3196 (0.6); 7.2607 (18.0); 6.7239 (1.5); 6.7220 (1.6); 6.7023 (1.5); 6.7005 (1.5); 4.9554 (7.4); 3.9244 (16.0); 3.7958 (13.8); 2.0453 (1.4); 1.5491 (6.9); 1.2597 (1.0); 0.8821 (0.7); 0.0079 (0.8); 0.0002 (27.1); 0.0085 (0.8) I-50: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.9883 (1.4); 8.3151 (0.8); 8.3128 (1.1); 8.3098 (0.9); 8.3035 (0.9); 8.3012 (1.2); 8.2983 (0.9); 8.1041 (1.7); 8.1024 (1.7); 8.0979 (1.8); 8.0962 (1.8); 7.9660 (0.6); 7.9625 (0.7); 7.9451 (0.8); 7.9415 (1.4); 7.9378 (0.8); 7.9205 (0.8); 7.9169 (0.8); 7.6123 (0.8); 7.6028 (1.0); 7.6007 (0.9); 7.5968 (1.7); 7.5909 (2.5); 7.5819 (0.8); 7.5799 (0.8); 7.5752 (1.8); 7.5690 (1.9); 6.8624 (1.9); 6.8606 (1.9); 6.8408 (1.9); 6.8390 (1.9); 5.7571 (0.6); 5.0423 (1.8); 5.0248 (1.9); 3.8484 (16.0); 3.3250 (4.9); 2.5199 (0.6); 2.5112 (8.7); 2.5066 (19.2); 2.5020 (27.1); 2.4975 (19.6); 2.4930 (9.6); 2.4707 (0.6); 2.0859 (1.4); 1.5681 (5.0); 1.5507 (5.0); 0.0080 (0.5); 0.0002 (17.6); 0.0085 (0.7) I-51: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4517 (2.9); 8.4448 (3.0); 8.3015 (1.7); 8.2977 (3.0); 8.2941 (1.7); 8.2482 (1.3); 8.2464 (1.5); 8.2445 (1.6); 8.2429 (1.4); 8.2365 (1.4); 8.2348 (1.6); 8.2329 (1.5); 8.2314 (1.3); 7.5287 (1.3); 7.5243 (2.4); 7.5216 (1.8); 7.5175 (1.3); 7.5065 (1.4); 7.5034 (1.9); 7.4998 (2.9); 7.4974 (1.5); 7.4953 (1.4); 7.4805 (1.4); 7.4768 (1.4); 7.3609 (1.4); 7.3518 (1.5); 7.3493 (1.4); 7.3402 (2.4); 7.3312 (1.1); 7.3286 (1.1); 7.3196 (1.0); 7.2637 (7.8); 5.3004 (1.5); 4.9389 (15.7); 4.2929 (1.9); 4.2751 (6.1); 4.2572 (6.2); 4.2394 (2.0); 1.6008 (1.7); 1.3049 (7.7); 1.2871 (16.0); 1.2693 (7.5); 0.0002 (11.3) I-52: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5510 (1.8); 8.5487 (2.0); 8.5467 (2.0); 8.5444 (1.7); 8.5390 (1.8); 8.5367 (2.1); 8.5345 (2.0); 8.5324 (1.6); 8.2331 (2.3); 8.2313 (2.5); 8.2294 (2.5); 8.2278 (2.1); 8.2214 (2.3); 8.2197 (2.6); 8.2178 (2.5); 8.1223 (3.2); 8.1161 (3.3); 7.8536 (1.6); 7.8473 (1.5); 7.8348 (2.0); 7.8324 (2.0); 7.8286 (1.9); 7.8262 (1.8); 7.8137 (1.6); 7.8074 (1.6); 7.5612 (1.2); 7.5567 (1.2); 7.5419 (2.6); 7.5375 (2.6); 7.5226 (1.7); 7.5185 (1.8); 7.5036 (1.6); 7.4999 (1.6); 7.4829 (2.4); 7.4795 (2.6); 7.4767 (1.8); 7.4598 (2.1); 7.4561 (2.0); 7.3511 (2.0); 7.3421 (2.5); 7.3395 (2.1); 7.3305 (3.8); 7.3216 (3.5); 7.3190 (2.1); 7.3098 (1.8); 7.3045 (2.4); 7.2605 (83.7); 7.1889 (1.5); 7.1756 (1.5); 7.1702 (1.5); 7.1581 (1.4); 6.9607 (2.3); 6.9533 (2.4); 6.9518 (2.1); 6.9395 (2.2); 6.9380 (2.1); 6.9320 (2.2); 6.9305 (1.9); 5.4288 (1.1); 5.4114 (4.3); 5.3940 (4.4); 5.3767 (1.1); 5.3338 (13.9); 1.7655 (16.0); 1.7481 (15.8); 1.5507 (10.8); 0.0079 (3.8); 0.0002 (129.1); 0.0061 (1.9); 0.0085 (3.8) I-53: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.6885 (0.9); 8.2923 (0.8); 8.2907 (0.9); 8.2888 (1.0); 8.2873 (0.9); 8.2808 (0.9); 8.2791 (1.0); 8.2772 (1.0); 8.1466 (1.3); 8.1404 (1.4); 7.8679 (0.6); 7.8616 (0.6); 7.8493 (0.7); 7.8467 (0.8); 7.8431 (0.8); 7.8405 (0.8); 7.8281 (0.7); 7.8218 (0.7); 7.5445 (0.6); 7.5409 (0.6); 7.5237 (1.0); 7.5201 (1.1); 7.5182 (0.8); 7.5010 (0.9); 7.4973 (0.8); 7.4078 (0.8); 7.3987 (1.0); 7.3963 (0.9); 7.3871 (1.4); 7.3779 (0.7); 7.3755 (0.7); 7.3664 (0.6); 7.2613 (15.8); 6.9881 (0.8); 6.9868 (0.9); 6.9806 (0.9); 6.9793 (0.9); 6.9669 (0.8); 6.9655 (0.9); 6.9595 (0.9); 6.9581 (0.9); 4.8859 (9.7); 4.2566 (0.8); 4.2398 (1.2); 4.2230 (0.9); 2.9082 (16.0); 2.0455 (0.6); 1.5543 (8.7); 1.2596 (0.6); 1.1572 (13.6); 1.1404 (13.6); 0.8819 (0.5); 0.0080 (0.7); 0.0002 (24.3); 0.0085 (1.0) I-54: .sup.1H-NMR(400.0 MHz, CDCl3): = 9.1339 (2.0); 8.2860 (2.0); 8.2746 (2.0); 8.1517 (2.7); 8.1460 (2.7); 7.8574 (1.0); 7.8512 (1.0); 7.8362 (1.5); 7.8302 (1.4); 7.8175 (1.1); 7.8112 (1.0); 7.5408 (0.9); 7.5200 (2.3); 7.4967 (1.1); 7.4053 (1.1); 7.3942 (1.6); 7.3846 (2.0); 7.3734 (1.2); 7.3641 (0.8); 7.2612 (74.0); 6.9805 (1.8); 6.9731 (1.8); 6.9592 (1.8); 6.9519 (1.8); 5.3003 (3.1); 4.9221 (13.0); 4.2494 (1.5); 4.2316 (4.7); 4.2138 (4.8); 4.1960 (1.7); 4.1761 (9.3); 4.1311 (0.8); 4.1130 (0.8); 3.0726 (16.0); 2.0451 (3.6); 1.5673 (13.2); 1.3048 (5.6); 1.2869 (11.3); 1.2775 (1.8); 1.2690 (6.4); 1.2596 (4.0); 1.2418 (1.1); 0.8982 (0.6); 0.8818 (1.3); 0.8645 (0.7); 0.0080 (1.2); 0.0002 (39.5); 0.0084 (1.2) I-55: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.2454 (1.1); 8.2356 (1.1); 8.1358 (1.4); 8.1295 (1.5); 7.8564 (0.7); 7.8502 (0.6); 7.8354 (0.9); 7.8314 (0.8); 7.8292 (0.8); 7.8165 (0.7); 7.8102 (0.7); 7.4959 (0.6); 7.4922 (0.6); 7.4752 (0.9); 7.4718 (1.2); 7.4522 (0.9); 7.4484 (0.8); 7.3429 (0.8); 7.3339 (1.0); 7.3314 (0.9); 7.3223 (1.5); 7.3131 (0.7); 7.3106 (0.7); 7.3017 (0.6); 7.2612 (42.3); 6.9602 (1.0); 6.9528 (1.0); 6.9390 (1.0); 6.9315 (0.9); 4.9300 (9.9); 4.2871 (1.2); 4.2692 (3.8); 4.2513 (3.8); 4.2335 (1.2); 1.5513 (16.0); 1.3026 (4.5); 1.2848 (9.2); 1.2669 (4.5); 0.0079 (0.8); 0.0002 (26.3); 0.0086 (0.7) I-56: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2591 (1.4); 8.2572 (1.4); 8.2475 (1.5); 8.2457 (1.5); 8.1173 (1.9); 8.1113 (2.0); 7.8362 (0.7); 7.8300 (0.7); 7.8156 (1.0); 7.8100 (1.0); 7.7965 (0.7); 7.7904 (0.7); 7.5148 (1.0); 7.5111 (1.0); 7.4940 (1.6); 7.4922 (1.5); 7.4903 (1.7); 7.4887 (1.3); 7.4715 (1.5); 7.4678 (1.4); 7.3878 (1.3); 7.3785 (1.5); 7.3763 (1.4); 7.3670 (2.1); 7.3577 (1.0); 7.3555 (1.0); 7.3462 (0.9); 7.2663 (4.6); 6.9493 (1.5); 6.9478 (1.5); 6.9418 (1.6); 6.9404 (1.5); 6.9281 (1.4); 6.9266 (1.4); 6.9207 (1.4); 6.9192 (1.4); 4.9394 (13.9); 4.2846 (2.0); 4.2667 (6.3); 4.2489 (6.3); 4.2311 (2.1); 3.8782 (0.5); 3.0300 (0.5); 2.9983 (0.5); 1.6151 (4.8); 1.3027 (0.7); 1.2975 (7.8); 1.2850 (1.6); 1.2797 (16.0); 1.2671 (0.8); 1.2619 (7.7); 0.0002 (6.3) I-57: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2960 (1.2); 8.2940 (1.2); 8.2845 (1.2); 8.2825 (1.2); 8.1270 (1.6); 8.1209 (1.6); 7.9824 (0.7); 7.9762 (0.7); 7.9639 (0.8); 7.9611 (0.9); 7.9577 (0.8); 7.9550 (0.8); 7.9427 (0.7); 7.9365 (0.7); 7.5492 (0.7); 7.5455 (0.7); 7.5281 (1.3); 7.5245 (1.3); 7.5061 (1.0); 7.5025 (1.0); 7.4495 (1.0); 7.4400 (1.2); 7.4381 (1.1); 7.4286 (1.6); 7.4191 (0.8); 7.4172 (0.8); 7.4078 (0.6); 7.2621 (11.3); 7.0078 (1.1); 7.0068 (1.1); 7.0005 (1.1); 6.9865 (1.0); 6.9854 (1.0); 6.9792 (1.1); 5.0231 (10.7); 4.2976 (1.4); 4.2797 (4.2); 4.2619 (4.3); 4.2441 (1.4); 2.0457 (0.9); 1.5588 (16.0); 1.3018 (5.0); 1.2840 (10.2); 1.2777 (0.6); 1.2661 (5.2); 1.2598 (0.9); 0.8819 (0.5); 0.0079 (0.6); 0.0002 (17.1); 0.0085 (0.6) I-59: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2170 (1.3); 8.2109 (1.4); 8.0929 (0.7); 8.0831 (0.7); 7.8722 (0.6); 7.8661 (0.6); 7.8533 (0.7); 7.8512 (0.8); 7.8471 (0.7); 7.8450 (0.7); 7.8324 (0.7); 7.8262 (0.6); 7.8117 (0.5); 7.8071 (0.5); 7.7930 (0.7); 7.7910 (0.9); 7.7886 (0.8); 7.7865 (0.9); 7.7727 (0.8); 7.7681 (0.8); 7.7016 (1.2); 7.6810 (0.8); 7.2675 (2.8); 7.1558 (0.7); 7.1536 (0.7); 7.1437 (0.7); 7.1414 (0.7); 7.1376 (0.7); 7.1353 (0.6); 7.1254 (0.6); 7.1231 (0.6); 7.0153 (0.9); 7.0082 (0.9); 6.9942 (0.8); 6.9871 (0.9); 4.9144 (7.8); 4.7249 (0.9); 4.7068 (1.3); 4.6887 (0.9); 3.7815 (16.0); 2.0093 (0.8); 1.5140 (6.5); 1.4961 (6.5); 0.0002 (3.4) I-60: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2130 (2.0); 8.2068 (2.2); 8.1268 (1.3); 8.1248 (1.3); 8.1222 (1.5); 8.1146 (1.4); 8.1100 (1.4); 7.8671 (1.0); 7.8609 (1.1); 7.8483 (1.3); 7.8460 (1.3); 7.8421 (1.3); 7.8398 (1.2); 7.8273 (1.1); 7.8222 (1.5); 7.8178 (1.2); 7.8019 (1.5); 7.7991 (1.4); 7.7972 (1.4); 7.7833 (1.5); 7.7786 (1.4); 7.6286 (2.7); 7.6081 (2.2); 7.5188 (0.9); 7.2603 (167.8); 7.1912 (1.4); 7.1887 (1.3); 7.1790 (1.4); 7.1765 (1.3); 7.1727 (1.3); 7.1702 (1.2); 7.1605 (1.3); 7.1580 (1.2); 7.0254 (1.4); 7.0182 (1.4); 7.0044 (1.5); 6.9968 (2.4); 5.0298 (0.7); 4.9840 (16.0); 4.3501 (1.6); 4.3287 (5.1); 4.3073 (5.3); 4.2859 (1.8); 1.6115 (4.3); 1.2538 (0.6); 0.1457 (0.7); 0.0080 (5.1); 0.0002 (208.2); 0.0085 (7.5); 0.0294 (0.6); 0.1494 (0.7) I-61: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2552 (1.8); 8.2422 (1.8); 8.0907 (0.9); 8.0881 (1.0); 8.0806 (0.9); 8.0786 (1.0); 8.0760 (1.0); 7.8361 (0.7); 7.8315 (0.6); 7.8176 (0.9); 7.8155 (1.1); 7.8129 (1.0); 7.8109 (1.0); 7.7971 (1.0); 7.7925 (1.0); 7.7156 (1.9); 7.6950 (1.3); 7.2606 (43.7); 7.1807 (0.9); 7.1781 (0.9); 7.1685 (0.9); 7.1660 (0.9); 7.1623 (1.0); 7.1598 (0.8); 7.1501 (0.9); 7.1475 (0.8); 7.1328 (0.8); 7.1293 (1.2); 7.1251 (0.9); 7.1199 (0.9); 7.1163 (1.2); 7.1122 (0.9); 6.9434 (1.9); 5.3003 (2.5); 4.9419 (8.0); 4.1829 (3.7); 4.1696 (3.7); 3.7948 (16.0); 1.5424 (16.0); 1.2556 (1.2); 0.0079 (2.2); 0.0002 (70.3); 0.0085 (2.7) I-62: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.3088 (1.1); 8.2504 (2.8); 8.2443 (2.9); 8.1007 (1.7); 8.0988 (1.9); 8.0962 (2.0); 8.0941 (1.8); 8.0887 (1.8); 8.0867 (2.1); 8.0840 (2.0); 8.0820 (1.8); 8.0231 (1.2); 8.0169 (1.1); 8.0020 (1.8); 7.9958 (1.7); 7.9824 (1.3); 7.9762 (1.2); 7.9594 (1.5); 7.9547 (1.4); 7.9409 (1.8); 7.9388 (2.0); 7.9362 (1.8); 7.9341 (1.8); 7.9203 (1.8); 7.9155 (1.7); 7.6788 (2.0); 7.6766 (3.6); 7.6746 (2.4); 7.6582 (1.8); 7.6561 (3.2); 7.6539 (2.0); 7.3018 (1.9); 7.2960 (2.0); 7.2803 (2.1); 7.2785 (2.5); 7.2757 (3.0); 7.2663 (1.8); 7.2639 (2.0); 7.2599 (1.8); 7.2575 (1.6); 7.2478 (1.7); 7.2453 (1.7); 5.1825 (0.6); 5.1460 (2.1); 5.0933 (2.0); 5.0579 (0.6); 4.2193 (0.6); 4.1869 (0.6); 4.0986 (0.8); 4.0808 (0.8); 4.0557 (1.1); 4.0379 (3.4); 4.0201 (3.4); 4.0024 (1.2); 3.8076 (0.6); 3.7738 (0.6); 3.3220 (30.6); 3.1522 (0.7); 2.7920 (0.7); 2.6705 (0.5); 2.5680 (0.6); 2.5583 (1.1); 2.5484 (0.7); 2.5411 (2.1); 2.5301 (0.8); 2.5243 (1.4); 2.5197 (1.8); 2.5108 (24.5); 2.5063 (54.7); 2.5017 (77.4); 2.4971 (54.8); 2.4926 (25.3); 2.1832 (0.6); 1.9887 (16.0); 1.9090 (1.5); 1.8718 (0.9); 1.8258 (0.7); 1.6402 (0.5); 1.4102 (0.5); 1.3554 (5.2); 1.2351 (0.9); 1.2036 (1.0); 1.1922 (4.7); 1.1858 (2.3); 1.1745 (9.3); 1.1681 (1.1); 1.1567 (4.5); 0.0080 (1.3); 0.0002 (48.1); 0.0085 (1.5) I-63: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.5889 (1.3); 8.2481 (6.1); 8.1032 (4.6); 8.0943 (4.5); 8.0215 (2.1); 8.0155 (2.2); 8.0009 (3.9); 7.9959 (3.8); 7.9808 (3.6); 7.9753 (3.6); 7.9595 (3.1); 7.7000 (3.0); 7.6799 (5.5); 7.6599 (2.8); 7.3025 (4.1); 7.2964 (4.3); 7.2822 (5.5); 7.2748 (7.1); 7.2566 (3.1); 6.8699 (0.6); 5.0144 (10.4); 4.9638 (0.7); 4.0552 (1.3); 4.0378 (3.7); 4.0200 (3.7); 4.0024 (1.3); 3.7947 (1.0); 3.7698 (1.8); 3.7501 (1.5); 3.6783 (1.6); 3.6607 (1.9); 3.6348 (1.6); 3.6097 (1.8); 3.5937 (2.7); 3.5751 (2.6); 3.5638 (4.3); 3.5448 (5.4); 3.5291 (2.7); 3.4985 (1.2); 3.4675 (1.4); 3.4491 (1.4); 3.4370 (1.0); 3.3927 (1.2); 3.3741 (2.3); 3.3206 (26.0); 3.2046 (1.4); 3.1859 (1.8); 3.1672 (1.3); 3.0778 (1.4); 3.0598 (1.9); 3.0420 (1.4); 2.6701 (1.6); 2.5404 (6.6); 2.5014 (226.7); 2.3286 (1.6); 2.2051 (1.2); 2.1850 (2.1); 2.1719 (1.6); 2.1444 (1.6); 2.1259 (1.8); 2.1129 (1.7); 2.0981 (1.7); 2.0809 (1.5); 2.0677 (1.2); 1.9886 (16.0); 1.9701 (1.8); 1.9576 (1.2); 1.9375 (0.9); 1.9087 (0.6); 1.7602 (0.6); 1.3551 (7.0); 1.2352 (3.8); 1.1921 (4.2); 1.1744 (8.0); 1.1565 (4.1); 0.0002 (65.7) I-64: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2218 (0.8); 8.2198 (1.2); 8.2178 (0.9); 8.2157 (0.9); 8.2136 (1.2); 8.2117 (0.8); 8.0975 (0.7); 8.0954 (0.8); 8.0928 (0.8); 8.0907 (0.8); 8.0854 (0.8); 8.0832 (0.8); 8.0807 (0.9); 8.0786 (0.8); 7.8676 (0.7); 7.8613 (0.7); 7.8487 (0.8); 7.8464 (0.8); 7.8426 (0.8); 7.8402 (0.8); 7.8276 (0.7); 7.8214 (0.7); 7.8129 (0.7); 7.8082 (0.6); 7.7946 (0.7); 7.7922 (1.0); 7.7899 (0.8); 7.7875 (1.0); 7.7739 (1.1); 7.7692 (1.0); 7.7117 (1.1); 7.7093 (1.8); 7.7069 (1.1); 7.6910 (0.7); 7.6887 (1.2); 7.6863 (0.7); 7.2624 (8.4); 7.1545 (0.9); 7.1519 (0.9); 7.1424 (0.8); 7.1397 (0.9); 7.1362 (0.9); 7.1335 (0.8); 7.1241 (0.9); 7.1214 (0.8); 7.0113 (0.9); 7.0097 (0.9); 7.0039 (0.9); 7.0023 (0.9); 6.9901 (0.8); 6.9885 (0.9); 6.9827 (0.8); 6.9811 (0.8); 5.3003 (3.8); 4.9474 (7.2); 4.1834 (3.2); 4.1699 (3.2); 3.7905 (16.0); 1.5748 (1.9); 0.0002 (13.5) I-65: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5021 (1.2); 8.4957 (1.3); 8.3435 (1.5); 8.1153 (1.2); 8.1122 (0.8); 8.1066 (0.8); 8.1034 (1.4); 8.1001 (0.8); 7.8413 (1.4); 7.8377 (2.5); 7.8293 (3.0); 7.8259 (2.5); 7.5117 (0.7); 7.5049 (0.8); 7.5006 (0.7); 7.4894 (0.7); 7.4852 (0.8); 7.4826 (0.8); 7.4783 (0.7); 7.2603 (46.8); 7.2092 (0.9); 7.1972 (1.4); 7.1867 (1.4); 7.1759 (0.8); 4.0858 (4.1); 4.0727 (4.2); 3.8973 (8.2); 3.7025 (16.0); 2.0455 (0.5); 1.5432 (6.4); 0.0081 (1.9); 0.0002 (73.8); 0.0085 (2.8) I-66: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.1115 (0.5); 8.2587 (3.0); 8.2525 (3.3); 8.1165 (2.0); 8.1144 (2.3); 8.1118 (2.6); 8.1097 (2.3); 8.1044 (2.2); 8.1023 (2.5); 8.0997 (2.5); 8.0976 (2.4); 8.0300 (1.5); 8.0238 (1.4); 8.0103 (1.9); 8.0089 (2.1); 8.0042 (1.9); 8.0027 (2.0); 7.9916 (2.3); 7.9893 (2.0); 7.9869 (2.3); 7.9830 (1.7); 7.9731 (2.4); 7.9710 (2.5); 7.9683 (2.3); 7.9663 (2.4); 7.9525 (2.5); 7.9477 (2.4); 7.6838 (2.4); 7.6816 (4.6); 7.6794 (2.7); 7.6632 (2.3); 7.6610 (4.2); 7.6587 (2.4); 7.3033 (2.1); 7.2962 (4.4); 7.2937 (2.8); 7.2838 (3.8); 7.2817 (4.2); 7.2774 (3.5); 7.2751 (4.2); 7.2655 (2.4); 7.2630 (2.2); 4.9230 (16.0); 4.0377 (1.5); 4.0199 (1.5); 4.0021 (0.5); 3.3209 (47.8); 2.6746 (0.8); 2.6700 (1.1); 2.6655 (0.8); 2.5406 (1.4); 2.5238 (2.0); 2.5191 (3.0); 2.5104 (56.8); 2.5058 (127.4); 2.5012 (181.4); 2.4966 (126.9); 2.4920 (57.9); 2.4748 (1.1); 2.4708 (0.6); 2.3329 (0.8); 2.3282 (1.1); 2.3236 (0.8); 1.9885 (7.1); 1.9084 (3.9); 1.1921 (2.1); 1.1744 (4.4); 1.1566 (2.1); 0.1457 (0.6); 0.0102 (0.5); 0.0080 (5.2); 0.0063 (1.1); 0.0055 (1.2); 0.0046 (1.5); 0.0038 (2.0); 0.0002 (189.9); 0.0027 (9.5); 0.0043 (4.1); 0.0051 (3.0); 0.0060 (2.5); 0.0068 (2.1); 0.0085 (5.8); 0.0107 (1.1); 0.0115 (0.9); 0.0123 (0.8); 0.0131 (0.7); 0.0139 (0.5); 0.0274 (0.7); 0.1494 (0.6) I-67: .sup.1H-NMR(400.0 MHz, CDCl3): = 9.2223 (4.2); 8.7933 (9.7); 8.0386 (1.1); 8.0292 (1.1); 7.7968 (0.6); 7.7920 (0.6); 7.7751 (1.2); 7.7578 (1.2); 7.7530 (1.1); 7.7132 (2.1); 7.6926 (1.2); 7.2614 (56.4); 7.1244 (1.0); 7.1098 (1.1); 7.1066 (1.0); 7.0941 (0.8); 4.9797 (9.5); 4.9559 (0.6); 3.8404 (16.0); 3.8303 (1.3); 1.6019 (1.0); 1.4373 (0.5); 1.2539 (1.8); 0.0073 (2.0); 0.0002 (32.8); 0.0084 (1.5) I-68: .sup.1H-NMR(599.6 MHz, CDCl3): = 9.2245 (0.3); 8.7897 (0.7); 8.6074 (0.4); 7.2712 (3.2); 4.9556 (0.7); 4.3109 (0.3); 4.2995 (0.3); 2.7549 (23.2); 2.6273 (50.0); 2.0446 (0.3); 2.0335 (0.4); 1.8407 (0.6); 1.3738 (0.3); 1.3334 (2.0); 1.3234 (1.1); 1.3110 (1.1); 1.2849 (3.2); 1.2567 (12.3); 0.8911 (0.8); 0.8806 (1.4); 0.8690 (0.8); 0.8422 (0.4); 0.0699 (1.8); 0.0001 (4.0) I-69: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.8847 (1.2); 8.6620 (4.8); 8.6550 (4.9); 8.4145 (2.5); 8.4102 (4.7); 8.4068 (2.3); 8.1432 (1.8); 8.1411 (2.0); 8.1386 (2.3); 8.1365 (2.1); 8.1311 (2.0); 8.1291 (2.2); 8.1264 (2.3); 8.1244 (2.1); 8.0475 (1.7); 8.0428 (1.6); 8.0289 (2.1); 8.0269 (2.2); 8.0242 (1.9); 8.0223 (2.1); 8.0084 (2.2); 8.0037 (2.1); 7.8809 (1.8); 7.8767 (1.8); 7.8740 (1.8); 7.8697 (1.7); 7.8569 (1.9); 7.8527 (2.0); 7.8499 (1.8); 7.8457 (1.7); 7.8140 (2.3); 7.8117 (4.1); 7.8095 (2.4); 7.7935 (2.1); 7.7912 (3.6); 7.7889 (2.0); 7.3571 (2.1); 7.3546 (2.1); 7.3450 (1.9); 7.3425 (2.1); 7.3385 (2.1); 7.3360 (1.9); 7.3264 (2.0); 7.3239 (2.0); 5.7566 (9.1); 4.0556 (0.7); 4.0351 (16.0); 4.0201 (2.0); 4.0023 (0.7); 3.3231 (51.0); 2.6703 (0.7); 2.5409 (1.2); 2.5240 (1.5); 2.5194 (2.3); 2.5107 (35.4); 2.5061 (77.7); 2.5015 (108.4); 2.4969 (74.2); 2.4924 (32.7); 2.4782 (0.6); 2.4738 (0.5); 2.3286 (0.6); 1.9886 (8.6); 1.1922 (2.6); 1.1745 (5.2); 1.1567 (2.6); 0.0080 (2.7); 0.0061 (0.6); 0.0002 (103.1); 0.0044 (1.4); 0.0053 (1.0); 0.0061 (0.9); 0.0070 (0.8); 0.0085 (2.9) I-70: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2098 (1.4); 8.2076 (1.1); 8.2056 (1.2); 8.2037 (1.4); 8.0585 (0.8); 8.0565 (0.9); 8.0538 (1.0); 8.0518 (0.8); 8.0463 (0.9); 8.0443 (0.9); 8.0417 (0.9); 8.0397 (0.8); 7.8172 (0.7); 7.8110 (0.6); 7.7980 (0.9); 7.7962 (0.9); 7.7918 (0.9); 7.7900 (0.8); 7.7771 (0.7); 7.7709 (0.7); 7.7492 (0.6); 7.7444 (0.6); 7.7309 (0.8); 7.7285 (1.1); 7.7262 (0.8); 7.7238 (1.0); 7.7103 (1.1); 7.7055 (1.0); 7.6507 (1.2); 7.6484 (1.9); 7.6461 (1.1); 7.6300 (0.8); 7.6278 (1.2); 7.6254 (0.6); 7.2617 (41.6); 7.0732 (1.0); 7.0705 (1.0); 7.0610 (1.2); 7.0583 (1.2); 7.0549 (1.2); 7.0522 (1.2); 7.0428 (1.2); 7.0401 (1.1); 6.9728 (1.0); 6.9714 (0.9); 6.9654 (1.0); 6.9518 (0.9); 6.9504 (0.9); 6.9444 (0.9); 5.3003 (2.0); 4.8918 (7.5); 4.1783 (3.4); 4.1656 (3.4); 3.7969 (16.0); 1.5643 (1.7); 1.5504 (0.8); 1.5424 (0.6); 1.5293 (1.2); 1.5161 (0.6); 1.5082 (0.7); 0.8240 (0.6); 0.8132 (1.6); 0.8079 (1.7); 0.8029 (0.8); 0.7975 (1.0); 0.7918 (1.6); 0.7867 (1.4); 0.7765 (0.8); 0.6697 (0.9); 0.6593 (1.7); 0.6560 (1.7); 0.6542 (1.6); 0.6463 (1.5); 0.6422 (1.5); 0.6301 (0.6); 0.0080 (0.7); 0.0002 (26.4); 0.0085 (0.7) I-71: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2101 (1.1); 8.2041 (1.2); 8.0361 (0.6); 8.0343 (0.7); 8.0315 (0.7); 8.0296 (0.7); 8.0240 (0.7); 8.0221 (0.7); 8.0194 (0.7); 8.0175 (0.6); 7.8217 (0.5); 7.8156 (0.5); 7.8024 (0.7); 7.8009 (0.7); 7.7962 (0.7); 7.7947 (0.7); 7.7815 (0.6); 7.7754 (0.5); 7.7207 (0.5); 7.7160 (0.5); 7.7023 (0.6); 7.7000 (0.8); 7.6977 (0.7); 7.6953 (0.8); 7.6817 (0.8); 7.6770 (0.7); 7.5932 (1.5); 7.5911 (0.9); 7.5726 (1.1); 7.5704 (0.6); 7.2613 (42.9); 7.2574 (0.7); 7.0382 (0.7); 7.0356 (0.7); 7.0260 (0.7); 7.0235 (0.7); 7.0199 (0.7); 7.0173 (0.6); 7.0078 (0.6); 7.0052 (0.6); 6.9609 (0.8); 6.9548 (0.8); 6.9411 (0.7); 6.9399 (0.7); 6.9338 (0.7); 6.9325 (0.7); 5.3003 (0.8); 4.8895 (7.8); 4.5046 (2.0); 4.4889 (4.0); 4.4732 (2.0); 3.6905 (16.0); 2.7120 (1.9); 2.6963 (3.8); 2.6806 (1.8); 1.5684 (0.6); 1.4835 (0.6); 1.4739 (0.5); 1.4703 (0.9); 1.4492 (0.6); 0.7779 (1.2); 0.7728 (1.2); 0.7654 (2.1); 0.7593 (1.2); 0.7518 (1.0); 0.7489 (0.5); 0.7397 (1.3); 0.7322 (1.2); 0.7278 (0.8); 0.7221 (0.6); 0.7191 (1.1); 0.7119 (1.3); 0.7063 (1.0); 0.0080 (0.7); 0.0002 (26.5); 0.0085 (0.8) I-72: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.9557 (0.7); 8.2209 (3.2); 8.2147 (3.3); 8.0566 (2.0); 8.0545 (2.2); 8.0519 (2.6); 8.0498 (2.3); 8.0445 (2.2); 8.0424 (2.5); 8.0397 (2.5); 8.0377 (2.4); 7.9728 (1.5); 7.9665 (1.4); 7.9519 (2.2); 7.9457 (2.1); 7.9319 (1.6); 7.9257 (1.5); 7.9206 (2.0); 7.9158 (1.9); 7.9021 (2.2); 7.8999 (2.4); 7.8973 (2.2); 7.8952 (2.4); 7.8815 (2.4); 7.8767 (2.3); 7.6173 (2.4); 7.6150 (4.5); 7.6128 (2.7); 7.5967 (2.2); 7.5944 (4.1); 7.5921 (2.3); 7.2479 (2.1); 7.2422 (2.1); 7.2268 (2.0); 7.2211 (2.0); 7.2198 (2.0); 7.2013 (2.3); 7.1988 (2.4); 7.1891 (2.1); 7.1867 (2.4); 7.1829 (2.3); 7.1804 (2.1); 7.1707 (2.3); 7.1682 (2.2); 4.8305 (16.0); 4.0555 (1.1); 4.0377 (3.3); 4.0199 (3.4); 4.0022 (1.1); 3.3194 (16.8); 2.6746 (0.7); 2.6700 (1.0); 2.6653 (0.7); 2.5282 (0.8); 2.5238 (3.2); 2.5191 (4.1); 2.5103 (54.2); 2.5058 (121.3); 2.5012 (172.8); 2.4966 (121.6); 2.4920 (54.2); 2.3329 (0.7); 2.3283 (1.0); 2.3236 (0.7); 1.9886 (16.0); 1.9084 (3.2); 1.5421 (0.6); 1.5288 (1.4); 1.5212 (1.4); 1.5160 (0.9); 1.5080 (2.4); 1.5045 (1.2); 1.4945 (1.4); 1.4871 (1.5); 1.4738 (0.7); 1.3551 (1.3); 1.1922 (4.7); 1.1744 (9.9); 1.1566 (4.7); 0.7032 (1.2); 0.6997 (0.6); 0.6907 (2.5); 0.6855 (3.8); 0.6825 (2.0); 0.6778 (2.7); 0.6725 (1.4); 0.6697 (2.7); 0.6640 (3.7); 0.6570 (2.8); 0.6463 (1.1); 0.6409 (2.5); 0.6333 (3.7); 0.6277 (5.6); 0.6205 (3.9); 0.6152 (3.6); 0.6023 (1.2); 0.0080 (3.5); 0.0064 (0.9); 0.0055 (1.0); 0.0047 (1.2); 0.0039 (1.6); 0.0022 (4.6); 0.0002 (119.2); 0.0026 (6.1); 0.0051 (1.7); 0.0059 (1.3); 0.0067 (1.0); 0.0085 (3.4) I-73: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4849 (1.8); 8.4780 (1.8); 8.3735 (0.9); 8.3696 (1.8); 8.3661 (0.9); 8.0390 (0.7); 8.0370 (0.8); 8.0343 (0.8); 8.0322 (0.8); 8.0269 (0.7); 8.0248 (0.8); 8.0222 (0.8); 8.0201 (0.8); 7.7893 (0.6); 7.7846 (0.6); 7.7709 (0.7); 7.7686 (0.9); 7.7662 (0.7); 7.7639 (0.9); 7.7502 (1.0); 7.7455 (0.9); 7.6727 (0.9); 7.6703 (1.7); 7.6680 (1.0); 7.6520 (0.7); 7.6497 (1.2); 7.6473 (0.7); 7.5231 (0.7); 7.5188 (0.8); 7.5162 (0.8); 7.5119 (0.7); 7.5006 (0.8); 7.4962 (0.8); 7.4936 (0.7); 7.4893 (0.7); 7.2617 (11.0); 7.1094 (0.8); 7.1067 (0.8); 7.0972 (0.8); 7.0946 (0.8); 7.0911 (0.8); 7.0884 (0.8); 7.0789 (0.8); 7.0763 (0.8); 5.2354 (1.6); 5.2180 (1.7); 4.4916 (0.9); 4.4840 (1.0); 4.4758 (2.0); 4.4685 (2.0); 4.4602 (1.0); 4.4529 (1.0); 3.6582 (16.0); 2.6896 (1.2); 2.6732 (2.0); 2.6577 (1.1); 1.7083 (5.8); 1.6908 (5.8); 1.5737 (0.8); 0.0023 (0.5); 0.0002 (14.6); 0.0027 (0.6) I-74: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4898 (1.6); 8.4829 (1.7); 8.3764 (0.9); 8.3725 (1.6); 8.3688 (0.9); 8.0743 (0.6); 8.0722 (0.7); 8.0696 (0.8); 8.0675 (0.7); 8.0621 (0.7); 8.0601 (0.8); 8.0575 (0.8); 8.0554 (0.7); 7.7962 (0.5); 7.7915 (0.5); 7.7778 (0.6); 7.7756 (0.8); 7.7731 (0.7); 7.7709 (0.8); 7.7572 (0.8); 7.7525 (0.8); 7.6721 (0.8); 7.6698 (1.6); 7.6675 (1.0); 7.6515 (0.6); 7.6492 (1.1); 7.6468 (0.6); 7.5349 (0.6); 7.5306 (0.6); 7.5280 (0.7); 7.5237 (0.6); 7.5124 (0.6); 7.5081 (0.6); 7.5055 (0.7); 7.5012 (0.6); 7.2611 (42.0); 7.1333 (0.7); 7.1308 (0.7); 7.1212 (0.7); 7.1186 (0.7); 7.1150 (0.8); 7.1124 (0.7); 7.1028 (0.7); 7.1002 (0.7); 4.9554 (7.2); 4.4230 (0.6); 4.4050 (0.6); 4.3959 (1.3); 4.3779 (1.4); 4.3527 (1.3); 4.3386 (1.4); 4.3256 (0.6); 4.3115 (0.6); 3.7263 (2.8); 3.7131 (0.6); 3.6746 (16.0); 2.8456 (0.7); 2.8315 (0.7); 1.2065 (6.6); 1.1981 (1.5); 1.1886 (6.5); 1.1800 (1.5); 0.0080 (0.6); 0.0002 (26.9); 0.0085 (0.8) I-75: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4881 (1.8); 8.4812 (1.8); 8.3750 (1.0); 8.3712 (1.8); 8.3674 (0.9); 8.0755 (0.7); 8.0734 (0.8); 8.0708 (0.8); 8.0687 (0.8); 8.0634 (0.8); 8.0613 (0.8); 8.0587 (0.8); 8.0566 (0.8); 7.7999 (0.6); 7.7952 (0.6); 7.7815 (0.7); 7.7793 (0.9); 7.7768 (0.7); 7.7746 (0.9); 7.7609 (0.9); 7.7561 (0.9); 7.6748 (1.0); 7.6725 (1.7); 7.6702 (1.0); 7.6542 (0.7); 7.6519 (1.2); 7.6495 (0.7); 7.5276 (0.7); 7.5233 (0.8); 7.5207 (0.8); 7.5164 (0.7); 7.5051 (0.7); 7.5008 (0.8); 7.4982 (0.7); 7.4938 (0.7); 7.2616 (12.7); 7.1347 (0.8); 7.1320 (0.8); 7.1225 (0.8); 7.1199 (0.8); 7.1163 (0.8); 7.1137 (0.8); 7.1041 (0.8); 7.1015 (0.7); 5.3003 (2.8); 4.9522 (8.2); 4.5262 (2.0); 4.5105 (4.1); 4.4949 (2.0); 3.7263 (0.8); 3.6861 (16.0); 2.7202 (1.9); 2.7046 (3.8); 2.6889 (1.9); 1.5751 (1.4); 0.0080 (0.6); 0.0002 (18.9); 0.0085 (0.6) I-76: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4909 (1.2); 8.4841 (1.3); 8.3698 (0.8); 8.3661 (1.3); 8.3626 (0.8); 8.0628 (0.6); 8.0608 (0.7); 8.0581 (0.8); 8.0561 (0.7); 8.0507 (0.7); 8.0486 (0.8); 8.0460 (0.8); 8.0439 (0.7); 7.7910 (0.5); 7.7863 (0.5); 7.7726 (0.6); 7.7703 (0.8); 7.7679 (0.6); 7.7656 (0.8); 7.7520 (0.8); 7.7473 (0.8); 7.6730 (0.8); 7.6707 (1.5); 7.6684 (0.9); 7.6524 (0.6); 7.6501 (1.0); 7.6477 (0.6); 7.5277 (0.6); 7.5234 (0.6); 7.5209 (0.7); 7.5165 (0.6); 7.5053 (0.6); 7.5009 (0.7); 7.4983 (0.6); 7.4940 (0.6); 7.2625 (15.4); 7.1263 (0.7); 7.1237 (0.7); 7.1141 (0.7); 7.1115 (0.7); 7.1079 (0.7); 7.1053 (0.7); 7.0958 (0.7); 7.0932 (0.6); 4.9541 (6.9); 4.4218 (0.6); 4.4039 (0.6); 4.3947 (1.3); 4.3768 (1.3); 4.3508 (1.3); 4.3367 (1.3); 4.3237 (0.6); 4.3096 (0.6); 3.6748 (16.0); 2.8441 (0.6); 2.8300 (0.6); 1.2054 (6.3); 1.1875 (6.2); 0.0002 (9.2) I-77: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4907 (1.0); 8.4840 (1.0); 8.3677 (1.2); 8.0635 (0.7); 8.0614 (0.8); 8.0588 (0.8); 8.0567 (0.8); 8.0514 (0.7); 8.0493 (0.8); 8.0467 (0.8); 8.0446 (0.7); 7.7950 (0.6); 7.7903 (0.6); 7.7766 (0.7); 7.7744 (0.9); 7.7719 (0.7); 7.7697 (0.9); 7.7560 (0.9); 7.7512 (0.9); 7.6765 (0.9); 7.6742 (1.7); 7.6719 (1.0); 7.6559 (0.7); 7.6536 (1.2); 7.6512 (0.7); 7.5262 (0.6); 7.5219 (0.7); 7.5195 (0.8); 7.5150 (0.6); 7.5038 (0.7); 7.4995 (0.7); 7.4969 (0.7); 7.4926 (0.6); 7.2614 (33.9); 7.1278 (0.8); 7.1252 (0.8); 7.1157 (0.8); 7.1131 (0.8); 7.1095 (0.8); 7.1068 (0.8); 7.0973 (0.8); 7.0947 (0.7); 4.9507 (8.0); 4.5244 (1.9); 4.5087 (4.0); 4.4930 (2.0); 3.6860 (16.0); 2.7187 (1.9); 2.7031 (3.8); 2.6874 (1.8); 0.0080 (0.6); 0.0002 (21.3); 0.0085 (0.6) I-78: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.2065 (2.5); 8.2005 (2.5); 8.0335 (1.5); 8.0305 (1.6); 8.0213 (1.5); 8.0185 (1.5); 7.8191 (1.2); 7.8130 (1.1); 7.7984 (1.6); 7.7923 (1.5); 7.7788 (1.2); 7.7727 (1.1); 7.7079 (1.0); 7.7031 (1.0); 7.6894 (1.3); 7.6871 (1.7); 7.6825 (1.5); 7.6688 (1.5); 7.6641 (1.4); 7.5863 (3.1); 7.5656 (2.1); 7.2612 (36.6); 7.0326 (1.4); 7.0301 (1.4); 7.0205 (1.4); 7.0179 (1.4); 7.0144 (1.4); 7.0119 (1.3); 7.0022 (1.3); 6.9997 (1.2); 6.9599 (1.7); 6.9529 (1.6); 6.9389 (1.6); 6.9316 (1.5); 4.8882 (16.0); 4.3012 (2.1); 4.2834 (6.4); 4.2655 (6.4); 4.2477 (2.1); 1.5788 (0.8); 1.4995 (1.0); 1.4918 (1.1); 1.4787 (1.7); 1.4705 (0.6); 1.4652 (1.1); 1.4575 (1.1); 1.4442 (0.6); 1.3262 (7.4); 1.3084 (14.9); 1.2905 (7.2); 0.8055 (0.8); 0.8022 (0.6); 0.7921 (2.6); 0.7869 (3.0); 0.7792 (3.7); 0.7745 (3.0); 0.7659 (1.7); 0.7560 (0.7); 0.7481 (1.0); 0.7442 (1.9); 0.7356 (2.7); 0.7314 (2.0); 0.7232 (1.9); 0.7152 (2.5); 0.7098 (1.9); 0.7030 (0.7); 0.6969 (0.7); 0.0080 (0.9); 0.0002 (22.0); 0.0085 (0.7) I-79: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5094 (4.7); 8.5025 (4.8); 8.3669 (3.0); 8.3632 (5.2); 8.3596 (3.0); 8.0593 (2.1); 8.0573 (2.3); 8.0546 (2.5); 8.0526 (2.3); 8.0472 (2.3); 8.0451 (2.5); 8.0425 (2.5); 8.0404 (2.3); 7.7393 (1.8); 7.7346 (1.8); 7.7208 (2.1); 7.7186 (2.6); 7.7161 (2.1); 7.7139 (2.6); 7.7002 (2.6); 7.6955 (2.6); 7.6142 (2.8); 7.6119 (4.9); 7.6096 (2.9); 7.5936 (2.1); 7.5913 (3.5); 7.5889 (2.0); 7.5373 (2.0); 7.5330 (2.1); 7.5304 (2.1); 7.5261 (1.9); 7.5150 (2.1); 7.5107 (2.3); 7.5082 (2.0); 7.5039 (1.9); 7.2610 (56.9); 7.1014 (2.3); 7.0988 (2.3); 7.0892 (2.3); 7.0866 (2.4); 7.0831 (2.4); 7.0804 (2.2); 7.0709 (2.2); 7.0682 (2.1); 5.3495 (1.2); 5.3320 (5.1); 5.3145 (5.2); 5.2970 (1.2); 2.7728 (4.6); 2.1031 (0.9); 2.0465 (1.8); 1.7714 (16.0); 1.7652 (1.7); 1.7539 (15.9); 1.7477 (1.6); 1.2773 (0.6); 1.2594 (1.2); 1.2415 (0.6); 1.2214 (1.5); 0.0080 (2.0); 0.0002 (76.0); 0.0067 (0.7); 0.0085 (2.2) I-80: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.6748 (1.4); 8.4653 (2.8); 8.4468 (2.9); 8.2494 (4.0); 8.2451 (3.1); 8.2433 (4.2); 8.0978 (2.6); 8.0958 (2.9); 8.0932 (3.4); 8.0911 (3.0); 8.0857 (2.8); 8.0837 (3.2); 8.0810 (3.2); 8.0789 (3.1); 8.0221 (1.9); 8.0158 (1.8); 8.0024 (2.4); 8.0009 (2.6); 7.9962 (2.4); 7.9947 (2.6); 7.9813 (2.1); 7.9747 (4.1); 7.9699 (2.4); 7.9561 (2.8); 7.9539 (3.2); 7.9514 (2.7); 7.9492 (3.1); 7.9355 (3.2); 7.9307 (3.0); 7.7671 (3.1); 7.7648 (5.8); 7.7626 (3.4); 7.7464 (2.8); 7.7442 (5.0); 7.7419 (2.8); 7.3041 (2.7); 7.2985 (2.7); 7.2972 (2.5); 7.2832 (5.4); 7.2808 (3.9); 7.2773 (2.8); 7.2759 (2.7); 7.2711 (2.8); 7.2686 (3.0); 7.2648 (3.0); 7.2623 (2.7); 7.2527 (3.0); 7.2501 (2.9); 4.8393 (16.0); 4.3306 (2.6); 4.3123 (4.1); 4.2940 (2.6); 4.2758 (0.5); 3.6216 (0.9); 3.6177 (5.2); 3.6155 (2.9); 3.6115 (2.7); 3.6093 (2.1); 3.6074 (3.6); 3.6028 (3.9); 3.6011 (12.0); 3.5989 (4.3); 3.5950 (3.8); 3.5930 (2.1); 3.5908 (2.7); 3.5867 (2.8); 3.5845 (5.4); 3.5806 (1.0); 3.3212 (11.7); 2.6751 (0.6); 2.6705 (0.8); 2.6658 (0.6); 2.5242 (2.1); 2.5196 (2.8); 2.5108 (40.1); 2.5062 (91.1); 2.5016 (129.2); 2.4970 (90.8); 2.4924 (40.8); 2.3333 (0.5); 2.3287 (0.8); 2.3241 (0.5); 2.1829 (0.8); 1.9087 (0.7); 1.7808 (0.8); 1.7761 (5.3); 1.7685 (4.2); 1.7640 (2.6); 1.7595 (15.2); 1.7548 (2.7); 1.7505 (4.2); 1.7429 (5.2); 1.7384 (0.8); 1.3554 (7.3); 1.3262 (15.9); 1.3080 (15.8); 0.1457 (0.6); 0.0079 (6.1); 0.0062 (1.3); 0.0054 (1.5); 0.0045 (1.9); 0.0002 (240.5); 0.0028 (10.9); 0.0052 (2.8); 0.0061 (2.2); 0.0069 (1.9); 0.0085 (6.9); 0.0108 (0.9); 0.0117 (0.8); 0.0124 (0.8); 0.0132 (0.6); 0.0140 (0.6); 0.1495 (0.7) I-81: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5080 (3.0); 8.5010 (3.0); 8.3784 (1.6); 8.3746 (2.7); 8.0840 (1.2); 8.0773 (1.4); 8.0719 (1.3); 8.0698 (1.3); 8.0673 (1.4); 7.7923 (1.1); 7.7875 (1.1); 7.7736 (1.2); 7.7716 (1.4); 7.7691 (1.1); 7.7668 (1.4); 7.7531 (1.5); 7.7484 (1.6); 7.6572 (2.8); 7.6365 (2.0); 7.5478 (0.8); 7.5433 (0.9); 7.5366 (0.8); 7.5186 (2.3); 7.2858 (0.8); 7.2602 (283.4); 7.2535 (1.7); 7.2326 (1.8); 7.1432 (1.4); 7.1407 (1.4); 7.1311 (1.2); 7.1285 (1.3); 7.1249 (1.2); 7.1223 (1.2); 7.1127 (1.3); 7.1101 (1.2); 6.9965 (1.6); 5.0311 (16.0); 4.1136 (0.5); 2.7772 (3.0); 2.1074 (0.9); 2.0459 (2.6); 1.8552 (0.6); 1.4322 (4.0); 1.2842 (0.6); 1.2775 (0.9); 1.2598 (1.9); 1.2435 (2.5); 1.2227 (1.5); 0.1459 (1.3); 0.0338 (0.5); 0.0255 (1.2); 0.0176 (0.8); 0.0080 (12.8); 0.0002 (462.3); 0.0085 (12.5); 0.0277 (3.2); 0.1492 (1.3) I-82: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5045 (1.9); 8.4976 (1.9); 8.3531 (1.0); 8.3493 (1.8); 8.3455 (1.0); 8.1167 (0.7); 8.1146 (0.8); 8.1121 (0.8); 8.1100 (0.8); 8.1046 (0.7); 8.1024 (0.8); 8.1001 (0.8); 8.0979 (0.8); 7.8481 (0.5); 7.8455 (1.0); 7.8437 (0.6); 7.8409 (1.0); 7.8276 (1.1); 7.8230 (1.1); 7.8043 (1.0); 7.8015 (1.7); 7.7991 (1.2); 7.7838 (0.6); 7.7813 (0.7); 7.5112 (0.7); 7.5068 (0.8); 7.5043 (0.8); 7.4999 (0.7); 7.4888 (0.7); 7.4845 (0.8); 7.4820 (0.8); 7.4776 (0.7); 7.2645 (5.7); 7.2098 (0.8); 7.2067 (0.8); 7.1977 (0.8); 7.1945 (0.8); 7.1919 (0.8); 7.1888 (0.8); 7.1798 (0.8); 7.1766 (0.7); 5.3006 (3.1); 3.8261 (7.5); 3.5681 (0.9); 3.5552 (16.0); 3.5380 (2.0); 3.5226 (0.9); 2.5160 (1.6); 2.5007 (2.4); 2.4860 (1.6); 0.0002 (8.4) I-83: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.0422 (0.6); 8.0403 (0.6); 8.0377 (0.7); 8.0357 (0.6); 8.0301 (0.6); 8.0282 (0.7); 8.0256 (0.7); 8.0236 (0.6); 7.7573 (0.6); 7.7551 (0.7); 7.7526 (0.6); 7.7504 (0.7); 7.7367 (0.7); 7.7320 (0.6); 7.6417 (0.8); 7.6396 (1.3); 7.6374 (0.8); 7.6211 (0.6); 7.6190 (1.0); 7.6168 (0.6); 7.2612 (30.9); 7.1092 (0.6); 7.1068 (0.6); 7.0971 (0.6); 7.0946 (0.6); 7.0909 (0.6); 7.0884 (0.6); 7.0788 (0.6); 7.0762 (0.6); 5.3001 (0.8); 5.2732 (1.3); 5.2558 (1.3); 3.8017 (16.0); 1.7227 (5.8); 1.7052 (5.7); 0.0080 (0.5); 0.0002 (19.0); 0.0085 (0.6) I-84: .sup.1H-NMR(400.6 MHz, CDCl3): = 9.0998 (1.0); 8.7062 (0.8); 8.6990 (0.8); 8.5164 (3.2); 8.5094 (3.1); 8.4023 (1.8); 8.3986 (2.9); 8.3949 (1.7); 8.0893 (1.3); 8.0868 (1.5); 8.0795 (1.2); 8.0772 (1.3); 8.0747 (1.3); 8.0725 (1.3); 8.0313 (0.6); 7.8007 (1.0); 7.7960 (1.1); 7.7801 (1.5); 7.7754 (1.6); 7.7617 (1.6); 7.7570 (1.6); 7.6650 (1.6); 7.6627 (2.7); 7.6603 (1.5); 7.6444 (1.3); 7.6420 (2.1); 7.6397 (1.3); 7.5832 (0.9); 7.5790 (1.0); 7.5721 (0.9); 7.5611 (0.8); 7.5543 (1.0); 7.5498 (0.9); 7.5186 (1.6); 7.2874 (1.4); 7.2689 (0.8); 7.2602 (301.0); 7.2528 (1.7); 7.2432 (0.6); 7.2265 (0.5); 7.1514 (1.3); 7.1488 (1.4); 7.1392 (1.4); 7.1366 (1.5); 7.1329 (1.4); 7.1304 (1.4); 7.1208 (1.3); 7.1182 (1.2); 6.9966 (1.6); 6.9797 (0.5); 5.0344 (16.0); 4.2590 (1.1); 4.1139 (0.5); 2.7781 (8.9); 2.2718 (1.2); 2.1117 (2.5); 2.0462 (2.5); 1.4322 (11.1); 1.3327 (0.6); 1.2841 (1.0); 1.2777 (1.0); 1.2599 (2.5); 1.2549 (2.2); 1.2433 (1.6); 1.2227 (3.1); 0.1458 (1.3); 0.0270 (2.4); 0.0080 (12.5); 0.0042 (4.7); 0.0002 (480.0); 0.0085 (12.5); 0.0174 (0.6); 0.0225 (0.6); 0.0338 (0.6); 0.1495 (1.4) I-85: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4876 (3.9); 8.4808 (3.8); 8.3693 (2.8); 8.3659 (4.0); 8.0736 (1.9); 8.0709 (2.0); 8.0615 (2.0); 8.0588 (1.9); 7.7872 (1.1); 7.7826 (1.1); 7.7666 (2.0); 7.7641 (1.8); 7.7621 (1.7); 7.7482 (1.6); 7.7435 (1.5); 7.6570 (3.4); 7.6364 (2.4); 7.5245 (1.4); 7.5202 (1.7); 7.5179 (1.6); 7.5135 (1.3); 7.5020 (1.4); 7.4977 (1.6); 7.4953 (1.5); 7.4910 (1.2); 7.2622 (8.4); 7.1301 (1.7); 7.1279 (1.5); 7.1180 (1.8); 7.1156 (1.8); 7.1119 (1.8); 7.1095 (1.5); 7.0997 (1.5); 7.0974 (1.3); 4.9503 (16.0); 4.3266 (2.1); 4.3088 (6.2); 4.2910 (6.2); 4.2732 (2.1); 2.7720 (1.6); 2.0452 (0.7); 1.3351 (7.0); 1.3173 (13.9); 1.2995 (6.8); 1.2594 (0.5); 0.0002 (13.1); 0.0084 (0.6) I-86: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4901 (3.1); 8.4832 (3.1); 8.3650 (1.7); 8.3612 (3.1); 8.3573 (1.7); 8.0637 (1.2); 8.0617 (1.4); 8.0590 (1.5); 8.0569 (1.4); 8.0516 (1.3); 8.0495 (1.4); 8.0469 (1.5); 8.0448 (1.4); 7.7819 (1.1); 7.7772 (1.1); 7.7635 (1.2); 7.7613 (1.7); 7.7588 (1.3); 7.7565 (1.6); 7.7428 (1.6); 7.7381 (1.6); 7.6604 (1.7); 7.6580 (3.1); 7.6557 (1.9); 7.6398 (1.3); 7.6374 (2.2); 7.6351 (1.3); 7.5229 (1.3); 7.5186 (1.3); 7.5161 (1.4); 7.5117 (1.3); 7.5005 (1.3); 7.4962 (1.4); 7.4936 (1.3); 7.4892 (1.2); 7.2618 (13.7); 7.1236 (1.4); 7.1210 (1.5); 7.1114 (1.4); 7.1088 (1.5); 7.1052 (1.4); 7.1026 (1.4); 7.0931 (1.4); 7.0904 (1.4); 5.3001 (4.4); 4.9488 (15.3); 4.3246 (1.9); 4.3068 (6.1); 4.2890 (6.1); 4.2712 (2.0); 2.7729 (1.6); 2.0453 (1.2); 1.3342 (7.8); 1.3164 (16.0); 1.2986 (7.7); 1.2595 (0.8); 0.0080 (0.6); 0.0002 (21.4); 0.0085 (0.6) I-87: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2225 (1.1); 8.2205 (0.8); 8.2183 (0.8); 8.2163 (1.1); 8.0975 (0.7); 8.0955 (0.7); 8.0928 (0.8); 8.0908 (0.7); 8.0854 (0.7); 8.0833 (0.8); 8.0807 (0.8); 8.0786 (0.7); 7.8710 (0.6); 7.8648 (0.6); 7.8522 (0.7); 7.8499 (0.7); 7.8460 (0.7); 7.8437 (0.7); 7.8311 (0.6); 7.8249 (0.6); 7.8108 (0.6); 7.8060 (0.6); 7.7924 (0.6); 7.7901 (0.9); 7.7877 (0.7); 7.7854 (0.8); 7.7718 (0.9); 7.7671 (0.9); 7.7070 (0.9); 7.7046 (1.6); 7.7023 (1.0); 7.6863 (0.6); 7.6840 (1.1); 7.6816 (0.6); 7.2615 (13.6); 7.1531 (0.8); 7.1504 (0.8); 7.1409 (0.9); 7.1382 (1.0); 7.1348 (1.0); 7.1321 (1.0); 7.1226 (1.0); 7.1199 (0.9); 7.0129 (0.7); 7.0115 (0.8); 7.0055 (0.8); 7.0041 (0.8); 6.9917 (0.7); 6.9903 (0.8); 6.9844 (0.8); 6.9829 (0.7); 5.3003 (0.7); 4.9083 (6.5); 4.7300 (0.7); 4.7118 (1.1); 4.6936 (0.8); 3.7782 (16.0); 1.5624 (1.3); 1.5106 (6.3); 1.4926 (6.2); 0.0079 (0.6); 0.0002 (20.0); 0.0085 (0.6) I-88: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2170 (1.2); 8.2148 (0.9); 8.2127 (1.0); 8.2108 (1.2); 8.0814 (0.7); 8.0795 (0.7); 8.0768 (0.8); 8.0748 (0.7); 8.0693 (0.7); 8.0673 (0.7); 8.0646 (0.8); 8.0627 (0.6); 7.8706 (0.6); 7.8644 (0.6); 7.8517 (0.8); 7.8495 (0.8); 7.8455 (0.8); 7.8433 (0.7); 7.8306 (0.7); 7.8244 (0.6); 7.7887 (0.6); 7.7839 (0.6); 7.7702 (0.7); 7.7680 (0.9); 7.7655 (0.8); 7.7633 (0.9); 7.7496 (0.9); 7.7449 (0.8); 7.6603 (1.0); 7.6581 (1.5); 7.6559 (0.9); 7.6396 (0.7); 7.6375 (1.1); 7.6353 (0.6); 7.2625 (6.7); 7.1273 (0.7); 7.1248 (0.7); 7.1151 (0.7); 7.1126 (0.7); 7.1089 (0.8); 7.1064 (0.7); 7.0968 (0.7); 7.0942 (0.6); 7.0000 (0.8); 6.9987 (0.8); 6.9927 (0.9); 6.9913 (0.8); 6.9789 (0.8); 6.9774 (0.8); 6.9715 (0.8); 6.9701 (0.7); 5.3003 (1.5); 4.9496 (8.3); 4.5246 (2.0); 4.5090 (4.2); 4.4933 (2.1); 3.7260 (1.0); 3.6846 (16.0); 2.7198 (2.0); 2.7041 (4.0); 2.6884 (1.9); 1.5699 (0.6); 0.0002 (9.3) I-89: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): = 12.2270 (0.6); 8.2508 (1.4); 8.2446 (1.4); 8.1006 (1.2); 8.0959 (1.1); 8.0837 (1.9); 8.0223 (0.5); 8.0161 (0.5); 8.0016 (0.9); 7.9953 (0.9); 7.9876 (0.7); 7.9821 (1.0); 7.9752 (0.6); 7.9670 (0.9); 7.9642 (0.8); 7.9624 (0.9); 7.9483 (0.8); 7.9437 (0.7); 7.7125 (1.6); 7.6919 (1.4); 7.3045 (0.9); 7.2981 (0.9); 7.2829 (1.6); 7.2764 (0.9); 7.2727 (0.8); 7.2704 (0.9); 7.2663 (0.8); 7.2641 (0.8); 7.2542 (0.8); 7.2519 (0.8); 4.7456 (4.4); 4.1694 (0.6); 3.6177 (1.1); 3.6114 (0.7); 3.6074 (1.0); 3.6011 (2.8); 3.5951 (1.0); 3.5910 (0.7); 3.5846 (1.2); 3.3213 (16.0); 2.5243 (0.5); 2.5195 (0.7); 2.5108 (11.1); 2.5063 (24.1); 2.5017 (33.8); 2.4972 (24.0); 2.4927 (10.8); 2.4756 (1.1); 2.4604 (1.1); 2.3774 (1.1); 2.3589 (1.1); 2.3383 (0.7); 2.3199 (0.7); 1.7761 (1.2); 1.7682 (1.2); 1.7595 (3.5); 1.7508 (1.2); 1.7431 (1.2); 1.3556 (3.0); 1.2348 (0.6); 1.1383 (4.7); 1.1217 (4.6); 0.0002 (17.2); 0.0085 (0.5) I-90: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2013 (2.4); 8.1993 (1.9); 8.1952 (2.5); 8.0821 (1.5); 8.0801 (1.6); 8.0774 (1.7); 8.0755 (1.5); 8.0700 (1.6); 8.0680 (1.7); 8.0653 (1.8); 8.0634 (1.5); 7.8604 (1.2); 7.8542 (1.2); 7.8414 (1.5); 7.8393 (1.5); 7.8352 (1.5); 7.8331 (1.4); 7.8204 (1.3); 7.8142 (1.3); 7.7761 (1.2); 7.7714 (1.2); 7.7576 (1.6); 7.7555 (1.8); 7.7528 (1.6); 7.7508 (1.7); 7.7371 (1.7); 7.7323 (1.7); 7.6254 (2.1); 7.6234 (3.4); 7.6212 (1.9); 7.6049 (1.6); 7.6028 (2.5); 7.6005 (1.4); 7.2614 (20.9); 7.1265 (1.6); 7.1240 (1.5); 7.1143 (1.6); 7.1119 (1.6); 7.1081 (1.6); 7.1056 (1.5); 7.0959 (1.6); 7.0934 (1.4); 6.9999 (1.7); 6.9985 (1.7); 6.9926 (1.8); 6.9913 (1.6); 6.9788 (1.7); 6.9774 (1.6); 6.9714 (1.7); 5.3002 (2.4); 4.9648 (16.0); 4.2712 (1.4); 4.2552 (1.5); 4.2442 (2.2); 4.2282 (2.2); 4.1520 (2.3); 4.1322 (2.4); 4.1250 (1.6); 4.1052 (1.6); 3.8525 (0.7); 3.8387 (0.8); 3.8317 (1.5); 3.8179 (1.6); 3.8110 (2.9); 3.7974 (1.2); 3.7931 (1.9); 3.7888 (2.1); 3.7710 (2.0); 3.7453 (1.2); 3.7270 (1.8); 3.7086 (1.5); 3.6875 (0.9); 3.5632 (1.9); 3.5495 (2.0); 3.5410 (1.7); 3.5273 (1.7); 2.6265 (0.6); 2.6094 (0.8); 2.5922 (0.7); 2.0324 (0.7); 2.0200 (0.9); 2.0116 (0.5); 2.0070 (0.6); 1.9991 (0.9); 1.9872 (0.7); 1.9803 (0.6); 1.9666 (0.5); 1.6600 (0.5); 1.6426 (0.8); 1.6280 (1.0); 1.6085 (1.0); 1.5937 (0.7); 1.5767 (0.5); 1.5579 (5.7); 1.2556 (0.9); 0.0080 (1.0); 0.0002 (32.8); 0.0057 (0.7); 0.0065 (0.6); 0.0086 (1.1) I-91: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4841 (3.1); 8.4772 (3.2); 8.3609 (1.6); 8.3571 (3.1); 8.3536 (1.7); 8.0380 (1.2); 8.0360 (1.4); 8.0334 (1.5); 8.0313 (1.4); 8.0259 (1.3); 8.0238 (1.4); 8.0212 (1.5); 8.0191 (1.4); 7.7681 (1.1); 7.7633 (1.1); 7.7497 (1.2); 7.7474 (1.6); 7.7450 (1.3); 7.7427 (1.6); 7.7291 (1.6); 7.7243 (1.6); 7.6514 (1.7); 7.6491 (3.0); 7.6467 (1.9); 7.6308 (1.3); 7.6284 (2.1); 7.6261 (1.2); 7.5152 (1.3); 7.5109 (1.4); 7.5083 (1.4); 7.5040 (1.3); 7.4927 (1.3); 7.4884 (1.4); 7.4857 (1.4); 7.4814 (1.3); 7.2623 (10.0); 7.1034 (1.4); 7.1008 (1.5); 7.0913 (1.4); 7.0886 (1.4); 7.0851 (1.4); 7.0824 (1.4); 7.0729 (1.4); 7.0703 (1.4); 5.2574 (0.8); 5.2400 (2.9); 5.2226 (3.0); 5.2052 (0.8); 4.2945 (0.9); 4.2881 (1.0); 4.2858 (0.5); 4.2766 (3.0); 4.2704 (3.0); 4.2588 (3.1); 4.2526 (3.0); 4.2410 (1.0); 4.2349 (1.0); 1.7179 (11.1); 1.7005 (11.0); 1.3054 (7.5); 1.2876 (16.0); 1.2698 (7.4); 0.0002 (15.1); 0.0085 (0.5) I-92: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2153 (1.1); 8.2133 (0.9); 8.2112 (0.9); 8.2091 (1.2); 8.2073 (0.8); 8.0826 (0.6); 8.0805 (0.7); 8.0779 (0.8); 8.0758 (0.7); 8.0704 (0.7); 8.0684 (0.8); 8.0658 (0.8); 8.0637 (0.8); 7.8637 (0.6); 7.8575 (0.6); 7.8449 (0.7); 7.8426 (0.8); 7.8387 (0.8); 7.8364 (0.8); 7.8238 (0.7); 7.8176 (0.7); 7.8057 (0.6); 7.8010 (0.6); 7.7874 (0.7); 7.7851 (1.0); 7.7827 (0.7); 7.7804 (1.0); 7.7668 (1.0); 7.7621 (1.0); 7.7060 (0.9); 7.7036 (1.6); 7.7013 (1.0); 7.6854 (0.6); 7.6830 (1.0); 7.6807 (0.6); 7.2631 (7.7); 7.1452 (0.7); 7.1426 (0.8); 7.1331 (0.7); 7.1304 (0.8); 7.1269 (0.8); 7.1243 (0.8); 7.1148 (0.8); 7.1121 (0.9); 7.0094 (0.8); 7.0078 (0.8); 7.0020 (0.8); 7.0004 (0.9); 6.9882 (0.8); 6.9867 (0.8); 6.9808 (0.8); 6.9793 (0.8); 5.3006 (1.3); 4.8618 (8.2); 3.6806 (16.0); 2.6050 (3.3); 2.5917 (3.2); 1.5888 (1.5); 1.3186 (5.8); 1.3017 (5.8); 0.0002 (11.0) I-93: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1976 (2.5); 8.1914 (2.6); 8.0650 (1.5); 8.0631 (1.6); 8.0603 (1.8); 8.0584 (1.6); 8.0528 (1.7); 8.0509 (1.8); 8.0482 (1.8); 8.0464 (1.6); 7.8583 (1.3); 7.8522 (1.3); 7.8393 (1.5); 7.8373 (1.6); 7.8331 (1.6); 7.8311 (1.6); 7.8183 (1.4); 7.8121 (1.3); 7.7691 (1.2); 7.7644 (1.2); 7.7507 (1.4); 7.7484 (1.9); 7.7460 (1.5); 7.7438 (1.8); 7.7302 (1.9); 7.7254 (1.9); 7.6649 (2.1); 7.6627 (3.6); 7.6604 (2.1); 7.6442 (1.5); 7.6421 (2.4); 7.6398 (1.4); 7.2609 (37.0); 7.1145 (1.6); 7.1119 (1.6); 7.1024 (1.6); 7.0997 (1.6); 7.0962 (1.7); 7.0936 (1.5); 7.0841 (1.5); 7.0814 (1.5); 6.9975 (2.0); 6.9902 (1.9); 6.9765 (1.8); 6.9691 (1.8); 5.3002 (6.6); 5.0017 (16.0); 4.3332 (0.5); 4.3176 (2.3); 4.2984 (3.3); 4.2919 (0.7); 4.2822 (1.2); 4.1967 (1.3); 4.1810 (3.4); 4.1771 (2.0); 4.1618 (5.8); 4.1541 (1.3); 4.1515 (1.2); 4.1453 (1.1); 3.9016 (0.9); 3.8846 (1.6); 3.8807 (1.6); 3.8681 (1.1); 3.8638 (2.6); 3.8473 (1.3); 3.8124 (1.2); 3.7947 (1.7); 3.7788 (1.4); 3.7743 (1.2); 3.7581 (0.8); 2.0003 (0.7); 1.9877 (0.7); 1.9796 (0.9); 1.9653 (0.8); 1.9499 (0.7); 1.9350 (0.7); 1.9237 (0.7); 1.9196 (1.0); 1.9149 (0.9); 1.9071 (2.0); 1.9026 (1.3); 1.8990 (1.2); 1.8903 (1.9); 1.8863 (1.6); 1.8726 (0.9); 1.8691 (1.3); 1.6458 (0.9); 1.6413 (0.5); 1.6322 (0.7); 1.6241 (0.8); 1.6152 (0.8); 1.5974 (0.7); 1.5487 (8.9); 0.0079 (1.4); 0.0002 (50.3); 0.0085 (1.9) I-94: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): = 8.2765 (1.2); 8.2708 (1.3); 8.1417 (0.8); 8.1390 (0.9); 8.1295 (0.9); 8.1268 (0.9); 8.0737 (0.8); 8.0677 (0.7); 8.0145 (0.6); 8.0098 (0.6); 7.9942 (0.9); 7.9896 (0.9); 7.9753 (0.8); 7.9707 (0.7); 7.6634 (1.6); 7.6429 (1.4); 7.3508 (0.8); 7.3485 (0.8); 7.3386 (0.7); 7.3364 (0.8); 7.3321 (0.8); 7.3298 (0.7); 7.3201 (0.8); 7.3177 (0.7); 7.2963 (0.8); 7.2899 (0.9); 7.2750 (0.8); 7.2684 (0.8); 5.1911 (1.5); 5.1736 (1.5); 3.3189 (16.0); 2.5238 (0.7); 2.5191 (1.0); 2.5103 (18.0); 2.5057 (40.1); 2.5012 (56.5); 2.4966 (40.2); 2.4921 (18.2); 1.9884 (1.1); 1.5950 (4.6); 1.5776 (4.6); 1.3554 (0.8); 1.2356 (0.8); 1.1745 (0.6); 0.0080 (1.3); 0.0002 (50.2); 0.0085 (1.5) I-95: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2023 (1.1); 8.1961 (1.2); 8.0763 (0.6); 8.0744 (0.7); 8.0717 (0.7); 8.0698 (0.7); 8.0642 (0.7); 8.0623 (0.7); 8.0595 (0.7); 8.0577 (0.7); 7.8609 (0.6); 7.8547 (0.5); 7.8419 (0.6); 7.8398 (0.7); 7.8357 (0.7); 7.8336 (0.7); 7.8209 (0.6); 7.8147 (0.6); 7.7755 (0.5); 7.7707 (0.5); 7.7570 (0.6); 7.7548 (0.8); 7.7523 (0.7); 7.7501 (0.8); 7.7365 (0.8); 7.7317 (0.8); 7.6538 (0.9); 7.6517 (1.5); 7.6496 (0.9); 7.6332 (0.6); 7.6311 (1.1); 7.6289 (0.6); 7.2612 (14.2); 7.1232 (0.7); 7.1206 (0.7); 7.1110 (0.6); 7.1085 (0.7); 7.1048 (0.7); 7.1023 (0.7); 7.0927 (0.6); 7.0901 (0.6); 6.9979 (0.8); 6.9917 (0.8); 6.9779 (0.7); 6.9706 (0.8); 4.9783 (7.7); 4.4228 (2.0); 4.4059 (4.1); 4.3890 (2.1); 2.7825 (2.2); 2.7657 (4.4); 2.7487 (2.1); 2.1441 (16.0); 1.5776 (0.9); 0.0002 (17.6); 0.0085 (0.6) I-96: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2002 (1.1); 8.1941 (1.2); 8.0656 (0.6); 8.0629 (0.7); 8.0535 (0.7); 8.0508 (0.7); 7.8599 (0.5); 7.8537 (0.5); 7.8408 (0.6); 7.8388 (0.7); 7.8347 (0.7); 7.8327 (0.6); 7.8199 (0.6); 7.8137 (0.6); 7.7512 (0.6); 7.7490 (0.8); 7.7466 (0.6); 7.7444 (0.7); 7.7307 (0.7); 7.7260 (0.7); 7.6545 (1.4); 7.6339 (1.0); 7.2613 (9.9); 7.1153 (0.6); 7.1128 (0.6); 7.1031 (0.6); 7.1006 (0.6); 7.0970 (0.7); 7.0945 (0.6); 7.0849 (0.6); 7.0823 (0.6); 6.9969 (0.8); 6.9896 (0.8); 6.9757 (0.7); 6.9684 (0.8); 5.0026 (7.3); 4.3973 (1.8); 4.3893 (1.0); 4.3858 (1.9); 4.3819 (1.0); 4.3741 (2.0); 3.6510 (2.1); 3.6431 (1.0); 3.6393 (2.0); 3.6357 (1.1); 3.6277 (2.0); 3.3793 (16.0); 0.0002 (12.0) I-97: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2122 (1.2); 8.2082 (1.0); 8.2060 (1.3); 8.0905 (0.7); 8.0885 (0.8); 8.0859 (0.9); 8.0838 (0.8); 8.0784 (0.8); 8.0763 (0.9); 8.0737 (0.9); 8.0717 (0.8); 7.8644 (0.7); 7.8582 (0.7); 7.8456 (0.8); 7.8433 (0.8); 7.8394 (0.8); 7.8372 (0.8); 7.8245 (0.8); 7.8183 (0.7); 7.8093 (0.6); 7.8046 (0.6); 7.7910 (0.7); 7.7887 (1.0); 7.7863 (0.8); 7.7840 (1.0); 7.7704 (1.0); 7.7657 (1.0); 7.7121 (1.0); 7.7097 (1.9); 7.7075 (1.2); 7.6915 (0.7); 7.6891 (1.2); 7.6868 (0.7); 7.2617 (15.3); 7.1504 (0.9); 7.1477 (0.9); 7.1382 (0.8); 7.1356 (0.9); 7.1321 (0.9); 7.1294 (0.9); 7.1199 (0.9); 7.1173 (0.8); 7.0091 (0.9); 7.0077 (0.9); 7.0017 (0.9); 7.0003 (0.9); 6.9880 (0.9); 6.9866 (0.9); 6.9806 (0.9); 6.9792 (0.9); 5.3003 (6.8); 4.9460 (7.7); 4.1838 (3.5); 4.1704 (3.5); 3.7928 (16.0); 1.5619 (8.1); 1.2557 (0.5); 0.0080 (0.5); 0.0002 (20.8); 0.0085 (0.8) I-98: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): = 8.2778 (3.2); 8.2716 (3.4); 8.1260 (1.9); 8.1241 (2.1); 8.1214 (2.4); 8.1195 (2.1); 8.1138 (2.0); 8.1120 (2.3); 8.1093 (2.3); 8.1074 (2.1); 8.0448 (1.4); 8.0386 (1.3); 8.0238 (2.0); 8.0177 (2.0); 8.0040 (1.5); 7.9979 (3.1); 7.9932 (1.6); 7.9792 (2.1); 7.9774 (2.3); 7.9746 (2.0); 7.9727 (2.1); 7.9588 (2.0); 7.9540 (1.9); 7.6868 (4.1); 7.6662 (3.7); 7.3089 (2.2); 7.3020 (4.2); 7.2921 (2.1); 7.2894 (3.4); 7.2862 (3.1); 7.2831 (2.9); 7.2737 (2.0); 7.2713 (1.9); 4.9361 (16.0); 4.0561 (0.5); 4.0382 (1.7); 4.0205 (1.7); 4.0027 (0.6); 3.3224 (3.0); 2.5246 (0.7); 2.5199 (1.0); 2.5112 (17.3); 2.5066 (38.2); 2.5021 (53.5); 2.4975 (37.8); 2.4929 (16.9); 1.9889 (7.4); 1.9094 (3.8); 1.1925 (2.0); 1.1747 (4.0); 1.1569 (2.0); 0.0080 (1.2); 0.0002 (45.3); 0.0085 (1.3) I-99: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.1584 (2.0); 8.1520 (2.2); 8.1026 (1.4); 8.1000 (1.4); 8.0878 (1.4); 7.8516 (0.8); 7.8459 (0.7); 7.8316 (1.2); 7.8118 (0.8); 7.8056 (0.8); 7.7909 (1.1); 7.7862 (1.0); 7.7704 (1.5); 7.7659 (1.4); 7.7517 (1.4); 7.7470 (1.3); 7.6111 (2.7); 7.5906 (2.1); 7.2605 (66.6); 7.1759 (1.3); 7.1637 (1.3); 7.1599 (1.2); 7.1453 (1.2); 6.9948 (1.6); 6.9869 (1.5); 6.9789 (1.2); 6.9730 (1.5); 6.9667 (1.4); 5.0311 (13.8); 5.0208 (0.9); 5.0075 (0.6); 4.9719 (0.6); 4.8594 (0.9); 3.8864 (1.1); 3.1157 (0.5); 2.2716 (1.8); 1.4322 (16.0); 1.2540 (2.8); 1.2224 (0.7); 0.8796 (0.5); 0.0690 (0.9); 0.0080 (2.0); 0.0002 (81.2); 0.0085 (2.6) II-01: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2147 (1.1); 8.2104 (1.4); 8.2070 (1.2); 8.2026 (1.2); 8.1992 (1.5); 8.1983 (1.5); 8.1949 (1.2); 8.0912 (2.0); 8.0892 (1.6); 8.0870 (1.6); 8.0849 (2.1); 8.0832 (1.5); 7.8797 (1.0); 7.8751 (1.0); 7.8605 (1.2); 7.8563 (1.6); 7.8524 (1.2); 7.8378 (1.2); 7.8332 (1.1); 7.7939 (1.1); 7.7876 (1.0); 7.7754 (1.2); 7.7727 (1.3); 7.7691 (1.2); 7.7665 (1.3); 7.7542 (1.1); 7.7479 (1.1); 7.3178 (1.2); 7.3150 (1.3); 7.3057 (1.2); 7.3029 (1.3); 7.2986 (1.2); 7.2958 (1.2); 7.2864 (1.2); 7.2836 (1.2); 7.2621 (17.1); 6.9957 (1.4); 6.9942 (1.4); 6.9882 (1.4); 6.9868 (1.4); 6.9745 (1.3); 6.9730 (1.4); 6.9670 (1.4); 6.9655 (1.4); 4.8917 (15.2); 4.3018 (1.9); 4.2840 (6.0); 4.2662 (6.1); 4.2484 (2.0); 2.0455 (0.6); 1.5590 (7.9); 1.5581 (8.4); 1.3141 (7.6); 1.2963 (16.0); 1.2877 (0.5); 1.2784 (7.7); 1.2644 (0.6); 1.2596 (0.7); 0.8819 (0.9); 0.0080 (0.6); 0.0002 (22.3); 0.0085 (0.7) II-03: .sup.1H-NMR(599.6 MHz, CDCl3): = 8.2192 (7.4); 8.2115 (7.3); 8.1073 (11.4); 8.1034 (11.3); 7.9010 (3.7); 7.8981 (3.7); 7.8856 (7.1); 7.8730 (3.9); 7.8702 (3.6); 7.7990 (3.6); 7.7949 (3.6); 7.7848 (5.7); 7.7825 (5.5); 7.7725 (3.8); 7.7684 (3.4); 7.3295 (5.8); 7.3212 (6.1); 7.3169 (5.9); 7.3087 (5.3); 7.2638 (14.2); 7.0023 (6.5); 6.9979 (6.5); 6.9881 (6.3); 6.9837 (6.1); 5.9493 (0.3); 5.2999 (12.4); 5.0641 (0.3); 4.9612 (50.0); 2.1801 (2.2); 1.3126 (0.7); 1.3015 (1.4); 1.2897 (1.7); 1.2798 (1.6); 1.2652 (3.6); 0.8932 (3.4); 0.8817 (7.7); 0.8697 (3.7); 0.0001 (17.0) II-05: .sup.1H-NMR(599.6 MHz, CDCl3): = 8.1957 (8.6); 8.1880 (8.5); 8.0835 (12.3); 8.0800 (12.8); 7.8348 (4.0); 7.8321 (4.4); 7.8195 (8.3); 7.8069 (4.3); 7.8042 (4.4); 7.7761 (3.9); 7.7721 (4.2); 7.7621 (6.7); 7.7597 (6.7); 7.7497 (4.1); 7.7456 (4.0); 7.2948 (6.5); 7.2866 (6.9); 7.2828 (6.7); 7.2740 (6.0); 7.2628 (23.5); 6.9817 (7.2); 6.9773 (7.4); 6.9676 (6.9); 6.9631 (6.9); 5.1781 (3.4); 5.1665 (10.9); 5.1549 (10.9); 5.1433 (3.4); 4.3424 (0.4); 4.3306 (0.3); 4.2776 (0.5); 4.2656 (1.4); 4.2596 (4.0); 4.2557 (4.8); 4.2477 (11.6); 4.2439 (12.5); 4.2358 (11.9); 4.2321 (12.2); 4.2240 (4.5); 4.2203 (4.1); 4.2140 (1.3); 4.2021 (0.4); 4.1278 (0.4); 4.1158 (0.4); 2.0443 (1.4); 1.6935 (42.5); 1.6819 (42.0); 1.6011 (0.4); 1.5896 (0.6); 1.5719 (39.4); 1.3895 (0.4); 1.3777 (0.8); 1.3660 (0.5); 1.3002 (1.1); 1.2766 (25.3); 1.2647 (50.0); 1.2529 (25.0); 1.2157 (0.3); 1.2037 (0.4); 0.8933 (2.0); 0.8819 (4.4); 0.8699 (2.2); 0.0001 (32.1) II-09: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.5139 (1.5); 8.5030 (1.5); 8.4435 (1.9); 8.1949 (2.9); 8.1891 (2.9); 7.7413 (1.0); 7.7352 (1.0); 7.7205 (1.5); 7.7145 (1.5); 7.7016 (1.1); 7.6955 (1.0); 7.4858 (1.4); 7.4645 (1.6); 7.2926 (1.3); 7.2808 (1.5); 7.2718 (1.6); 7.2608 (82.8); 7.0153 (1.8); 7.0081 (1.9); 6.9942 (1.7); 6.9867 (1.7); 4.9214 (16.0); 4.3124 (1.9); 4.2945 (6.0); 4.2766 (6.0); 4.2589 (2.0); 2.9572 (0.9); 2.8845 (0.7); 1.5848 (2.3); 1.3288 (6.7); 1.3110 (13.5); 1.2932 (6.6); 0.0080 (1.2); 0.0002 (43.2); 0.0084 (1.4) II-36: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2052 (0.5); 8.2018 (0.7); 8.2008 (0.7); 8.1975 (0.6); 8.1931 (0.6); 8.1896 (0.7); 8.1888 (0.8); 8.1853 (0.6); 8.0862 (1.0); 8.0841 (0.8); 8.0820 (0.8); 8.0799 (1.1); 8.0781 (0.7); 7.8409 (0.6); 7.8362 (0.6); 7.8216 (0.6); 7.8175 (0.8); 7.8135 (0.6); 7.7989 (0.6); 7.7943 (0.6); 7.7832 (0.6); 7.7769 (0.6); 7.7646 (0.6); 7.7619 (0.7); 7.7583 (0.6); 7.7557 (0.6); 7.7434 (0.6); 7.7371 (0.6); 7.3055 (0.7); 7.3027 (0.7); 7.2933 (0.7); 7.2906 (0.7); 7.2862 (0.6); 7.2834 (0.6); 7.2741 (0.6); 7.2713 (0.6); 7.2622 (8.3); 6.9897 (0.7); 6.9882 (0.8); 6.9822 (0.8); 6.9807 (0.8); 6.9685 (0.7); 6.9669 (0.7); 6.9610 (0.7); 6.9594 (0.7); 5.2008 (1.5); 5.1833 (1.5); 3.7816 (16.0); 2.0454 (0.9); 1.7016 (6.2); 1.6842 (6.1); 1.5607 (4.6); 1.2596 (0.8); 0.8818 (0.8); 0.0002 (10.6) III-01: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2767 (2.0); 8.2745 (1.5); 8.2724 (1.6); 8.2704 (2.0); 8.2685 (1.3); 8.0783 (2.9); 8.0642 (3.0); 7.7967 (1.1); 7.7905 (1.1); 7.7784 (1.2); 7.7756 (1.3); 7.7721 (1.2); 7.7693 (1.3); 7.7572 (1.2); 7.7510 (1.2); 7.2610 (34.6); 7.1099 (1.4); 7.1083 (1.4); 7.1023 (1.4); 7.1007 (1.4); 7.0887 (1.4); 7.0872 (1.4); 7.0811 (1.4); 7.0795 (1.3); 6.8357 (1.1); 6.8328 (1.3); 6.8311 (1.5); 6.8283 (1.4); 6.8216 (1.0); 6.8187 (1.2); 6.8170 (1.6); 6.8143 (1.5); 6.7998 (2.1); 6.7966 (2.8); 6.7932 (1.6); 4.9354 (14.4); 4.3306 (1.8); 4.3128 (5.9); 4.2950 (6.0); 4.2772 (1.9); 2.0455 (0.9); 1.5450 (8.2); 1.3469 (7.6); 1.3291 (16.0); 1.3113 (7.5); 1.2641 (0.7); 1.2597 (1.0); 0.8820 (1.6); 0.8643 (0.6); 0.0080 (1.2); 0.0002 (46.5); 0.0085 (1.3) III-02: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.1557 (0.6); 8.3798 (3.0); 8.3736 (3.1); 8.1842 (4.4); 8.1701 (4.5); 8.1164 (1.3); 8.1100 (1.2); 8.0969 (1.6); 8.0952 (1.8); 8.0908 (1.6); 8.0889 (1.7); 8.0758 (1.4); 8.0695 (1.4); 7.4184 (1.9); 7.4129 (1.9); 7.3971 (1.8); 7.3917 (1.8); 7.0277 (1.4); 7.0233 (2.1); 7.0201 (1.7); 7.0137 (1.4); 7.0093 (2.2); 7.0061 (1.8); 6.9802 (3.7); 4.9454 (12.8); 4.0554 (1.1); 4.0377 (3.4); 4.0199 (3.4); 4.0021 (1.1); 3.3185 (43.8); 2.6790 (0.6); 2.6744 (1.3); 2.6698 (1.8); 2.6652 (1.3); 2.6605 (0.6); 2.5342 (1.0); 2.5294 (1.5); 2.5236 (5.5); 2.5190 (7.4); 2.5102 (97.6); 2.5056 (219.0); 2.5010 (309.1); 2.4964 (217.1); 2.4918 (96.9); 2.4596 (0.7); 2.4561 (0.7); 2.3374 (0.6); 2.3327 (1.3); 2.3281 (1.8); 2.3234 (1.3); 2.3190 (0.6); 1.9885 (16.0); 1.9082 (6.6); 1.1922 (4.7); 1.1744 (9.7); 1.1566 (4.7); 0.1458 (1.0); 0.0294 (0.5); 0.0279 (0.8); 0.0174 (0.5); 0.0150 (0.6); 0.0143 (0.7); 0.0134 (0.7); 0.0127 (0.8); 0.0119 (0.9); 0.0111 (1.0); 0.0102 (1.4); 0.0080 (9.5); 0.0064 (2.4); 0.0055 (2.6); 0.0047 (3.2); 0.0038 (4.5); 0.0002 (322.9); 0.0050 (4.7); 0.0059 (3.4); 0.0067 (2.8); 0.0085 (9.1); 0.0107 (1.2); 0.0115 (1.1); 0.0122 (0.8); 0.0130 (0.6); 0.0394 (0.6); 0.1493 (1.0) III-07: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2904 (1.3); 8.2861 (1.0); 8.2841 (1.3); 8.1193 (1.8); 8.1052 (1.9); 7.7981 (0.7); 7.7918 (0.7); 7.7798 (0.7); 7.7769 (0.8); 7.7735 (0.8); 7.7706 (0.8); 7.7586 (0.7); 7.7523 (0.7); 7.2633 (17.0); 7.1206 (0.9); 7.1193 (0.9); 7.1130 (0.9); 7.1117 (0.9); 7.0995 (0.8); 7.0980 (0.9); 7.0919 (0.8); 7.0905 (0.8); 6.9198 (0.8); 6.9170 (0.9); 6.9153 (0.9); 6.9126 (0.8); 6.9058 (0.7); 6.9030 (0.9); 6.9012 (0.9); 6.8985 (0.8); 6.8176 (1.2); 6.8141 (1.9); 6.8106 (1.1); 5.3011 (4.1); 4.9294 (7.5); 4.1853 (3.5); 4.1720 (3.4); 3.7992 (16.0); 2.0456 (1.8); 1.5772 (7.7); 1.2776 (0.5); 1.2597 (1.1); 1.2419 (0.5); 0.0002 (11.7) III-08: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5203 (1.6); 8.5065 (1.6); 8.2626 (1.2); 8.2606 (1.8); 8.2586 (1.5); 8.2565 (1.5); 8.2544 (1.9); 8.2524 (1.4); 7.7684 (1.0); 7.7622 (1.0); 7.7499 (1.2); 7.7473 (1.3); 7.7437 (1.2); 7.7410 (1.3); 7.7288 (1.2); 7.7225 (1.2); 7.2625 (28.3); 7.0724 (1.3); 7.0708 (1.4); 7.0648 (1.6); 7.0632 (1.8); 7.0589 (3.2); 7.0549 (2.3); 7.0513 (1.9); 7.0496 (2.1); 7.0471 (2.4); 7.0434 (4.2); 5.3005 (1.7); 4.9364 (13.7); 4.3247 (1.8); 4.3069 (5.9); 4.2891 (6.0); 4.2713 (2.0); 2.7729 (4.0); 1.3386 (7.7); 1.3208 (16.0); 1.3030 (7.6); 1.2847 (0.5); 0.0079 (0.7); 0.0002 (25.2); 0.0052 (0.5); 0.0085 (0.8) III-09: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.1233 (0.7); 8.5404 (6.3); 8.5364 (4.4); 8.5288 (4.4); 8.5248 (6.5); 8.3405 (3.4); 8.3342 (3.7); 8.0736 (1.5); 8.0674 (1.5); 8.0542 (1.8); 8.0525 (2.0); 8.0480 (1.9); 8.0462 (2.0); 8.0331 (1.6); 8.0268 (1.6); 7.3970 (2.3); 7.3915 (2.3); 7.3757 (2.2); 7.3702 (2.1); 7.1641 (7.8); 7.1602 (5.2); 7.1525 (5.2); 7.1485 (7.8); 5.4145 (0.7); 4.9237 (16.0); 3.6010 (1.0); 3.3361 (9.1); 2.6792 (0.6); 2.6745 (1.4); 2.6698 (1.9); 2.6653 (1.3); 2.6606 (0.6); 2.5643 (7.0); 2.5237 (5.5); 2.5190 (7.1); 2.5102 (102.6); 2.5057 (226.2); 2.5011 (317.8); 2.4965 (217.1); 2.4919 (95.5); 2.3374 (0.6); 2.3327 (1.3); 2.3281 (1.9); 2.3235 (1.3); 2.3189 (0.6); 2.1830 (0.5); 1.9083 (1.3); 1.7596 (1.2); 1.3549 (4.9); 1.2980 (1.0); 1.2584 (1.6); 1.2352 (1.8); 1.1809 (0.5); 0.8568 (0.6); 0.8404 (0.6); 0.0080 (3.3); 0.0002 (131.7); 0.0085 (3.6) III-17: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2900 (1.0); 8.2858 (0.8); 8.2838 (1.1); 8.2369 (1.5); 8.2229 (1.5); 7.7967 (0.5); 7.7905 (0.5); 7.7784 (0.6); 7.7756 (0.7); 7.7721 (0.6); 7.7693 (0.6); 7.7572 (0.6); 7.7509 (0.6); 7.2622 (23.5); 7.2472 (1.5); 7.2431 (1.5); 7.2425 (1.5); 7.1074 (0.7); 7.1059 (0.7); 7.0998 (0.7); 7.0984 (0.7); 7.0862 (0.6); 7.0847 (0.7); 7.0786 (0.7); 7.0771 (0.7); 6.8507 (1.2); 6.8457 (1.1); 6.8367 (1.2); 6.8318 (1.2); 5.3008 (2.4); 4.9451 (6.9); 4.4248 (0.5); 4.4071 (0.5); 4.3977 (1.4); 4.3800 (1.5); 4.3691 (1.4); 4.3554 (1.5); 4.3420 (0.6); 4.3283 (0.5); 3.7264 (5.8); 3.6838 (16.0); 2.8442 (0.7); 2.8304 (0.7); 1.5598 (1.0); 1.2166 (6.4); 1.1985 (8.8); 1.1801 (2.8); 0.0080 (0.5); 0.0002 (20.0); 0.0085 (0.6) III-18: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2943 (1.2); 8.2920 (0.9); 8.2880 (1.2); 8.2667 (1.9); 8.2527 (2.0); 7.7848 (0.6); 7.7785 (0.6); 7.7664 (0.7); 7.7636 (0.7); 7.7602 (0.7); 7.7574 (0.7); 7.7454 (0.6); 7.7391 (0.6); 7.2730 (2.0); 7.2718 (1.9); 7.2681 (2.3); 7.2669 (2.2); 7.2613 (66.1); 7.2571 (1.1); 7.2547 (0.6); 7.1186 (0.9); 7.1110 (0.9); 7.0974 (1.0); 7.0959 (0.9); 7.0898 (1.2); 6.8962 (1.4); 6.8913 (1.4); 6.8822 (1.4); 6.8773 (1.4); 5.3005 (5.6); 4.8910 (7.1); 4.7277 (0.8); 4.7097 (1.2); 4.6916 (0.8); 3.7897 (16.0); 2.0457 (0.9); 1.5610 (0.8); 1.5155 (6.4); 1.4976 (6.4); 1.2598 (0.8); 0.0080 (1.3); 0.0002 (43.5); 0.0085 (1.2) III-19: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2865 (1.7); 8.2806 (1.7); 8.2423 (2.2); 8.2284 (2.2); 7.7914 (0.6); 7.7851 (0.6); 7.7728 (0.9); 7.7702 (1.0); 7.7667 (0.9); 7.7642 (0.9); 7.7518 (0.7); 7.7456 (0.7); 7.2618 (22.0); 7.2373 (2.4); 7.2328 (2.5); 7.1055 (1.1); 7.0987 (1.1); 7.0844 (1.0); 7.0776 (1.0); 6.8606 (1.5); 6.8557 (1.5); 6.8466 (1.5); 6.8417 (1.4); 5.3007 (3.1); 4.9430 (8.9); 4.5290 (2.3); 4.5135 (4.5); 4.4980 (2.3); 3.6977 (16.0); 2.7244 (2.3); 2.7090 (4.5); 2.6934 (2.2); 1.5550 (4.1); 0.0077 (1.0); 0.0002 (18.4); 0.0085 (0.8) III-20: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.8739 (2.0); 8.3010 (4.7); 8.2871 (7.3); 7.7875 (1.5); 7.7666 (2.3); 7.7485 (1.3); 7.5191 (0.9); 7.2606 (138.6); 7.2459 (5.6); 7.1329 (2.3); 7.1119 (2.3); 6.9969 (1.0); 6.8927 (2.9); 6.8787 (2.6); 5.3001 (6.6); 4.9916 (16.0); 4.3623 (1.9); 4.3410 (5.6); 4.3199 (5.6); 4.2984 (2.1); 3.7009 (1.1); 3.6783 (3.4); 2.3863 (1.1); 2.0480 (1.9); 1.2551 (5.1); 0.8813 (1.0); 0.0002 (86.1) III-21: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2761 (1.6); 8.2700 (1.7); 8.2213 (2.2); 8.2074 (2.2); 7.7718 (0.8); 7.7655 (0.8); 7.7533 (1.0); 7.7506 (1.0); 7.7470 (1.0); 7.7444 (1.0); 7.7322 (0.9); 7.7259 (0.9); 7.3382 (2.1); 7.3341 (2.2); 7.2618 (48.0); 7.0931 (1.1); 7.0869 (1.0); 7.0720 (1.1); 7.0657 (0.9); 6.8511 (1.6); 6.8462 (1.6); 6.8371 (1.6); 6.8322 (1.8); 5.3006 (10.2); 5.1282 (8.2); 5.0132 (1.4); 4.1923 (7.1); 4.1629 (1.4); 3.8196 (2.8); 3.7545 (16.0); 3.7263 (1.9); 3.6778 (1.2); 3.1780 (15.4); 3.0640 (2.4); 2.0455 (1.5); 1.5623 (2.7); 1.2775 (0.5); 1.2596 (1.2); 1.1981 (0.9); 1.1800 (0.9); 0.0079 (1.2); 0.0002 (41.9); 0.0085 (1.3) III-22: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2716 (1.1); 8.2695 (0.8); 8.2674 (0.9); 8.2653 (1.1); 8.2244 (1.7); 8.2233 (1.7); 8.2104 (1.8); 8.2093 (1.7); 7.7748 (0.6); 7.7685 (0.6); 7.7563 (0.7); 7.7536 (0.7); 7.7501 (0.7); 7.7473 (0.7); 7.7352 (0.6); 7.7289 (0.6); 7.2610 (18.5); 7.2044 (1.7); 7.2033 (1.8); 7.1995 (1.8); 7.1984 (1.7); 7.1034 (0.8); 7.1018 (0.8); 7.0957 (0.8); 7.0942 (0.8); 7.0822 (0.7); 7.0807 (0.8); 7.0746 (0.8); 7.0731 (0.7); 6.8187 (1.6); 6.8138 (1.5); 6.8047 (1.5); 6.7998 (1.5); 5.3003 (4.6); 5.2557 (1.5); 5.2383 (1.5); 3.8171 (16.0); 1.7238 (6.1); 1.7064 (6.0); 1.5446 (5.7); 0.0079 (0.8); 0.0002 (29.6); 0.0044 (0.7); 0.0085 (0.9) III-23: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 8.3828 (3.2); 8.3765 (3.4); 8.3304 (5.1); 8.3293 (5.1); 8.3165 (5.3); 8.3153 (5.3); 8.1194 (1.3); 8.1132 (1.3); 8.1000 (1.7); 8.0982 (1.8); 8.0938 (1.7); 8.0920 (1.8); 8.0789 (1.4); 8.0726 (1.4); 7.4231 (1.9); 7.4175 (2.0); 7.4017 (2.0); 7.3962 (1.8); 7.3949 (1.8); 7.3413 (5.0); 7.3402 (5.4); 7.3365 (5.5); 7.3353 (5.0); 7.0466 (4.6); 7.0418 (4.3); 7.0327 (4.5); 7.0278 (4.5); 4.9455 (13.8); 4.0555 (1.0); 4.0377 (3.3); 4.0200 (3.4); 4.0022 (1.1); 3.3197 (14.5); 2.6746 (0.7); 2.6700 (1.0); 2.6654 (0.7); 2.5238 (2.6); 2.5191 (3.6); 2.5104 (53.3); 2.5058 (117.6); 2.5012 (165.8); 2.4966 (113.7); 2.4920 (50.1); 2.3329 (0.7); 2.3282 (1.0); 2.3236 (0.7); 1.9886 (16.0); 1.9084 (6.4); 1.1922 (4.8); 1.1744 (9.8); 1.1566 (4.6); 0.0079 (3.5); 0.0063 (0.8); 0.0055 (0.8); 0.0047 (1.0); 0.0039 (1.5); 0.0030 (2.6); 0.0022 (4.6); 0.0002 (126.0); 0.0027 (5.4); 0.0035 (3.7); 0.0043 (2.2); 0.0052 (1.6); 0.0060 (1.4); 0.0068 (1.2); 0.0085 (3.7); 0.0098 (0.8); 0.0107 (0.6) III-24: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2774 (2.2); 8.2755 (1.7); 8.2730 (1.8); 8.2712 (2.3); 8.2274 (3.4); 8.2135 (3.5); 7.7848 (1.1); 7.7785 (1.1); 7.7664 (1.2); 7.7637 (1.4); 7.7601 (1.3); 7.7574 (1.3); 7.7453 (1.2); 7.7390 (1.2); 7.2659 (5.4); 7.2566 (3.4); 7.2559 (3.3); 7.2518 (3.7); 7.1090 (1.5); 7.1076 (1.5); 7.1014 (1.6); 7.1000 (1.5); 7.0878 (1.4); 7.0865 (1.4); 7.0802 (1.5); 7.0789 (1.4); 6.8223 (2.7); 6.8174 (2.6); 6.8083 (2.6); 6.8034 (2.6); 5.3015 (10.6); 4.9365 (15.5); 4.3343 (2.0); 4.3165 (6.4); 4.2987 (6.4); 4.2809 (2.1); 1.5976 (1.8); 1.3536 (7.8); 1.3358 (16.0); 1.3180 (7.5); 0.0002 (7.7) III-25: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.6699 (1.3); 8.5145 (2.9); 8.4960 (3.0); 8.3741 (4.4); 8.3678 (4.5); 8.1583 (6.5); 8.1441 (6.8); 8.1147 (1.8); 8.1085 (1.8); 8.0953 (2.3); 8.0936 (2.5); 8.0891 (2.2); 8.0873 (2.4); 8.0742 (1.9); 8.0679 (1.9); 7.4245 (2.7); 7.4190 (2.7); 7.4046 (2.4); 7.4032 (2.6); 7.3977 (2.6); 7.3964 (2.4); 7.0636 (4.8); 7.0622 (4.9); 7.0059 (2.4); 7.0027 (3.1); 6.9984 (2.1); 6.9918 (2.4); 6.9886 (3.0); 6.9843 (2.1); 6.8707 (0.7); 4.8530 (15.4); 4.3384 (0.5); 4.3203 (2.6); 4.3020 (4.1); 4.2836 (2.7); 4.2656 (0.5); 3.6216 (0.9); 3.6177 (5.2); 3.6155 (2.9); 3.6114 (2.7); 3.6093 (2.0); 3.6074 (3.6); 3.6011 (12.2); 3.5989 (4.2); 3.5949 (3.8); 3.5930 (2.0); 3.5908 (2.7); 3.5866 (2.7); 3.5845 (5.4); 3.5806 (0.9); 3.3208 (25.7); 3.2024 (1.4); 2.6749 (0.6); 2.6703 (0.9); 2.6657 (0.6); 2.5409 (1.9); 2.5241 (2.4); 2.5195 (3.2); 2.5107 (48.1); 2.5061 (105.8); 2.5015 (148.8); 2.4969 (102.1); 2.4923 (44.6); 2.3332 (0.6); 2.3286 (0.9); 2.3239 (0.6); 2.1829 (1.2); 1.9949 (1.1); 1.9086 (0.8); 1.7809 (0.8); 1.7763 (5.3); 1.7686 (4.2); 1.7642 (2.5); 1.7597 (15.2); 1.7549 (2.6); 1.7507 (4.1); 1.7431 (5.2); 1.7385 (0.8); 1.3552 (11.4); 1.3254 (16.0); 1.3072 (15.9); 1.2363 (0.8); 1.0897 (0.6); 1.0743 (0.6); 0.0080 (1.4); 0.0039 (0.7); 0.0022 (1.9); 0.0002 (46.9); 0.0027 (1.9); 0.0034 (1.2); 0.0043 (0.6); 0.0085 (1.2) III-26: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.6543 (1.2); 8.4833 (1.4); 8.4686 (2.9); 8.4537 (1.4); 8.3683 (4.3); 8.3620 (4.4); 8.1613 (6.3); 8.1472 (6.6); 8.1062 (1.7); 8.0999 (1.6); 8.0850 (2.4); 8.0804 (2.2); 8.0788 (2.3); 8.0656 (1.8); 8.0594 (1.8); 7.4229 (2.7); 7.4172 (2.6); 7.4016 (2.6); 7.3959 (2.5); 7.0825 (5.1); 7.0259 (2.4); 7.0227 (3.1); 7.0186 (2.0); 7.0118 (2.3); 7.0086 (3.0); 7.0044 (2.0); 4.8783 (16.0); 3.8523 (8.0); 3.8376 (8.1); 3.6176 (0.8); 3.6072 (0.6); 3.6010 (1.9); 3.5948 (0.7); 3.5865 (0.5); 3.5844 (0.8); 3.3207 (28.0); 2.6747 (0.7); 2.6702 (1.0); 2.6657 (0.7); 2.5239 (2.7); 2.5193 (4.1); 2.5104 (54.6); 2.5059 (116.9); 2.5013 (161.6); 2.4968 (111.6); 2.4922 (49.2); 2.4737 (0.6); 2.4692 (0.7); 2.3331 (0.7); 2.3285 (1.0); 2.3238 (0.7); 1.7762 (0.8); 1.7686 (0.7); 1.7596 (2.4); 1.7506 (0.7); 1.7431 (0.8); 1.3550 (3.8); 0.0080 (1.2); 0.0002 (45.9); 0.0085 (1.3) III-27: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2873 (1.2); 8.2853 (0.9); 8.2831 (0.9); 8.2810 (1.2); 8.0864 (1.6); 8.0724 (1.6); 7.8080 (0.6); 7.8017 (0.6); 7.7896 (0.7); 7.7869 (0.8); 7.7834 (0.7); 7.7806 (0.7); 7.7685 (0.7); 7.7622 (0.7); 7.2627 (17.0); 7.1099 (0.8); 7.1084 (0.8); 7.1023 (0.8); 7.1008 (0.8); 7.0888 (0.8); 7.0872 (0.8); 7.0811 (0.8); 7.0796 (0.8); 6.8565 (0.6); 6.8537 (0.8); 6.8520 (0.9); 6.8492 (0.8); 6.8425 (0.6); 6.8396 (0.7); 6.8379 (0.9); 6.8351 (0.8); 6.8129 (1.2); 6.8096 (1.6); 6.8063 (0.9); 5.3009 (2.2); 4.9395 (8.0); 4.5278 (2.0); 4.5123 (3.8); 4.4969 (2.0); 3.6987 (16.0); 2.7208 (1.9); 2.7054 (3.7); 2.6899 (1.9); 1.5644 (10.0); 0.0002 (11.8) III-28: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2929 (1.1); 8.2908 (0.9); 8.2885 (0.9); 8.2867 (1.2); 8.1171 (1.5); 8.1031 (1.5); 7.8021 (0.6); 7.7958 (0.6); 7.7838 (0.7); 7.7809 (0.7); 7.7775 (0.7); 7.7747 (0.7); 7.7626 (0.6); 7.7563 (0.6); 7.2643 (11.6); 7.1225 (0.8); 7.1211 (0.8); 7.1149 (0.9); 7.1135 (0.8); 7.1013 (1.0); 7.0999 (1.0); 7.0938 (1.1); 7.0924 (1.0); 6.9154 (0.7); 6.9126 (0.8); 6.9108 (0.8); 6.9082 (0.7); 6.9013 (0.6); 6.8985 (0.8); 6.8968 (0.8); 6.8941 (0.7); 6.8166 (1.0); 6.8132 (1.6); 6.8097 (1.0); 5.3014 (4.0); 4.8908 (7.1); 4.7269 (0.8); 4.7088 (1.2); 4.6908 (0.8); 3.7883 (16.0); 2.0458 (1.6); 1.5928 (5.1); 1.5143 (6.4); 1.4964 (6.3); 1.2777 (0.5); 1.2599 (1.1); 0.0002 (8.1) I-127: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2376 (2.6); 8.2356 (2.7); 8.2259 (2.7); 8.2239 (2.7); 8.1668 (4.8); 8.1539 (5.0); 7.4907 (1.7); 7.4871 (1.7); 7.4701 (2.5); 7.4668 (3.3); 7.4637 (2.0); 7.4467 (2.2); 7.4430 (2.1); 7.3144 (2.0); 7.3054 (2.4); 7.3028 (2.2); 7.2938 (3.6); 7.2848 (1.8); 7.2822 (1.8); 7.2732 (1.6); 7.2621 (22.4); 7.0469 (2.1); 7.0429 (3.0); 7.0390 (2.1); 7.0339 (2.2); 7.0300 (3.0); 7.0261 (2.0); 6.8544 (5.3); 5.3339 (1.2); 5.3165 (5.0); 5.2991 (5.2); 5.2819 (1.3); 2.2717 (0.5); 1.6805 (16.0); 1.6702 (2.1); 1.6631 (15.9); 1.6527 (2.0); 1.6361 (1.4); 1.6333 (1.3); 1.6241 (0.9); 1.6176 (2.9); 1.6106 (1.0); 1.6039 (1.1); 1.6011 (1.3); 1.5995 (1.4); 1.5968 (0.9); 1.5832 (0.9); 1.4321 (5.3); 1.2646 (1.8); 0.8987 (1.0); 0.8818 (3.6); 0.8642 (1.4); 0.8268 (1.2); 0.8212 (6.2); 0.8154 (8.6); 0.8143 (8.8); 0.8089 (4.8); 0.8077 (4.7); 0.8033 (5.4); 0.7935 (10.3); 0.7764 (0.5); 0.0080 (0.9); 0.0002 (32.1); 0.0085 (1.0) I-128: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2263 (1.2); 8.2244 (1.4); 8.2226 (1.4); 8.2208 (1.2); 8.2146 (1.3); 8.2127 (1.4); 8.2110 (1.4); 8.2091 (1.2); 8.1564 (2.4); 8.1434 (2.5); 7.5008 (1.1); 7.4971 (1.1); 7.4802 (1.4); 7.4767 (1.8); 7.4737 (1.1); 7.4568 (1.4); 7.4531 (1.3); 7.3167 (1.3); 7.3078 (1.4); 7.3051 (1.3); 7.2961 (2.3); 7.2872 (1.1); 7.2845 (1.1); 7.2755 (1.0); 7.2623 (15.3); 7.0528 (1.1); 7.0492 (1.4); 7.0482 (1.5); 7.0448 (1.1); 7.0398 (1.1); 7.0363 (1.4); 7.0353 (1.4); 7.0318 (1.1); 6.8644 (1.3); 6.8629 (1.6); 6.8597 (2.6); 6.8565 (1.5); 6.8550 (1.3); 4.8811 (14.3); 4.2732 (1.8); 4.2554 (5.6); 4.2375 (5.7); 4.2197 (1.8); 1.6619 (0.5); 1.6607 (0.6); 1.6552 (0.8); 1.6479 (0.6); 1.6412 (1.8); 1.6334 (0.6); 1.6280 (0.6); 1.6262 (0.6); 1.6212 (0.8); 1.6068 (0.5); 1.5698 (3.5); 1.2992 (7.6); 1.2814 (16.0); 1.2636 (7.6); 1.2596 (0.5); 0.8547 (0.5); 0.8516 (1.2); 0.8490 (1.5); 0.8466 (3.1); 0.8430 (2.4); 0.8382 (3.6); 0.8340 (4.7); 0.8328 (4.2); 0.8285 (2.8); 0.8185 (2.1); 0.8143 (2.8); 0.8110 (1.4); 0.8083 (1.4); 0.0079 (0.5); 0.0002 (20.0); 0.0085 (0.6) I-129: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2292 (0.8); 8.2274 (0.9); 8.2256 (0.9); 8.2238 (0.8); 8.2176 (0.8); 8.2157 (1.0); 8.2139 (0.9); 8.2121 (0.8); 8.1574 (1.6); 8.1445 (1.6); 7.5023 (0.7); 7.4986 (0.7); 7.4817 (0.9); 7.4783 (1.1); 7.4752 (0.8); 7.4583 (0.8); 7.4546 (0.8); 7.3199 (0.8); 7.3110 (0.9); 7.3083 (0.9); 7.2993 (1.5); 7.2903 (0.7); 7.2876 (0.7); 7.2787 (0.6); 7.2614 (18.2); 7.0522 (0.7); 7.0478 (1.0); 7.0442 (0.8); 7.0393 (0.7); 7.0356 (0.9); 7.0312 (0.7); 6.8626 (1.0); 6.8594 (1.7); 6.8562 (1.0); 6.8548 (0.9); 4.8996 (8.5); 3.7846 (16.0); 1.6567 (0.5); 1.6405 (1.1); 1.6226 (0.6); 1.5569 (7.6); 0.8341 (11.1); 0.8245 (0.8); 0.8226 (0.8); 0.8181 (2.5); 0.8160 (2.6); 0.8148 (2.6); 0.8114 (0.8); 0.8095 (0.8); 0.0080 (0.6); 0.0002 (23.4); 0.0085 (0.6) I-130: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2560 (0.9); 8.2462 (0.9); 8.2030 (1.2); 8.1900 (1.3); 7.5471 (0.6); 7.5435 (0.6); 7.5264 (0.9); 7.5230 (1.1); 7.5206 (0.8); 7.5034 (0.8); 7.4997 (0.8); 7.3891 (0.6); 7.3800 (0.7); 7.3777 (0.7); 7.3685 (1.1); 7.3594 (0.6); 7.3570 (0.6); 7.2620 (7.4); 7.1054 (0.7); 7.1016 (1.1); 7.0978 (0.8); 7.0925 (0.7); 7.0886 (1.1); 7.0847 (0.7); 6.9137 (1.6); 4.9545 (8.4); 3.8005 (16.0); 1.5626 (2.3); 0.0002 (10.9) I-131: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2750 (1.6); 8.2733 (1.8); 8.2713 (1.9); 8.2697 (1.7); 8.2633 (1.7); 8.2615 (1.9); 8.2596 (1.9); 8.2581 (1.6); 8.1740 (3.2); 8.1610 (3.3); 7.4993 (1.2); 7.4956 (1.3); 7.4787 (1.7); 7.4752 (2.1); 7.4723 (1.5); 7.4554 (1.6); 7.4517 (1.6); 7.3385 (1.6); 7.3294 (1.8); 7.3268 (1.7); 7.3178 (2.8); 7.3088 (1.3); 7.3062 (1.3); 7.2972 (1.2); 7.2626 (13.9); 7.0533 (1.3); 7.0491 (2.0); 7.0454 (1.4); 7.0403 (1.4); 7.0363 (2.0); 7.0324 (1.4); 6.8644 (2.1); 6.8613 (3.4); 6.8583 (2.1); 4.9420 (16.0); 1.6519 (0.8); 1.6462 (1.0); 1.6399 (0.7); 1.6322 (2.0); 1.6256 (0.7); 1.6192 (0.7); 1.6176 (0.9); 1.6120 (1.0); 1.5980 (0.6); 1.4321 (1.6); 0.8307 (1.6); 0.8249 (3.2); 0.8204 (2.5); 0.8090 (3.6); 0.8046 (6.8); 0.8009 (4.3); 0.7945 (2.8); 0.7907 (3.9); 0.7878 (1.9); 0.7854 (1.8); 0.0002 (19.4); 0.0085 (0.6) I-132: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1722 (0.7); 8.1705 (0.8); 8.1686 (0.8); 8.1669 (0.7); 8.1606 (0.7); 8.1587 (0.8); 8.1570 (0.8); 8.1552 (0.8); 8.1489 (1.4); 8.1360 (1.4); 7.5042 (0.6); 7.5005 (0.6); 7.4837 (0.8); 7.4802 (1.1); 7.4769 (0.7); 7.4600 (0.7); 7.4563 (0.7); 7.2932 (0.7); 7.2843 (0.8); 7.2815 (0.7); 7.2726 (1.3); 7.2620 (9.4); 7.2521 (0.6); 7.0450 (0.6); 7.0406 (0.9); 7.0370 (0.7); 7.0321 (0.6); 7.0285 (0.8); 7.0276 (0.8); 7.0240 (0.6); 6.8588 (0.9); 6.8556 (1.5); 6.8525 (0.9); 6.8510 (0.8); 5.2600 (1.5); 5.2426 (1.5); 3.7498 (16.0); 1.6473 (0.5); 1.6399 (0.8); 1.6351 (6.4); 1.6295 (0.8); 1.6269 (0.8); 1.6178 (6.5); 1.6134 (0.7); 1.6057 (0.6); 1.5688 (3.1); 0.8666 (0.5); 0.8633 (1.0); 0.8603 (1.2); 0.8569 (0.8); 0.8533 (1.2); 0.8502 (1.0); 0.8471 (1.2); 0.8438 (0.6); 0.8400 (1.0); 0.8288 (1.1); 0.8225 (1.0); 0.8208 (1.1); 0.8165 (0.7); 0.8146 (0.7); 0.8076 (0.9); 0.8009 (1.1); 0.7950 (0.7); 0.0002 (12.1) I-133: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2092 (1.8); 8.1958 (2.2); 8.1924 (2.5); 8.1794 (2.4); 7.5432 (1.1); 7.5396 (1.1); 7.5224 (1.6); 7.5195 (2.2); 7.5165 (1.4); 7.4993 (1.4); 7.4957 (1.4); 7.3639 (1.2); 7.3549 (1.4); 7.3525 (1.3); 7.3434 (2.1); 7.3343 (1.1); 7.3318 (1.1); 7.3228 (0.9); 7.2615 (15.6); 7.0990 (1.3); 7.0951 (2.2); 7.0913 (1.4); 7.0860 (1.3); 7.0822 (2.1); 7.0784 (1.3); 6.9101 (3.1); 5.2722 (0.9); 5.2548 (3.2); 5.2374 (3.2); 5.2201 (0.9); 4.2525 (1.7); 4.2347 (5.4); 4.2169 (5.7); 4.1992 (1.9); 1.6942 (12.7); 1.6768 (12.6); 1.5601 (3.1); 1.2695 (7.9); 1.2517 (16.0); 1.2339 (7.6); 0.0078 (0.5); 0.0002 (22.5); 0.0085 (0.7) I-135: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1737 (1.3); 8.1718 (1.5); 8.1701 (1.5); 8.1682 (1.4); 8.1621 (1.4); 8.1602 (1.6); 8.1584 (1.6); 8.1566 (1.4); 8.1475 (2.7); 8.1345 (2.8); 7.4992 (1.1); 7.4955 (1.2); 7.4786 (1.4); 7.4753 (2.1); 7.4719 (1.3); 7.4551 (1.4); 7.4513 (1.3); 7.2902 (1.4); 7.2813 (1.5); 7.2785 (1.4); 7.2696 (2.5); 7.2611 (39.8); 7.2491 (1.1); 7.0454 (1.2); 7.0409 (1.6); 7.0374 (1.2); 7.0324 (1.2); 7.0289 (1.6); 7.0244 (1.2); 6.8583 (1.7); 6.8551 (2.8); 6.8520 (1.8); 6.8505 (1.4); 5.2599 (0.8); 5.2426 (3.0); 5.2252 (3.1); 5.2079 (0.8); 4.2326 (2.0); 4.2148 (6.6); 4.1970 (6.7); 4.1793 (2.2); 1.6489 (0.9); 1.6412 (1.1); 1.6313 (12.0); 1.6199 (1.0); 1.6140 (12.3); 1.6071 (1.4); 1.5938 (0.6); 1.5546 (16.0); 1.2635 (7.5); 1.2458 (15.7); 1.2279 (7.3); 0.8906 (0.5); 0.8883 (0.8); 0.8793 (1.0); 0.8766 (1.6); 0.8734 (2.5); 0.8652 (1.7); 0.8634 (1.7); 0.8604 (2.4); 0.8580 (1.4); 0.8520 (1.2); 0.8305 (0.8); 0.8285 (1.1); 0.8241 (0.7); 0.8191 (2.4); 0.8153 (1.9); 0.8075 (1.0); 0.8047 (1.0); 0.7987 (2.2); 0.7936 (1.7); 0.7866 (0.6); 0.0079 (1.3); 0.0002 (49.7); 0.0085 (1.5) I-141: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5112 (1.0); 8.3275 (1.2); 8.2270 (1.5); 8.2155 (1.5); 7.5664 (1.0); 7.5467 (2.0); 7.5432 (1.8); 7.5259 (1.6); 7.5240 (1.6); 7.5224 (1.7); 7.5205 (1.3); 7.5032 (1.4); 7.4996 (1.3); 7.3920 (1.1); 7.3828 (1.3); 7.3806 (1.2); 7.3713 (1.9); 7.3621 (1.0); 7.3598 (1.0); 7.3505 (0.8); 7.2610 (20.9); 4.9413 (14.8); 4.2908 (2.0); 4.2730 (6.3); 4.2552 (6.4); 4.2374 (2.1); 2.7814 (1.8); 1.3027 (7.7); 1.2849 (16.0); 1.2671 (7.6); 0.0080 (1.0); 0.0002 (29.8); 0.0085 (0.9) I-142: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4037 (1.8); 8.3968 (1.8); 8.3139 (0.9); 8.3100 (1.8); 8.3061 (1.0); 8.1684 (0.7); 8.1665 (0.8); 8.1648 (0.9); 8.1630 (0.8); 8.1568 (0.8); 8.1549 (0.9); 8.1531 (0.9); 8.1513 (0.8); 7.4838 (0.6); 7.4801 (0.6); 7.4632 (0.8); 7.4598 (1.2); 7.4564 (0.7); 7.4395 (0.8); 7.4358 (0.8); 7.4252 (0.7); 7.4209 (0.7); 7.4183 (0.7); 7.4140 (0.7); 7.4025 (0.7); 7.3982 (0.8); 7.3956 (0.7); 7.3913 (0.7); 7.2710 (0.8); 7.2625 (10.7); 7.2595 (1.1); 7.2505 (1.4); 7.2416 (0.6); 7.2388 (0.7); 7.2300 (0.6); 5.2366 (1.6); 5.2193 (1.6); 4.4686 (0.6); 4.4572 (0.8); 4.4408 (1.7); 4.4303 (0.8); 4.4244 (0.8); 4.4142 (1.7); 4.3983 (0.8); 4.3865 (0.6); 3.6689 (16.0); 2.6727 (1.5); 2.6563 (3.0); 2.6403 (1.4); 1.6245 (6.0); 1.6071 (6.3); 1.5994 (0.8); 1.5860 (3.7); 1.5782 (0.6); 1.5725 (0.6); 1.5652 (0.6); 0.8330 (1.0); 0.8290 (1.4); 0.8210 (1.5); 0.8158 (1.2); 0.8083 (0.8); 0.7994 (1.1); 0.7917 (1.2); 0.7872 (0.8); 0.7785 (0.7); 0.7713 (1.3); 0.7658 (0.9); 0.0002 (13.9) I-143: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4390 (3.2); 8.4321 (3.3); 8.2812 (2.0); 8.2776 (3.4); 8.2741 (2.0); 7.5874 (1.0); 7.5723 (1.1); 7.5659 (1.6); 7.5509 (1.5); 7.5455 (1.3); 7.5305 (1.0); 7.4219 (1.2); 7.4175 (1.3); 7.4151 (1.4); 7.4107 (1.2); 7.3998 (1.2); 7.3954 (1.4); 7.3930 (1.4); 7.3886 (1.2); 7.2625 (13.3); 6.8936 (1.2); 6.8873 (1.3); 6.8843 (1.3); 6.8780 (1.2); 6.8717 (1.1); 6.8655 (1.2); 6.8625 (1.2); 6.8562 (1.1); 5.1539 (0.7); 5.1501 (2.2); 5.1460 (3.4); 5.1420 (2.4); 5.0559 (2.5); 5.0537 (3.1); 5.0516 (3.1); 5.0494 (2.4); 4.9412 (0.6); 4.9182 (1.2); 4.9109 (16.0); 4.2887 (2.2); 4.2708 (6.4); 4.2665 (1.3); 4.2530 (6.3); 4.2486 (1.3); 4.2352 (2.1); 1.9291 (8.0); 1.9270 (11.3); 1.9258 (11.6); 1.9236 (8.8); 1.5869 (4.1); 1.3102 (7.4); 1.3048 (1.4); 1.2924 (15.1); 1.2868 (1.9); 1.2746 (7.3); 1.2689 (1.0); 0.0079 (0.6); 0.0002 (18.3); 0.0084 (0.6) I-147: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5479 (0.6); 8.3498 (0.7); 8.2082 (1.0); 8.2061 (1.1); 8.2038 (1.2); 8.2016 (1.1); 8.1961 (1.1); 8.1938 (1.2); 8.1919 (1.2); 8.1896 (1.0); 7.9352 (0.7); 7.9306 (0.7); 7.9175 (0.6); 7.9147 (1.8); 7.9102 (1.8); 7.8972 (2.1); 7.8928 (2.1); 7.8876 (1.8); 7.8852 (2.2); 7.8842 (2.4); 7.8817 (1.9); 7.8672 (0.7); 7.8650 (0.8); 7.5403 (0.8); 7.5360 (0.9); 7.5336 (1.0); 7.5293 (0.8); 7.5185 (0.8); 7.5142 (1.0); 7.5117 (0.9); 7.5075 (0.8); 7.3437 (1.2); 7.3401 (1.2); 7.3316 (1.2); 7.3277 (1.3); 7.3263 (1.4); 7.3225 (1.1); 7.3142 (1.1); 7.3104 (1.1); 7.2631 (11.1); 5.3008 (10.8); 4.4158 (16.0); 4.2758 (2.1); 4.2580 (6.7); 4.2401 (6.8); 4.2223 (2.2); 1.5815 (1.8); 1.2842 (7.5); 1.2664 (15.6); 1.2485 (7.3); 0.0702 (1.4); 0.0002 (15.8) I-148: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.9537 (2.0); 8.6263 (5.6); 8.6193 (5.6); 8.3765 (3.0); 8.3725 (5.6); 8.3686 (2.7); 8.1359 (1.2); 8.1203 (1.3); 8.1138 (2.4); 8.0982 (2.4); 8.0917 (1.3); 8.0761 (1.2); 7.8388 (1.8); 7.8344 (1.9); 7.8319 (1.9); 7.8275 (1.6); 7.8148 (1.9); 7.8104 (2.1); 7.8079 (1.8); 7.8035 (1.6); 7.3160 (1.3); 7.3096 (1.8); 7.3078 (1.7); 7.3013 (1.4); 7.2939 (1.3); 7.2875 (1.6); 7.2857 (1.5); 7.2794 (1.1); 4.7878 (16.0); 3.3202 (12.8); 2.6706 (0.5); 2.5245 (1.4); 2.5197 (2.2); 2.5110 (29.9); 2.5065 (65.8); 2.5018 (91.4); 2.4972 (63.6); 2.4926 (27.7); 1.7598 (0.6); 1.7055 (0.6); 1.6925 (1.4); 1.6845 (1.4); 1.6796 (0.9); 1.6715 (2.9); 1.6637 (0.8); 1.6583 (1.5); 1.6504 (1.5); 1.6374 (0.7); 1.3558 (2.8); 0.7629 (1.4); 0.7519 (3.0); 0.7465 (4.0); 0.7419 (1.8); 0.7373 (2.3); 0.7309 (3.2); 0.7251 (3.8); 0.7164 (1.9); 0.6414 (2.0); 0.6324 (4.1); 0.6276 (4.2); 0.6196 (4.0); 0.6141 (3.4); 0.6030 (1.3); 0.0080 (1.5); 0.0002 (51.9); 0.0085 (1.4) I-149: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4521 (2.0); 8.4454 (2.0); 8.3218 (2.2); 7.5768 (1.0); 7.5618 (1.0); 7.5561 (1.4); 7.5411 (1.5); 7.5347 (1.1); 7.5197 (1.1); 7.4614 (0.9); 7.4570 (1.1); 7.4546 (1.1); 7.4503 (1.0); 7.4390 (1.0); 7.4347 (1.1); 7.4322 (1.1); 7.4279 (0.9); 7.2621 (13.7); 6.8718 (1.1); 6.8656 (1.2); 6.8624 (1.2); 6.8563 (1.1); 6.8500 (1.0); 6.8439 (1.1); 6.8407 (1.1); 6.8345 (1.0); 4.8702 (15.8); 4.2824 (2.0); 4.2646 (6.2); 4.2468 (6.2); 4.2290 (2.0); 1.6001 (0.7); 1.5937 (1.0); 1.5865 (0.6); 1.5801 (1.9); 1.5694 (3.4); 1.5596 (1.1); 1.5457 (0.6); 1.3099 (7.8); 1.2921 (16.0); 1.2743 (7.6); 0.8819 (0.5); 0.8266 (1.4); 0.8209 (3.2); 0.8166 (2.5); 0.8137 (1.8); 0.8081 (4.5); 0.8028 (4.3); 0.7985 (1.6); 0.7881 (2.1); 0.7824 (2.5); 0.7770 (1.7); 0.0080 (0.6); 0.0002 (20.9); 0.0085 (0.7) I-150: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5332 (3.1); 8.5263 (3.1); 8.3396 (1.7); 8.3359 (3.1); 8.3322 (1.7); 8.1937 (1.3); 8.1916 (1.4); 8.1892 (1.5); 8.1871 (1.4); 8.1816 (1.3); 8.1794 (1.4); 8.1772 (1.5); 8.1749 (1.3); 7.9220 (0.9); 7.9174 (0.8); 7.9039 (0.9); 7.9015 (1.9); 7.8996 (1.0); 7.8969 (1.8); 7.8835 (2.1); 7.8790 (2.0); 7.8648 (2.0); 7.8618 (3.0); 7.8594 (2.2); 7.8443 (1.0); 7.8419 (1.2); 7.8389 (0.7); 7.5160 (1.3); 7.5116 (1.4); 7.5091 (1.4); 7.5047 (1.3); 7.4940 (1.3); 7.4896 (1.4); 7.4872 (1.3); 7.4828 (1.2); 7.3154 (1.4); 7.3122 (1.4); 7.3034 (1.4); 7.3000 (1.4); 7.2975 (1.5); 7.2943 (1.4); 7.2855 (1.4); 7.2822 (1.3); 7.2633 (11.8); 5.3005 (11.4); 4.4155 (10.2); 4.4143 (10.4); 4.2810 (1.9); 4.2631 (6.1); 4.2453 (6.3); 4.2275 (2.0); 1.5970 (0.7); 1.2959 (7.6); 1.2781 (16.0); 1.2602 (7.5); 0.0700 (0.9); 0.0080 (0.5); 0.0002 (17.9) I-151: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4942 (1.7); 8.4873 (1.7); 8.3401 (0.9); 8.3395 (0.9); 8.3358 (1.6); 8.3322 (0.9); 8.1010 (0.7); 8.0989 (0.7); 8.0965 (0.8); 8.0943 (0.7); 8.0890 (0.7); 8.0866 (0.8); 8.0844 (0.8); 8.0821 (0.7); 7.8174 (1.1); 7.8158 (0.5); 7.8128 (1.0); 7.7997 (1.2); 7.7951 (1.2); 7.7840 (1.2); 7.7816 (1.4); 7.7808 (1.5); 7.7783 (1.2); 7.7634 (0.5); 7.7611 (0.6); 7.7602 (0.5); 7.5019 (0.7); 7.4976 (0.8); 7.4951 (0.8); 7.4907 (0.7); 7.4796 (0.7); 7.4752 (0.8); 7.4726 (0.7); 7.4683 (0.7); 7.2626 (5.6); 7.1844 (0.8); 7.1810 (0.8); 7.1722 (0.8); 7.1687 (0.8); 7.1667 (0.9); 7.1633 (0.7); 7.1546 (0.8); 7.1511 (0.7); 3.9599 (8.7); 3.7902 (16.0); 0.0002 (8.4) I-153: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): = 12.7540 (0.8); 8.5944 (5.3); 8.5875 (5.3); 8.3680 (3.0); 8.3638 (5.5); 8.3598 (2.9); 8.1051 (2.0); 8.1032 (2.3); 8.1006 (2.5); 8.0986 (2.3); 8.0931 (2.1); 8.0911 (2.5); 8.0885 (2.5); 8.0865 (2.2); 7.9877 (1.7); 7.9829 (1.5); 7.9689 (2.3); 7.9671 (2.4); 7.9643 (2.0); 7.9624 (2.0); 7.9486 (2.2); 7.9438 (1.8); 7.7980 (1.9); 7.7937 (2.0); 7.7910 (2.0); 7.7868 (1.7); 7.7735 (2.0); 7.7693 (2.2); 7.7666 (1.9); 7.7623 (1.8); 7.7521 (4.0); 7.7336 (2.1); 7.7315 (3.4); 7.7196 (0.5); 7.2862 (2.1); 7.2838 (2.1); 7.2740 (2.0); 7.2716 (2.2); 7.2677 (2.2); 7.2653 (1.9); 7.2555 (2.0); 7.2530 (1.9); 5.7562 (7.2); 4.1401 (1.1); 4.1223 (1.1); 4.0291 (2.1); 3.9771 (16.0); 3.3198 (6.2); 2.6706 (0.5); 2.5241 (1.3); 2.5194 (1.9); 2.5106 (29.6); 2.5061 (65.1); 2.5015 (91.0); 2.4969 (64.5); 2.4924 (29.2); 1.6965 (0.5); 1.6833 (1.2); 1.6756 (1.2); 1.6702 (0.8); 1.6625 (2.5); 1.6548 (0.8); 1.6492 (1.3); 1.6416 (1.3); 1.6284 (0.7); 1.1947 (1.2); 1.1770 (2.6); 1.1592 (1.3); 0.7219 (1.3); 0.7112 (3.7); 0.7062 (3.8); 0.7010 (1.8); 0.6960 (1.9); 0.6903 (3.8); 0.6853 (3.6); 0.6752 (1.4); 0.3328 (1.6); 0.3226 (4.1); 0.3179 (4.6); 0.3094 (4.3); 0.3045 (4.3); 0.2940 (1.4); 0.0080 (2.2); 0.0002 (80.7); 0.0085 (2.5) I-154: .sup.1H-NMR(400.6 MHz, CDCl3): = 7.6210 (0.5); 7.6151 (0.9); 7.6003 (0.9); 7.5939 (0.6); 7.5791 (0.6); 7.5384 (0.8); 7.5181 (0.8); 7.2616 (8.8); 6.9425 (0.6); 6.9360 (0.7); 6.9335 (0.7); 6.9272 (0.6); 6.9207 (0.6); 6.9143 (0.7); 6.9117 (0.7); 6.9055 (0.6); 5.2595 (1.7); 5.2421 (1.7); 5.2248 (0.5); 3.7816 (16.0); 1.7040 (6.9); 1.6866 (6.8); 1.5791 (1.2); 0.0002 (11.4) I-155: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4972 (4.1); 8.4904 (4.1); 8.3133 (4.2); 7.6137 (1.5); 7.5982 (3.1); 7.5935 (3.9); 7.5915 (3.7); 7.5868 (2.0); 7.5765 (3.4); 7.5718 (3.8); 7.5695 (2.4); 7.5650 (1.9); 7.5568 (1.5); 7.2609 (41.7); 6.9416 (1.6); 6.9353 (1.9); 6.9325 (1.8); 6.9262 (1.7); 6.9198 (1.5); 6.9135 (1.7); 6.9106 (1.7); 6.9044 (1.4); 5.3191 (1.2); 5.3017 (4.8); 5.2842 (4.9); 5.2667 (1.2); 1.7482 (16.0); 1.7307 (15.9); 1.7053 (0.8); 1.6879 (0.7); 1.4321 (2.8); 1.2639 (0.5); 0.8819 (0.9); 0.0079 (1.6); 0.0002 (60.9); 0.0085 (1.7) I-156: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4527 (3.7); 8.4458 (3.8); 8.3335 (2.1); 8.3296 (3.8); 8.3259 (2.1); 8.0701 (1.7); 8.0582 (2.1); 7.7570 (1.9); 7.7526 (1.8); 7.7408 (4.6); 7.7371 (4.8); 7.7207 (0.6); 7.4341 (1.1); 7.4291 (1.3); 7.4278 (1.4); 7.4231 (1.1); 7.4112 (1.1); 7.4064 (1.3); 7.4049 (1.3); 7.4002 (1.1); 7.2625 (8.1); 7.1123 (1.2); 7.1073 (1.1); 7.1000 (1.2); 7.0954 (1.9); 7.0915 (1.2); 7.0845 (1.1); 7.0791 (1.0); 4.2622 (2.0); 4.2444 (6.0); 4.2266 (6.1); 4.2088 (2.0); 3.9607 (16.0); 1.6057 (1.0); 1.5980 (1.0); 1.5876 (5.9); 1.5772 (0.6); 1.5715 (1.0); 1.5639 (1.0); 1.5506 (0.5); 1.2992 (6.5); 1.2814 (13.0); 1.2636 (6.4); 0.7819 (1.0); 0.7705 (2.9); 0.7660 (2.8); 0.7614 (1.3); 0.7551 (1.4); 0.7496 (2.9); 0.7451 (2.7); 0.7343 (1.1); 0.4521 (1.2); 0.4406 (3.1); 0.4374 (3.4); 0.4276 (3.0); 0.4241 (3.2); 0.4122 (0.9); 0.0002 (11.5) I-157: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4655 (0.6); 8.4615 (0.6); 8.4536 (0.6); 8.4496 (0.6); 8.4282 (0.8); 8.4215 (0.8); 8.2772 (1.0); 8.1593 (0.7); 8.1549 (0.7); 8.1394 (0.7); 8.1351 (0.7); 7.5277 (0.5); 7.5234 (0.6); 7.5208 (0.6); 7.5165 (0.5); 7.5055 (0.5); 7.5012 (0.6); 7.4987 (0.6); 7.4943 (0.5); 7.4537 (0.5); 7.4417 (0.5); 7.2615 (9.2); 4.9309 (6.8); 4.3566 (1.7); 4.3482 (0.9); 4.3449 (1.7); 4.3412 (0.8); 4.3330 (1.8); 3.6233 (2.0); 3.6150 (0.9); 3.6113 (1.8); 3.6081 (0.9); 3.5996 (1.8); 3.3686 (16.0); 1.5885 (0.8); 0.0002 (13.0) I-158: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4475 (1.6); 8.4407 (1.6); 8.3270 (0.9); 8.3231 (1.6); 8.3193 (0.9); 7.5781 (0.5); 7.5630 (0.6); 7.5568 (0.8); 7.5420 (0.8); 7.5357 (0.6); 7.5207 (0.6); 7.4614 (0.7); 7.4571 (0.7); 7.4545 (0.7); 7.4502 (0.7); 7.4390 (0.7); 7.4346 (0.7); 7.4320 (0.7); 7.4277 (0.6); 7.2624 (10.6); 6.8486 (0.6); 6.8426 (0.6); 6.8392 (0.6); 6.8332 (0.6); 6.8269 (0.5); 6.8208 (0.6); 6.8175 (0.6); 6.8114 (0.5); 5.1992 (1.6); 5.1819 (1.6); 4.4787 (0.6); 4.4671 (0.8); 4.4509 (1.4); 4.4347 (1.5); 4.4189 (1.5); 4.4031 (0.8); 4.3911 (0.6); 3.6753 (16.0); 2.6788 (1.0); 2.6763 (1.0); 2.6627 (1.7); 2.6602 (2.1); 2.6466 (1.0); 2.6442 (1.0); 1.6245 (5.8); 1.6071 (5.8); 1.5801 (1.9); 1.5683 (0.6); 1.5552 (0.9); 1.5340 (0.6); 0.8395 (1.1); 0.8347 (1.4); 0.8268 (1.5); 0.8216 (1.2); 0.8137 (0.8); 0.7935 (0.7); 0.7849 (1.3); 0.7802 (0.9); 0.7724 (0.8); 0.7641 (1.0); 0.7596 (0.8); 0.0002 (13.4) I-159: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.0998 (2.2); 8.6970 (6.9); 8.6900 (7.0); 8.4349 (3.6); 8.4308 (6.6); 8.4272 (3.4); 8.2063 (1.5); 8.1909 (1.6); 8.1842 (3.0); 8.1688 (3.0); 8.1621 (1.7); 8.1467 (1.5); 7.9327 (2.5); 7.9283 (2.6); 7.9258 (2.6); 7.9214 (2.4); 7.9091 (2.7); 7.9047 (2.9); 7.9021 (2.5); 7.8977 (2.4); 7.4069 (1.6); 7.4004 (2.3); 7.3989 (2.3); 7.3923 (1.8); 7.3847 (1.6); 7.3782 (2.0); 7.3702 (1.5); 5.7570 (1.0); 5.1097 (1.2); 5.0924 (5.9); 5.0750 (6.0); 5.0576 (1.2); 3.3211 (12.7); 2.6752 (0.5); 2.6706 (0.7); 2.6660 (0.5); 2.5243 (1.8); 2.5197 (2.6); 2.5110 (37.5); 2.5064 (82.6); 2.5018 (116.3); 2.4972 (81.4); 2.4926 (36.8); 2.4785 (0.6); 2.4737 (0.6); 2.4690 (0.5); 2.3289 (0.7); 1.5898 (16.0); 1.5723 (15.9); 1.3556 (2.8); 1.2795 (0.6); 1.2576 (1.1); 1.2471 (3.2); 0.8750 (1.6); 0.8581 (6.5); 0.8404 (2.2); 0.0079 (3.8); 0.0064 (0.8); 0.0055 (0.9); 0.0046 (1.1); 0.0002 (140.8); 0.0051 (2.4); 0.0059 (2.0); 0.0068 (1.7); 0.0085 (4.4); 0.0115 (0.6); 0.0123 (0.5); 0.0131 (0.5); 0.0282 (0.6) I-160: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4706 (0.7); 8.4669 (0.8); 8.4588 (0.8); 8.4548 (0.8); 8.4305 (1.0); 8.4238 (1.1); 8.2813 (1.2); 8.1624 (0.8); 8.1582 (0.8); 8.1425 (0.9); 8.1384 (0.8); 7.5303 (0.6); 7.5259 (0.7); 7.5234 (0.7); 7.5191 (0.7); 7.5080 (0.7); 7.5037 (0.7); 7.5012 (0.7); 7.4968 (0.6); 7.4599 (0.6); 7.4583 (0.6); 7.4479 (0.6); 7.4463 (0.6); 7.4402 (0.6); 7.4385 (0.6); 7.4282 (0.6); 7.4266 (0.6); 7.2612 (15.6); 4.8830 (8.0); 4.4824 (1.9); 4.4663 (4.2); 4.4502 (2.0); 3.6934 (16.0); 2.6928 (1.9); 2.6767 (4.0); 2.6606 (1.9); 1.5936 (1.1); 0.0079 (0.6); 0.0002 (22.1); 0.0085 (0.6) I-161: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5184 (3.0); 8.5115 (3.1); 8.3842 (1.6); 8.3804 (3.0); 8.3765 (1.6); 7.8207 (3.3); 7.7993 (3.6); 7.5232 (1.2); 7.5189 (1.3); 7.5162 (1.3); 7.5119 (1.2); 7.5007 (1.3); 7.4964 (1.3); 7.4939 (1.3); 7.4896 (1.2); 7.4039 (2.5); 7.4024 (2.6); 7.3824 (2.3); 7.3810 (2.4); 7.2628 (8.0); 5.3003 (1.3); 4.9341 (14.4); 4.3228 (1.9); 4.3050 (6.0); 4.2872 (6.1); 4.2694 (2.0); 2.1741 (16.0); 1.6035 (0.6); 1.3338 (7.7); 1.3160 (15.9); 1.2982 (7.5); 0.0704 (1.2); 0.0002 (12.0) I-162: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4732 (1.4); 8.4694 (1.6); 8.4613 (1.5); 8.4574 (1.6); 8.4320 (2.3); 8.4252 (2.4); 8.2788 (2.6); 8.1632 (1.6); 8.1590 (1.6); 8.1433 (1.8); 8.1391 (1.7); 7.5279 (1.3); 7.5235 (1.4); 7.5210 (1.5); 7.5167 (1.3); 7.5057 (1.4); 7.5014 (1.5); 7.4989 (1.4); 7.4945 (1.3); 7.4624 (1.2); 7.4607 (1.2); 7.4504 (1.2); 7.4488 (1.2); 7.4426 (1.2); 7.4410 (1.2); 7.4307 (1.1); 7.4291 (1.1); 7.2613 (30.6); 4.8972 (16.0); 4.2274 (1.4); 4.2110 (1.4); 4.2005 (2.2); 4.1840 (2.2); 4.1112 (2.3); 4.0914 (2.3); 4.0842 (1.5); 4.0644 (1.5); 3.8533 (0.7); 3.8394 (0.8); 3.8323 (1.5); 3.8185 (1.6); 3.8121 (2.9); 3.7982 (1.2); 3.7943 (1.9); 3.7900 (2.1); 3.7721 (2.0); 3.7483 (1.2); 3.7294 (1.8); 3.7119 (1.4); 3.7097 (1.3); 3.6906 (0.9); 3.5478 (1.9); 3.5339 (2.0); 3.5256 (1.7); 3.5116 (1.7); 2.5981 (0.6); 2.5806 (0.8); 2.5634 (0.6); 2.0234 (0.6); 2.0109 (0.8); 2.0024 (0.5); 1.9978 (0.6); 1.9897 (0.8); 1.9780 (0.6); 1.9712 (0.5); 1.6502 (0.5); 1.6330 (0.7); 1.6182 (1.0); 1.5986 (1.0); 1.5819 (1.0); 1.5711 (4.3); 0.0080 (1.1); 0.0002 (44.6); 0.0085 (1.3) I-163: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4910 (1.9); 8.4846 (1.8); 8.3009 (2.2); 7.6340 (1.0); 7.6191 (1.1); 7.6125 (1.5); 7.5977 (1.5); 7.5921 (1.1); 7.5772 (1.0); 7.5445 (1.2); 7.5401 (1.3); 7.5378 (1.3); 7.5333 (1.1); 7.5225 (1.2); 7.5182 (1.3); 7.5159 (1.3); 7.5113 (1.1); 7.2613 (19.7); 6.9618 (1.1); 6.9555 (1.2); 6.9527 (1.2); 6.9463 (1.1); 6.9399 (1.0); 6.9337 (1.1); 6.9308 (1.1); 6.9245 (1.0); 4.9268 (16.0); 4.3021 (2.0); 4.2843 (6.1); 4.2665 (6.1); 4.2487 (2.0); 1.5663 (3.8); 1.3155 (7.2); 1.2977 (14.5); 1.2798 (7.0); 0.0079 (0.9); 0.0002 (25.9); 0.0085 (0.8) I-164: .sup.1H-NMR(400.6 MHz, CDCl3): = 7.5796 (0.6); 7.5646 (0.6); 7.5581 (0.8); 7.5431 (0.8); 7.5374 (0.6); 7.5224 (0.6); 7.4583 (0.5); 7.4558 (0.6); 7.4360 (0.5); 7.4334 (0.5); 7.2624 (7.2); 6.8754 (0.6); 6.8693 (0.7); 6.8661 (0.7); 6.8599 (0.7); 6.8537 (0.6); 6.8475 (0.6); 6.8443 (0.6); 6.8382 (0.6); 4.8887 (8.5); 3.7935 (16.0); 1.5873 (0.5); 1.5804 (1.6); 0.8131 (0.6); 0.8068 (3.3); 0.8057 (3.4); 0.8040 (2.7); 0.8012 (1.4); 0.7998 (1.5); 0.7980 (1.3); 0.7948 (2.2); 0.7915 (1.5); 0.7868 (1.6); 0.7835 (2.2); 0.7805 (0.9); 0.7783 (0.9); 0.0002 (10.3) I-167: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4118 (2.1); 8.4049 (2.1); 8.3147 (1.2); 8.3107 (2.1); 8.3069 (1.1); 8.2188 (1.0); 8.2171 (1.0); 8.2153 (1.0); 8.2071 (1.0); 8.2055 (1.1); 7.4804 (0.6); 7.4767 (0.7); 7.4598 (0.8); 7.4563 (1.3); 7.4533 (0.8); 7.4364 (0.8); 7.4326 (0.8); 7.4265 (0.8); 7.4222 (0.8); 7.4198 (0.8); 7.4154 (0.7); 7.4039 (0.7); 7.3996 (0.8); 7.3971 (0.8); 7.3927 (0.7); 7.2943 (0.8); 7.2853 (0.9); 7.2827 (0.9); 7.2737 (1.4); 7.2607 (20.2); 7.2531 (0.8); 4.9054 (9.2); 3.7871 (16.0); 1.6272 (0.9); 1.6103 (1.4); 1.5930 (1.0); 0.8070 (7.9); 0.7899 (9.3); 0.0081 (0.8); 0.0002 (30.0); 0.0085 (0.9) I-171: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4473 (1.3); 8.4406 (1.3); 8.3204 (1.6); 7.5755 (0.5); 7.5605 (0.6); 7.5543 (1.0); 7.5393 (1.0); 7.5332 (0.6); 7.5182 (0.6); 7.4588 (0.6); 7.4545 (0.7); 7.4521 (0.7); 7.4477 (0.6); 7.4364 (0.6); 7.4320 (0.7); 7.4296 (0.7); 7.4253 (0.6); 7.2613 (8.5); 6.8445 (0.6); 6.8384 (0.7); 6.8352 (0.7); 6.8291 (0.6); 6.8228 (0.6); 6.8168 (0.6); 6.8135 (0.6); 6.8074 (0.5); 5.2291 (1.6); 5.2117 (1.7); 3.7634 (16.0); 1.6381 (6.7); 1.6208 (6.7); 1.5834 (0.6); 1.5756 (0.9); 1.5671 (1.7); 1.5630 (1.5); 1.5491 (0.6); 1.5415 (0.6); 0.8407 (1.4); 0.8338 (1.5); 0.8278 (1.0); 0.8230 (1.0); 0.8201 (1.3); 0.8026 (0.5); 0.7989 (0.6); 0.7963 (0.6); 0.7897 (1.4); 0.7855 (1.0); 0.7784 (0.7); 0.7702 (1.3); 0.7642 (0.8); 0.0002 (11.6) I-173: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4937 (2.8); 8.4868 (2.9); 8.4178 (2.2); 8.1019 (1.2); 8.0998 (1.3); 8.0972 (1.4); 8.0951 (1.3); 8.0897 (1.3); 8.0876 (1.4); 8.0850 (1.4); 8.0829 (1.2); 7.8023 (1.1); 7.7976 (1.1); 7.7839 (1.3); 7.7816 (1.6); 7.7792 (1.3); 7.7769 (1.5); 7.7632 (1.6); 7.7585 (1.6); 7.6793 (1.7); 7.6770 (2.9); 7.6747 (1.7); 7.6586 (1.2); 7.6564 (2.0); 7.6539 (1.1); 7.5629 (0.7); 7.5616 (0.7); 7.5567 (1.0); 7.5519 (0.7); 7.5406 (0.7); 7.5392 (0.7); 7.5363 (0.8); 7.5344 (1.0); 7.5295 (0.7); 7.2612 (23.2); 7.1446 (1.4); 7.1420 (1.4); 7.1324 (1.4); 7.1298 (1.4); 7.1262 (1.4); 7.1237 (1.3); 7.1141 (1.3); 7.1115 (1.3); 4.9379 (14.6); 4.3299 (1.8); 4.3121 (5.7); 4.2943 (5.8); 4.2765 (1.9); 1.3376 (7.7); 1.3198 (16.0); 1.3020 (7.4); 0.0081 (1.0); 0.0002 (36.7); 0.0085 (1.0) I-174: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4107 (3.1); 8.4038 (3.1); 8.3149 (1.8); 8.3110 (3.2); 8.3072 (1.7); 8.2183 (1.3); 8.2165 (1.6); 8.2147 (1.6); 8.2130 (1.4); 8.2066 (1.4); 8.2048 (1.6); 8.2031 (1.5); 8.2013 (1.3); 7.4789 (1.1); 7.4752 (1.1); 7.4583 (1.5); 7.4550 (2.0); 7.4517 (1.2); 7.4349 (1.4); 7.4311 (1.4); 7.4265 (1.2); 7.4222 (1.2); 7.4196 (1.2); 7.4153 (1.1); 7.4039 (1.2); 7.3995 (1.3); 7.3970 (1.2); 7.3926 (1.1); 7.2916 (1.4); 7.2826 (1.5); 7.2800 (1.4); 7.2710 (2.5); 7.2619 (15.8); 7.2504 (1.1); 4.8876 (15.8); 4.2761 (2.0); 4.2583 (6.2); 4.2405 (6.2); 4.2227 (2.0); 2.0451 (0.6); 1.6311 (0.6); 1.6293 (0.6); 1.6249 (0.8); 1.6173 (0.6); 1.6104 (2.0); 1.6028 (0.6); 1.5971 (0.7); 1.5950 (0.7); 1.5909 (0.9); 1.5760 (1.2); 1.3018 (7.8); 1.2840 (16.0); 1.2773 (0.6); 1.2661 (7.9); 1.2595 (0.8); 0.8819 (1.0); 0.8218 (1.2); 0.8170 (4.0); 0.8147 (3.6); 0.8123 (3.7); 0.8097 (4.9); 0.8035 (4.1); 0.7995 (2.3); 0.7933 (2.4); 0.7896 (3.6); 0.7866 (1.6); 0.7841 (1.5); 0.0079 (0.6); 0.0002 (22.2); 0.0085 (0.6) I-175: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): = 12.9139 (2.1); 8.5774 (5.4); 8.5704 (5.5); 8.3111 (2.9); 8.3069 (5.5); 8.3030 (2.8); 8.2048 (2.8); 8.1934 (2.9); 7.9328 (1.6); 7.9292 (1.6); 7.9119 (1.8); 7.9079 (2.8); 7.9039 (1.8); 7.8866 (1.8); 7.8830 (1.7); 7.7473 (1.7); 7.7429 (1.8); 7.7404 (1.9); 7.7360 (1.6); 7.7231 (1.8); 7.7188 (2.0); 7.7163 (1.8); 7.7119 (1.6); 7.5295 (1.8); 7.5202 (2.1); 7.5180 (2.0); 7.5086 (3.2); 7.4994 (1.6); 7.4971 (1.7); 7.4878 (1.4); 5.7561 (0.8); 4.7741 (16.0); 3.6012 (1.2); 3.3192 (13.4); 2.5241 (1.2); 2.5194 (1.7); 2.5106 (27.5); 2.5061 (61.0); 2.5015 (85.5); 2.4969 (60.6); 2.4924 (27.3); 1.7596 (1.4); 1.7244 (0.6); 1.7114 (1.3); 1.7034 (1.3); 1.6985 (0.8); 1.6903 (2.7); 1.6825 (0.8); 1.6772 (1.4); 1.6693 (1.4); 1.6563 (0.7); 0.7655 (1.3); 0.7546 (3.1); 0.7490 (4.1); 0.7446 (1.8); 0.7400 (2.2); 0.7336 (3.2); 0.7278 (3.8); 0.7190 (1.8); 0.6395 (1.8); 0.6304 (4.0); 0.6255 (4.3); 0.6175 (4.0); 0.6122 (3.5); 0.6011 (1.2); 0.0080 (1.5); 0.0002 (52.5); 0.0085 (1.5) I-177: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4451 (3.1); 8.4382 (3.2); 8.3220 (1.7); 8.3182 (3.2); 8.3144 (1.8); 7.5708 (1.0); 7.5557 (1.1); 7.5495 (1.6); 7.5345 (1.6); 7.5284 (1.2); 7.5134 (1.1); 7.4578 (1.3); 7.4534 (1.4); 7.4509 (1.4); 7.4465 (1.3); 7.4353 (1.3); 7.4310 (1.4); 7.4284 (1.3); 7.4241 (1.2); 7.2621 (14.6); 6.8424 (1.1); 6.8364 (1.3); 6.8330 (1.2); 6.8269 (1.2); 6.8207 (1.1); 6.8146 (1.1); 6.8113 (1.1); 6.8052 (1.0); 5.2303 (0.8); 5.2129 (3.2); 5.1956 (3.2); 5.1783 (0.9); 4.2463 (2.1); 4.2285 (6.8); 4.2108 (6.9); 4.1930 (2.2); 1.6346 (12.3); 1.6173 (12.4); 1.5979 (0.9); 1.5847 (1.1); 1.5768 (1.1); 1.5701 (0.6); 1.5639 (2.0); 1.5556 (0.7); 1.5503 (1.0); 1.5426 (1.2); 1.5294 (0.6); 1.2813 (7.7); 1.2636 (16.0); 1.2458 (7.5); 0.8693 (0.7); 0.8632 (0.7); 0.8562 (2.3); 0.8519 (2.4); 0.8436 (3.1); 0.8384 (2.3); 0.8303 (1.8); 0.8086 (0.6); 0.7970 (1.6); 0.7882 (2.7); 0.7845 (1.4); 0.7829 (1.3); 0.7762 (2.0); 0.7712 (1.0); 0.7672 (2.2); 0.7629 (1.6); 0.7577 (0.8); 0.7504 (0.8); 0.0080 (0.5); 0.0002 (20.1); 0.0084 (0.6) I-178: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4669 (1.3); 8.4601 (1.3); 8.2901 (1.2); 8.2034 (0.7); 8.2017 (0.8); 8.1998 (0.8); 8.1981 (0.8); 8.1918 (0.7); 8.1901 (0.9); 8.1882 (0.8); 8.1866 (0.8); 7.5241 (0.6); 7.5204 (0.6); 7.5033 (0.8); 7.5013 (0.8); 7.4997 (0.9); 7.4977 (0.7); 7.4806 (0.8); 7.4768 (1.1); 7.4704 (0.5); 7.3655 (0.7); 7.3564 (0.8); 7.3539 (0.8); 7.3447 (1.3); 7.3356 (0.6); 7.3331 (0.6); 7.3240 (0.6); 7.2621 (10.9); 5.2838 (1.4); 5.2664 (1.4); 3.7680 (16.0); 3.7605 (0.6); 1.6876 (6.2); 1.6702 (6.2); 1.5809 (2.3); 0.0002 (12.0) I-179: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4013 (1.8); 8.3944 (1.8); 8.2682 (1.0); 8.2645 (1.8); 8.2609 (1.0); 8.2073 (0.7); 8.2058 (0.7); 8.2028 (0.7); 8.2014 (0.7); 8.1954 (0.7); 8.1940 (0.7); 8.1910 (0.7); 8.1895 (0.7); 7.6495 (0.7); 7.6476 (0.7); 7.6450 (0.7); 7.6432 (0.7); 7.6304 (0.7); 7.6286 (0.8); 7.6259 (0.8); 7.6241 (0.7); 7.5154 (0.8); 7.5110 (0.8); 7.5085 (0.8); 7.5041 (0.8); 7.4928 (0.8); 7.4884 (0.9); 7.4858 (0.8); 7.4814 (0.8); 7.2626 (8.0); 7.2427 (1.0); 7.2308 (1.0); 7.2303 (1.0); 7.2236 (0.9); 7.2118 (0.9); 5.3001 (2.1); 4.9162 (8.1); 3.7893 (16.0); 2.2133 (7.8); 1.6020 (0.9); 0.0699 (0.8); 0.0002 (10.9) I-180: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4709 (2.1); 8.4647 (2.1); 8.3341 (2.6); 7.5761 (1.5); 7.5611 (1.6); 7.5548 (2.3); 7.5401 (2.3); 7.5338 (1.6); 7.5190 (1.6); 7.4893 (1.7); 7.4850 (1.8); 7.4825 (1.8); 7.4782 (1.6); 7.4671 (1.7); 7.4628 (1.9); 7.4603 (1.7); 7.4560 (1.5); 7.2681 (0.7); 7.2674 (0.7); 7.2614 (104.2); 6.9978 (0.5); 6.8603 (1.6); 6.8542 (1.8); 6.8510 (1.8); 6.8448 (1.7); 6.8385 (1.5); 6.8324 (1.6); 6.8292 (1.6); 6.8231 (1.4); 5.3002 (1.2); 5.2980 (1.2); 5.2806 (5.0); 5.2632 (5.2); 5.2458 (1.2); 1.6875 (16.0); 1.6701 (15.9); 1.6553 (0.5); 1.5925 (0.7); 1.5779 (1.5); 1.5737 (1.0); 1.5719 (0.8); 1.5628 (0.9); 1.5589 (2.3); 1.5507 (1.0); 1.5428 (1.2); 1.5400 (1.1); 1.5374 (0.9); 1.5239 (0.9); 1.4322 (2.7); 1.2412 (0.6); 0.8306 (0.7); 0.8203 (0.7); 0.8151 (2.0); 0.8123 (2.4); 0.8070 (1.8); 0.7996 (5.6); 0.7931 (8.0); 0.7858 (3.3); 0.7797 (3.0); 0.7725 (8.0); 0.7576 (1.1); 0.0080 (1.5); 0.0002 (60.8); 0.0049 (0.8); 0.0057 (0.7); 0.0085 (1.7) I-181: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3986 (1.7); 8.3918 (1.8); 8.2486 (2.0); 8.2142 (1.0); 8.2128 (1.1); 8.2098 (1.2); 8.2084 (1.1); 8.2023 (1.1); 8.2009 (1.2); 8.1979 (1.2); 8.1965 (1.1); 7.6559 (1.0); 7.6541 (1.1); 7.6515 (1.2); 7.6497 (1.0); 7.6369 (1.1); 7.6350 (1.3); 7.6324 (1.3); 7.6306 (1.1); 7.4991 (1.1); 7.4947 (1.1); 7.4922 (1.2); 7.4878 (1.1); 7.4764 (1.1); 7.4720 (1.2); 7.4695 (1.2); 7.4651 (1.1); 7.2624 (13.8); 7.2484 (1.5); 7.2364 (1.5); 7.2294 (1.4); 7.2175 (1.4); 5.3000 (8.8); 4.8995 (14.4); 4.2816 (1.8); 4.2637 (5.8); 4.2459 (5.9); 4.2281 (1.9); 2.2205 (12.7); 1.5888 (2.7); 1.3043 (7.6); 1.2865 (16.0); 1.2687 (7.5); 0.0699 (0.7); 0.0022 (0.5); 0.0002 (17.1); 0.0027 (0.9); 0.0085 (0.5) I-182: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.0901 (0.8); 8.6015 (4.4); 8.5945 (4.5); 8.3090 (2.4); 8.3048 (4.5); 8.3008 (2.2); 8.1755 (1.6); 8.1725 (1.8); 8.1711 (1.7); 8.1651 (1.6); 8.1637 (1.8); 8.1607 (1.7); 8.1594 (1.7); 7.8908 (1.4); 7.8891 (1.6); 7.8865 (1.7); 7.8848 (1.4); 7.8718 (1.6); 7.8700 (1.8); 7.8675 (1.7); 7.8657 (1.5); 7.7387 (1.5); 7.7344 (1.6); 7.7318 (1.6); 7.7274 (1.4); 7.7149 (1.6); 7.7106 (1.8); 7.7080 (1.6); 7.7036 (1.4); 7.4044 (2.3); 7.3926 (2.2); 7.3855 (2.2); 7.3736 (2.1); 5.7565 (14.3); 4.8556 (12.5); 3.3217 (2.1); 2.5247 (0.8); 2.5199 (1.2); 2.5111 (16.1); 2.5066 (35.6); 2.5020 (49.7); 2.4974 (35.0); 2.4928 (15.4); 2.2502 (16.0); 1.3560 (0.7); 0.0080 (1.0); 0.0002 (35.3); 0.0085 (1.0) I-388: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4847 (1.5); 8.4781 (1.5); 8.3022 (1.8); 7.6211 (1.0); 7.6062 (1.1); 7.6008 (1.2); 7.5994 (1.3); 7.5859 (1.3); 7.5845 (1.3); 7.5791 (1.1); 7.5642 (1.1); 7.5486 (1.2); 7.5443 (1.2); 7.5417 (1.2); 7.5373 (1.1); 7.5266 (1.2); 7.5222 (1.3); 7.5196 (1.4); 7.5153 (1.1); 7.2609 (30.6); 6.9326 (1.1); 6.9264 (1.2); 6.9234 (1.2); 6.9171 (1.2); 6.9108 (1.0); 6.9046 (1.1); 6.9015 (1.1); 6.8953 (1.0); 5.2474 (0.8); 5.2300 (3.1); 5.2126 (3.1); 5.1952 (0.8); 4.2655 (2.1); 4.2477 (6.8); 4.2299 (6.8); 4.2121 (2.2); 1.6977 (11.8); 1.6803 (11.7); 1.5681 (0.6); 1.2872 (7.6); 1.2694 (16.0); 1.2516 (7.4); 0.0080 (1.2); 0.0002 (41.4); 0.0085 (1.1) I-183: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4912 (3.1); 8.4843 (3.1); 8.3422 (1.6); 8.3383 (3.0); 8.3345 (1.6); 8.1153 (1.1); 8.1131 (1.2); 8.1109 (1.4); 8.1086 (1.2); 8.1032 (1.2); 8.1008 (1.3); 8.0990 (1.4); 8.0965 (1.2); 7.8395 (0.6); 7.8349 (0.6); 7.8223 (0.5); 7.8188 (1.8); 7.8143 (1.7); 7.8017 (2.1); 7.7973 (2.2); 7.7955 (2.2); 7.7931 (2.3); 7.7916 (2.5); 7.7890 (2.2); 7.7748 (0.7); 7.7725 (0.8); 7.5049 (1.2); 7.5005 (1.2); 7.4980 (1.2); 7.4936 (1.2); 7.4824 (1.2); 7.4781 (1.2); 7.4755 (1.2); 7.4712 (1.1); 7.2617 (13.5); 7.1931 (1.2); 7.1892 (1.2); 7.1810 (1.2); 7.1763 (1.9); 7.1720 (1.2); 7.1640 (1.2); 7.1599 (1.2); 5.3000 (5.8); 4.2637 (1.9); 4.2459 (6.1); 4.2281 (6.2); 4.2103 (2.0); 3.9279 (16.0); 1.7277 (1.0); 1.2988 (7.3); 1.2810 (14.6); 1.2632 (7.1); 1.2563 (1.4); 0.0080 (0.6); 0.0002 (20.5); 0.0085 (0.6) I-184: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4822 (3.3); 8.4753 (3.4); 8.3671 (1.7); 8.3632 (3.3); 8.3594 (1.7); 8.0506 (1.2); 8.0486 (1.4); 8.0460 (1.4); 8.0439 (1.4); 8.0385 (1.3); 8.0364 (1.4); 8.0338 (1.4); 8.0317 (1.3); 7.7734 (1.1); 7.7687 (1.1); 7.7550 (1.2); 7.7528 (1.6); 7.7503 (1.3); 7.7481 (1.6); 7.7344 (1.6); 7.7296 (1.6); 7.6493 (1.7); 7.6470 (3.1); 7.6447 (1.8); 7.6287 (1.3); 7.6263 (2.2); 7.6240 (1.2); 7.5183 (1.3); 7.5139 (1.3); 7.5114 (1.4); 7.5070 (1.2); 7.4957 (1.3); 7.4914 (1.4); 7.4888 (1.3); 7.4844 (1.2); 7.2614 (19.3); 7.1106 (1.4); 7.1080 (1.4); 7.0984 (1.4); 7.0958 (1.4); 7.0923 (1.4); 7.0896 (1.4); 7.0801 (1.4); 7.0775 (1.3); 5.3001 (1.8); 5.2611 (0.8); 5.2437 (3.1); 5.2263 (3.1); 5.2089 (0.9); 4.2958 (1.0); 4.2892 (1.0); 4.2872 (0.6); 4.2780 (3.1); 4.2714 (3.1); 4.2602 (3.2); 4.2537 (3.1); 4.2424 (1.1); 4.2360 (1.0); 1.7188 (11.8); 1.7014 (11.7); 1.5695 (2.4); 1.3058 (7.6); 1.2880 (16.0); 1.2702 (7.5); 1.2545 (0.7); 0.0080 (0.8); 0.0002 (26.2); 0.0085 (0.8) I-185: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4970 (1.9); 8.4901 (1.9); 8.3770 (1.0); 8.3731 (1.9); 8.3694 (1.0); 8.0749 (0.8); 8.0728 (0.8); 8.0702 (0.9); 8.0681 (0.8); 8.0627 (0.8); 8.0606 (0.9); 8.0581 (0.9); 8.0560 (0.8); 7.8130 (0.6); 7.8083 (0.6); 7.7947 (0.7); 7.7924 (1.0); 7.7901 (0.7); 7.7877 (1.0); 7.7741 (1.1); 7.7694 (1.1); 7.7239 (1.1); 7.7214 (1.9); 7.7190 (1.2); 7.7032 (0.7); 7.7009 (1.1); 7.6984 (0.7); 7.5219 (0.8); 7.5176 (0.8); 7.5151 (0.8); 7.5107 (0.8); 7.4995 (0.8); 7.4951 (0.8); 7.4926 (0.8); 7.4882 (0.8); 7.2615 (17.3); 7.1488 (0.9); 7.1460 (0.9); 7.1366 (0.8); 7.1338 (0.9); 7.1306 (0.9); 7.1278 (0.8); 7.1184 (0.9); 7.1156 (0.8); 5.3970 (1.4); 5.3799 (1.5); 5.3002 (1.3); 4.1468 (1.6); 4.1332 (1.5); 4.1177 (1.5); 4.1045 (1.5); 3.7705 (16.0); 1.7442 (7.0); 1.7272 (7.0); 1.5700 (2.7); 0.0079 (0.7); 0.0002 (23.3); 0.0085 (0.6) I-186: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.9870 (0.5); 8.6258 (3.1); 8.6188 (3.1); 8.5955 (1.1); 8.5916 (1.3); 8.5834 (1.2); 8.5795 (1.3); 8.4593 (1.3); 8.4552 (1.3); 8.4393 (1.4); 8.4352 (1.3); 8.2746 (1.6); 8.2705 (3.0); 8.2668 (1.5); 7.7471 (1.1); 7.7427 (1.1); 7.7402 (1.1); 7.7358 (1.0); 7.7237 (1.1); 7.7193 (1.2); 7.7168 (1.1); 7.7124 (1.1); 7.7066 (0.9); 7.6944 (0.9); 7.6880 (0.9); 7.6760 (0.8); 5.7571 (16.0); 4.8018 (7.9); 3.3236 (3.5); 2.5252 (0.7); 2.5205 (1.0); 2.5117 (13.6); 2.5072 (29.4); 2.5026 (41.0); 2.4980 (27.9); 2.4934 (12.1); 0.0080 (1.1); 0.0002 (37.3); 0.0085 (1.0) I-187: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4985 (2.0); 8.4916 (2.0); 8.3711 (1.1); 8.3674 (2.0); 8.3637 (1.0); 8.0643 (0.8); 8.0623 (0.9); 8.0597 (0.9); 8.0576 (0.8); 8.0522 (0.8); 8.0501 (0.9); 8.0476 (0.9); 8.0455 (0.8); 7.8088 (0.6); 7.8041 (0.6); 7.7905 (0.7); 7.7881 (1.1); 7.7859 (0.7); 7.7835 (1.0); 7.7699 (1.1); 7.7652 (1.0); 7.7259 (1.2); 7.7234 (1.9); 7.7210 (1.2); 7.7052 (0.7); 7.7029 (1.1); 7.7003 (0.6); 7.5191 (0.8); 7.5147 (0.8); 7.5121 (0.8); 7.5078 (0.7); 7.4966 (0.8); 7.4923 (0.9); 7.4897 (0.8); 7.4854 (0.7); 7.2622 (10.3); 7.1427 (0.9); 7.1399 (0.9); 7.1306 (0.8); 7.1278 (0.9); 7.1245 (0.9); 7.1217 (0.8); 7.1124 (0.9); 7.1096 (0.8); 5.3979 (1.4); 5.3809 (1.5); 5.3001 (3.2); 4.1484 (1.6); 4.1348 (1.5); 4.1189 (1.4); 4.1058 (1.5); 3.7732 (16.0); 1.7469 (7.0); 1.7299 (6.9); 1.5880 (0.8); 1.2594 (0.5); 0.0002 (14.4); 0.0027 (0.6) I-188: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4848 (3.5); 8.4779 (3.6); 8.3678 (1.6); 8.3639 (3.1); 8.3601 (1.8); 8.0415 (0.7); 8.0394 (0.8); 8.0368 (1.4); 8.0348 (1.5); 8.0321 (1.0); 8.0297 (1.4); 8.0274 (1.0); 8.0246 (1.5); 8.0226 (1.5); 8.0200 (0.9); 8.0179 (0.8); 7.7866 (0.6); 7.7819 (0.6); 7.7784 (0.6); 7.7737 (0.6); 7.7682 (0.7); 7.7659 (0.9); 7.7635 (0.8); 7.7606 (1.1); 7.7578 (1.0); 7.7553 (0.8); 7.7530 (0.9); 7.7476 (0.9); 7.7429 (0.9); 7.7394 (0.9); 7.7347 (0.8); 7.6656 (0.9); 7.6633 (1.7); 7.6608 (1.8); 7.6583 (1.7); 7.6561 (1.0); 7.6450 (0.7); 7.6426 (1.2); 7.6401 (1.3); 7.6377 (1.2); 7.6354 (0.7); 7.5215 (1.0); 7.5172 (1.1); 7.5146 (1.1); 7.5103 (1.0); 7.4990 (1.0); 7.4947 (1.2); 7.4922 (1.1); 7.4878 (1.0); 7.2618 (18.7); 7.1086 (0.9); 7.1063 (1.3); 7.1047 (1.0); 7.0942 (1.3); 7.0925 (1.1); 7.0904 (1.0); 7.0881 (1.2); 7.0864 (0.9); 7.0782 (0.9); 7.0759 (1.1); 7.0742 (0.9); 5.3001 (4.5); 5.2597 (1.6); 5.2516 (1.6); 5.2423 (1.6); 5.2342 (1.6); 4.4130 (0.9); 4.3951 (0.9); 4.3859 (1.3); 4.3680 (1.4); 4.3357 (2.3); 4.3338 (2.4); 4.3186 (3.7); 4.2795 (1.3); 4.2654 (1.4); 4.2525 (0.9); 4.2383 (1.0); 3.8017 (1.1); 3.7258 (2.1); 3.6588 (16.0); 3.6508 (16.0); 2.8363 (0.6); 2.8325 (0.8); 2.8227 (0.8); 2.8184 (0.8); 2.8147 (0.6); 2.8060 (0.8); 2.8005 (0.5); 1.7096 (6.6); 1.7075 (6.8); 1.6922 (6.6); 1.6901 (6.7); 1.5742 (1.9); 1.1979 (1.1); 1.1881 (6.5); 1.1797 (1.3); 1.1702 (12.9); 1.1522 (6.4); 0.0080 (0.7); 0.0002 (24.5); 0.0085 (0.6) I-189: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4830 (1.8); 8.4761 (1.8); 8.3681 (1.0); 8.3642 (1.8); 8.3604 (1.0); 8.0546 (0.7); 8.0526 (0.7); 8.0499 (0.8); 8.0479 (0.7); 8.0425 (0.7); 8.0405 (0.8); 8.0378 (0.8); 8.0358 (0.7); 7.7809 (0.6); 7.7762 (0.6); 7.7624 (0.7); 7.7603 (0.8); 7.7578 (0.7); 7.7556 (0.8); 7.7418 (0.8); 7.7371 (0.8); 7.6404 (0.9); 7.6381 (1.6); 7.6358 (1.0); 7.6197 (0.7); 7.6174 (1.2); 7.6151 (0.7); 7.5179 (0.7); 7.5136 (0.7); 7.5110 (0.7); 7.5067 (0.7); 7.4953 (0.7); 7.4910 (0.7); 7.4884 (0.7); 7.4841 (0.6); 7.2620 (6.3); 7.1162 (0.7); 7.1136 (0.8); 7.1041 (0.7); 7.1015 (0.8); 7.0978 (0.8); 7.0953 (0.7); 7.0857 (0.7); 7.0831 (0.7); 5.2786 (1.5); 5.2612 (1.5); 3.8030 (16.0); 1.7236 (6.3); 1.7061 (6.2); 1.5995 (0.7); 1.2643 (0.7); 0.8818 (1.5); 0.8641 (0.6); 0.0002 (8.3) I-190: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5005 (3.3); 8.4936 (3.5); 8.3773 (1.0); 8.3734 (1.9); 8.3702 (1.8); 8.3668 (1.9); 8.3631 (1.1); 8.0649 (0.8); 8.0630 (1.4); 8.0606 (1.4); 8.0584 (1.5); 8.0564 (0.9); 8.0528 (0.9); 8.0509 (1.5); 8.0486 (1.5); 8.0462 (1.5); 8.0443 (0.8); 7.8091 (0.6); 7.8052 (0.8); 7.8008 (0.5); 7.7907 (0.7); 7.7882 (1.2); 7.7846 (1.4); 7.7801 (0.9); 7.7702 (1.0); 7.7664 (1.3); 7.7620 (1.0); 7.7246 (1.1); 7.7221 (1.8); 7.7200 (1.9); 7.7179 (1.8); 7.7154 (1.1); 7.7040 (0.7); 7.7016 (1.0); 7.6994 (1.1); 7.6973 (1.1); 7.6947 (0.6); 7.5252 (0.7); 7.5203 (1.3); 7.5184 (0.9); 7.5156 (0.9); 7.5137 (1.2); 7.5088 (0.7); 7.5028 (0.8); 7.4981 (1.2); 7.4959 (0.9); 7.4932 (0.9); 7.4913 (1.2); 7.4864 (0.7); 7.2616 (26.8); 7.1435 (1.0); 7.1407 (1.2); 7.1393 (1.2); 7.1364 (1.2); 7.1314 (1.2); 7.1285 (1.3); 7.1271 (1.3); 7.1252 (1.6); 7.1225 (1.4); 7.1212 (1.4); 7.1183 (1.2); 7.1132 (1.0); 7.1102 (1.1); 7.1091 (1.1); 7.1061 (1.0); 5.3563 (0.5); 5.3518 (1.6); 5.3394 (1.6); 5.3348 (1.6); 5.3224 (1.6); 5.3002 (4.0); 4.6575 (1.1); 4.6397 (1.7); 4.6218 (1.1); 3.7862 (16.0); 3.7272 (15.5); 1.7332 (7.9); 1.7321 (7.6); 1.7161 (7.9); 1.7151 (7.6); 1.5735 (2.2); 1.4986 (6.2); 1.4808 (6.1); 1.4493 (6.3); 1.4314 (6.2); 1.2596 (0.8); 0.8819 (1.2); 0.0080 (1.1); 0.0002 (36.6); 0.0085 (1.0) I-191: .sup.1H-NMR(400.6 MHz, CDCl3): = 7.6281 (0.5); 7.6133 (0.6); 7.6078 (0.7); 7.6064 (0.7); 7.5929 (0.7); 7.5916 (0.7); 7.5861 (0.6); 7.5712 (0.6); 7.5453 (0.5); 7.5429 (0.6); 7.5233 (0.6); 7.5207 (0.6); 7.2619 (8.2); 6.9365 (0.6); 6.9302 (0.6); 6.9272 (0.6); 6.9210 (0.6); 6.9146 (0.5); 6.9084 (0.6); 6.9054 (0.6); 6.8991 (0.5); 5.2545 (1.5); 5.2371 (1.6); 3.7798 (16.0); 1.7026 (6.4); 1.6852 (6.3); 1.5724 (1.2); 0.0002 (10.9) I-192: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.0750 (0.6); 8.0730 (0.6); 8.0704 (0.7); 8.0683 (0.6); 8.0629 (0.6); 8.0609 (0.7); 8.0582 (0.7); 8.0562 (0.6); 7.7959 (0.5); 7.7911 (0.5); 7.7774 (0.6); 7.7752 (0.8); 7.7727 (0.6); 7.7705 (0.8); 7.7568 (0.8); 7.7521 (0.7); 7.6713 (0.8); 7.6689 (1.4); 7.6667 (0.8); 7.6506 (0.6); 7.6483 (1.0); 7.6460 (0.6); 7.5221 (0.5); 7.2622 (7.1); 7.1330 (0.6); 7.1304 (0.6); 7.1208 (0.6); 7.1182 (0.7); 7.1146 (0.7); 7.1120 (0.6); 7.1025 (0.6); 7.0999 (0.6); 4.9554 (6.7); 4.4232 (0.6); 4.4053 (0.6); 4.3961 (1.3); 4.3782 (1.4); 4.3527 (1.3); 4.3386 (1.4); 4.3256 (0.6); 4.3115 (0.6); 3.6748 (16.0); 2.8460 (0.7); 2.8319 (0.7); 1.2067 (6.4); 1.1887 (6.3); 0.0002 (10.4) I-193: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4917 (2.5); 8.4848 (2.5); 8.3113 (1.6); 8.3078 (2.6); 8.3045 (1.6); 7.6268 (1.0); 7.6120 (1.0); 7.6067 (1.2); 7.6051 (1.3); 7.5918 (1.2); 7.5903 (1.3); 7.5850 (1.1); 7.5701 (1.0); 7.5528 (1.2); 7.5484 (1.3); 7.5459 (1.3); 7.5415 (1.2); 7.5308 (1.3); 7.5264 (1.4); 7.5240 (1.3); 7.5196 (1.2); 7.2622 (14.0); 6.9565 (1.1); 6.9502 (1.2); 6.9473 (1.2); 6.9410 (1.1); 6.9346 (1.0); 6.9284 (1.1); 6.9254 (1.1); 6.9192 (1.0); 4.9252 (15.6); 4.2998 (1.9); 4.2820 (6.1); 4.2642 (6.2); 4.2464 (2.0); 1.5690 (5.0); 1.3141 (7.7); 1.2963 (16.0); 1.2785 (7.5); 0.0080 (0.6); 0.0002 (18.9); 0.0084 (0.6) I-194: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4912 (1.0); 8.4848 (1.0); 8.3661 (1.2); 8.0633 (0.7); 8.0613 (0.8); 8.0587 (0.8); 8.0567 (0.8); 8.0512 (0.8); 8.0492 (0.8); 8.0466 (0.8); 8.0446 (0.7); 7.7908 (0.6); 7.7861 (0.6); 7.7724 (0.7); 7.7702 (0.9); 7.7677 (0.8); 7.7655 (0.8); 7.7518 (0.9); 7.7471 (0.8); 7.6724 (1.0); 7.6704 (1.6); 7.6683 (1.0); 7.6518 (0.7); 7.6498 (1.1); 7.6476 (0.6); 7.5261 (0.6); 7.5218 (0.7); 7.5193 (0.7); 7.5150 (0.6); 7.5037 (0.6); 7.4993 (0.7); 7.4968 (0.7); 7.4925 (0.6); 7.2621 (7.3); 7.1262 (0.8); 7.1237 (0.8); 7.1141 (0.8); 7.1115 (0.8); 7.1079 (0.8); 7.1053 (0.7); 7.0958 (0.7); 7.0932 (0.7); 5.3002 (1.5); 4.9543 (7.8); 4.4220 (0.7); 4.4041 (0.7); 4.3949 (1.4); 4.3770 (1.5); 4.3509 (1.4); 4.3369 (1.5); 4.3238 (0.7); 4.3098 (0.7); 3.7258 (2.2); 3.6749 (16.0); 2.8480 (0.6); 2.8443 (0.8); 2.8301 (0.8); 2.8264 (0.5); 1.2054 (6.8); 1.1979 (1.3); 1.1875 (6.7); 1.1798 (1.2); 0.0002 (10.7) I-195: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4909 (1.2); 8.4841 (1.2); 8.3691 (0.8); 8.3655 (1.3); 8.0634 (0.6); 8.0614 (0.7); 8.0588 (0.8); 8.0567 (0.7); 8.0513 (0.7); 8.0493 (0.8); 8.0466 (0.8); 8.0446 (0.7); 7.7907 (0.6); 7.7860 (0.6); 7.7723 (0.6); 7.7701 (0.8); 7.7677 (0.7); 7.7654 (0.8); 7.7517 (0.8); 7.7470 (0.8); 7.6725 (0.8); 7.6702 (1.6); 7.6680 (0.9); 7.6519 (0.6); 7.6496 (1.1); 7.6474 (0.6); 7.5262 (0.6); 7.5218 (0.7); 7.5193 (0.7); 7.5150 (0.6); 7.5037 (0.6); 7.4994 (0.7); 7.4968 (0.7); 7.4925 (0.6); 7.2614 (12.1); 7.1263 (0.7); 7.1237 (0.7); 7.1141 (0.7); 7.1115 (0.8); 7.1079 (0.8); 7.1053 (0.7); 7.0958 (0.7); 7.0931 (0.7); 5.3002 (3.0); 4.9542 (7.5); 4.4219 (0.7); 4.4040 (0.7); 4.3948 (1.4); 4.3769 (1.4); 4.3509 (1.4); 4.3368 (1.5); 4.3238 (0.7); 4.3097 (0.7); 3.7262 (3.0); 3.6749 (16.0); 2.8479 (0.5); 2.8441 (0.7); 2.8300 (0.7); 2.8263 (0.5); 1.2053 (6.7); 1.1981 (1.6); 1.1874 (6.6); 1.1800 (1.5); 0.0002 (17.6); 0.0083 (0.6) I-196: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4836 (1.8); 8.4766 (1.8); 8.3793 (0.9); 8.3756 (1.7); 8.3720 (0.9); 8.0511 (0.7); 8.0490 (0.8); 8.0464 (0.9); 8.0443 (0.8); 8.0389 (0.8); 8.0368 (0.8); 8.0342 (0.8); 8.0321 (0.8); 7.7942 (0.6); 7.7895 (0.6); 7.7758 (0.8); 7.7735 (0.9); 7.7711 (0.7); 7.7688 (0.9); 7.7552 (1.0); 7.7504 (1.0); 7.6711 (1.0); 7.6688 (1.8); 7.6664 (1.0); 7.6505 (0.7); 7.6481 (1.2); 7.6457 (0.7); 7.5266 (0.8); 7.5223 (0.8); 7.5198 (0.8); 7.5154 (0.7); 7.5040 (0.8); 7.4997 (0.8); 7.4971 (0.8); 7.4928 (0.7); 7.2615 (13.9); 7.1164 (0.8); 7.1138 (0.8); 7.1043 (0.8); 7.1016 (0.9); 7.0981 (0.9); 7.0954 (0.8); 7.0859 (0.8); 7.0833 (0.8); 5.3002 (0.6); 5.2392 (1.7); 5.2218 (1.8); 4.4921 (1.0); 4.4864 (1.1); 4.4763 (2.2); 4.4709 (2.2); 4.4607 (1.1); 4.4552 (1.1); 3.6574 (16.0); 2.6909 (1.4); 2.6746 (2.2); 2.6592 (1.2); 1.7091 (6.2); 1.6916 (6.1); 1.5716 (1.3); 0.0079 (0.6); 0.0002 (20.0); 0.0085 (0.6) I-198: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4835 (3.4); 8.4766 (3.5); 8.3743 (1.7); 8.3704 (3.1); 8.3664 (1.7); 8.0535 (0.7); 8.0514 (0.8); 8.0488 (1.5); 8.0468 (1.5); 8.0442 (1.0); 8.0417 (1.3); 8.0393 (0.9); 8.0367 (1.5); 8.0346 (1.5); 8.0321 (0.9); 8.0300 (0.8); 7.7917 (0.6); 7.7869 (0.6); 7.7835 (0.6); 7.7787 (0.6); 7.7732 (0.7); 7.7710 (0.9); 7.7685 (0.7); 7.7659 (1.1); 7.7628 (1.0); 7.7604 (0.8); 7.7581 (0.9); 7.7526 (0.9); 7.7479 (0.9); 7.7445 (0.9); 7.7397 (0.8); 7.6641 (0.9); 7.6618 (1.7); 7.6592 (1.7); 7.6565 (1.7); 7.6542 (1.0); 7.6435 (0.7); 7.6411 (1.2); 7.6385 (1.3); 7.6359 (1.3); 7.6335 (0.7); 7.5256 (1.0); 7.5207 (1.1); 7.5145 (1.0); 7.5030 (1.0); 7.4985 (1.1); 7.4968 (1.0); 7.4919 (0.9); 7.2617 (21.9); 7.1137 (1.2); 7.1015 (1.2); 7.0956 (1.2); 7.0834 (1.1); 5.3002 (4.0); 5.2627 (1.6); 5.2545 (1.6); 5.2453 (1.6); 5.2370 (1.6); 4.4121 (0.9); 4.3941 (0.9); 4.3850 (1.3); 4.3671 (1.4); 4.3380 (2.2); 4.3347 (2.2); 4.3207 (2.7); 4.3197 (2.7); 4.2828 (1.4); 4.2687 (1.4); 4.2557 (0.9); 4.2417 (0.9); 3.8031 (0.9); 3.7261 (1.1); 3.6571 (15.9); 3.6502 (16.0); 2.8405 (0.5); 2.8382 (0.6); 2.8344 (0.8); 2.8231 (0.8); 2.8203 (0.9); 2.8165 (0.6); 2.8075 (0.8); 2.8024 (0.6); 1.7103 (6.7); 1.7081 (6.8); 1.6928 (6.6); 1.6907 (6.7); 1.5717 (1.8); 1.1980 (0.6); 1.1894 (6.6); 1.1797 (0.9); 1.1713 (12.4); 1.1531 (6.5); 0.0079 (0.9); 0.0002 (30.3); 0.0085 (0.9) I-199: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4978 (3.2); 8.4909 (3.3); 8.3822 (1.0); 8.3784 (1.9); 8.3752 (1.8); 8.3718 (1.8); 8.3681 (0.9); 8.0732 (1.3); 8.0704 (1.3); 8.0687 (1.4); 8.0610 (1.4); 8.0584 (1.2); 8.0565 (1.3); 7.8131 (0.6); 7.8086 (0.8); 7.8048 (0.6); 7.7947 (0.7); 7.7922 (1.1); 7.7887 (1.4); 7.7879 (1.4); 7.7841 (1.0); 7.7741 (1.0); 7.7703 (1.2); 7.7697 (1.3); 7.7659 (0.9); 7.7224 (1.1); 7.7198 (1.9); 7.7178 (1.8); 7.7158 (1.9); 7.7134 (1.1); 7.7017 (0.7); 7.6992 (1.1); 7.6972 (1.1); 7.6952 (1.2); 7.6927 (0.6); 7.5280 (0.8); 7.5235 (0.9); 7.5213 (1.1); 7.5169 (1.1); 7.5154 (0.9); 7.5110 (0.7); 7.5055 (0.8); 7.5010 (1.0); 7.4997 (1.1); 7.4944 (1.1); 7.4931 (0.9); 7.4885 (0.7); 7.2618 (26.7); 7.1494 (0.8); 7.1465 (1.0); 7.1455 (1.0); 7.1425 (0.9); 7.1372 (0.9); 7.1343 (1.2); 7.1332 (1.2); 7.1306 (1.5); 7.1272 (1.4); 7.1243 (1.2); 7.1189 (1.1); 7.1161 (1.2); 7.1151 (1.2); 7.1121 (1.0); 5.3526 (1.9); 5.3355 (3.0); 5.3184 (1.9); 5.3003 (4.6); 4.6601 (1.1); 4.6423 (1.6); 4.6247 (1.1); 3.7837 (16.0); 3.7236 (15.6); 1.7295 (7.1); 1.7273 (7.0); 1.7124 (7.1); 1.7103 (7.0); 1.5749 (4.4); 1.4953 (6.2); 1.4774 (6.1); 1.4460 (6.3); 1.4281 (6.2); 1.2635 (0.6); 0.8818 (1.1); 0.0080 (1.2); 0.0002 (37.2); 0.0085 (1.0) I-200: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 8.6539 (7.6); 8.6469 (7.8); 8.3755 (4.3); 8.3713 (7.8); 8.3675 (4.1); 8.1382 (3.3); 8.1356 (3.6); 8.1336 (3.3); 8.1279 (3.0); 8.1260 (3.6); 8.1234 (3.5); 8.1215 (3.3); 8.0430 (2.4); 8.0384 (2.2); 8.0243 (3.1); 8.0225 (3.4); 8.0198 (3.1); 8.0180 (3.2); 8.0039 (3.0); 7.9993 (2.8); 7.8648 (6.6); 7.8622 (8.0); 7.8488 (2.4); 7.8438 (11.0); 7.8408 (8.6); 7.8365 (3.6); 7.8321 (2.6); 7.8192 (2.8); 7.8149 (3.0); 7.8123 (2.7); 7.8080 (2.4); 7.7689 (6.0); 7.7484 (5.3); 7.6191 (1.9); 7.6005 (4.5); 7.5847 (1.8); 7.5818 (3.0); 7.4631 (6.4); 7.4590 (2.6); 7.4426 (8.8); 7.4283 (1.7); 7.4239 (4.5); 7.3733 (3.0); 7.3709 (3.1); 7.3612 (2.8); 7.3588 (3.0); 7.3548 (3.1); 7.3524 (2.9); 7.3426 (2.9); 7.3403 (2.8); 5.7558 (3.0); 4.0427 (16.0); 3.6150 (0.6); 3.3497 (78.5); 3.1844 (2.1); 3.1567 (0.8); 3.1461 (0.8); 3.1381 (0.7); 3.1280 (0.7); 2.6754 (1.1); 2.6708 (1.4); 2.6663 (1.1); 2.5413 (2.9); 2.5343 (0.8); 2.5246 (3.9); 2.5199 (5.7); 2.5111 (82.3); 2.5065 (176.2); 2.5020 (243.6); 2.4974 (170.7); 2.4929 (77.4); 2.3337 (1.0); 2.3290 (1.5); 2.3245 (1.0); 1.4871 (0.5); 1.2716 (3.6); 1.2578 (5.2); 1.2418 (6.1); 1.2234 (1.1); 0.9599 (0.7); 0.9419 (1.2); 0.9288 (0.9); 0.0080 (3.8); 0.0002 (125.7); 0.0085 (4.0); 0.1496 (0.5) I-201: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5097 (3.7); 8.5028 (3.7); 8.3428 (2.2); 8.3391 (3.8); 8.3354 (2.2); 8.1471 (1.5); 8.1452 (1.7); 8.1426 (1.8); 8.1405 (1.7); 8.1351 (1.6); 8.1330 (1.8); 8.1304 (1.8); 8.1284 (1.7); 7.8619 (1.3); 7.8572 (1.2); 7.8433 (1.6); 7.8414 (2.0); 7.8387 (1.6); 7.8368 (1.9); 7.8229 (1.9); 7.8182 (1.8); 7.7289 (2.1); 7.7266 (3.7); 7.7244 (2.3); 7.7083 (1.6); 7.7061 (2.6); 7.7039 (1.6); 7.5045 (1.4); 7.5001 (1.6); 7.4977 (1.6); 7.4933 (1.5); 7.4823 (1.5); 7.4779 (1.6); 7.4754 (1.6); 7.4710 (1.5); 7.2635 (13.4); 7.2295 (1.6); 7.2270 (1.7); 7.2174 (1.6); 7.2148 (1.7); 7.2110 (1.7); 7.2084 (1.6); 7.1989 (1.6); 7.1963 (1.6); 7.1359 (0.9); 3.7824 (16.0); 2.7607 (0.6); 2.7521 (1.1); 2.7429 (1.6); 2.7342 (1.6); 2.7250 (1.2); 2.7164 (0.7); 0.7836 (1.0); 0.7698 (2.7); 0.7663 (4.0); 0.7637 (1.9); 0.7524 (3.6); 0.7485 (3.0); 0.7458 (1.6); 0.7351 (1.2); 0.4874 (1.2); 0.4774 (2.5); 0.4744 (2.9); 0.4708 (2.8); 0.4685 (2.6); 0.4648 (3.0); 0.4612 (2.8); 0.4476 (1.0); 0.0080 (0.5); 0.0002 (20.1); 0.0085 (0.6) I-202: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4689 (1.3); 8.4652 (1.3); 8.4569 (1.3); 8.4533 (1.3); 8.4276 (3.2); 8.4207 (3.2); 8.2834 (1.8); 8.2797 (3.1); 8.2760 (1.7); 8.1605 (1.4); 8.1565 (1.4); 8.1407 (1.5); 8.1364 (1.4); 7.5302 (1.3); 7.5258 (1.3); 7.5233 (1.4); 7.5189 (1.3); 7.5080 (1.3); 7.5036 (1.4); 7.5011 (1.3); 7.4967 (1.2); 7.4564 (1.0); 7.4547 (1.1); 7.4444 (1.0); 7.4427 (1.1); 7.4367 (1.0); 7.4350 (1.0); 7.4247 (0.9); 7.4230 (1.0); 7.2616 (16.3); 4.8798 (14.9); 4.2809 (1.9); 4.2630 (5.9); 4.2452 (6.0); 4.2274 (1.9); 1.5640 (8.0); 1.4638 (1.0); 1.4400 (1.0); 1.2998 (7.8); 1.2819 (16.0); 1.2756 (0.7); 1.2641 (8.5); 0.8986 (0.6); 0.8818 (2.3); 0.8641 (0.9); 0.0079 (0.7); 0.0002 (23.6); 0.0085 (0.6) I-203: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4739 (3.0); 8.4670 (3.1); 8.2882 (1.6); 8.2844 (3.0); 8.2807 (1.7); 7.5855 (1.0); 7.5705 (1.1); 7.5640 (1.5); 7.5495 (1.4); 7.5432 (1.1); 7.5282 (1.1); 7.4116 (1.3); 7.4072 (1.3); 7.4047 (1.3); 7.4003 (1.2); 7.3896 (1.3); 7.3852 (1.4); 7.3826 (1.3); 7.3783 (1.2); 7.2615 (20.6); 6.8660 (1.1); 6.8599 (1.2); 6.8566 (1.2); 6.8505 (1.2); 6.8442 (1.0); 6.8382 (1.1); 6.8349 (1.1); 6.8287 (1.0); 6.3692 (1.8); 6.3404 (2.2); 6.3251 (2.8); 6.2962 (2.6); 6.0335 (2.7); 6.0289 (2.8); 5.9893 (2.1); 5.9848 (2.0); 5.3362 (2.6); 5.3317 (2.3); 5.3074 (2.3); 5.3028 (2.7); 5.2840 (3.2); 5.2666 (3.2); 5.2493 (0.8); 4.2719 (1.9); 4.2541 (6.2); 4.2363 (6.4); 4.2185 (2.1); 1.6996 (12.0); 1.6823 (11.8); 1.5670 (4.2); 1.2927 (7.6); 1.2749 (16.0); 1.2571 (7.5); 0.0079 (0.8); 0.0002 (30.0); 0.0085 (0.8) I-204: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.0682 (0.9); 8.5970 (4.6); 8.5900 (4.6); 8.3152 (2.4); 8.3111 (4.5); 8.3074 (2.2); 8.1670 (1.6); 8.1656 (1.7); 8.1626 (1.9); 8.1611 (1.7); 8.1552 (1.7); 8.1538 (1.8); 8.1508 (1.8); 8.1493 (1.7); 7.8816 (1.5); 7.8797 (1.6); 7.8771 (1.7); 7.8753 (1.5); 7.8625 (1.7); 7.8607 (1.9); 7.8581 (1.7); 7.8563 (1.6); 7.7414 (1.6); 7.7371 (1.7); 7.7345 (1.7); 7.7301 (1.6); 7.7176 (1.7); 7.7133 (1.9); 7.7107 (1.6); 7.7063 (1.6); 7.3928 (2.3); 7.3810 (2.2); 7.3740 (2.2); 7.3621 (2.1); 5.7571 (3.0); 4.8447 (12.6); 3.3243 (2.9); 2.5247 (0.8); 2.5201 (1.0); 2.5113 (14.4); 2.5067 (31.7); 2.5022 (44.5); 2.4976 (30.6); 2.4930 (13.3); 2.2468 (16.0); 1.9889 (0.6); 0.0079 (1.4); 0.0002 (47.8); 0.0085 (1.2) I-205: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5204 (0.7); 8.5168 (0.8); 8.5085 (0.8); 8.5048 (0.8); 8.4435 (1.4); 8.4367 (1.4); 8.3042 (0.9); 8.3006 (1.5); 8.2971 (0.9); 8.1778 (0.8); 8.1735 (0.8); 8.1577 (0.9); 8.1536 (0.8); 7.5267 (0.7); 7.5223 (0.8); 7.5198 (0.8); 7.5154 (0.7); 7.5045 (0.9); 7.5002 (1.4); 7.4978 (1.0); 7.4933 (0.8); 7.4901 (0.6); 7.4882 (0.6); 7.4823 (0.6); 7.4805 (0.6); 7.4702 (0.6); 7.4685 (0.6); 7.2623 (11.6); 4.8669 (7.0); 4.1743 (3.2); 4.1611 (3.2); 3.7991 (16.0); 0.0002 (16.8) I-206: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4722 (0.8); 8.4686 (0.8); 8.4602 (0.8); 8.4565 (0.8); 8.4302 (1.2); 8.4235 (1.2); 8.2825 (1.3); 8.1623 (0.8); 8.1584 (0.9); 8.1424 (0.9); 8.1385 (0.9); 7.5305 (0.7); 7.5261 (0.8); 7.5236 (0.8); 7.5192 (0.8); 7.5083 (0.7); 7.5039 (0.8); 7.5014 (0.8); 7.4970 (0.7); 7.4605 (0.6); 7.4587 (0.7); 7.4485 (0.6); 7.4467 (0.6); 7.4407 (0.6); 7.4389 (0.6); 7.4287 (0.6); 7.4269 (0.6); 7.2608 (22.8); 7.2559 (0.5); 4.8958 (8.6); 3.7931 (16.0); 1.5626 (3.1); 0.0080 (0.8); 0.0002 (32.8); 0.0085 (0.9) I-207: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.1181 (1.3); 8.6952 (5.9); 8.6883 (5.8); 8.4334 (3.0); 8.4293 (5.5); 8.4257 (2.8); 8.1989 (1.2); 8.1835 (1.3); 8.1768 (2.5); 8.1614 (2.5); 8.1547 (1.4); 8.1393 (1.3); 7.9290 (2.2); 7.9246 (2.2); 7.9220 (2.2); 7.9177 (2.0); 7.9053 (2.3); 7.9009 (2.5); 7.8984 (2.1); 7.8940 (2.0); 7.4045 (1.4); 7.3981 (1.9); 7.3964 (1.8); 7.3899 (1.5); 7.3824 (1.3); 7.3759 (1.6); 7.3743 (1.6); 7.3678 (1.2); 5.7569 (3.5); 4.8758 (16.0); 3.3209 (18.5); 2.6750 (0.6); 2.6704 (0.8); 2.6658 (0.6); 2.5409 (0.8); 2.5242 (2.3); 2.5195 (3.0); 2.5108 (43.7); 2.5062 (97.7); 2.5016 (139.0); 2.4970 (95.6); 2.4924 (41.8); 2.3333 (0.6); 2.3287 (0.8); 2.3240 (0.6); 0.0080 (3.6); 0.0064 (0.7); 0.0055 (0.8); 0.0047 (1.0); 0.0039 (1.3); 0.0031 (2.4); 0.0023 (4.3); 0.0015 (6.8); 0.0002 (133.1); 0.0018 (8.6); 0.0027 (5.6); 0.0035 (3.8); 0.0043 (2.3); 0.0051 (1.8); 0.0060 (1.5); 0.0067 (1.3); 0.0076 (1.4); 0.0085 (3.9); 0.0098 (0.9); 0.0107 (0.6); 0.0115 (0.6); 0.0123 (0.5) I-208: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4840 (1.6); 8.4776 (1.7); 8.2957 (2.0); 7.6297 (1.0); 7.6149 (1.1); 7.6094 (1.4); 7.6081 (1.4); 7.5945 (1.4); 7.5932 (1.3); 7.5877 (1.2); 7.5729 (1.1); 7.5400 (1.2); 7.5356 (1.3); 7.5331 (1.3); 7.5288 (1.2); 7.5179 (1.2); 7.5135 (1.3); 7.5111 (1.3); 7.5067 (1.2); 7.2617 (19.6); 6.9393 (1.1); 6.9331 (1.3); 6.9300 (1.2); 6.9238 (1.2); 6.9174 (1.1); 6.9112 (1.1); 6.9082 (1.1); 6.9020 (1.0); 5.2509 (0.8); 5.2335 (3.2); 5.2161 (3.2); 5.1987 (0.9); 4.2674 (2.2); 4.2496 (7.0); 4.2318 (7.0); 4.2140 (2.2); 1.6990 (12.2); 1.6816 (12.1); 1.5664 (6.3); 1.2881 (7.7); 1.2703 (16.0); 1.2525 (7.4); 0.0080 (0.8); 0.0002 (28.8); 0.0085 (0.9) I-209: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4318 (2.7); 8.4249 (2.8); 8.2763 (1.6); 8.2725 (2.8); 8.2689 (1.6); 7.5787 (1.0); 7.5637 (1.1); 7.5581 (1.3); 7.5570 (1.4); 7.5431 (1.3); 7.5420 (1.4); 7.5366 (1.2); 7.5216 (1.1); 7.4204 (1.2); 7.4161 (1.2); 7.4134 (1.3); 7.4092 (1.2); 7.3982 (1.2); 7.3939 (1.3); 7.3913 (1.3); 7.3870 (1.2); 7.2610 (34.4); 6.8643 (1.1); 6.8582 (1.2); 6.8549 (1.2); 6.8488 (1.2); 6.8425 (1.0); 6.8364 (1.1); 6.8332 (1.1); 6.8270 (1.1); 5.2676 (0.8); 5.2503 (3.1); 5.2329 (3.2); 5.2156 (0.9); 5.1283 (0.6); 5.1244 (2.1); 5.1202 (3.0); 5.1161 (2.3); 5.1122 (0.7); 5.0317 (2.2); 5.0294 (2.8); 5.0271 (2.7); 5.0248 (2.1); 4.2551 (2.0); 4.2373 (6.6); 4.2196 (6.7); 4.2018 (2.2); 1.9331 (7.4); 1.9308 (9.8); 1.9295 (9.9); 1.9272 (8.0); 1.6594 (11.6); 1.6526 (1.0); 1.6420 (11.6); 1.6354 (0.9); 1.6278 (1.0); 1.5632 (2.7); 1.2825 (7.7); 1.2738 (0.7); 1.2648 (16.0); 1.2570 (1.1); 1.2470 (7.4); 0.0080 (1.4); 0.0002 (48.6); 0.0085 (1.4) I-210: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4940 (0.8); 8.4878 (0.8); 8.3097 (1.0); 7.6292 (0.6); 7.6144 (0.6); 7.6091 (0.7); 7.6074 (0.8); 7.5942 (0.8); 7.5926 (0.8); 7.5874 (0.7); 7.5725 (0.6); 7.5536 (0.6); 7.5492 (0.7); 7.5467 (0.7); 7.5423 (0.6); 7.5316 (0.7); 7.5272 (0.7); 7.5248 (0.7); 7.5203 (0.7); 7.2610 (22.1); 6.9597 (0.6); 6.9534 (0.7); 6.9504 (0.7); 6.9441 (0.7); 6.9378 (0.6); 6.9315 (0.7); 6.9285 (0.7); 6.9223 (0.6); 4.9456 (8.6); 3.8096 (16.0); 1.5521 (9.2); 0.0080 (0.8); 0.0002 (30.3); 0.0085 (0.8) I-211: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3992 (2.4); 8.3924 (2.4); 8.2673 (1.4); 8.2636 (2.5); 8.2600 (1.5); 8.2060 (1.1); 8.2047 (1.2); 8.2016 (1.3); 8.2003 (1.2); 8.1942 (1.2); 8.1928 (1.2); 8.1898 (1.2); 8.1884 (1.1); 7.6467 (1.1); 7.6448 (1.2); 7.6422 (1.2); 7.6405 (1.1); 7.6276 (1.2); 7.6258 (1.4); 7.6232 (1.3); 7.6214 (1.2); 7.5157 (1.2); 7.5113 (1.2); 7.5088 (1.3); 7.5044 (1.2); 7.4931 (1.2); 7.4887 (1.3); 7.4862 (1.2); 7.4818 (1.2); 7.2624 (12.2); 7.2392 (1.6); 7.2273 (1.6); 7.2202 (1.5); 7.2084 (1.4); 4.8984 (14.6); 4.2787 (1.8); 4.2608 (5.9); 4.2430 (5.9); 4.2252 (1.9); 2.2154 (13.5); 1.5807 (7.7); 1.4372 (1.0); 1.3029 (7.8); 1.2851 (16.0); 1.2672 (8.3); 0.8987 (0.6); 0.8818 (2.2); 0.8641 (0.8); 0.0002 (17.1) I-212: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3996 (1.3); 8.3927 (1.3); 8.2641 (0.7); 8.2603 (1.3); 8.2566 (0.7); 8.2011 (0.5); 8.1997 (0.5); 8.1967 (0.6); 8.1953 (0.5); 8.1892 (0.5); 8.1878 (0.6); 8.1848 (0.6); 8.1834 (0.5); 7.6444 (0.5); 7.6418 (0.6); 7.6272 (0.5); 7.6254 (0.6); 7.6228 (0.6); 7.6210 (0.5); 7.5150 (0.6); 7.5106 (0.6); 7.5081 (0.6); 7.5037 (0.6); 7.4924 (0.6); 7.4880 (0.6); 7.4855 (0.6); 7.4811 (0.5); 7.2627 (5.4); 7.2376 (0.7); 7.2257 (0.7); 7.2186 (0.7); 7.2067 (0.7); 4.9504 (6.4); 4.3496 (1.6); 4.3412 (0.8); 4.3379 (1.6); 4.3342 (0.8); 4.3260 (1.7); 3.6202 (1.9); 3.6134 (0.7); 3.6121 (0.9); 3.6084 (1.7); 3.6051 (0.9); 3.6037 (0.6); 3.5967 (1.8); 3.4875 (1.0); 3.3574 (16.0); 2.2174 (5.9); 0.0002 (8.0) I-213: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4834 (2.7); 8.4768 (2.9); 8.2941 (3.2); 7.6030 (0.7); 7.5814 (1.4); 7.5664 (1.4); 7.5458 (0.8); 7.4363 (1.2); 7.4312 (1.5); 7.4253 (1.3); 7.4145 (1.3); 7.4096 (1.6); 7.4032 (1.2); 7.2608 (29.5); 6.9037 (0.6); 6.8942 (1.2); 6.8881 (1.3); 6.8786 (0.9); 6.8724 (1.2); 6.8663 (1.2); 6.8568 (0.6); 5.2956 (1.3); 5.2782 (1.3); 5.2439 (0.5); 5.2264 (1.6); 5.2090 (1.7); 5.1917 (0.5); 3.7802 (16.0); 3.7559 (12.5); 2.4370 (0.9); 2.4298 (0.7); 2.4170 (0.6); 2.4081 (1.4); 2.4006 (0.5); 2.3878 (1.2); 2.3787 (0.8); 2.3586 (0.6); 1.9197 (0.8); 1.8997 (0.8); 1.8888 (0.6); 1.7903 (0.6); 1.7782 (0.9); 1.7623 (1.5); 1.7490 (1.4); 1.7424 (0.9); 1.7341 (1.1); 1.7196 (0.8); 1.7144 (0.6); 1.6999 (0.6); 1.6861 (0.5); 1.6638 (5.5); 1.6468 (11.7); 1.6297 (7.0); 1.5505 (10.2); 0.0079 (1.7); 0.0002 (42.3); 0.0085 (2.0) I-214: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.0004 (0.6); 8.6175 (5.0); 8.6105 (5.2); 8.3408 (2.6); 8.3366 (5.0); 8.3328 (2.6); 8.1530 (1.1); 8.1375 (1.2); 8.1310 (2.2); 8.1155 (2.2); 8.1090 (1.2); 8.0935 (1.1); 7.8213 (1.6); 7.8170 (1.7); 7.8144 (1.8); 7.8101 (1.6); 7.7976 (1.7); 7.7933 (1.9); 7.7907 (1.7); 7.7864 (1.6); 7.3408 (1.2); 7.3343 (1.7); 7.3326 (1.7); 7.3260 (1.4); 7.3186 (1.2); 7.3122 (1.5); 7.3104 (1.5); 7.3040 (1.1); 5.7568 (2.5); 5.1135 (2.4); 5.1087 (3.5); 5.1047 (2.7); 5.0002 (3.0); 4.9979 (3.6); 4.9952 (3.5); 4.9929 (2.9); 4.8290 (14.6); 4.8149 (0.9); 3.3234 (16.0); 2.6708 (0.5); 2.5244 (1.5); 2.5198 (2.0); 2.5110 (29.4); 2.5065 (65.3); 2.5019 (92.4); 2.4973 (64.4); 2.4928 (28.9); 2.3290 (0.5); 1.8903 (9.6); 1.8881 (14.2); 1.8870 (14.5); 1.8848 (10.3); 0.0080 (1.8); 0.0002 (70.5); 0.0085 (2.0) I-215: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.4404 (1.9); 8.4335 (1.8); 8.2790 (2.0); 7.5887 (0.6); 7.5739 (0.7); 7.5675 (1.1); 7.5527 (1.0); 7.5469 (0.8); 7.5320 (0.6); 7.4226 (0.7); 7.4159 (0.8); 7.4113 (0.7); 7.4002 (0.7); 7.3961 (0.8); 7.3892 (0.7); 7.2606 (32.7); 6.8950 (0.8); 6.8859 (0.8); 6.8794 (0.8); 6.8731 (0.8); 6.8641 (0.8); 6.8575 (0.6); 5.1515 (1.4); 5.1476 (2.1); 5.1436 (1.4); 5.0531 (2.0); 4.9599 (0.6); 4.9369 (1.0); 4.9285 (9.5); 3.8146 (1.0); 3.7995 (16.0); 3.7943 (3.5); 1.9220 (7.3); 1.5486 (14.2); 0.0079 (1.8); 0.0002 (42.6); 0.0084 (1.3) I-216: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4927 (1.7); 8.4858 (1.8); 8.3056 (1.0); 8.3019 (1.8); 8.2982 (1.0); 7.6374 (0.6); 7.6226 (0.6); 7.6173 (0.8); 7.6157 (0.8); 7.6025 (0.8); 7.6008 (0.8); 7.5955 (0.7); 7.5807 (0.6); 7.5453 (0.7); 7.5409 (0.8); 7.5384 (0.8); 7.5340 (0.8); 7.5233 (0.8); 7.5189 (0.8); 7.5165 (0.8); 7.5120 (0.7); 7.2618 (8.6); 6.9661 (0.7); 6.9598 (0.7); 6.9569 (0.7); 6.9506 (0.7); 6.9442 (0.6); 6.9379 (0.7); 6.9350 (0.7); 6.9287 (0.6); 4.9480 (8.8); 3.8118 (16.0); 1.5750 (0.7); 0.0002 (13.3) I-217: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.8988 (0.8); 8.6666 (4.7); 8.6597 (4.7); 8.4273 (2.4); 8.4230 (4.6); 8.4195 (2.2); 8.1574 (1.8); 8.1554 (2.0); 8.1528 (2.2); 8.1508 (2.0); 8.1454 (1.9); 8.1433 (2.1); 8.1408 (2.2); 8.1387 (1.9); 8.0570 (1.7); 8.0523 (1.6); 8.0384 (2.1); 8.0365 (2.2); 8.0337 (1.9); 8.0318 (2.0); 8.0179 (2.2); 8.0132 (2.0); 7.8920 (1.8); 7.8877 (1.8); 7.8850 (1.8); 7.8808 (1.6); 7.8680 (1.8); 7.8637 (1.9); 7.8610 (1.7); 7.8567 (1.6); 7.8204 (2.3); 7.8181 (4.1); 7.8159 (2.3); 7.7999 (2.0); 7.7976 (3.5); 7.7953 (1.8); 7.3709 (2.1); 7.3684 (2.1); 7.3588 (1.9); 7.3563 (2.0); 7.3524 (2.0); 7.3499 (1.8); 7.3402 (2.0); 7.3377 (1.9); 5.7571 (4.3); 4.0346 (16.0); 3.3284 (8.6); 2.5251 (1.0); 2.5205 (1.2); 2.5118 (13.4); 2.5072 (28.7); 2.5026 (39.7); 2.4980 (27.0); 2.4935 (11.5); 1.6731 (1.3); 0.0079 (1.0); 0.0002 (33.8); 0.0085 (0.9) I-218: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.0976 (1.1); 8.6633 (6.8); 8.6563 (7.0); 8.4314 (3.7); 8.4272 (7.0); 8.4232 (3.3); 8.1024 (2.6); 8.1004 (2.9); 8.0978 (3.3); 8.0957 (3.0); 8.0903 (2.7); 8.0883 (3.2); 8.0857 (3.2); 8.0836 (3.0); 8.0095 (2.5); 8.0048 (2.3); 7.9909 (3.0); 7.9889 (3.1); 7.9862 (2.8); 7.9842 (3.0); 7.9703 (3.1); 7.9656 (2.9); 7.8933 (2.6); 7.8891 (2.6); 7.8864 (2.6); 7.8821 (2.4); 7.8693 (2.7); 7.8650 (2.9); 7.8623 (2.5); 7.8581 (2.4); 7.6770 (3.1); 7.6748 (5.8); 7.6726 (3.3); 7.6564 (2.9); 7.6542 (5.3); 7.6519 (2.9); 7.3017 (3.0); 7.2992 (3.0); 7.2895 (2.7); 7.2871 (3.0); 7.2832 (3.0); 7.2807 (2.7); 7.2710 (2.8); 7.2685 (2.8); 5.1891 (1.2); 5.1718 (6.0); 5.1544 (6.2); 5.1370 (1.2); 4.0382 (0.6); 4.0205 (0.6); 3.3263 (6.8); 2.5250 (1.0); 2.5203 (1.3); 2.5115 (18.4); 2.5070 (39.9); 2.5024 (55.8); 2.4978 (38.0); 2.4932 (16.5); 1.9890 (2.6); 1.9097 (0.8); 1.6088 (16.0); 1.5914 (15.9); 1.3561 (0.6); 1.1924 (0.8); 1.1746 (1.6); 1.1569 (0.8); 0.0080 (1.7); 0.0048 (0.6); 0.0040 (0.8); 0.0023 (2.3); 0.0002 (56.8); 0.0041 (1.0); 0.0050 (0.7); 0.0059 (0.5); 0.0085 (1.5) I-219: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4930 (4.5); 8.4861 (4.6); 8.3014 (2.8); 8.2978 (4.7); 8.2943 (3.0); 7.5817 (1.6); 7.5667 (1.6); 7.5602 (2.3); 7.5454 (2.3); 7.5394 (1.7); 7.5244 (1.7); 7.5193 (0.5); 7.4447 (1.9); 7.4404 (2.1); 7.4379 (2.1); 7.4335 (1.9); 7.4229 (2.0); 7.4186 (2.2); 7.4160 (2.0); 7.4117 (1.8); 7.2682 (0.5); 7.2608 (52.1); 6.8774 (1.7); 6.8713 (1.9); 6.8682 (1.9); 6.8620 (1.8); 6.8556 (1.6); 6.8495 (1.8); 6.8463 (1.8); 6.8402 (1.5); 6.3625 (2.7); 6.3336 (3.3); 6.3184 (4.0); 6.2895 (3.7); 6.0014 (3.9); 5.9971 (4.1); 5.9573 (3.1); 5.9529 (3.1); 5.3801 (1.3); 5.3628 (5.1); 5.3453 (5.8); 5.3437 (5.2); 5.3393 (3.8); 5.3280 (1.4); 5.3147 (3.4); 5.3103 (3.7); 5.3002 (0.6); 1.7525 (16.0); 1.7351 (15.8); 1.7109 (0.9); 1.4322 (1.5); 1.2641 (2.1); 0.8989 (1.1); 0.8820 (3.9); 0.8643 (1.5); 0.0080 (2.2); 0.0002 (75.6); 0.0085 (2.7) I-220: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4601 (3.2); 8.4532 (3.3); 8.2822 (1.8); 8.2783 (3.3); 8.2744 (1.8); 7.9906 (1.2); 7.9885 (1.4); 7.9859 (1.5); 7.9838 (1.4); 7.9785 (1.3); 7.9764 (1.4); 7.9738 (1.5); 7.9717 (1.4); 7.7065 (1.2); 7.7017 (1.2); 7.6883 (1.2); 7.6858 (1.7); 7.6836 (1.4); 7.6810 (1.7); 7.6676 (1.7); 7.6629 (1.7); 7.6136 (1.7); 7.6111 (3.1); 7.6087 (2.0); 7.5929 (1.2); 7.5905 (1.9); 7.5880 (1.1); 7.3466 (1.2); 7.3424 (1.3); 7.3397 (1.3); 7.3355 (1.2); 7.3240 (1.3); 7.3197 (1.3); 7.3171 (1.3); 7.3128 (1.2); 7.2613 (19.6); 7.0165 (1.5); 7.0138 (1.4); 7.0044 (1.4); 7.0016 (1.4); 6.9983 (1.5); 6.9956 (1.3); 6.9862 (1.4); 6.9834 (1.3); 4.9659 (15.0); 4.9229 (0.6); 4.3199 (1.9); 4.3020 (6.1); 4.2842 (6.2); 4.2664 (2.0); 4.1713 (0.8); 4.1685 (1.3); 3.2503 (0.6); 3.2296 (1.1); 3.2279 (1.0); 3.2051 (0.7); 2.5058 (1.2); 2.5002 (0.9); 2.4815 (1.6); 2.4754 (1.6); 2.4574 (0.9); 2.4530 (1.0); 2.4508 (1.0); 2.4283 (0.5); 2.1251 (0.6); 2.1182 (0.7); 2.1101 (0.8); 2.1032 (1.0); 2.0976 (1.4); 2.0921 (0.8); 2.0893 (1.0); 2.0831 (1.0); 2.0759 (1.4); 2.0698 (0.9); 2.0630 (0.5); 2.0557 (0.6); 1.9021 (0.6); 1.8832 (0.9); 1.8771 (0.9); 1.8729 (0.5); 1.8637 (1.1); 1.8573 (1.7); 1.8511 (0.9); 1.8430 (1.2); 1.8407 (1.3); 1.8328 (1.2); 1.8204 (0.8); 1.8181 (0.7); 1.8146 (0.7); 1.3371 (7.8); 1.3193 (16.0); 1.3015 (7.5); 1.2542 (0.9); 0.0079 (0.7); 0.0002 (30.3); 0.0085 (0.9) I-221: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4890 (1.2); 8.4821 (1.2); 8.3740 (0.8); 8.3704 (1.3); 8.3669 (0.8); 8.0752 (0.7); 8.0731 (0.7); 8.0705 (0.8); 8.0684 (0.7); 8.0630 (0.7); 8.0609 (0.8); 8.0583 (0.8); 8.0562 (0.7); 7.7957 (0.6); 7.7910 (0.5); 7.7773 (0.7); 7.7750 (0.8); 7.7726 (0.7); 7.7703 (0.8); 7.7567 (0.8); 7.7519 (0.8); 7.6710 (0.9); 7.6687 (1.5); 7.6664 (0.9); 7.6504 (0.7); 7.6481 (1.1); 7.6457 (0.6); 7.5287 (0.6); 7.5244 (0.7); 7.5218 (0.7); 7.5175 (0.6); 7.5062 (0.6); 7.5019 (0.7); 7.4993 (0.6); 7.4950 (0.6); 7.2612 (12.9); 7.1330 (0.8); 7.1304 (0.7); 7.1208 (0.7); 7.1182 (0.8); 7.1146 (0.8); 7.1120 (0.7); 7.1024 (0.7); 7.0998 (0.7); 5.3002 (1.7); 4.9553 (7.0); 4.4231 (0.6); 4.4052 (0.6); 4.3960 (1.3); 4.3781 (1.4); 4.3526 (1.3); 4.3386 (1.4); 4.3255 (0.6); 4.3115 (0.6); 3.7262 (0.7); 3.6748 (16.0); 2.8459 (0.7); 2.8318 (0.7); 1.5629 (0.8); 1.2066 (6.4); 1.1981 (0.5); 1.1887 (6.4); 0.0079 (0.6); 0.0002 (19.5); 0.0028 (0.9); 0.0085 (0.6) I-222: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4342 (1.9); 8.4273 (1.9); 8.2797 (1.0); 8.2758 (1.8); 8.2721 (1.0); 7.5853 (0.6); 7.5703 (0.6); 7.5647 (0.7); 7.5636 (0.8); 7.5497 (0.8); 7.5486 (0.7); 7.5432 (0.6); 7.5281 (0.6); 7.4246 (0.7); 7.4203 (0.7); 7.4176 (0.7); 7.4133 (0.6); 7.4024 (0.7); 7.3981 (0.7); 7.3955 (0.7); 7.3912 (0.6); 7.2620 (9.0); 6.8664 (0.6); 6.8603 (0.7); 6.8570 (0.6); 6.8509 (0.6); 6.8446 (0.6); 6.8385 (0.6); 6.8352 (0.6); 6.8291 (0.6); 5.2656 (1.7); 5.2483 (1.7); 5.1256 (1.2); 5.1215 (1.6); 5.1174 (1.2); 5.0324 (1.2); 5.0301 (1.6); 5.0278 (1.5); 5.0255 (1.2); 3.7719 (16.0); 3.7663 (1.1); 1.9278 (4.1); 1.9255 (5.4); 1.9241 (5.3); 1.9218 (4.3); 1.6633 (6.4); 1.6576 (0.6); 1.6460 (6.4); 1.6402 (0.6); 1.6315 (0.5); 0.0002 (12.6); 0.0027 (0.7) I-223: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4619 (0.8); 8.4582 (0.9); 8.4500 (0.8); 8.4462 (0.9); 8.4295 (0.8); 8.4232 (0.9); 8.2936 (1.0); 8.1479 (0.9); 8.1437 (0.9); 8.1281 (0.9); 8.1239 (0.9); 7.5184 (0.7); 7.5140 (0.7); 7.5115 (0.7); 7.5072 (0.7); 7.4962 (0.7); 7.4919 (0.8); 7.4894 (0.7); 7.4850 (0.7); 7.4448 (0.6); 7.4430 (0.7); 7.4328 (0.6); 7.4310 (0.7); 7.4250 (0.6); 7.4233 (0.6); 7.4130 (0.6); 7.4113 (0.6); 7.2618 (8.8); 5.3003 (1.7); 4.8886 (8.7); 3.7888 (16.0); 1.5754 (0.5); 0.0698 (0.8); 0.0002 (13.2) I-224: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4802 (2.9); 8.4733 (3.0); 8.2923 (1.7); 8.2885 (3.0); 8.2848 (1.9); 7.5909 (1.0); 7.5759 (1.1); 7.5692 (1.5); 7.5543 (1.4); 7.5488 (1.2); 7.5338 (1.1); 7.4140 (1.2); 7.4097 (1.3); 7.4072 (1.4); 7.4028 (1.3); 7.3922 (1.3); 7.3878 (1.4); 7.3853 (1.4); 7.3809 (1.3); 7.2609 (33.3); 6.8954 (1.1); 6.8893 (1.2); 6.8861 (1.3); 6.8799 (1.2); 6.8736 (1.1); 6.8675 (1.1); 6.8643 (1.2); 6.8581 (1.1); 6.3772 (1.8); 6.3484 (2.1); 6.3331 (2.7); 6.3042 (2.5); 6.0494 (2.7); 6.0451 (2.9); 6.0052 (2.1); 6.0009 (2.1); 5.3567 (2.6); 5.3524 (2.4); 5.3278 (2.2); 5.3235 (2.5); 4.9551 (15.6); 4.3086 (2.0); 4.2908 (6.0); 4.2729 (6.1); 4.2551 (2.0); 1.5545 (8.8); 1.3237 (7.7); 1.3059 (16.0); 1.2954 (0.6); 1.2881 (7.6); 0.0079 (1.5); 0.0002 (47.9); 0.0085 (1.7) I-225: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4587 (1.3); 8.4551 (1.4); 8.4467 (1.4); 8.4429 (1.4); 8.4272 (2.7); 8.4203 (2.8); 8.2941 (1.6); 8.2904 (2.8); 8.2868 (1.6); 8.1457 (1.4); 8.1417 (1.5); 8.1259 (1.6); 8.1218 (1.5); 7.5186 (1.2); 7.5142 (1.3); 7.5117 (1.3); 7.5073 (1.2); 7.4964 (1.3); 7.4920 (1.4); 7.4895 (1.3); 7.4851 (1.2); 7.4406 (1.1); 7.4388 (1.2); 7.4286 (1.0); 7.4269 (1.1); 7.4208 (1.0); 7.4191 (1.1); 7.4089 (1.0); 7.4071 (1.0); 7.2619 (13.8); 5.3002 (7.6); 4.8736 (15.2); 4.2765 (1.9); 4.2586 (6.2); 4.2408 (6.2); 4.2230 (2.0); 1.2984 (7.8); 1.2876 (0.6); 1.2806 (16.0); 1.2628 (7.6); 0.0699 (1.0); 0.0080 (0.6); 0.0002 (20.5); 0.0085 (0.6) I-226: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4763 (1.6); 8.4695 (1.7); 8.2907 (1.0); 8.2870 (1.7); 8.2834 (1.0); 7.5925 (0.6); 7.5775 (0.6); 7.5715 (0.9); 7.5566 (1.0); 7.5502 (0.6); 7.5352 (0.6); 7.4157 (0.7); 7.4114 (0.7); 7.4089 (0.8); 7.4045 (0.7); 7.3938 (0.7); 7.3894 (0.8); 7.3869 (0.7); 7.3825 (0.7); 7.2621 (6.5); 6.8690 (0.6); 6.8629 (0.7); 6.8597 (0.7); 6.8535 (0.6); 6.8473 (0.6); 6.8411 (0.6); 6.8379 (0.6); 6.8318 (0.6); 6.3666 (1.0); 6.3377 (1.2); 6.3225 (1.4); 6.2936 (1.4); 6.0202 (1.5); 6.0157 (1.5); 5.9761 (1.2); 5.9716 (1.1); 5.3369 (1.4); 5.3325 (1.3); 5.3081 (1.3); 5.3034 (1.8); 5.3005 (3.1); 5.2841 (1.7); 3.7853 (16.0); 1.7040 (6.7); 1.6867 (6.6); 1.5838 (1.4); 0.0002 (8.9) I-228: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5127 (0.6); 8.5005 (4.8); 8.4938 (4.8); 8.3398 (3.3); 8.3365 (4.6); 8.3333 (3.3); 7.5979 (1.5); 7.5830 (1.7); 7.5765 (2.4); 7.5737 (2.1); 7.5691 (2.0); 7.5668 (2.0); 7.5623 (3.5); 7.5557 (1.8); 7.5521 (1.8); 7.5477 (1.9); 7.5453 (1.8); 7.5409 (2.7); 7.2620 (36.0); 6.8757 (1.6); 6.8695 (1.8); 6.8664 (1.8); 6.8603 (1.7); 6.8539 (1.5); 6.8478 (1.6); 6.8446 (1.6); 6.8385 (1.4); 5.3262 (1.2); 5.3088 (5.0); 5.2913 (5.1); 5.2740 (1.2); 5.1408 (1.1); 5.1371 (3.5); 5.1330 (5.3); 5.1290 (3.5); 5.1253 (0.9); 4.9934 (3.7); 4.9912 (4.7); 4.9891 (4.4); 4.9869 (3.4); 1.9639 (0.6); 1.9604 (0.8); 1.9582 (0.7); 1.9304 (11.6); 1.9281 (16.0); 1.9268 (15.8); 1.9246 (12.0); 1.7450 (0.7); 1.7275 (0.7); 1.7090 (15.3); 1.7032 (1.9); 1.6916 (15.6); 1.6858 (1.8); 1.6790 (1.6); 1.6763 (1.2); 1.6496 (0.5); 1.4321 (1.9); 0.0079 (1.3); 0.0002 (50.6); 0.0085 (1.5) I-229: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.8671 (0.8); 8.6493 (5.2); 8.6423 (5.2); 8.3809 (2.8); 8.3766 (5.1); 8.3726 (2.4); 8.1191 (1.9); 8.1171 (2.1); 8.1145 (2.5); 8.1124 (2.2); 8.1070 (2.0); 8.1050 (2.4); 8.1023 (2.3); 8.1003 (2.2); 8.0252 (1.8); 8.0205 (1.7); 8.0066 (2.2); 8.0046 (2.4); 8.0019 (2.0); 7.9999 (2.2); 7.9860 (2.4); 7.9813 (2.2); 7.8371 (1.9); 7.8328 (1.9); 7.8301 (1.9); 7.8258 (1.7); 7.8130 (2.0); 7.8088 (2.1); 7.8061 (1.9); 7.8012 (3.3); 7.7986 (4.4); 7.7964 (2.5); 7.7803 (2.1); 7.7781 (3.7); 7.7757 (2.0); 7.3260 (2.2); 7.3234 (2.3); 7.3138 (2.0); 7.3114 (2.2); 7.3075 (2.2); 7.3049 (1.9); 7.2953 (2.1); 7.2928 (2.1); 5.7569 (2.8); 4.0156 (16.0); 3.3228 (0.7); 2.5244 (1.1); 2.5197 (1.3); 2.5109 (17.5); 2.5064 (37.9); 2.5018 (52.8); 2.4972 (35.7); 2.4926 (15.4); 0.0080 (1.9); 0.0002 (70.2); 0.0085 (1.9) I-230: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.0445 (1.0); 8.6443 (5.9); 8.6373 (5.8); 8.6167 (2.2); 8.6128 (2.4); 8.6046 (2.4); 8.6007 (2.4); 8.4824 (2.5); 8.4783 (2.5); 8.4624 (2.8); 8.4582 (2.5); 8.2956 (3.0); 8.2915 (5.6); 8.2878 (2.8); 7.7884 (2.0); 7.7840 (2.1); 7.7815 (2.1); 7.7771 (1.9); 7.7650 (2.2); 7.7606 (2.3); 7.7581 (2.0); 7.7537 (1.9); 7.7371 (1.7); 7.7356 (1.7); 7.7235 (1.7); 7.7171 (1.7); 7.7051 (1.6); 5.7575 (4.6); 4.8331 (16.0); 3.3256 (8.8); 2.5255 (1.0); 2.5209 (1.4); 2.5122 (21.4); 2.5076 (46.2); 2.5030 (64.4); 2.4984 (43.6); 2.4939 (18.9); 2.0865 (1.4); 1.9894 (0.6); 1.3335 (0.9); 1.1814 (0.8); 0.0080 (1.2); 0.0002 (51.4); 0.0085 (1.4) I-231: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.1411 (2.0); 8.7009 (5.3); 8.6940 (5.4); 8.4433 (2.8); 8.4393 (5.1); 8.4357 (2.7); 8.2082 (1.2); 8.1928 (1.3); 8.1861 (2.4); 8.1707 (2.4); 8.1640 (1.3); 8.1486 (1.2); 7.9413 (2.0); 7.9369 (2.0); 7.9343 (2.1); 7.9300 (1.9); 7.9176 (2.1); 7.9132 (2.3); 7.9107 (2.0); 7.9063 (1.8); 7.4136 (1.3); 7.4071 (1.8); 7.4055 (1.8); 7.3990 (1.5); 7.3914 (1.2); 7.3849 (1.6); 7.3834 (1.6); 7.3769 (1.2); 4.8906 (16.0); 3.3243 (2.5); 2.5254 (0.8); 2.5207 (1.2); 2.5119 (16.4); 2.5074 (36.2); 2.5028 (51.4); 2.4982 (36.2); 2.4936 (16.6); 1.7598 (0.6); 1.3562 (3.2); 0.0080 (1.8); 0.0048 (0.5); 0.0039 (0.7); 0.0002 (66.0); 0.0058 (1.1); 0.0066 (0.9); 0.0085 (2.1) I-232: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4337 (1.0); 8.4269 (1.1); 8.2766 (1.2); 8.1658 (0.7); 8.1640 (0.8); 8.1622 (0.8); 8.1605 (0.8); 8.1542 (0.7); 8.1523 (0.9); 8.1506 (0.8); 8.1488 (0.8); 7.4930 (0.6); 7.4894 (0.7); 7.4725 (0.8); 7.4691 (1.2); 7.4658 (0.7); 7.4488 (0.8); 7.4452 (0.8); 7.3786 (0.7); 7.3743 (0.7); 7.3718 (0.7); 7.3674 (0.7); 7.3564 (0.7); 7.3521 (0.7); 7.3495 (0.7); 7.3452 (0.7); 7.2864 (0.7); 7.2774 (0.8); 7.2747 (0.8); 7.2658 (1.4); 7.2619 (8.4); 7.2570 (0.8); 7.2541 (0.7); 7.2452 (0.6); 6.4062 (1.0); 6.3774 (1.2); 6.3621 (1.4); 6.3332 (1.3); 6.0239 (1.4); 6.0193 (1.5); 5.9798 (1.2); 5.9752 (1.2); 5.3378 (1.5); 5.3271 (1.5); 5.3224 (1.6); 5.3206 (1.8); 5.2983 (1.3); 5.2936 (1.3); 3.7751 (16.0); 3.7677 (0.8); 1.7026 (6.5); 1.6852 (6.5); 1.5763 (4.1); 0.0002 (12.6) I-233: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4005 (1.7); 8.3936 (1.7); 8.2530 (1.0); 8.2491 (1.7); 8.2454 (1.0); 8.2159 (0.7); 8.2145 (0.7); 8.2115 (0.8); 8.2101 (0.7); 8.2040 (0.7); 8.2027 (0.8); 8.1996 (0.8); 8.1982 (0.7); 7.6585 (0.7); 7.6567 (0.7); 7.6541 (0.8); 7.6522 (0.6); 7.6394 (0.7); 7.6376 (0.8); 7.6350 (0.8); 7.6332 (0.7); 7.4986 (0.8); 7.4942 (0.8); 7.4917 (0.8); 7.4873 (0.7); 7.4759 (0.8); 7.4715 (0.8); 7.4690 (0.8); 7.4646 (0.7); 7.2623 (8.2); 7.2519 (1.0); 7.2401 (1.0); 7.2329 (0.9); 7.2210 (0.9); 5.3001 (2.4); 4.9180 (8.4); 3.7921 (16.0); 2.2181 (8.4); 1.5924 (1.4); 0.0002 (10.6) I-236: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.1306 (0.5); 8.4323 (3.6); 8.4305 (3.8); 8.4261 (3.9); 8.4243 (3.6); 8.1361 (1.6); 8.1340 (1.8); 8.1314 (2.0); 8.1293 (1.8); 8.1240 (1.8); 8.1219 (2.0); 8.1193 (2.0); 8.1172 (1.8); 8.0051 (1.6); 8.0003 (1.5); 7.9865 (1.8); 7.9845 (1.9); 7.9818 (1.7); 7.9797 (1.8); 7.9659 (1.9); 7.9612 (1.8); 7.9053 (3.4); 7.8991 (3.3); 7.8845 (4.0); 7.8784 (4.0); 7.6972 (2.0); 7.6949 (3.6); 7.6927 (2.0); 7.6766 (1.8); 7.6744 (3.2); 7.6721 (1.7); 7.6371 (4.3); 7.6353 (4.2); 7.6164 (3.8); 7.6146 (3.8); 7.3102 (1.9); 7.3078 (1.9); 7.2981 (1.7); 7.2956 (1.8); 7.2917 (1.8); 7.2892 (1.7); 7.2796 (1.8); 7.2771 (1.7); 4.9366 (12.6); 3.6216 (1.0); 3.6177 (5.5); 3.6155 (3.2); 3.6115 (3.0); 3.6093 (2.3); 3.6074 (3.9); 3.6028 (4.4); 3.6011 (12.7); 3.5989 (4.5); 3.5950 (4.1); 3.5930 (2.3); 3.5908 (2.9); 3.5867 (3.0); 3.5845 (5.7); 3.5806 (1.0); 3.3191 (12.4); 2.6701 (0.6); 2.5239 (1.7); 2.5192 (2.4); 2.5105 (31.1); 2.5059 (68.0); 2.5013 (94.3); 2.4966 (65.6); 2.4920 (28.7); 2.3283 (0.6); 1.9086 (2.7); 1.7808 (1.0); 1.7762 (5.6); 1.7685 (4.6); 1.7671 (3.5); 1.7641 (2.8); 1.7596 (16.0); 1.7548 (2.9); 1.7507 (4.4); 1.7430 (5.3); 1.7384 (0.8); 1.3553 (3.6); 0.0080 (2.2); 0.0002 (79.5); 0.0085 (2.2) I-237: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3594 (1.4); 8.3578 (1.5); 8.3534 (1.5); 8.3517 (1.5); 8.0676 (0.7); 8.0656 (0.8); 8.0630 (0.8); 8.0609 (0.8); 8.0555 (0.8); 8.0535 (0.8); 8.0508 (0.8); 8.0488 (0.8); 7.7733 (0.6); 7.7686 (0.6); 7.7548 (0.7); 7.7527 (0.9); 7.7502 (0.7); 7.7480 (0.8); 7.7342 (0.9); 7.7295 (0.8); 7.7228 (1.4); 7.7167 (1.4); 7.7022 (1.6); 7.6961 (1.6); 7.6330 (1.0); 7.6307 (1.7); 7.6285 (1.0); 7.6123 (0.7); 7.6100 (1.3); 7.6078 (0.7); 7.3871 (1.7); 7.3854 (1.9); 7.3665 (1.6); 7.3648 (1.7); 7.2619 (5.7); 7.1128 (0.8); 7.1103 (0.8); 7.1007 (0.8); 7.0981 (0.8); 7.0945 (0.8); 7.0919 (0.8); 7.0823 (0.8); 7.0797 (0.7); 5.2996 (2.7); 5.2719 (1.6); 5.2545 (1.6); 3.7988 (16.0); 3.7227 (0.9); 1.7185 (6.3); 1.7011 (6.2); 1.5692 (1.2); 0.0002 (8.4) I-238: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.0765 (0.7); 8.4267 (6.0); 8.4249 (6.5); 8.4205 (6.6); 8.4187 (6.1); 8.1293 (2.8); 8.1273 (3.0); 8.1247 (3.4); 8.1226 (3.0); 8.1173 (3.0); 8.1152 (3.3); 8.1126 (3.2); 8.1105 (2.9); 8.0061 (2.6); 8.0014 (2.4); 7.9876 (3.1); 7.9855 (3.1); 7.9829 (2.8); 7.9808 (3.0); 7.9670 (3.3); 7.9622 (3.0); 7.9024 (5.8); 7.8962 (5.4); 7.8817 (6.8); 7.8754 (6.8); 7.6686 (3.3); 7.6663 (6.0); 7.6640 (3.3); 7.6479 (3.1); 7.6457 (5.5); 7.6434 (3.0); 7.6349 (7.3); 7.6330 (7.1); 7.6142 (6.4); 7.6123 (6.4); 7.3040 (3.1); 7.3016 (3.1); 7.2919 (2.8); 7.2894 (3.0); 7.2855 (3.1); 7.2830 (2.7); 7.2734 (3.0); 7.2709 (2.8); 5.1820 (1.2); 5.1645 (6.2); 5.1471 (6.3); 5.1298 (1.2); 4.0555 (0.6); 4.0377 (1.9); 4.0200 (2.0); 4.0022 (0.6); 3.3176 (46.1); 2.6791 (0.8); 2.6744 (1.5); 2.6697 (2.1); 2.6651 (1.4); 2.6603 (0.7); 2.5507 (0.8); 2.5459 (0.9); 2.5404 (1.8); 2.5235 (4.8); 2.5188 (7.6); 2.5101 (111.1); 2.5055 (244.9); 2.5009 (341.1); 2.4963 (235.9); 2.4917 (103.2); 2.3371 (0.7); 2.3327 (1.4); 2.3280 (1.9); 2.3233 (1.4); 2.3187 (0.6); 1.9883 (9.1); 1.9082 (5.4); 1.6033 (16.0); 1.5859 (15.9); 1.3550 (3.5); 1.2382 (1.7); 1.2211 (1.3); 1.1922 (2.8); 1.1744 (5.8); 1.1566 (2.7); 0.1458 (0.8); 0.0079 (7.7); 0.0063 (1.9); 0.0055 (2.1); 0.0046 (2.7); 0.0038 (3.9); 0.0002 (281.4); 0.0027 (11.1); 0.0043 (4.3); 0.0052 (3.2); 0.0060 (2.7); 0.0068 (2.3); 0.0085 (8.2); 0.0108 (1.4); 0.0115 (1.2); 0.0123 (1.0); 0.0132 (0.8); 0.0139 (0.8); 0.0147 (0.8); 0.0155 (0.6); 0.0164 (0.6); 0.0171 (0.6); 0.0179 (0.6); 0.0187 (0.5); 0.0195 (0.6); 0.0211 (0.5); 0.0266 (0.7); 0.0275 (0.8); 0.0307 (0.6); 0.1494 (0.7) I-239: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3563 (2.8); 8.3547 (2.7); 8.3502 (3.0); 8.3486 (2.6); 8.0794 (1.4); 8.0774 (1.5); 8.0747 (1.6); 8.0727 (1.4); 8.0673 (1.4); 8.0652 (1.5); 8.0626 (1.6); 8.0606 (1.4); 7.7750 (1.1); 7.7702 (1.1); 7.7565 (1.4); 7.7543 (1.7); 7.7518 (1.4); 7.7496 (1.6); 7.7360 (1.7); 7.7312 (1.6); 7.7224 (2.6); 7.7163 (2.6); 7.7018 (2.9); 7.6957 (2.9); 7.6520 (1.9); 7.6498 (3.2); 7.6475 (1.8); 7.6313 (1.4); 7.6292 (2.2); 7.6269 (1.2); 7.3886 (3.5); 7.3870 (3.3); 7.3681 (3.2); 7.3664 (2.9); 7.2619 (10.0); 7.1215 (1.5); 7.1189 (1.4); 7.1093 (1.4); 7.1068 (1.5); 7.1031 (1.5); 7.1005 (1.4); 7.0910 (1.4); 7.0884 (1.3); 5.2997 (6.1); 4.9426 (16.0); 4.3207 (2.0); 4.3029 (6.4); 4.2851 (6.4); 4.2673 (2.1); 1.5677 (1.1); 1.3316 (7.6); 1.3138 (15.7); 1.2960 (7.5); 0.0002 (15.0) I-240: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): = 8.4105 (3.3); 8.4056 (3.4); 8.1171 (1.7); 8.1143 (1.9); 8.1049 (1.8); 8.1022 (1.8); 7.9997 (1.2); 7.9950 (1.2); 7.9791 (1.8); 7.9763 (1.6); 7.9605 (1.5); 7.9558 (1.4); 7.8885 (2.5); 7.8823 (2.4); 7.8678 (2.9); 7.8616 (2.9); 7.6645 (3.1); 7.6439 (2.8); 7.6297 (3.7); 7.6090 (3.2); 7.2948 (1.6); 7.2927 (1.5); 7.2827 (1.5); 7.2805 (1.6); 7.2764 (1.6); 7.2742 (1.4); 7.2642 (1.5); 7.2620 (1.4); 5.1700 (0.7); 5.1527 (3.0); 5.1352 (3.1); 5.1180 (0.7); 4.0380 (1.5); 4.0202 (1.6); 4.0023 (0.5); 3.3220 (16.0); 2.5240 (1.1); 2.5192 (1.7); 2.5105 (25.3); 2.5060 (54.3); 2.5015 (75.0); 2.4969 (53.5); 2.4925 (24.7); 1.9886 (6.8); 1.9088 (8.9); 1.5992 (9.0); 1.5818 (9.0); 1.3554 (1.4); 1.2389 (0.7); 1.2218 (0.6); 1.1923 (1.8); 1.1745 (3.6); 1.1567 (1.8); 0.0080 (1.3); 0.0002 (40.9); 0.0085 (1.4) I-241: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3593 (3.0); 8.3543 (2.6); 8.3532 (3.0); 8.0868 (1.5); 8.0840 (1.5); 8.0822 (1.5); 8.0763 (1.3); 8.0747 (1.5); 8.0719 (1.5); 8.0701 (1.4); 7.7795 (1.0); 7.7748 (1.0); 7.7609 (1.2); 7.7590 (1.6); 7.7566 (1.3); 7.7543 (1.6); 7.7404 (1.5); 7.7357 (1.5); 7.7264 (2.4); 7.7203 (2.3); 7.7058 (2.7); 7.6997 (2.6); 7.6491 (3.1); 7.6284 (2.2); 7.3904 (3.0); 7.3891 (3.6); 7.3698 (2.7); 7.3685 (3.2); 7.2618 (9.2); 7.1267 (1.3); 7.1243 (1.4); 7.1145 (1.3); 7.1122 (1.4); 7.1084 (1.4); 7.1059 (1.3); 7.0962 (1.3); 7.0938 (1.2); 5.2997 (1.4); 4.9436 (16.0); 4.3226 (2.0); 4.3048 (6.2); 4.2870 (6.3); 4.2692 (2.1); 1.5674 (1.7); 1.3327 (7.2); 1.3149 (14.4); 1.2971 (7.0); 0.0002 (13.3) I-242: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3539 (1.5); 8.3522 (1.5); 8.3479 (1.6); 8.3460 (1.4); 8.0582 (0.7); 8.0561 (0.8); 8.0535 (0.8); 8.0513 (0.7); 8.0460 (0.7); 8.0439 (0.8); 8.0413 (0.8); 8.0392 (0.7); 7.7688 (0.6); 7.7641 (0.6); 7.7504 (0.7); 7.7481 (0.9); 7.7457 (0.7); 7.7434 (0.9); 7.7298 (0.9); 7.7250 (0.9); 7.7181 (1.5); 7.7120 (1.4); 7.6975 (1.7); 7.6914 (1.6); 7.6340 (1.0); 7.6316 (1.7); 7.6293 (1.0); 7.6133 (0.7); 7.6110 (1.2); 7.6087 (0.7); 7.3848 (1.8); 7.3830 (1.9); 7.3643 (1.7); 7.3624 (1.7); 7.2618 (6.6); 7.1073 (0.8); 7.1048 (0.8); 7.0952 (0.8); 7.0926 (0.8); 7.0890 (0.8); 7.0863 (0.8); 7.0768 (0.8); 7.0742 (0.7); 5.2996 (2.2); 5.2668 (1.5); 5.2494 (1.6); 3.7973 (16.0); 3.7242 (0.7); 3.7218 (0.8); 1.7175 (6.1); 1.7001 (6.0); 1.5682 (0.7); 0.0002 (10.2) I-243: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3671 (1.9); 8.3610 (1.9); 8.0880 (0.9); 8.0860 (0.9); 8.0834 (1.0); 8.0759 (1.0); 8.0739 (1.0); 8.0713 (1.0); 7.7927 (0.6); 7.7880 (0.6); 7.7741 (0.9); 7.7720 (1.0); 7.7695 (0.9); 7.7675 (0.8); 7.7537 (0.9); 7.7490 (0.8); 7.7300 (1.4); 7.7239 (1.4); 7.7093 (1.6); 7.7033 (1.5); 7.6671 (1.4); 7.6651 (1.9); 7.6465 (1.0); 7.6445 (1.3); 7.3910 (2.2); 7.3704 (2.0); 7.2617 (7.9); 7.1311 (0.9); 7.1288 (0.8); 7.1189 (0.9); 7.1165 (0.8); 7.1128 (0.9); 7.1104 (0.7); 7.1006 (0.8); 7.0983 (0.7); 4.9461 (8.9); 4.5224 (2.2); 4.5067 (4.5); 4.4911 (2.2); 3.6827 (16.0); 2.7174 (2.2); 2.7017 (4.4); 2.6860 (2.1); 1.5591 (2.6); 0.0002 (11.3) I-244: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3651 (1.6); 8.3634 (1.7); 8.3590 (1.6); 8.3574 (1.7); 8.0547 (0.7); 8.0527 (0.8); 8.0500 (0.9); 8.0480 (0.8); 8.0426 (0.8); 8.0406 (0.9); 8.0379 (0.9); 8.0359 (0.8); 7.7830 (0.6); 7.7783 (0.6); 7.7646 (0.7); 7.7623 (1.0); 7.7599 (0.8); 7.7576 (0.9); 7.7440 (0.9); 7.7392 (0.9); 7.7259 (1.5); 7.7198 (1.4); 7.7053 (1.6); 7.6992 (1.7); 7.6649 (1.0); 7.6626 (1.8); 7.6604 (1.1); 7.6443 (0.8); 7.6420 (1.2); 7.6397 (0.8); 7.3845 (1.9); 7.3828 (2.0); 7.3639 (1.7); 7.3622 (1.8); 7.2611 (13.5); 7.1078 (0.8); 7.1052 (0.8); 7.0957 (0.8); 7.0931 (0.8); 7.0895 (0.8); 7.0869 (0.8); 7.0774 (0.8); 7.0748 (0.8); 5.2290 (1.7); 5.2116 (1.7); 4.4870 (1.0); 4.4800 (1.0); 4.4713 (2.1); 4.4645 (2.1); 4.4557 (1.1); 4.4488 (1.0); 3.6540 (16.0); 2.6865 (1.6); 2.6706 (2.6); 2.6551 (1.4); 1.7035 (6.1); 1.6860 (6.1); 1.5518 (3.7); 0.0002 (19.6); 0.0085 (0.6) I-245: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3702 (1.7); 8.3685 (1.6); 8.3641 (1.8); 8.3624 (1.5); 8.0640 (0.8); 8.0620 (0.9); 8.0593 (0.9); 8.0573 (0.8); 8.0519 (0.9); 8.0498 (0.9); 8.0472 (0.9); 8.0451 (0.8); 7.7870 (0.6); 7.7823 (0.6); 7.7685 (0.8); 7.7663 (1.0); 7.7638 (0.8); 7.7616 (0.8); 7.7479 (1.0); 7.7432 (0.9); 7.7301 (1.5); 7.7240 (1.5); 7.7095 (1.6); 7.7034 (1.7); 7.6635 (1.2); 7.6613 (1.8); 7.6590 (1.0); 7.6429 (0.9); 7.6407 (1.3); 7.6383 (0.6); 7.3868 (2.1); 7.3851 (1.8); 7.3662 (1.9); 7.3645 (1.6); 7.2611 (13.9); 7.1132 (0.9); 7.1106 (0.8); 7.1010 (0.9); 7.0984 (0.8); 7.0948 (0.9); 7.0923 (0.7); 7.0827 (0.8); 7.0801 (0.7); 5.3000 (2.1); 5.2327 (1.7); 5.2153 (1.7); 4.4877 (1.1); 4.4825 (1.1); 4.4719 (2.2); 4.4670 (2.1); 4.4563 (1.2); 4.4513 (1.0); 3.6533 (16.0); 2.6881 (1.6); 2.6727 (2.7); 2.6570 (1.4); 1.7043 (6.1); 1.6869 (6.0); 1.5511 (4.6); 0.0080 (0.7); 0.0002 (20.1); 0.0085 (0.6) I-246: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.3631 (1.8); 8.3615 (1.7); 8.3570 (1.8); 8.3555 (1.6); 8.0790 (0.9); 8.0771 (1.0); 8.0744 (1.0); 8.0725 (0.8); 8.0669 (0.9); 8.0649 (1.0); 8.0622 (1.0); 8.0603 (0.8); 7.7885 (0.6); 7.7838 (0.6); 7.7701 (0.9); 7.7679 (1.1); 7.7655 (0.9); 7.7633 (0.9); 7.7495 (1.0); 7.7448 (0.9); 7.7262 (1.5); 7.7201 (1.4); 7.7056 (1.6); 7.6995 (1.6); 7.6681 (1.3); 7.6659 (1.9); 7.6475 (1.0); 7.6453 (1.3); 7.3890 (2.1); 7.3874 (1.9); 7.3684 (1.9); 7.3668 (1.7); 7.2614 (9.9); 7.1259 (0.9); 7.1234 (0.8); 7.1138 (0.9); 7.1112 (0.9); 7.1076 (0.9); 7.1051 (0.8); 7.0955 (0.8); 7.0929 (0.7); 5.2999 (1.4); 4.9444 (8.6); 4.5203 (2.1); 4.5046 (4.4); 4.4889 (2.2); 3.6823 (16.0); 2.7157 (2.1); 2.7000 (4.2); 2.6843 (2.0); 1.5553 (3.3); 0.0002 (14.8) I-248: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1714 (1.6); 8.1695 (1.8); 8.1675 (1.6); 8.1653 (1.9); 8.1634 (1.7); 8.0500 (1.2); 8.0478 (1.3); 8.0453 (1.5); 8.0432 (1.3); 8.0378 (1.3); 8.0356 (1.3); 8.0333 (1.5); 8.0310 (1.3); 7.8168 (0.9); 7.8106 (0.9); 7.7976 (1.1); 7.7958 (1.2); 7.7914 (1.1); 7.7897 (1.1); 7.7767 (1.0); 7.7705 (1.0); 7.7525 (0.6); 7.7478 (0.5); 7.7346 (1.5); 7.7318 (1.1); 7.7299 (1.5); 7.7271 (1.0); 7.7170 (1.1); 7.7138 (1.2); 7.7125 (1.3); 7.7092 (1.1); 7.7013 (1.0); 7.6988 (1.2); 7.6981 (1.4); 7.6956 (1.1); 7.6853 (1.0); 7.6825 (1.5); 7.6802 (1.4); 7.6785 (0.7); 7.6647 (0.5); 7.6622 (0.7); 7.2612 (22.4); 7.0817 (1.5); 7.0785 (1.4); 7.0696 (1.5); 7.0663 (1.5); 7.0639 (1.5); 7.0607 (1.4); 7.0518 (1.4); 7.0486 (1.4); 6.9879 (1.4); 6.9863 (1.5); 6.9805 (1.4); 6.9790 (1.4); 6.9668 (1.4); 6.9653 (1.4); 6.9594 (1.4); 6.9578 (1.4); 5.2999 (4.5); 5.2523 (1.5); 5.2509 (1.6); 5.2346 (1.6); 5.2333 (1.6); 5.0717 (1.0); 5.0314 (3.4); 5.0204 (7.2); 5.0060 (3.4); 4.9657 (1.0); 3.8161 (1.7); 3.7499 (16.0); 3.7450 (15.8); 2.3354 (0.6); 2.3257 (0.9); 2.3226 (0.8); 2.3060 (1.0); 2.3029 (0.9); 1.8693 (0.6); 1.8624 (0.6); 1.8496 (0.6); 1.8427 (0.6); 1.6816 (0.5); 1.5578 (1.2); 1.5526 (6.7); 1.5443 (6.6); 1.5350 (6.3); 1.5266 (6.4); 0.0079 (0.9); 0.0002 (32.4); 0.0085 (0.9) I-249: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.0053 (1.1); 8.2439 (4.5); 8.2376 (4.6); 8.1077 (2.9); 8.1057 (3.2); 8.1030 (3.7); 8.1009 (3.3); 8.0956 (3.1); 8.0935 (3.6); 8.0909 (3.5); 8.0888 (3.2); 7.9676 (2.3); 7.9656 (3.4); 7.9610 (4.2); 7.9470 (5.9); 7.9451 (4.6); 7.9421 (5.2); 7.9403 (6.0); 7.9266 (5.3); 7.9216 (4.3); 7.6663 (3.4); 7.6640 (6.3); 7.6618 (3.6); 7.6458 (3.2); 7.6435 (5.8); 7.6412 (3.1); 7.2682 (3.1); 7.2653 (4.3); 7.2628 (6.1); 7.2532 (3.1); 7.2507 (3.8); 7.2469 (6.0); 7.2443 (3.8); 7.2414 (3.0); 7.2401 (2.8); 7.2347 (3.3); 7.2322 (3.1); 6.8712 (0.6); 4.9189 (2.0); 4.8789 (11.6); 4.8695 (11.2); 4.8295 (2.0); 3.6217 (0.8); 3.6178 (4.6); 3.6155 (2.6); 3.6115 (2.4); 3.6094 (1.8); 3.6075 (3.2); 3.6011 (11.0); 3.5990 (3.8); 3.5950 (3.4); 3.5931 (1.8); 3.5908 (2.4); 3.5867 (2.4); 3.5845 (5.0); 3.5806 (0.8); 3.3215 (16.0); 2.7481 (1.0); 2.7284 (1.2); 2.7183 (1.9); 2.6982 (2.1); 2.6880 (1.2); 2.6749 (0.6); 2.6683 (1.4); 2.5409 (3.8); 2.5287 (0.6); 2.5241 (2.1); 2.5195 (2.6); 2.5107 (37.1); 2.5061 (82.2); 2.5015 (115.5); 2.4969 (79.5); 2.4923 (34.9); 2.3286 (0.7); 2.1830 (0.9); 1.9154 (0.5); 1.9088 (2.5); 1.9038 (1.1); 1.8905 (0.9); 1.8852 (0.9); 1.8729 (1.0); 1.8608 (0.6); 1.7807 (0.7); 1.7761 (4.8); 1.7745 (2.0); 1.7685 (3.7); 1.7670 (2.9); 1.7641 (2.2); 1.7595 (13.4); 1.7548 (2.3); 1.7506 (3.6); 1.7430 (4.5); 1.7384 (0.7); 1.6103 (0.6); 1.6008 (0.8); 1.5903 (1.2); 1.5783 (0.8); 1.5694 (1.1); 1.5584 (0.9); 1.3556 (8.6); 0.0271 (0.6); 0.0112 (0.5); 0.0104 (0.5); 0.0095 (0.6); 0.0080 (3.5); 0.0065 (1.0); 0.0056 (1.1); 0.0048 (1.3); 0.0040 (1.8); 0.0031 (2.8); 0.0023 (4.6); 0.0002 (108.5); 0.0041 (1.2); 0.0050 (0.7); 0.0058 (0.5); 0.0085 (2.6) I-250: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2620 (1.3); 8.2601 (1.6); 8.2584 (1.7); 8.2566 (1.5); 8.2504 (1.4); 8.2485 (1.7); 8.2468 (1.7); 8.2450 (1.5); 8.1437 (2.1); 8.1375 (2.3); 7.7569 (1.0); 7.7506 (1.0); 7.7379 (1.2); 7.7358 (1.4); 7.7317 (1.3); 7.7296 (1.4); 7.7168 (1.1); 7.7106 (1.1); 7.4876 (1.1); 7.4839 (1.2); 7.4669 (1.5); 7.4634 (1.9); 7.4607 (1.4); 7.4438 (1.5); 7.4400 (1.4); 7.3264 (1.4); 7.3174 (1.6); 7.3148 (1.5); 7.3058 (2.5); 7.2968 (1.1); 7.2942 (1.2); 7.2851 (1.0); 7.2641 (16.7); 7.1188 (0.7); 6.9260 (1.4); 6.9245 (1.5); 6.9185 (1.5); 6.9171 (1.5); 6.9049 (1.4); 6.9034 (1.5); 6.8974 (1.4); 6.8959 (1.5); 5.3009 (2.3); 4.8100 (12.6); 4.1895 (1.9); 4.1716 (6.2); 4.1538 (6.3); 4.1360 (2.0); 3.6714 (1.2); 3.6560 (2.9); 3.6413 (3.0); 3.6259 (1.3); 2.6032 (2.8); 2.5879 (4.0); 2.5733 (2.7); 2.0456 (1.0); 1.6296 (1.0); 1.6216 (1.0); 1.6164 (0.8); 1.6080 (5.3); 1.6010 (8.3); 1.5876 (1.2); 1.5745 (0.6); 1.2861 (7.6); 1.2775 (0.6); 1.2683 (16.0); 1.2597 (1.0); 1.2561 (0.5); 1.2505 (7.5); 0.8518 (1.1); 0.8409 (2.4); 0.8360 (2.8); 0.8309 (1.4); 0.8253 (1.5); 0.8197 (2.8); 0.8149 (2.5); 0.8044 (1.3); 0.6162 (1.3); 0.6055 (2.7); 0.6008 (2.9); 0.5925 (2.6); 0.5878 (2.9); 0.5767 (1.0); 0.0080 (0.6); 0.0002 (23.9); 0.0084 (0.8) I-251: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2284 (1.6); 8.2265 (1.9); 8.2248 (1.8); 8.2168 (1.7); 8.2149 (1.9); 8.2132 (1.8); 8.1313 (2.5); 8.1251 (2.5); 7.7697 (1.1); 7.7635 (1.1); 7.7505 (1.5); 7.7486 (1.4); 7.7443 (1.4); 7.7424 (1.4); 7.7296 (1.2); 7.7234 (1.2); 7.4591 (1.2); 7.4554 (1.1); 7.4384 (1.7); 7.4354 (2.2); 7.4320 (1.3); 7.4151 (1.5); 7.4114 (1.4); 7.2847 (1.4); 7.2757 (1.7); 7.2730 (1.6); 7.2613 (21.0); 7.2551 (1.3); 7.2524 (1.2); 7.2436 (1.1); 6.9201 (1.7); 6.9127 (1.8); 6.8990 (1.7); 6.8916 (1.7); 4.8932 (16.0); 4.0831 (7.4); 4.0656 (7.6); 2.2232 (1.1); 2.2044 (1.6); 2.1857 (1.2); 1.7228 (0.8); 1.7069 (1.0); 1.6906 (1.4); 1.6783 (0.8); 1.6708 (0.7); 1.6611 (0.5); 1.6119 (0.6); 1.5986 (1.3); 1.5920 (1.7); 1.5846 (1.4); 1.5780 (3.5); 1.5700 (1.6); 1.5626 (2.6); 1.5545 (7.3); 1.5465 (1.7); 1.5389 (1.1); 1.5298 (1.9); 1.5226 (1.3); 1.5138 (1.4); 1.5038 (1.0); 1.4933 (0.6); 1.4905 (0.6); 1.2523 (0.6); 1.2465 (1.1); 1.2332 (1.1); 1.2288 (1.2); 1.2148 (1.1); 1.1974 (0.9); 0.7977 (1.5); 0.7930 (4.3); 0.7898 (3.1); 0.7857 (4.5); 0.7826 (5.7); 0.7796 (5.1); 0.7751 (2.6); 0.7667 (2.6); 0.7626 (3.9); 0.7570 (1.8); 0.0079 (1.0); 0.0002 (31.9); 0.0085 (0.9) I-253: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.6065 (1.4); 8.5669 (1.0); 8.5562 (1.0); 8.2289 (1.5); 8.2270 (1.7); 8.2252 (1.7); 8.2236 (1.4); 8.2172 (1.6); 8.2153 (1.8); 8.2136 (1.7); 8.1350 (2.4); 8.1328 (1.8); 8.1307 (2.0); 8.1289 (2.4); 7.7748 (1.1); 7.7686 (1.1); 7.7558 (1.4); 7.7538 (1.4); 7.7496 (1.4); 7.7476 (1.4); 7.7348 (1.2); 7.7286 (1.2); 7.6978 (0.8); 7.6935 (1.3); 7.6881 (0.8); 7.6782 (1.0); 7.6739 (1.5); 7.6685 (0.9); 7.4677 (1.2); 7.4640 (1.2); 7.4471 (1.7); 7.4439 (2.1); 7.4405 (1.3); 7.4237 (1.6); 7.4199 (1.4); 7.2973 (1.4); 7.2883 (1.6); 7.2857 (1.4); 7.2767 (2.5); 7.2676 (2.2); 7.2635 (38.7); 7.2586 (0.7); 7.2561 (1.6); 7.2530 (1.3); 7.2452 (1.1); 7.2332 (1.0); 6.9236 (1.7); 6.9222 (1.6); 6.9162 (1.7); 6.9147 (1.5); 6.9025 (1.6); 6.9010 (1.5); 6.8951 (1.6); 6.8936 (1.4); 5.2442 (10.7); 4.9477 (16.0); 1.5842 (0.8); 1.5787 (0.9); 1.5723 (0.6); 1.5647 (1.9); 1.5579 (0.6); 1.5516 (0.7); 1.5499 (0.8); 1.5446 (0.9); 1.5305 (0.6); 0.7688 (1.5); 0.7642 (3.0); 0.7632 (3.2); 0.7588 (2.4); 0.7481 (4.0); 0.7431 (6.8); 0.7405 (3.4); 0.7392 (3.8); 0.7335 (2.8); 0.7299 (3.9); 0.7270 (1.8); 0.7247 (1.7); 0.7220 (0.8); 0.0080 (0.7); 0.0002 (23.9); 0.0085 (0.6) I-254: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2700 (0.8); 8.2681 (1.0); 8.2664 (1.0); 8.2645 (0.9); 8.2584 (0.8); 8.2565 (1.0); 8.2548 (1.0); 8.2529 (0.9); 8.1492 (1.2); 8.1473 (1.0); 8.1451 (1.0); 8.1430 (1.3); 7.7664 (0.6); 7.7601 (0.6); 7.7475 (0.7); 7.7453 (0.8); 7.7413 (0.7); 7.7391 (0.8); 7.7264 (0.7); 7.7201 (0.7); 7.4901 (0.7); 7.4863 (0.7); 7.4694 (0.9); 7.4658 (1.1); 7.4632 (0.8); 7.4463 (0.9); 7.4426 (0.9); 7.3315 (0.9); 7.3224 (1.0); 7.3199 (0.9); 7.3108 (1.5); 7.3018 (0.7); 7.2992 (0.7); 7.2901 (0.6); 7.2633 (12.8); 6.9303 (0.8); 6.9288 (0.9); 6.9229 (0.9); 6.9214 (0.9); 6.9093 (0.8); 6.9077 (0.9); 6.9018 (0.8); 6.9002 (0.8); 4.8742 (7.0); 4.1735 (3.2); 4.1608 (3.2); 3.8018 (16.0); 1.6496 (0.6); 1.6417 (0.6); 1.6287 (1.2); 1.6154 (0.6); 1.6077 (0.7); 1.5849 (5.0); 0.8728 (0.7); 0.8619 (1.4); 0.8569 (1.7); 0.8518 (0.8); 0.8463 (0.9); 0.8406 (1.6); 0.8357 (1.4); 0.8253 (0.8); 0.6547 (0.8); 0.6440 (1.6); 0.6412 (1.3); 0.6392 (1.7); 0.6310 (1.5); 0.6280 (1.2); 0.6262 (1.7); 0.6152 (0.6); 0.0080 (0.6); 0.0023 (0.7); 0.0002 (18.7); 0.0084 (0.5) I-255: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4608 (1.2); 8.4567 (1.3); 8.4491 (1.2); 8.4448 (1.3); 8.1404 (2.0); 8.1343 (2.2); 8.1164 (1.3); 8.1125 (1.4); 8.0969 (1.4); 8.0923 (1.4); 7.7864 (1.0); 7.7803 (0.9); 7.7674 (1.1); 7.7654 (1.2); 7.7612 (1.1); 7.7592 (1.2); 7.7464 (1.0); 7.7402 (1.0); 7.4001 (1.0); 7.3898 (1.0); 7.3821 (1.0); 7.3684 (1.0); 7.2605 (88.4); 6.9133 (1.4); 6.9058 (1.4); 6.8921 (1.3); 6.8847 (1.3); 5.3002 (2.0); 4.9466 (0.7); 4.8840 (13.2); 2.1081 (1.1); 2.0462 (1.1); 1.5898 (0.7); 1.5776 (0.6); 1.5720 (1.6); 1.5657 (0.6); 1.5556 (0.8); 1.5377 (0.6); 1.4322 (1.2); 1.2597 (0.8); 1.2226 (0.8); 0.7916 (3.5); 0.7893 (3.6); 0.7870 (3.6); 0.7848 (3.9); 0.7710 (16.0); 0.0080 (2.9); 0.0002 (110.8); 0.0085 (3.2) I-256: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4746 (0.7); 8.4703 (0.7); 8.4627 (0.8); 8.4583 (0.8); 8.1488 (0.8); 8.1444 (0.8); 8.1286 (0.8); 8.1247 (0.9); 8.1131 (1.1); 8.1108 (0.8); 8.1087 (0.9); 8.1068 (1.2); 7.8495 (0.6); 7.8432 (0.6); 7.8307 (0.7); 7.8282 (0.7); 7.8245 (0.7); 7.8220 (0.7); 7.8095 (0.6); 7.8033 (0.6); 7.4517 (0.6); 7.4500 (0.6); 7.4397 (0.6); 7.4380 (0.6); 7.4319 (0.6); 7.4302 (0.6); 7.4199 (0.6); 7.4182 (0.5); 7.2617 (13.6); 6.9524 (0.8); 6.9509 (0.8); 6.9449 (0.8); 6.9434 (0.8); 6.9312 (0.8); 6.9297 (0.7); 6.9237 (0.8); 6.9222 (0.8); 5.1721 (1.6); 5.1546 (1.6); 4.4618 (0.6); 4.4504 (0.8); 4.4340 (1.7); 4.4253 (0.8); 4.4176 (0.8); 4.4093 (1.7); 4.3934 (0.8); 4.3816 (0.6); 3.6782 (1.1); 3.6744 (16.0); 2.6586 (1.9); 2.6425 (3.8); 2.6263 (1.8); 1.6747 (5.9); 1.6690 (0.5); 1.6573 (5.8); 1.5568 (7.1); 0.0080 (0.5); 0.0002 (20.6); 0.0085 (0.5) I-257: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4918 (0.7); 8.4883 (0.7); 8.4799 (0.8); 8.4762 (0.8); 8.1483 (1.1); 8.1448 (1.1); 8.1287 (1.2); 8.1250 (1.2); 8.1066 (1.3); 8.1043 (1.3); 8.1004 (1.7); 8.0982 (1.3); 8.0958 (0.8); 7.8539 (0.6); 7.8477 (0.6); 7.8353 (1.0); 7.8327 (0.8); 7.8290 (0.8); 7.8265 (0.8); 7.8230 (0.6); 7.8205 (0.5); 7.8141 (1.0); 7.8078 (0.7); 7.4625 (0.6); 7.4522 (0.6); 7.4505 (0.6); 7.4427 (0.6); 7.4399 (0.5); 7.4307 (0.7); 7.2613 (28.8); 6.9516 (1.3); 6.9442 (1.3); 6.9304 (1.3); 6.9229 (1.3); 5.2491 (1.0); 5.2409 (1.8); 5.2316 (1.0); 5.2235 (1.8); 5.2062 (0.5); 5.1907 (0.9); 5.1730 (0.9); 5.1632 (1.5); 5.1455 (1.5); 3.7562 (1.5); 3.7336 (9.4); 3.7033 (16.0); 3.6744 (0.5); 1.7657 (3.4); 1.7482 (3.7); 1.7446 (6.2); 1.7271 (5.8); 1.7212 (0.6); 1.6903 (0.6); 1.6730 (0.7); 1.5524 (14.9); 1.4981 (3.6); 1.4804 (9.9); 1.4627 (6.4); 0.0080 (1.1); 0.0002 (40.6); 0.0058 (0.7); 0.0085 (1.2) I-258: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4345 (1.2); 8.4306 (1.3); 8.4225 (1.3); 8.4186 (1.3); 8.1337 (2.1); 8.1274 (2.2); 8.1068 (1.4); 8.1025 (1.4); 8.0871 (1.5); 8.0827 (1.4); 7.7809 (1.0); 7.7747 (1.0); 7.7618 (1.2); 7.7599 (1.3); 7.7557 (1.2); 7.7537 (1.2); 7.7408 (1.1); 7.7346 (1.1); 7.3747 (1.0); 7.3730 (1.0); 7.3627 (1.0); 7.3610 (1.0); 7.3550 (1.0); 7.3533 (1.0); 7.3430 (1.0); 7.3413 (1.0); 7.2611 (25.0); 6.9083 (1.3); 6.9069 (1.4); 6.9009 (1.4); 6.8995 (1.4); 6.8872 (1.3); 6.8858 (1.4); 6.8798 (1.4); 6.8784 (1.3); 4.8771 (0.8); 4.8219 (14.7); 4.2614 (2.1); 4.2436 (6.1); 4.2258 (6.0); 4.2079 (1.9); 3.9304 (0.5); 1.5934 (0.9); 1.5860 (1.0); 1.5767 (0.7); 1.5728 (1.6); 1.5647 (0.6); 1.5591 (1.0); 1.5523 (16.0); 1.5384 (0.6); 1.2988 (0.7); 1.2950 (7.4); 1.2872 (0.6); 1.2810 (1.4); 1.2771 (15.4); 1.2632 (1.6); 1.2593 (7.9); 0.8988 (0.6); 0.8819 (2.0); 0.8642 (0.8); 0.8425 (0.6); 0.8284 (2.1); 0.8232 (2.1); 0.8160 (3.2); 0.8099 (2.1); 0.8024 (2.0); 0.7936 (2.0); 0.7918 (1.4); 0.7863 (2.0); 0.7817 (1.4); 0.7731 (2.1); 0.7659 (2.2); 0.7603 (1.7); 0.7468 (0.8); 0.0080 (0.9); 0.0002 (35.2); 0.0085 (1.0) I-259: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2694 (1.2); 8.2675 (1.4); 8.2658 (1.4); 8.2641 (1.2); 8.2577 (1.2); 8.2559 (1.4); 8.2541 (1.4); 8.2525 (1.1); 8.1489 (1.9); 8.1468 (1.5); 8.1446 (1.5); 8.1427 (2.0); 7.7658 (0.9); 7.7596 (0.9); 7.7469 (1.1); 7.7447 (1.2); 7.7407 (1.1); 7.7385 (1.1); 7.7258 (1.0); 7.7196 (1.0); 7.4888 (1.0); 7.4851 (1.0); 7.4682 (1.4); 7.4647 (1.6); 7.4619 (1.1); 7.4450 (1.3); 7.4413 (1.3); 7.3301 (1.2); 7.3210 (1.3); 7.3185 (1.2); 7.3094 (2.0); 7.3004 (0.9); 7.2979 (0.9); 7.2888 (0.9); 7.2643 (31.5); 7.0965 (0.6); 6.9294 (1.2); 6.9280 (1.3); 6.9220 (1.3); 6.9206 (1.2); 6.9083 (1.2); 6.9068 (1.2); 6.9008 (1.3); 6.8994 (1.2); 4.8727 (10.6); 4.2865 (1.7); 4.2687 (5.6); 4.2508 (5.6); 4.2330 (1.8); 4.1545 (5.0); 4.1420 (5.0); 2.0454 (1.6); 1.6489 (0.9); 1.6410 (1.0); 1.6358 (0.6); 1.6280 (2.0); 1.6200 (1.0); 1.6147 (1.8); 1.6070 (1.6); 1.5939 (0.7); 1.3277 (7.6); 1.3099 (16.0); 1.2920 (7.5); 1.2774 (0.6); 1.2595 (1.1); 0.8713 (1.1); 0.8605 (2.3); 0.8555 (2.6); 0.8503 (1.2); 0.8448 (1.4); 0.8392 (2.5); 0.8343 (2.1); 0.8239 (1.2); 0.6563 (1.3); 0.6456 (2.5); 0.6428 (2.0); 0.6409 (2.5); 0.6326 (2.3); 0.6279 (2.5); 0.6167 (0.9); 0.0080 (0.6); 0.0002 (19.8); 0.0085 (0.5) I-261: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1763 (0.7); 8.1744 (1.1); 8.1724 (0.9); 8.1704 (0.9); 8.1682 (1.1); 8.1662 (0.8); 8.0545 (0.7); 8.0524 (0.8); 8.0497 (0.8); 8.0476 (0.8); 8.0423 (0.8); 8.0402 (0.8); 8.0376 (0.8); 8.0355 (0.8); 7.8185 (0.6); 7.8123 (0.6); 7.7995 (0.7); 7.7975 (0.8); 7.7934 (0.7); 7.7913 (0.7); 7.7785 (0.6); 7.7723 (0.6); 7.7543 (0.6); 7.7495 (0.6); 7.7359 (0.7); 7.7336 (1.0); 7.7312 (0.7); 7.7289 (1.0); 7.7153 (1.0); 7.7105 (1.0); 7.6411 (1.0); 7.6386 (1.7); 7.6363 (1.1); 7.6204 (0.7); 7.6181 (1.2); 7.6157 (0.7); 7.2610 (18.6); 7.0848 (0.8); 7.0822 (0.8); 7.0727 (0.8); 7.0700 (0.8); 7.0665 (0.8); 7.0638 (0.8); 7.0544 (0.8); 7.0517 (0.8); 6.9887 (0.8); 6.9871 (0.8); 6.9813 (0.8); 6.9798 (0.8); 6.9676 (0.7); 6.9660 (0.8); 6.9602 (0.8); 6.9587 (0.7); 5.3001 (0.9); 4.9226 (3.8); 4.9153 (3.8); 4.5089 (1.8); 4.4932 (4.0); 4.4776 (2.0); 3.6913 (16.0); 2.7127 (1.9); 2.6971 (3.7); 2.6814 (1.8); 2.3256 (0.9); 2.3059 (0.9); 1.8381 (0.5); 1.8183 (0.6); 1.5511 (2.7); 0.0080 (0.8); 0.0002 (28.8); 0.0085 (0.8) I-263: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2909 (1.8); 8.2891 (2.2); 8.2872 (2.3); 8.2856 (2.1); 8.2792 (2.0); 8.2775 (2.3); 8.2755 (2.3); 8.2740 (2.0); 8.1031 (3.0); 8.0969 (3.1); 7.7738 (1.3); 7.7676 (1.3); 7.7550 (1.5); 7.7527 (1.7); 7.7488 (1.5); 7.7464 (1.6); 7.7340 (1.4); 7.7277 (1.4); 7.4886 (1.4); 7.4849 (1.5); 7.4679 (2.0); 7.4643 (2.4); 7.4619 (1.8); 7.4448 (1.9); 7.4411 (1.9); 7.3470 (1.9); 7.3379 (2.2); 7.3354 (2.0); 7.3263 (3.3); 7.3172 (1.5); 7.3147 (1.5); 7.3056 (1.4); 7.2619 (18.8); 6.9569 (1.8); 6.9555 (2.0); 6.9496 (2.0); 6.9482 (2.0); 6.9358 (1.8); 6.9343 (1.9); 6.9284 (1.8); 6.9270 (1.8); 5.0301 (0.7); 4.9967 (0.7); 4.9694 (16.0); 2.4525 (0.9); 2.4327 (1.0); 2.4233 (1.9); 2.4035 (2.0); 2.3939 (1.1); 2.3742 (1.0); 1.8223 (0.8); 1.8113 (1.1); 1.8022 (0.6); 1.7919 (1.3); 1.7806 (1.1); 1.7704 (0.8); 1.7609 (0.7); 1.7533 (1.0); 1.7402 (1.0); 1.7337 (0.6); 1.7236 (0.6); 1.7206 (0.6); 1.7106 (0.6); 1.4321 (4.4); 0.8818 (0.7); 0.0080 (0.7); 0.0002 (24.3); 0.0085 (0.6) I-264: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2284 (1.9); 8.2168 (1.9); 8.1346 (2.6); 8.1285 (2.6); 7.7697 (1.1); 7.7635 (1.1); 7.7487 (1.5); 7.7425 (1.4); 7.7296 (1.2); 7.7234 (1.2); 7.4706 (1.2); 7.4669 (1.2); 7.4500 (1.6); 7.4468 (2.3); 7.4435 (1.3); 7.4266 (1.5); 7.4229 (1.4); 7.2946 (1.3); 7.2855 (1.7); 7.2829 (1.6); 7.2739 (2.6); 7.2611 (29.9); 7.2535 (1.1); 6.9196 (1.7); 6.9130 (1.7); 6.8992 (1.6); 6.8919 (1.6); 4.9088 (16.0); 4.7631 (4.4); 4.7474 (5.2); 4.7435 (4.9); 4.7277 (4.9); 4.4560 (4.2); 4.4406 (7.8); 4.4249 (4.7); 4.4214 (7.6); 4.4046 (7.5); 3.3342 (0.8); 3.3308 (0.9); 3.3147 (1.4); 3.2983 (0.9); 1.5960 (0.8); 1.5928 (0.8); 1.5846 (0.6); 1.5778 (2.0); 1.5708 (0.8); 1.5546 (7.8); 1.5436 (0.8); 0.8821 (0.8); 0.7811 (4.4); 0.7779 (3.3); 0.7740 (3.3); 0.7711 (4.4); 0.7656 (2.7); 0.7590 (10.5); 0.0079 (1.6); 0.0002 (41.4); 0.0084 (1.1) I-265: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2312 (1.3); 8.2293 (1.5); 8.2276 (1.5); 8.2258 (1.4); 8.2196 (1.4); 8.2177 (1.5); 8.2159 (1.5); 8.2142 (1.4); 8.0739 (2.0); 8.0677 (2.0); 7.7515 (1.0); 7.7453 (0.9); 7.7324 (1.1); 7.7304 (1.2); 7.7263 (1.2); 7.7242 (1.2); 7.7114 (1.0); 7.7052 (1.0); 7.4688 (1.1); 7.4651 (1.2); 7.4482 (1.5); 7.4445 (1.7); 7.4420 (1.3); 7.4251 (1.4); 7.4213 (1.4); 7.3037 (1.3); 7.2947 (1.4); 7.2921 (1.4); 7.2830 (2.3); 7.2741 (1.1); 7.2714 (1.2); 7.2613 (38.0); 6.8867 (1.4); 6.8852 (1.5); 6.8793 (1.5); 6.8778 (1.4); 6.8656 (1.4); 6.8641 (1.4); 6.8582 (1.4); 6.8567 (1.3); 5.1293 (0.6); 5.1255 (2.0); 5.1212 (2.8); 5.1170 (2.2); 5.1132 (0.6); 5.0671 (2.3); 5.0648 (2.8); 5.0624 (2.6); 5.0601 (2.0); 4.9559 (0.8); 4.9328 (0.8); 4.9257 (15.5); 4.2804 (2.2); 4.2626 (6.3); 4.2581 (0.6); 4.2447 (6.2); 4.2402 (0.6); 4.2269 (2.0); 1.9345 (7.5); 1.9322 (9.9); 1.9308 (9.7); 1.9285 (7.7); 1.5542 (14.5); 1.3009 (7.8); 1.2954 (1.3); 1.2831 (16.0); 1.2774 (1.3); 1.2653 (7.6); 1.2595 (0.5); 0.0080 (1.3); 0.0002 (52.6); 0.0085 (1.5) I-266: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.0994 (1.0); 8.2740 (2.1); 8.2718 (2.6); 8.2708 (2.6); 8.2686 (2.1); 8.2625 (2.2); 8.2602 (2.8); 8.2570 (2.0); 8.2312 (3.3); 8.2249 (3.4); 7.9952 (1.9); 7.9920 (2.7); 7.9863 (1.5); 7.9740 (3.2); 7.9708 (4.5); 7.9667 (3.5); 7.9521 (1.8); 7.9493 (2.2); 7.9457 (3.4); 7.6129 (2.0); 7.6035 (2.3); 7.6013 (2.0); 7.5919 (3.5); 7.5827 (1.7); 7.5804 (1.8); 7.5711 (1.5); 7.2950 (2.1); 7.2893 (2.1); 7.2881 (2.0); 7.2749 (2.0); 7.2736 (2.1); 7.2680 (2.0); 7.2667 (1.9); 4.8684 (16.0); 3.3233 (2.6); 2.5252 (0.8); 2.5205 (1.3); 2.5118 (17.2); 2.5073 (37.7); 2.5026 (52.3); 2.4980 (36.4); 2.4934 (15.7); 1.3563 (0.9); 1.2468 (0.6); 0.8579 (1.1); 0.0080 (2.1); 0.0056 (0.8); 0.0048 (1.0); 0.0002 (65.8); 0.0085 (1.7) I-267: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2135 (0.7); 8.2117 (1.0); 8.2094 (0.8); 8.2075 (0.8); 8.2055 (1.1); 8.2033 (0.8); 8.0399 (0.7); 8.0376 (0.8); 8.0353 (0.8); 8.0331 (0.7); 8.0277 (0.7); 8.0255 (0.8); 8.0231 (0.8); 8.0209 (0.7); 7.8641 (0.6); 7.8579 (0.6); 7.8452 (0.7); 7.8430 (0.8); 7.8390 (0.8); 7.8368 (0.8); 7.8241 (1.0); 7.8209 (0.8); 7.8184 (0.9); 7.8034 (1.2); 7.8010 (1.6); 7.8004 (1.4); 7.7979 (1.0); 7.7839 (1.0); 7.7793 (1.0); 7.7662 (1.0); 7.7615 (1.0); 7.7455 (0.5); 7.7407 (0.6); 7.2620 (8.3); 7.1010 (0.8); 7.0976 (0.9); 7.0888 (0.8); 7.0856 (0.8); 7.0834 (0.8); 7.0800 (0.8); 7.0711 (0.7); 7.0679 (0.7); 6.9944 (0.9); 6.9928 (0.9); 6.9871 (0.9); 6.9855 (0.9); 6.9733 (0.9); 6.9717 (0.9); 6.9659 (0.9); 6.9643 (0.8); 5.3531 (1.7); 5.3356 (1.8); 5.3179 (0.5); 5.3001 (3.6); 5.2121 (1.4); 5.1945 (1.4); 3.7264 (4.0); 3.7239 (16.0); 1.7872 (1.1); 1.7697 (1.2); 1.7635 (5.7); 1.7460 (5.6); 1.5606 (1.4); 1.5429 (1.3); 1.5269 (6.5); 1.5093 (6.4); 0.0002 (12.7) I-268: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1715 (1.8); 8.1694 (1.4); 8.1673 (1.5); 8.1653 (1.9); 8.0537 (1.1); 8.0516 (1.3); 8.0490 (1.3); 8.0468 (1.2); 8.0415 (1.2); 8.0395 (1.3); 8.0368 (1.3); 8.0347 (1.2); 7.8170 (1.0); 7.8108 (1.0); 7.7980 (1.2); 7.7960 (1.2); 7.7918 (1.2); 7.7898 (1.2); 7.7770 (1.1); 7.7708 (1.0); 7.7509 (0.8); 7.7462 (0.8); 7.7325 (1.0); 7.7302 (1.3); 7.7278 (1.1); 7.7255 (1.3); 7.7119 (1.3); 7.7072 (1.3); 7.6371 (1.6); 7.6347 (2.7); 7.6323 (1.6); 7.6164 (1.1); 7.6141 (1.9); 7.6116 (1.0); 7.2614 (21.2); 7.0838 (1.3); 7.0812 (1.3); 7.0717 (1.2); 7.0691 (1.3); 7.0656 (1.3); 7.0629 (1.2); 7.0534 (1.2); 7.0508 (1.2); 6.9889 (1.3); 6.9875 (1.3); 6.9816 (1.3); 6.9802 (1.3); 6.9679 (1.2); 6.9664 (1.3); 6.9606 (1.2); 6.9590 (1.2); 5.3000 (0.5); 4.9240 (3.4); 4.9208 (3.6); 4.9170 (5.1); 4.4180 (0.6); 4.4129 (0.6); 4.4002 (0.6); 4.3951 (0.7); 4.3909 (1.2); 4.3858 (1.2); 4.3731 (1.2); 4.3680 (1.2); 4.3301 (1.2); 4.3271 (1.2); 4.3160 (1.3); 4.3131 (1.2); 4.3030 (0.7); 4.3000 (0.7); 4.2889 (0.7); 4.2860 (0.7); 3.8162 (1.0); 3.7261 (1.4); 3.6942 (0.5); 3.6827 (16.0); 3.6812 (15.8); 2.8597 (0.7); 2.8456 (0.8); 2.8418 (1.2); 2.8277 (1.2); 2.8240 (0.8); 2.8098 (0.8); 2.3563 (0.6); 2.3365 (0.8); 2.3269 (1.4); 2.3071 (1.5); 2.2975 (0.7); 2.2777 (0.7); 1.8341 (0.6); 1.8318 (0.6); 1.8142 (0.6); 1.8120 (0.6); 1.6960 (0.6); 1.6832 (0.6); 1.5582 (1.5); 1.2027 (8.0); 1.2022 (7.9); 1.1981 (1.3); 1.1848 (7.9); 1.1844 (7.7); 1.1799 (1.2); 0.0079 (1.0); 0.0002 (34.1); 0.0028 (1.2); 0.0085 (0.9) I-269: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4890 (0.8); 8.4853 (1.0); 8.4777 (0.9); 8.4733 (1.0); 8.1496 (1.0); 8.1453 (1.0); 8.1296 (1.2); 8.1254 (1.2); 8.1177 (1.6); 8.1157 (1.2); 8.1135 (1.2); 8.1115 (1.6); 7.8548 (0.8); 7.8486 (0.7); 7.8361 (0.9); 7.8335 (1.0); 7.8299 (1.0); 7.8273 (0.8); 7.8149 (0.8); 7.8086 (0.7); 7.4638 (0.8); 7.4621 (0.8); 7.4518 (0.8); 7.4501 (0.8); 7.4440 (0.8); 7.4424 (0.8); 7.4320 (0.7); 7.4304 (0.7); 7.2621 (13.9); 6.9569 (1.0); 6.9554 (1.0); 6.9495 (1.1); 6.9480 (1.1); 6.9356 (1.0); 6.9341 (1.0); 6.9282 (1.0); 6.9267 (1.0); 5.2242 (2.1); 5.2067 (2.1); 5.1893 (0.5); 4.1500 (1.1); 4.1321 (3.2); 4.1143 (3.3); 4.0965 (1.1); 3.7264 (1.4); 2.1063 (6.8); 2.0467 (16.0); 1.7417 (7.3); 1.7361 (0.8); 1.7242 (7.2); 1.7186 (0.7); 1.4321 (1.4); 1.2773 (4.8); 1.2594 (9.8); 1.2416 (4.8); 0.0080 (0.6); 0.0002 (20.4); 0.0085 (0.5) I-270: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2229 (1.4); 8.2209 (1.6); 8.2192 (1.6); 8.2174 (1.4); 8.2112 (1.5); 8.2093 (1.7); 8.2075 (1.6); 8.2057 (1.4); 8.1360 (2.1); 8.1340 (1.6); 8.1319 (1.7); 8.1299 (2.2); 7.7715 (1.1); 7.7653 (1.1); 7.7525 (1.3); 7.7504 (1.4); 7.7463 (1.3); 7.7442 (1.3); 7.7314 (1.2); 7.7252 (1.1); 7.4651 (1.2); 7.4614 (1.2); 7.4445 (1.6); 7.4411 (2.0); 7.4379 (1.3); 7.4210 (1.5); 7.4173 (1.4); 7.2905 (1.5); 7.2815 (1.6); 7.2788 (1.5); 7.2699 (2.7); 7.2614 (28.2); 7.2583 (1.6); 7.2493 (1.1); 6.9215 (1.5); 6.9200 (1.5); 6.9140 (1.5); 6.9125 (1.5); 6.9004 (1.4); 6.8988 (1.4); 6.8929 (1.5); 6.8914 (1.4); 4.9405 (16.0); 4.4301 (2.0); 4.4189 (2.6); 4.4067 (2.4); 4.1743 (4.6); 4.1686 (1.2); 4.1657 (2.1); 4.1623 (4.0); 4.1598 (2.2); 4.1569 (1.2); 4.1507 (3.7); 3.7845 (0.8); 1.6112 (0.5); 1.5977 (0.6); 1.5950 (0.9); 1.5928 (0.9); 1.5909 (0.9); 1.5830 (1.4); 1.5769 (4.0); 1.5639 (1.1); 1.5608 (1.2); 1.5587 (1.0); 1.5567 (0.9); 1.5429 (0.6); 0.8341 (0.5); 0.7864 (1.2); 0.7821 (3.9); 0.7793 (3.4); 0.7767 (3.4); 0.7741 (4.0); 0.7693 (1.4); 0.7609 (16.0); 0.0079 (1.0); 0.0002 (35.4); 0.0085 (0.9) I-272: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1154 (0.5); 7.2632 (5.8); 4.8819 (3.6); 4.4830 (0.9); 4.4668 (1.9); 4.4507 (0.9); 3.6923 (7.0); 3.4905 (16.0); 2.6940 (0.9); 2.6779 (1.8); 2.6618 (0.8); 0.0002 (8.8) I-273: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1536 (1.9); 8.1516 (1.5); 8.1496 (1.5); 8.1475 (1.9); 8.1455 (1.3); 8.0303 (1.1); 8.0282 (1.2); 8.0256 (1.4); 8.0235 (1.2); 8.0182 (1.2); 8.0161 (1.3); 8.0135 (1.3); 8.0114 (1.2); 7.7907 (1.1); 7.7845 (1.1); 7.7716 (1.2); 7.7697 (1.4); 7.7654 (1.2); 7.7635 (1.3); 7.7506 (1.2); 7.7444 (1.1); 7.7298 (1.0); 7.7251 (1.0); 7.7117 (1.1); 7.7091 (1.6); 7.7070 (1.1); 7.7044 (1.6); 7.6910 (1.8); 7.6863 (1.7); 7.6472 (1.6); 7.6447 (2.8); 7.6423 (1.8); 7.6265 (1.0); 7.6241 (1.6); 7.6216 (0.9); 7.2618 (10.8); 7.0561 (1.3); 7.0532 (1.3); 7.0439 (1.3); 7.0411 (1.3); 7.0380 (1.4); 7.0351 (1.2); 7.0258 (1.3); 7.0230 (1.2); 6.9818 (1.3); 6.9803 (1.4); 6.9745 (1.4); 6.9729 (1.4); 6.9608 (1.3); 6.9592 (1.4); 6.9534 (1.3); 6.9519 (1.3); 6.2758 (1.7); 6.2469 (2.1); 6.2315 (2.6); 6.2026 (2.4); 5.9616 (2.6); 5.9569 (2.7); 5.9173 (2.0); 5.9127 (1.9); 5.2668 (2.5); 5.2622 (2.2); 5.2380 (2.1); 5.2333 (2.3); 4.9764 (14.7); 4.3304 (1.8); 4.3126 (5.8); 4.2947 (5.9); 4.2769 (1.9); 1.5727 (2.3); 1.3412 (7.7); 1.3234 (16.0); 1.3056 (7.5); 1.2643 (0.6); 0.8817 (1.3); 0.0002 (15.2) I-274: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2190 (1.8); 8.2081 (1.9); 8.1306 (2.5); 8.1245 (2.6); 7.7708 (1.1); 7.7646 (1.1); 7.7498 (1.5); 7.7453 (1.4); 7.7307 (1.2); 7.7245 (1.1); 7.4619 (1.1); 7.4582 (1.1); 7.4412 (1.5); 7.4380 (2.2); 7.4349 (1.2); 7.4179 (1.4); 7.4142 (1.4); 7.2850 (1.4); 7.2759 (1.7); 7.2734 (1.6); 7.2615 (21.9); 7.2555 (1.5); 7.2529 (1.3); 7.2439 (1.0); 6.9187 (1.7); 6.9116 (1.7); 6.8977 (1.6); 6.8905 (1.6); 4.9345 (16.0); 4.2554 (0.5); 4.2488 (1.6); 4.2308 (2.4); 4.2242 (1.3); 4.2150 (0.5); 4.2109 (0.5); 4.1745 (1.9); 4.1598 (3.6); 4.1463 (1.5); 4.1418 (0.9); 4.1358 (3.4); 4.1307 (1.7); 4.1220 (0.8); 4.1151 (0.7); 3.8902 (0.8); 3.8732 (1.6); 3.8693 (1.4); 3.8566 (1.0); 3.8524 (2.2); 3.8361 (1.1); 3.7959 (1.1); 3.7785 (1.6); 3.7624 (1.3); 3.7578 (1.1); 3.7420 (0.6); 1.9670 (0.7); 1.9502 (0.9); 1.9377 (0.7); 1.9229 (0.6); 1.9159 (0.7); 1.9045 (0.7); 1.9008 (1.0); 1.8963 (0.8); 1.8865 (1.7); 1.8697 (1.6); 1.8659 (1.6); 1.8491 (1.2); 1.6426 (0.8); 1.6295 (0.6); 1.6211 (0.8); 1.6088 (1.0); 1.6046 (0.6); 1.5933 (1.4); 1.5887 (1.1); 1.5816 (0.8); 1.5746 (2.5); 1.5630 (5.4); 1.5553 (1.3); 1.5404 (0.6); 0.7845 (4.7); 0.7797 (5.6); 0.7728 (4.2); 0.7692 (2.5); 0.7629 (2.6); 0.7594 (4.0); 0.0077 (0.9); 0.0002 (31.0); 0.0085 (1.1) I-275: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2024 (0.8); 8.2004 (1.1); 8.1984 (0.8); 8.1963 (0.8); 8.1942 (1.1); 8.1922 (0.7); 8.0656 (0.7); 8.0636 (0.7); 8.0609 (0.8); 8.0588 (0.7); 8.0535 (0.7); 8.0514 (0.8); 8.0488 (0.8); 8.0467 (0.7); 7.8599 (0.6); 7.8537 (0.6); 7.8409 (0.7); 7.8388 (0.9); 7.8348 (0.7); 7.8326 (0.7); 7.8198 (0.7); 7.8136 (0.6); 7.7610 (0.7); 7.7561 (0.6); 7.7425 (0.7); 7.7402 (0.9); 7.7378 (0.7); 7.7355 (0.8); 7.7218 (0.9); 7.7171 (0.8); 7.6274 (0.9); 7.6250 (1.6); 7.6227 (1.0); 7.6067 (0.7); 7.6044 (1.2); 7.6020 (0.7); 7.2620 (8.6); 7.1092 (0.8); 7.1066 (0.8); 7.0971 (0.8); 7.0944 (0.8); 7.0908 (0.8); 7.0882 (0.8); 7.0787 (0.8); 7.0760 (0.7); 6.9942 (0.9); 6.9927 (0.9); 6.9869 (0.9); 6.9854 (0.9); 6.9731 (0.9); 6.9716 (0.9); 6.9657 (0.9); 6.9642 (0.8); 5.3341 (1.8); 5.3166 (1.8); 5.3000 (3.8); 5.2536 (1.4); 5.2360 (1.5); 3.8014 (0.5); 3.7264 (16.0); 3.7239 (4.1); 1.7871 (5.8); 1.7697 (5.7); 1.7634 (1.4); 1.7459 (1.2); 1.5605 (6.7); 1.5428 (6.6); 1.5268 (1.4); 1.5092 (1.3); 0.0002 (12.1) I-276: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2272 (1.2); 8.2253 (1.0); 8.2232 (1.0); 8.2210 (1.2); 7.8837 (0.6); 7.8775 (0.6); 7.8647 (0.7); 7.8626 (0.8); 7.8585 (0.7); 7.8565 (0.8); 7.8436 (0.7); 7.8374 (0.6); 7.6472 (1.0); 7.6274 (1.6); 7.6081 (1.3); 7.4343 (1.4); 7.4141 (1.2); 7.2610 (19.6); 6.9965 (0.8); 6.9950 (0.9); 6.9891 (0.8); 6.9877 (0.9); 6.9753 (0.8); 6.9738 (0.9); 6.9679 (0.8); 6.9665 (0.8); 6.9523 (1.3); 6.9335 (1.2); 4.9450 (8.5); 4.5216 (2.0); 4.5058 (4.2); 4.4901 (2.1); 3.6867 (16.0); 2.7183 (2.0); 2.7026 (4.0); 2.6868 (1.9); 2.1562 (9.5); 1.5699 (1.8); 0.0080 (0.8); 0.0002 (28.0); 0.0085 (0.7) I-277: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2103 (0.9); 8.2081 (0.7); 8.2060 (0.8); 8.2043 (0.9); 7.8703 (0.5); 7.8513 (0.6); 7.8492 (0.6); 7.8451 (0.6); 7.8430 (0.6); 7.8302 (0.5); 7.8240 (0.5); 7.6302 (0.8); 7.6104 (1.2); 7.5910 (1.0); 7.4357 (1.1); 7.4154 (0.8); 7.2613 (10.4); 6.9944 (0.6); 6.9929 (0.6); 6.9870 (0.7); 6.9856 (0.6); 6.9733 (0.6); 6.9717 (0.6); 6.9659 (0.6); 6.9644 (0.6); 6.9403 (1.0); 6.9216 (1.0); 4.9978 (6.7); 4.3947 (1.6); 4.3865 (0.8); 4.3831 (1.6); 4.3793 (0.8); 4.3713 (1.7); 3.6503 (2.0); 3.6436 (0.7); 3.6423 (0.9); 3.6386 (1.7); 3.6351 (0.9); 3.6270 (1.8); 3.3802 (16.0); 2.1428 (7.3); 1.5668 (1.2); 0.0002 (13.9); 0.0027 (0.6) I-278: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2207 (0.7); 8.2188 (1.1); 8.2168 (0.9); 8.2147 (0.9); 8.2126 (1.1); 8.2107 (0.8); 7.8773 (0.6); 7.8712 (0.6); 7.8583 (0.7); 7.8562 (0.8); 7.8522 (0.7); 7.8501 (0.8); 7.8372 (0.7); 7.8311 (0.7); 7.6438 (1.0); 7.6239 (1.5); 7.6047 (1.2); 7.4378 (1.3); 7.4175 (1.1); 7.2617 (11.6); 6.9955 (0.8); 6.9940 (0.8); 6.9881 (0.8); 6.9866 (0.8); 6.9744 (0.8); 6.9729 (0.8); 6.9670 (0.8); 6.9655 (0.8); 6.9471 (1.2); 6.9284 (1.1); 4.9437 (8.1); 4.5198 (2.0); 4.5040 (4.1); 4.4883 (2.0); 3.6867 (16.0); 2.7171 (1.9); 2.7014 (3.9); 2.6856 (1.8); 2.1463 (8.9); 1.5779 (1.0); 0.0002 (16.7) I-279: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2196 (0.9); 8.2176 (0.7); 8.2156 (0.7); 8.2135 (0.9); 7.8776 (0.5); 7.8586 (0.6); 7.8565 (0.6); 7.8524 (0.6); 7.8503 (0.6); 7.8375 (0.6); 7.8313 (0.5); 7.6341 (0.8); 7.6142 (1.2); 7.5950 (1.0); 7.4318 (1.0); 7.4115 (0.8); 7.2605 (37.0); 7.2564 (1.0); 7.2547 (0.6); 6.9956 (0.7); 6.9940 (0.7); 6.9881 (0.7); 6.9866 (0.7); 6.9744 (0.6); 6.9729 (0.6); 6.9670 (0.6); 6.9655 (0.6); 6.9457 (1.0); 6.9270 (0.9); 4.9989 (6.7); 4.3965 (1.6); 4.3885 (0.8); 4.3850 (1.6); 4.3812 (0.8); 4.3732 (1.7); 3.6508 (2.0); 3.6428 (0.9); 3.6390 (1.7); 3.6356 (0.9); 3.6274 (1.9); 3.3807 (16.0); 2.1530 (7.2); 1.5634 (3.4); 0.0080 (1.4); 0.0002 (53.3); 0.0085 (1.5) I-280: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5199 (1.8); 8.5066 (1.8); 8.2588 (1.4); 8.2569 (1.7); 8.2552 (1.7); 8.2534 (1.5); 8.2472 (1.5); 8.2453 (1.7); 8.2435 (1.7); 8.2418 (1.5); 8.1399 (2.4); 8.1338 (2.5); 7.7601 (1.2); 7.7538 (1.2); 7.7411 (1.4); 7.7390 (1.5); 7.7349 (1.4); 7.7328 (1.5); 7.7201 (1.3); 7.7139 (1.2); 7.5198 (1.0); 7.4808 (1.2); 7.4771 (1.2); 7.4602 (1.7); 7.4569 (2.1); 7.4538 (1.4); 7.4369 (1.6); 7.4331 (1.6); 7.3269 (1.5); 7.3179 (1.7); 7.3154 (1.6); 7.3063 (2.8); 7.2971 (3.2); 7.2947 (3.8); 7.2856 (3.0); 7.2813 (2.5); 7.2741 (0.8); 7.2734 (0.8); 7.2709 (0.6); 7.2701 (0.7); 7.2693 (0.8); 7.2686 (0.9); 7.2677 (0.8); 7.2614 (192.2); 7.2564 (3.1); 7.2540 (1.0); 7.2523 (0.6); 7.2514 (0.5); 7.2507 (0.7); 6.9977 (1.0); 6.9267 (1.5); 6.9253 (1.7); 6.9193 (1.6); 6.9178 (1.6); 6.9055 (1.6); 6.9041 (1.7); 6.8981 (1.6); 6.8966 (1.6); 5.2688 (8.8); 5.0016 (16.0); 4.9501 (1.1); 1.6175 (0.6); 1.6032 (0.9); 1.5969 (1.1); 1.5910 (0.8); 1.5832 (2.0); 1.5769 (0.8); 1.5690 (0.9); 1.5628 (1.1); 1.5491 (0.6); 0.8042 (0.6); 0.7887 (1.7); 0.7843 (2.7); 0.7779 (2.7); 0.7681 (1.8); 0.7654 (2.1); 0.7625 (5.7); 0.7578 (4.4); 0.7515 (2.0); 0.7484 (2.6); 0.7441 (3.6); 0.7410 (1.9); 0.7383 (1.9); 0.0080 (3.2); 0.0002 (115.2); 0.0085 (3.0) I-281: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4749 (0.7); 8.4713 (0.7); 8.4629 (0.8); 8.4592 (0.8); 8.1488 (0.8); 8.1449 (0.8); 8.1290 (0.9); 8.1251 (0.9); 8.1140 (1.1); 8.1120 (0.9); 8.1099 (0.9); 8.1077 (1.2); 8.1059 (0.8); 7.8486 (0.6); 7.8424 (0.6); 7.8299 (0.7); 7.8274 (0.8); 7.8237 (0.7); 7.8211 (0.8); 7.8087 (0.7); 7.8024 (0.7); 7.4528 (0.6); 7.4509 (0.6); 7.4408 (0.6); 7.4389 (0.6); 7.4329 (0.6); 7.4312 (0.6); 7.4210 (0.6); 7.4192 (0.6); 7.2623 (10.2); 6.9518 (0.8); 6.9502 (0.9); 6.9443 (0.9); 6.9428 (0.9); 6.9306 (0.8); 6.9290 (0.8); 6.9231 (0.8); 6.9215 (0.8); 5.3004 (5.0); 5.1942 (1.6); 5.1768 (1.6); 3.7562 (16.0); 3.7496 (0.9); 1.6903 (6.7); 1.6840 (0.6); 1.6729 (6.6); 1.6666 (0.5); 1.5657 (7.6); 0.0002 (11.5) I-282: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.5791 (1.2); 8.5768 (1.3); 8.5748 (1.4); 8.5726 (1.2); 8.5669 (1.3); 8.5646 (1.4); 8.5626 (1.4); 8.5604 (1.2); 8.2347 (1.4); 8.2328 (1.7); 8.2311 (1.7); 8.2292 (1.5); 8.2231 (1.5); 8.2212 (1.8); 8.2195 (1.7); 8.2177 (1.5); 8.1307 (2.2); 8.1286 (1.7); 8.1264 (1.8); 8.1245 (2.4); 7.7718 (1.1); 7.7656 (1.1); 7.7528 (1.3); 7.7507 (1.4); 7.7466 (1.4); 7.7445 (1.4); 7.7317 (1.2); 7.7255 (1.2); 7.6501 (0.7); 7.6457 (0.7); 7.6307 (1.5); 7.6264 (1.5); 7.6115 (0.9); 7.6071 (0.9); 7.4675 (1.2); 7.4638 (1.2); 7.4469 (1.6); 7.4436 (2.0); 7.4404 (1.4); 7.4235 (1.6); 7.4198 (1.6); 7.3711 (1.7); 7.3516 (1.6); 7.3000 (1.4); 7.2911 (1.8); 7.2884 (1.5); 7.2795 (2.6); 7.2704 (1.3); 7.2678 (1.6); 7.2661 (1.2); 7.2621 (71.9); 7.2596 (3.6); 7.2571 (1.2); 7.2563 (0.9); 7.2555 (0.8); 7.2547 (0.6); 7.2539 (0.5); 7.2443 (1.0); 7.2435 (1.0); 7.2428 (1.0); 7.2293 (1.0); 7.2239 (1.0); 7.2126 (0.8); 6.9238 (1.5); 6.9223 (1.6); 6.9164 (1.6); 6.9148 (1.5); 6.9027 (1.5); 6.9012 (1.5); 6.8952 (1.5); 6.8937 (1.5); 5.3675 (9.2); 5.0180 (15.8); 1.5934 (1.6); 1.5764 (2.3); 1.5657 (0.6); 1.5593 (1.8); 1.5423 (0.6); 0.7728 (16.0); 0.7610 (1.1); 0.7557 (14.3); 0.0080 (1.2); 0.0040 (0.5); 0.0002 (46.5); 0.0049 (0.7); 0.0057 (0.6); 0.0066 (0.6); 0.0085 (1.3) I-283: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4706 (0.9); 8.4587 (0.9); 8.1471 (0.9); 8.1429 (0.8); 8.1273 (1.0); 8.1231 (1.0); 8.1100 (1.3); 8.1048 (1.3); 7.8488 (0.6); 7.8426 (0.6); 7.8300 (0.8); 7.8276 (0.8); 7.8238 (0.8); 7.8214 (0.8); 7.8089 (0.7); 7.8026 (0.7); 7.4494 (0.7); 7.4374 (0.7); 7.4296 (0.7); 7.4177 (0.6); 7.2618 (16.2); 6.9525 (1.0); 6.9512 (0.9); 6.9450 (1.0); 6.9312 (1.0); 6.9300 (0.9); 6.9238 (1.0); 5.1847 (1.2); 5.1835 (1.1); 5.1672 (1.2); 5.1660 (1.1); 4.3780 (0.6); 4.3601 (0.6); 4.3509 (0.8); 4.3330 (0.8); 4.2868 (1.2); 4.2792 (1.1); 4.2699 (1.2); 4.2636 (1.2); 4.2152 (0.8); 4.2003 (0.8); 4.1881 (0.6); 4.1732 (0.6); 3.7563 (0.8); 3.7265 (2.0); 3.7136 (0.8); 3.6741 (1.0); 3.6689 (16.0); 2.7978 (0.9); 2.7803 (0.8); 1.6741 (5.7); 1.6568 (5.6); 1.5584 (5.0); 1.1982 (1.0); 1.1800 (1.0); 1.1618 (4.2); 1.1576 (4.4); 1.1439 (4.2); 1.1398 (4.1); 0.0080 (0.7); 0.0002 (24.1); 0.0085 (0.6) I-287: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2283 (1.7); 8.2167 (1.7); 8.1304 (2.3); 8.1242 (2.3); 7.7679 (1.0); 7.7617 (1.0); 7.7469 (1.3); 7.7425 (1.3); 7.7278 (1.1); 7.7216 (1.0); 7.4623 (1.1); 7.4586 (1.0); 7.4417 (1.5); 7.4385 (2.0); 7.4352 (1.1); 7.4183 (1.4); 7.4146 (1.3); 7.3381 (1.5); 7.3302 (3.3); 7.3244 (8.6); 7.3205 (8.4); 7.3153 (2.8); 7.3105 (2.7); 7.3068 (2.0); 7.3005 (1.2); 7.2905 (1.4); 7.2815 (1.5); 7.2788 (1.4); 7.2699 (2.4); 7.2601 (25.4); 7.2493 (1.0); 6.9202 (1.6); 6.9127 (1.6); 6.8990 (1.5); 6.8916 (1.5); 5.2228 (13.8); 4.9489 (15.0); 1.5797 (1.3); 1.5630 (2.0); 1.5496 (2.6); 1.5287 (0.6); 0.7578 (10.8); 0.7407 (16.0); 0.0079 (1.1); 0.0002 (34.6); 0.0085 (1.0) I-289: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2292 (1.6); 8.2273 (1.8); 8.2257 (1.8); 8.2175 (1.7); 8.2157 (1.9); 8.1354 (2.5); 8.1293 (2.5); 7.7712 (1.1); 7.7650 (1.1); 7.7521 (1.5); 7.7502 (1.4); 7.7459 (1.4); 7.7441 (1.3); 7.7312 (1.2); 7.7250 (1.2); 7.4666 (1.2); 7.4629 (1.2); 7.4459 (1.7); 7.4427 (2.2); 7.4395 (1.2); 7.4226 (1.5); 7.4188 (1.4); 7.2918 (1.4); 7.2828 (1.7); 7.2802 (1.5); 7.2712 (2.7); 7.2612 (31.0); 7.2506 (1.2); 6.9214 (1.7); 6.9140 (1.7); 6.9004 (1.6); 6.8930 (1.6); 4.8961 (16.0); 4.2290 (1.4); 4.2127 (1.5); 4.2021 (2.2); 4.1857 (2.2); 4.1093 (2.3); 4.0894 (2.4); 4.0824 (1.5); 4.0624 (1.5); 3.8483 (0.7); 3.8346 (0.8); 3.8275 (1.6); 3.8137 (1.7); 3.8087 (2.3); 3.7917 (2.2); 3.7869 (2.1); 3.7689 (2.0); 3.7464 (1.2); 3.7286 (1.9); 3.7099 (1.6); 3.6888 (0.8); 3.5447 (2.0); 3.5307 (2.0); 3.5224 (1.7); 3.5085 (1.7); 2.6070 (0.7); 2.5904 (0.8); 2.5730 (0.6); 2.0176 (0.6); 2.0050 (0.9); 1.9965 (0.5); 1.9920 (0.6); 1.9841 (0.8); 1.9720 (0.7); 1.9653 (0.6); 1.6466 (0.5); 1.6300 (0.8); 1.6132 (1.2); 1.5958 (2.5); 1.5897 (0.6); 1.5789 (3.0); 1.5681 (0.8); 1.5617 (2.6); 1.5554 (7.5); 1.5447 (0.8); 0.7839 (15.7); 0.7668 (14.6); 0.0080 (1.3); 0.0002 (42.8); 0.0084 (1.1) I-291: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2143 (2.1); 8.2113 (1.7); 8.2083 (2.2); 8.0584 (0.8); 8.0563 (0.9); 8.0537 (1.5); 8.0517 (1.5); 8.0490 (1.0); 8.0466 (1.4); 8.0442 (1.0); 8.0415 (1.5); 8.0395 (1.5); 8.0369 (0.9); 8.0348 (0.8); 7.8689 (1.1); 7.8628 (1.1); 7.8499 (1.3); 7.8479 (1.4); 7.8438 (1.3); 7.8418 (1.3); 7.8289 (1.1); 7.8228 (1.1); 7.7804 (0.6); 7.7756 (0.6); 7.7720 (0.6); 7.7673 (0.6); 7.7619 (0.7); 7.7597 (0.9); 7.7573 (0.8); 7.7547 (1.0); 7.7513 (1.0); 7.7489 (0.8); 7.7466 (0.9); 7.7413 (0.9); 7.7365 (0.9); 7.7330 (0.9); 7.7282 (0.8); 7.6511 (0.9); 7.6489 (1.7); 7.6461 (1.5); 7.6434 (1.7); 7.6411 (1.0); 7.6305 (0.7); 7.6282 (1.2); 7.6254 (1.2); 7.6228 (1.2); 7.6204 (0.7); 7.2614 (19.9); 7.1055 (1.2); 7.0933 (1.3); 7.0917 (1.1); 7.0894 (1.0); 7.0877 (1.2); 7.0756 (1.1); 6.9937 (1.7); 6.9876 (1.6); 6.9863 (1.6); 6.9738 (1.5); 6.9725 (1.6); 6.9665 (1.5); 6.9651 (1.5); 5.2612 (1.6); 5.2529 (1.6); 5.2438 (1.6); 5.2355 (1.6); 4.4105 (0.9); 4.3925 (0.9); 4.3834 (1.3); 4.3654 (1.4); 4.3363 (2.1); 4.3326 (2.1); 4.3192 (2.5); 4.3176 (2.5); 4.2805 (1.3); 4.2664 (1.4); 4.2534 (0.9); 4.2393 (0.9); 3.8013 (1.0); 3.6555 (16.0); 3.6484 (16.0); 2.8406 (0.5); 2.8377 (0.6); 2.8339 (0.8); 2.8232 (0.8); 2.8198 (0.8); 2.8160 (0.6); 2.8076 (0.8); 2.8019 (0.6); 1.7210 (0.5); 1.7077 (6.7); 1.7056 (6.8); 1.6902 (6.6); 1.6881 (6.7); 1.5567 (2.2); 1.1889 (6.6); 1.1709 (12.8); 1.1529 (6.4); 0.0080 (0.9); 0.0002 (30.3); 0.0085 (0.8) I-293: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1700 (1.2); 8.1639 (1.2); 8.0432 (0.8); 8.0413 (0.8); 8.0386 (0.9); 8.0366 (0.8); 8.0311 (0.8); 8.0292 (0.9); 8.0265 (0.9); 8.0245 (0.8); 7.8366 (0.7); 7.8306 (0.6); 7.8172 (0.5); 7.7921 (0.6); 7.7873 (0.6); 7.7735 (0.8); 7.7715 (1.0); 7.7688 (0.8); 7.7668 (0.9); 7.7530 (0.9); 7.7483 (0.9); 7.6524 (1.0); 7.6501 (1.7); 7.6479 (1.0); 7.6318 (0.8); 7.6296 (1.3); 7.6274 (0.7); 7.2609 (15.0); 7.1421 (0.8); 7.1396 (0.8); 7.1300 (0.8); 7.1275 (0.8); 7.1236 (0.8); 7.1211 (0.8); 7.1116 (0.8); 7.1090 (0.7); 6.9806 (0.9); 6.9733 (0.9); 6.9595 (0.8); 6.9522 (0.8); 5.2507 (1.6); 5.2333 (1.7); 4.4858 (0.9); 4.4694 (2.1); 4.4542 (2.2); 4.4380 (0.9); 3.6597 (0.9); 3.6502 (16.0); 2.6794 (1.1); 2.6761 (1.1); 2.6617 (1.9); 2.6486 (1.0); 2.6451 (1.0); 1.6909 (6.3); 1.6845 (0.6); 1.6735 (6.2); 1.5482 (6.1); 0.0079 (0.7); 0.0002 (21.0); 0.0085 (0.6) I-294: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2242 (1.7); 8.2223 (1.8); 8.2206 (1.7); 8.2125 (1.8); 8.2106 (1.8); 8.2090 (1.6); 8.1457 (2.4); 8.1434 (1.9); 8.1413 (2.2); 8.1396 (2.2); 7.7787 (1.0); 7.7725 (0.9); 7.7597 (1.5); 7.7576 (1.2); 7.7535 (1.4); 7.7515 (1.1); 7.7387 (1.0); 7.7325 (0.9); 7.4797 (1.1); 7.4761 (0.9); 7.4590 (1.7); 7.4560 (1.9); 7.4526 (1.0); 7.4356 (1.3); 7.4320 (1.1); 7.3018 (1.2); 7.2927 (1.7); 7.2901 (1.2); 7.2812 (2.0); 7.2721 (1.4); 7.2695 (1.1); 7.2617 (12.4); 6.9261 (1.6); 6.9186 (1.6); 6.9050 (1.6); 6.8975 (1.5); 4.9825 (13.7); 4.8234 (16.0); 3.7849 (0.7); 2.0450 (0.6); 1.5997 (0.8); 1.5922 (0.9); 1.5865 (0.6); 1.5788 (1.6); 1.5757 (0.9); 1.5734 (0.8); 1.5647 (2.1); 1.5446 (0.5); 1.2770 (0.5); 1.2653 (1.0); 1.2594 (0.9); 0.8991 (0.5); 0.8820 (1.4); 0.8644 (0.6); 0.8112 (0.6); 0.7964 (1.8); 0.7933 (2.5); 0.7859 (1.9); 0.7760 (1.8); 0.7729 (2.1); 0.7707 (2.3); 0.7672 (1.7); 0.7643 (1.9); 0.7602 (2.3); 0.7537 (2.4); 0.7481 (2.5); 0.7467 (2.6); 0.7431 (1.9); 0.7407 (2.3); 0.7377 (1.8); 0.7351 (1.8); 0.0080 (0.7); 0.0002 (18.5) I-295: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2650 (1.6); 8.2632 (1.9); 8.2613 (1.9); 8.2596 (1.7); 8.2533 (1.7); 8.2515 (1.9); 8.2496 (1.9); 8.2480 (1.7); 8.0775 (2.4); 8.0714 (2.5); 7.7524 (1.1); 7.7462 (1.0); 7.7334 (1.3); 7.7313 (1.4); 7.7272 (1.3); 7.7252 (1.3); 7.7124 (1.2); 7.7062 (1.2); 7.4729 (1.3); 7.4692 (1.3); 7.4522 (1.8); 7.4498 (1.8); 7.4486 (2.0); 7.4463 (1.5); 7.4293 (1.7); 7.4255 (1.6); 7.3226 (1.7); 7.3135 (1.9); 7.3110 (1.8); 7.3019 (2.9); 7.2928 (1.3); 7.2903 (1.4); 7.2812 (1.2); 7.2622 (17.5); 6.8943 (1.6); 6.8929 (1.7); 6.8871 (1.7); 6.8856 (1.6); 6.8733 (1.6); 6.8718 (1.7); 6.8659 (1.6); 6.8644 (1.6); 5.3001 (1.2); 5.1370 (0.7); 5.1331 (2.4); 5.1289 (3.5); 5.1248 (2.6); 5.1210 (0.8); 5.0591 (2.6); 5.0568 (3.3); 5.0545 (3.2); 5.0522 (2.5); 5.0135 (0.6); 4.9866 (0.7); 4.9786 (16.0); 1.9126 (8.5); 1.9103 (11.5); 1.9090 (11.7); 1.9067 (9.2); 1.5007 (0.6); 1.4321 (1.6); 1.2865 (0.5); 1.2645 (2.0); 0.8987 (1.1); 0.8818 (4.2); 0.8641 (1.5); 0.0080 (0.6); 0.0002 (22.9); 0.0085 (0.6) I-296: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1542 (3.5); 8.1480 (3.5); 7.8252 (1.6); 7.8190 (1.6); 7.8063 (2.0); 7.8042 (2.1); 7.8001 (1.9); 7.7980 (1.8); 7.7853 (1.7); 7.7791 (1.6); 7.5685 (1.5); 7.5534 (1.6); 7.5475 (2.3); 7.5327 (2.3); 7.5263 (1.6); 7.5113 (1.5); 7.2607 (38.9); 6.9712 (2.3); 6.9699 (2.2); 6.9638 (2.4); 6.9500 (2.2); 6.9488 (2.2); 6.9427 (2.2); 6.8644 (1.7); 6.8583 (1.9); 6.8551 (1.8); 6.8489 (1.7); 6.8427 (1.6); 6.8365 (1.6); 6.8334 (1.6); 6.8272 (1.4); 5.3051 (1.2); 5.2877 (4.9); 5.2703 (4.9); 5.2530 (1.2); 1.6879 (16.0); 1.6705 (15.9); 1.5637 (0.7); 1.5485 (1.1); 1.5449 (1.1); 1.5347 (0.8); 1.5299 (2.7); 1.5227 (0.8); 1.5162 (0.9); 1.5121 (1.5); 1.5086 (0.9); 1.4952 (0.8); 1.4322 (3.2); 1.2643 (1.7); 1.2424 (0.7); 0.8988 (0.9); 0.8820 (3.1); 0.8643 (1.2); 0.7962 (0.7); 0.7854 (0.9); 0.7829 (1.1); 0.7775 (4.5); 0.7672 (10.6); 0.7609 (3.2); 0.7569 (3.0); 0.7527 (4.5); 0.7471 (12.0); 0.7426 (2.2); 0.7258 (0.6); 0.0079 (1.7); 0.0002 (56.6); 0.0085 (1.5) I-298: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1482 (1.2); 8.1420 (1.2); 7.8182 (0.6); 7.8120 (0.6); 7.7992 (0.7); 7.7972 (0.7); 7.7930 (0.7); 7.7910 (0.7); 7.7782 (0.6); 7.7720 (0.6); 7.5606 (0.6); 7.5455 (0.6); 7.5393 (0.9); 7.5243 (0.9); 7.5184 (0.6); 7.5033 (0.6); 7.2618 (6.6); 6.9592 (0.8); 6.9530 (0.8); 6.9518 (0.8); 6.9393 (0.8); 6.9381 (0.8); 6.9319 (0.8); 6.9306 (0.8); 6.8395 (0.6); 6.8334 (0.7); 6.8301 (0.6); 6.8240 (0.6); 6.8178 (0.6); 6.8117 (0.6); 6.8083 (0.6); 6.8023 (0.5); 5.2297 (1.6); 5.2124 (1.6); 3.7622 (16.0); 1.6362 (6.5); 1.6188 (6.5); 1.5580 (2.3); 1.5521 (0.6); 1.5444 (0.6); 1.5313 (0.9); 1.5177 (0.5); 1.5101 (0.6); 0.8194 (0.9); 0.8172 (0.9); 0.8126 (1.4); 0.8104 (1.1); 0.8066 (0.7); 0.8037 (0.6); 0.7995 (0.9); 0.7971 (1.2); 0.7748 (0.6); 0.7640 (1.6); 0.7606 (0.9); 0.7582 (0.7); 0.7557 (0.6); 0.7541 (0.6); 0.7436 (1.5); 0.7388 (0.8); 0.0002 (10.2) I-300: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1503 (1.3); 8.1441 (1.2); 7.8201 (0.7); 7.8139 (0.6); 7.8012 (0.8); 7.7991 (0.8); 7.7950 (0.8); 7.7928 (0.8); 7.7801 (0.7); 7.7739 (0.7); 7.5638 (0.6); 7.5487 (0.7); 7.5424 (0.8); 7.5274 (0.8); 7.5217 (0.7); 7.5067 (0.6); 7.2606 (22.6); 6.9649 (0.8); 6.9635 (0.9); 6.9575 (0.9); 6.9560 (0.9); 6.9438 (0.8); 6.9424 (0.8); 6.9364 (0.8); 6.9349 (0.8); 6.8695 (0.6); 6.8634 (0.7); 6.8602 (0.7); 6.8540 (0.7); 6.8478 (0.6); 6.8416 (0.6); 6.8384 (0.6); 6.8323 (0.6); 4.8869 (8.7); 3.7920 (16.0); 1.5491 (1.4); 1.5422 (11.2); 1.5297 (0.5); 0.7895 (0.8); 0.7848 (2.5); 0.7827 (2.4); 0.7804 (2.4); 0.7781 (2.7); 0.7739 (1.6); 0.7712 (2.3); 0.7674 (1.4); 0.7616 (1.5); 0.7579 (2.2); 0.7548 (0.9); 0.7525 (0.9); 0.0080 (1.0); 0.0002 (32.6); 0.0085 (0.9) I-301: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2616 (0.7); 8.2598 (0.8); 8.2581 (0.8); 8.2563 (0.7); 8.2500 (0.7); 8.2482 (0.8); 8.2465 (0.8); 8.2448 (0.7); 8.1459 (1.2); 8.1439 (0.9); 8.1418 (0.9); 8.1397 (1.2); 7.7586 (0.6); 7.7524 (0.6); 7.7397 (0.7); 7.7376 (0.7); 7.7335 (0.7); 7.7313 (0.7); 7.7186 (0.6); 7.7124 (0.6); 7.4876 (0.6); 7.4838 (0.6); 7.4669 (0.8); 7.4634 (1.0); 7.4607 (0.7); 7.4437 (0.8); 7.4400 (0.8); 7.3261 (0.6); 7.3170 (0.7); 7.3144 (0.7); 7.3054 (1.1); 7.2964 (0.5); 7.2938 (0.5); 7.2619 (18.2); 6.9265 (0.8); 6.9250 (0.8); 6.9191 (0.8); 6.9176 (0.8); 6.9054 (0.8); 6.9039 (0.8); 6.8979 (0.8); 6.8964 (0.8); 4.8090 (7.1); 3.7065 (16.0); 3.6744 (0.7); 3.6590 (1.6); 3.6444 (1.7); 3.6290 (0.7); 2.6197 (1.6); 2.6044 (2.1); 2.5899 (1.4); 1.6348 (0.6); 1.6269 (0.5); 1.6138 (1.1); 1.6006 (0.6); 1.5928 (0.6); 1.5656 (6.1); 0.8573 (0.6); 0.8465 (1.4); 0.8415 (1.6); 0.8363 (0.8); 0.8308 (0.8); 0.8251 (1.6); 0.8204 (1.3); 0.8099 (0.8); 0.6231 (0.8); 0.6124 (1.5); 0.6096 (1.2); 0.6076 (1.6); 0.5993 (1.4); 0.5946 (1.6); 0.5835 (0.6); 0.0079 (0.7); 0.0002 (28.2); 0.0085 (0.8) I-302: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.9466 (2.6); 8.2322 (3.5); 8.2260 (3.6); 8.1267 (1.2); 8.1111 (1.3); 8.1046 (2.4); 8.0891 (2.4); 8.0826 (1.3); 8.0670 (1.2); 7.9683 (1.4); 7.9620 (1.4); 7.9473 (2.1); 7.9409 (2.0); 7.9276 (1.5); 7.9213 (1.4); 7.3225 (1.3); 7.3161 (1.8); 7.3143 (1.8); 7.3078 (1.4); 7.3004 (1.3); 7.2922 (1.6); 7.2858 (1.2); 7.2615 (2.2); 7.2545 (2.2); 7.2402 (2.2); 7.2332 (2.1); 5.7565 (1.7); 4.7784 (16.0); 3.3185 (4.9); 2.6704 (0.6); 2.5241 (1.5); 2.5194 (2.3); 2.5106 (34.4); 2.5061 (75.3); 2.5015 (105.6); 2.4968 (73.4); 2.4923 (32.4); 2.4734 (0.5); 2.3286 (0.6); 1.6644 (0.6); 1.6513 (1.4); 1.6433 (1.4); 1.6384 (0.9); 1.6303 (2.8); 1.6225 (0.8); 1.6172 (1.5); 1.6093 (1.5); 1.5962 (0.8); 0.7519 (1.4); 0.7406 (3.0); 0.7352 (4.1); 0.7309 (1.9); 0.7263 (2.4); 0.7197 (3.1); 0.7140 (3.9); 0.7054 (2.0); 0.6380 (2.1); 0.6289 (4.0); 0.6240 (4.4); 0.6160 (4.0); 0.6107 (3.5); 0.5994 (1.3); 0.0080 (3.0); 0.0002 (125.7); 0.0085 (3.7) I-303: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2678 (1.2); 8.2659 (1.4); 8.2641 (1.5); 8.2623 (1.3); 8.2562 (1.3); 8.2543 (1.5); 8.2525 (1.5); 8.2508 (1.3); 8.1498 (2.0); 8.1479 (1.5); 8.1456 (1.6); 8.1436 (2.0); 7.7676 (1.0); 7.7614 (1.0); 7.7487 (1.1); 7.7465 (1.2); 7.7424 (1.1); 7.7403 (1.2); 7.7276 (1.0); 7.7214 (1.0); 7.4881 (1.0); 7.4844 (1.1); 7.4674 (1.4); 7.4639 (1.7); 7.4612 (1.2); 7.4443 (1.4); 7.4405 (1.3); 7.3282 (1.3); 7.3191 (1.4); 7.3166 (1.3); 7.3075 (2.2); 7.2984 (1.0); 7.2960 (1.1); 7.2868 (1.0); 7.2627 (60.6); 7.2068 (0.7); 7.1893 (0.7); 6.9292 (1.3); 6.9277 (1.4); 6.9218 (1.4); 6.9203 (1.3); 6.9081 (1.2); 6.9066 (1.3); 6.9006 (1.3); 6.8991 (1.3); 4.8868 (1.4); 4.8485 (5.4); 4.8261 (5.8); 4.7878 (1.5); 4.6871 (1.3); 4.6691 (2.0); 4.6511 (1.4); 4.2673 (2.0); 4.2495 (6.5); 4.2317 (6.7); 4.2138 (2.1); 4.1309 (0.5); 4.1131 (0.6); 2.0454 (2.7); 1.6557 (1.0); 1.6478 (0.9); 1.6426 (0.6); 1.6348 (1.9); 1.6269 (0.6); 1.6216 (1.0); 1.6138 (1.1); 1.6006 (0.7); 1.5819 (2.8); 1.4952 (10.8); 1.4774 (10.8); 1.3209 (7.5); 1.3031 (16.0); 1.2852 (7.5); 1.2774 (1.1); 1.2596 (2.1); 1.2417 (0.9); 0.8819 (1.1); 0.8775 (0.6); 0.8731 (0.6); 0.8663 (2.2); 0.8612 (2.6); 0.8564 (0.8); 0.8545 (0.8); 0.8522 (0.8); 0.8502 (0.9); 0.8449 (2.3); 0.8401 (2.1); 0.8335 (0.6); 0.8293 (0.7); 0.6639 (1.1); 0.6584 (1.0); 0.6563 (1.3); 0.6529 (1.9); 0.6506 (1.7); 0.6479 (1.9); 0.6455 (1.3); 0.6430 (1.4); 0.6403 (2.4); 0.6348 (1.6); 0.6276 (1.0); 0.0079 (0.8); 0.0002 (36.4); 0.0085 (1.1) III-29: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4999 (4.4); 8.4869 (4.5); 8.4140 (3.9); 8.4084 (3.9); 8.1283 (2.4); 8.1220 (2.4); 7.7759 (1.1); 7.7696 (1.1); 7.7574 (1.2); 7.7547 (1.4); 7.7511 (1.3); 7.7484 (1.3); 7.7362 (1.2); 7.7299 (1.1); 7.4249 (2.0); 7.4118 (2.2); 7.4098 (2.4); 7.3965 (2.0); 7.2617 (17.2); 7.0108 (1.7); 7.0033 (1.6); 6.9896 (1.6); 6.9821 (1.5); 5.3001 (3.8); 4.9079 (16.0); 4.3121 (2.0); 4.2943 (6.4); 4.2765 (6.5); 4.2587 (2.1); 1.3248 (7.7); 1.3070 (15.8); 1.2891 (7.6); 0.0079 (0.8); 0.0002 (24.8); 0.0085 (0.7) I-304: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2665 (1.0); 8.2648 (1.0); 8.2550 (1.0); 8.2531 (1.0); 8.1300 (1.4); 8.1238 (1.4); 7.8610 (0.7); 7.8547 (0.7); 7.8422 (0.8); 7.8397 (0.8); 7.8360 (0.8); 7.8335 (0.8); 7.8211 (0.7); 7.8148 (0.7); 7.5190 (0.7); 7.5153 (0.6); 7.4982 (1.0); 7.4948 (1.1); 7.4922 (0.8); 7.4752 (0.9); 7.4715 (0.8); 7.3654 (0.8); 7.3563 (0.9); 7.3538 (0.8); 7.3448 (1.4); 7.3356 (0.7); 7.3332 (0.6); 7.3241 (0.6); 7.2608 (17.8); 6.9702 (0.9); 6.9688 (0.9); 6.9627 (1.0); 6.9489 (0.9); 6.9475 (0.9); 6.9414 (0.9); 4.9586 (9.0); 3.8034 (16.0); 1.5463 (2.6); 0.0079 (0.8); 0.0002 (26.7); 0.0085 (0.7) I-305: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2303 (1.4); 8.2283 (1.4); 8.2263 (1.3); 8.2243 (1.5); 8.2222 (1.4); 8.1028 (1.1); 8.1007 (1.2); 8.0981 (1.3); 8.0960 (1.2); 8.0907 (1.2); 8.0885 (1.3); 8.0860 (1.3); 8.0838 (1.2); 7.8593 (0.6); 7.8578 (0.6); 7.8531 (0.6); 7.8516 (0.6); 7.8404 (0.7); 7.8385 (1.0); 7.8366 (0.8); 7.8343 (0.7); 7.8323 (1.0); 7.8305 (0.7); 7.8193 (0.6); 7.8178 (0.6); 7.8130 (0.6); 7.8116 (0.6); 7.7806 (1.1); 7.7759 (1.1); 7.7623 (1.2); 7.7599 (1.6); 7.7575 (1.2); 7.7552 (1.6); 7.7416 (1.7); 7.7368 (1.6); 7.6570 (1.6); 7.6546 (2.8); 7.6523 (1.7); 7.6363 (1.2); 7.6339 (2.0); 7.6315 (1.1); 7.2623 (9.9); 7.1243 (1.4); 7.1217 (1.4); 7.1121 (1.3); 7.1095 (1.4); 7.1060 (1.4); 7.1033 (1.3); 7.0938 (1.3); 7.0912 (1.3); 6.9890 (1.3); 6.9874 (1.4); 6.9816 (1.3); 6.9799 (1.4); 6.9679 (1.3); 6.9662 (1.3); 6.9604 (1.3); 6.9588 (1.3); 5.3000 (5.4); 4.9336 (14.4); 4.3272 (1.8); 4.3094 (5.7); 4.2916 (5.7); 4.2738 (1.8); 1.5678 (0.7); 1.4399 (0.6); 1.3359 (7.8); 1.3181 (16.0); 1.3132 (0.5); 1.3003 (7.4); 0.0002 (15.4); 0.0027 (0.6) I-306: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2724 (2.3); 8.2704 (2.3); 8.2689 (2.2); 8.2623 (2.1); 8.2607 (2.4); 8.2588 (2.4); 8.0921 (2.8); 8.0861 (2.9); 7.7904 (1.0); 7.7843 (1.0); 7.7710 (1.6); 7.7648 (1.5); 7.7507 (1.1); 7.7455 (1.1); 7.5406 (1.6); 7.5368 (1.6); 7.5197 (2.3); 7.5166 (2.8); 7.5135 (1.8); 7.4965 (2.0); 7.4928 (2.0); 7.3675 (1.9); 7.3585 (2.2); 7.3558 (2.0); 7.3468 (3.4); 7.3378 (1.6); 7.3352 (1.6); 7.3262 (1.4); 7.2606 (86.8); 7.2334 (0.8); 6.9666 (2.1); 6.9652 (2.2); 6.9591 (2.2); 6.9576 (2.2); 6.9454 (2.1); 6.9439 (2.2); 6.9379 (2.2); 6.9364 (2.1); 5.3686 (1.1); 5.3512 (4.7); 5.3337 (4.8); 5.3163 (1.2); 5.3002 (0.6); 1.7431 (16.0); 1.7356 (1.4); 1.7256 (16.0); 1.7182 (1.3); 1.4322 (1.4); 1.2628 (1.3); 0.8991 (0.6); 0.8820 (2.3); 0.8642 (0.9); 0.0080 (3.7); 0.0002 (132.9); 0.0085 (3.9); 0.0272 (1.4) I-307: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1737 (0.8); 8.1718 (0.9); 8.1702 (0.9); 8.1620 (0.8); 8.1602 (0.9); 8.1585 (0.9); 8.1363 (1.3); 8.1301 (1.3); 7.7708 (0.6); 7.7647 (0.6); 7.7517 (0.7); 7.7498 (0.8); 7.7455 (0.7); 7.7437 (0.7); 7.7307 (0.6); 7.7245 (0.6); 7.4651 (0.6); 7.4614 (0.6); 7.4445 (0.8); 7.4411 (1.2); 7.4378 (0.7); 7.4209 (0.8); 7.4172 (0.7); 7.2625 (6.2); 7.2529 (0.8); 7.2502 (0.8); 7.2413 (1.3); 7.2324 (0.6); 7.2296 (0.6); 7.2208 (0.6); 6.9129 (0.8); 6.9118 (0.8); 6.9055 (0.9); 6.8919 (0.8); 6.8906 (0.8); 6.8844 (0.8); 6.8833 (0.8); 5.2726 (1.6); 5.2552 (1.6); 3.7521 (16.0); 1.6366 (6.6); 1.6193 (6.5); 1.5856 (0.6); 1.5783 (1.6); 1.5656 (0.9); 1.5515 (0.5); 1.5442 (0.6); 0.8163 (0.6); 0.8111 (1.4); 0.8066 (0.9); 0.8052 (0.9); 0.8026 (1.0); 0.7979 (1.4); 0.7937 (1.2); 0.7887 (0.6); 0.7801 (1.3); 0.7706 (2.0); 0.7670 (0.9); 0.7631 (0.6); 0.7597 (0.6); 0.7499 (1.8); 0.7455 (0.9); 0.0002 (8.1) I-308: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2251 (1.4); 8.2235 (1.6); 8.2216 (1.6); 8.2200 (1.5); 8.2135 (1.5); 8.2119 (1.7); 8.2100 (1.7); 8.2085 (1.5); 8.1100 (2.0); 8.1039 (2.1); 7.8291 (0.7); 7.8229 (0.7); 7.8088 (1.1); 7.8030 (1.0); 7.7894 (0.8); 7.7832 (0.7); 7.5067 (1.1); 7.5030 (1.1); 7.4859 (1.6); 7.4840 (1.6); 7.4823 (1.8); 7.4805 (1.4); 7.4633 (1.5); 7.4595 (1.5); 7.3658 (1.5); 7.3566 (1.6); 7.3542 (1.6); 7.3450 (2.5); 7.3358 (1.1); 7.3335 (1.2); 7.3243 (1.0); 7.2622 (10.4); 6.9400 (1.5); 6.9387 (1.6); 6.9326 (1.6); 6.9314 (1.6); 6.9189 (1.4); 6.9175 (1.5); 6.9114 (1.5); 6.9101 (1.5); 5.2859 (0.8); 5.2685 (3.0); 5.2512 (3.0); 5.2338 (0.8); 4.2499 (1.0); 4.2447 (1.1); 4.2321 (3.3); 4.2270 (3.4); 4.2142 (3.4); 4.2092 (3.4); 4.1964 (1.1); 4.1915 (1.1); 1.6798 (12.6); 1.6624 (12.5); 1.2647 (7.8); 1.2538 (1.0); 1.2469 (16.0); 1.2291 (7.5); 0.0002 (17.0); 0.0085 (0.6) I-309: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2322 (1.0); 8.2301 (0.9); 8.2279 (1.0); 8.2262 (1.0); 8.1021 (0.7); 8.1001 (0.8); 8.0974 (0.8); 8.0953 (0.8); 8.0900 (0.8); 8.0879 (0.8); 8.0853 (0.8); 8.0832 (0.8); 7.8414 (0.7); 7.8352 (0.6); 7.7920 (0.6); 7.7873 (0.6); 7.7737 (0.7); 7.7713 (0.9); 7.7690 (0.8); 7.7666 (0.9); 7.7530 (0.9); 7.7482 (0.9); 7.6690 (1.0); 7.6666 (1.7); 7.6643 (1.0); 7.6483 (0.7); 7.6460 (1.2); 7.6436 (0.7); 7.2620 (8.8); 7.1283 (0.8); 7.1257 (0.8); 7.1161 (0.8); 7.1135 (0.8); 7.1100 (0.8); 7.1073 (0.8); 7.0978 (0.8); 7.0952 (0.7); 6.9896 (0.8); 6.9882 (0.8); 6.9822 (0.8); 6.9808 (0.8); 6.9684 (0.8); 6.9669 (0.8); 6.9610 (0.8); 6.9596 (0.8); 5.3003 (0.9); 4.9362 (8.5); 4.5272 (2.0); 4.5115 (4.2); 4.4958 (2.1); 3.6877 (16.0); 2.7228 (2.0); 2.7071 (4.0); 2.6914 (2.0); 1.5626 (4.1); 0.0002 (12.9) I-311: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1481 (3.2); 8.1462 (2.4); 8.1439 (2.5); 8.1418 (3.4); 7.8952 (1.7); 7.8889 (1.6); 7.8765 (1.9); 7.8740 (2.0); 7.8703 (1.9); 7.8677 (2.0); 7.8554 (1.8); 7.8491 (1.7); 7.6224 (1.4); 7.6075 (1.6); 7.6022 (1.8); 7.6006 (1.9); 7.5874 (1.8); 7.5858 (1.9); 7.5805 (1.6); 7.5656 (1.5); 7.2650 (1.1); 7.2607 (85.7); 7.0136 (2.1); 7.0121 (2.2); 7.0062 (2.2); 7.0047 (2.2); 6.9972 (0.6); 6.9924 (2.1); 6.9908 (2.2); 6.9849 (2.1); 6.9834 (2.1); 6.9546 (1.6); 6.9483 (1.8); 6.9454 (1.8); 6.9391 (1.7); 6.9327 (1.5); 6.9265 (1.6); 6.9235 (1.6); 6.9172 (1.4); 5.3541 (1.1); 5.3367 (4.6); 5.3192 (4.7); 5.3017 (1.2); 1.7544 (16.0); 1.7369 (16.0); 1.2645 (0.9); 0.8820 (1.8); 0.8643 (0.7); 0.0690 (1.6); 0.0080 (2.9); 0.0041 (1.0); 0.0002 (118.3); 0.0085 (3.5) I-312: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2221 (1.9); 8.2202 (1.5); 8.2181 (1.5); 8.2159 (2.0); 8.2142 (1.4); 7.8801 (1.1); 7.8740 (1.1); 7.8612 (1.3); 7.8591 (1.4); 7.8550 (1.2); 7.8529 (1.3); 7.8401 (1.2); 7.8339 (1.1); 7.6363 (1.7); 7.6165 (2.7); 7.5972 (2.2); 7.4238 (2.3); 7.4035 (1.9); 7.2623 (10.2); 6.9962 (1.4); 6.9947 (1.5); 6.9888 (1.4); 6.9873 (1.5); 6.9751 (1.3); 6.9736 (1.4); 6.9677 (1.3); 6.9662 (1.4); 6.9483 (2.1); 6.9295 (2.0); 5.3002 (3.4); 4.9423 (15.1); 4.3220 (1.9); 4.3042 (5.9); 4.2864 (6.0); 4.2686 (2.0); 2.1561 (16.0); 1.5706 (4.8); 1.5017 (0.9); 1.3332 (7.6); 1.3154 (15.7); 1.2975 (7.4); 0.0002 (14.5) I-313: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1976 (2.2); 8.1914 (2.3); 8.1202 (1.3); 8.1175 (1.4); 8.1082 (1.4); 8.1054 (1.4); 7.8461 (1.0); 7.8399 (1.0); 7.8251 (1.3); 7.8213 (1.2); 7.8190 (1.2); 7.8062 (1.1); 7.8004 (1.5); 7.7968 (1.1); 7.7812 (1.5); 7.7763 (1.4); 7.7625 (1.3); 7.7577 (1.3); 7.5901 (2.6); 7.5696 (2.2); 7.5189 (0.5); 7.2604 (97.6); 7.1596 (1.3); 7.1474 (1.3); 7.1434 (1.2); 7.1410 (1.2); 7.1313 (1.2); 7.0035 (1.5); 6.9968 (1.9); 6.9823 (1.4); 6.9750 (1.4); 5.3002 (7.3); 4.9975 (14.0); 4.6975 (3.2); 4.6837 (3.9); 4.6694 (3.3); 3.3760 (2.0); 3.3618 (3.2); 3.3480 (1.9); 2.9716 (16.0); 1.6302 (1.9); 1.2549 (1.2); 0.1456 (0.5); 0.0130 (0.6); 0.0080 (4.0); 0.0002 (149.0); 0.0085 (4.6); 0.1497 (0.6) III-30: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 13.1222 (0.9); 8.3790 (3.8); 8.3727 (3.9); 8.3280 (6.1); 8.3269 (6.0); 8.3140 (6.4); 8.3129 (6.3); 8.1177 (1.6); 8.1114 (1.5); 8.0982 (2.0); 8.0964 (2.2); 8.0920 (2.0); 8.0902 (2.0); 8.0771 (1.7); 8.0708 (1.6); 7.4236 (2.2); 7.4224 (2.3); 7.4169 (2.3); 7.4156 (2.2); 7.4024 (2.1); 7.4011 (2.2); 7.3956 (2.2); 7.3942 (2.0); 7.3187 (5.7); 7.3176 (6.4); 7.3139 (6.5); 7.3127 (6.1); 7.0230 (5.4); 7.0181 (4.9); 7.0091 (5.2); 7.0041 (5.1); 5.1986 (1.0); 5.1813 (5.3); 5.1639 (5.4); 5.1466 (1.0); 3.6216 (1.0); 3.6177 (5.5); 3.6155 (3.1); 3.6115 (3.0); 3.6093 (2.2); 3.6075 (3.9); 3.6029 (4.3); 3.6011 (12.9); 3.5989 (4.4); 3.5950 (4.1); 3.5930 (2.2); 3.5908 (2.8); 3.5867 (2.9); 3.5845 (5.9); 3.5806 (1.0); 3.3226 (15.0); 2.6705 (0.5); 2.5242 (1.6); 2.5196 (2.2); 2.5109 (27.2); 2.5063 (58.7); 2.5017 (81.7); 2.4971 (55.4); 2.4925 (23.8); 2.1831 (0.8); 1.9088 (1.1); 1.7809 (0.9); 1.7780 (1.0); 1.7762 (5.7); 1.7746 (2.4); 1.7686 (4.5); 1.7671 (3.5); 1.7643 (2.7); 1.7597 (16.0); 1.7550 (2.8); 1.7507 (4.4); 1.7447 (2.2); 1.7431 (5.5); 1.7385 (0.8); 1.5997 (13.6); 1.5823 (13.4); 1.3554 (7.7); 1.2390 (0.7); 1.2350 (0.9); 0.0080 (2.7); 0.0002 (102.8); 0.0060 (0.6); 0.0069 (0.5); 0.0085 (2.8) I-315: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1466 (2.0); 8.1404 (2.1); 7.8929 (1.1); 7.8866 (1.0); 7.8742 (1.2); 7.8717 (1.3); 7.8680 (1.2); 7.8654 (1.2); 7.8530 (1.2); 7.8468 (1.1); 7.6205 (1.0); 7.6056 (1.0); 7.6003 (1.2); 7.5988 (1.3); 7.5854 (1.3); 7.5840 (1.3); 7.5787 (1.1); 7.5638 (1.1); 7.2614 (24.6); 7.0106 (1.4); 7.0094 (1.5); 7.0032 (1.5); 7.0020 (1.4); 6.9895 (1.4); 6.9881 (1.4); 6.9820 (1.4); 6.9580 (1.1); 6.9518 (1.2); 6.9488 (1.2); 6.9425 (1.1); 6.9362 (1.0); 6.9299 (1.1); 6.9270 (1.1); 6.9207 (1.0); 4.9244 (16.0); 4.3006 (2.0); 4.2827 (6.1); 4.2649 (6.2); 4.2471 (2.0); 1.5505 (13.2); 1.3146 (7.4); 1.2967 (15.2); 1.2789 (7.3); 0.0079 (0.9); 0.0002 (33.1); 0.0085 (0.9) I-316: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2295 (1.1); 8.2282 (1.2); 8.2251 (1.3); 8.2237 (1.2); 8.2177 (1.2); 8.2163 (1.2); 8.2132 (1.2); 8.2118 (1.1); 8.1024 (1.3); 8.1005 (1.9); 8.0983 (1.5); 8.0962 (1.5); 8.0942 (2.0); 8.0922 (1.3); 7.8406 (1.2); 7.8343 (1.1); 7.8218 (1.3); 7.8193 (1.4); 7.8156 (1.2); 7.8130 (1.3); 7.8006 (1.2); 7.7943 (1.2); 7.6387 (1.1); 7.6369 (1.2); 7.6343 (1.2); 7.6325 (1.1); 7.6197 (1.2); 7.6178 (1.4); 7.6153 (1.3); 7.6134 (1.2); 7.2629 (10.1); 7.2458 (1.7); 7.2339 (1.6); 7.2268 (1.6); 7.2149 (1.5); 6.9238 (1.4); 6.9223 (1.4); 6.9163 (1.4); 6.9148 (1.4); 6.9026 (1.4); 6.9010 (1.3); 6.8951 (1.4); 6.8935 (1.3); 4.8987 (15.0); 4.2792 (1.9); 4.2613 (6.0); 4.2435 (6.0); 4.2257 (2.0); 2.1822 (13.7); 1.5768 (5.4); 1.3030 (7.6); 1.2852 (16.0); 1.2673 (7.6); 0.0701 (0.8); 0.0002 (14.9) I-317: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2587 (2.1); 8.2571 (2.4); 8.2551 (2.4); 8.2471 (2.3); 8.2455 (2.5); 8.2435 (2.5); 8.1152 (3.1); 8.1091 (3.2); 7.8398 (1.0); 7.8335 (1.0); 7.8198 (1.5); 7.8134 (1.4); 7.8001 (1.0); 7.7940 (1.0); 7.5146 (1.6); 7.5109 (1.7); 7.4938 (2.5); 7.4922 (2.3); 7.4901 (2.6); 7.4886 (2.1); 7.4713 (2.3); 7.4676 (2.3); 7.3875 (2.2); 7.3783 (2.5); 7.3759 (2.3); 7.3667 (3.7); 7.3575 (1.6); 7.3552 (1.7); 7.3459 (1.5); 7.2608 (50.0); 6.9525 (2.2); 6.9511 (2.3); 6.9453 (2.4); 6.9438 (2.3); 6.9314 (2.2); 6.9299 (2.2); 6.9240 (2.2); 6.9225 (2.2); 5.3708 (1.1); 5.3534 (4.2); 5.3359 (4.3); 5.3185 (1.2); 5.3002 (11.9); 1.7345 (16.0); 1.7170 (16.0); 1.7047 (0.9); 1.2540 (0.9); 0.0079 (2.4); 0.0002 (78.1); 0.0085 (2.2) I-318: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2287 (0.7); 8.2268 (0.9); 8.2251 (0.9); 8.2232 (0.8); 8.2171 (0.8); 8.2152 (0.9); 8.2134 (0.9); 8.2116 (0.8); 8.1362 (1.2); 8.1341 (0.9); 8.1320 (0.9); 8.1299 (1.2); 7.7748 (0.6); 7.7685 (0.6); 7.7557 (0.7); 7.7537 (0.8); 7.7495 (0.7); 7.7475 (0.8); 7.7347 (0.7); 7.7285 (0.6); 7.4615 (0.6); 7.4578 (0.7); 7.4409 (0.8); 7.4375 (1.1); 7.4344 (0.7); 7.4175 (0.8); 7.4138 (0.8); 7.2861 (0.8); 7.2772 (0.9); 7.2745 (0.8); 7.2655 (1.7); 7.2614 (27.8); 7.2568 (0.9); 7.2539 (0.8); 7.2450 (0.6); 6.9202 (0.8); 6.9188 (0.8); 6.9128 (0.8); 6.9113 (0.8); 6.8992 (0.8); 6.8976 (0.8); 6.8917 (0.8); 6.8902 (0.8); 4.9141 (8.9); 4.0314 (3.8); 4.0132 (3.9); 1.5972 (0.6); 1.5833 (1.1); 1.5685 (0.6); 1.5581 (12.9); 1.5563 (16.0); 1.5553 (15.3); 1.1408 (0.7); 0.8038 (0.8); 0.8011 (1.0); 0.7987 (2.0); 0.7949 (1.6); 0.7889 (2.0); 0.7850 (3.6); 0.7804 (2.0); 0.7694 (1.3); 0.7648 (1.7); 0.7617 (0.9); 0.7588 (1.0); 0.5559 (1.3); 0.5527 (1.6); 0.5503 (0.9); 0.5481 (0.6); 0.5409 (0.6); 0.5358 (1.5); 0.5325 (1.2); 0.5209 (0.6); 0.2972 (0.6); 0.2856 (1.7); 0.2825 (1.4); 0.2737 (1.3); 0.2705 (1.7); 0.0080 (1.4); 0.0049 (0.5); 0.0002 (46.4); 0.0085 (1.2) I-320: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2211 (2.1); 8.2112 (2.1); 8.0896 (2.6); 8.0839 (2.6); 7.7890 (0.9); 7.7835 (0.9); 7.7694 (1.5); 7.7633 (1.5); 7.7497 (1.0); 7.7436 (0.9); 7.5421 (1.2); 7.5384 (1.2); 7.5213 (1.8); 7.5183 (2.5); 7.4980 (1.5); 7.4943 (1.4); 7.3462 (1.3); 7.3373 (1.6); 7.3347 (1.5); 7.3257 (2.4); 7.3166 (1.3); 7.3142 (1.2); 7.3051 (1.0); 7.2610 (35.4); 6.9561 (1.9); 6.9487 (1.9); 6.9340 (1.8); 6.9275 (1.8); 5.2684 (1.0); 5.2510 (3.3); 5.2336 (3.4); 5.2163 (1.0); 4.2602 (2.2); 4.2423 (6.9); 4.2245 (7.1); 4.2067 (2.4); 1.6867 (13.3); 1.6693 (13.2); 1.5525 (12.1); 1.2765 (7.8); 1.2587 (16.0); 1.2409 (7.6); 0.0275 (0.5); 0.0079 (2.3); 0.0002 (51.2); 0.0085 (1.9) I-321: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2227 (1.0); 8.2213 (1.1); 8.2182 (1.2); 8.2168 (1.1); 8.2109 (1.1); 8.2094 (1.2); 8.2064 (1.2); 8.2050 (1.1); 8.1167 (1.2); 8.1147 (1.8); 8.1126 (1.4); 8.1105 (1.5); 8.1084 (1.9); 8.1064 (1.3); 7.8530 (1.1); 7.8467 (1.1); 7.8342 (1.2); 7.8317 (1.3); 7.8279 (1.2); 7.8254 (1.3); 7.8129 (1.2); 7.8067 (1.2); 7.6302 (1.0); 7.6284 (1.1); 7.6257 (1.2); 7.6239 (1.1); 7.6111 (1.1); 7.6093 (1.3); 7.6067 (1.3); 7.6048 (1.2); 7.2627 (12.1); 7.2374 (1.6); 7.2255 (1.5); 7.2184 (1.4); 7.2065 (1.4); 6.9198 (1.3); 6.9182 (1.4); 6.9123 (1.4); 6.9107 (1.4); 6.8985 (1.3); 6.8969 (1.4); 6.8910 (1.3); 6.8894 (1.3); 5.3003 (2.9); 4.8974 (14.1); 4.2761 (1.8); 4.2583 (5.8); 4.2405 (5.8); 4.2226 (1.9); 2.1766 (12.5); 1.5748 (3.0); 1.3015 (7.6); 1.2837 (16.0); 1.2658 (7.5); 0.0699 (1.0); 0.0002 (17.5); 0.0085 (0.5) I-322: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2087 (0.9); 8.2024 (1.0); 8.0596 (0.6); 8.0570 (0.6); 8.0549 (0.6); 8.0495 (0.6); 8.0475 (0.7); 8.0448 (0.7); 8.0428 (0.6); 7.8449 (0.5); 7.8428 (0.6); 7.8388 (0.6); 7.8366 (0.6); 7.8239 (0.5); 7.8177 (0.5); 7.7501 (0.6); 7.7479 (0.7); 7.7454 (0.6); 7.7432 (0.7); 7.7294 (0.7); 7.7247 (0.7); 7.6106 (1.3); 7.6084 (0.8); 7.5923 (0.6); 7.5900 (1.0); 7.2603 (30.9); 7.1124 (0.6); 7.1099 (0.6); 7.1003 (0.6); 7.0978 (0.6); 7.0941 (0.6); 7.0915 (0.6); 7.0819 (0.6); 7.0794 (0.6); 6.9961 (0.7); 6.9872 (0.7); 6.9733 (0.7); 6.9661 (0.6); 6.2991 (1.7); 6.2967 (1.8); 5.8631 (0.6); 5.8595 (1.4); 5.8569 (1.3); 5.8532 (0.6); 5.3044 (1.3); 5.2999 (2.4); 5.2870 (1.3); 4.9341 (2.8); 3.7478 (14.2); 1.7412 (4.5); 1.7237 (4.5); 1.5400 (16.0); 0.0079 (1.4); 0.0055 (0.5); 0.0002 (46.2); 0.0085 (1.3) I-323: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 8.1910 (1.1); 8.1895 (1.1); 8.1865 (1.2); 8.1851 (1.2); 8.1791 (1.2); 8.1776 (1.2); 8.1747 (1.2); 8.1732 (1.2); 8.1632 (1.8); 8.1613 (1.3); 8.1589 (1.4); 8.1569 (1.8); 7.9250 (0.8); 7.9187 (0.8); 7.9056 (1.1); 7.9037 (1.1); 7.8993 (1.0); 7.8974 (1.1); 7.8844 (1.0); 7.8778 (1.8); 7.8759 (1.2); 7.8732 (1.2); 7.8714 (1.0); 7.8586 (1.1); 7.8567 (1.3); 7.8542 (1.2); 7.8523 (1.0); 7.4040 (1.5); 7.3921 (1.5); 7.3852 (1.4); 7.3733 (1.4); 7.2611 (1.1); 7.2598 (1.2); 7.2542 (1.2); 7.2528 (1.1); 7.2399 (1.1); 7.2384 (1.2); 7.2328 (1.1); 7.2314 (1.1); 5.7570 (16.0); 4.8449 (8.5); 3.3238 (2.8); 2.5246 (0.8); 2.5200 (1.1); 2.5113 (14.5); 2.5067 (31.3); 2.5021 (43.6); 2.4975 (29.4); 2.4929 (12.6); 2.2167 (10.8); 1.9890 (0.5); 0.0080 (1.2); 0.0002 (39.2); 0.0085 (1.0) I-324: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 8.1821 (1.5); 8.1806 (1.6); 8.1776 (1.8); 8.1761 (1.7); 8.1703 (1.8); 8.1688 (1.9); 8.1639 (3.7); 8.1588 (2.1); 8.1568 (2.8); 7.9280 (1.2); 7.9217 (1.2); 7.9086 (1.5); 7.9068 (1.6); 7.9023 (1.5); 7.9005 (1.6); 7.8874 (1.3); 7.8811 (1.3); 7.8674 (1.5); 7.8656 (1.6); 7.8630 (1.8); 7.8612 (1.5); 7.8484 (1.6); 7.8466 (1.9); 7.8440 (1.8); 7.8421 (1.6); 7.3922 (2.3); 7.3804 (2.2); 7.3735 (2.2); 7.3616 (2.1); 7.2551 (1.6); 7.2538 (1.7); 7.2482 (1.8); 7.2469 (1.7); 7.2339 (1.6); 7.2325 (1.7); 7.2269 (1.7); 7.2255 (1.6); 5.7572 (4.7); 4.8287 (11.9); 4.0383 (0.8); 4.0206 (0.8); 3.3273 (0.9); 2.5418 (0.6); 2.5251 (0.8); 2.5204 (1.0); 2.5117 (15.1); 2.5071 (33.0); 2.5025 (46.2); 2.4979 (31.4); 2.4933 (13.6); 2.2127 (16.0); 1.9892 (4.0); 1.1924 (1.2); 1.1746 (2.4); 1.1569 (1.2); 0.0081 (1.0); 0.0002 (37.2); 0.0085 (1.0) I-325: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4912 (1.4); 8.4870 (1.5); 8.4792 (1.5); 8.4750 (1.5); 8.1544 (1.5); 8.1500 (1.6); 8.1346 (1.7); 8.1302 (1.7); 8.1202 (2.2); 8.1185 (1.8); 8.1162 (1.8); 8.1140 (2.3); 7.8567 (1.1); 7.8505 (1.1); 7.8380 (1.3); 7.8355 (1.4); 7.8318 (1.3); 7.8293 (1.3); 7.8168 (1.2); 7.8105 (1.2); 7.4626 (1.1); 7.4610 (1.2); 7.4506 (1.1); 7.4490 (1.2); 7.4429 (1.1); 7.4413 (1.2); 7.4308 (1.0); 7.4293 (1.1); 7.2620 (12.0); 6.9576 (1.4); 6.9563 (1.6); 6.9502 (1.5); 6.9488 (1.6); 6.9364 (1.4); 6.9350 (1.6); 6.9289 (1.4); 6.9275 (1.6); 4.8784 (16.0); 4.2818 (2.0); 4.2639 (6.2); 4.2461 (6.3); 4.2282 (2.0); 1.5618 (7.9); 1.5033 (2.5); 1.3006 (7.8); 1.2828 (16.0); 1.2649 (9.0); 0.8986 (0.9); 0.8818 (3.1); 0.8640 (1.2); 0.0002 (17.8); 0.0085 (0.6) I-328: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2210 (0.7); 8.2190 (0.8); 8.2173 (0.8); 8.2155 (0.7); 8.2093 (0.7); 8.2074 (0.8); 8.2056 (0.8); 8.2038 (0.7); 8.1357 (1.1); 8.1295 (1.1); 7.7744 (0.6); 7.7682 (0.6); 7.7554 (0.6); 7.7534 (0.7); 7.7492 (0.6); 7.7472 (0.7); 7.7343 (0.6); 7.7282 (0.6); 7.4628 (0.6); 7.4591 (0.6); 7.4422 (0.8); 7.4388 (1.1); 7.4357 (0.7); 7.4188 (0.8); 7.4151 (0.8); 7.2832 (0.7); 7.2743 (0.8); 7.2716 (0.8); 7.2624 (13.9); 7.2537 (0.6); 7.2510 (0.6); 7.2421 (0.6); 6.9192 (0.7); 6.9177 (0.8); 6.9118 (0.8); 6.9103 (0.8); 6.8981 (0.7); 6.8966 (0.8); 6.8906 (0.7); 6.8891 (0.7); 5.1308 (0.9); 5.1151 (1.3); 5.0995 (0.9); 4.8507 (9.6); 1.5937 (0.5); 1.5798 (2.3); 1.5722 (5.8); 1.5596 (0.7); 1.2653 (16.0); 1.2497 (15.9); 0.8068 (0.7); 0.8013 (1.8); 0.7971 (1.3); 0.7938 (0.9); 0.7891 (2.2); 0.7852 (2.0); 0.7829 (2.0); 0.7798 (0.8); 0.7693 (1.2); 0.7638 (1.4); 0.7614 (0.8); 0.7583 (0.9); 0.0002 (18.2) I-329: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 8.1146 (1.8); 8.1109 (2.0); 8.1032 (2.0); 8.0995 (2.0); 8.0844 (1.5); 8.0800 (1.1); 8.0781 (1.5); 7.8629 (0.7); 7.8566 (0.7); 7.8436 (0.9); 7.8417 (0.9); 7.8373 (0.8); 7.8353 (0.9); 7.8224 (0.8); 7.8160 (0.7); 7.5998 (1.0); 7.5961 (1.1); 7.5787 (2.0); 7.5750 (1.8); 7.5391 (2.5); 7.5277 (2.3); 7.5182 (1.3); 7.5068 (1.4); 7.2634 (1.0); 7.2620 (1.0); 7.2564 (1.0); 7.2552 (0.9); 7.2421 (0.9); 7.2406 (1.0); 7.2351 (0.9); 7.2337 (0.9); 5.7571 (6.0); 4.8243 (7.4); 3.5793 (16.0); 3.3237 (0.8); 2.5248 (0.6); 2.5201 (0.7); 2.5114 (8.8); 2.5068 (18.8); 2.5022 (26.1); 2.4976 (17.6); 2.4931 (7.5); 0.0079 (0.9); 0.0002 (33.1); 0.0027 (1.1); 0.0085 (0.9) I-331: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2191 (0.9); 8.2172 (1.0); 8.2074 (0.9); 8.2056 (1.0); 8.1132 (1.2); 8.1072 (1.2); 7.8114 (0.6); 7.8056 (0.6); 7.5110 (0.6); 7.5073 (0.6); 7.4901 (0.9); 7.4866 (1.0); 7.4675 (0.8); 7.4638 (0.8); 7.3660 (0.8); 7.3568 (0.9); 7.3545 (0.8); 7.3453 (1.3); 7.3360 (0.6); 7.3337 (0.6); 7.3245 (0.6); 7.2607 (13.4); 6.9399 (0.9); 6.9327 (0.9); 6.9179 (0.8); 6.9114 (0.8); 5.2861 (1.5); 5.2687 (1.5); 3.7646 (16.0); 1.6841 (6.6); 1.6667 (6.6); 1.5454 (4.0); 0.0080 (0.6); 0.0002 (19.6); 0.0085 (0.5) I-332: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1469 (0.7); 8.1449 (1.0); 8.1429 (0.8); 8.1408 (0.8); 8.1387 (1.0); 8.1368 (0.7); 7.8898 (0.6); 7.8835 (0.6); 7.8711 (0.7); 7.8685 (0.7); 7.8649 (0.7); 7.8623 (0.7); 7.8499 (0.6); 7.8436 (0.6); 7.6223 (0.5); 7.6074 (0.6); 7.6020 (0.6); 7.6005 (0.7); 7.5871 (0.7); 7.5856 (0.7); 7.5803 (0.6); 7.5654 (0.6); 7.2623 (7.6); 7.0064 (0.7); 7.0048 (0.8); 6.9989 (0.8); 6.9974 (0.7); 6.9852 (0.7); 6.9836 (0.7); 6.9777 (0.7); 6.9761 (0.7); 6.9388 (0.6); 6.9325 (0.7); 6.9294 (0.6); 6.9232 (0.6); 6.9169 (0.5); 6.9107 (0.6); 6.9076 (0.6); 6.9014 (0.5); 5.2588 (1.5); 5.2414 (1.5); 3.7799 (16.0); 1.7012 (6.4); 1.6838 (6.3); 1.5616 (3.1); 0.0002 (10.7) I-333: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1523 (3.2); 8.1460 (3.3); 7.9004 (1.7); 7.8941 (1.6); 7.8818 (1.9); 7.8792 (2.0); 7.8755 (1.8); 7.8730 (1.9); 7.8606 (1.8); 7.8543 (1.6); 7.6160 (1.5); 7.6012 (1.6); 7.5960 (1.8); 7.5943 (1.8); 7.5811 (1.9); 7.5794 (1.8); 7.5742 (1.6); 7.5594 (1.5); 7.2607 (81.4); 7.0094 (2.1); 7.0079 (2.2); 7.0020 (2.2); 7.0005 (2.2); 6.9972 (0.6); 6.9881 (2.1); 6.9866 (2.2); 6.9808 (2.1); 6.9792 (2.0); 6.9507 (1.6); 6.9444 (1.8); 6.9415 (1.8); 6.9352 (1.7); 6.9288 (1.5); 6.9225 (1.6); 6.9196 (1.6); 6.9133 (1.4); 5.3501 (1.1); 5.3326 (4.5); 5.3151 (4.7); 5.3003 (1.1); 5.2977 (1.3); 1.7528 (16.0); 1.7354 (16.0); 1.2645 (2.2); 0.8989 (1.2); 0.8820 (4.4); 0.8643 (1.7); 0.0079 (2.7); 0.0062 (0.6); 0.0053 (0.6); 0.0045 (0.8); 0.0002 (109.9); 0.0053 (1.4); 0.0061 (1.1); 0.0070 (1.0); 0.0085 (3.2); 0.0277 (0.6) I-334: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1553 (2.1); 8.1491 (2.2); 7.9075 (1.1); 7.9013 (1.0); 7.8890 (1.3); 7.8863 (1.4); 7.8827 (1.2); 7.8801 (1.3); 7.8678 (1.2); 7.8615 (1.2); 7.6221 (1.0); 7.6074 (1.1); 7.6022 (1.2); 7.6003 (1.2); 7.5874 (1.2); 7.5855 (1.2); 7.5804 (1.2); 7.5656 (1.0); 7.2606 (87.4); 7.0157 (1.5); 7.0142 (1.5); 7.0083 (1.5); 7.0068 (1.4); 6.9968 (0.6); 6.9944 (1.5); 6.9929 (1.5); 6.9871 (1.5); 6.9855 (1.4); 6.9706 (1.1); 6.9642 (1.3); 6.9614 (1.2); 6.9551 (1.2); 6.9487 (1.0); 6.9424 (1.1); 6.9395 (1.1); 6.9332 (1.0); 5.3003 (1.4); 4.9971 (16.0); 1.8570 (0.6); 1.4322 (4.0); 1.2541 (1.0); 0.0080 (3.2); 0.0002 (119.1); 0.0085 (3.5) I-335: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4874 (1.3); 8.4836 (1.4); 8.4755 (1.4); 8.4717 (1.4); 8.1464 (1.5); 8.1422 (1.6); 8.1322 (2.2); 8.1301 (1.8); 8.1262 (3.7); 8.1239 (2.6); 7.8643 (1.2); 7.8580 (1.1); 7.8455 (1.3); 7.8431 (1.4); 7.8393 (1.3); 7.8369 (1.3); 7.8243 (1.2); 7.8181 (1.2); 7.4570 (1.1); 7.4553 (1.2); 7.4450 (1.1); 7.4433 (1.2); 7.4373 (1.1); 7.4356 (1.1); 7.4252 (1.0); 7.4236 (1.0); 7.2621 (11.3); 6.9530 (1.5); 6.9516 (1.6); 6.9457 (1.5); 6.9442 (1.6); 6.9318 (1.4); 6.9304 (1.5); 6.9244 (1.5); 6.9229 (1.5); 5.3004 (2.6); 4.8774 (15.8); 4.2787 (2.0); 4.2608 (6.3); 4.2430 (6.4); 4.2252 (2.1); 1.5606 (7.6); 1.2988 (7.7); 1.2810 (16.0); 1.2631 (7.6); 0.0699 (1.0); 0.0079 (0.5); 0.0002 (17.6); 0.0085 (0.5) I-336: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.1456 (1.1); 8.1396 (1.1); 7.8928 (0.5); 7.8866 (0.5); 7.8717 (0.7); 7.8678 (0.6); 7.8530 (0.5); 7.8464 (0.5); 7.5922 (0.5); 7.5857 (0.7); 7.5712 (0.7); 7.2606 (19.1); 6.9989 (0.8); 6.9916 (0.8); 6.9778 (0.7); 6.9707 (0.7); 6.9294 (0.5); 6.9234 (0.6); 6.9203 (0.6); 6.9142 (0.5); 6.9016 (0.5); 6.8985 (0.5); 5.2298 (1.4); 5.2123 (1.4); 4.2639 (1.0); 4.2461 (3.1); 4.2283 (3.1); 4.2104 (1.0); 1.6948 (5.5); 1.6774 (5.4); 1.5440 (16.0); 1.2864 (3.3); 1.2686 (6.6); 1.2508 (3.2); 0.0078 (1.0); 0.0002 (24.9); 0.0086 (0.8) I-337: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1510 (2.2); 8.1491 (1.7); 8.1468 (1.7); 8.1447 (2.3); 7.9048 (1.2); 7.8986 (1.2); 7.8863 (1.4); 7.8836 (1.5); 7.8800 (1.3); 7.8773 (1.4); 7.8650 (1.3); 7.8587 (1.2); 7.6271 (1.1); 7.6122 (1.1); 7.6071 (1.2); 7.6053 (1.3); 7.5923 (1.3); 7.5905 (1.3); 7.5853 (1.2); 7.5705 (1.1); 7.2607 (55.0); 7.0205 (1.5); 7.0189 (1.6); 7.0131 (1.6); 7.0115 (1.6); 6.9992 (1.5); 6.9975 (1.7); 6.9918 (1.6); 6.9902 (1.5); 6.9739 (1.2); 6.9676 (1.3); 6.9647 (1.3); 6.9584 (1.2); 6.9520 (1.1); 6.9457 (1.2); 6.9428 (1.1); 6.9365 (1.0); 5.3003 (0.7); 5.0011 (16.0); 0.0080 (1.8); 0.0049 (0.5); 0.0002 (73.2); 0.0085 (2.0) I-338: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.6158 (1.1); 8.4721 (1.6); 8.4574 (3.5); 8.4426 (1.7); 8.2583 (4.6); 8.2522 (4.8); 8.1001 (2.8); 8.0982 (3.1); 8.0956 (3.4); 8.0935 (3.1); 8.0881 (3.0); 8.0861 (3.3); 8.0834 (3.4); 8.0815 (3.0); 8.0271 (2.0); 8.0209 (1.9); 8.0061 (2.9); 7.9999 (2.8); 7.9864 (2.1); 7.9802 (2.1); 7.9705 (2.3); 7.9658 (2.2); 7.9519 (2.8); 7.9498 (3.2); 7.9473 (2.8); 7.9452 (3.1); 7.9314 (3.1); 7.9267 (2.9); 7.7925 (3.6); 7.7903 (6.2); 7.7883 (3.6); 7.7719 (3.0); 7.7697 (5.0); 7.7676 (2.8); 7.3070 (3.0); 7.3010 (3.0); 7.2867 (5.7); 7.2798 (3.1); 7.2746 (3.0); 7.2721 (3.1); 7.2683 (3.0); 7.2658 (2.7); 7.2562 (2.9); 7.2537 (2.7); 6.8708 (0.9); 6.6408 (0.5); 5.2294 (1.2); 5.2126 (5.2); 5.1957 (5.3); 5.1789 (1.2); 3.8901 (1.3); 3.8748 (1.4); 3.8463 (4.4); 3.8312 (4.1); 3.8175 (4.0); 3.8030 (4.4); 3.7738 (1.4); 3.7595 (1.3); 3.6217 (1.0); 3.6178 (5.0); 3.6155 (3.2); 3.6115 (2.9); 3.6074 (4.0); 3.6011 (12.2); 3.5951 (4.2); 3.5909 (2.9); 3.5867 (3.2); 3.5846 (5.2); 3.5806 (1.0); 3.3228 (14.6); 3.2025 (1.4); 2.6752 (0.5); 2.6707 (0.7); 2.6660 (0.5); 2.5244 (1.9); 2.5197 (2.6); 2.5109 (39.2); 2.5064 (84.6); 2.5018 (116.8); 2.4973 (80.8); 2.4927 (35.9); 2.3290 (0.7); 2.1831 (1.4); 1.9950 (1.2); 1.7806 (1.0); 1.7761 (5.1); 1.7684 (4.7); 1.7642 (3.1); 1.7595 (15.0); 1.7547 (3.2); 1.7507 (4.7); 1.7430 (5.0); 1.7385 (0.9); 1.5517 (16.0); 1.5348 (15.9); 1.3555 (11.8); 1.2388 (1.2); 1.0898 (0.6); 1.0744 (0.6); 0.8540 (0.5); 0.0080 (1.0); 0.0002 (33.9); 0.0085 (1.0) I-341: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2034 (0.9); 8.2016 (0.9); 8.2000 (0.9); 8.1917 (0.9); 8.1900 (0.9); 8.1884 (0.8); 8.1337 (1.2); 8.1275 (1.3); 7.8519 (0.6); 7.8456 (0.6); 7.8331 (0.7); 7.8308 (0.8); 7.8269 (0.7); 7.8246 (0.7); 7.8120 (0.6); 7.8058 (0.6); 7.4998 (0.6); 7.4961 (0.6); 7.4791 (0.8); 7.4757 (1.1); 7.4730 (0.7); 7.4559 (0.8); 7.4522 (0.7); 7.3252 (0.7); 7.3162 (0.8); 7.3136 (0.8); 7.3046 (1.2); 7.2955 (0.6); 7.2930 (0.6); 7.2839 (0.5); 7.2629 (6.5); 6.9545 (0.9); 6.9484 (0.8); 6.9471 (0.9); 6.9346 (0.8); 6.9333 (0.8); 6.9272 (0.8); 6.9259 (0.8); 5.2762 (1.6); 5.2588 (1.6); 3.7655 (16.0); 2.0454 (1.5); 1.6983 (0.8); 1.6939 (6.6); 1.6809 (0.9); 1.6765 (6.5); 1.5801 (4.2); 1.2595 (0.9); 0.0002 (10.6) I-342: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2360 (3.1); 8.2342 (3.2); 8.2327 (2.8); 8.2243 (3.2); 8.2225 (3.1); 8.1353 (4.3); 8.1293 (4.4); 7.7673 (1.7); 7.7611 (1.6); 7.7481 (2.2); 7.7464 (2.6); 7.7421 (2.2); 7.7402 (2.4); 7.7273 (1.8); 7.7211 (1.7); 7.4566 (1.7); 7.4529 (1.8); 7.4359 (2.5); 7.4326 (3.4); 7.4297 (2.2); 7.4125 (2.2); 7.4089 (2.2); 7.2854 (2.2); 7.2763 (2.6); 7.2738 (2.6); 7.2621 (17.4); 7.2557 (1.9); 7.2532 (2.0); 7.2441 (1.6); 6.9214 (2.8); 6.9141 (2.7); 6.9003 (2.7); 6.8929 (2.5); 5.3358 (1.2); 5.3185 (4.6); 5.3011 (4.8); 5.2837 (1.4); 3.7551 (0.5); 1.8557 (0.6); 1.6786 (15.6); 1.6613 (16.0); 1.6488 (0.9); 1.6448 (0.7); 1.5896 (0.7); 1.5719 (1.5); 1.5555 (3.0); 1.5422 (1.0); 1.5382 (1.8); 1.5212 (0.8); 1.4320 (3.3); 0.7763 (1.4); 0.7649 (10.4); 0.7587 (5.7); 0.7530 (6.0); 0.7439 (10.1); 0.7212 (0.5); 0.0079 (0.7); 0.0002 (23.6); 0.0084 (0.6) I-343: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2530 (2.2); 8.2514 (2.5); 8.2494 (2.5); 8.2479 (2.2); 8.2414 (2.2); 8.2398 (2.5); 8.2378 (2.3); 8.1339 (3.5); 8.1277 (3.6); 7.8537 (1.6); 7.8474 (1.6); 7.8349 (1.8); 7.8325 (2.0); 7.8287 (1.8); 7.8262 (1.9); 7.8138 (1.6); 7.8076 (1.6); 7.4991 (1.6); 7.4954 (1.7); 7.4784 (2.3); 7.4749 (2.7); 7.4724 (1.9); 7.4554 (2.2); 7.4517 (2.1); 7.3461 (2.2); 7.3371 (2.6); 7.3345 (2.2); 7.3254 (3.7); 7.3164 (1.7); 7.3138 (1.7); 7.3047 (1.5); 7.2606 (79.4); 6.9661 (2.2); 6.9646 (2.3); 6.9587 (2.2); 6.9573 (2.1); 6.9449 (2.1); 6.9434 (2.2); 6.9375 (2.1); 6.9361 (2.0); 5.3652 (1.2); 5.3477 (4.7); 5.3429 (0.6); 5.3303 (4.8); 5.3129 (1.3); 1.7452 (16.0); 1.7359 (1.4); 1.7278 (15.9); 1.7186 (1.0); 1.4321 (1.7); 1.2643 (1.3); 0.8988 (0.7); 0.8820 (2.4); 0.8643 (0.9); 0.0080 (3.4); 0.0002 (118.0); 0.0085 (2.9) I-345: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2208 (1.1); 8.2187 (0.8); 8.2166 (0.9); 8.2146 (1.1); 8.0913 (0.7); 8.0893 (0.7); 8.0867 (0.8); 8.0846 (0.7); 8.0792 (0.7); 8.0771 (0.8); 8.0746 (0.8); 8.0725 (0.7); 7.8707 (0.6); 7.8646 (0.6); 7.8519 (0.7); 7.8496 (0.7); 7.8457 (0.7); 7.8434 (0.7); 7.8308 (0.6); 7.8246 (0.6); 7.8135 (0.6); 7.8087 (0.6); 7.7951 (0.6); 7.7928 (0.9); 7.7904 (0.7); 7.7881 (0.9); 7.7745 (0.9); 7.7698 (0.9); 7.7114 (0.9); 7.7091 (1.6); 7.7068 (1.0); 7.6908 (0.6); 7.6885 (1.0); 7.6861 (0.6); 7.2615 (14.8); 7.1572 (0.8); 7.1546 (0.8); 7.1451 (0.7); 7.1424 (0.8); 7.1389 (0.8); 7.1363 (0.7); 7.1268 (0.7); 7.1241 (0.7); 7.0140 (0.8); 7.0125 (0.8); 7.0066 (0.8); 7.0051 (0.7); 6.9928 (0.8); 6.9914 (0.7); 6.9854 (0.8); 6.9840 (0.7); 6.9540 (1.2); 6.9419 (1.3); 6.9147 (1.3); 6.9026 (1.4); 5.9312 (1.4); 5.9267 (1.3); 5.8919 (1.2); 5.8874 (1.3); 5.3003 (2.1); 4.9584 (1.0); 4.9201 (3.1); 4.8918 (3.3); 4.8534 (1.1); 3.6910 (16.0); 1.5759 (0.8); 1.3925 (5.0); 1.3749 (4.9); 0.0079 (0.6); 0.0002 (21.3); 0.0085 (0.6) I-346: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1681 (1.4); 8.1645 (1.5); 8.1564 (1.5); 8.1528 (1.5); 8.1271 (0.8); 8.1251 (1.2); 8.1229 (0.9); 8.1209 (0.9); 8.1188 (1.2); 8.1169 (0.8); 7.7841 (0.7); 7.7778 (0.7); 7.7653 (0.8); 7.7629 (0.8); 7.7590 (0.8); 7.7566 (0.8); 7.7440 (0.7); 7.7378 (0.7); 7.3500 (1.3); 7.3383 (1.3); 7.3293 (1.8); 7.3176 (1.8); 7.2638 (6.3); 7.2212 (1.3); 7.2176 (1.4); 7.2003 (1.0); 7.1968 (1.0); 6.9101 (0.8); 6.9085 (0.9); 6.9026 (0.9); 6.9010 (0.8); 6.8888 (0.8); 6.8873 (0.8); 6.8813 (0.8); 6.8798 (0.8); 5.3006 (4.8); 4.9718 (8.7); 3.7922 (16.0); 3.5623 (15.6); 1.5869 (1.3); 0.0700 (0.7); 0.0002 (9.8) I-347: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): = 8.2626 (3.0); 8.2565 (3.2); 8.1086 (1.7); 8.1068 (2.0); 8.1041 (2.1); 8.1023 (1.9); 8.0965 (1.8); 8.0947 (2.1); 8.0919 (2.1); 8.0901 (1.9); 8.0347 (1.2); 8.0285 (1.1); 8.0138 (1.8); 8.0076 (1.8); 7.9939 (1.3); 7.9873 (2.5); 7.9825 (1.4); 7.9684 (1.9); 7.9666 (2.0); 7.9638 (1.8); 7.9619 (1.8); 7.9479 (1.7); 7.9432 (1.6); 7.6534 (3.6); 7.6328 (3.2); 7.2998 (2.0); 7.2935 (2.0); 7.2864 (2.0); 7.2841 (2.0); 7.2783 (2.1); 7.2719 (3.6); 7.2680 (2.0); 7.2656 (1.8); 7.2558 (1.8); 7.2533 (1.7); 4.8589 (4.9); 4.8471 (5.0); 4.0383 (1.1); 4.0205 (1.1); 3.3261 (3.5); 2.5245 (0.5); 2.5198 (0.7); 2.5111 (14.7); 2.5065 (33.0); 2.5020 (46.5); 2.4974 (33.2); 2.4928 (15.2); 2.3020 (0.8); 2.2901 (0.8); 2.2849 (1.1); 2.2730 (1.1); 2.2678 (0.8); 2.2559 (0.8); 1.9887 (4.9); 1.9096 (2.8); 1.1925 (1.3); 1.1817 (0.8); 1.1747 (2.8); 1.1699 (1.2); 1.1569 (1.3); 1.0879 (9.2); 1.0698 (16.0); 1.0521 (9.7); 1.0387 (0.7); 0.0080 (0.8); 0.0002 (30.2); 0.0085 (1.0) I-348: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1493 (2.0); 8.1431 (2.2); 7.8196 (1.1); 7.8133 (1.0); 7.8006 (1.2); 7.7985 (1.3); 7.7944 (1.3); 7.7923 (1.3); 7.7795 (1.1); 7.7734 (1.1); 7.5626 (1.0); 7.5475 (1.0); 7.5411 (1.4); 7.5261 (1.4); 7.5205 (1.2); 7.5054 (1.1); 7.2624 (13.7); 6.9649 (1.4); 6.9635 (1.5); 6.9575 (1.4); 6.9561 (1.4); 6.9438 (1.4); 6.9424 (1.4); 6.9363 (1.4); 6.9349 (1.4); 6.8676 (1.1); 6.8615 (1.2); 6.8583 (1.2); 6.8521 (1.2); 6.8459 (1.0); 6.8397 (1.1); 6.8365 (1.1); 6.8304 (1.0); 4.8688 (15.9); 4.2810 (1.9); 4.2632 (6.1); 4.2454 (6.2); 4.2276 (2.0); 2.0454 (2.4); 1.5660 (5.0); 1.5552 (0.7); 1.5490 (1.9); 1.5410 (0.6); 1.5346 (0.8); 1.5283 (1.0); 1.5145 (0.6); 1.3092 (7.7); 1.2914 (16.0); 1.2774 (1.2); 1.2736 (7.8); 1.2646 (0.9); 1.2596 (1.9); 1.2418 (0.7); 0.8818 (1.5); 0.8641 (0.6); 0.8025 (1.5); 0.7967 (3.2); 0.7923 (2.5); 0.7896 (1.8); 0.7864 (1.8); 0.7827 (3.9); 0.7783 (5.0); 0.7727 (1.6); 0.7625 (2.1); 0.7589 (1.7); 0.7565 (2.6); 0.7542 (1.6); 0.7511 (1.7); 0.0080 (0.5); 0.0002 (19.2); 0.0085 (0.6) I-349: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2007 (2.5); 8.1946 (2.5); 8.0339 (1.6); 8.0312 (1.7); 8.0236 (1.6); 8.0218 (1.6); 8.0190 (1.6); 7.8576 (1.2); 7.8515 (1.2); 7.8385 (1.5); 7.8366 (1.5); 7.8324 (1.5); 7.8305 (1.4); 7.8176 (1.2); 7.8114 (1.2); 7.7503 (1.1); 7.7456 (1.1); 7.7296 (1.8); 7.7273 (1.4); 7.7250 (1.6); 7.7113 (1.7); 7.7066 (1.6); 7.6429 (3.4); 7.6223 (2.2); 7.3781 (0.6); 7.2603 (40.2); 7.0867 (1.5); 7.0842 (1.6); 7.0746 (1.6); 7.0720 (1.6); 7.0685 (1.6); 7.0659 (1.4); 7.0564 (1.5); 7.0537 (1.4); 6.9901 (1.8); 6.9830 (1.8); 6.9690 (1.7); 6.9619 (1.7); 4.9008 (4.6); 4.8878 (4.6); 4.2952 (1.2); 4.2929 (1.2); 4.2775 (3.8); 4.2751 (3.7); 4.2596 (4.0); 4.2575 (3.7); 4.2418 (1.4); 2.3924 (0.8); 2.3792 (0.9); 2.3752 (1.1); 2.3623 (1.1); 2.3581 (0.9); 2.3451 (0.8); 1.5440 (15.5); 1.3043 (7.9); 1.2865 (16.0); 1.2687 (9.4); 1.1545 (11.0); 1.1465 (11.2); 1.1375 (11.3); 1.1293 (10.7); 0.8989 (1.5); 0.8820 (4.8); 0.8643 (1.9); 0.0080 (1.6); 0.0002 (57.2); 0.0084 (1.8) I-350: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 12.6373 (2.1); 8.5246 (2.4); 8.5055 (2.4); 8.4816 (2.5); 8.4627 (2.5); 8.2625 (5.5); 8.2594 (4.4); 8.2566 (5.6); 8.0989 (2.0); 8.0969 (2.1); 8.0943 (2.5); 8.0922 (2.2); 8.0868 (2.3); 8.0846 (3.1); 8.0819 (4.0); 8.0800 (3.4); 8.0768 (2.2); 8.0713 (2.1); 8.0693 (2.4); 8.0667 (2.4); 8.0646 (2.1); 8.0343 (1.6); 8.0314 (1.7); 8.0281 (1.6); 8.0252 (1.6); 8.0128 (2.8); 8.0101 (2.7); 8.0067 (2.8); 7.9935 (1.9); 7.9906 (3.5); 7.9859 (2.6); 7.9720 (2.2); 7.9699 (2.2); 7.9673 (2.0); 7.9653 (2.1); 7.9554 (1.7); 7.9513 (3.2); 7.9467 (2.2); 7.9371 (1.8); 7.9347 (2.4); 7.9324 (1.8); 7.9300 (2.2); 7.9164 (2.5); 7.9117 (2.3); 7.8528 (2.7); 7.8505 (4.5); 7.8482 (2.6); 7.8322 (1.9); 7.8299 (3.0); 7.8275 (1.6); 7.7205 (2.4); 7.7183 (4.1); 7.7162 (2.3); 7.6999 (2.2); 7.6977 (3.6); 7.6954 (1.9); 7.3064 (3.6); 7.2996 (3.6); 7.2852 (3.7); 7.2804 (4.6); 7.2782 (5.9); 7.2761 (4.1); 7.2733 (2.5); 7.2686 (2.2); 7.2661 (2.5); 7.2621 (3.4); 7.2576 (2.4); 7.2549 (2.0); 7.2501 (2.3); 7.2475 (2.4); 7.2455 (2.3); 7.2428 (2.0); 6.8711 (1.1); 6.6408 (0.7); 5.1941 (1.3); 5.1777 (5.4); 5.1609 (5.4); 5.1439 (1.3); 4.3196 (2.0); 4.3120 (2.1); 4.3011 (3.0); 4.2936 (3.2); 4.2825 (2.1); 4.2751 (2.1); 3.6217 (0.9); 3.6177 (4.8); 3.6155 (2.8); 3.6115 (2.7); 3.6093 (2.1); 3.6075 (3.6); 3.6012 (11.5); 3.5990 (4.1); 3.5950 (3.7); 3.5930 (2.0); 3.5909 (2.5); 3.5867 (2.8); 3.5846 (5.1); 3.5807 (0.9); 3.3223 (35.7); 3.2025 (1.8); 2.6753 (0.7); 2.6706 (1.0); 2.6660 (0.7); 2.5244 (2.8); 2.5197 (3.8); 2.5110 (57.0); 2.5065 (124.1); 2.5019 (172.6); 2.4973 (117.1); 2.4927 (51.0); 2.3336 (0.8); 2.3289 (1.0); 2.3243 (0.7); 2.1834 (1.7); 1.9950 (1.5); 1.7808 (0.8); 1.7761 (5.1); 1.7685 (4.2); 1.7642 (2.4); 1.7595 (14.5); 1.7548 (2.7); 1.7506 (4.0); 1.7429 (4.8); 1.7385 (0.8); 1.5354 (11.8); 1.5309 (11.8); 1.5186 (12.1); 1.5140 (11.4); 1.3555 (15.5); 1.3159 (15.8); 1.3142 (14.9); 1.2977 (16.0); 1.2961 (14.8); 1.2354 (1.0); 1.1822 (0.5); 1.0898 (0.8); 1.0744 (0.7); 0.0080 (1.6); 0.0002 (60.9); 0.0085 (1.6) I-351: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 8.2782 (2.2); 8.2720 (2.3); 8.0650 (1.0); 8.0587 (1.0); 8.0452 (1.4); 8.0439 (1.4); 8.0390 (1.3); 8.0377 (1.4); 8.0242 (1.1); 8.0179 (1.0); 7.8481 (2.0); 7.8285 (3.0); 7.8089 (2.4); 7.4664 (2.6); 7.4475 (1.7); 7.4461 (2.4); 7.3159 (1.4); 7.3148 (1.4); 7.3091 (1.5); 7.2948 (1.4); 7.2934 (1.4); 7.2878 (1.4); 7.2866 (1.3); 7.1358 (2.5); 7.1170 (2.4); 5.7570 (0.8); 4.9308 (11.6); 3.3250 (8.4); 2.5247 (0.9); 2.5201 (1.2); 2.5114 (16.6); 2.5068 (35.7); 2.5022 (49.4); 2.4976 (33.5); 2.4930 (14.4); 2.0742 (16.0); 0.0079 (1.2); 0.0002 (45.9); 0.0085 (1.2) I-352: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2130 (1.9); 8.2110 (1.5); 8.2090 (1.5); 8.2069 (2.0); 8.2049 (1.4); 7.8733 (1.1); 7.8671 (1.1); 7.8543 (1.3); 7.8522 (1.4); 7.8481 (1.3); 7.8461 (1.3); 7.8332 (1.2); 7.8271 (1.2); 7.6321 (1.7); 7.6123 (2.7); 7.5930 (2.2); 7.4267 (2.3); 7.4064 (1.9); 7.2620 (11.4); 6.9950 (1.4); 6.9936 (1.4); 6.9877 (1.4); 6.9862 (1.4); 6.9739 (1.4); 6.9724 (1.4); 6.9665 (1.4); 6.9650 (1.4); 6.9427 (2.1); 6.9239 (2.0); 4.9408 (15.1); 4.3199 (1.9); 4.3021 (6.1); 4.2843 (6.2); 4.2665 (2.0); 2.1460 (16.0); 1.5686 (2.8); 1.3320 (7.8); 1.3142 (16.0); 1.2964 (7.5); 0.0002 (15.8) I-353: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2646 (1.0); 8.2546 (1.0); 7.9858 (1.3); 7.9795 (1.4); 7.6068 (0.7); 7.6006 (0.6); 7.5857 (0.8); 7.5816 (0.8); 7.5796 (0.8); 7.5667 (0.7); 7.5605 (0.7); 7.4886 (0.7); 7.4848 (0.7); 7.4680 (0.9); 7.4649 (1.2); 7.4615 (0.8); 7.4446 (0.8); 7.4409 (0.8); 7.3189 (0.9); 7.3100 (1.1); 7.3073 (1.0); 7.2984 (1.5); 7.2893 (1.0); 7.2868 (0.8); 7.2778 (0.8); 7.2686 (0.6); 7.2604 (62.6); 6.8563 (1.0); 6.8490 (1.0); 6.8352 (0.9); 6.8278 (0.9); 4.9349 (2.7); 3.7686 (16.0); 1.8496 (3.5); 1.8471 (4.5); 1.7495 (6.0); 1.5659 (4.9); 1.5074 (5.0); 1.5038 (5.0); 0.0079 (2.9); 0.0002 (93.2); 0.0085 (2.9); 0.0109 (0.7); 0.0125 (0.5) I-354: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2658 (1.5); 8.2640 (1.6); 8.2542 (1.6); 8.2523 (1.6); 8.0904 (1.9); 8.0845 (1.9); 7.7956 (0.7); 7.7891 (0.7); 7.7748 (1.1); 7.7687 (1.1); 7.7556 (0.7); 7.7493 (0.7); 7.5431 (1.1); 7.5394 (1.1); 7.5224 (1.6); 7.5190 (2.2); 7.5161 (1.2); 7.4991 (1.4); 7.4954 (1.3); 7.3675 (1.3); 7.3586 (1.5); 7.3559 (1.4); 7.3469 (2.3); 7.3379 (1.1); 7.3353 (1.1); 7.3263 (1.0); 7.2605 (67.3); 6.9630 (1.5); 6.9615 (1.5); 6.9555 (1.5); 6.9417 (1.4); 6.9342 (1.4); 4.9243 (16.0); 4.2988 (2.0); 4.2810 (6.0); 4.2631 (6.1); 4.2453 (2.0); 1.5411 (13.4); 1.3094 (7.6); 1.2916 (15.8); 1.2738 (7.5); 0.0080 (3.1); 0.0002 (102.5); 0.0085 (2.9) I-355: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.2516 (1.1); 8.2417 (1.0); 8.0988 (1.5); 8.0926 (1.4); 7.7774 (0.6); 7.7712 (0.6); 7.7584 (0.8); 7.7564 (0.8); 7.7522 (0.8); 7.7502 (0.8); 7.7374 (0.7); 7.7312 (0.6); 7.4869 (0.7); 7.4832 (0.6); 7.4662 (0.9); 7.4630 (1.2); 7.4602 (0.7); 7.4430 (0.8); 7.4393 (0.8); 7.3295 (0.8); 7.3204 (0.9); 7.3180 (0.9); 7.3089 (1.4); 7.2998 (0.7); 7.2973 (0.7); 7.2882 (0.6); 7.2613 (11.6); 6.9501 (1.0); 6.9428 (1.0); 6.9289 (1.0); 6.9216 (0.9); 4.9317 (4.5); 4.9257 (4.4); 3.8007 (0.6); 3.7906 (16.0); 2.4352 (0.6); 2.4255 (1.0); 2.4058 (1.1); 2.3960 (0.5); 2.3763 (0.6); 2.0450 (0.6); 1.8715 (0.7); 1.8517 (0.7); 1.8406 (0.5); 1.7604 (0.5); 1.7477 (0.5); 1.5543 (10.0); 0.0079 (0.5); 0.0002 (15.0) I-356: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4355 (0.7); 8.4317 (0.7); 8.4235 (0.7); 8.4198 (0.7); 8.1339 (1.2); 8.1320 (0.9); 8.1278 (1.3); 8.1087 (0.8); 8.1044 (0.8); 8.0888 (0.8); 8.0845 (0.8); 7.7803 (0.6); 7.7741 (0.6); 7.7612 (0.7); 7.7593 (0.7); 7.7551 (0.7); 7.7530 (0.7); 7.7402 (0.6); 7.7340 (0.6); 7.3786 (0.6); 7.3769 (0.6); 7.3666 (0.6); 7.3649 (0.6); 7.3588 (0.6); 7.3573 (0.6); 7.3469 (0.5); 7.3452 (0.5); 7.2621 (10.9); 6.9101 (0.7); 6.9086 (0.8); 6.9026 (0.8); 6.9012 (0.8); 6.8890 (0.7); 6.8875 (0.8); 6.8815 (0.8); 6.8801 (0.7); 5.3004 (1.6); 4.8233 (7.8); 4.4655 (2.0); 4.4495 (4.1); 4.4334 (2.0); 3.7264 (0.5); 3.6965 (16.0); 3.6925 (1.3); 2.6877 (1.9); 2.6716 (3.9); 2.6556 (1.8); 1.5768 (0.6); 1.5632 (2.6); 1.5555 (0.5); 1.5426 (0.6); 0.8176 (1.0); 0.8118 (1.2); 0.8091 (0.9); 0.8053 (1.5); 0.8004 (0.9); 0.7986 (1.2); 0.7918 (1.1); 0.7890 (1.2); 0.7852 (0.9); 0.7823 (1.2); 0.7778 (0.8); 0.7685 (1.2); 0.7621 (1.3); 0.7597 (0.8); 0.7564 (0.9); 0.0002 (14.1) I-357: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2203 (1.3); 8.2183 (1.0); 8.2162 (1.1); 8.2141 (1.3); 7.8746 (0.7); 7.8684 (0.7); 7.8557 (0.8); 7.8535 (0.9); 7.8495 (0.8); 7.8473 (0.9); 7.8346 (0.7); 7.8284 (0.7); 7.6669 (1.0); 7.6471 (1.8); 7.6277 (1.4); 7.4795 (1.5); 7.4593 (1.2); 7.2624 (9.5); 7.0066 (0.9); 7.0051 (1.0); 6.9992 (1.0); 6.9978 (0.9); 6.9855 (0.9); 6.9840 (1.0); 6.9767 (2.3); 6.9582 (1.3); 4.9426 (7.4); 4.1817 (3.4); 4.1683 (3.4); 3.7927 (16.0); 2.1655 (10.1); 1.6102 (0.5); 0.0002 (13.8) I-359: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1482 (2.1); 8.1463 (1.6); 8.1440 (1.7); 8.1419 (2.3); 8.1329 (1.3); 8.1309 (1.5); 8.1283 (1.5); 8.1263 (1.4); 8.1208 (1.4); 8.1189 (1.5); 8.1162 (1.5); 8.1142 (1.4); 7.9567 (1.2); 7.9505 (1.1); 7.9382 (1.3); 7.9355 (1.4); 7.9319 (1.3); 7.9293 (1.3); 7.9170 (1.3); 7.9108 (1.2); 7.8395 (1.2); 7.8347 (1.3); 7.8207 (1.5); 7.8190 (1.7); 7.8160 (1.5); 7.8143 (1.7); 7.8003 (1.7); 7.7956 (1.6); 7.6423 (1.6); 7.6401 (3.0); 7.6379 (1.8); 7.6219 (1.4); 7.6197 (2.5); 7.6174 (1.4); 7.2616 (27.6); 7.2450 (1.6); 7.2425 (1.6); 7.2329 (1.6); 7.2304 (1.5); 7.2264 (1.5); 7.2238 (1.5); 7.2143 (1.5); 7.2118 (1.4); 7.0427 (1.5); 7.0413 (1.6); 7.0354 (1.5); 7.0341 (1.5); 7.0215 (1.4); 7.0201 (1.5); 7.0142 (1.5); 7.0128 (1.5); 5.3005 (5.6); 5.0446 (15.8); 4.3296 (2.1); 4.3117 (6.4); 4.2939 (6.4); 4.2761 (2.1); 1.5553 (12.3); 1.3330 (7.8); 1.3152 (16.0); 1.2974 (7.6); 0.0080 (1.0); 0.0002 (39.5); 0.0085 (1.2) I-360: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2065 (1.3); 8.2045 (1.9); 8.2024 (1.5); 8.2004 (1.5); 8.1983 (2.0); 8.1963 (1.4); 8.0707 (1.2); 8.0686 (1.4); 8.0660 (1.5); 8.0639 (1.4); 8.0586 (1.4); 8.0565 (1.4); 8.0539 (1.5); 8.0518 (1.4); 7.8636 (1.2); 7.8574 (1.2); 7.8447 (1.3); 7.8425 (1.4); 7.8385 (1.3); 7.8363 (1.4); 7.8236 (1.3); 7.8174 (1.2); 7.7683 (1.1); 7.7636 (1.1); 7.7500 (1.3); 7.7477 (1.8); 7.7453 (1.3); 7.7429 (1.7); 7.7293 (1.8); 7.7246 (1.8); 7.6628 (1.7); 7.6604 (3.1); 7.6580 (2.0); 7.6421 (1.2); 7.6398 (2.0); 7.6373 (1.2); 7.2612 (21.7); 7.1197 (1.5); 7.1170 (1.5); 7.1076 (1.5); 7.1049 (1.5); 7.1014 (1.5); 7.0987 (1.4); 7.0893 (1.5); 7.0865 (1.4); 6.9997 (1.4); 6.9981 (1.6); 6.9923 (1.5); 6.9907 (1.5); 6.9785 (1.4); 6.9770 (1.4); 6.9711 (1.4); 6.9696 (1.4); 5.3002 (2.0); 5.0034 (16.0); 4.8356 (9.5); 4.8294 (9.7); 2.4949 (2.7); 2.4887 (6.0); 2.4825 (2.8); 1.5520 (10.2); 0.0079 (0.8); 0.0002 (31.0); 0.0085 (0.9) I-361: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.4355 (0.7); 8.4315 (0.7); 8.4233 (0.7); 8.4195 (0.7); 8.1314 (1.1); 8.1295 (0.9); 8.1273 (0.9); 8.1253 (1.2); 8.1076 (0.8); 8.1033 (0.8); 8.0878 (0.8); 8.0835 (0.8); 7.7798 (0.5); 7.7736 (0.5); 7.7607 (0.7); 7.7587 (0.7); 7.7545 (0.7); 7.7526 (0.6); 7.7397 (0.6); 7.7335 (0.6); 7.3777 (0.6); 7.3761 (0.6); 7.3657 (0.6); 7.3641 (0.5); 7.3580 (0.5); 7.3460 (0.5); 7.2617 (14.8); 6.9103 (0.7); 6.9089 (0.8); 6.9029 (0.8); 6.9015 (0.7); 6.8892 (0.7); 6.8878 (0.7); 6.8818 (0.7); 6.8803 (0.7); 5.3004 (0.6); 4.8256 (7.0); 4.3723 (0.7); 4.3547 (0.7); 4.3452 (1.2); 4.3277 (1.3); 4.2768 (1.3); 4.2620 (1.3); 4.2497 (0.8); 4.2349 (0.7); 3.7746 (0.6); 3.7264 (1.1); 3.6867 (16.0); 3.6833 (1.3); 2.8173 (0.5); 2.8144 (0.7); 2.7996 (0.7); 1.5765 (0.5); 1.5631 (1.0); 1.5565 (4.6); 1.5550 (4.2); 1.5498 (0.6); 1.5423 (0.6); 1.1981 (0.7); 1.1919 (6.4); 1.1800 (0.8); 1.1740 (6.3); 0.8217 (1.0); 0.8162 (1.1); 0.8122 (0.8); 0.8091 (1.6); 0.8045 (0.9); 0.8028 (1.1); 0.7958 (1.2); 0.7901 (1.1); 0.7871 (0.8); 0.7830 (1.1); 0.7786 (0.8); 0.7694 (1.2); 0.7628 (1.2); 0.7571 (0.9); 0.0080 (0.5); 0.0002 (20.6); 0.0085 (0.6) I-362: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1109 (0.5); 7.2632 (5.4); 4.9297 (3.6); 4.3575 (0.9); 4.3457 (0.9); 4.3339 (0.9); 3.6240 (1.0); 3.6121 (0.9); 3.6004 (1.0); 3.4902 (16.0); 3.3684 (8.5); 0.0002 (8.2) I-365: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2533 (0.7); 8.2514 (0.8); 8.2496 (0.9); 8.2478 (0.8); 8.2417 (0.8); 8.2398 (0.9); 8.2380 (0.8); 8.2362 (0.8); 8.0995 (1.1); 8.0974 (0.9); 8.0952 (0.9); 8.0932 (1.2); 7.7786 (0.6); 7.7723 (0.5); 7.7598 (0.6); 7.7575 (0.7); 7.7536 (0.6); 7.7513 (0.7); 7.7387 (0.6); 7.7325 (0.6); 7.4901 (0.6); 7.4864 (0.6); 7.4695 (0.8); 7.4659 (1.0); 7.4632 (0.7); 7.4462 (0.8); 7.4425 (0.8); 7.3311 (0.8); 7.3220 (0.9); 7.3195 (0.8); 7.3105 (1.4); 7.3014 (0.6); 7.2988 (0.6); 7.2899 (0.6); 7.2625 (9.1); 6.9522 (0.8); 6.9507 (0.8); 6.9447 (0.8); 6.9432 (0.8); 6.9311 (0.7); 6.9296 (0.8); 6.9236 (0.8); 6.9221 (0.7); 4.9590 (0.5); 4.9188 (3.8); 4.9082 (3.7); 4.8681 (0.5); 4.4838 (1.9); 4.4678 (4.1); 4.4518 (2.0); 3.6936 (16.0); 2.6981 (1.9); 2.6821 (3.9); 2.6662 (1.8); 2.4163 (0.8); 2.3966 (0.9); 2.1719 (0.7); 1.8647 (0.5); 1.8450 (0.6); 1.5652 (3.4); 0.0002 (13.7) I-366: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2458 (0.7); 8.2439 (0.8); 8.2422 (0.8); 8.2403 (0.7); 8.2341 (0.7); 8.2323 (0.8); 8.2305 (0.8); 8.2287 (0.7); 8.1291 (1.1); 8.1229 (1.1); 7.7709 (0.5); 7.7647 (0.5); 7.7519 (0.6); 7.7499 (0.7); 7.7457 (0.6); 7.7436 (0.6); 7.7308 (0.6); 7.7246 (0.6); 7.4551 (0.6); 7.4513 (0.6); 7.4345 (0.8); 7.4310 (1.0); 7.4281 (0.6); 7.4112 (0.7); 7.4074 (0.7); 7.2954 (0.7); 7.2864 (0.8); 7.2838 (0.7); 7.2748 (1.3); 7.2658 (0.7); 7.2617 (11.7); 7.2542 (0.6); 6.9227 (0.7); 6.9213 (0.7); 6.9153 (0.7); 6.9138 (0.7); 6.9016 (0.7); 6.9002 (0.7); 6.8941 (0.7); 6.8927 (0.7); 5.0555 (8.9); 2.0432 (14.6); 1.9634 (16.0); 1.5841 (1.1); 1.5763 (0.5); 1.5692 (0.7); 1.5641 (0.8); 0.8029 (0.7); 0.7978 (1.8); 0.7942 (1.4); 0.7895 (2.0); 0.7852 (2.7); 0.7798 (1.6); 0.7698 (1.1); 0.7655 (1.6); 0.7596 (0.8); 0.0002 (17.2); 0.0085 (0.6) I-367: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.2286 (1.1); 8.2170 (1.1); 8.0756 (1.5); 8.0695 (1.5); 7.7522 (0.6); 7.7460 (0.6); 7.7316 (0.9); 7.7265 (0.8); 7.7121 (0.7); 7.7059 (0.6); 7.4714 (0.7); 7.4677 (0.7); 7.4506 (1.0); 7.4477 (1.2); 7.4276 (0.8); 7.4240 (0.8); 7.3058 (0.8); 7.2966 (1.0); 7.2942 (0.9); 7.2851 (1.4); 7.2760 (0.8); 7.2735 (0.8); 7.2627 (6.2); 6.8870 (1.1); 6.8798 (1.0); 6.8659 (1.0); 6.8586 (1.0); 5.1269 (1.4); 5.1228 (2.0); 5.1188 (1.4); 5.0640 (1.9); 5.0617 (1.7); 4.9433 (9.4); 3.8062 (0.5); 3.8003 (0.6); 3.7907 (16.0); 3.7855 (1.1); 1.9273 (7.2); 1.5743 (2.9); 0.0002 (7.9) I-368: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2391 (1.3); 8.2372 (1.5); 8.2355 (1.6); 8.2336 (1.4); 8.2275 (1.4); 8.2256 (1.6); 8.2238 (1.6); 8.2220 (1.4); 8.0989 (2.0); 8.0970 (1.6); 8.0948 (1.6); 8.0927 (2.1); 7.7416 (1.0); 7.7354 (1.0); 7.7227 (1.2); 7.7205 (1.3); 7.7165 (1.2); 7.7143 (1.3); 7.7016 (1.1); 7.6954 (1.1); 7.4736 (1.1); 7.4698 (1.2); 7.4529 (1.4); 7.4494 (1.9); 7.4465 (1.3); 7.4296 (1.4); 7.4259 (1.4); 7.3087 (1.4); 7.2997 (1.5); 7.2971 (1.5); 7.2881 (2.5); 7.2790 (1.1); 7.2764 (1.2); 7.2674 (1.1); 7.2623 (13.4); 6.9384 (1.4); 6.9369 (1.5); 6.9309 (1.4); 6.9294 (1.5); 6.9173 (1.3); 6.9158 (1.4); 6.9098 (1.4); 6.9083 (1.4); 6.3811 (1.8); 6.3522 (2.2); 6.3369 (2.7); 6.3080 (2.5); 6.0266 (2.6); 6.0221 (2.8); 5.9824 (2.1); 5.9779 (2.0); 5.3175 (2.5); 5.3130 (2.3); 5.2886 (2.2); 5.2841 (2.4); 4.9688 (15.7); 4.9370 (0.6); 4.3004 (1.9); 4.2826 (6.0); 4.2648 (6.1); 4.2470 (2.0); 2.0452 (1.6); 1.5684 (4.2); 1.3144 (7.7); 1.3037 (0.5); 1.2966 (16.0); 1.2858 (0.9); 1.2788 (7.7); 1.2679 (0.8); 1.2595 (1.3); 0.8818 (1.2); 0.0002 (18.9); 0.0085 (0.5) I-369: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1533 (1.2); 8.1513 (0.9); 8.1492 (1.0); 8.1471 (1.3); 7.8993 (0.7); 7.8930 (0.6); 7.8807 (0.8); 7.8781 (0.8); 7.8744 (0.8); 7.8719 (0.8); 7.8595 (0.7); 7.8532 (0.7); 7.6172 (0.6); 7.6023 (0.6); 7.5972 (0.7); 7.5955 (0.8); 7.5823 (0.7); 7.5806 (0.8); 7.5754 (0.7); 7.5605 (0.6); 7.2618 (10.8); 7.0080 (0.8); 7.0065 (0.9); 7.0005 (0.9); 6.9990 (0.9); 6.9868 (0.8); 6.9853 (0.9); 6.9793 (0.9); 6.9778 (0.8); 6.9576 (0.6); 6.9513 (0.7); 6.9484 (0.7); 6.9421 (0.7); 6.9357 (0.6); 6.9295 (0.7); 6.9265 (0.7); 6.9202 (0.6); 4.9429 (8.6); 3.8076 (16.0); 1.5541 (5.8); 0.0002 (14.0) I-370: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2046 (1.0); 8.2026 (0.7); 8.2005 (0.8); 8.1985 (1.0); 8.0773 (0.6); 8.0752 (0.7); 8.0726 (0.7); 8.0705 (0.7); 8.0651 (0.7); 8.0631 (0.7); 8.0604 (0.7); 8.0583 (0.6); 7.8632 (0.6); 7.8570 (0.5); 7.8443 (0.6); 7.8421 (0.7); 7.8382 (0.6); 7.8359 (0.6); 7.8232 (0.6); 7.8170 (0.6); 7.7771 (0.6); 7.7723 (0.6); 7.7586 (0.6); 7.7564 (0.8); 7.7539 (0.6); 7.7517 (0.8); 7.7380 (0.8); 7.7332 (0.8); 7.6284 (0.8); 7.6261 (1.4); 7.6238 (0.8); 7.6078 (0.6); 7.6055 (1.1); 7.6031 (0.6); 7.2609 (16.3); 7.1258 (0.7); 7.1233 (0.7); 7.1137 (0.7); 7.1111 (0.7); 7.1075 (0.7); 7.1049 (0.6); 7.0953 (0.7); 7.0927 (0.6); 6.9994 (0.7); 6.9978 (0.7); 6.9920 (0.7); 6.9905 (0.7); 6.9783 (0.6); 6.9767 (0.7); 6.9709 (0.7); 6.9694 (0.6); 6.3498 (0.7); 6.3476 (2.0); 6.3452 (1.9); 6.3430 (0.7); 5.8973 (0.6); 5.8936 (1.5); 5.8911 (1.5); 5.8874 (0.6); 5.0017 (6.9); 4.9708 (2.2); 4.9683 (3.0); 4.9650 (2.1); 3.7700 (16.0); 1.5471 (1.4); 0.0080 (0.7); 0.0002 (25.6); 0.0085 (0.7) I-371: .sup.1H-NMR(400.0 MHz, CDCl3): = 8.1603 (1.2); 8.1569 (1.3); 8.1486 (1.3); 8.1452 (1.3); 8.1362 (1.5); 8.1302 (1.5); 7.7898 (0.7); 7.7835 (0.7); 7.7706 (0.8); 7.7687 (0.9); 7.7645 (0.8); 7.7626 (0.8); 7.7496 (0.7); 7.7434 (0.7); 7.3400 (1.0); 7.3283 (1.0); 7.3193 (1.4); 7.3076 (1.3); 7.2629 (6.8); 7.2092 (1.5); 7.2059 (1.5); 7.1885 (1.1); 7.1851 (1.0); 6.9009 (1.0); 6.8937 (1.0); 6.8797 (1.0); 6.8725 (0.9); 5.3003 (3.5); 4.9497 (9.7); 4.2780 (1.3); 4.2601 (3.8); 4.2423 (3.9); 4.2245 (1.3); 3.5596 (16.0); 1.5808 (1.1); 1.2953 (4.5); 1.2775 (8.9); 1.2596 (4.5); 0.0002 (9.5) I-372: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.0832 (1.2); 8.0815 (1.9); 8.0794 (1.5); 8.0774 (1.6); 8.0753 (2.0); 8.0734 (1.4); 7.9998 (1.2); 7.9977 (1.3); 7.9951 (1.4); 7.9929 (1.4); 7.9877 (1.3); 7.9855 (1.4); 7.9829 (1.4); 7.9808 (1.3); 7.7158 (1.2); 7.7096 (1.1); 7.6957 (2.3); 7.6907 (2.2); 7.6887 (1.5); 7.6774 (1.6); 7.6752 (2.7); 7.6728 (1.5); 7.6700 (2.4); 7.6568 (2.0); 7.6520 (1.8); 7.5981 (1.7); 7.5957 (3.0); 7.5933 (1.9); 7.5774 (1.2); 7.5751 (1.9); 7.5726 (1.1); 7.2616 (16.9); 7.0109 (1.6); 7.0081 (1.6); 6.9988 (1.4); 6.9960 (1.6); 6.9928 (1.6); 6.9900 (1.4); 6.9806 (1.4); 6.9778 (1.4); 6.9512 (1.4); 6.9496 (1.5); 6.9438 (1.4); 6.9422 (1.5); 6.9302 (1.3); 6.9286 (1.4); 6.9228 (1.4); 6.9212 (1.4); 4.9628 (14.5); 4.3181 (1.9); 4.3002 (6.0); 4.2824 (6.0); 4.2646 (1.9); 4.1701 (0.6); 4.1670 (1.4); 3.2355 (0.6); 3.2149 (1.0); 3.2133 (1.0); 3.1905 (0.6); 2.4972 (1.2); 2.4917 (0.9); 2.4728 (1.5); 2.4669 (1.5); 2.4504 (0.8); 2.4488 (0.9); 2.4445 (1.0); 2.4421 (1.0); 2.4198 (0.5); 2.1074 (0.6); 2.1051 (0.6); 2.0992 (0.7); 2.0948 (0.8); 2.0924 (0.9); 2.0899 (0.9); 2.0867 (1.2); 2.0815 (0.8); 2.0782 (1.0); 2.0725 (1.0); 2.0652 (1.4); 2.0609 (0.8); 2.0589 (0.8); 2.0524 (0.5); 2.0450 (0.6); 1.8942 (0.6); 1.8753 (0.8); 1.8691 (1.0); 1.8596 (0.7); 1.8570 (0.8); 1.8495 (1.6); 1.8439 (1.1); 1.8367 (1.1); 1.8346 (1.1); 1.8316 (1.0); 1.8260 (1.1); 1.8140 (0.7); 1.8119 (0.7); 1.8076 (0.7); 1.3364 (7.7); 1.3186 (16.0); 1.3008 (7.5); 0.0079 (0.8); 0.0002 (24.1); 0.0085 (0.6) I-373: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2290 (1.7); 8.2270 (1.5); 8.2247 (1.8); 8.1559 (1.2); 8.1539 (1.3); 8.1512 (1.4); 8.1491 (1.3); 8.1437 (1.3); 8.1417 (1.4); 8.1390 (1.4); 8.1369 (1.3); 7.8533 (0.7); 7.8470 (0.7); 7.8338 (1.0); 7.8276 (1.0); 7.8133 (0.7); 7.8072 (0.7); 7.7800 (1.1); 7.7752 (1.1); 7.7615 (1.4); 7.7593 (1.6); 7.7568 (1.4); 7.7546 (1.5); 7.7409 (1.6); 7.7361 (1.5); 7.6036 (1.6); 7.6012 (2.8); 7.5990 (1.6); 7.5829 (1.3); 7.5806 (2.2); 7.5783 (1.2); 7.2605 (49.6); 7.1478 (1.4); 7.1453 (1.4); 7.1356 (1.4); 7.1331 (1.4); 7.1294 (1.4); 7.1268 (1.3); 7.1172 (1.4); 7.1146 (1.3); 6.9982 (1.4); 6.9967 (1.7); 6.9908 (1.4); 6.9893 (1.4); 6.9770 (1.3); 6.9755 (1.4); 6.9696 (1.3); 6.9681 (1.3); 5.0196 (16.0); 2.0471 (1.0); 1.4671 (0.7); 1.4322 (0.6); 1.2598 (0.7); 0.0080 (2.1); 0.0056 (0.6); 0.0002 (72.6); 0.0051 (0.7); 0.0085 (2.0) I-374: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2415 (0.7); 8.2398 (0.8); 8.2379 (0.8); 8.2362 (0.7); 8.2299 (0.8); 8.2281 (0.8); 8.2263 (0.8); 8.2246 (0.7); 8.1209 (1.0); 8.1188 (0.8); 8.1166 (0.9); 8.1147 (1.1); 7.8536 (0.6); 7.8473 (0.5); 7.8348 (0.6); 7.8324 (0.7); 7.8286 (0.6); 7.8261 (0.6); 7.8137 (0.6); 7.8074 (0.6); 7.4995 (0.6); 7.4958 (0.6); 7.4788 (0.8); 7.4753 (0.9); 7.4728 (0.6); 7.4558 (0.7); 7.4520 (0.7); 7.3517 (0.7); 7.3427 (0.8); 7.3401 (0.7); 7.3311 (1.2); 7.3220 (0.6); 7.3194 (0.6); 7.3104 (0.5); 7.2633 (18.6); 6.9662 (0.7); 6.9648 (0.7); 6.9589 (0.8); 6.9573 (0.7); 6.9451 (0.7); 6.9436 (0.7); 6.9376 (0.7); 6.9361 (0.7); 5.4494 (1.6); 5.4321 (1.6); 2.0416 (14.2); 1.9316 (16.0); 1.7781 (5.5); 1.7607 (5.4); 1.5652 (7.9); 0.8819 (0.8); 0.0080 (0.9); 0.0002 (28.3); 0.0085 (0.8) I-375: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1760 (1.1); 8.1741 (1.3); 8.1724 (1.3); 8.1643 (1.2); 8.1625 (1.3); 8.1607 (1.3); 8.1343 (1.7); 8.1281 (1.8); 7.7699 (0.9); 7.7637 (0.8); 7.7507 (1.0); 7.7488 (1.1); 7.7446 (1.0); 7.7427 (1.0); 7.7297 (0.9); 7.7236 (0.9); 7.4599 (0.9); 7.4562 (0.9); 7.4394 (1.1); 7.4360 (1.7); 7.4326 (1.0); 7.4158 (1.1); 7.4121 (1.0); 7.2607 (34.7); 7.2502 (1.3); 7.2474 (1.1); 7.2385 (1.9); 7.2296 (0.9); 7.2269 (0.9); 7.2180 (0.8); 6.9105 (1.2); 6.9044 (1.2); 6.8908 (1.1); 6.8894 (1.1); 6.8833 (1.1); 5.2739 (0.6); 5.2565 (2.4); 5.2392 (2.4); 5.2220 (0.7); 4.2354 (1.4); 4.2176 (4.6); 4.1998 (4.8); 4.1820 (1.6); 1.6328 (9.2); 1.6154 (9.2); 1.5858 (0.8); 1.5781 (0.8); 1.5650 (1.3); 1.5569 (0.6); 1.5469 (16.0); 1.5306 (0.5); 1.2671 (5.9); 1.2494 (11.9); 1.2316 (5.6); 0.8397 (0.6); 0.8263 (1.8); 0.8218 (2.0); 0.8137 (2.6); 0.8088 (2.2); 0.8004 (1.2); 0.7822 (0.6); 0.7774 (1.4); 0.7690 (1.9); 0.7648 (1.2); 0.7565 (1.5); 0.7487 (1.7); 0.7433 (1.3); 0.7366 (0.5); 0.7306 (0.6); 0.0080 (1.3); 0.0002 (50.0); 0.0085 (1.6) I-376: .sup.1H-NMR(400.6 MHz, d.sub.6-DMSO): = 8.2560 (2.2); 8.2498 (2.3); 8.0476 (1.0); 8.0414 (1.0); 8.0278 (1.4); 8.0266 (1.4); 8.0216 (1.4); 8.0204 (1.4); 8.0069 (1.1); 8.0006 (1.0); 7.8419 (2.0); 7.8223 (3.1); 7.8027 (2.4); 7.4654 (2.6); 7.4451 (2.4); 7.3110 (1.4); 7.3099 (1.4); 7.3042 (1.5); 7.2899 (1.4); 7.2886 (1.4); 7.2829 (1.4); 7.2818 (1.3); 7.1270 (2.5); 7.1082 (2.4); 5.7572 (1.4); 4.9196 (11.1); 3.3259 (1.7); 2.5204 (0.7); 2.5117 (11.2); 2.5071 (24.1); 2.5025 (33.4); 2.4979 (22.7); 2.4934 (9.9); 2.0651 (16.0); 0.0080 (0.8); 0.0002 (28.8); 0.0085 (0.8) I-377: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2379 (1.0); 8.2358 (0.9); 8.2336 (1.1); 8.2318 (1.0); 8.1164 (0.7); 8.1144 (0.8); 8.1118 (0.9); 8.1097 (0.8); 8.1043 (0.8); 8.1022 (0.9); 8.0996 (0.9); 8.0975 (0.8); 7.8394 (0.7); 7.8331 (0.7); 7.8165 (0.7); 7.8119 (0.9); 7.7981 (0.7); 7.7958 (1.0); 7.7935 (0.8); 7.7910 (1.0); 7.7775 (1.1); 7.7728 (1.0); 7.7178 (1.0); 7.7154 (1.9); 7.7130 (1.1); 7.6971 (0.7); 7.6947 (1.2); 7.6923 (0.7); 7.2617 (15.4); 7.1555 (0.8); 7.1529 (0.9); 7.1434 (0.8); 7.1407 (0.9); 7.1373 (0.9); 7.1346 (0.8); 7.1251 (0.8); 7.1224 (0.8); 7.0020 (0.9); 7.0005 (0.9); 6.9945 (0.9); 6.9931 (0.9); 6.9807 (0.8); 6.9793 (0.9); 6.9733 (0.9); 6.9718 (0.9); 4.9338 (7.5); 4.1817 (3.4); 4.1680 (3.4); 3.7876 (16.0); 1.5618 (9.1); 0.0080 (0.6); 0.0002 (21.7); 0.0085 (0.6) I-380: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2492 (1.4); 8.2474 (1.7); 8.2457 (1.6); 8.2439 (1.4); 8.2376 (1.5); 8.2357 (1.7); 8.2340 (1.6); 8.1298 (2.3); 8.1237 (2.3); 7.7706 (1.0); 7.7644 (1.0); 7.7516 (1.3); 7.7496 (1.3); 7.7454 (1.3); 7.7435 (1.2); 7.7306 (1.1); 7.7244 (1.0); 7.4547 (1.1); 7.4510 (1.0); 7.4340 (1.6); 7.4307 (1.9); 7.4277 (1.2); 7.4108 (1.4); 7.4071 (1.3); 7.2969 (1.3); 7.2878 (1.5); 7.2853 (1.4); 7.2763 (2.3); 7.2671 (1.6); 7.2621 (19.2); 7.2556 (1.0); 6.9239 (1.5); 6.9227 (1.4); 6.9166 (1.5); 6.9028 (1.4); 6.9014 (1.4); 6.8954 (1.4); 5.0361 (16.0); 2.5554 (1.2); 2.5372 (3.1); 2.5204 (1.6); 2.5130 (1.3); 2.4940 (2.8); 2.4750 (1.4); 2.0451 (2.0); 1.8188 (1.2); 1.8054 (1.5); 1.7995 (4.5); 1.7910 (3.0); 1.7885 (3.1); 1.7798 (3.9); 1.7731 (1.4); 1.7599 (1.1); 1.6054 (0.7); 1.5996 (0.9); 1.5923 (0.6); 1.5857 (1.9); 1.5778 (0.7); 1.5709 (1.1); 1.5654 (1.8); 1.5514 (0.7); 1.2772 (0.8); 1.2595 (1.6); 1.2416 (0.6); 0.8819 (1.2); 0.8069 (1.6); 0.8018 (3.6); 0.7980 (2.7); 0.7922 (3.8); 0.7883 (6.3); 0.7836 (3.4); 0.7726 (2.2); 0.7681 (3.1); 0.7622 (1.6); 0.0079 (1.0); 0.0002 (27.5); 0.0085 (0.7) I-382: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2268 (1.0); 8.2152 (1.0); 8.1337 (1.4); 8.1276 (1.3); 7.7740 (0.6); 7.7679 (0.6); 7.7548 (0.8); 7.7485 (0.8); 7.7340 (0.6); 7.7278 (0.6); 7.4641 (0.6); 7.4604 (0.6); 7.4434 (0.9); 7.4401 (1.2); 7.4370 (0.7); 7.4201 (0.8); 7.4164 (0.7); 7.2892 (0.8); 7.2803 (0.9); 7.2777 (0.8); 7.2687 (1.4); 7.2615 (13.9); 7.2481 (0.6); 6.9208 (0.9); 6.9134 (0.9); 6.8997 (0.9); 6.8923 (0.9); 4.8907 (8.0); 4.3897 (0.8); 4.3722 (0.8); 4.3626 (1.3); 4.3451 (1.4); 4.2919 (1.4); 4.2771 (1.4); 4.2648 (0.8); 4.2500 (0.8); 3.7857 (0.6); 3.7134 (0.9); 3.6829 (16.0); 2.8432 (0.5); 2.8256 (0.8); 2.8105 (0.8); 1.5868 (0.6); 1.5711 (1.4); 1.5643 (0.9); 1.5576 (0.9); 1.1871 (6.8); 1.1761 (0.7); 1.1692 (6.6); 0.7811 (7.6); 0.7677 (2.4); 0.7623 (2.0); 0.7601 (2.3); 0.0080 (0.6); 0.0002 (19.6); 0.0085 (0.6) I-383: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2260 (1.0); 8.2243 (1.0); 8.2225 (0.9); 8.2143 (1.0); 8.2126 (1.0); 8.1374 (1.3); 8.1313 (1.3); 7.7758 (0.6); 7.7696 (0.6); 7.7568 (0.7); 7.7548 (0.8); 7.7506 (0.7); 7.7487 (0.8); 7.7358 (0.6); 7.7296 (0.6); 7.4663 (0.6); 7.4626 (0.6); 7.4457 (0.8); 7.4423 (1.2); 7.4392 (0.7); 7.4223 (0.8); 7.4186 (0.8); 7.2893 (0.8); 7.2803 (0.8); 7.2777 (0.8); 7.2687 (1.4); 7.2615 (12.6); 7.2481 (0.6); 6.9191 (0.9); 6.9116 (0.9); 6.8979 (0.9); 6.8906 (0.8); 4.8878 (8.6); 4.4797 (2.1); 4.4637 (4.4); 4.4476 (2.2); 3.6919 (16.0); 2.6983 (2.1); 2.6823 (4.3); 2.6663 (2.0); 1.5889 (0.6); 1.5863 (0.6); 1.5707 (1.2); 1.5522 (0.6); 0.7803 (7.4); 0.7724 (1.1); 0.7672 (2.2); 0.7649 (1.9); 0.7617 (1.8); 0.7592 (2.4); 0.7542 (0.9); 0.0002 (18.0); 0.0085 (0.5) I-384: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2542 (1.3); 8.2523 (1.5); 8.2505 (1.6); 8.2487 (1.5); 8.2426 (1.4); 8.2407 (1.6); 8.2389 (1.6); 8.2371 (1.5); 8.0978 (2.0); 8.0916 (2.2); 7.7783 (1.0); 7.7721 (1.0); 7.7595 (1.2); 7.7572 (1.3); 7.7533 (1.2); 7.7510 (1.2); 7.7384 (1.1); 7.7322 (1.0); 7.4861 (1.1); 7.4824 (1.2); 7.4654 (1.5); 7.4619 (1.8); 7.4592 (1.3); 7.4423 (1.4); 7.4385 (1.4); 7.3282 (1.5); 7.3192 (1.6); 7.3166 (1.5); 7.3076 (2.5); 7.2986 (1.2); 7.2959 (1.2); 7.2870 (1.1); 7.2626 (16.3); 6.9510 (1.4); 6.9495 (1.5); 6.9435 (1.5); 6.9420 (1.5); 6.9299 (1.4); 6.9284 (1.4); 6.9224 (1.4); 6.9209 (1.4); 4.9687 (0.6); 4.9572 (1.0); 4.9371 (0.6); 4.9173 (6.8); 4.9048 (6.7); 4.8649 (1.0); 4.2786 (1.8); 4.2607 (5.6); 4.2429 (5.8); 4.2251 (1.9); 4.1308 (1.1); 4.1130 (1.1); 2.4536 (0.7); 2.4339 (0.8); 2.4242 (1.5); 2.4046 (1.7); 2.3948 (0.8); 2.3752 (0.8); 2.0453 (5.3); 1.9064 (0.6); 1.8953 (1.0); 1.8756 (1.0); 1.8645 (0.7); 1.7601 (0.7); 1.7475 (0.6); 1.7407 (0.5); 1.7304 (0.6); 1.5698 (12.8); 1.3003 (7.7); 1.2968 (1.3); 1.2857 (1.3); 1.2825 (16.0); 1.2774 (2.3); 1.2646 (8.5); 1.2595 (3.8); 1.2416 (1.5); 0.8988 (0.6); 0.8819 (2.2); 0.8642 (0.8); 0.0080 (0.5); 0.0002 (20.6); 0.0085 (0.7) I-385: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.2728 (1.4); 8.2710 (1.7); 8.2691 (1.7); 8.2674 (1.6); 8.2611 (1.6); 8.2593 (1.8); 8.2575 (1.7); 8.2557 (1.6); 8.1024 (2.3); 8.0962 (2.4); 7.7431 (1.1); 7.7369 (1.1); 7.7243 (1.3); 7.7221 (1.4); 7.7181 (1.3); 7.7159 (1.3); 7.7032 (1.2); 7.6970 (1.2); 7.4782 (1.2); 7.4745 (1.2); 7.4576 (1.7); 7.4540 (2.0); 7.4513 (1.4); 7.4343 (1.6); 7.4306 (1.5); 7.3275 (1.6); 7.3184 (1.8); 7.3158 (1.6); 7.3068 (2.7); 7.2977 (1.2); 7.2951 (1.3); 7.2861 (1.1); 7.2613 (34.4); 6.9459 (1.5); 6.9444 (1.6); 6.9386 (1.6); 6.9371 (1.5); 6.9248 (1.4); 6.9233 (1.6); 6.9175 (1.5); 6.9160 (1.4); 6.3717 (2.0); 6.3429 (2.4); 6.3275 (2.8); 6.2987 (2.6); 5.9815 (2.7); 5.9772 (2.8); 5.9373 (2.3); 5.9330 (2.2); 5.3237 (2.7); 5.3194 (2.4); 5.3003 (1.2); 5.2948 (2.3); 5.2905 (2.5); 5.0367 (16.0); 5.0039 (0.6); 1.2646 (0.9); 0.8989 (0.5); 0.8819 (2.0); 0.8642 (0.7); 0.0080 (1.2); 0.0002 (44.0); 0.0085 (1.2) I-387: .sup.1H-NMR(400.6 MHz, CDCl3): = 8.1734 (1.2); 8.1714 (1.8); 8.1693 (1.4); 8.1673 (1.5); 8.1652 (1.9); 8.1633 (1.3); 8.0549 (1.2); 8.0528 (1.2); 8.0501 (1.4); 8.0480 (1.2); 8.0427 (1.2); 8.0406 (1.3); 8.0380 (1.3); 8.0359 (1.2); 7.8172 (1.1); 7.8110 (1.1); 7.7982 (1.2); 7.7961 (1.3); 7.7920 (1.2); 7.7899 (1.3); 7.7771 (1.1); 7.7709 (1.1); 7.7426 (1.1); 7.7378 (1.0); 7.7242 (1.2); 7.7219 (1.6); 7.7195 (1.2); 7.7172 (1.6); 7.7036 (1.6); 7.6988 (1.6); 7.6311 (1.6); 7.6287 (2.8); 7.6263 (1.7); 7.6105 (1.2); 7.6081 (1.9); 7.6057 (1.1); 7.2617 (11.2); 7.0805 (1.3); 7.0779 (1.3); 7.0684 (1.3); 7.0657 (1.4); 7.0622 (1.4); 7.0596 (1.2); 7.0501 (1.3); 7.0474 (1.2); 6.9883 (1.3); 6.9868 (1.4); 6.9810 (1.4); 6.9794 (1.3); 6.9673 (1.3); 6.9657 (1.3); 6.9599 (1.3); 6.9583 (1.3); 5.2996 (0.8); 4.9608 (0.7); 4.9211 (6.7); 4.9126 (6.6); 4.8729 (0.7); 4.3055 (1.8); 4.2876 (5.7); 4.2698 (5.8); 4.2520 (1.9); 2.3625 (0.7); 2.3428 (0.8); 2.3331 (1.5); 2.3134 (1.6); 2.3037 (0.8); 2.2840 (0.8); 1.8820 (0.6); 1.8710 (1.0); 1.8512 (1.0); 1.8402 (0.7); 1.7024 (0.6); 1.6896 (0.6); 1.6726 (0.5); 1.6708 (0.5); 1.3253 (7.7); 1.3075 (16.0); 1.2896 (7.4); 0.0002 (16.3) I-390: 1H-NMR(400.6 MHz, d6-DMSO): = 8.6148 (3.0); 8.6079 (3.0); 8.2670 (1.7); 8.2629 (3.1); 8.2591 (1.6); 8.2158 (1.2); 8.2128 (1.6); 8.2041 (1.2); 8.2017 (1.6); 7.9529 (0.9); 7.9494 (1.0); 7.9321 (1.1); 7.9281 (1.6); 7.9242 (1.0); 7.9069 (1.0); 7.9034 (1.0); 7.7567 (1.0); 7.7524 (1.1); 7.7499 (1.1); 7.7455 (1.0); 7.7331 (1.0); 7.7287 (1.1); 7.7263 (1.0); 7.7219 (0.9); 7.5501 (1.1); 7.5408 (1.2); 7.5386 (1.2); 7.5292 (1.8); 7.5200 (0.9); 7.5178 (1.0); 7.5085 (0.8); 6.4211 (1.3); 6.3924 (1.6); 6.3772 (1.7); 6.3483 (1.6); 5.9091 (1.6); 5.9037 (1.7); 5.8651 (1.4); 5.8596 (1.4); 5.3176 (1.7); 5.3123 (1.4); 5.2888 (1.4); 5.2834 (1.6); 5.1128 (0.6); 5.0956 (2.4); 5.0782 (2.4); 5.0609 (0.5); 3.3253 (16.0); 2.5414 (0.9); 2.5244 (1.5); 2.5198 (1.9); 2.5110 (16.7); 2.5065 (35.6); 2.5020 (49.2); 2.4974 (34.7); 2.4929 (15.7); 1.5939 (7.0); 1.5765 (7.0); 0.0080 (0.9); 0.0002 (26.9); 0.0084 (0.8) I-393: 1H-NMR(400.6 MHz, CDCl3): = 8.4405 (1.5); 8.4336 (1.6); 8.2773 (1.7); 8.2285 (0.8); 8.2266 (1.0); 8.2249 (1.1); 8.2231 (1.0); 8.2169 (0.9); 8.2150 (1.1); 8.2133 (1.1); 8.2115 (1.0); 7.4905 (0.7); 7.4868 (0.7); 7.4698 (1.0); 7.4664 (1.2); 7.4634 (0.9); 7.4465 (0.9); 7.4428 (0.9); 7.3791 (0.7); 7.3748 (0.8); 7.3723 (0.8); 7.3679 (0.8); 7.3570 (0.8); 7.3527 (0.9); 7.3501 (0.9); 7.3458 (0.8); 7.3146 (0.9); 7.3056 (1.1); 7.3030 (1.0); 7.2940 (1.6); 7.2850 (0.8); 7.2824 (0.8); 7.2734 (0.7); 7.2609 (32.7); 6.4130 (1.1); 6.3842 (1.3); 6.3689 (1.6); 6.3400 (1.5); 6.0425 (1.6); 6.0381 (1.7); 5.9983 (1.3); 5.9939 (1.3); 5.3497 (1.6); 5.3453 (1.5); 5.3208 (1.4); 5.3164 (1.5); 4.9894 (8.7); 3.8110 (16.0); 3.8033 (0.8); 1.5566 (12.7); 0.0079 (1.5); 0.0054 (0.6); 0.0002 (46.1); 0.0085 (1.7) I-394: 1H-NMR(400.6 MHz, CDCl3): = 8.4469 (3.3); 8.4400 (3.4); 8.2891 (1.8); 8.2854 (3.3); 8.2817 (1.8); 8.2441 (1.4); 8.2424 (1.6); 8.2406 (1.6); 8.2389 (1.4); 8.2325 (1.5); 8.2307 (1.7); 8.2290 (1.7); 8.2272 (1.4); 7.5013 (1.1); 7.4977 (1.1); 7.4807 (1.5); 7.4772 (1.9); 7.4744 (1.3); 7.4574 (1.4); 7.4537 (1.4); 7.4032 (1.2); 7.3988 (1.3); 7.3963 (1.3); 7.3919 (1.2); 7.3810 (1.2); 7.3766 (1.3); 7.3742 (1.2); 7.3697 (1.1); 7.3330 (1.4); 7.3239 (1.6); 7.3213 (1.4); 7.3123 (2.4); 7.3033 (1.2); 7.3007 (1.2); 7.2917 (1.0); 7.2624 (12.6); 4.9593 (1.1); 4.9194 (7.0); 4.9066 (6.9); 4.8667 (1.1); 4.2802 (1.8); 4.2624 (5.9); 4.2446 (6.0); 4.2267 (2.0); 2.4857 (0.7); 2.4661 (0.9); 2.4564 (1.6); 2.4368 (1.7); 2.4271 (0.9); 2.4075 (0.9); 1.9022 (0.7); 1.8911 (1.0); 1.8823 (0.5); 1.8801 (0.5); 1.8714 (1.1); 1.8602 (0.8); 1.7763 (0.8); 1.7635 (0.7); 1.7567 (0.6); 1.7443 (0.6); 1.5913 (1.6); 1.3010 (7.8); 1.2832 (16.0); 1.2654 (7.5); 0.0079 (0.6); 0.0002 (18.5); 0.0085 (0.6) I-397: 1H-NMR(400.6 MHz, CDCl3): = 8.4667 (5.0); 8.4598 (5.1); 8.2978 (2.8); 8.2941 (4.8); 8.2904 (2.7); 8.2582 (2.0); 8.2565 (2.3); 8.2546 (2.4); 8.2530 (2.1); 8.2466 (2.1); 8.2448 (2.4); 8.2429 (2.3); 8.2413 (2.1); 7.5018 (1.6); 7.4981 (1.6); 7.4811 (2.2); 7.4777 (2.5); 7.4750 (1.8); 7.4579 (2.1); 7.4543 (2.0); 7.4251 (1.7); 7.4207 (1.8); 7.4183 (1.8); 7.4139 (1.6); 7.4031 (1.7); 7.3988 (1.9); 7.3963 (1.8); 7.3919 (1.6); 7.3455 (2.0); 7.3365 (2.3); 7.3339 (2.1); 7.3248 (3.5); 7.3158 (1.6); 7.3132 (1.7); 7.3042 (1.4); 7.2611 (43.8); 4.9683 (16.0); 2.4912 (1.0); 2.4708 (1.0); 2.4624 (1.8); 2.4422 (2.2); 2.4330 (1.2); 2.4131 (1.1); 1.8267 (0.8); 1.8152 (1.0); 1.8074 (1.1); 1.7950 (1.4); 1.7848 (1.2); 1.7788 (1.5); 1.7653 (1.9); 1.7595 (0.7); 1.7499 (0.7); 1.7457 (0.5); 1.7363 (0.7); 0.0080 (1.7); 0.0049 (0.5); 0.0002 (64.4); 0.0085 (1.8) I-399: 1H-NMR(400.6 MHz, CDCl3): = 8.4937 (4.4); 8.4869 (4.3); 8.3003 (2.8); 8.2968 (4.4); 7.5783 (1.2); 7.5634 (1.3); 7.5574 (1.8); 7.5426 (1.8); 7.5362 (1.3); 7.5212 (1.2); 7.4714 (1.5); 7.4671 (1.7); 7.4646 (1.7); 7.4603 (1.4); 7.4497 (1.5); 7.4454 (1.8); 7.4430 (1.6); 7.4386 (1.4); 7.2612 (29.7); 6.8970 (1.3); 6.8908 (1.6); 6.8879 (1.6); 6.8816 (1.4); 6.8752 (1.2); 6.8689 (1.4); 6.8661 (1.4); 6.8598 (1.1); 6.3839 (2.0); 6.3550 (2.4); 6.3398 (2.8); 6.3109 (2.8); 6.0221 (2.9); 6.0180 (3.0); 5.9780 (2.4); 5.9738 (2.3); 5.3692 (2.9); 5.3650 (2.5); 5.3403 (2.5); 5.3362 (2.7); 5.3003 (0.8); 5.0092 (16.0); 1.4322 (1.0); 0.0079 (1.3); 0.0002 (43.8); 0.0085 (1.4) I-391: 1H-NMR(400.6 MHz, d6-DMSO): = 8.6186 (3.0); 8.6117 (3.1); 8.2722 (1.7); 8.2680 (3.1); 8.2641 (1.6); 8.2257 (1.2); 8.2225 (1.6); 8.2203 (1.2); 8.2141 (1.2); 8.2118 (1.6); 8.2087 (1.2); 7.9565 (1.0); 7.9530 (1.0); 7.9357 (1.1); 7.9316 (1.6); 7.9277 (1.0); 7.9105 (1.0); 7.9069 (1.0); 7.7640 (1.0); 7.7596 (1.1); 7.7571 (1.1); 7.7528 (1.0); 7.7404 (1.1); 7.7360 (1.2); 7.7335 (1.0); 7.7291 (0.9); 7.5568 (1.1); 7.5475 (1.3); 7.5452 (1.2); 7.5359 (1.9); 7.5266 (0.9); 7.5244 (1.0); 7.5151 (0.8); 6.4306 (1.3); 6.4018 (1.6); 6.3867 (1.8); 6.3578 (1.7); 5.9068 (1.7); 5.9015 (1.8); 5.8628 (1.5); 5.8574 (1.4); 5.7567 (0.8); 5.3253 (1.8); 5.3199 (1.4); 5.2964 (1.4); 5.2911 (1.7); 4.8740 (9.1); 3.6011 (0.8); 3.3237 (16.0); 2.5411 (1.2); 2.5352 (1.0); 2.5242 (1.9); 2.5196 (2.3); 2.5108 (20.9); 2.5062 (44.8); 2.5017 (62.1); 2.4971 (43.3); 2.4925 (19.2); 1.7595 (1.0); 0.0079 (1.1); 0.0002 (40.8); 0.0060 (0.5); 0.0085 (1.2)
B. Formulation Examples
[0541] a) A dusting product is obtained by mixing 10 parts by weight of a compound of the formula (I) and/or salts thereof and 90 parts by weight of talc as inert substance and comminuting the mixture in an impact mill. [0542] b) A readily water-dispersible, wettable powder is obtained by mixing 25 parts by weight of a compound of the formula (I) and/or salts thereof, 64 parts by weight of kaolin-containing quartz as inert substance, 10 parts by weight of potassium lignosulfonate and 1 part by weight of sodium oleoylmethyltaurate as wetting agent and dispersant and grinding in a pinned-disc mill. [0543] c) A readily water-dispersible dispersion concentrate is obtained by mixing 20 parts by weight of a compound of the formula (I) and/or salts thereof with 6 parts by weight of alkylphenol polyglycol ether (Triton X 207), 3 parts by weight of isotridecanol polyglycol ether (8 EO) and 71 parts by weight of paraffinic mineral oil (boiling range e.g. about 255 to more than 277 C.) and grinding to a fineness of below 5 microns in an attrition ball mill. [0544] d) An emulsifiable concentrate is obtained from 15 parts by weight of a compound of the formula (I) and/or salts thereof, 75 parts by weight of cyclohexanone as solvent and 10 parts by weight of oxethylated nonylphenol as emulsifier. [0545] e) Water-dispersible granules are obtained by mixing [0546] 75 parts by weight of a compound of the formula (I) and/or salts thereof, [0547] 10 parts by weight of calcium lignosulfonate, [0548] 5 parts by weight of sodium lauryl sulfate, [0549] 3 parts by weight of polyvinyl alcohol and [0550] 7 parts by weight of kaolin, [0551] grinding the mixture in a pinned-disk mill, and granulating the powder in a fluidized bed by spray application of water as a granulating liquid. [0552] f) Water-dispersible granules are also obtained by homogenizing and precomminuting, in a colloid mill, [0553] 25 parts by weight of a compound of the formula (I) and/or salts thereof, [0554] 5 parts by weight of sodium 2,2-dinaphthylmethane-6,6-disulfonate, [0555] 2 parts by weight of sodium oleoylmethyltaurate, [0556] 1 part by weight of polyvinyl alcohol, [0557] 17 parts by weight of calcium carbonate and [0558] 50 parts by weight of water, [0559] then grinding the mixture in a bead mill and atomizing and drying the resulting suspension in a spray tower by means of a one-phase nozzle.
C. Biological Examples
[0560] A. Pre-Emergence Herbicidal Action and Crop Plant Compatibility
[0561] Seeds of monocotyledonous and dicotyledonous weed plants and crop plants are placed in plastic or organic planting pots and covered with soil. The compounds of the invention, formulated in the form of wettable powders (WP) or as emulsion concentrates (EC), are then applied to the surface of the covering soil as aqueous suspension or emulsion with addition of 0.5% additive at a water application rate equivalent to 600 l/ha. After the treatment, the pots are placed in a greenhouse and kept under good growth conditions for the trial plants. After about 3 weeks, the effect of the preparations is scored visually in comparison with untreated controls as percentages. For example, 100% activity=the plants have died, 0% activity=like control plants.
[0562] Tables A1 to A13 below show the effects of selected compounds of the general formula (I) on various harmful plants and at an application rate corresponding to 320 g/ha or lower, which were obtained by the experimental procedure mentioned above. The appendices a, b and c give differentiation by dosage used with otherwise the same harmful plants tested.
TABLE-US-00005 TABLE A1a Pre-emergence action at 80 g/ha against ABUTH in % Example number Dosage [g/ha] ABUTH I-159 80 80 I-175 80 80 I-18 80 80 I-184 80 90 I-187 80 80 I-188 80 80 I-189 80 80 I-196 80 80 I-199 80 80 I-208 80 80 I-218 80 80 I-325 80 90 I-327 80 100 I-331 80 80 I-332 80 80 I-341 80 90 I-343 80 80 I-73 80 80 I-79 80 80 I-86 80 80 III-24 80 90
TABLE-US-00006 TABLE A1b Pre-emergence action at 3200 g/ha against ABUTH in % Example number Dosage [g/ha] ABUTH I-05 320 80 I-07 320 90 I-08 320 80 I-10 320 80 I-111 320 80 I-13 320 90 I-149 320 80 I-15 320 90 I-154 320 90 I-155 320 90 I-159 320 80 I-164 320 80 I-167 320 90 I-17 320 90 I-171 320 90 I-174 320 90 I-175 320 90 I-18 320 90 I-180 320 80 I-183 320 80 I-184 320 90 I-185 320 80 I-187 320 90 I-188 320 90 I-189 320 90 I-190 320 80 I-191 320 90 I-192 320 80 I-194 320 80 I-195 320 80 I-196 320 90 I-198 320 90 I-199 320 90 I-20 320 90 I-201 320 80 I-204 320 80 I-207 320 80 I-208 320 90 I-211 320 80 I-212 320 80 I-218 320 90 I-221 320 80 I-296 320 80 I-307 320 80 I-308 320 100 I-310 320 80 I-315 320 80 I-317 320 90 I-319 320 80 I-324 320 80 I-325 320 90 I-327 320 100 I-33 320 80 I-330 320 100 I-331 320 90 I-332 320 80 I-339 320 90 I-340 320 80 I-341 320 90 I-342 320 90 I-343 320 100 I-36 320 80 I-375 320 100 I-388 320 90 I-39 320 90 I-41 320 90 I-48 320 80 I-52 320 80 I-60 320 80 I-73 320 90 I-74 320 90 I-76 320 80 I-77 320 80 I-79 320 90 I-81 320 90 I-83 320 80 I-84 320 80 I-86 320 100 I-88 320 80 I-96 320 80 III-22 320 100 III-24 320 100
TABLE-US-00007 TABLE A2a Pre-emergence action at 80 g/ha against ALOMY in % Example number Dosage [g/ha] ALOMY I-02 80 100 I-03 80 90 I-05 80 90 I-07 80 90 I-08 80 100 I-10 80 100 I-100 80 100 I-102 80 100 I-107 80 90 I-11 80 90 I-116 80 90 I-118 80 90 I-122 80 80 I-13 80 90 I-148 80 100 I-149 80 90 I-15 80 100 I-154 80 80 I-159 80 80 I-16 80 100 I-164 80 100 I-167 80 90 I-17 80 100 I-171 80 100 I-174 80 90 I-175 80 100 I-18 80 100 I-180 80 90 I-184 80 90 I-185 80 80 I-187 80 90 I-188 80 90 I-189 80 80 I-19 80 100 I-190 80 80 I-191 80 80 I-192 80 90 I-194 80 80 I-195 80 80 I-198 80 80 I-199 80 90 I-20 80 90 I-204 80 90 I-208 80 90 I-210 80 80 I-211 80 80 I-212 80 100 I-218 80 90 I-225 80 80 I-24 80 100 I-247 80 80 I-25 80 80 I-29 80 90 I-291 80 100 I-293 80 90 I-296 80 80 I-30 80 100 I-307 80 80 I-308 80 100 I-311 80 80 I-313 80 90 I-315 80 100 I-316 80 90 I-317 80 100 I-32 80 90 I-322 80 80 I-323 80 100 I-324 80 100 I-33 80 100 I-331 80 100 I-333 80 90 I-334 80 80 I-336 80 80 I-337 80 80 I-338 80 100 I-339 80 100 I-34 80 90 I-342 80 100 I-343 80 90 I-35 80 90 I-350 80 100 I-358 80 80 I-36 80 100 I-360 80 100 I-369 80 80 I-37 80 100 I-370 80 80 I-374 80 90 I-375 80 80 I-38 80 100 I-388 80 80 I-39 80 100 I-40 80 100 I-41 80 80 I-42 80 100 I-43 80 100 I-44 80 100 I-45 80 90 I-46 80 90 I-47 80 90 I-48 80 80 I-51 80 90 I-52 80 90 I-53 80 80 I-56 80 100 I-59 80 80 I-64 80 90 I-66 80 100 I-73 80 90 I-74 80 80 I-75 80 80 I-76 80 90 I-79 80 90 I-80 80 100 I-81 80 80 I-83 80 90 I-84 80 80 I-85 80 80 I-86 80 100 I-87 80 90 I-88 80 80 I-90 80 90 I-91 80 90 I-93 80 90 I-94 80 80 I-96 80 80 I-97 80 90 I-98 80 90 I-99 80 80 III-22 80 100 III-24 80 100
TABLE-US-00008 TABLE A2b Pre-emergence action at 320 g/ha against ALOMY in % Example number Dosage [g/ha] ALOMY I-01 320 100 I-02 320 90 I-03 320 100 I-04 320 100 I-05 320 100 I-07 320 100 I-08 320 100 I-10 320 100 I-100 320 100 I-101 320 100 I-102 320 100 I-103 320 100 I-107 320 90 I-11 320 100 I-111 320 90 I-114 320 100 I-116 320 100 I-118 320 100 I-119 320 100 I-120 320 80 I-121 320 100 I-122 320 100 I-125 320 80 I-126 320 80 I-13 320 100 I-148 320 100 I-149 320 100 I-15 320 100 I-151 320 100 I-152 320 80 I-153 320 90 I-154 320 90 I-155 320 100 I-157 320 80 I-159 320 90 I-16 320 100 I-163 320 90 I-164 320 100 I-167 320 100 I-17 320 100 I-171 320 100 I-174 320 100 I-175 320 100 I-18 320 100 I-180 320 100 I-183 320 80 I-184 320 100 I-185 320 90 I-186 320 90 I-187 320 100 I-188 320 100 I-189 320 90 I-19 320 100 I-190 320 90 I-191 320 90 I-192 320 90 I-193 320 90 I-194 320 100 I-195 320 90 I-196 320 90 I-198 320 90 I-199 320 90 I-20 320 100 I-202 320 80 I-204 320 100 I-206 320 80 I-207 320 80 I-208 320 100 I-210 320 90 I-211 320 100 I-212 320 100 I-216 320 90 I-218 320 90 I-221 320 90 I-223 320 90 I-225 320 90 I-23 320 100 I-231 320 90 I-237 320 90 I-238 320 90 I-24 320 100 I-240 320 90 I-241 320 80 I-242 320 80 I-244 320 90 I-245 320 90 I-247 320 100 I-25 320 90 I-26 320 100 I-27 320 100 I-272 320 90 I-276 320 80 I-28 320 100 I-29 320 100 I-291 320 100 I-293 320 100 I-296 320 100 I-297 320 80 I-298 320 90 I-30 320 100 I-302 320 90 I-305 320 90 I-306 320 90 I-307 320 90 I-308 320 100 I-309 320 90 I-310 320 100 I-311 320 90 I-313 320 100 I-315 320 100 I-316 320 100 I-317 320 100 I-319 320 100 I-32 320 100 I-320 320 90 I-321 320 100 I-322 320 100 I-323 320 100 I-324 320 100 I-325 320 100 I-327 320 100 I-33 320 100 I-330 320 100 I-331 320 100 I-332 320 100 I-333 320 100 I-334 320 90 I-335 320 80 I-336 320 100 I-337 320 90 I-338 320 100 I-339 320 100 I-34 320 100 I-340 320 100 I-341 320 100 I-342 320 100 I-343 320 90 I-347 320 80 I-348 320 80 I-35 320 100 I-350 320 100 I-354 320 80 I-358 320 100 I-36 320 100 I-360 320 100 I-362 320 100 I-369 320 100 I-37 320 100 I-370 320 100 I-373 320 90 I-374 320 100 I-375 320 90 I-376 320 80 I-377 320 80 I-378 320 80 I-38 320 100 I-381 320 90 I-388 320 100 I-39 320 100 I-40 320 100 I-41 320 100 I-42 320 100 I-43 320 100 I-44 320 100 I-46 320 100 I-47 320 90 I-48 320 100 I-51 320 100 I-52 320 100 I-53 320 100 I-54 320 100 I-56 320 100 I-58 320 90 I-59 320 100 I-64 320 100 I-65 320 80 I-66 320 100 I-70 320 90 I-71 320 90 I-72 320 100 I-73 320 100 I-74 320 100 I-75 320 90 I-76 320 100 I-77 320 90 I-78 320 90 I-79 320 100 I-80 320 100 I-81 320 100 I-83 320 100 I-84 320 100 I-85 320 90 I-86 320 100 I-87 320 100 I-88 320 100 I-90 320 100 I-91 320 100 I-93 320 100 I-94 320 100 I-95 320 80 I-96 320 100 I-97 320 100 I-98 320 100 I-99 320 100 II-36 320 100 III-07 320 80 III-22 320 100 III-23 320 90 III-24 320 100
TABLE-US-00009 TABLE A3a Pre-emergence action at 80 g/ha against AMARE in % Example number Dosage [g/ha] AMARE I-01 80 80 I-02 80 100 I-03 80 90 I-04 80 90 I-05 80 90 I-07 80 90 I-08 80 100 I-10 80 100 I-100 80 90 I-102 80 80 I-103 80 80 I-111 80 90 I-116 80 90 I-118 80 90 I-121 80 100 I-122 80 80 I-13 80 90 I-148 80 100 I-149 80 90 I-15 80 100 I-151 80 90 I-154 80 90 I-155 80 90 I-159 80 90 I-16 80 100 I-164 80 100 I-167 80 100 I-17 80 100 I-171 80 100 I-174 80 100 I-175 80 100 I-18 80 100 I-180 80 100 I-183 80 80 I-184 80 100 I-185 80 100 I-187 80 80 I-188 80 100 I-189 80 100 I-19 80 100 I-190 80 90 I-191 80 90 I-192 80 80 I-193 80 80 I-194 80 100 I-195 80 90 I-196 80 100 I-198 80 100 I-199 80 100 I-20 80 100 I-204 80 90 I-207 80 90 I-208 80 90 I-210 80 80 I-211 80 100 I-212 80 90 I-216 80 90 I-217 80 80 I-218 80 100 I-221 80 80 I-23 80 90 I-235 80 80 I-239 80 80 I-24 80 90 I-243 80 80 I-247 80 80 I-25 80 90 I-27 80 90 I-28 80 90 I-29 80 90 I-291 80 80 I-296 80 80 I-30 80 100 I-305 80 80 I-307 80 100 I-308 80 100 I-310 80 80 I-311 80 80 I-313 80 90 I-315 80 90 I-316 80 100 I-317 80 100 I-32 80 90 I-320 80 80 I-321 80 100 I-323 80 100 I-324 80 100 I-325 80 100 I-33 80 90 I-331 80 100 I-332 80 80 I-333 80 90 I-334 80 90 I-336 80 90 I-337 80 90 I-338 80 100 I-339 80 100 I-34 80 100 I-340 80 90 I-341 80 100 I-342 80 100 I-343 80 100 I-35 80 100 I-350 80 100 I-354 80 80 I-358 80 80 I-360 80 90 I-369 80 90 I-37 80 100 I-370 80 100 I-374 80 100 I-375 80 100 I-377 80 80 I-378 80 80 I-38 80 100 I-388 80 90 I-39 80 100 I-40 80 80 I-41 80 100 I-42 80 90 I-43 80 80 I-44 80 80 I-45 80 90 I-46 80 100 I-47 80 100 I-48 80 90 I-51 80 100 I-52 80 80 I-53 80 90 I-56 80 100 I-59 80 100 I-64 80 100 I-66 80 90 I-69 80 80 I-73 80 100 I-74 80 90 I-75 80 80 I-76 80 90 I-77 80 90 I-79 80 100 I-80 80 90 I-81 80 80 I-83 80 90 I-84 80 80 I-85 80 90 I-86 80 100 I-87 80 90 I-88 80 80 I-90 80 100 I-91 80 90 I-93 80 90 I-94 80 80 I-95 80 90 I-96 80 90 I-97 80 90 I-98 80 100 III-22 80 90 III-24 80 100
TABLE-US-00010 TABLE A3b Pre-emergence action at 320 g/ha against AMARE in % Example number Dosage [g/ha] AMARE I-01 320 90 I-02 320 100 I-03 320 100 I-04 320 100 I-05 320 100 I-07 320 90 I-08 320 100 I-10 320 100 I-100 320 100 I-101 320 100 I-102 320 90 I-103 320 90 I-107 320 100 I-11 320 100 I-111 320 100 I-116 320 100 I-118 320 100 I-119 320 100 I-120 320 90 I-121 320 100 I-122 320 100 I-125 320 100 I-126 320 100 I-13 320 100 I-147 320 90 I-148 320 100 I-149 320 100 I-15 320 100 I-150 320 80 I-151 320 100 I-152 320 100 I-153 320 100 I-154 320 100 I-155 320 100 I-156 320 100 I-159 320 100 I-16 320 100 I-160 320 80 I-162 320 90 I-163 320 90 I-164 320 100 I-167 320 100 I-17 320 100 I-171 320 100 I-174 320 100 I-175 320 100 I-18 320 100 I-180 320 100 I-183 320 100 I-184 320 100 I-185 320 100 I-186 320 90 I-187 320 100 I-188 320 100 I-189 320 100 I-19 320 100 I-190 320 100 I-191 320 100 I-192 320 100 I-193 320 100 I-194 320 100 I-195 320 100 I-196 320 100 I-198 320 100 I-199 320 100 I-20 320 100 I-202 320 90 I-204 320 100 I-205 320 80 I-206 320 90 I-207 320 100 I-208 320 100 I-210 320 100 I-211 320 100 I-212 320 100 I-216 320 90 I-217 320 100 I-218 320 100 I-221 320 90 I-223 320 90 I-225 320 100 I-229 320 80 I-23 320 100 I-230 320 80 I-231 320 90 I-235 320 90 I-236 320 80 I-237 320 100 I-238 320 80 I-239 320 90 I-24 320 100 I-240 320 90 I-241 320 90 I-242 320 100 I-243 320 90 I-244 320 90 I-245 320 80 I-246 320 90 I-247 320 100 I-25 320 100 I-26 320 100 I-27 320 100 I-272 320 90 I-276 320 90 I-277 320 80 I-278 320 80 I-28 320 100 I-29 320 100 I-291 320 100 I-293 320 100 I-296 320 90 I-297 320 80 I-298 320 100 I-30 320 100 I-300 320 90 I-302 320 90 I-305 320 90 I-306 320 90 I-307 320 100 I-308 320 100 I-309 320 90 I-31 320 90 I-310 320 100 I-311 320 90 I-312 320 90 I-313 320 100 I-315 320 90 I-316 320 100 I-317 320 100 I-319 320 100 I-32 320 100 I-320 320 90 I-321 320 100 I-322 320 100 I-323 320 100 I-324 320 100 I-325 320 100 I-327 320 100 I-33 320 100 I-330 320 100 I-331 320 100 I-332 320 100 I-333 320 100 I-334 320 100 I-335 320 90 I-336 320 100 I-337 320 90 I-338 320 100 I-339 320 100 I-34 320 100 I-340 320 100 I-341 320 100 I-342 320 100 I-343 320 100 I-348 320 90 I-35 320 100 I-350 320 100 I-351 320 80 I-352 320 90 I-354 320 90 I-358 320 100 I-359 320 90 I-36 320 100 I-360 320 100 I-362 320 90 I-369 320 90 I-37 320 100 I-370 320 100 I-373 320 90 I-374 320 100 I-375 320 100 I-376 320 90 I-377 320 90 I-378 320 90 I-38 320 100 I-381 320 90 I-388 320 100 I-39 320 100 I-40 320 100 I-41 320 100 I-42 320 100 I-43 320 90 I-44 320 90 I-46 320 100 I-47 320 100 I-48 320 100 I-51 320 100 I-52 320 100 I-53 320 100 I-54 320 100 I-56 320 100 I-59 320 100 I-60 320 90 I-64 320 100 I-65 320 90 I-66 320 100 I-69 320 90 I-70 320 90 I-72 320 90 I-73 320 100 I-74 320 100 I-75 320 90 I-76 320 100 I-77 320 100 I-79 320 100 I-80 320 90 I-81 320 90 I-83 320 100 I-84 320 100 I-85 320 100 I-86 320 100 I-87 320 100 I-88 320 100 I-90 320 100 I-91 320 100 I-93 320 100 I-94 320 100 I-95 320 100 I-96 320 100 I-97 320 100 I-98 320 100 I-99 320 90 II-36 320 100 III-02 320 80 III-08 320 80 III-09 320 80 III-17 320 90 III-19 320 80 III-22 320 100 III-23 320 90 III-24 320 100 III-25 320 80 III-28 320 80
TABLE-US-00011 TABLE A4a Pre-emergence action at 80 g/ha against AVEFA in % Example number Dosage [g/ha] AVEFA I-02 80 90 I-08 80 80 I-100 80 80 I-148 80 80 I-149 80 80 I-15 80 80 I-164 80 90 I-167 80 90 I-17 80 80 I-171 80 90 I-18 80 90 I-180 80 90 I-184 80 80 I-188 80 80 I-189 80 90 I-19 80 80 I-194 80 80 I-196 80 80 I-199 80 80 I-20 80 90 I-208 80 80 I-212 80 80 I-218 80 80 I-25 80 90 I-291 80 80 I-293 80 80 I-307 80 90 I-308 80 100 I-317 80 90 I-32 80 90 I-323 80 90 I-33 80 80 I-330 80 80 I-331 80 100 I-333 80 80 I-338 80 90 I-339 80 100 I-34 80 80 I-340 80 80 I-342 80 90 I-343 80 80 I-370 80 90 I-375 80 90 I-41 80 90 I-52 80 90 I-77 80 80 I-83 80 80 I-84 80 80 I-87 80 80 I-94 80 80 III-22 80 80 III-24 80 100
TABLE-US-00012 TABLE A4b Pre-emergence action at 320 g/ha against AVEFA in % Example number Dosage [g/ha] AVEFA I-01 320 80 I-02 320 100 I-03 320 80 I-05 320 90 I-07 320 90 I-08 320 90 I-10 320 100 I-100 320 90 I-101 320 90 I-102 320 90 I-103 320 80 I-107 320 80 I-11 320 90 I-111 320 80 I-116 320 90 I-118 320 90 I-119 320 80 I-121 320 90 I-122 320 90 I-13 320 90 I-147 320 80 I-148 320 90 I-149 320 90 I-15 320 100 I-154 320 80 I-155 320 90 I-159 320 90 I-16 320 90 I-164 320 90 I-167 320 90 I-17 320 100 I-171 320 100 I-174 320 90 I-175 320 90 I-18 320 100 I-180 320 90 I-183 320 80 I-184 320 90 I-185 320 90 I-186 320 80 I-187 320 90 I-188 320 90 I-189 320 90 I-19 320 100 I-190 320 90 I-191 320 100 I-192 320 90 I-193 320 90 I-194 320 90 I-195 320 90 I-196 320 90 I-198 320 90 I-199 320 90 I-20 320 100 I-204 320 80 I-207 320 80 I-208 320 90 I-211 320 90 I-212 320 90 I-218 320 90 I-223 320 100 I-225 320 90 I-23 320 90 I-231 320 90 I-24 320 100 I-247 320 80 I-25 320 100 I-26 320 90 I-27 320 100 I-272 320 100 I-28 320 100 I-29 320 90 I-291 320 90 I-293 320 90 I-296 320 90 I-298 320 90 I-30 320 100 I-306 320 80 I-307 320 100 I-308 320 100 I-31 320 80 I-310 320 90 I-311 320 90 I-313 320 90 I-315 320 90 I-316 320 100 I-317 320 100 I-319 320 100 I-32 320 100 I-320 320 90 I-321 320 90 I-322 320 90 I-323 320 100 I-324 320 100 I-325 320 100 I-327 320 80 I-33 320 100 I-330 320 90 I-331 320 100 I-332 320 100 I-333 320 90 I-334 320 90 I-335 320 80 I-336 320 90 I-337 320 90 I-338 320 90 I-339 320 100 I-34 320 90 I-340 320 90 I-341 320 90 I-342 320 100 I-343 320 90 I-348 320 90 I-35 320 100 I-350 320 100 I-351 320 80 I-358 320 80 I-36 320 90 I-360 320 90 I-369 320 80 I-37 320 90 I-370 320 90 I-374 320 100 I-375 320 100 I-38 320 100 I-388 320 90 I-39 320 90 I-40 320 100 I-41 320 100 I-42 320 100 I-43 320 100 I-44 320 90 I-46 320 90 I-47 320 90 I-48 320 100 I-51 320 90 I-52 320 100 I-53 320 100 I-56 320 100 I-58 320 80 I-59 320 80 I-64 320 90 I-66 320 90 I-69 320 80 I-73 320 80 I-74 320 80 I-75 320 80 I-76 320 90 I-77 320 90 I-79 320 100 I-80 320 90 I-81 320 80 I-83 320 90 I-84 320 90 I-85 320 90 I-86 320 90 I-87 320 90 I-88 320 90 I-91 320 100 I-93 320 90 I-94 320 90 I-95 320 80 I-96 320 90 I-97 320 80 I-98 320 80 I-99 320 90 II-36 320 80 III-22 320 100 III-24 320 100
TABLE-US-00013 TABLE A5a Pre-emergence action at 80 g/ha against DIGSA in % Example number Dosage [g/ha] DIGSA I-01 80 80 I-03 80 90 I-05 80 100 I-07 80 100 I-08 80 100 I-10 80 100 I-11 80 100 I-118 80 100 I-119 80 100 I-120 80 100 I-121 80 100 I-122 80 100 I-126 80 90 I-13 80 100 I-148 80 90 I-149 80 90 I-15 80 100 I-154 80 90 I-159 80 90 I-16 80 100 I-163 80 90 I-164 80 90 I-167 80 100 I-17 80 100 I-171 80 80 I-174 80 100 I-175 80 100 I-18 80 100 I-180 80 90 I-19 80 100 I-192 80 90 I-194 80 90 I-195 80 90 I-208 80 90 I-212 80 100 I-216 80 90 I-221 80 90 I-231 80 90 I-247 80 100 I-29 80 100 I-291 80 100 I-293 80 80 I-296 80 90 I-298 80 100 I-30 80 100 I-300 80 90 I-302 80 90 I-322 80 100 I-348 80 90 I-349 80 80 I-36 80 100 I-360 80 90 I-37 80 100 I-38 80 100 I-39 80 100 I-45 80 100 I-46 80 100 I-54 80 100 I-56 80 100 I-59 80 100 I-64 80 100 I-66 80 100 I-90 80 100 I-97 80 100
TABLE-US-00014 TABLE A5b Pre-emergence action at 320 g/ha against DIGSA in % Example number Dosage [g/ha] DIGSA I-01 320 100 I-03 320 100 I-05 320 100 I-07 320 100 I-08 320 100 I-10 320 100 I-11 320 100 I-114 320 90 I-118 320 100 I-119 320 100 I-120 320 100 I-121 320 100 I-122 320 100 I-125 320 100 I-126 320 100 I-13 320 100 I-148 320 100 I-149 320 100 I-15 320 100 I-154 320 100 I-159 320 100 I-16 320 100 I-163 320 100 I-164 320 100 I-167 320 100 I-17 320 100 I-171 320 100 I-174 320 100 I-175 320 100 I-18 320 100 I-180 320 100 I-19 320 100 I-192 320 100 I-194 320 100 I-195 320 100 I-206 320 90 I-208 320 100 I-212 320 100 I-216 320 100 I-221 320 100 I-223 320 80 I-231 320 100 I-235 320 90 I-236 320 90 I-237 320 90 I-238 320 90 I-239 320 90 I-240 320 90 I-241 320 90 I-242 320 90 I-243 320 80 I-244 320 90 I-245 320 90 I-246 320 90 I-247 320 100 I-29 320 100 I-291 320 100 I-293 320 100 I-296 320 100 I-297 320 80 I-298 320 100 I-30 320 100 I-300 320 100 I-302 320 100 I-322 320 100 I-345 320 90 I-347 320 90 I-348 320 100 I-349 320 90 I-36 320 100 I-360 320 100 I-37 320 100 I-38 320 100 I-39 320 100 I-46 320 100 I-54 320 100 I-56 320 100 I-59 320 100 I-64 320 100 I-66 320 100 I-90 320 100 I-97 320 100 II-36 320 100
TABLE-US-00015 TABLE A6a Pre-emergence action at 80 g/ha against ECHCG in % Example number Dosage [g/ha] ECHCG I-08 80 80 I-10 80 80 I-100 80 80 I-119 80 80 I-148 80 90 I-149 80 90 I-153 80 80 I-154 80 90 I-155 80 90 I-159 80 90 I-16 80 90 I-163 80 80 I-164 80 90 I-167 80 100 I-17 80 90 I-171 80 100 I-174 80 100 I-175 80 100 I-18 80 90 I-180 80 100 I-184 80 90 I-185 80 80 I-187 80 90 I-188 80 100 I-189 80 90 I-190 80 90 I-191 80 90 I-192 80 90 I-193 80 90 I-194 80 80 I-196 80 90 I-198 80 90 I-199 80 90 I-204 80 90 I-207 80 90 I-208 80 90 I-210 80 90 I-211 80 90 I-212 80 100 I-216 80 80 I-218 80 90 I-221 80 90 I-231 80 90 I-298 80 90 I-307 80 100 I-308 80 100 I-315 80 90 I-316 80 100 I-317 80 100 I-321 80 100 I-322 80 80 I-323 80 90 I-33 80 90 I-331 80 80 I-332 80 80 I-334 80 80 I-336 80 80 I-337 80 80 I-338 80 90 I-341 80 80 I-342 80 100 I-35 80 90 I-350 80 100 I-375 80 80 I-388 80 80 I-40 80 90 I-41 80 80 I-42 80 100 I-44 80 80 I-45 80 90 I-51 80 80 I-66 80 80 I-74 80 80 I-75 80 80 I-79 80 80 I-81 80 90 I-84 80 80 I-85 80 100 I-86 80 100 I-87 80 100 I-88 80 90 I-96 80 80 III-22 80 100 III-24 80 90
TABLE-US-00016 TABLE A6b Pre-emergence action at 320 g/ha against ECHCG in % Example number Dosage [g/ha] ECHCG I-01 320 90 I-02 320 100 I-03 320 80 I-04 320 90 I-05 320 100 I-07 320 100 I-08 320 100 I-10 320 90 I-100 320 100 I-101 320 90 I-107 320 100 I-11 320 80 I-111 320 100 I-116 320 100 I-118 320 100 I-119 320 100 I-121 320 100 I-122 320 100 I-125 320 80 I-126 320 90 I-13 320 90 I-148 320 100 I-149 320 100 I-15 320 90 I-151 320 90 I-152 320 90 I-153 320 100 I-154 320 100 I-155 320 100 I-156 320 90 I-157 320 80 I-159 320 90 I-16 320 90 I-160 320 90 I-162 320 80 I-163 320 90 I-164 320 100 I-167 320 100 I-17 320 90 I-171 320 100 I-174 320 100 I-175 320 100 I-18 320 90 I-180 320 100 I-183 320 100 I-184 320 100 I-185 320 90 I-186 320 80 I-187 320 100 I-188 320 100 I-189 320 100 I-19 320 100 I-190 320 100 I-191 320 100 I-192 320 100 I-193 320 100 I-194 320 100 I-195 320 100 I-196 320 90 I-198 320 100 I-199 320 90 I-20 320 100 I-201 320 90 I-202 320 90 I-204 320 100 I-205 320 80 I-206 320 80 I-207 320 100 I-208 320 100 I-210 320 100 I-211 320 100 I-212 320 100 I-216 320 100 I-217 320 90 I-218 320 100 I-221 320 100 I-223 320 80 I-225 320 80 I-229 320 90 I-23 320 100 I-230 320 90 I-231 320 90 I-24 320 100 I-247 320 100 I-25 320 90 I-27 320 100 I-276 320 90 I-277 320 80 I-28 320 100 I-29 320 100 I-291 320 90 I-293 320 90 I-296 320 100 I-298 320 100 I-30 320 100 I-300 320 90 I-302 320 90 I-305 320 90 I-307 320 100 I-308 320 100 I-309 320 80 I-31 320 90 I-311 320 100 I-313 320 100 I-315 320 100 I-316 320 100 I-317 320 100 I-319 320 100 I-32 320 100 I-320 320 90 I-321 320 100 I-322 320 100 I-323 320 100 I-324 320 100 I-33 320 100 I-330 320 100 I-331 320 100 I-332 320 100 I-333 320 90 I-334 320 90 I-336 320 100 I-337 320 90 I-338 320 100 I-339 320 100 I-34 320 100 I-340 320 100 I-341 320 100 I-342 320 100 I-343 320 100 I-348 320 90 I-35 320 100 I-350 320 100 I-351 320 90 I-352 320 90 I-354 320 100 I-358 320 100 I-359 320 80 I-36 320 100 I-360 320 100 I-369 320 100 I-37 320 100 I-370 320 100 I-373 320 90 I-374 320 100 I-375 320 100 I-376 320 90 I-38 320 100 I-388 320 100 I-39 320 100 I-40 320 100 I-41 320 100 I-42 320 100 I-43 320 100 I-44 320 100 I-46 320 90 I-47 320 90 I-48 320 100 I-51 320 90 I-52 320 100 I-53 320 80 I-54 320 100 I-56 320 100 I-59 320 100 I-64 320 100 I-65 320 90 I-66 320 100 I-69 320 90 I-73 320 90 I-74 320 100 I-75 320 100 I-76 320 90 I-77 320 100 I-79 320 100 I-80 320 100 I-81 320 100 I-82 320 90 I-83 320 100 I-84 320 100 I-85 320 100 I-86 320 100 I-87 320 100 I-88 320 100 I-90 320 100 I-91 320 100 I-93 320 100 I-94 320 80 I-96 320 100 I-98 320 100 III-22 320 100 III-24 320 100
TABLE-US-00017 TABLE A7a Pre-emergence action at 80 g/ha against LOLRI in % [g/ha] Example number Dosage [g/ha] LOLRI I-02 80 90 I-05 80 80 I-08 80 80 I-10 80 100 I-102 80 80 I-107 80 80 I-118 80 90 I-148 80 90 I-149 80 100 I-15 80 90 I-154 80 90 I-155 80 90 I-159 80 90 I-16 80 90 I-164 80 100 I-167 80 100 I-171 80 100 I-174 80 100 I-175 80 100 I-18 80 90 I-180 80 100 I-184 80 100 I-185 80 100 I-187 80 90 I-188 80 100 I-189 80 100 I-190 80 100 I-191 80 90 I-192 80 80 I-194 80 90 I-195 80 80 I-196 80 100 I-198 80 100 I-199 80 100 I-20 80 100 I-208 80 90 I-212 80 80 I-218 80 100 I-221 80 80 I-27 80 100 I-291 80 90 I-293 80 100 I-298 80 90 I-30 80 90 I-300 80 80 I-302 80 80 I-307 80 100 I-308 80 100 I-311 80 90 I-316 80 100 I-317 80 100 I-319 80 90 I-32 80 90 I-321 80 100 I-322 80 90 I-323 80 100 I-324 80 100 I-33 80 90 I-331 80 90 I-332 80 90 I-333 80 80 I-336 80 80 I-338 80 100 I-339 80 100 I-34 80 90 I-340 80 100 I-341 80 100 I-342 80 100 I-343 80 90 I-348 80 90 I-35 80 90 I-350 80 100 I-358 80 100 I-37 80 80 I-370 80 90 I-374 80 80 I-375 80 100 I-388 80 80 I-40 80 90 I-41 80 100 I-43 80 90 I-44 80 80 I-46 80 90 I-48 80 100 I-52 80 90 I-56 80 100 I-59 80 80 I-64 80 80 I-66 80 80 I-73 80 100 I-75 80 80 I-76 80 90 I-77 80 90 I-79 80 100 I-81 80 90 I-83 80 100 I-84 80 90 I-86 80 100 I-91 80 100 I-94 80 100 I-96 80 90 I-97 80 80 III-22 80 100 III-24 80 100
TABLE-US-00018 TABLE A7b Pre-emergence action at 320 g/ha against LOLRI in % Example number Dosage [g/ha] LOLRI I-01 320 100 I-02 320 100 I-03 320 100 I-04 320 90 I-05 320 100 I-07 320 100 I-08 320 100 I-10 320 100 I-100 320 100 I-101 320 100 I-102 320 100 I-103 320 100 I-107 320 100 I-11 320 100 I-111 320 100 I-116 320 100 I-118 320 100 I-119 320 100 I-120 320 80 I-121 320 100 I-122 320 100 I-125 320 80 I-126 320 100 I-13 320 90 I-148 320 100 I-149 320 100 I-15 320 100 I-151 320 90 I-153 320 80 I-154 320 100 I-155 320 100 I-156 320 80 I-159 320 100 I-16 320 100 I-163 320 90 I-164 320 100 I-167 320 100 I-17 320 100 I-171 320 100 I-174 320 100 I-175 320 100 I-18 320 100 I-180 320 100 I-183 320 90 I-184 320 100 I-185 320 100 I-187 320 100 I-188 320 100 I-189 320 100 I-19 320 100 I-190 320 100 I-191 320 90 I-192 320 100 I-193 320 90 I-194 320 100 I-195 320 100 I-196 320 100 I-198 320 100 I-199 320 100 I-20 320 100 I-208 320 100 I-210 320 80 I-211 320 80 I-212 320 90 I-216 320 80 I-217 320 100 I-218 320 100 I-221 320 100 I-229 320 80 I-23 320 100 I-231 320 80 I-236 320 90 I-237 320 90 I-238 320 90 I-24 320 100 I-240 320 90 I-241 320 90 I-242 320 90 I-244 320 100 I-245 320 90 I-247 320 100 I-25 320 100 I-27 320 100 I-272 320 80 I-276 320 100 I-277 320 90 I-278 320 80 I-279 320 80 I-28 320 100 I-29 320 100 I-291 320 100 I-293 320 100 I-296 320 100 I-298 320 100 I-30 320 100 I-300 320 90 I-302 320 90 I-305 320 90 I-306 320 100 I-307 320 100 I-308 320 100 I-310 320 100 I-311 320 90 I-313 320 100 I-315 320 100 I-316 320 100 I-317 320 100 I-319 320 100 I-32 320 100 I-320 320 100 I-321 320 100 I-322 320 100 I-323 320 100 I-324 320 100 I-325 320 100 I-327 320 100 I-33 320 100 I-330 320 90 I-331 320 100 I-332 320 100 I-333 320 100 I-334 320 90 I-335 320 90 I-336 320 100 I-337 320 100 I-338 320 100 I-339 320 100 I-34 320 100 I-340 320 100 I-341 320 100 I-342 320 100 I-343 320 90 I-348 320 100 I-35 320 100 I-350 320 100 I-352 320 80 I-358 320 100 I-359 320 80 I-36 320 100 I-360 320 100 I-362 320 100 I-369 320 90 I-37 320 100 I-370 320 100 I-373 320 80 I-374 320 100 I-375 320 100 I-376 320 90 I-378 320 90 I-38 320 100 I-381 320 90 I-388 320 100 I-39 320 100 I-40 320 100 I-41 320 100 I-42 320 100 I-43 320 100 I-44 320 100 I-46 320 100 I-47 320 100 I-48 320 100 I-51 320 90 I-52 320 100 I-53 320 100 I-56 320 100 I-58 320 80 I-59 320 100 I-60 320 80 I-64 320 100 I-65 320 90 I-66 320 100 I-69 320 80 I-70 320 90 I-71 320 90 I-72 320 100 I-73 320 100 I-74 320 100 I-75 320 100 I-76 320 100 I-77 320 100 I-79 320 100 I-80 320 100 I-81 320 100 I-83 320 100 I-84 320 100 I-85 320 100 I-86 320 100 I-87 320 100 I-88 320 100 I-90 320 100 I-91 320 100 I-93 320 100 I-94 320 100 I-96 320 100 I-97 320 100 I-98 320 100 I-99 320 100 II-36 320 80 III-22 320 100 III-23 320 100 III-24 320 100
TABLE-US-00019 TABLE A8a Pre-emergence action at 80 g/ha against MATIN in % Example number Dosage [g/ha] MATIN I-07 80 80 I-10 80 80 I-100 80 80 I-13 80 80 I-148 80 90 I-149 80 90 I-15 80 100 I-151 80 90 I-154 80 90 I-155 80 90 I-159 80 90 I-16 80 100 I-163 80 90 I-164 80 90 I-167 80 90 I-17 80 90 I-171 80 90 I-174 80 90 I-175 80 90 I-18 80 100 I-180 80 90 I-183 80 90 I-184 80 90 I-185 80 80 I-187 80 90 I-188 80 90 I-189 80 90 I-190 80 90 I-191 80 90 I-192 80 90 I-193 80 90 I-194 80 90 I-195 80 90 I-196 80 90 I-198 80 90 I-199 80 90 I-207 80 90 I-208 80 90 I-210 80 90 I-211 80 90 I-212 80 80 I-216 80 90 I-217 80 80 I-218 80 90 I-221 80 90 I-231 80 90 I-296 80 80 I-305 80 80 I-306 80 90 I-307 80 90 I-308 80 100 I-311 80 80 I-315 80 80 I-317 80 100 I-325 80 100 I-327 80 80 I-330 80 80 I-331 80 100 I-333 80 80 I-334 80 80 I-336 80 80 I-341 80 90 I-342 80 100 I-369 80 80 I-375 80 100 I-377 80 80 I-38 80 100 I-388 80 90 I-45 80 80 I-46 80 90 I-51 80 90 I-65 80 80 I-74 80 90 I-75 80 90 I-76 80 90 I-77 80 80 I-79 80 80 I-81 80 80 I-83 80 90 I-84 80 90 I-85 80 100
TABLE-US-00020 TABLE A8b Pre-emergence action at 320 g/ha against MATIN in % Example number Dosage [g/ha] MATIN I-01 320 100 I-02 320 100 I-03 320 100 I-04 320 90 I-05 320 90 I-07 320 100 I-08 320 100 I-10 320 100 I-100 320 80 I-107 320 90 I-11 320 90 I-111 320 80 I-116 320 90 I-118 320 90 I-119 320 90 I-121 320 80 I-122 320 80 I-125 320 90 I-126 320 90 I-13 320 80 I-148 320 90 I-149 320 90 I-15 320 100 I-151 320 90 I-152 320 90 I-153 320 80 I-154 320 100 I-155 320 90 I-156 320 80 I-159 320 90 I-16 320 100 I-160 320 80 I-163 320 90 I-164 320 100 I-167 320 90 I-17 320 100 I-171 320 90 I-174 320 90 I-175 320 90 I-18 320 100 I-180 320 90 I-183 320 90 I-184 320 90 I-185 320 90 I-187 320 90 I-188 320 90 I-189 320 100 I-19 320 90 I-190 320 90 I-191 320 90 I-192 320 90 I-193 320 90 I-194 320 90 I-195 320 90 I-196 320 90 I-198 320 90 I-199 320 100 I-20 320 100 I-201 320 80 I-202 320 80 I-204 320 90 I-206 320 90 I-207 320 90 I-208 320 90 I-210 320 90 I-211 320 90 I-212 320 90 I-216 320 90 I-217 320 90 I-218 320 100 I-221 320 90 I-225 320 80 I-229 320 80 I-23 320 90 I-231 320 90 I-24 320 90 I-247 320 90 I-25 320 90 I-27 320 80 I-276 320 80 I-278 320 80 I-279 320 80 I-28 320 90 I-29 320 100 I-291 320 90 I-293 320 80 I-296 320 90 I-298 320 90 I-30 320 90 I-300 320 80 I-302 320 90 I-305 320 90 I-306 320 90 I-307 320 100 I-308 320 100 I-309 320 90 I-311 320 90 I-312 320 90 I-313 320 90 I-315 320 90 I-316 320 100 I-317 320 100 I-319 320 90 I-32 320 90 I-320 320 80 I-321 320 100 I-322 320 80 I-323 320 100 I-324 320 90 I-325 320 100 I-327 320 80 I-33 320 90 I-330 320 90 I-331 320 100 I-332 320 90 I-333 320 90 I-334 320 100 I-336 320 90 I-337 320 90 I-338 320 80 I-339 320 100 I-34 320 90 I-341 320 100 I-342 320 100 I-343 320 100 I-347 320 80 I-348 320 90 I-35 320 100 I-350 320 90 I-351 320 80 I-352 320 90 I-354 320 90 I-359 320 90 I-36 320 100 I-360 320 90 I-369 320 90 I-37 320 100 I-370 320 100 I-373 320 90 I-374 320 90 I-375 320 100 I-376 320 80 I-377 320 90 I-38 320 100 I-388 320 90 I-39 320 100 I-41 320 80 I-42 320 100 I-43 320 80 I-44 320 90 I-46 320 90 I-48 320 100 I-51 320 90 I-52 320 90 I-53 320 90 I-54 320 100 I-56 320 100 I-64 320 90 I-65 320 90 I-66 320 90 I-69 320 90 I-73 320 90 I-74 320 90 I-75 320 90 I-76 320 90 I-77 320 90 I-79 320 90 I-80 320 90 I-81 320 90 I-82 320 90 I-83 320 100 I-84 320 90 I-85 320 100 I-86 320 100 I-87 320 90 I-88 320 90 I-90 320 90 I-91 320 90 I-93 320 100 I-94 320 100 I-95 320 80 I-96 320 100 I-97 320 80 I-98 320 90 I-99 320 90 III-22 320 100 III-24 320 100
TABLE-US-00021 TABLE A9a Pre-emergence action at 80 g/ha against PHBPU in % Example number Dosage [g/ha] PHBPU I-10 80 90 I-149 80 80 I-151 80 80 I-154 80 80 I-155 80 90 I-159 80 80 I-160 80 80 I-163 80 90 I-164 80 80 I-167 80 90 I-171 80 80 I-174 80 90 I-175 80 80 I-180 80 90 I-184 80 80 I-185 80 80 I-187 80 90 I-188 80 80 I-189 80 90 I-190 80 90 I-191 80 80 I-192 80 90 I-193 80 80 I-194 80 90 I-196 80 90 I-198 80 80 I-199 80 80 I-204 80 90 I-207 80 90 I-208 80 90 I-210 80 90 I-211 80 90 I-212 80 90 I-216 80 90 I-218 80 90 I-221 80 90 I-231 80 90 I-308 80 90 I-315 80 90 I-317 80 90 I-321 80 80 I-337 80 80 I-342 80 80 I-343 80 80 I-360 80 80 I-375 80 80 I-388 80 90 I-64 80 90 I-74 80 90 I-75 80 90 I-77 80 80 I-79 80 90 I-81 80 90 I-83 80 80 I-84 80 90 I-85 80 90 I-96 80 90
TABLE-US-00022 TABLE A9b Pre-emergence action at 320 g/ha against PHBPU in % Example number Dosage [g/ha] PHBPU I-02 320 90 I-03 320 90 I-07 320 90 I-08 320 80 I-10 320 90 I-100 320 90 I-102 320 80 I-103 320 80 I-116 320 90 I-118 320 90 I-122 320 90 I-125 320 90 I-148 320 90 I-149 320 90 I-15 320 80 I-151 320 80 I-153 320 80 I-154 320 90 I-155 320 90 I-156 320 80 I-157 320 90 I-159 320 90 I-16 320 80 I-160 320 90 I-162 320 90 I-163 320 90 I-164 320 90 I-167 320 90 I-17 320 90 I-171 320 90 I-174 320 90 I-175 320 90 I-18 320 90 I-180 320 90 I-184 320 90 I-185 320 90 I-186 320 90 I-187 320 90 I-188 320 90 I-189 320 90 I-19 320 90 I-190 320 90 I-191 320 90 I-192 320 90 I-193 320 90 I-194 320 90 I-195 320 90 I-196 320 90 I-198 320 90 I-199 320 90 I-20 320 90 I-202 320 90 I-204 320 90 I-206 320 80 I-207 320 90 I-208 320 90 I-210 320 90 I-211 320 90 I-212 320 90 I-216 320 90 I-217 320 90 I-218 320 90 I-221 320 90 I-223 320 80 I-23 320 90 I-230 320 90 I-231 320 90 I-247 320 80 I-276 320 80 I-277 320 80 I-278 320 80 I-279 320 100 I-291 320 80 I-293 320 80 I-296 320 90 I-30 320 90 I-300 320 80 I-307 320 90 I-308 320 90 I-313 320 80 I-315 320 90 I-316 320 90 I-317 320 90 I-319 320 90 I-32 320 80 I-321 320 90 I-322 320 90 I-323 320 90 I-324 320 90 I-325 320 80 I-327 320 80 I-33 320 90 I-330 320 90 I-331 320 90 I-332 320 100 I-334 320 90 I-335 320 80 I-336 320 80 I-337 320 80 I-338 320 80 I-340 320 80 I-341 320 90 I-342 320 90 I-343 320 90 I-348 320 90 I-35 320 90 I-350 320 80 I-352 320 80 I-358 320 80 I-36 320 100 I-360 320 90 I-369 320 90 I-37 320 90 I-370 320 90 I-374 320 90 I-375 320 90 I-376 320 90 I-38 320 90 I-388 320 90 I-40 320 80 I-41 320 90 I-42 320 90 I-43 320 80 I-51 320 90 I-52 320 90 I-56 320 90 I-64 320 90 I-73 320 90 I-74 320 90 I-75 320 90 I-76 320 90 I-77 320 90 I-79 320 90 I-80 320 90 I-81 320 100 I-83 320 90 I-84 320 90 I-85 320 100 I-86 320 90 I-87 320 90 I-88 320 80 I-90 320 90 I-93 320 80 I-96 320 90 I-97 320 90 I-98 320 90 III-24 320 100
TABLE-US-00023 TABLE A10a Pre-emergence action at 80 g/ha against POLCO in % Example number Dosage [g/ha] POLCO I-02 80 80 I-03 80 90 I-05 80 90 I-07 80 90 I-08 80 80 I-10 80 100 I-11 80 90 I-111 80 80 I-118 80 80 I-119 80 80 I-148 80 80 I-149 80 80 I-15 80 90 I-155 80 90 I-159 80 90 I-16 80 90 I-163 80 80 I-167 80 90 I-17 80 90 I-171 80 90 I-174 80 90 I-175 80 90 I-18 80 100 I-180 80 90 I-183 80 80 I-184 80 90 I-185 80 80 I-187 80 90 I-188 80 90 I-189 80 100 I-19 80 90 I-190 80 90 I-191 80 80 I-192 80 90 I-193 80 80 I-194 80 80 I-195 80 90 I-196 80 90 I-198 80 90 I-199 80 80 I-20 80 90 I-204 80 90 I-206 80 80 I-207 80 90 I-208 80 90 I-210 80 90 I-211 80 90 I-212 80 90 I-216 80 90 I-218 80 90 I-221 80 80 I-230 80 80 I-24 80 90 I-25 80 80 I-27 80 90 I-28 80 80 I-291 80 80 I-296 80 80 I-30 80 80 I-307 80 90 I-308 80 100 I-311 80 80 I-313 80 80 I-315 80 80 I-316 80 100 I-317 80 100 I-32 80 90 I-321 80 90 I-322 80 80 I-324 80 90 I-33 80 90 I-331 80 100 I-332 80 80 I-333 80 90 I-336 80 80 I-337 80 80 I-338 80 100 I-339 80 90 I-34 80 80 I-340 80 80 I-341 80 90 I-342 80 90 I-343 80 90 I-350 80 90 I-351 80 80 I-352 80 80 I-358 80 80 I-36 80 80 I-37 80 80 I-370 80 80 I-374 80 80 I-375 80 90 I-38 80 90 I-388 80 90 I-41 80 80 I-44 80 90 I-45 80 90 I-47 80 80 I-48 80 90 I-51 80 80 I-56 80 80 I-59 80 80 I-66 80 90 I-73 80 80 I-76 80 80 I-79 80 90 I-81 80 90 I-83 80 80 I-87 80 80 I-88 80 80 I-93 80 90 I-94 80 90 I-96 80 90
TABLE-US-00024 TABLE A10b Pre-emergence action at 320 g/ha against POLCO in % Example number Dosage [g/ha] POLCO I-01 320 90 I-02 320 80 I-03 320 100 I-04 320 100 I-05 320 90 I-07 320 100 I-08 320 100 I-10 320 100 I-100 320 90 I-102 320 90 I-107 320 80 I-11 320 90 I-111 320 100 I-116 320 90 I-118 320 90 I-119 320 90 I-121 320 100 I-122 320 80 I-125 320 90 I-126 320 90 I-13 320 100 I-147 320 90 I-148 320 90 I-149 320 90 I-15 320 100 I-151 320 90 I-154 320 90 I-155 320 90 I-157 320 90 I-159 320 90 I-16 320 90 I-160 320 90 I-162 320 100 I-163 320 80 I-164 320 100 I-167 320 90 I-17 320 100 I-171 320 90 I-174 320 100 I-175 320 90 I-18 320 100 I-180 320 100 I-183 320 90 I-184 320 90 I-185 320 90 I-186 320 80 I-187 320 90 I-188 320 90 I-189 320 100 I-19 320 100 I-190 320 90 I-191 320 90 I-192 320 100 I-193 320 100 I-194 320 100 I-195 320 100 I-196 320 90 I-198 320 90 I-199 320 90 I-20 320 100 I-202 320 90 I-204 320 90 I-205 320 80 I-206 320 80 I-207 320 100 I-208 320 90 I-210 320 100 I-211 320 90 I-212 320 90 I-216 320 90 I-217 320 80 I-218 320 90 I-221 320 90 I-223 320 80 I-225 320 90 I-229 320 90 I-23 320 90 I-230 320 90 I-237 320 80 I-238 320 80 I-24 320 90 I-242 320 80 I-244 320 80 I-247 320 90 I-25 320 90 I-26 320 90 I-27 320 100 I-276 320 80 I-279 320 80 I-28 320 90 I-29 320 90 I-291 320 90 I-293 320 80 I-296 320 90 I-30 320 90 I-307 320 100 I-308 320 100 I-309 320 80 I-31 320 80 I-310 320 90 I-311 320 90 I-313 320 80 I-315 320 90 I-316 320 100 I-317 320 100 I-319 320 90 I-32 320 90 I-320 320 90 I-321 320 100 I-322 320 90 I-323 320 100 I-324 320 100 I-325 320 90 I-327 320 90 I-33 320 100 I-330 320 90 I-331 320 100 I-332 320 80 I-333 320 90 I-334 320 90 I-335 320 90 I-336 320 90 I-337 320 90 I-338 320 100 I-339 320 100 I-34 320 90 I-340 320 90 I-341 320 100 I-342 320 100 I-343 320 100 I-347 320 80 I-349 320 80 I-35 320 90 I-350 320 90 I-351 320 80 I-352 320 90 I-354 320 80 I-358 320 90 I-359 320 80 I-36 320 90 I-360 320 100 I-362 320 80 I-369 320 90 I-37 320 90 I-370 320 100 I-373 320 90 I-374 320 90 I-375 320 90 I-378 320 80 I-38 320 100 I-381 320 80 I-388 320 90 I-39 320 90 I-40 320 80 I-41 320 90 I-42 320 90 I-43 320 80 I-44 320 90 I-46 320 80 I-47 320 90 I-48 320 90 I-51 320 90 I-52 320 90 I-53 320 90 I-54 320 90 I-56 320 90 I-58 320 90 I-59 320 90 I-64 320 90 I-65 320 90 I-66 320 90 I-73 320 90 I-74 320 100 I-75 320 90 I-76 320 90 I-77 320 90 I-79 320 90 I-80 320 90 I-81 320 90 I-83 320 90 I-84 320 90 I-85 320 100 I-86 320 100 I-87 320 90 I-88 320 90 I-90 320 90 I-93 320 90 I-94 320 90 I-95 320 90 I-96 320 90 I-97 320 90 I-98 320 90 I-99 320 90 III-22 320 100 III-24 320 100
TABLE-US-00025 TABLE A11a Pre-emergence action at 80 g/ha against SETVI in % Example number Dosage [g/ha] SETVI I-02 80 100 I-05 80 100 I-08 80 90 I-10 80 100 I-100 80 90 I-101 80 90 I-102 80 90 I-11 80 90 I-111 80 90 I-116 80 90 I-118 80 90 I-122 80 100 I-148 80 90 I-149 80 100 I-15 80 100 I-151 80 90 I-154 80 90 I-155 80 80 I-159 80 90 I-16 80 90 I-163 80 80 I-164 80 100 I-167 80 100 I-17 80 100 I-171 80 100 I-174 80 90 I-175 80 90 I-18 80 100 I-180 80 100 I-184 80 100 I-185 80 80 I-187 80 100 I-188 80 100 I-189 80 100 I-19 80 100 I-190 80 90 I-191 80 80 I-192 80 90 I-193 80 100 I-194 80 90 I-195 80 100 I-196 80 90 I-198 80 100 I-199 80 90 I-204 80 90 I-207 80 80 I-208 80 90 I-210 80 90 I-211 80 90 I-212 80 100 I-216 80 80 I-218 80 90 I-221 80 90 I-231 80 90 I-29 80 90 I-291 80 90 I-296 80 90 I-298 80 100 I-30 80 90 I-307 80 100 I-313 80 100 I-316 80 100 I-317 80 80 I-32 80 100 I-322 80 90 I-33 80 90 I-334 80 90 I-337 80 90 I-338 80 100 I-339 80 100 I-34 80 90 I-341 80 80 I-342 80 90 I-343 80 100 I-348 80 80 I-35 80 100 I-350 80 100 I-359 80 90 I-36 80 100 I-360 80 90 I-37 80 100 I-370 80 100 I-375 80 90 I-38 80 100 I-388 80 90 I-39 80 100 I-40 80 100 I-41 80 90 I-42 80 100 I-43 80 100 I-44 80 90 I-46 80 90 I-48 80 100 I-51 80 90 I-53 80 90 I-59 80 90 I-64 80 90 I-66 80 100 I-73 80 90 I-74 80 90 I-76 80 80 I-79 80 100 I-80 80 90 I-81 80 90 I-83 80 90 I-85 80 100 I-86 80 100 I-87 80 90 I-90 80 90 I-91 80 100 I-96 80 100 I-97 80 80 III-22 80 100 III-24 80 100
TABLE-US-00026 TABLE A11b Pre-emergence action at 320 g/ha against SETVI in % Example number Dosage [g/ha] SETVI I-01 320 100 I-02 320 100 I-03 320 100 I-04 320 100 I-05 320 100 I-07 320 100 I-08 320 100 I-10 320 100 I-100 320 100 I-101 320 100 I-102 320 100 I-103 320 90 I-107 320 100 I-11 320 100 I-111 320 100 I-116 320 100 I-118 320 100 I-119 320 100 I-120 320 100 I-121 320 100 I-122 320 100 I-125 320 90 I-126 320 90 I-13 320 90 I-148 320 100 I-149 320 100 I-15 320 100 I-151 320 100 I-152 320 90 I-153 320 90 I-154 320 100 I-155 320 100 I-156 320 90 I-159 320 100 I-16 320 100 I-163 320 100 I-164 320 100 I-167 320 100 I-17 320 100 I-171 320 100 I-174 320 100 I-175 320 100 I-18 320 100 I-180 320 100 I-183 320 90 I-184 320 100 I-185 320 100 I-186 320 80 I-187 320 100 I-188 320 100 I-189 320 100 I-19 320 100 I-190 320 100 I-191 320 100 I-192 320 100 I-193 320 100 I-194 320 100 I-195 320 100 I-196 320 100 I-198 320 100 I-199 320 100 I-20 320 100 I-202 320 90 I-204 320 100 I-207 320 100 I-208 320 100 I-210 320 100 I-211 320 100 I-212 320 100 I-216 320 100 I-217 320 90 I-218 320 100 I-221 320 100 I-225 320 80 I-229 320 90 I-23 320 100 I-230 320 100 I-231 320 90 I-24 320 90 I-247 320 100 I-25 320 100 I-26 320 100 I-27 320 100 I-272 320 90 I-276 320 90 I-277 320 80 I-278 320 100 I-279 320 90 I-28 320 100 I-29 320 100 I-291 320 90 I-296 320 100 I-298 320 100 I-30 320 100 I-300 320 90 I-302 320 100 I-305 320 90 I-306 320 80 I-307 320 100 I-308 320 100 I-309 320 90 I-31 320 90 I-311 320 100 I-312 320 90 I-313 320 100 I-315 320 100 I-316 320 100 I-317 320 90 I-319 320 100 I-32 320 100 I-320 320 90 I-321 320 100 I-322 320 100 I-323 320 100 I-324 320 100 I-327 320 100 I-33 320 100 I-330 320 100 I-331 320 90 I-332 320 100 I-333 320 90 I-334 320 90 I-336 320 100 I-337 320 100 I-338 320 100 I-339 320 100 I-34 320 100 I-341 320 100 I-342 320 100 I-343 320 100 I-347 320 80 I-348 320 100 I-35 320 100 I-350 320 100 I-351 320 100 I-352 320 90 I-354 320 90 I-358 320 100 I-359 320 100 I-36 320 100 I-360 320 100 I-362 320 80 I-369 320 90 I-37 320 100 I-370 320 100 I-373 320 80 I-374 320 100 I-375 320 100 I-376 320 100 I-377 320 90 I-38 320 100 I-388 320 100 I-39 320 100 I-40 320 100 I-41 320 100 I-42 320 100 I-43 320 100 I-44 320 100 I-46 320 100 I-47 320 100 I-48 320 100 I-51 320 100 I-52 320 100 I-53 320 100 I-54 320 100 I-56 320 100 I-59 320 100 I-60 320 80 I-64 320 100 I-65 320 90 I-66 320 100 I-69 320 100 I-70 320 90 I-71 320 100 I-72 320 90 I-73 320 100 I-74 320 100 I-75 320 100 I-76 320 100 I-77 320 100 I-78 320 80 I-79 320 100 I-80 320 100 I-81 320 100 I-82 320 90 I-83 320 100 I-84 320 100 I-85 320 100 I-86 320 100 I-87 320 100 I-88 320 100 I-90 320 100 I-91 320 100 I-93 320 100 I-94 320 100 I-95 320 100 I-96 320 100 I-97 320 100 I-98 320 100 I-99 320 90 II-36 320 80 III-02 320 80 III-22 320 100 III-23 320 100 III-24 320 100 III-27 320 90
TABLE-US-00027 TABLE A12a Pre-emergence action at 80 g/ha against VERPE in % Example number Dosage [g/ha] VERPE I-03 80 90 I-05 80 100 I-10 80 80 I-110 80 100 I-116 80 90 I-148 80 90 I-162 80 90 I-164 80 90 I-167 80 100 I-171 80 100 I-174 80 100 I-175 80 100 I-18 80 90 I-180 80 100 I-184 80 90 I-185 80 80 I-186 80 90 I-187 80 90 I-188 80 100 I-189 80 90 I-190 80 80 I-191 80 100 I-193 80 80 I-196 80 90 I-198 80 90 I-199 80 90 I-202 80 80 I-208 80 90 I-212 80 80 I-218 80 90 I-225 80 80 I-231 80 80 I-24 80 80 I-27 80 80 I-296 80 90 I-307 80 90 I-308 80 100 I-311 80 80 I-313 80 80 I-317 80 80 I-319 80 80 I-32 80 80 I-331 80 100 I-332 80 80 I-336 80 80 I-337 80 90 I-34 80 90 I-342 80 90 I-350 80 90 I-369 80 90 I-37 80 80 I-370 80 90 I-375 80 100 I-376 80 80 I-388 80 90 I-41 80 90 I-51 80 100 I-52 80 80 I-76 80 100 I-79 80 80 I-83 80 90 I-84 80 90 I-85 80 100 I-87 80 80 I-88 80 80 I-96 80 90
TABLE-US-00028 TABLE A12b Pre-emergence action at 320 g/ha against VERPE in % Example number Dosage [g/ha] VERPE I-01 320 90 I-02 320 90 I-03 320 100 I-04 320 100 I-05 320 100 I-07 320 100 I-08 320 100 I-10 320 100 I-100 320 100 I-101 320 100 I-102 320 80 I-103 320 90 I-11 320 90 I-111 320 90 I-112 320 80 I-116 320 90 I-118 320 90 I-120 320 90 I-121 320 100 I-122 320 100 I-126 320 80 I-13 320 80 I-148 320 100 I-149 320 100 I-15 320 100 I-154 320 100 I-155 320 100 I-157 320 90 I-159 320 100 I-16 320 90 I-160 320 90 I-161 320 80 I-162 320 90 I-163 320 80 I-164 320 100 I-167 320 100 I-17 320 100 I-171 320 100 I-174 320 100 I-175 320 100 I-18 320 100 I-180 320 100 I-184 320 100 I-185 320 90 I-186 320 90 I-187 320 90 I-188 320 100 I-189 320 100 I-19 320 100 I-190 320 100 I-191 320 100 I-192 320 90 I-193 320 90 I-194 320 90 I-195 320 100 I-196 320 100 I-198 320 100 I-199 320 100 I-20 320 100 I-202 320 90 I-204 320 100 I-205 320 100 I-207 320 90 I-208 320 100 I-210 320 100 I-211 320 100 I-212 320 100 I-216 320 90 I-218 320 100 I-221 320 90 I-223 320 80 I-225 320 90 I-23 320 90 I-231 320 80 I-235 320 80 I-24 320 100 I-246 320 80 I-247 320 90 I-25 320 90 I-27 320 100 I-279 320 80 I-28 320 100 I-29 320 90 I-291 320 80 I-296 320 100 I-298 320 100 I-30 320 90 I-302 320 90 I-307 320 100 I-308 320 100 I-31 320 90 I-311 320 90 I-313 320 90 I-315 320 100 I-316 320 100 I-317 320 100 I-319 320 90 I-32 320 100 I-321 320 100 I-323 320 100 I-324 320 100 I-33 320 100 I-330 320 90 I-331 320 100 I-332 320 90 I-333 320 100 I-334 320 80 I-335 320 80 I-336 320 90 I-337 320 90 I-338 320 100 I-339 320 100 I-34 320 100 I-340 320 100 I-341 320 100 I-342 320 100 I-343 320 100 I-348 320 90 I-35 320 100 I-350 320 100 I-351 320 80 I-352 320 80 I-36 320 100 I-360 320 90 I-369 320 90 I-37 320 100 I-370 320 100 I-374 320 100 I-375 320 100 I-376 320 80 I-377 320 80 I-38 320 100 I-388 320 100 I-39 320 100 I-40 320 100 I-41 320 100 I-42 320 100 I-43 320 90 I-44 320 80 I-46 320 100 I-47 320 90 I-48 320 100 I-51 320 100 I-52 320 100 I-53 320 100 I-54 320 100 I-56 320 100 I-59 320 90 I-64 320 90 I-65 320 80 I-66 320 100 I-70 320 80 I-73 320 100 I-74 320 100 I-75 320 90 I-76 320 100 I-77 320 90 I-79 320 100 I-80 320 90 I-81 320 90 I-83 320 100 I-84 320 100 I-85 320 100 I-86 320 90 I-87 320 90 I-88 320 90 I-90 320 90 I-91 320 100 I-93 320 100 I-94 320 90 I-95 320 100 I-96 320 90 I-97 320 90 I-98 320 100 I-99 320 90 II-36 320 80 III-22 320 100 III-24 320 100 III-28 320 80
TABLE-US-00029 TABLE A13a Pre-emergence action at 80 g/ha against VIOTR in % Example number Dosage [g/ha] VIOTR I-02 80 100 I-03 80 100 I-05 80 90 I-07 80 90 I-08 80 100 I-10 80 100 I-101 80 80 I-102 80 90 I-111 80 80 I-114 80 80 I-119 80 80 I-122 80 100 I-126 80 100 I-148 80 100 I-149 80 100 I-15 80 100 I-152 80 80 I-153 80 90 I-154 80 100 I-155 80 100 I-156 80 80 I-157 80 80 I-159 80 100 I-16 80 100 I-160 80 90 I-162 80 80 I-163 80 90 I-164 80 100 I-167 80 100 I-17 80 100 I-171 80 100 I-174 80 100 I-175 80 100 I-18 80 100 I-180 80 100 I-183 80 80 I-184 80 100 I-185 80 100 I-186 80 80 I-187 80 100 I-188 80 100 I-189 80 100 I-19 80 100 I-190 80 100 I-191 80 100 I-192 80 80 I-193 80 100 I-195 80 80 I-196 80 90 I-198 80 90 I-199 80 100 I-20 80 100 I-202 80 90 I-204 80 100 I-206 80 90 I-207 80 100 I-208 80 100 I-210 80 90 I-211 80 90 I-212 80 100 I-216 80 100 I-218 80 100 I-221 80 90 I-223 80 90 I-225 80 90 I-23 80 90 I-230 80 80 I-231 80 100 I-24 80 90 I-25 80 100 I-26 80 100 I-27 80 100 I-28 80 100 I-29 80 90 I-291 80 90 I-293 80 80 I-296 80 90 I-298 80 100 I-30 80 90 I-307 80 100 I-308 80 100 I-310 80 90 I-311 80 90 I-315 80 90 I-316 80 100 I-317 80 100 I-319 80 100 I-32 80 100 I-321 80 90 I-322 80 80 I-323 80 100 I-324 80 100 I-325 80 90 I-327 80 100 I-33 80 100 I-330 80 90 I-331 80 100 I-332 80 90 I-333 80 100 I-336 80 90 I-337 80 80 I-338 80 100 I-339 80 100 I-34 80 100 I-340 80 100 I-341 80 100 I-342 80 100 I-343 80 100 I-347 80 90 I-348 80 80 I-35 80 100 I-350 80 100 I-358 80 80 I-36 80 100 I-369 80 80 I-37 80 100 I-374 80 90 I-375 80 100 I-38 80 100 I-381 80 80 I-388 80 100 I-39 80 100 I-40 80 90 I-41 80 100 I-42 80 100 I-43 80 100 I-44 80 100 I-45 80 90 I-46 80 90 I-47 80 100 I-48 80 100 I-51 80 100 I-52 80 100 I-53 80 90 I-54 80 100 I-56 80 100 I-59 80 90 I-66 80 90 I-73 80 100 I-74 80 90 I-76 80 100 I-77 80 90 I-79 80 100 I-81 80 80 I-83 80 100 I-84 80 90 I-85 80 100 I-86 80 80 I-91 80 90 I-94 80 100 I-95 80 100 II-36 80 80 III-22 80 90 III-24 80 100
TABLE-US-00030 TABLE A13b Pre-emergence action at 320 g/ha against VIOTR in % Example number Dosage [g/ha] VIOTR I-01 320 90 I-02 320 100 I-03 320 100 I-04 320 100 I-05 320 100 I-07 320 100 I-08 320 100 I-10 320 100 I-100 320 90 I-101 320 100 I-102 320 100 I-103 320 90 I-107 320 100 I-11 320 100 I-111 320 100 I-114 320 90 I-116 320 90 I-118 320 100 I-119 320 90 I-120 320 80 I-121 320 100 I-122 320 100 I-125 320 90 I-126 320 100 I-13 320 90 I-147 320 90 I-148 320 100 I-149 320 100 I-15 320 100 I-151 320 100 I-152 320 90 I-153 320 100 I-154 320 100 I-155 320 100 I-156 320 90 I-157 320 100 I-159 320 100 I-16 320 100 I-160 320 100 I-161 320 90 I-162 320 100 I-163 320 100 I-164 320 100 I-167 320 100 I-17 320 100 I-171 320 100 I-174 320 100 I-175 320 100 I-18 320 100 I-180 320 100 I-183 320 100 I-184 320 100 I-185 320 100 I-186 320 90 I-187 320 100 I-188 320 100 I-189 320 100 I-19 320 100 I-190 320 100 I-191 320 100 I-192 320 100 I-193 320 100 I-194 320 100 I-195 320 100 I-196 320 100 I-198 320 100 I-199 320 100 I-20 320 100 I-200 320 100 I-202 320 100 I-204 320 100 I-205 320 100 I-206 320 100 I-207 320 100 I-208 320 100 I-210 320 100 I-211 320 100 I-212 320 100 I-216 320 100 I-217 320 90 I-218 320 100 I-221 320 90 I-223 320 100 I-225 320 100 I-229 320 90 I-23 320 100 I-230 320 90 I-231 320 100 I-238 320 90 I-24 320 100 I-240 320 90 I-242 320 100 I-244 320 90 I-245 320 80 I-25 320 100 I-26 320 100 I-27 320 100 I-272 320 90 I-28 320 100 I-29 320 100 I-291 320 100 I-293 320 100 I-296 320 100 I-298 320 100 I-30 320 100 I-300 320 90 I-302 320 90 I-306 320 80 I-307 320 100 I-308 320 100 I-31 320 90 I-310 320 100 I-311 320 100 I-313 320 90 I-315 320 100 I-316 320 100 I-317 320 100 I-319 320 100 I-32 320 100 I-320 320 100 I-321 320 100 I-322 320 100 I-323 320 100 I-324 320 100 I-325 320 100 I-327 320 100 I-33 320 100 I-330 320 100 I-331 320 100 I-332 320 100 I-333 320 100 I-334 320 90 I-335 320 100 I-336 320 100 I-337 320 100 I-338 320 100 I-339 320 100 I-34 320 100 I-340 320 100 I-341 320 100 I-342 320 100 I-343 320 100 I-346 320 80 I-347 320 100 I-348 320 90 I-349 320 80 I-35 320 100 I-350 320 100 I-358 320 100 I-359 320 100 I-36 320 100 I-360 320 100 I-362 320 100 I-369 320 100 I-37 320 100 I-370 320 100 I-374 320 100 I-375 320 100 I-378 320 90 I-38 320 100 I-381 320 90 I-388 320 100 I-39 320 100 I-40 320 100 I-41 320 100 I-42 320 100 I-43 320 100 I-44 320 100 I-46 320 100 I-47 320 100 I-48 320 100 I-51 320 100 I-52 320 100 I-53 320 100 I-54 320 100 I-56 320 100 I-58 320 80 I-59 320 90 I-60 320 80 I-64 320 90 I-65 320 100 I-66 320 100 I-69 320 90 I-70 320 90 I-72 320 90 I-73 320 100 I-74 320 100 I-75 320 100 I-76 320 100 I-77 320 100 I-78 320 80 I-79 320 100 I-80 320 90 I-81 320 100 I-83 320 100 I-84 320 100 I-85 320 100 I-86 320 100 I-87 320 80 I-88 320 90 I-90 320 90 I-91 320 100 I-93 320 100 I-94 320 100 I-95 320 100 I-96 320 90 I-97 320 100 I-98 320 100 I-99 320 90 II-36 320 100 III-08 320 90 III-09 320 80 III-22 320 100 III-24 320 100
[0563] Tables A14 to A18 below show the crop plant compatibilities of selected compounds of the general formula (I) according to Table 1 at an application rate corresponding to 320 g/ha or less, which were observed in trials by the experimental procedure mentioned above. The observed effects on selected crop plants are reported here in comparison to the untreated controls (values in %). The appendices a b and c give differentiation by dosage used with otherwise the same crop plants tested.
TABLE-US-00031 TABLE A14a Pre-emergence action at 20 g/ha against ZEAMX in % Example number Dosage [g/ha] ZEAMX I-01 20 0 I-02 20 0 I-11 20 10 I-13 20 10 I-16 20 10
TABLE-US-00032 TABLE A14b Pre-emergence action at 80 g/ha against ZEAMX in % Example number Dosage [g/ha] ZEAMX I-01 80 0 I-04 80 0 I-05 80 0 I-10 80 20 I-103 80 0 I-108 80 10 I-109 80 10 I-11 80 10 I-110 80 10 I-111 80 0 I-112 80 0 I-114 80 10 I-122 80 0 I-125 80 10 I-147 80 0 I-152 80 10 I-156 80 0 I-157 80 10 I-161 80 20 I-19 80 0 I-200 80 0 I-201 80 20 I-202 80 20 I-223 80 20 I-225 80 10 I-229 80 0 I-23 80 10 I-235 80 0 I-236 80 20 I-237 80 0 I-239 80 0 I-24 80 10 I-241 80 0 I-242 80 0 I-243 80 10 I-244 80 0 I-245 80 0 I-246 80 20 I-247 80 20 I-25 80 10 I-26 80 0 I-27 80 20 I-272 80 0 I-278 80 0 I-28 80 10 I-293 80 20 I-297 80 10 I-30 80 10 I-300 80 10 I-302 80 10 I-305 80 0 I-306 80 20 I-309 80 0 I-31 80 0 I-310 80 0 I-312 80 20 I-315 80 10 I-325 80 0 I-327 80 20 I-329 80 0 I-330 80 20 I-334 80 20 I-335 80 20 I-345 80 0 I-346 80 0 I-349 80 10 I-354 80 0 I-357 80 20 I-359 80 10 I-36 80 0 I-362 80 0 I-363 80 0 I-371 80 0 I-373 80 0 I-376 80 10 I-377 80 0 I-378 80 0 I-381 80 0 I-386 80 0 I-47 80 20 I-49 80 0 I-50 80 0 I-53 80 20 I-54 80 0 I-55 80 0 I-58 80 20 I-60 80 0 I-62 80 0 I-63 80 10 I-70 80 0 I-71 80 10 I-72 80 0 I-78 80 0 I-88 80 20 I-90 80 20 I-93 80 0 I-95 80 0 I-96 80 0 I-99 80 0 II-36 80 20 III-01 80 10 III-02 80 20 III-07 80 0 III-09 80 0 III-17 80 20 III-18 80 20 III-20 80 0 III-21 80 0 III-23 80 0 III-25 80 20 III-26 80 0 III-27 80 10 III-28 80 0 III-30 80 0
TABLE-US-00033 TABLE A14c Pre-emergence action at 320 g/ha against ZEAMX in % Example number Dosage [g/ha] ZEAMX I-108 320 10 I-109 320 10 I-112 320 10 I-114 320 20 I-156 320 20 I-161 320 20 I-200 320 0 I-239 320 20 I-309 320 10 I-325 320 0 I-329 320 10 I-345 320 10 I-346 320 0 I-349 320 20 I-363 320 0 I-371 320 10 I-373 320 0 I-377 320 0 I-386 320 0 I-49 320 0 I-50 320 0 I-55 320 0 I-63 320 10 I-70 320 0 I-72 320 0 I-78 320 0 I-95 320 0 III-01 320 20 III-07 320 10 III-09 320 0 III-17 320 20 III-18 320 20 III-20 320 0 III-21 320 20 III-23 320 0 III-26 320 0 III-27 320 20 III-28 320 10 III-30 320 10
TABLE-US-00034 TABLE A15a Pre-emergence action at 20 g/ha against TRZAS in % Example number Dosage [g/ha] TRZAS I-01 20 0 I-11 20 0 I-13 20 10 I-15 20 10 I-16 20 10 I-17 20 10
TABLE-US-00035 TABLE A15b Pre-emergence action at 80 g/ha against TRZAS in % Example number Dosage [g/ha] TRZAS I-01 80 0 I-03 80 10 I-04 80 0 I-108 80 0 I-109 80 0 I-112 80 0 I-114 80 20 I-119 80 20 I-125 80 10 I-126 80 20 I-13 80 20 I-147 80 0 I-150 80 0 I-151 80 10 I-16 80 20 I-160 80 20 I-161 80 0 I-183 80 0 I-200 80 0 I-201 80 0 I-206 80 0 I-217 80 0 I-236 80 20 I-239 80 20 I-26 80 0 I-276 80 0 I-277 80 0 I-278 80 0 I-279 80 20 I-312 80 10 I-345 80 10 I-346 80 0 I-349 80 10 I-352 80 10 I-357 80 10 I-359 80 0 I-376 80 10 I-386 80 20 I-49 80 0 I-50 80 10 I-55 80 0 I-60 80 0 I-62 80 0 I-63 80 0 I-65 80 20 I-69 80 0 I-70 80 10 I-71 80 10 I-72 80 10 I-78 80 0 I-82 80 0 III-01 80 0 III-02 80 0 III-07 80 0 III-08 80 0 III-09 80 0 III-17 80 0 III-18 80 0 III-19 80 20 III-20 80 0 III-21 80 20 III-23 80 0 III-26 80 0 III-27 80 20 III-28 80 0
TABLE-US-00036 TABLE A15c Pre-emergence action at 320 g/ha against TRZAS in % Example number Dosage [g/ha] TRZAS I-108 320 10 I-109 320 10 I-112 320 10 I-147 320 20 I-150 320 0 I-161 320 20 I-200 320 10 I-276 320 0 I-312 320 20 I-357 320 10 I-49 320 0 I-50 320 10 I-55 320 0 I-62 320 0 I-63 320 0 I-82 320 20 III-02 320 20 III-07 320 0 III-08 320 0 III-09 320 0 III-18 320 20 III-20 320 0 III-26 320 20
TABLE-US-00037 TABLE A16a Pre-emergence action at 20 g/ha against ORYSA in % Example number Dosage [g/ha] ORYSA I-02 20 0 I-11 20 0 I-13 20 0 I-16 20 20 I-17 20 0
TABLE-US-00038 TABLE A16b Pre-emergence action at 80 g/ha against ORYSA in % Example number Dosage [g/ha] ORYSA I-103 80 0 I-107 80 10 I-108 80 0 I-109 80 10 I-11 80 20 I-110 80 10 I-111 80 0 I-112 80 0 I-114 80 0 I-119 80 10 I-120 80 0 I-121 80 0 I-122 80 0 I-125 80 10 I-126 80 20 I-13 80 10 I-150 80 20 I-152 80 20 I-156 80 0 I-161 80 0 I-193 80 20 I-200 80 20 I-201 80 0 I-223 80 10 I-225 80 20 I-23 80 10 I-246 80 0 I-26 80 0 I-272 80 10 I-278 80 0 I-279 80 0 I-28 80 0 I-297 80 10 I-302 80 20 I-31 80 0 I-310 80 0 I-312 80 20 I-329 80 0 I-335 80 0 I-336 80 20 I-337 80 20 I-345 80 10 I-35 80 20 I-351 80 20 I-352 80 20 I-357 80 20 I-360 80 10 I-362 80 20 I-369 80 20 I-371 80 0 I-376 80 20 I-378 80 0 I-381 80 20 I-386 80 0 I-49 80 10 I-55 80 0 I-58 80 0 I-59 80 20 I-60 80 0 I-62 80 0 I-63 80 0 I-64 80 20 I-69 80 0 I-70 80 0 I-71 80 10 I-72 80 0 I-78 80 0 I-82 80 0 I-90 80 10 I-95 80 0 I-96 80 20 I-97 80 10 I-99 80 0 II-36 80 0 III-01 80 0 III-02 80 0 III-07 80 0 III-08 80 0 III-09 80 0 III-17 80 0 III-18 80 0 III-19 80 0 III-20 80 0 III-21 80 0 III-23 80 0 III-25 80 0 III-26 80 0 III-27 80 0 III-28 80 0 III-30 80 10
TABLE-US-00039 TABLE A16c Pre-emergence action at 320 g/ha against ORYSA in % Example number Dosage [g/ha] ORYSA I-108 320 10 I-109 320 10 I-112 320 10 I-114 320 0 I-120 320 10 I-161 320 0 I-200 320 20 I-201 320 20 I-297 320 20 I-31 320 0 I-329 320 20 I-345 320 20 I-346 320 0 I-357 320 20 I-371 320 0 I-386 320 20 I-49 320 20 I-55 320 0 I-62 320 0 I-63 320 0 I-70 320 10 I-72 320 20 I-78 320 0 I-95 320 0 III-01 320 0 III-02 320 0 III-07 320 20 III-08 320 0 III-09 320 0 III-17 320 10 III-18 320 0 III-19 320 20 III-20 320 10 III-21 320 0 III-25 320 0 III-26 320 0 III-27 320 20 III-28 320 10 III-30 320 20
TABLE-US-00040 TABLE A17a Pre-emergence action at 20 g/ha against GLXMA in % Example number Dosage [g/ha] GLXMA I-01 20 0 I-11 20 10 I-13 20 10 I-17 20 10
TABLE-US-00041 TABLE A17b Pre-emergence action at 80 g/ha against GLXMA in % Example number Dosage [g/ha] GLXMA I-01 80 20 I-108 80 0 I-109 80 20 I-13 80 10 I-147 80 0 I-150 80 0 I-151 80 10 I-161 80 0 I-183 80 0 I-200 80 20 I-201 80 0 I-206 80 10 I-230 80 20 I-238 80 20 I-240 80 20 I-242 80 0 I-244 80 0 I-298 80 20 I-306 80 0 I-309 80 0 I-312 80 20 I-329 80 0 I-345 80 0 I-346 80 0 I-347 80 10 I-349 80 0 I-363 80 0 I-371 80 20 I-386 80 0 I-55 80 0 I-58 80 0 I-60 80 20 I-65 80 20 I-70 80 10 I-71 80 20 I-72 80 0 I-77 80 0 I-78 80 0 I-82 80 0 II-36 80 0 III-09 80 20 III-17 80 0 III-18 80 0 III-19 80 0 III-21 80 0 III-23 80 0 III-25 80 0 III-26 80 0 III-27 80 0 III-30 80 20
TABLE-US-00042 TABLE A17c Pre-emergence action at 320 g/ha against GLXMA in % Example number Dosage [g/ha] GLXMA I-69 320 20 I-55 320 0 I-108 320 0 I-109 320 20 I-112 320 20 III-21 320 0 III-20 320 20 I-200 320 20 I-151 320 20 I-147 320 0 I-150 320 0 III-30 320 20 I-386 320 0 I-346 320 20 I-363 320 0 I-349 320 10
TABLE-US-00043 TABLE A18a Pre-emergence action at 20 g/ha against BRSNW in % Example number Dosage [g/ha] BRSNW I-01 20 0 I-11 20 10 I-13 20 10 I-15 20 10 I-16 20 10
TABLE-US-00044 TABLE A18b Pre-emergence action at 80 g/ha against BRSNW in % Example number Dosage [g/ha] BRSNW I-101 80 10 I-108 80 10 I-109 80 10 I-11 80 20 I-110 80 20 I-112 80 10 I-125 80 20 I-13 80 10 I-147 80 0 I-150 80 0 I-161 80 10 I-200 80 0 I-24 80 20 I-242 80 20 I-245 80 0 I-25 80 10 I-26 80 20 I-272 80 0 I-297 80 20 I-300 80 20 I-312 80 20 I-319 80 20 I-325 80 20 I-329 80 0 I-335 80 0 I-345 80 20 I-346 80 0 I-351 80 20 I-363 80 0 I-371 80 0 I-377 80 0 I-378 80 0 I-381 80 0 I-386 80 0 I-49 80 10 I-50 80 0 I-55 80 0 I-58 80 0 I-62 80 0 I-63 80 0 I-65 80 20 I-69 80 20 I-70 80 20 I-71 80 0 I-72 80 10 I-82 80 20 II-36 80 0 III-01 80 0 III-07 80 0 III-20 80 0 III-21 80 20 III-23 80 0 III-26 80 0
TABLE-US-00045 TABLE A18c Pre-emergence action at 320 g/ha against BRSNW in % Example number Dosage [g/ha] BRSNW I-108 320 20 I-109 320 10 I-112 320 10 I-13 320 20 I-161 320 10 I-200 320 0 I-335 320 0 I-346 320 20 I-363 320 20 I-371 320 20 I-386 320 0 I-50 320 20 I-55 320 0 I-63 320 20 I-82 320 20 III-21 320 20 III-23 320 0
[0564] As the results from Tables A1 to A18 show, inventive compounds of the general formula (I) in the case of pre-emergence treatment have good herbicidal efficacy against harmful plants, for example Abutilon theophrasti (ABUTH), Alopecurus myosuroides (ALOMY), Amaranthus retroflexus (AMARE), Avena fatua (AVEFA), Digitaria sanguinalis (DIGSA), Echinochloa crus-galli (ECHCG), Lolium rigidum (LOLRI), Matricaria inodora (MATIN), Pharbitis purpurea (PHBPU), Polygonum convolvulus (POLCO), Setaria viridis (SETVI), Verconica persica (VERPE) and Viola tricolor (VIOTR) at an application rate of 320 g of active substance or less per hectare, and good crop plant compatibility in the case of organisms such as Oryza sativa (ORYSA), Zea mays (ZEAMX), Brassica napus (BRSNW), Glycine max (GLXMA) and Triticum aestivum (TRZAS) at an application rate of 320 g or less per hectare.
[0565] The compounds of the invention are therefore suitable for control of unwanted plant growth by the pre-emergence method.
[0566] B. Post-Emergence Herbicidal Action and Crop Plant Compatibility
[0567] Seeds of monocotyledonous and dicotyledonous weeds and crop plants are placed in sandy loam in plastic or organic planting pots, covered with soil and cultivated in a greenhouse under controlled growth conditions. 2 to 3 weeks after sowing, the test plants are treated at the one-leaf stage. The compounds of the invention, formulated in the form of wettable powders (WP) or as emulsion concentrates (EC), are then sprayed onto the green parts of the plants as aqueous suspension or emulsion with addition of 0.5% additive at a water application rate of 600 l/ha (converted). After the test plants have been kept in the greenhouse under optimum growth conditions for about 3 weeks, the activity of the preparations is rated visually in comparison to untreated controls. For example, 100% activity=the plants have died, 0% activity=like control plants.
[0568] Tables B1 to B13 below show the effects of selected compounds of the general formula (I) according to Table 1 on various harmful plants and at an application rate corresponding to 320 g/ha or lower, which were obtained by the experimental procedure mentioned above. The appendices a, b and c give differentiation by dosage used with otherwise the same harmful plants tested.
TABLE-US-00046 TABLE B1a Post-emergence action at 80 g/ha against ABUTH in % Example number Dosage [g/ha] ABUTH I-02 80 80 I-03 80 80 I-04 80 90 I-05 80 80 I-07 80 80 I-08 80 80 I-100 80 80 I-102 80 80 I-103 80 80 I-118 80 80 I-119 80 80 I-120 80 80 I-125 80 80 I-126 80 80 I-130 80 80 I-144 80 80 I-145 80 90 I-146 80 80 I-151 80 80 I-165 80 90 I-167 80 80 I-168 80 80 I-174 80 80 I-175 80 80 I-177 80 90 I-179 80 80 I-181 80 80 I-182 80 80 I-183 80 80 I-184 80 80 I-185 80 80 I-188 80 80 I-19 80 80 I-190 80 80 I-191 80 80 I-193 80 80 I-196 80 80 I-197 80 90 I-198 80 80 I-208 80 80 I-212 80 80 I-217 80 80 I-218 80 80 I-227 80 90 I-267 80 80 I-275 80 80 I-28 80 80 I-304 80 80 I-314 80 80 I-315 80 80 I-318 80 80 I-325 80 80 I-326 80 80 I-327 80 80 I-328 80 80 I-330 80 80 I-331 80 90 I-332 80 80 I-334 80 80 I-337 80 80 I-339 80 80 I-341 80 80 I-342 80 80 I-343 80 80 I-344 80 80 I-35 80 90 I-36 80 80 I-366 80 80 I-37 80 80 I-374 80 80 I-375 80 90 I-38 80 80 I-380 80 80 I-39 80 90 I-42 80 90 I-45 80 80 I-48 80 90 I-54 80 80 I-56 80 80 I-59 80 80 I-64 80 90 I-73 80 80 I-74 80 80 I-75 80 80 I-76 80 90 I-77 80 80 I-78 80 80 I-79 80 80 I-81 80 80 I-83 80 90 I-84 80 80 I-85 80 90 I-86 80 90 I-88 80 80 I-95 80 80 I-96 80 90 I-97 80 90 III-22 80 90 III-24 80 90
TABLE-US-00047 TABLE B1b Post-emergence action at 320 g/ha against ABUTH in % Example number Dosage [g/ha] ABUTH I-01 320 80 I-02 320 80 I-03 320 90 I-04 320 90 I-05 320 80 I-07 320 90 I-08 320 90 I-10 320 80 I-130 320 90 I-133 320 80 I-137 320 80 I-138 320 80 I-139 320 80 I-140 320 80 I-144 320 90 I-145 320 90 I-146 320 90 I-151 320 80 I-152 320 80 I-157 320 80 I-159 320 80 I-165 320 90 I-167 320 80 I-168 320 80 I-171 320 90 I-172 320 80 I-174 320 80 I-175 320 80 I-176 320 80 I-177 320 90 I-179 320 80 I-18 320 80 I-181 320 80 I-182 320 80 I-183 320 80 I-184 320 90 I-185 320 80 I-186 320 80 I-187 320 80 I-188 320 80 I-190 320 80 I-191 320 80 I-192 320 80 I-193 320 80 I-194 320 80 I-195 320 90 I-196 320 80 I-197 320 90 I-198 320 80 I-199 320 80 I-202 320 80 I-207 320 80 I-208 320 90 I-210 320 80 I-212 320 80 I-216 320 80 I-217 320 90 I-218 320 80 I-223 320 80 I-225 320 80 I-227 320 90 I-249 320 80 I-26 320 90 I-260 320 80 I-261 320 80 I-267 320 90 I-268 320 80 I-27 320 90 I-273 320 80 I-274 320 80 I-275 320 80 I-28 320 90 I-285 320 80 I-287 320 90 I-289 320 80 I-291 320 80 I-294 320 80 I-296 320 80 I-304 320 90 I-307 320 90 I-309 320 80 I-311 320 80 I-312 320 80 I-314 320 80 I-315 320 80 I-318 320 80 I-319 320 80 I-320 320 80 I-325 320 90 I-326 320 80 I-327 320 90 I-328 320 80 I-330 320 80 I-331 320 90 I-332 320 80 I-333 320 80 I-334 320 80 I-336 320 80 I-337 320 80 I-339 320 90 I-340 320 80 I-341 320 90 I-342 320 90 I-343 320 90 I-344 320 80 I-348 320 80 I-350 320 90 I-358 320 80 I-359 320 80 I-360 320 80 I-366 320 90 I-369 320 80 I-373 320 80 I-375 320 90 I-376 320 80 I-378 320 80 I-380 320 90 I-388 320 80 I-41 320 80 I-42 320 90 I-48 320 90 I-66 320 80 I-69 320 80 I-85 320 90 I-86 320 90 I-88 320 80 I-94 320 80 I-95 320 80 I-96 320 90 II-38 320 80 II-39 320 80 II-40 320 80 II-41 320 80 II-43 320 80 II-44 320 80 II-45 320 80 III-07 320 80 III-22 320 90 III-23 320 80 III-24 320 90 III-29 320 80
TABLE-US-00048 TABLE B2a Post-emergence action at 80 g/ha against ALOMY in % Example number Dosage [g/ha] ALOMY I-01 80 100 I-02 80 80 I-05 80 90 I-07 80 90 I-08 80 100 I-10 80 100 I-100 80 100 I-101 80 90 I-102 80 90 I-107 80 90 I-11 80 90 I-110 80 80 I-114 80 90 I-116 80 90 I-118 80 100 I-119 80 90 I-120 80 100 I-121 80 80 I-125 80 90 I-13 80 90 I-139 80 90 I-144 80 90 I-145 80 80 I-148 80 80 I-149 80 80 I-15 80 90 I-151 80 80 I-16 80 90 I-164 80 100 I-166 80 90 I-167 80 90 I-17 80 90 I-171 80 90 I-172 80 90 I-174 80 90 I-175 80 90 I-18 80 90 I-180 80 90 I-181 80 80 I-184 80 80 I-188 80 80 I-189 80 80 I-19 80 100 I-190 80 80 I-191 80 80 I-192 80 90 I-193 80 90 I-194 80 90 I-195 80 80 I-196 80 80 I-197 80 90 I-198 80 80 I-20 80 100 I-204 80 90 I-211 80 80 I-212 80 90 I-221 80 80 I-227 80 80 I-23 80 90 I-24 80 90 I-25 80 90 I-252 80 80 I-27 80 80 I-275 80 80 I-28 80 100 I-285 80 90 I-289 80 80 I-29 80 100 I-291 80 80 I-293 80 90 I-296 80 80 I-299 80 80 I-30 80 90 I-300 80 80 I-302 80 80 I-307 80 100 I-308 80 100 I-311 80 80 I-313 80 90 I-314 80 90 I-315 80 80 I-316 80 100 I-317 80 100 I-318 80 90 I-319 80 90 I-32 80 90 I-321 80 90 I-323 80 100 I-325 80 80 I-326 80 90 I-328 80 90 I-33 80 90 I-330 80 80 I-331 80 100 I-332 80 80 I-333 80 90 I-336 80 90 I-337 80 90 I-339 80 90 I-34 80 90 I-340 80 90 I-341 80 80 I-342 80 100 I-343 80 90 I-344 80 90 I-348 80 80 I-35 80 90 I-358 80 90 I-36 80 90 I-360 80 90 I-369 80 80 I-37 80 90 I-370 80 100 I-374 80 100 I-375 80 100 I-38 80 100 I-39 80 100 I-40 80 100 I-41 80 90 I-42 80 100 I-43 80 90 I-44 80 80 I-45 80 90 I-46 80 90 I-48 80 100 I-51 80 90 I-52 80 90 I-53 80 90 I-54 80 90 I-56 80 90 I-59 80 90 I-64 80 100 I-66 80 100 I-71 80 90 I-72 80 90 I-73 80 100 I-74 80 100 I-75 80 90 I-76 80 100 I-77 80 90 I-79 80 80 I-81 80 90 I-83 80 100 I-84 80 80 I-86 80 100 I-87 80 80 I-88 80 80 I-90 80 90 I-91 80 90 I-93 80 100 I-94 80 80 I-96 80 90 I-97 80 90 I-98 80 90 I-99 80 90 II-42 80 80 III-22 80 100 III-24 80 100
TABLE-US-00049 TABLE B2b Post-emergence action at 320 g/ha against ALOMY in % Example number Dosage [g/ha] ALOMY I-01 320 100 I-02 320 100 I-03 320 100 I-05 320 100 I-07 320 100 I-08 320 100 I-10 320 100 I-11 320 90 I-111 320 100 I-13 320 90 I-130 320 90 I-133 320 90 I-134 320 90 I-136 320 90 I-137 320 80 I-139 320 90 I-140 320 100 I-141 320 90 I-144 320 90 I-145 320 90 I-146 320 90 I-148 320 90 I-149 320 90 I-15 320 90 I-151 320 80 I-152 320 80 I-153 320 80 I-155 320 80 I-156 320 80 I-16 320 90 I-163 320 80 I-164 320 100 I-165 320 100 I-166 320 90 I-167 320 90 I-17 320 90 I-171 320 90 I-172 320 90 I-174 320 90 I-175 320 90 I-176 320 90 I-177 320 100 I-179 320 90 I-18 320 100 I-180 320 90 I-181 320 90 I-182 320 80 I-184 320 90 I-185 320 80 I-187 320 90 I-188 320 90 I-189 320 90 I-190 320 100 I-191 320 90 I-192 320 90 I-193 320 100 I-194 320 90 I-195 320 90 I-196 320 90 I-197 320 90 I-198 320 80 I-199 320 90 I-20 320 100 I-204 320 90 I-206 320 80 I-207 320 90 I-208 320 80 I-210 320 90 I-211 320 90 I-212 320 90 I-218 320 90 I-221 320 80 I-223 320 80 I-225 320 90 I-227 320 90 I-237 320 80 I-238 320 80 I-240 320 80 I-242 320 80 I-244 320 80 I-245 320 80 I-247 320 80 I-251 320 80 I-252 320 90 I-26 320 90 I-260 320 90 I-264 320 90 I-266 320 90 I-267 320 90 I-27 320 100 I-272 320 90 I-274 320 90 I-275 320 100 I-28 320 100 I-285 320 90 I-287 320 90 I-288 320 90 I-289 320 90 I-290 320 90 I-291 320 80 I-293 320 90 I-294 320 90 I-296 320 90 I-298 320 90 I-299 320 90 I-300 320 90 I-302 320 90 I-304 320 90 I-305 320 100 I-306 320 100 I-307 320 100 I-308 320 100 I-310 320 90 I-311 320 90 I-312 320 90 I-313 320 90 I-314 320 90 I-315 320 90 I-316 320 100 I-317 320 100 I-318 320 90 I-319 320 90 I-320 320 100 I-321 320 100 I-322 320 80 I-323 320 100 I-324 320 100 I-325 320 100 I-326 320 90 I-327 320 100 I-328 320 90 I-330 320 90 I-331 320 100 I-332 320 90 I-333 320 90 I-334 320 90 I-335 320 100 I-336 320 90 I-337 320 90 I-338 320 90 I-339 320 100 I-340 320 100 I-341 320 100 I-342 320 100 I-343 320 100 I-344 320 90 I-347 320 80 I-348 320 90 I-350 320 90 I-354 320 90 I-358 320 90 I-359 320 90 I-360 320 90 I-362 320 90 I-366 320 90 I-369 320 100 I-370 320 100 I-375 320 100 I-376 320 80 I-380 320 90 I-382 320 90 I-383 320 90 I-388 320 80 I-41 320 90 I-42 320 100 I-48 320 100 I-58 320 90 I-66 320 100 I-69 320 90 I-80 320 90 I-85 320 100 I-86 320 100 I-87 320 90 I-88 320 90 I-94 320 100 I-95 320 100 I-96 320 90 II-38 320 100 II-39 320 90 II-40 320 90 II-41 320 90 II-42 320 90 II-43 320 100 II-44 320 100 II-45 320 90 II-46 320 80 III-08 320 80 III-22 320 100 III-23 320 100 III-24 320 100 III-29 320 90 III-30 320 80
TABLE-US-00050 TABLE B3a Post-emergence action at 80 g/ha against AMARE in % Example number Dosage [g/ha] AMARE I-02 80 80 I-03 80 80 I-04 80 90 I-05 80 90 I-07 80 90 I-08 80 80 I-100 80 90 I-102 80 80 I-103 80 80 I-107 80 80 I-111 80 80 I-116 80 90 I-118 80 90 I-119 80 90 I-120 80 80 I-122 80 90 I-126 80 80 I-130 80 80 I-139 80 80 I-141 80 80 I-144 80 90 I-145 80 80 I-146 80 90 I-150 80 80 I-151 80 90 I-152 80 80 I-153 80 90 I-156 80 80 I-167 80 80 I-171 80 80 I-174 80 80 I-175 80 80 I-177 80 90 I-179 80 90 I-181 80 80 I-182 80 80 I-183 80 90 I-184 80 80 I-19 80 80 I-191 80 80 I-192 80 80 I-193 80 80 I-194 80 80 I-196 80 80 I-197 80 90 I-198 80 80 I-199 80 80 I-20 80 90 I-204 80 80 I-217 80 90 I-218 80 80 I-221 80 80 I-227 80 90 I-229 80 80 I-235 80 80 I-247 80 80 I-26 80 80 I-267 80 80 I-27 80 90 I-28 80 90 I-287 80 80 I-291 80 80 I-302 80 80 I-304 80 80 I-305 80 80 I-306 80 80 I-307 80 80 I-309 80 90 I-310 80 80 I-313 80 80 I-314 80 90 I-315 80 80 I-318 80 90 I-320 80 80 I-321 80 80 I-322 80 80 I-324 80 90 I-326 80 90 I-327 80 90 I-328 80 90 I-330 80 80 I-331 80 80 I-332 80 80 I-334 80 80 I-335 80 80 I-338 80 80 I-339 80 90 I-340 80 80 I-341 80 80 I-342 80 90 I-343 80 80 I-344 80 90 I-35 80 100 I-350 80 90 I-351 80 80 I-354 80 80 I-36 80 80 I-37 80 90 I-370 80 80 I-373 80 80 I-374 80 80 I-375 80 80 I-377 80 80 I-40 80 80 I-41 80 80 I-42 80 90 I-43 80 80 I-44 80 80 I-45 80 80 I-46 80 90 I-48 80 80 I-51 80 90 I-53 80 90 I-54 80 80 I-56 80 80 I-59 80 90 I-60 80 80 I-64 80 90 I-66 80 80 I-70 80 90 I-71 80 90 I-72 80 80 I-73 80 90 I-74 80 80 I-75 80 80 I-76 80 80 I-77 80 80 I-78 80 80 I-79 80 90 I-80 80 80 I-81 80 90 I-83 80 90 I-84 80 90 I-85 80 90 I-87 80 80 I-88 80 80 I-90 80 80 I-91 80 90 I-93 80 80 I-94 80 90 I-95 80 80 I-96 80 80 I-97 80 90 I-98 80 80 I-99 80 80 III-17 80 80 III-18 80 80 III-19 80 80 III-22 80 90 III-23 80 90 III-27 80 80 III-28 80 80 III-30 80 80
TABLE-US-00051 TABLE B3b Post-emergence action at 320 g/ha against AMARE in % Example number Dosage [g/ha] AMARE I-01 320 80 I-02 320 80 I-03 320 90 I-04 320 90 I-05 320 90 I-07 320 90 I-08 320 90 I-111 320 90 I-130 320 90 I-137 320 80 I-139 320 90 I-140 320 90 I-141 320 90 I-144 320 90 I-145 320 80 I-146 320 90 I-147 320 90 I-150 320 80 I-151 320 100 I-152 320 80 I-153 320 90 I-156 320 90 I-16 320 80 I-162 320 80 I-165 320 80 I-167 320 80 I-171 320 80 I-172 320 80 I-174 320 80 I-175 320 80 I-177 320 90 I-179 320 90 I-180 320 90 I-181 320 90 I-182 320 90 I-183 320 90 I-184 320 80 I-185 320 80 I-188 320 80 I-190 320 80 I-191 320 80 I-192 320 80 I-193 320 80 I-194 320 90 I-196 320 80 I-197 320 90 I-198 320 90 I-199 320 90 I-20 320 90 I-202 320 80 I-204 320 80 I-207 320 80 I-208 320 80 I-210 320 80 I-212 320 80 I-217 320 90 I-218 320 80 I-221 320 90 I-227 320 90 I-229 320 80 I-230 320 90 I-235 320 80 I-236 320 80 I-237 320 90 I-238 320 80 I-239 320 80 I-241 320 80 I-242 320 80 I-243 320 80 I-245 320 80 I-246 320 80 I-247 320 80 I-251 320 90 I-26 320 80 I-266 320 90 I-267 320 80 I-27 320 90 I-273 320 80 I-274 320 90 I-275 320 80 I-276 320 90 I-28 320 90 I-287 320 80 I-291 320 80 I-293 320 80 I-294 320 80 I-298 320 80 I-299 320 80 I-300 320 80 I-302 320 90 I-304 320 90 I-305 320 90 I-306 320 80 I-307 320 90 I-309 320 90 I-31 320 80 I-310 320 80 I-313 320 90 I-314 320 90 I-315 320 80 I-318 320 90 I-319 320 80 I-320 320 80 I-321 320 80 I-322 320 80 I-324 320 90 I-325 320 80 I-326 320 90 I-327 320 90 I-328 320 90 I-330 320 80 I-331 320 80 I-332 320 80 I-333 320 80 I-334 320 80 I-335 320 80 I-336 320 80 I-337 320 80 I-338 320 80 I-339 320 90 I-340 320 90 I-341 320 80 I-342 320 90 I-343 320 80 I-344 320 90 I-345 320 80 I-348 320 80 I-350 320 90 I-351 320 80 I-352 320 80 I-354 320 80 I-358 320 90 I-359 320 90 I-366 320 80 I-369 320 80 I-370 320 80 I-371 320 80 I-373 320 80 I-375 320 80 I-376 320 80 I-377 320 90 I-383 320 80 I-41 320 90 I-42 320 90 I-48 320 80 I-60 320 80 I-65 320 80 I-66 320 90 I-69 320 80 I-80 320 80 I-85 320 90 I-86 320 90 I-87 320 80 I-88 320 80 I-94 320 90 I-95 320 90 I-96 320 80 II-38 320 80 II-39 320 80 II-40 320 80 II-41 320 80 II-42 320 90 II-43 320 90 II-44 320 90 II-45 320 80 III-01 320 80 III-02 320 80 III-08 320 80 III-09 320 80 III-22 320 90 III-23 320 90 III-24 320 100 III-25 320 80 III-27 320 80 III-28 320 80 III-30 320 90
TABLE-US-00052 TABLE B4a Post-emergence action at 80 g/ha against AVEFA in % Example number Dosage [g/ha] AVEFA I-01 80 90 I-05 80 90 I-08 80 80 I-10 80 80 I-100 80 100 I-101 80 80 I-102 80 90 I-107 80 90 I-11 80 80 I-125 80 90 I-13 80 80 I-144 80 90 I-146 80 90 I-151 80 90 I-153 80 80 I-164 80 80 I-166 80 90 I-167 80 80 I-171 80 90 I-172 80 80 I-174 80 80 I-175 80 80 I-177 80 90 I-180 80 80 I-184 80 80 I-188 80 80 I-189 80 90 I-19 80 90 I-191 80 80 I-193 80 80 I-196 80 80 I-197 80 90 I-198 80 80 I-20 80 90 I-212 80 80 I-218 80 80 I-227 80 90 I-23 80 90 I-24 80 90 I-25 80 90 I-252 80 80 I-26 80 100 I-260 80 80 I-264 80 80 I-267 80 90 I-27 80 100 I-275 80 90 I-28 80 100 I-288 80 80 I-289 80 80 I-29 80 80 I-291 80 80 I-293 80 80 I-296 80 80 I-298 80 80 I-299 80 80 I-302 80 80 I-307 80 90 I-308 80 90 I-314 80 90 I-316 80 90 I-317 80 90 I-318 80 90 I-319 80 80 I-32 80 90 I-321 80 90 I-322 80 80 I-323 80 90 I-324 80 100 I-326 80 90 I-328 80 90 I-33 80 90 I-331 80 90 I-332 80 80 I-333 80 80 I-336 80 80 I-339 80 90 I-34 80 90 I-340 80 90 I-341 80 80 I-342 80 90 I-343 80 80 I-344 80 90 I-348 80 80 I-35 80 100 I-350 80 90 I-358 80 90 I-366 80 90 I-374 80 90 I-375 80 90 I-380 80 90 I-382 80 90 I-383 80 80 I-40 80 80 I-41 80 90 I-42 80 100 I-43 80 90 I-44 80 90 I-45 80 80 I-46 80 80 I-51 80 90 I-52 80 90 I-56 80 80 I-59 80 80 I-64 80 80 I-69 80 80 I-73 80 80 I-74 80 90 I-75 80 80 I-76 80 90 I-77 80 90 I-79 80 100 I-80 80 80 I-81 80 90 I-83 80 100 I-84 80 80 I-87 80 80 I-91 80 90 I-94 80 80 I-95 80 80 I-96 80 80 I-97 80 80 I-98 80 80 III-22 80 100
TABLE-US-00053 TABLE B4b Post-emergence action at 320 g/ha against AVEFA in % Example number Dosage [g/ha] AVEFA I-01 320 100 I-02 320 80 I-03 320 90 I-05 320 90 I-07 320 90 I-08 320 90 I-10 320 90 I-11 320 90 I-13 320 90 I-130 320 90 I-133 320 80 I-140 320 90 I-141 320 80 I-144 320 90 I-145 320 90 I-146 320 90 I-148 320 80 I-149 320 80 I-151 320 90 I-153 320 90 I-154 320 80 I-155 320 80 I-156 320 90 I-164 320 80 I-165 320 90 I-166 320 90 I-167 320 90 I-168 320 80 I-169 320 80 I-17 320 80 I-171 320 90 I-172 320 90 I-174 320 90 I-175 320 80 I-177 320 90 I-179 320 90 I-18 320 80 I-180 320 90 I-181 320 90 I-182 320 90 I-183 320 90 I-184 320 90 I-185 320 80 I-186 320 80 I-187 320 80 I-188 320 80 I-189 320 90 I-190 320 80 I-191 320 90 I-192 320 80 I-193 320 90 I-194 320 90 I-195 320 90 I-196 320 90 I-197 320 90 I-198 320 80 I-199 320 80 I-20 320 90 I-204 320 80 I-212 320 90 I-216 320 80 I-217 320 90 I-218 320 90 I-221 320 80 I-223 320 80 I-225 320 80 I-227 320 90 I-237 320 80 I-242 320 80 I-245 320 80 I-251 320 90 I-252 320 80 I-26 320 100 I-260 320 80 I-264 320 90 I-267 320 90 I-27 320 100 I-272 320 80 I-274 320 90 I-275 320 90 I-28 320 100 I-285 320 80 I-287 320 90 I-288 320 90 I-289 320 90 I-291 320 80 I-293 320 90 I-294 320 90 I-296 320 80 I-298 320 90 I-299 320 80 I-302 320 80 I-304 320 90 I-305 320 80 I-306 320 80 I-307 320 90 I-308 320 90 I-310 320 100 I-311 320 80 I-313 320 80 I-314 320 90 I-315 320 80 I-316 320 100 I-317 320 90 I-318 320 90 I-319 320 80 I-320 320 80 I-321 320 90 I-322 320 80 I-323 320 90 I-324 320 100 I-326 320 90 I-328 320 90 I-330 320 80 I-331 320 90 I-332 320 90 I-333 320 90 I-334 320 80 I-335 320 90 I-336 320 90 I-337 320 80 I-338 320 90 I-339 320 90 I-340 320 90 I-341 320 80 I-342 320 100 I-343 320 80 I-344 320 90 I-348 320 80 I-350 320 90 I-352 320 80 I-354 320 80 I-358 320 90 I-359 320 90 I-360 320 80 I-366 320 90 I-369 320 80 I-370 320 90 I-375 320 90 I-380 320 90 I-382 320 90 I-383 320 80 I-388 320 80 I-41 320 90 I-42 320 100 I-48 320 100 I-58 320 90 I-60 320 90 I-65 320 80 I-66 320 100 I-69 320 100 I-80 320 80 I-85 320 100 I-86 320 100 I-87 320 90 I-88 320 90 I-94 320 100 I-95 320 80 I-96 320 90 II-38 320 90 II-39 320 90 II-40 320 90 II-41 320 90 II-42 320 90 II-43 320 90 II-45 320 90 III-01 320 80 III-22 320 100 III-23 320 80 III-24 320 80
TABLE-US-00054 TABLE B5a Post-emergence action at 80 g/ha against DIGSA in % Example number Dosage [g/ha] DIGSA I-07 80 90 I-10 80 90 I-11 80 90 I-118 80 80 I-121 80 80 I-13 80 90 I-130 80 80 I-141 80 90 I-144 80 90 I-148 80 80 I-149 80 80 I-15 80 90 I-154 80 80 I-164 80 80 I-165 80 90 I-166 80 90 I-167 80 90 I-168 80 80 I-17 80 90 I-172 80 80 I-174 80 90 I-175 80 90 I-176 80 80 I-179 80 90 I-18 80 90 I-180 80 80 I-181 80 90 I-182 80 90 I-19 80 80 I-192 80 80 I-194 80 80 I-195 80 90 I-197 80 90 I-208 80 80 I-212 80 90 I-216 80 80 I-223 80 80 I-227 80 80 I-247 80 80 I-251 80 80 I-252 80 90 I-260 80 90 I-264 80 80 I-285 80 80 I-287 80 80 I-288 80 80 I-29 80 90 I-290 80 90 I-294 80 80 I-296 80 80 I-299 80 80 I-30 80 90 I-304 80 90 I-314 80 90 I-318 80 90 I-322 80 80 I-326 80 80 I-328 80 90 I-344 80 90 I-348 80 80 I-36 80 90 I-360 80 80 I-366 80 80 I-37 80 90 I-38 80 90 I-380 80 80 I-382 80 80 I-383 80 80 I-39 80 90 I-45 80 90 I-46 80 90 I-56 80 90 I-64 80 90 I-90 80 90 I-97 80 80
TABLE-US-00055 TABLE B5b Post-emergence action at 320 g/ha against DIGSA in % Example number Dosage [g/ha] DIGSA I-04 320 80 I-05 320 90 I-07 320 90 I-08 320 90 I-10 320 90 I-11 320 90 I-13 320 90 I-130 320 90 I-133 320 80 I-134 320 80 I-136 320 80 I-139 320 90 I-140 320 80 I-141 320 90 I-144 320 90 I-145 320 90 I-146 320 90 I-148 320 90 I-149 320 90 I-15 320 90 I-154 320 90 I-159 320 80 I-163 320 80 I-164 320 90 I-165 320 90 I-166 320 90 I-167 320 90 I-168 320 90 I-169 320 90 I-17 320 90 I-171 320 80 I-172 320 90 I-174 320 90 I-175 320 90 I-176 320 90 I-177 320 90 I-179 320 90 I-18 320 90 I-180 320 80 I-181 320 90 I-182 320 100 I-192 320 80 I-194 320 90 I-195 320 90 I-197 320 90 I-208 320 90 I-212 320 90 I-216 320 80 I-221 320 80 I-223 320 90 I-227 320 90 I-231 320 90 I-237 320 90 I-242 320 80 I-244 320 80 I-247 320 80 I-251 320 90 I-252 320 90 I-260 320 90 I-264 320 80 I-266 320 90 I-267 320 90 I-274 320 90 I-275 320 90 I-285 320 90 I-286 320 90 I-287 320 80 I-288 320 90 I-289 320 80 I-290 320 90 I-293 320 80 I-294 320 90 I-296 320 90 I-298 320 80 I-299 320 90 I-300 320 80 I-302 320 80 I-304 320 90 I-314 320 90 I-318 320 90 I-322 320 80 I-326 320 90 I-328 320 90 I-344 320 90 I-347 320 80 I-348 320 90 I-360 320 80 I-366 320 90 I-380 320 90 I-382 320 90 I-383 320 90 I-66 320 90 II-41 320 80 II-42 320 80 II-43 320 80 II-44 320 80 II-45 320 80 III-29 320 90
TABLE-US-00056 TABLE B6a Post-emergence action at 80 g/ha against ECHCG in % Example number Dosage [g/ha] ECHCG I-01 80 80 I-02 80 90 I-08 80 80 I-100 80 90 I-116 80 80 I-118 80 80 I-119 80 80 I-121 80 80 I-125 80 90 I-126 80 80 I-141 80 80 I-144 80 90 I-145 80 90 I-146 80 90 I-148 80 80 I-149 80 80 I-151 80 90 I-152 80 80 I-153 80 80 I-154 80 80 I-155 80 80 I-156 80 80 I-157 80 80 I-159 80 80 I-16 80 80 I-163 80 80 I-164 80 80 I-165 80 90 I-166 80 80 I-167 80 80 I-168 80 80 I-169 80 80 I-17 80 80 I-171 80 80 I-172 80 80 I-174 80 80 I-175 80 80 I-176 80 80 I-177 80 100 I-179 80 90 I-18 80 80 I-180 80 80 I-181 80 90 I-182 80 90 I-183 80 90 I-184 80 90 I-185 80 80 I-186 80 80 I-187 80 80 I-188 80 80 I-189 80 90 I-190 80 80 I-191 80 80 I-192 80 90 I-193 80 90 I-194 80 80 I-196 80 80 I-197 80 90 I-198 80 80 I-199 80 90 I-202 80 80 I-204 80 80 I-207 80 80 I-208 80 80 I-210 80 80 I-211 80 80 I-212 80 90 I-216 80 80 I-217 80 90 I-218 80 80 I-221 80 80 I-223 80 80 I-225 80 80 I-227 80 90 I-229 80 80 I-23 80 80 I-231 80 80 I-24 80 80 I-247 80 80 I-251 80 80 I-252 80 80 I-26 80 80 I-264 80 90 I-266 80 80 I-27 80 90 I-274 80 80 I-28 80 80 I-287 80 90 I-289 80 80 I-29 80 80 I-290 80 80 I-291 80 80 I-294 80 80 I-296 80 80 I-298 80 80 I-299 80 80 I-30 80 80 I-300 80 80 I-304 80 80 I-305 80 90 I-307 80 90 I-308 80 90 I-311 80 80 I-314 80 90 I-315 80 90 I-316 80 90 I-317 80 80 I-318 80 90 I-319 80 80 I-32 80 80 I-321 80 90 I-323 80 90 I-324 80 90 I-325 80 90 I-326 80 90 I-327 80 80 I-328 80 90 I-33 80 90 I-330 80 80 I-331 80 90 I-332 80 80 I-333 80 80 I-334 80 80 I-335 80 80 I-336 80 80 I-337 80 80 I-339 80 90 I-340 80 80 I-341 80 100 I-342 80 90 I-343 80 90 I-344 80 90 I-348 80 90 I-35 80 90 I-350 80 80 I-36 80 90 I-360 80 80 I-366 80 90 I-369 80 80 I-37 80 80 I-370 80 80 I-375 80 90 I-377 80 80 I-38 80 90 I-380 80 80 I-382 80 80 I-383 80 80 I-388 80 90 I-39 80 80 I-40 80 90 I-42 80 90 I-43 80 90 I-47 80 80 I-48 80 80 I-51 80 90 I-53 80 80 I-59 80 80 I-64 80 90 I-65 80 80 I-66 80 80 I-73 80 80 I-74 80 90 I-75 80 90 I-76 80 90 I-77 80 90 I-80 80 80 I-81 80 90 I-83 80 90 I-84 80 80 I-85 80 90 I-86 80 100 I-88 80 80 I-91 80 80 I-96 80 90 I-97 80 80 I-98 80 80 III-22 80 100 III-24 80 80 III-29 80 80
TABLE-US-00057 TABLE B6b Post-emergence action at 320 g/ha against ECHCG in % Example number Dosage [g/ha] ECHCG I-01 320 90 I-02 320 90 I-03 320 90 I-05 320 90 I-07 320 90 I-08 320 90 I-10 320 80 I-11 320 80 I-111 320 90 I-130 320 90 I-133 320 90 I-134 320 80 I-136 320 80 I-137 320 80 I-138 320 90 I-139 320 80 I-140 320 80 I-141 320 80 I-144 320 90 I-145 320 90 I-146 320 90 I-148 320 80 I-149 320 80 I-151 320 90 I-152 320 80 I-153 320 90 I-154 320 80 I-155 320 80 I-156 320 80 I-157 320 90 I-159 320 90 I-16 320 80 I-162 320 80 I-163 320 80 I-164 320 80 I-165 320 90 I-166 320 80 I-167 320 80 I-168 320 90 I-169 320 90 I-17 320 80 I-171 320 80 I-172 320 90 I-174 320 80 I-175 320 80 I-176 320 90 I-177 320 100 I-179 320 90 I-18 320 80 I-180 320 90 I-181 320 100 I-182 320 90 I-183 320 90 I-184 320 90 I-185 320 90 I-186 320 90 I-187 320 80 I-188 320 90 I-189 320 90 I-190 320 80 I-191 320 80 I-192 320 90 I-193 320 90 I-194 320 80 I-195 320 80 I-196 320 80 I-197 320 90 I-198 320 80 I-199 320 90 I-20 320 80 I-202 320 90 I-204 320 80 I-206 320 80 I-207 320 80 I-208 320 90 I-210 320 80 I-211 320 80 I-212 320 90 I-216 320 80 I-217 320 90 I-218 320 90 I-221 320 80 I-223 320 90 I-225 320 90 I-227 320 100 I-229 320 80 I-230 320 80 I-231 320 90 I-238 320 80 I-247 320 80 I-251 320 90 I-252 320 90 I-26 320 80 I-260 320 90 I-264 320 90 I-266 320 90 I-267 320 90 I-27 320 90 I-272 320 80 I-273 320 90 I-274 320 90 I-275 320 90 I-276 320 80 I-277 320 80 I-278 320 80 I-279 320 80 I-28 320 90 I-285 320 80 I-286 320 80 I-287 320 90 I-288 320 80 I-289 320 80 I-290 320 90 I-291 320 80 I-293 320 80 I-294 320 90 I-296 320 80 I-298 320 90 I-299 320 90 I-300 320 90 I-302 320 80 I-304 320 90 I-305 320 90 I-306 320 90 I-307 320 90 I-308 320 90 I-309 320 90 I-310 320 90 I-311 320 90 I-312 320 90 I-313 320 90 I-314 320 90 I-315 320 100 I-316 320 90 I-317 320 90 I-318 320 90 I-319 320 90 I-320 320 90 I-321 320 90 I-322 320 80 I-323 320 90 I-324 320 90 I-325 320 90 I-326 320 90 I-327 320 90 I-328 320 90 I-330 320 90 I-331 320 90 I-332 320 90 I-333 320 90 I-334 320 90 I-335 320 90 I-336 320 80 I-337 320 90 I-338 320 80 I-339 320 90 I-340 320 90 I-341 320 100 I-342 320 90 I-343 320 90 I-344 320 90 I-347 320 80 I-348 320 90 I-350 320 90 I-351 320 80 I-352 320 80 I-354 320 100 I-358 320 90 I-359 320 80 I-360 320 80 I-362 320 80 I-363 320 80 I-366 320 90 I-369 320 80 I-370 320 80 I-373 320 90 I-375 320 90 I-376 320 90 I-377 320 90 I-378 320 80 I-380 320 90 I-381 320 80 I-382 320 90 I-383 320 90 I-388 320 90 I-41 320 80 I-42 320 90 I-48 320 90 I-58 320 80 I-60 320 80 I-65 320 80 I-66 320 90 I-80 320 80 I-82 320 80 I-85 320 90 I-86 320 100 I-87 320 80 I-88 320 90 I-94 320 90 I-95 320 90 I-96 320 90 II-37 320 80 II-38 320 90 II-39 320 90 II-40 320 90 II-41 320 90 II-42 320 90 II-43 320 90 II-44 320 90 II-45 320 90 III-01 320 80 III-22 320 100 III-24 320 100 III-29 320 80
TABLE-US-00058 TABLE B7a Post-emergence action at 80 g/ha against LOLRI in % Example number Dosage [g/ha] LOLRI I-01 80 80 I-02 80 80 I-10 80 90 I-100 80 80 I-101 80 90 I-102 80 90 I-107 80 80 I-125 80 80 I-126 80 80 I-134 80 80 I-144 80 90 I-145 80 90 I-148 80 80 I-149 80 80 I-154 80 80 I-164 80 80 I-166 80 80 I-167 80 80 I-171 80 80 I-172 80 90 I-174 80 80 I-175 80 80 I-176 80 80 I-177 80 100 I-180 80 90 I-184 80 90 I-185 80 80 I-187 80 90 I-188 80 90 I-189 80 100 I-19 80 80 I-190 80 90 I-191 80 90 I-194 80 80 I-196 80 90 I-197 80 90 I-198 80 80 I-199 80 90 I-20 80 90 I-218 80 80 I-221 80 80 I-227 80 80 I-24 80 90 I-25 80 80 I-251 80 90 I-252 80 80 I-264 80 90 I-267 80 90 I-27 80 90 I-274 80 80 I-275 80 90 I-285 80 80 I-287 80 90 I-288 80 80 I-289 80 80 I-291 80 80 I-293 80 80 I-296 80 80 I-298 80 90 I-299 80 80 I-300 80 90 I-307 80 100 I-308 80 90 I-314 80 90 I-316 80 100 I-317 80 90 I-318 80 90 I-319 80 80 I-32 80 90 I-321 80 100 I-322 80 80 I-323 80 90 I-326 80 90 I-328 80 90 I-33 80 80 I-331 80 90 I-332 80 80 I-336 80 80 I-339 80 90 I-34 80 80 I-340 80 90 I-341 80 90 I-342 80 90 I-344 80 90 I-348 80 80 I-35 80 90 I-350 80 80 I-358 80 90 I-366 80 90 I-369 80 80 I-374 80 90 I-375 80 90 I-380 80 90 I-383 80 80 I-388 80 80 I-40 80 90 I-41 80 80 I-42 80 100 I-52 80 80 I-59 80 80 I-64 80 80 I-73 80 80 I-74 80 90 I-75 80 90 I-76 80 80 I-83 80 90 I-84 80 90 I-85 80 100 I-86 80 100 I-91 80 90 I-96 80 90 III-24 80 100
TABLE-US-00059 TABLE B7b Post-emergence action at 320 g/ha against LOLRI in % Example number Dosage [g/ha] LOLRI I-01 320 90 I-02 320 80 I-05 320 90 I-07 320 90 I-08 320 90 I-10 320 90 I-11 320 80 I-13 320 90 I-130 320 90 I-133 320 90 I-134 320 90 I-136 320 80 I-137 320 90 I-138 320 90 I-140 320 90 I-141 320 90 I-144 320 90 I-145 320 90 I-146 320 90 I-148 320 80 I-149 320 90 I-15 320 80 I-151 320 90 I-154 320 90 I-155 320 80 I-159 320 80 I-163 320 80 I-164 320 90 I-165 320 100 I-166 320 90 I-167 320 80 I-168 320 80 I-169 320 80 I-17 320 80 I-171 320 90 I-172 320 90 I-174 320 80 I-175 320 80 I-176 320 80 I-177 320 100 I-18 320 80 I-180 320 90 I-181 320 80 I-183 320 90 I-184 320 90 I-185 320 80 I-187 320 90 I-188 320 90 I-189 320 100 I-190 320 90 I-191 320 90 I-192 320 80 I-193 320 90 I-194 320 90 I-195 320 80 I-196 320 90 I-197 320 90 I-198 320 80 I-199 320 90 I-20 320 90 I-208 320 80 I-210 320 80 I-211 320 80 I-212 320 80 I-217 320 80 I-218 320 90 I-221 320 90 I-227 320 90 I-237 320 80 I-238 320 80 I-240 320 80 I-242 320 80 I-244 320 80 I-247 320 80 I-251 320 90 I-252 320 80 I-26 320 80 I-260 320 80 I-264 320 90 I-266 320 90 I-267 320 100 I-27 320 90 I-274 320 90 I-275 320 90 I-276 320 80 I-278 320 80 I-279 320 80 I-28 320 90 I-285 320 90 I-287 320 90 I-288 320 80 I-289 320 90 I-290 320 80 I-291 320 80 I-293 320 80 I-294 320 90 I-296 320 80 I-298 320 90 I-299 320 80 I-300 320 90 I-302 320 80 I-304 320 90 I-305 320 90 I-306 320 90 I-307 320 100 I-308 320 100 I-309 320 90 I-310 320 90 I-311 320 80 I-312 320 90 I-313 320 90 I-314 320 90 I-315 320 90 I-316 320 100 I-317 320 90 I-318 320 90 I-319 320 80 I-320 320 90 I-321 320 100 I-322 320 80 I-323 320 90 I-324 320 90 I-325 320 90 I-326 320 90 I-327 320 90 I-328 320 90 I-330 320 90 I-331 320 90 I-332 320 90 I-333 320 90 I-334 320 90 I-335 320 90 I-336 320 80 I-338 320 90 I-339 320 90 I-340 320 90 I-341 320 90 I-342 320 90 I-343 320 90 I-344 320 90 I-348 320 80 I-350 320 90 I-351 320 80 I-352 320 80 I-354 320 90 I-358 320 90 I-359 320 80 I-360 320 90 I-362 320 80 I-366 320 90 I-369 320 90 I-370 320 90 I-371 320 90 I-375 320 90 I-376 320 90 I-380 320 90 I-381 320 80 I-382 320 90 I-383 320 90 I-388 320 80 I-41 320 90 I-42 320 100 I-48 320 80 I-58 320 80 I-66 320 90 I-69 320 80 I-85 320 100 I-86 320 100 I-87 320 80 I-88 320 80 I-94 320 100 I-95 320 80 I-96 320 90 III-22 320 100 III-24 320 100 III-29 320 80
TABLE-US-00060 TABLE B8a Post-emergence action at 80 g/ha against MATIN in % Example number Dosage [g/ha] MATIN I-02 80 80 I-03 80 80 I-07 80 90 I-08 80 90 I-100 80 90 I-116 80 80 I-118 80 80 I-125 80 80 I-126 80 80 I-141 80 80 I-144 80 90 I-145 80 80 I-146 80 90 I-148 80 80 I-149 80 80 I-15 80 80 I-151 80 80 I-165 80 80 I-166 80 80 I-168 80 90 I-169 80 80 I-171 80 80 I-172 80 90 I-177 80 90 I-179 80 80 I-18 80 80 I-181 80 80 I-182 80 80 I-183 80 80 I-189 80 90 I-197 80 80 I-208 80 80 I-210 80 80 I-211 80 80 I-216 80 80 I-227 80 80 I-231 80 80 I-266 80 80 I-275 80 80 I-29 80 90 I-30 80 90 I-304 80 90 I-308 80 80 I-313 80 80 I-316 80 80 I-317 80 90 I-318 80 80 I-33 80 80 I-331 80 80 I-344 80 80 I-35 80 90 I-354 80 80 I-370 80 80 I-374 80 80 I-42 80 80 I-51 80 80 I-59 80 80 I-64 80 90 I-66 80 80 I-74 80 90 I-75 80 90 I-76 80 80 I-77 80 90 I-81 80 90 I-85 80 80 I-93 80 80 I-97 80 80 I-98 80 80 III-29 80 80
TABLE-US-00061 TABLE B8b Post-emergence action at 320 g/ha against MATIN in % Example number Dosage [g/ha] MATIN I-01 320 90 I-02 320 80 I-03 320 90 I-05 320 100 I-07 320 100 I-08 320 90 I-130 320 80 I-136 320 80 I-141 320 90 I-144 320 90 I-145 320 90 I-146 320 90 I-148 320 80 I-149 320 90 I-15 320 90 I-151 320 90 I-153 320 80 I-154 320 80 I-155 320 80 I-156 320 80 I-159 320 80 I-16 320 80 I-164 320 80 I-165 320 90 I-166 320 90 I-168 320 90 I-169 320 90 I-171 320 90 I-172 320 90 I-176 320 80 I-177 320 90 I-179 320 90 I-18 320 80 I-180 320 90 I-181 320 80 I-182 320 90 I-183 320 80 I-184 320 80 I-185 320 80 I-187 320 80 I-188 320 80 I-189 320 90 I-190 320 80 I-191 320 80 I-192 320 80 I-193 320 80 I-196 320 80 I-197 320 90 I-198 320 80 I-199 320 80 I-204 320 80 I-206 320 80 I-207 320 80 I-208 320 80 I-210 320 80 I-211 320 80 I-212 320 80 I-216 320 80 I-217 320 80 I-218 320 80 I-227 320 90 I-229 320 80 I-231 320 80 I-236 320 80 I-239 320 80 I-241 320 80 I-243 320 80 I-246 320 80 I-251 320 90 I-252 320 80 I-264 320 80 I-266 320 90 I-273 320 80 I-274 320 90 I-275 320 90 I-276 320 80 I-28 320 80 I-285 320 80 I-287 320 80 I-289 320 90 I-293 320 80 I-294 320 90 I-298 320 80 I-300 320 80 I-304 320 90 I-305 320 80 I-307 320 80 I-308 320 90 I-309 320 80 I-313 320 90 I-314 320 80 I-316 320 90 I-317 320 90 I-318 320 80 I-321 320 80 I-323 320 90 I-324 320 80 I-326 320 80 I-331 320 80 I-334 320 80 I-338 320 90 I-341 320 90 I-342 320 100 I-343 320 80 I-344 320 80 I-348 320 80 I-354 320 80 I-366 320 80 I-369 320 80 I-370 320 80 I-373 320 90 I-375 320 80 I-383 320 80 I-41 320 80 I-42 320 90 I-66 320 90 I-69 320 80 I-85 320 90 I-86 320 80 I-87 320 80 I-88 320 80 I-94 320 80 I-95 320 80 I-96 320 80 II-41 320 80 II-42 320 80 II-43 320 80 II-45 320 90 III-29 320 90
TABLE-US-00062 TABLE B9a Post-emergence action at 80 g/ha against PHBPU in % Example number Dosage [g/ha] PHBPU I-01 80 80 I-02 80 90 I-03 80 90 I-07 80 80 I-08 80 80 I-100 80 90 I-103 80 80 I-118 80 80 I-119 80 80 I-120 80 80 I-125 80 80 I-141 80 80 I-144 80 90 I-145 80 90 I-146 80 90 I-148 80 80 I-149 80 80 I-151 80 90 I-152 80 80 I-153 80 80 I-154 80 80 I-155 80 80 I-159 80 80 I-16 80 90 I-163 80 80 I-164 80 80 I-165 80 80 I-166 80 80 I-167 80 90 I-168 80 90 I-169 80 80 I-171 80 80 I-172 80 80 I-174 80 80 I-175 80 80 I-177 80 90 I-179 80 80 I-181 80 90 I-182 80 90 I-183 80 80 I-184 80 90 I-188 80 90 I-189 80 90 I-19 80 90 I-191 80 90 I-192 80 90 I-193 80 90 I-194 80 90 I-195 80 90 I-196 80 90 I-197 80 90 I-198 80 80 I-20 80 90 I-207 80 80 I-208 80 80 I-210 80 90 I-211 80 90 I-212 80 90 I-216 80 80 I-218 80 90 I-221 80 90 I-223 80 80 I-225 80 80 I-227 80 90 I-235 80 80 I-237 80 80 I-239 80 80 I-241 80 80 I-242 80 80 I-245 80 80 I-246 80 80 I-247 80 90 I-264 80 80 I-266 80 80 I-273 80 80 I-275 80 90 I-276 80 80 I-278 80 80 I-279 80 80 I-28 80 80 I-285 80 80 I-288 80 80 I-289 80 80 I-291 80 80 I-304 80 80 I-307 80 80 I-309 80 80 I-312 80 80 I-313 80 90 I-314 80 90 I-315 80 80 I-316 80 90 I-318 80 90 I-319 80 80 I-32 80 80 I-322 80 80 I-326 80 80 I-328 80 90 I-330 80 80 I-332 80 80 I-333 80 80 I-336 80 90 I-337 80 90 I-34 80 80 I-340 80 90 I-341 80 90 I-342 80 80 I-344 80 90 I-348 80 80 I-352 80 90 I-357 80 80 I-36 80 80 I-360 80 80 I-366 80 80 I-369 80 80 I-37 80 80 I-370 80 80 I-375 80 80 I-38 80 90 I-382 80 80 I-388 80 80 I-39 80 80 I-40 80 80 I-46 80 80 I-51 80 90 I-56 80 80 I-59 80 80 I-64 80 90 I-69 80 80 I-73 80 90 I-74 80 90 I-75 80 90 I-76 80 90 I-77 80 90 I-79 80 80 I-80 80 80 I-81 80 90 I-83 80 90 I-84 80 90 I-85 80 90 I-88 80 80 I-91 80 80 I-96 80 90 I-97 80 80 I-99 80 80 II-41 80 80 II-43 80 80 III-17 80 80 III-19 80 80 III-29 80 80
TABLE-US-00063 TABLE B9b Post-emergence action at 320 g/ha against PHBPU in % Example number Dosage [g/ha] PHBPU I-01 320 80 I-02 320 100 I-03 320 100 I-04 320 100 I-05 320 90 I-07 320 80 I-08 320 80 I-11 320 90 I-130 320 80 I-133 320 80 I-136 320 90 I-138 320 80 I-139 320 80 I-141 320 90 I-144 320 90 I-145 320 90 I-146 320 90 I-147 320 90 I-148 320 90 I-149 320 80 I-15 320 90 I-151 320 90 I-152 320 90 I-153 320 90 I-154 320 90 I-155 320 90 I-156 320 90 I-157 320 80 I-159 320 80 I-16 320 90 I-160 320 90 I-162 320 90 I-163 320 90 I-164 320 90 I-165 320 90 I-166 320 90 I-167 320 90 I-168 320 90 I-169 320 90 I-17 320 80 I-171 320 90 I-172 320 90 I-174 320 90 I-175 320 90 I-177 320 90 I-179 320 90 I-181 320 100 I-182 320 90 I-183 320 90 I-184 320 90 I-187 320 80 I-188 320 90 I-189 320 90 I-191 320 100 I-192 320 90 I-193 320 100 I-194 320 90 I-195 320 90 I-196 320 90 I-197 320 100 I-198 320 90 I-199 320 80 I-20 320 90 I-202 320 90 I-204 320 80 I-206 320 90 I-207 320 90 I-208 320 90 I-210 320 100 I-211 320 100 I-212 320 100 I-216 320 80 I-218 320 100 I-221 320 100 I-223 320 80 I-225 320 80 I-227 320 100 I-229 320 80 I-230 320 90 I-231 320 80 I-235 320 80 I-236 320 80 I-237 320 90 I-238 320 80 I-239 320 90 I-241 320 90 I-242 320 80 I-244 320 80 I-245 320 90 I-246 320 80 I-247 320 90 I-248 320 90 I-252 320 90 I-260 320 80 I-261 320 80 I-264 320 80 I-266 320 90 I-267 320 90 I-268 320 80 I-273 320 90 I-274 320 80 I-275 320 100 I-276 320 90 I-277 320 80 I-278 320 80 I-279 320 80 I-28 320 80 I-285 320 90 I-287 320 80 I-288 320 90 I-289 320 80 I-290 320 90 I-291 320 90 I-293 320 80 I-296 320 90 I-298 320 90 I-299 320 90 I-300 320 80 I-302 320 80 I-304 320 90 I-305 320 90 I-307 320 90 I-308 320 90 I-309 320 90 I-311 320 90 I-312 320 90 I-313 320 90 I-314 320 90 I-315 320 80 I-316 320 90 I-317 320 80 I-318 320 90 I-319 320 90 I-320 320 80 I-321 320 90 I-322 320 80 I-323 320 80 I-324 320 90 I-325 320 80 I-326 320 90 I-328 320 90 I-329 320 80 I-330 320 90 I-331 320 90 I-332 320 80 I-333 320 90 I-334 320 80 I-336 320 100 I-337 320 90 I-339 320 80 I-340 320 90 I-341 320 100 I-342 320 90 I-343 320 90 I-344 320 90 I-346 320 90 I-348 320 80 I-351 320 80 I-352 320 90 I-354 320 90 I-357 320 80 I-359 320 80 I-360 320 80 I-362 320 80 I-363 320 80 I-366 320 80 I-369 320 90 I-370 320 90 I-371 320 80 I-373 320 80 I-375 320 90 I-376 320 80 I-377 320 90 I-382 320 80 I-388 320 100 I-41 320 90 I-42 320 90 I-48 320 90 I-58 320 80 I-66 320 80 I-69 320 80 I-80 320 80 I-85 320 90 I-87 320 90 I-88 320 80 I-94 320 80 I-96 320 90 II-38 320 80 II-39 320 90 II-40 320 80 II-41 320 90 II-42 320 90 II-43 320 90 II-45 320 90 III-22 320 80 III-23 320 80 III-29 320 90
TABLE-US-00064 TABLE 10a Post-emergence action at 80 g/ha against POLCO in % Example number Dosage [g/ha] POLCO I-02 80 80 I-03 80 90 I-05 80 90 I-07 80 80 I-08 80 90 I-10 80 80 I-100 80 90 I-102 80 90 I-121 80 80 I-122 80 90 I-133 80 80 I-137 80 80 I-141 80 80 I-144 80 80 I-145 80 90 I-146 80 80 I-165 80 80 I-166 80 80 I-167 80 80 I-169 80 80 I-171 80 80 I-175 80 80 I-176 80 80 I-177 80 90 I-179 80 90 I-180 80 80 I-181 80 80 I-182 80 80 I-184 80 80 I-187 80 80 I-188 80 80 I-19 80 90 I-190 80 80 I-193 80 80 I-196 80 80 I-197 80 90 I-212 80 80 I-217 80 80 I-223 80 80 I-227 80 90 I-239 80 80 I-241 80 80 I-242 80 80 I-244 80 80 I-247 80 80 I-26 80 80 I-260 80 80 I-266 80 80 I-267 80 80 I-27 80 80 I-275 80 80 I-291 80 80 I-293 80 80 I-307 80 80 I-310 80 80 I-312 80 80 I-315 80 80 I-318 80 90 I-321 80 80 I-322 80 80 I-324 80 80 I-326 80 80 I-328 80 90 I-331 80 80 I-335 80 80 I-337 80 80 I-338 80 80 I-339 80 90 I-341 80 80 I-342 80 80 I-343 80 80 I-344 80 80 I-350 80 80 I-358 80 90 I-36 80 80 I-37 80 80 I-375 80 80 I-38 80 80 I-39 80 90 I-41 80 80 I-42 80 80 I-44 80 90 I-48 80 80 I-56 80 80 I-59 80 80 I-66 80 80 I-73 80 90 I-74 80 90 I-75 80 90 I-76 80 80 I-77 80 80 I-79 80 80 I-80 80 80 I-81 80 80 I-84 80 90 I-85 80 90 I-87 80 80 I-88 80 80 I-94 80 80 I-95 80 80 I-96 80 80 I-99 80 90 II-40 80 80 II-45 80 80
TABLE-US-00065 TABLE 10b Post-emergence action at 320 g/ha against POLCO in % Example number Dosage [g/ha] POLCO I-02 320 80 I-03 320 90 I-04 320 90 I-05 320 90 I-07 320 80 I-08 320 90 I-10 320 80 I-111 320 80 I-130 320 80 I-133 320 80 I-137 320 80 I-138 320 80 I-139 320 90 I-140 320 90 I-141 320 80 I-144 320 80 I-145 320 90 I-146 320 90 I-147 320 90 I-149 320 80 I-150 320 90 I-151 320 80 I-152 320 80 I-153 320 80 I-154 320 80 I-156 320 80 I-165 320 90 I-166 320 80 I-167 320 80 I-168 320 80 I-169 320 80 I-171 320 90 I-172 320 80 I-174 320 80 I-175 320 80 I-176 320 80 I-177 320 90 I-179 320 90 I-180 320 90 I-181 320 80 I-182 320 90 I-183 320 90 I-184 320 80 I-185 320 80 I-186 320 80 I-187 320 80 I-188 320 80 I-190 320 80 I-192 320 80 I-193 320 80 I-195 320 80 I-196 320 80 I-197 320 90 I-20 320 80 I-202 320 80 I-208 320 80 I-212 320 90 I-217 320 80 I-218 320 80 I-223 320 80 I-227 320 90 I-229 320 80 I-230 320 80 I-235 320 80 I-236 320 80 I-237 320 80 I-238 320 80 I-239 320 80 I-240 320 80 I-241 320 80 I-242 320 80 I-244 320 80 I-245 320 80 I-246 320 80 I-247 320 80 I-252 320 80 I-26 320 80 I-260 320 80 I-261 320 80 I-266 320 90 I-267 320 80 I-27 320 80 I-272 320 80 I-273 320 80 I-274 320 80 I-275 320 80 I-28 320 80 I-285 320 80 I-288 320 80 I-289 320 80 I-290 320 80 I-291 320 80 I-293 320 80 I-296 320 80 I-298 320 80 I-299 320 80 I-302 320 80 I-305 320 80 I-306 320 80 I-307 320 80 I-309 320 80 I-31 320 80 I-310 320 80 I-311 320 80 I-312 320 80 I-314 320 90 I-315 320 80 I-318 320 90 I-319 320 80 I-320 320 80 I-321 320 90 I-322 320 80 I-324 320 80 I-325 320 80 I-326 320 90 I-327 320 80 I-328 320 90 I-331 320 80 I-333 320 80 I-334 320 80 I-335 320 80 I-336 320 80 I-337 320 80 I-338 320 80 I-339 320 90 I-340 320 90 I-341 320 80 I-342 320 90 I-343 320 80 I-344 320 90 I-347 320 80 I-348 320 80 I-350 320 90 I-351 320 80 I-354 320 80 I-358 320 90 I-359 320 80 I-366 320 80 I-369 320 80 I-373 320 80 I-375 320 90 I-376 320 80 I-377 320 80 I-380 320 80 I-382 320 80 I-41 320 80 I-42 320 90 I-48 320 90 I-60 320 80 I-65 320 80 I-66 320 90 I-80 320 80 I-85 320 90 I-86 320 90 I-87 320 80 I-88 320 80 I-94 320 90 I-95 320 80 I-96 320 80 II-38 320 90 II-40 320 80 II-42 320 80 II-43 320 80 II-44 320 90 II-45 320 90 II-46 320 80 III-08 320 80 III-24 320 90 III-29 320 80 III-30 320 90
TABLE-US-00066 TABLE 11a Post-emergence action at 80 g/ha against SETVI in % Example number Dosage [g/ha] SETVI I-02 80 80 I-05 80 80 I-07 80 90 I-08 80 80 I-10 80 80 I-100 80 80 I-107 80 80 I-11 80 80 I-114 80 80 I-116 80 80 I-118 80 80 I-119 80 80 I-125 80 80 I-126 80 80 I-13 80 80 I-141 80 90 I-144 80 90 I-145 80 90 I-146 80 90 I-148 80 80 I-149 80 80 I-15 80 80 I-151 80 90 I-152 80 80 I-155 80 80 I-16 80 80 I-163 80 80 I-164 80 80 I-165 80 90 I-166 80 90 I-168 80 80 I-17 80 80 I-171 80 90 I-172 80 80 I-176 80 80 I-177 80 90 I-179 80 90 I-18 80 80 I-180 80 80 I-181 80 80 I-182 80 80 I-183 80 90 I-184 80 80 I-188 80 80 I-189 80 90 I-19 80 80 I-190 80 80 I-191 80 80 I-192 80 80 I-194 80 90 I-195 80 90 I-196 80 80 I-197 80 90 I-198 80 80 I-199 80 80 I-204 80 90 I-207 80 90 I-208 80 80 I-210 80 80 I-211 80 80 I-212 80 80 I-217 80 80 I-218 80 80 I-221 80 90 I-227 80 90 I-229 80 80 I-252 80 80 I-264 80 90 I-267 80 90 I-274 80 90 I-275 80 90 I-279 80 80 I-28 80 80 I-285 80 90 I-287 80 90 I-288 80 90 I-289 80 90 I-29 80 80 I-290 80 90 I-291 80 80 I-294 80 90 I-298 80 90 I-302 80 80 I-304 80 90 I-307 80 90 I-313 80 90 I-314 80 90 I-316 80 90 I-318 80 90 I-321 80 90 I-322 80 80 I-324 80 80 I-326 80 90 I-328 80 90 I-331 80 90 I-338 80 90 I-339 80 90 I-340 80 80 I-341 80 80 I-342 80 90 I-343 80 90 I-344 80 90 I-348 80 80 I-35 80 100 I-350 80 80 I-354 80 80 I-36 80 80 I-360 80 80 I-366 80 90 I-37 80 80 I-370 80 80 I-374 80 90 I-375 80 90 I-38 80 80 I-380 80 80 I-382 80 90 I-383 80 80 I-388 80 90 I-39 80 80 I-40 80 80 I-42 80 90 I-43 80 90 I-47 80 90 I-48 80 80 I-51 80 90 I-52 80 80 I-53 80 80 I-54 80 80 I-64 80 90 I-66 80 80 I-69 80 80 I-73 80 80 I-74 80 80 I-75 80 80 I-76 80 90 I-77 80 80 I-79 80 80 I-81 80 80 I-83 80 90 I-84 80 80 I-85 80 90 I-86 80 100 I-87 80 80 I-91 80 80 I-94 80 80 I-96 80 90 I-97 80 80 III-22 80 100 III-23 80 80 III-24 80 100
TABLE-US-00067 TABLE B11b Post-emergence action at 320 g/ha against SETVI in % Example number Dosage [g/ha] SETVI I-01 320 80 I-02 320 80 I-03 320 90 I-04 320 100 I-05 320 90 I-07 320 90 I-08 320 90 I-10 320 80 I-11 320 90 I-13 320 90 I-133 320 80 I-134 320 80 I-136 320 90 I-138 320 80 I-141 320 90 I-144 320 90 I-145 320 90 I-146 320 90 I-148 320 80 I-149 320 80 I-15 320 90 I-150 320 80 I-151 320 90 I-152 320 80 I-153 320 80 I-154 320 80 I-155 320 90 I-156 320 80 I-157 320 80 I-159 320 80 I-16 320 80 I-160 320 80 I-162 320 80 I-163 320 90 I-164 320 80 I-165 320 90 I-166 320 90 I-167 320 80 I-168 320 90 I-169 320 80 I-17 320 80 I-171 320 90 I-172 320 80 I-175 320 80 I-176 320 80 I-177 320 90 I-179 320 90 I-18 320 80 I-180 320 90 I-181 320 90 I-182 320 80 I-183 320 90 I-184 320 90 I-185 320 80 I-187 320 80 I-188 320 80 I-189 320 90 I-190 320 80 I-191 320 80 I-192 320 80 I-193 320 90 I-194 320 90 I-195 320 90 I-196 320 80 I-197 320 90 I-198 320 80 I-199 320 90 I-20 320 90 I-202 320 80 I-204 320 90 I-207 320 90 I-208 320 80 I-210 320 80 I-211 320 80 I-212 320 80 I-216 320 80 I-217 320 90 I-218 320 80 I-221 320 90 I-223 320 80 I-225 320 80 I-227 320 90 I-229 320 80 I-230 320 80 I-231 320 80 I-247 320 80 I-251 320 90 I-252 320 80 I-26 320 90 I-260 320 90 I-264 320 90 I-266 320 80 I-267 320 90 I-27 320 90 I-272 320 80 I-274 320 90 I-275 320 90 I-276 320 90 I-278 320 90 I-279 320 80 I-28 320 90 I-285 320 90 I-286 320 80 I-287 320 90 I-288 320 90 I-289 320 90 I-290 320 90 I-291 320 80 I-293 320 80 I-294 320 90 I-296 320 80 I-298 320 90 I-299 320 90 I-300 320 80 I-302 320 90 I-304 320 90 I-305 320 90 I-306 320 90 I-307 320 90 I-309 320 90 I-310 320 90 I-311 320 80 I-312 320 80 I-313 320 90 I-314 320 90 I-315 320 80 I-316 320 90 I-318 320 90 I-319 320 80 I-320 320 90 I-321 320 90 I-322 320 80 I-323 320 90 I-324 320 90 I-326 320 90 I-327 320 90 I-328 320 90 I-330 320 80 I-331 320 90 I-332 320 80 I-333 320 80 I-335 320 90 I-336 320 80 I-337 320 80 I-338 320 90 I-339 320 90 I-340 320 90 I-341 320 80 I-342 320 90 I-343 320 90 I-344 320 90 I-348 320 90 I-350 320 90 I-351 320 80 I-352 320 80 I-354 320 80 I-357 320 80 I-358 320 90 I-360 320 80 I-362 320 80 I-366 320 90 I-370 320 80 I-371 320 80 I-373 320 90 I-375 320 90 I-376 320 80 I-377 320 90 I-378 320 80 I-380 320 90 I-382 320 90 I-383 320 80 I-388 320 90 I-41 320 80 I-42 320 90 I-48 320 80 I-65 320 80 I-66 320 90 I-69 320 80 I-80 320 80 I-85 320 100 I-86 320 100 I-87 320 80 I-88 320 80 I-94 320 90 I-95 320 90 I-96 320 90 II-37 320 80 II-38 320 90 II-39 320 90 II-40 320 90 II-41 320 90 II-42 320 90 II-43 320 90 II-44 320 90 II-45 320 90 III-22 320 100 III-23 320 100 III-24 320 100 III-29 320 90
TABLE-US-00068 TABLE B12a Post-emergence action at 80 g/ha against VERPE in % Example number Dosage [g/ha] VERPE I-01 80 80 I-02 80 80 I-03 80 80 I-05 80 90 I-07 80 90 I-08 80 90 I-100 80 80 I-103 80 80 I-116 80 80 I-118 80 90 I-119 80 80 I-120 80 90 I-121 80 80 I-122 80 80 I-130 80 80 I-133 80 80 I-134 80 80 I-139 80 80 I-141 80 90 I-144 80 90 I-145 80 90 I-146 80 90 I-148 80 80 I-15 80 80 I-155 80 80 I-157 80 80 I-16 80 80 I-160 80 80 I-162 80 80 I-164 80 80 I-165 80 90 I-166 80 80 I-167 80 80 I-168 80 80 I-169 80 80 I-171 80 80 I-172 80 80 I-174 80 80 I-175 80 80 I-177 80 100 I-179 80 90 I-180 80 80 I-181 80 90 I-182 80 80 I-184 80 90 I-185 80 80 I-187 80 90 I-188 80 80 I-189 80 90 I-190 80 80 I-191 80 80 I-192 80 80 I-193 80 80 I-195 80 80 I-196 80 80 I-197 80 90 I-198 80 80 I-199 80 90 I-204 80 90 I-207 80 80 I-208 80 80 I-210 80 90 I-211 80 80 I-212 80 80 I-218 80 80 I-225 80 80 I-227 80 90 I-23 80 80 I-230 80 80 I-239 80 80 I-247 80 80 I-25 80 80 I-251 80 80 I-252 80 80 I-264 80 80 I-266 80 80 I-267 80 90 I-27 80 80 I-273 80 80 I-274 80 90 I-275 80 90 I-276 80 80 I-278 80 80 I-279 80 80 I-285 80 80 I-287 80 80 I-288 80 80 I-289 80 80 I-29 80 80 I-290 80 80 I-294 80 90 I-298 80 80 I-299 80 80 I-304 80 80 I-307 80 90 I-308 80 90 I-309 80 80 I-313 80 90 I-314 80 90 I-315 80 80 I-316 80 90 I-317 80 90 I-318 80 90 I-32 80 80 I-322 80 80 I-323 80 90 I-324 80 90 I-325 80 80 I-326 80 90 I-327 80 80 I-328 80 90 I-33 80 90 I-330 80 80 I-331 80 90 I-335 80 90 I-336 80 80 I-337 80 80 I-339 80 80 I-34 80 90 I-340 80 80 I-341 80 90 I-342 80 90 I-343 80 80 I-344 80 90 I-348 80 80 I-35 80 100 I-352 80 80 I-360 80 80 I-366 80 80 I-369 80 80 I-37 80 80 I-370 80 90 I-374 80 80 I-375 80 80 I-38 80 80 I-380 80 80 I-382 80 80 I-383 80 80 I-388 80 80 I-39 80 80 I-40 80 80 I-41 80 80 I-42 80 90 I-44 80 80 I-45 80 80 I-46 80 80 I-48 80 90 I-51 80 80 I-52 80 90 I-53 80 80 I-56 80 80 I-59 80 90 I-64 80 90 I-66 80 90 I-73 80 80 I-74 80 80 I-75 80 80 I-76 80 80 I-77 80 90 I-79 80 80 I-81 80 90 I-83 80 80 I-84 80 80 I-85 80 90 I-87 80 80 I-88 80 80 I-90 80 90 I-91 80 80 I-93 80 80 I-95 80 80 I-96 80 80 I-97 80 90 I-98 80 80 I-99 80 80 II-38 80 80 II-39 80 80 II-40 80 80 II-41 80 90 II-42 80 80 II-43 80 90 II-44 80 80 II-45 80 90 III-22 80 80
TABLE-US-00069 TABLE B12b Post-emergence action at 320 g/ha against VERPE in % Example number Dosage [g/ha] VERPE I-01 320 90 I-02 320 80 I-03 320 90 I-05 320 90 I-07 320 90 I-08 320 90 I-10 320 80 I-11 320 80 I-13 320 80 I-130 320 80 I-133 320 80 I-134 320 80 I-137 320 80 I-138 320 80 I-139 320 90 I-140 320 90 I-141 320 90 I-144 320 90 I-145 320 90 I-146 320 90 I-148 320 80 I-149 320 80 I-15 320 80 I-151 320 90 I-152 320 80 I-155 320 80 I-156 320 80 I-157 320 90 I-16 320 90 I-160 320 90 I-161 320 80 I-162 320 90 I-164 320 80 I-165 320 90 I-166 320 80 I-167 320 80 I-168 320 90 I-169 320 90 I-17 320 80 I-171 320 90 I-172 320 90 I-174 320 80 I-175 320 80 I-177 320 100 I-179 320 90 I-180 320 90 I-181 320 90 I-182 320 90 I-183 320 90 I-184 320 90 I-185 320 80 I-186 320 80 I-187 320 90 I-188 320 90 I-189 320 90 I-190 320 90 I-191 320 90 I-192 320 80 I-193 320 80 I-194 320 80 I-195 320 80 I-196 320 90 I-197 320 90 I-198 320 80 I-199 320 90 I-20 320 80 I-202 320 80 I-204 320 90 I-206 320 80 I-207 320 90 I-208 320 80 I-210 320 90 I-211 320 90 I-212 320 80 I-218 320 80 I-223 320 80 I-225 320 90 I-227 320 90 I-230 320 80 I-231 320 80 I-235 320 80 I-236 320 80 I-239 320 80 I-241 320 80 I-243 320 80 I-246 320 80 I-247 320 80 I-248 320 80 I-249 320 80 I-251 320 90 I-252 320 80 I-26 320 80 I-260 320 80 I-261 320 80 I-264 320 90 I-266 320 90 I-267 320 90 I-268 320 80 I-27 320 90 I-272 320 80 I-273 320 90 I-274 320 90 I-275 320 90 I-276 320 90 I-277 320 80 I-278 320 90 I-279 320 90 I-28 320 80 I-285 320 80 I-287 320 80 I-288 320 80 I-289 320 80 I-290 320 80 I-291 320 80 I-294 320 90 I-296 320 80 I-297 320 80 I-298 320 80 I-299 320 80 I-300 320 80 I-302 320 80 I-304 320 90 I-305 320 90 I-306 320 90 I-307 320 90 I-308 320 90 I-309 320 80 I-310 320 80 I-311 320 90 I-312 320 80 I-313 320 90 I-314 320 90 I-315 320 90 I-316 320 90 I-317 320 90 I-318 320 90 I-319 320 80 I-320 320 90 I-321 320 90 I-322 320 80 I-323 320 90 I-324 320 90 I-325 320 90 I-326 320 90 I-327 320 90 I-328 320 90 I-330 320 80 I-331 320 90 I-332 320 80 I-333 320 90 I-334 320 80 I-335 320 90 I-336 320 90 I-337 320 80 I-338 320 90 I-339 320 90 I-340 320 90 I-341 320 90 I-342 320 90 I-343 320 80 I-344 320 90 I-345 320 80 I-348 320 80 I-350 320 90 I-351 320 80 I-352 320 80 I-354 320 90 I-358 320 80 I-360 320 80 I-366 320 90 I-369 320 80 I-370 320 90 I-373 320 90 I-375 320 90 I-376 320 80 I-377 320 80 I-378 320 80 I-380 320 90 I-381 320 80 I-382 320 80 I-383 320 90 I-388 320 80 I-41 320 80 I-42 320 90 I-48 320 90 I-66 320 90 I-80 320 80 I-85 320 90 I-86 320 80 I-87 320 90 I-88 320 80 I-94 320 90 I-95 320 80 I-96 320 90 II-37 320 90 II-38 320 90 II-39 320 90 II-40 320 90 II-41 320 90 II-42 320 90 II-43 320 90 II-44 320 90 II-45 320 90 II-46 320 90 III-01 320 80 III-22 320 90 III-23 320 90 III-24 320 80 III-29 320 80 III-30 320 80
TABLE-US-00070 TABLE B13a Post-emergence action at 80 g/ha against VIOTR in % Example number Dosage [g/ha] VIOTR I-01 80 90 I-03 80 90 I-05 80 100 I-07 80 90 I-08 80 80 I-101 80 80 I-121 80 80 I-130 80 90 I-133 80 80 I-136 80 80 I-137 80 80 I-138 80 80 I-139 80 80 I-140 80 90 I-141 80 80 I-144 80 90 I-145 80 90 I-146 80 90 I-148 80 80 I-149 80 80 I-151 80 80 I-155 80 80 I-16 80 80 I-165 80 90 I-166 80 80 I-167 80 80 I-168 80 80 I-17 80 80 I-171 80 90 I-172 80 80 I-174 80 80 I-175 80 80 I-177 80 100 I-179 80 90 I-180 80 80 I-181 80 90 I-182 80 80 I-183 80 90 I-184 80 80 I-185 80 80 I-187 80 80 I-188 80 80 I-189 80 90 I-19 80 90 I-190 80 80 I-193 80 80 I-194 80 80 I-195 80 80 I-196 80 80 I-197 80 90 I-199 80 80 I-20 80 90 I-202 80 80 I-204 80 80 I-208 80 80 I-211 80 80 I-212 80 80 I-216 80 80 I-217 80 80 I-218 80 80 I-221 80 80 I-225 80 80 I-227 80 90 I-229 80 80 I-235 80 80 I-239 80 80 I-242 80 80 I-244 80 80 I-246 80 80 I-247 80 80 I-248 80 80 I-249 80 80 I-264 80 90 I-266 80 80 I-267 80 90 I-268 80 80 I-27 80 80 I-273 80 90 I-274 80 80 I-275 80 90 I-28 80 80 I-285 80 80 I-287 80 80 I-289 80 80 I-291 80 80 I-293 80 80 I-294 80 90 I-296 80 80 I-298 80 80 I-299 80 80 I-30 80 80 I-300 80 80 I-304 80 80 I-307 80 80 I-308 80 90 I-310 80 80 I-311 80 80 I-314 80 90 I-316 80 90 I-317 80 90 I-318 80 80 I-319 80 80 I-32 80 80 I-321 80 80 I-322 80 80 I-323 80 90 I-324 80 80 I-325 80 90 I-326 80 90 I-327 80 90 I-328 80 80 I-331 80 80 I-334 80 80 I-335 80 80 I-337 80 80 I-339 80 90 I-340 80 90 I-341 80 80 I-342 80 90 I-343 80 80 I-344 80 80 I-347 80 80 I-348 80 80 I-35 80 90 I-350 80 90 I-354 80 80 I-358 80 90 I-36 80 90 I-362 80 80 I-366 80 80 I-369 80 80 I-375 80 80 I-38 80 80 I-380 80 90 I-382 80 80 I-383 80 80 I-39 80 80 I-41 80 80 I-42 80 90 I-48 80 80 I-51 80 80 I-56 80 80 I-59 80 80 I-64 80 80 I-66 80 80 I-69 80 80 I-85 80 100 I-86 80 80 I-94 80 90 I-96 80 90 I-97 80 80 II-36 80 80 II-38 80 90 II-39 80 80 II-40 80 90 II-41 80 80 II-42 80 80 II-43 80 90 II-44 80 80 II-45 80 90 III-22 80 90 III-24 80 80
TABLE-US-00071 TABLE B13b Post-emergence action at 320 g/ha against VIOTR in % Example number Dosage [g/ha] VIOTR I-01 320 100 I-02 320 80 I-03 320 90 I-04 320 80 I-05 320 100 I-07 320 90 I-08 320 80 I-10 320 80 I-11 320 80 I-13 320 80 I-130 320 90 I-133 320 90 I-136 320 80 I-137 320 80 I-138 320 80 I-139 320 90 I-140 320 90 I-141 320 80 I-144 320 90 I-145 320 90 I-146 320 90 I-147 320 90 I-148 320 80 I-149 320 80 I-15 320 80 I-150 320 80 I-151 320 90 I-153 320 80 I-154 320 80 I-155 320 80 I-159 320 80 I-16 320 80 I-161 320 80 I-163 320 80 I-164 320 80 I-165 320 90 I-166 320 80 I-167 320 80 I-168 320 90 I-169 320 80 I-17 320 80 I-171 320 90 I-172 320 90 I-174 320 80 I-175 320 80 I-176 320 80 I-177 320 100 I-179 320 90 I-18 320 80 I-180 320 80 I-181 320 90 I-182 320 90 I-183 320 90 I-184 320 90 I-185 320 80 I-187 320 90 I-188 320 80 I-189 320 90 I-190 320 90 I-191 320 80 I-192 320 80 I-193 320 90 I-194 320 80 I-195 320 80 I-196 320 80 I-197 320 90 I-198 320 80 I-199 320 80 I-20 320 90 I-202 320 80 I-204 320 80 I-206 320 80 I-207 320 80 I-208 320 80 I-211 320 90 I-212 320 80 I-216 320 80 I-217 320 90 I-218 320 80 I-221 320 80 I-223 320 80 I-225 320 80 I-227 320 90 I-229 320 80 I-230 320 80 I-231 320 80 I-235 320 80 I-237 320 80 I-238 320 80 I-239 320 80 I-240 320 80 I-241 320 80 I-242 320 80 I-243 320 80 I-244 320 80 I-245 320 80 I-246 320 80 I-247 320 80 I-248 320 80 I-249 320 80 I-251 320 90 I-252 320 80 I-26 320 80 I-261 320 80 I-264 320 90 I-266 320 90 I-267 320 90 I-268 320 80 I-27 320 80 I-273 320 90 I-274 320 90 I-275 320 90 I-28 320 80 I--284 320 80 I-285 320 80 I-286 320 80 I-287 320 90 I-288 320 80 I-289 320 80 I-290 320 80 I-291 320 80 I-293 320 80 I-294 320 90 I-296 320 80 I-298 320 90 I-299 320 90 I-300 320 90 I-302 320 80 I-304 320 90 I-306 320 80 I-307 320 90 I-308 320 90 I-31 320 80 I-310 320 90 I-311 320 80 I-313 320 80 I-314 320 90 I-315 320 80 I-316 320 90 I-317 320 90 I-318 320 90 I-319 320 90 I-320 320 80 I-321 320 80 I-322 320 80 I-323 320 90 I-324 320 80 I-325 320 90 I-326 320 90 I-327 320 90 I-328 320 90 I-330 320 80 I-331 320 80 I-332 320 80 I-333 320 80 I-334 320 80 I-335 320 90 I-336 320 80 I-337 320 80 I-338 320 80 I-339 320 90 I-340 320 90 I-341 320 80 I-342 320 90 I-343 320 80 I-344 320 80 I-347 320 80 I-348 320 80 I-349 320 80 I-350 320 90 I-354 320 80 I-358 320 90 I-362 320 80 I-366 320 90 I-369 320 80 I-370 320 80 I-375 320 90 I-376 320 80 I-380 320 90 I-382 320 90 I-383 320 90 I-388 320 80 I-41 320 80 I-42 320 90 I-48 320 90 I-66 320 90 I-69 320 80 I-82 320 80 I-85 320 100 I-86 320 90 I-94 320 90 I-95 320 80 I-96 320 90 II-37 320 80 II-38 320 90 II-39 320 90 II-40 320 90 II-41 320 90 II-42 320 90 II-43 320 90 II-44 320 90 II-45 320 90 II-46 320 90 III-01 320 80 III-08 320 80 III-22 320 90 III-23 320 90 III-24 320 90 III-27 320 80 III-30 320 80
[0569] Tables B14 to B18 below show the crop plant compatibilities of selected compounds of the general formula (I) according to Table 1 at an application rate corresponding to 320 g/ha or less, which were observed in trials by the experimental procedure mentioned above. The observed effects on selected crop plants are reported here in comparison to the untreated controls (values in %). The appendices a, b and c give differentiation by dosage used with otherwise the same crop plants tested.
TABLE-US-00072 TABLE B14a Post-emergence action at 20 g/ha against ZEAMX in % Example number Dosage [g/ha] ZEAMX I-01 20 0 I-11 20 10 I-16 20 10 I-13 20 0 I-17 20 10 I-19 20 0 I-126 20 10 I-39 20 0 I-55 20 0 I-54 20 0 I-36 20 20 I-56 20 0 I-122 20 0 I-100 20 10 I-102 20 0 I-101 20 10 I-33 20 10 I-32 20 20 I-107 20 20 I-99 20 0 I-98 20 10 I-91 20 20 I-93 20 20 I-90 20 0 I-29 20 10 I-46 20 0 I-30 20 20 I-45 20 0 I-44 20 0 I-23 20 0 I-24 20 10 I-47 20 10 I-116 20 20 I-53 20 10 I-374 20 10 I-114 20 0 I-119 20 10 I-108 20 0 I-109 20 10 I-110 20 10 I-112 20 0 I-25 20 10 I-52 20 0 I-35 20 10 I-34 20 10 I-51 20 20 I-50 20 0 I-49 20 0 III-21 20 0 III-20 20 0 III-19 20 0 I-81 20 0 III-17 20 20 I-75 20 10 I-74 20 10 I-77 20 0 I-76 20 20 III-18 20 0 I-40 20 0 I-71 20 0 I-70 20 0 I-43 20 10 III-29 20 10 I-252 20 10 I-314 20 0 I-344 20 0 I-328 20 0 I-318 20 0 I-326 20 0 I-299 20 0 II-44 20 0 II-38 20 0 II-40 20 0 II-41 20 0 II-43 20 0 II-39 20 0 II-37 20 0 II-42 20 20 I-286 20 10 I-290 20 0 I-169 20 10 I-136 20 10 I-134 20 10 I-168 20 20 I-166 20 10 I-285 20 10 II-46 20 0 I-139 20 0 I-137 20 0 I-138 20 20 I-130 20 0 I-133 20 0 I-181 20 20 I-182 20 10 I-304 20 20 I-383 20 10 I-294 20 20 I-251 20 20 I-366 20 10 I-382 20 0 I-380 20 0 I-287 20 10 I-264 20 10 I-274 20 10 I-289 20 0 I-275 20 0 I-267 20 0 I-387 20 0 I-249 20 0 I-261 20 0 I-268 20 0 I-248 20 0 I--284 20 0
TABLE-US-00073 TABLE B14b Post-emergence action at 80 g/ha against ZEAMX in % Example number Dosage [g/ha] ZEAMX I-01 80 0 I-03 80 0 I-04 80 0 I-05 80 0 I-07 80 0 I-10 80 0 I-101 80 10 I-102 80 20 I-108 80 10 I-109 80 10 I-110 80 10 I-112 80 10 I-114 80 0 I-130 80 0 I-133 80 0 I-136 80 10 I-137 80 0 I-138 80 20 I-139 80 0 I-147 80 0 I-150 80 0 I-153 80 10 I-157 80 20 I-16 80 20 I-161 80 10 I-169 80 10 I-179 80 20 I-182 80 20 I-186 80 20 I-200 80 0 I-201 80 0 I-205 80 0 I-225 80 20 I-23 80 10 I-230 80 0 I-235 80 20 I-236 80 0 I-237 80 10 I-238 80 10 I-239 80 0 I-24 80 20 I-240 80 10 I-241 80 0 I-242 80 10 I-243 80 0 I-244 80 20 I-246 80 10 I-248 80 0 I-249 80 20 I-25 80 20 I-251 80 20 I-26 80 0 I-261 80 0 I-264 80 20 I-267 80 20 I-268 80 0 I-272 80 10 I-274 80 20 I-275 80 20 I-277 80 10 I-278 80 20 I-28 80 0 I--284 80 0 I-286 80 20 I-287 80 20 I-289 80 10 I-29 80 20 I-290 80 10 I-299 80 10 I-30 80 20 I-302 80 0 I-305 80 0 I-31 80 0 I-310 80 0 I-311 80 10 I-312 80 10 I-314 80 10 I-315 80 20 I-316 80 0 I-318 80 0 I-319 80 10 I-320 80 0 I-321 80 0 I-323 80 0 I-324 80 0 I-325 80 0 I-326 80 0 I-327 80 0 I-328 80 0 I-329 80 0 I-330 80 10 I-332 80 10 I-334 80 10 I-335 80 0 I-337 80 10 I-338 80 0 I-34 80 10 I-341 80 0 I-344 80 0 I-345 80 0 I-346 80 0 I-347 80 20 I-348 80 20 I-35 80 10 I-351 80 10 I-354 80 0 I-357 80 0 I-358 80 0 I-362 80 0 I-363 80 0 I-369 80 10 I-371 80 20 I-373 80 0 I-376 80 10 I-377 80 0 I-378 80 10 I-380 80 20 I-381 80 0 I-382 80 20 I-383 80 20 I-386 80 0 I-387 80 0 I-40 80 20 I-41 80 20 I-43 80 10 I-44 80 10 I-45 80 10 I-46 80 10 I-47 80 10 I-48 80 20 I-49 80 10 I-50 80 0 I-52 80 10 I-55 80 0 I-56 80 0 I-58 80 20 I-63 80 0 I-70 80 10 I-71 80 10 I-75 80 20 I-80 80 20 I-81 80 0 I-90 80 10 I-94 80 20 II-37 80 0 II-38 80 0 II-39 80 0 II-40 80 0 II-41 80 0 II-43 80 20 II-44 80 0 II-46 80 0 III-01 80 0 III-02 80 10 III-07 80 0 III-09 80 10 III-17 80 20 III-18 80 0 III-21 80 0 III-23 80 0 III-25 80 0 III-26 80 20 III-27 80 10 III-28 80 0 III-30 80 20 I-10 320 20 I-130 320 20 I-133 320 20 I-136 320 20 I-137 320 20 I-139 320 10 I-147 320 20 I-150 320 0 I-161 320 10 I-200 320 0 I-201 320 20 I-205 320 0 I-239 320 20 I-240 320 20 I--284 320 0 I-297 320 0 I-302 320 10 I-31 320 0 I-320 320 20 I-329 320 0 I-334 320 20 I-335 320 20 I-345 320 10 I-346 320 0 I-357 320 10 I-363 320 0 I-371 320 20 I-386 320 0 I-387 320 0 I-62 320 20 I-63 320 10 II-37 320 0 II-38 320 0 II-39 320 20 II-40 320 10 II-46 320 20 III-01 320 0 III-02 320 20 III-07 320 0 III-09 320 10 III-25 320 0 III-27 320 10 III-28 320 0
TABLE-US-00074 TABLE B15a Post-emergence action at 20 g/ha against TRZAS in % Example number Dosage [g/ha] TRZAS I-103 20 0 I-108 20 0 I-109 20 0 I-110 20 0 I-112 20 0 I-114 20 0 I-119 20 20 I-125 20 10 I-126 20 20 I-130 20 20 I-134 20 20 I-136 20 10 I-137 20 20 I-138 20 10 I-139 20 0 I-140 20 10 I-145 20 20 I-16 20 20 I-165 20 20 I-168 20 10 I-169 20 0 I-17 20 10 I-179 20 0 I-181 20 20 I-182 20 10 I-248 20 0 I-249 20 0 I-251 20 10 I-261 20 0 I-266 20 20 I-268 20 0 I-273 20 0 I--284 20 0 I-286 20 20 I-287 20 20 I-289 20 20 I-294 20 10 I-380 20 20 I-383 20 20 I-387 20 0 I-44 20 20 I-47 20 10 I-49 20 0 I-50 20 10 I-51 20 20 I-55 20 0 I-70 20 0 I-71 20 10 I-72 20 10 I-74 20 0 I-75 20 20 I-78 20 0 I-99 20 20 II-37 20 0 II-38 20 0 II-39 20 0 II-40 20 0 II-41 20 0 II-42 20 0 II-43 20 10 II-44 20 20 II-45 20 0 II-46 20 0 III-17 20 20 III-18 20 0 III-19 20 20 III-20 20 0 III-21 20 0 III-29 20 20
TABLE-US-00075 TABLE 15b Post-emergence action at 80 g/ha against TRZAS in % Example number Dosage [g/ha] TRZAS I-04 80 20 I-108 80 20 I-109 80 10 I-111 80 0 I-112 80 0 I-114 80 0 I-137 80 20 I-147 80 0 I-150 80 0 I-160 80 20 I-161 80 0 I-162 80 10 I-186 80 10 I-187 80 20 I-200 80 0 I-201 80 0 I-202 80 20 I-205 80 10 I-225 80 20 I-230 80 10 I-243 80 20 I-248 80 0 I-249 80 0 I-261 80 0 I-268 80 0 I-276 80 0 I-277 80 0 I-278 80 0 I-279 80 10 I--284 80 0 I-297 80 10 I-31 80 10 I-312 80 20 I-329 80 0 I-345 80 10 I-346 80 10 I-351 80 0 I-352 80 10 I-354 80 0 I-357 80 10 I-363 80 0 I-371 80 20 I-376 80 0 I-377 80 0 I-387 80 0 I-49 80 10 I-50 80 10 I-55 80 0 I-62 80 0 I-63 80 0 I-69 80 0 I-70 80 10 I-78 80 20 II-37 80 0 II-38 80 10 II-39 80 20 II-40 80 20 II-41 80 0 II-42 80 20 II-44 80 20 II-46 80 0 III-01 80 0 III-02 80 20 III-07 80 0 III-08 80 0 III-09 80 0 III-18 80 0 III-20 80 0 III-21 80 0 III-23 80 0 III-24 80 0 III-25 80 0 III-26 80 20
TABLE-US-00076 TABLE B15c Post-emergence action at 320 g/ha against TRZAS in % Example number Dosage [g/ha] TRZAS I-147 320 20 I-150 320 10 I-161 320 10 I-200 320 0 I-201 320 10 I-205 320 10 I-249 320 0 I-276 320 20 I-277 320 20 I--284 320 0 I-351 320 10 I-357 320 10 I-376 320 20 I-387 320 0 I-62 320 0 I-63 320 0 II-37 320 0 III-09 320 0 III-24 320 0
TABLE-US-00077 TABLE B16a Post-emergence action at 20 g/ha against ORYSA in % Example number Dosage [g/ha] ORYSA I-01 20 0 I-100 20 0 I-101 20 0 I-102 20 0 I-103 20 0 I-107 20 0 I-108 20 0 I-109 20 0 I-11 20 0 I-110 20 0 I-112 20 0 I-114 20 0 I-116 20 10 I-118 20 0 I-119 20 0 I-120 20 10 I-121 20 0 I-122 20 0 I-125 20 0 I-126 20 0 I-13 20 0 I-130 20 0 I-133 20 0 I-134 20 0 I-136 20 10 I-137 20 0 I-138 20 0 I-139 20 0 I-140 20 0 I-141 20 10 I-144 20 0 I-145 20 0 I-146 20 0 I-15 20 0 I-16 20 0 I-165 20 0 I-166 20 0 I-168 20 10 I-169 20 0 I-17 20 0 I-172 20 20 I-176 20 0 I-177 20 0 I-179 20 0 I-18 20 0 I-181 20 0 I-182 20 10 I-19 20 0 I-197 20 0 I-227 20 0 I-23 20 0 I-24 20 0 I-25 20 0 I-251 20 10 I-252 20 10 I-260 20 10 I-264 20 0 I-266 20 20 I-274 20 0 I-285 20 10 I-286 20 10 I-287 20 0 I-288 20 0 I-289 20 0 I-29 20 10 I-290 20 0 I-294 20 10 I-299 20 10 I-314 20 0 I-318 20 0 I-32 20 0 I-326 20 0 I-328 20 0 I-33 20 0 I-34 20 10 I-344 20 0 I-35 20 0 I-36 20 0 I-366 20 0 I-374 20 10 I-380 20 0 I-382 20 0 I-39 20 0 I-43 20 10 I-44 20 20 I-45 20 10 I-46 20 10 I-47 20 20 I-49 20 0 I-50 20 10 I-51 20 20 I-52 20 0 I-53 20 10 I-54 20 0 I-55 20 0 I-56 20 0 I-59 20 0 I-64 20 10 I-70 20 0 I-71 20 10 I-72 20 10 I-73 20 0 I-74 20 0 I-75 20 0 I-76 20 0 I-77 20 0 I-78 20 0 I-79 20 0 I-81 20 0 I-83 20 0 I-84 20 0 I-90 20 0 I-91 20 0 I-93 20 10 I-97 20 0 I-98 20 10 I-99 20 0 II-36 20 0 II-37 20 0 II-38 20 0 II-39 20 0 II-40 20 0 II-41 20 0 II-42 20 0 II-43 20 0 II-44 20 0 II-45 20 0 II-46 20 0 III-17 20 0 III-18 20 0 III-19 20 0 III-20 20 0 III-21 20 0 III-29 20 10
TABLE-US-00078 TABLE B16b Post-emergence action at 80 g/ha against ORYSA in % Example number Dosage [g/ha] ORYSA I-01 80 0 I-03 80 0 I-04 80 0 I-05 80 0 I-07 80 0 I-101 80 10 I-102 80 0 I-103 80 0 I-107 80 10 I-108 80 10 I-109 80 0 I-11 80 0 I-110 80 10 I-111 80 0 I-112 80 0 I-114 80 0 I-116 80 10 I-118 80 0 I-119 80 10 I-120 80 20 I-121 80 0 I-122 80 0 I-125 80 0 I-126 80 0 I-13 80 10 I-133 80 10 I-134 80 10 I-136 80 20 I-137 80 10 I-138 80 0 I-139 80 0 I-140 80 0 I-147 80 0 I-15 80 10 I-150 80 0 I-151 80 0 I-152 80 0 I-153 80 0 I-155 80 10 I-156 80 0 I-157 80 10 I-159 80 10 I-16 80 10 I-160 80 0 I-161 80 0 I-162 80 0 I-166 80 20 I-169 80 10 I-17 80 10 I-175 80 20 I-176 80 10 I-179 80 20 I-18 80 10 I-185 80 20 I-186 80 10 I-187 80 10 I-188 80 20 I-19 80 0 I-190 80 20 I-192 80 0 I-193 80 10 I-194 80 20 I-197 80 10 I-200 80 0 I-201 80 0 I-202 80 20 I-204 80 0 I-205 80 0 I-207 80 10 I-208 80 0 I-210 80 10 I-212 80 10 I-216 80 10 I-217 80 0 I-221 80 20 I-223 80 10 I-225 80 10 I-229 80 0 I-23 80 10 I-230 80 0 I-231 80 10 I-235 80 0 I-236 80 0 I-237 80 0 I-238 80 0 I-239 80 0 I-24 80 10 I-240 80 0 I-241 80 0 I-242 80 0 I-243 80 0 I-245 80 0 I-246 80 0 I-247 80 10 I-25 80 10 I-260 80 10 I-264 80 10 I-27 80 0 I-272 80 10 I-276 80 10 I-277 80 10 I-278 80 0 I-279 80 10 I-28 80 0 I-285 80 10 I-286 80 20 I-287 80 20 I-288 80 10 I-289 80 10 I-29 80 20 I-290 80 10 I-291 80 0 I-293 80 0 I-296 80 0 I-298 80 20 I-299 80 20 I-302 80 20 I-306 80 0 I-31 80 0 I-310 80 10 I-311 80 20 I-312 80 10 I-313 80 10 I-314 80 20 I-315 80 20 I-319 80 0 I-32 80 0 I-320 80 0 I-321 80 0 I-322 80 10 I-325 80 20 I-327 80 0 I-329 80 0 I-33 80 10 I-330 80 10 I-332 80 20 I-333 80 20 I-334 80 20 I-335 80 0 I-336 80 20 I-337 80 20 I-338 80 0 I-339 80 0 I-34 80 20 I-340 80 0 I-341 80 0 I-343 80 10 I-344 80 0 I-345 80 20 I-346 80 0 I-347 80 0 I-348 80 0 I-349 80 0 I-35 80 0 I-350 80 0 I-351 80 0 I-352 80 20 I-357 80 0 I-358 80 0 I-359 80 0 I-36 80 0 I-360 80 20 I-362 80 10 I-363 80 0 I-366 80 20 I-369 80 20 I-370 80 0 I-371 80 0 I-373 80 0 I-376 80 0 I-377 80 0 I-378 80 10 I-380 80 10 I-381 80 20 I-382 80 10 I-386 80 0 I-41 80 0 I-47 80 20 I-49 80 10 I-50 80 10 I-52 80 10 I-54 80 0 I-55 80 0 I-56 80 0 I-58 80 0 I-59 80 0 I-60 80 0 I-62 80 0 I-63 80 0 I-65 80 0 I-66 80 10 I-69 80 0 I-70 80 0 I-71 80 20 I-72 80 20 I-73 80 10 I-74 80 10 I-75 80 0 I-76 80 0 I-78 80 20 I-79 80 0 I-80 80 20 I-81 80 0 I-82 80 20 I-83 80 20 I-84 80 10 I-87 80 0 I-88 80 0 I-90 80 0 I-91 80 20 I-93 80 20 I-94 80 20 I-95 80 0 I-97 80 10 I-99 80 0 II-36 80 0 II-37 80 0 II-38 80 0 II-39 80 0 II-40 80 0 II-41 80 0 II-42 80 0 II-43 80 0 II-44 80 0 II-45 80 0 II-46 80 0 III-01 80 0 III-02 80 0 III-07 80 0 III-08 80 0 III-09 80 0 III-17 80 0 III-18 80 0 III-19 80 0 III-20 80 0 III-21 80 20 III-22 80 0 III-23 80 0 III-24 80 0 III-25 80 0 III-26 80 10 III-27 80 0 III-28 80 0 III-29 80 20 III-30 80 10
TABLE-US-00079 TABLE B16c Post-emergence action at 320 g/ha against ORYSA in % Example number Dosage [g/ha] ORYSA I-04 320 0 I-11 320 10 I-111 320 0 I-137 320 20 I-138 320 20 I-139 320 10 I-140 320 10 I-147 320 0 I-150 320 0 I-161 320 0 I-18 320 20 I-186 320 20 I-187 320 20 I-200 320 0 I-201 320 0 I-205 320 10 I-223 320 20 I-235 320 0 I-236 320 0 I-237 320 20 I-238 320 10 I-240 320 0 I-241 320 0 I-242 320 0 I-243 320 10 I-244 320 0 I-246 320 10 I-278 320 10 I-286 320 20 I-31 320 10 I-310 320 20 I-329 320 0 I-340 320 0 I-346 320 0 I-347 320 0 I-349 320 10 I-350 320 10 I-357 320 10 I-358 320 0 I-359 320 0 I-363 320 0 I-371 320 0 I-376 320 20 I-381 320 20 I-386 320 0 I-60 320 0 I-62 320 0 I-63 320 10 I-65 320 0 I-66 320 20 I-69 320 10 I-80 320 20 II-37 320 0 II-38 320 0 II-39 320 0 II-40 320 0 II-41 320 0 II-42 320 0 II-43 320 0 II-46 320 0 III-01 320 0 III-02 320 20 III-07 320 0 III-08 320 0 III-09 320 0 III-23 320 20 III-25 320 0 III-26 320 20 III-27 320 0 III-28 320 0 III-30 320 20
TABLE-US-00080 TABLE B17a Post-emergence action at 20 g/ha against GLXMA in % Example number Dosage [g/ha] GLXMA I-108 20 0 I-112 20 0 I-114 20 0 I-125 20 20 I-126 20 20 I-261 20 0 I--284 20 0 I-49 20 10 I-50 20 0 I-55 20 0 II-37 20 0 III-20 20 0 III-21 20 0
TABLE-US-00081 TABLE B17b Post-emergence action at 80 g/ha against GLXMA in % Example number Dosage [g/ha] GLXMA I-108 80 10 I-112 80 10 I-114 80 0 I-147 80 0 I-150 80 0 I-161 80 0 I-200 80 0 I-201 80 20 I--284 80 0 I-349 80 0 I-50 80 10 I-55 80 0 I-82 80 0 III-20 80 0 III-21 80 0
TABLE-US-00082 TABLE B17c Post-emergence action at 320 g/ha against GLXMA in % Example number Dosage [g/ha] GLXMA I-147 320 10 I-150 320 0 I-200 320 0 I--284 320 0
TABLE-US-00083 TABLE B18a Post-emergence action at 20 g/ha against BRSNW in % Example number Dosage [g/ha] BRSNW I-108 20 10 I-109 20 0 I-110 20 10 I-112 20 0 I--284 20 0 I-289 20 20 I-47 20 10 I-50 20 10 I-55 20 0 I-70 20 20 II-37 20 0 III-20 20 0 III-21 20 0
TABLE-US-00084 TABLE B18b Post-emergence action at 80 g/ha against BRSNW in % Example number Dosage [g/ha] BRSNW I-109 80 10 I-110 80 20 I-112 80 10 I-200 80 10 I--284 80 0 I-349 80 20 I-50 80 20 I-55 80 0 I-62 80 20 III-21 80 0
TABLE-US-00085 TABLE B18c Post-emergence action at 320 g/ha against BRSNW in % Example number Dosage [g/ha] BRSNW I-200 320 20 I--284 320 0
[0570] As the results from Tables B1 to B18 show, inventive compounds of the general formula (I) in the case of post-emergence treatment have good herbicidal efficacy against harmful plants, for example Abutilon theophrasti (ABUTH), Alopecurus myosuroides (ALOMY), Amaranthus retroflexus (AMARE), Avena fatua (AVEFA), Digitaria sanguinalis (DIGSA), Echinochloa crus-galli (ECHCG), Lolium rigidum (LOLRI), Matricaria inodora (MATIN), Pharbitis purpurea (PHBPU), Polygonum convolvulus (POLCO), Setaria viridis (SETVI), Verconica persica (VERPE) and Viola tricolor (VIOTR) at an application rate of 320 g of active substance or less per hectare, and good crop plant compatibility in the case of organisms such as Oryza sativa (ORYSA), Zea mays (ZEAMX), Brassica napus (BRSNW), Glycine max (GLXMA) and Triticum aestivum (TRZAS) at an application rate of 320 g or less per hectare.
[0571] The compounds of the invention are therefore suitable for control of unwanted plant growth by the post-emergence method.