Spin-orbit qubit using quantum dots
10482388 ยท 2019-11-19
Assignee
Inventors
- Ryan Michael Jock (Albuquerque, NM, US)
- Martin Rudolph (Albuquerque, NM, US)
- Andrew David Baczewski (Albuquerque, NM, US)
- Wayne Witzel (Albuquerque, NM, US)
- Malcom S. Carroll (Albuquerque, NM, US)
- Patrick Harvey-Collard (Magog, CA)
- John King Gamble, IV (Redmond, WA, US)
- Noah Tobias Jacobson (Albuquerque, NM, US)
- Andrew Mounce (Albuquerque, NM, US)
- Daniel Robert Ward (Albuquerque, NM, US)
Cpc classification
G06N10/40
PHYSICS
B82Y10/00
PERFORMING OPERATIONS; TRANSPORTING
H01L29/423
ELECTRICITY
H01L29/16
ELECTRICITY
H01L29/7613
ELECTRICITY
H01L29/045
ELECTRICITY
H01L29/66977
ELECTRICITY
H01L29/82
ELECTRICITY
International classification
G06N10/00
PHYSICS
Abstract
Methods and apparatus of quantum information processing using quantum dots are provided. Electrons from a 2DEG are confined to the quantum dots and subjected to a magnetic field having a component directed parallel to the interface. Due to interfacial asymmetries, there is created an effective magnetic field that perturbs the energies of the spin states via an interfacial spin-orbit (SO) interaction. This SO interaction is utilized to controllably produce rotations of the electronic spin state, such as X-rotations of the electronic spin state in a double quantum dot (DQD) singlet-triplet (ST) qubit. The desired state rotations are controlled solely by the use of electrical pulses.
Claims
1. A method of quantum information processing using a lateral double quantum dot (DQD) disposed at a substrate surface and having a first quantum dot (QD.sub.1) tunnel-coupled to a second quantum dot (QD.sub.2), comprising: populating QD.sub.1 with two confined electrons; transferring one confined electron to QD.sub.2 to create a (1, 1) charge state; performing at least two state rotations on the confined electrons while the DQD is in the (1, 1) charge state; and reading out a final quantum state of the DQD, wherein: the at least two state rotations are performed while exposing the DQD to an externally sourced magnetic field having a component directed parallel to the substrate surface; the performing of each of the at least two state rotations consists of applying a voltage pulse sequence to a planar gate electrode or combination of planar gate electrodes that is electrostatically coupled to the confined electrons so as to vary a relative tuning between QD.sub.1 and QD.sub.2; at least a first one of the voltage pulse sequences comprises maintaining, for a first specified duration, a first relative tuning between QD.sub.1 and QD.sub.2; and at least a second one of the voltage pulse sequences comprises maintaining, for a second specified duration, a second relative tuning between QD.sub.1 and QD.sub.2 that is different from the first relative tuning.
2. The method of claim 1, wherein QD.sub.1 and QD.sub.2 are laterally disposed relative to each other.
3. The method of claim 1, wherein the populating, transferring, state-rotation-performing, and readout steps are cyclically repeated multiple times.
4. The method of claim 1, further comprising forming QD.sub.1 and QD.sub.2 by applying voltages to planar gate electrodes that overlie the substrate surface.
5. The method of claim 1, wherein the substrate surface is a surface of a silicon body, and wherein the surface of the silicon body is directly overlain by a layer of silicon oxide.
6. The method of claim 1, wherein the state-rotating voltage-pulse sequences are applied to a single layer of polysilicon planar gate electrodes that overlie the layer of silicon oxide.
7. The method of claim 1, wherein the at least two state rotations comprise: at least one state rotation that, at least in part, is a rotation between singlet and triplet states of the DQD; and at least one state rotation that, at least in part, is a rotation between | and |
states of the DQD.
8. A method of quantum information processing using a single-electron spin qubit embodied in a quantum dot (QD) disposed at a silicon substrate surface overlain by a layer of silicon oxide, comprising: populating the QD with a confined electron having two spin states relative to a quantization axis; performing at least one state rotation on the confined electron; and reading out a final quantum state of the QD, wherein: the at least one state rotation is performed while exposing the QD to an externally sourced magnetic field having a component directed parallel to the substrate surface; the QD has a tuning state that moves up and down in energy in response to a voltage applied to a controlling gate electrode arrangement; the performing of the at least one state rotation consists of applying a voltage pulse sequence to the controlling gate electrode arrangement; and the voltage pulse sequence is effective to invoke an effective magnetic field perpendicular to the quantization axis of the spin state of the QD electron and to induce spin state rotations.
Description
BRIEF DESCRIPTION OF THE DRAWINGS
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DETAILED DESCRIPTION
Introduction
(13) The spin-orbit (SO) interaction is a coupling of an elementary particle's spin with an effective magnetic field experienced by the particle due to its motion within an electric field. This interaction can lead to an energy splitting between different spin states of the electron, similar to the well-known Zeeman effect in which an applied magnetic field splits atomic spectral lines. In reference to the Zeeman effect, the splitting due to the SO interaction is also sometimes referred to as a Zeeman splitting. Below, the term Zeeman splitting will be used in reference to energy splittings between spin states that are due to SO interactions as well as those that are directly due to an externally applied magnetic field.
(14) Simple treatments of an electron interacting in vacuum with a magnetic field B give the interaction energy H.sub.SO as
H.sub.SO=[g.sub.S.sub.B/]B.Math.S,
where g.sub.S is the g-factor of the electron spin, .sub.B is the Bohr magneton, and S is the electronic spin angular momentum vector. (More specifically, S is a quantum mechanical operator expressible in terms of the Pauli matrices for spin , which are discussed below.) However, the interaction energy in anisotropic materials calls for a more detailed treatment, in which g.sub.S is replaced by a g-tensor.
(15)
(16) The silicon oxide layer, in turn, is overlain by a n.sup.+-doped layer 120 of patterned polysilicon electrodes as shown in
(17) Due to the cyclotron motion and the inversion asymmetry at the interface, the electronic motion acquires a non-zero net momentum component along the interface. There is also an effective electric field at the interface having a normal component, i.e., a component perpendicular to the electronic momentum along the interface. The coupling between mutually perpendicular components of electronic momentum and effective electric field gives rise to an effective magnetic field B.sub.eff. This effective magnetic field B.sub.eff produces an SO interaction that is additive to the SO interaction produced by the applied magnetic field.
(18) Two contributions to the effective electric field are especially germane. The so-called Rashba contribution relates to a vertical field at the silicon/SiO.sub.2 boundary due to the confining gate potentials and to the structural inversion asymmetry across the interface.
(19) The so-called Dresselhaus contribution occurs in materials, including bulk materials, that lack inversion symmetry. It has a microscopic origin. Silicon does in fact have bulk inversion symmetry; the Dresselhaus contribution instead arises (in the system described here) from interatomic fields at the interface or between silicon and oxygen atoms. In effect, these dipole fields are sampled by the electronic momentum, yielding a net contribution over many atoms. Even though silicon-dioxide is largely amorphous, the Dresselhaus contribution is generally dependent on crystallographic orientation. This is understood to be due to residual order that extends somewhat into the layer of silicon oxide when it is grown.
(20) The Rashba and Dresselhaus contributions to the SO interaction can be subsumed into an effective Zeeman Hamiltonian H.sub.eff:
(21)
Here, B is the applied magnetic field vector (the subscript will be dropped in the rest of this discussion), is the vector of Pauli spin matrices (.sub.x, .sub.y, .sub.z), and g is the effective g-tensor which, in a useful approximation, is given by
(22)
where g.sub. is the g-tensor component for the directions perpendicular to the [001] valley of bulk silicon, g.sub. is the g-tensor component for the directions parallel to [001] the valley of bulk silicon, and and are the respective corrections to the g-tensor due to the Rashba and Dresselhaus SO coupling. (It is assumed here that the growth direction for the structure of
(23) The strength of the SO interaction will depend on the applied electric field, the lateral confinement, the valley-orbit configuration, and the atomic-scale structure of the interface. As a consequence, the local interfacial and electrostatic environments will be particular to each QD. Because these environments will differ between the respective QDs, there will likewise be differences between their effective g-tensors.
(24) The differences between the effective g-tensors are manifested as differences in the effective in-plane magnetic field. But it is the in-plane magnetic field that produces, in each QD, the Zeeman splittings in energy between the different spin states. Hence the local variations in the effective g-tensor will cause the electron spins in the respective dots of the pair to have different spin splittings.
(25) More specifically, the S-T.sub.0 spin splitting will differ between the left-hand and right-hand dots by an amount .sub.SO. This energy difference .sub.SO will drive X-rotations on the Bloch sphere between the S(1,1) and T.sub.0(1,1) states at a frequency .sub.rot(, ) given theoretically by:
(26)
where h=2, is the direction of the in-plane component of the applied field B as measured with respect to the [100] crystallographic direction (i.e., as measured azimuthally from the x-axis), is the out-of-plane angle of B as measured relative to the [001] crystallographic direction (i.e., as measured from the z-axis), and and quantify the differences between the two QDs in the Rashba and Dresselhaus g-tensor perturbations, respectively.
(27) Those skilled in the art will understand from the above equation that the frequency of X-rotation is proportional to the applied magnetic field. It will also be understood that the rotation frequency depends on the difference
(28)
in gyromagnetic ratio between the two dots of the QD pair. In practice, the operator will have some ability to select g by using suitable voltages on the gate electrodes to control the vertical confinement of the induced 2 DEG, thereby modulating the overlap of the electron with the silicon/silicon-dioxide interface.
(29) As explained above, coupling between states via the exchange energy J can be exploited to cause Z-rotations of the DQD spin state. In addition, as we have just shown, the coupling between states due to differences in the Rashba and Dresselhaus perturbations can be exploited to cause X-rotations of the DQD spin state. Through combinations of these two approaches, access can be afforded to any desired spin state of the DQD.
Apparatus
(30) An example DQD is shown in plain view in
(31) The [110] crystallographic direction is indicated by an arrow in each figure. The growth direction is [001]. Four large gate electrodes shown in the corners of
(32) Charge sensing is used to read out the spin state of the DQD. Charge sensing is performed here using a single electron transistor (SET). The curved arrow 230 in
(33) Two circles 240, 250 added to
(34) Procedures in which applied voltages are used to fill and empty the quantum dots are known in the art and insofar as they are general in application, they need not be described here in detail. A specific methodology for achieving two-axis control of the DQD spin state will be described below.
(35) Details of the apparatus of
Method
(36) Using pulse sequences described below, two electrons are electrostatically confined within a double well potential, where the dominant interaction between the electrons can be electrically tuned between two regimes. When the electronic wave functions of the QDs overlap significantly, the exchange energy J is dominant. But when the two electrons are well separated, J is small and instead, the dominant effect is an effective magnetic field gradient due to differences in interfacial SO coupling. (Below, we will refer to this effective magnetic field as the gradient field.) The DQD can be switched between the two regimes through control of applied electric and magnetic fields.
(37) This is illustrated in the schematic energy diagram of
(38) The inset to the figure provides a view of the Bloch sphere. The Z-rotations are indicated by the legend J and by an arrow indicating rotation about the z-axis. The X-rotations are indicated by the legend .sub.SO and by an arrow indicating rotation about the x-axis. As indicated in the figure, equatorial Z-rotations vary the mixture of | and |
states, and meridional X-rotations vary the mixture of singlet and triplet states.
(39) The singlet and triplet states of interest here are the two states S and T.sub.0 of the m=0 subspace. They form a decoherence-free subspace relative to fluctuations in a uniform magnetic field, and they are chosen here as the computational basis. An applied magnetic field causes a Zeeman splitting of the m=1 spin triplet states (respectively denominated T.sup.+ (1, 1) and T.sup. (1, 1)) from each other and from the m=0 state, thereby isolating the m=0 subspace.
(40) A qubit state can be initialized in a singlet ground state S when the two QDs are electrically detuned out of resonance so as to favor the (2, 0) charge state. Rapid adiabatic passage (adiabatically transferring the charge, while diabatically transferring the spin state) from S(2, 0) produces a singlet state in the (1,1) charge configuration, i.e., S(1,1). The rapid adiabatic passage involves adiabatically transferring the charge, while diabatically transferring the spin state.
(41) In this regard, it will be understood that in the adiabatic transition, the charge state evolves continuously so as to remain an eigenstate of the (spatial) electronic Hamiltonian. In the diabatic transition, by contrast, the spin state retains its physical character while the (spin) Hamiltonian changes. As a consequence, the spin state at the end of the transition is a superposition of the new (spin) eigenstates.
(42) X-rotations are induced between the S(1, 1) and T.sub.0(1, 1) states at the frequency .sub.rot(,) by utilizing the SO coupling, as discussed above. Z-rotations can be turned on by shifting the detuning (within the (1, 1) regime called out in the figure by reference numeral 300) closer to the charge anti-crossing where J is larger, driving oscillations around the equator of the Bloch sphere.
(43) The spin state is detected using Pauli blockade in cooperation with a remote charge sensor. In our experiments, the remote charge sensor was an SET, as explained above.
(44) Illustratively, the SET is capacitively coupled to the DQD, so that the current passed through the SET can be used to distinguish between different charge configurations of the DQD (e.g., (1,0), (1,1), (2,0), (2,1) . . . ). Spin is conserved in the charge-state transitions, so an initial singlet state remains a singlet state, and an initial triplet state remains a triplet state. If the qubit state (of the DQD) is initially S(1, 1), it can permissively pass to the S(2, 0) charge state because the electrons have opposite spins, thus satisfying the Pauli Exclusion Principle. However, the same principle prohibits an initial T.sub.0(1, 1) state from passing to a triplet (2, 0) state in which the two electrons occupy the same orbital.
(45) Under the available operating voltages, however, the next-higher orbital is energetically out of reach. The so-called Pauli blockade therefore locks the qubit in the state T.sub.0(1, 1). The failure to transfer an electron (which would otherwise produce a (2, 0) charge state) during the readout stage can thus be interpreted as a T.sub.0(1, 1) detection.
(46) X-Rotations.
(47) We will now describe X rotations more fully, with reference to
(48)
(49) As will be seen below, the detuning can be determined in our example system by a pair (V.sub.LLP, V.sub.LCP) of gate voltages. In the resulting two-dimensional space, the anticrossing can be mapped to loci that we refer to as charge-preserving lines. There are different charge-preserving lines for the singlet and triplet states, respectively.
(50)
(51) The charge-preserving lines 420, 430 are also shown on
(52) In the geometrical configuration of the quantum dots that we adopted in our experiments, the dipole field of the DQD as experienced by the charge sensor does not change substantially when an electron tunnels from one dot of the DQD to the other without changing the total confined charge. As a consequence, we would not expect to observe a change in charge sensor current for charge transitions at the charge-preserving lines.
(53) One consequence, as will be explained below, is that we use detection of changes in the total electronic occupancy as an indirect route to measuring changes in the two-electron spin state. It should be noted, however, that the detection method described here is offered merely for purposes of illustration. It is only one example among numerous detection methods that are known in the art, and thus should be understood only as a non-limiting example.
(54) The arrows superposed on
(55) According to the process illustrated in
(56) The pulse sequence shown in the figures is repeated cyclically while the current through the SET is monitored.
(57) The system is initialized in the (2,0) charge sector by unloading (point U) the DQD into the (1,0) charge configuration and then applying an energy-selective pulse into the (2,0) charge state between the singlet and triplet energy levels such that an S(2,0) ground state is loaded (point L). The system is then plunged (point P) to a detuning (<0) close to the charge anticrossing. The electrons are then separated (point C), and qubit manipulations are performed in the (1,1) charge region (>0).
(58) The system is then pulsed back to the (2,0) charge sector (point P). At point P, a singlet spin state is permitted to transfer to the (2,0) charge state, but due to Pauli spin blockade, a triplet spin state is energetically blocked and remains as a (1,1) charge state.
(59) We then pulse to point M, where the read-out is performed by spin-to-charge conversion. We use an enhanced latching mechanism for spin-to-charge conversion. The DQD state is read out as follows: If it is a triplet, it is mapped to a (2,1) charge state; if it is a singlet, it is read out as (2,0).
(60) More specifically, the triplet (1, 1) state can transfer relatively quickly to the (2, 1) charge state by inelastic tunneling of an electron into QD.sub.1 from the LRG charge reservoir. The resulting change in the total charge on the DQD is detected by the SET. On the other hand, the singlet remains locked in a metastable (2, 0) charge state at point M, because the path for relaxation to a (2, 1) charge state is only through a slow co-tunneling process.
(61) One important conclusion from our work is that the spin-orbit effect is useful not only for producing state rotations in two-electron qubits, but also in single-electron spin qubits. That is, a single quantum dot of the kind described here is populated with an electron, and an applied magnetic field having a component parallel to the interface induces cyclotron motion of the electron near the interface.
(62) As explained above, the resulting electronic momentum component parallel to the interface makes the electron susceptible to interfacial spin-orbit effects. In particular, these effects are manifested as an effective magnetic field that affects Larmor precession of the electronic spin state. The spin state of the electron can be collapsed to one of the two possible observable states and read out by techniques that are well known in the art.
(63) The tuning mechanism described above can be used to control the Larmor frequency. That is, the gate voltages control the depth of interaction of the electronic wavefunction with the electric fields due to the interfacial phenomena. Consequently, a desired Larmor frequency can be selected by selecting suitable gate voltages, and electron spin state rotations can be produced by applying suitably tailored voltage pulse sequences to the gate electrodes.
(64) More specifically, an external magnetic field applied parallel to the interface (e.g., along the [100] crystallographic direction) causes a Zeeman splitting of the spin states, and in addition, it invokes a non-zero momentum component of the electron at the interface. The interfacial momentum component causes Rashba and Dresselhaus contributions to an interfacial spin-orbit effect, resulting in effective Rashba and Dresselhaus magnetic fields.
(65) The Rashba field (in the case of an external magnetic field applied along the [100] crystallographic direction) will be parallel (or anti-parallel) to the external magnetic field and will add to (or decrease, if anti-parallel) the spin splitting.
(66) The Dresselhaus field (in the case of the external magnetic field being along the [100] crystallographic direction) will be perpendicular to the external magnetic field and therefore will not affect the spin splitting.
(67) A voltage with alternating current (AC) modulation is applied to the QD confinement gate, thereby producing an oscillating vertical electric field. The oscillating vertical field causes the spin-orbit strength to oscillate, and it also causes an effective AC magnetic field (due to the Dresselhaus SO contribution) directed perpendicular to the spin quantization axis (i.e., perpendicular to the external magnetic field direction).
(68) When the AC magnetic field is on resonance with the Larmor frequency, it will drive rotations of the electronic spin state.
(69) Z-Rotations.
(70) The second axis of coherent control for ST qubits is achieved through the tunable exchange coupling of the (1, 1) and (2, 0) charge states. This leads to hybridization between the (2, 0) and (1, 1) charge states and an exchange splitting, J(), between the S and T.sub.0 qubit states that depends on the detuning . By varying the strength of this interaction, we can achieve controlled coherent rotations.
(71)
(72) The DQD is initialized into a S(2, 0) ground state. We then adiabatically separate the electrons into the (1, 1) charge configuration where J() is nearly zero and the qubit is initialized in the ground state of the SO field (| or |
), which is a superposition of the S(1, 1) and T.sub.0(1, 1) states.
(73) We apply a fast pulse to a finite J() at near 0 for some waiting time, and then we apply a fast return pulse. The finite J() rotates the qubit state around the Bloch sphere about a rotation axis that depends both on J and on SO, i.e., on the SO-induced splitting of the | and |
states.
(74) In an example, we applied a field of 0.2 T along the [100] direction, which provided a small (0.5 MHz) residual X-rotation frequency. At detuning near =0, we observed an increased rotation frequency. As the exchange pulse moved to deeper detuning, we observed a decrease in rotation frequency as well as a decrease in visibility. This was expected, because with deeper detuning, J tends to decrease and the rotation axis tends to tilt toward the direction of the SO field difference.
(75)
e,rad J().sup.2+.sub.SO .sup.2,
since the respective components add in quadrature. Indeed, our measurements show that at deep detuning the rotation frequency saturated near 0.5 MHz due to the SO field at the applied magnetic field strength and orientation.
EXAMPLE
(76) We fabricated a singlet-triplet (ST) qubit in a fully foundry-compatible process using a single-gate-layer, metal-oxide-semiconductor (MOS) polysilicon gate stack with an epitaxially-enriched .sup.28Si epilayer.
(77) The material stack consisted of 200 nm highly arsenic-doped (510.sup.15 cm.sup.2 at 50 keV) polysilicon and 35 nm of silicon oxide on top of a silicon substrate with an isotopically enriched epitaxial layer hosting 500 ppm residual .sup.29Si. Ohmic implants were formed using optical lithography and implantation of arsenic at 310.sup.15 cm.sup.2 at 100 keV. The confinement and depletion gates were defined by electron beam lithography followed by selective dry etching of the polysilicon.
(78) Hall bars from the same sample wafer with the same gate oxide were used to extract the critical density (n.sub.c=5.710.sup.11 cm.sup.2), the peak mobility (=4500 cm.sup.2 V.sup.1 s.sup.1), threshold voltage (V.sub.th=1.1 V), the RMS interface roughness (=2.4 ), and roughness correlation length (=26 ).
(79)
(80) The device was operated in an enhancement mode using voltage biasing of the highly doped n+ polysilicon gates to confine electrons to quantum dot (QD) potentials under gates LCP and UCP. The gates ULG, URG, LLG and LRG, which overlapped n+ regions and ohmic contacts, were biased to accumulate a two-dimensional electron gas (2 DEG) under each gate. The 2 DEGs act as source and drain electron reservoirs for the quantum dots.
(81) The lower half of the device was tuned such that a double quantum dot (DQD) was formed. The quantum dot denominated QD.sub.1 was tunnel coupled to the reservoir under LRG. The other quantum dot, designated QD.sub.2, was positioned such that it could occupied only by tunneling of electrons through QD.sub.1.
(82) QD.sub.1 was defined by the gate geometry. QD.sub.2 was formed incidentally, but it survived thermal cycling and was thus a built-in feature of the device.
(83)
(84) One quantum dot in the upper half of the device was used as a single electron transistor (SET) remote charge sensor for spin-to-charge conversion. The SET was biased with 70 V (rms) AC bias at 0V DC and the current was measured with an AC lock-in technique at 979 Hz. The electron temperature, T.sub.e of about 150 mK was measured by QD charge transition line width.
(85) More details about the fabrication process can be found in S. Rochette et al., Single-electron-occupation metal-oxide-semiconductor quantum dots formed from efficient polysilicon gate layout, Preprint at http://arxiv.org/abs/1707.03895 (2017), the entirety of which is hereby incorporated herein by reference.
(86) Measurements were performed in a 3 He/4 He dilution refrigerator with a base temperature of around 8 mK. The effective electron temperature in the device was 150 mK as measured by QD charge transition line width. Fast RF lines were connected to cryogenic RC bias tees on the sample board, which allowed for the application of fast gate pulses. An external magnetic field was applied using a 3-axis vector magnet.
(87) The number of electrons in each QD was inferred from changes in the current through the SET as the voltages on gate LLP and gate LCP were varied. A contour plot of the SET current gradient over the two-dimensional space defined by the respective gate voltages exhibited charge-stability regions separated by boundaries where the current gradient was high. Each of these boundaries indicated a transition in the charge state. This technique for inferring QD occupation numbers is known in the art and need not be described here in further detail.
(88) We used capacitance measurements to determine the locations of QD.sub.1 and QD.sub.2. By scanning combinations of the polysilicon gates, we were able to obtain the relative capacitance of each quantum dot to each gate, relative to the capacitance of gate LCP. (Gate LCP had the strongest capacitive coupling to both QDs.) From these values, we could triangulate the dot locations. This technique is known in the art and need not be described here in further detail.
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where =/2 in
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