Single magnetic-layer microwave oscillator
11533020 · 2022-12-20
Assignee
Inventors
- Karsten Rode (Dublin, IE)
- Plamen Stamenov (Dublin, IE)
- John Michael David Coey (Dublin, IE)
- Yong Chang Lau (Tokyo, JP)
- Davide Betto (Triuggio, IT)
- Arne Brataas (Trondheim, NO)
- Roberto Troncoso (Trondheim, NO)
Cpc classification
H05B6/686
ELECTRICITY
H03B15/006
ELECTRICITY
International classification
H03B15/00
ELECTRICITY
Abstract
A method and system for generating voltage and/or current oscillations in a single magnetic layer is provided. The method comprises applying a direct voltage/current to the layer in a longitudinal direction; and developing a longitudinal voltage between a pair of longitudinal voltage leads and/or a transverse voltage between a pair of transverse voltage leads. The magnetic layer comprises a ferrimagnetic or antiferrimagnetic material having a first and second magnetic sub-lattice, wherein the first sub-lattice is a dominant sub-lattice such that the charge carriers at the Fermi energy originate predominantly from the dominant sub-lattice and the charge carriers at the Fermi energy are spin polarised. In some embodiments, the dominant current carrying sub-lattice may lack inversion symmetry.
Claims
1. A method of generating voltage and/or current oscillations in a single magnetic layer, the magnetic layer having a thickness in a thickness direction, comprising: applying a direct voltage and/or current to the layer in a longitudinal direction perpendicular to the thickness direction; and developing a longitudinal voltage between a pair of longitudinal voltage leads and/or a transverse voltage between a pair of transverse voltage leads; wherein the layer comprises a ferrimagnetic or anti-ferrimagnetic material having a first and second magnetic sub-lattice, wherein the first sub-lattice is a dominant sub-lattice such that the charge carriers at the Fermi energy originate predominantly from the dominant sub-lattice and the charge carriers at the Fermi energy are spin polarised; and wherein: i) the first and second magnetic sub-lattices have an ordered non-collinear magnetic structure such that the angle between the local magnetic moment of the first and second magnetic sub-lattices is uniform in the layer and an azimuthal angle of the local magnetic moment of the first magnetic sub-lattice about the direction of the local magnetic moment of the second magnetic sub-lattice varies periodically along one or more spatial directions giving a magnetic texture, and the wavelength of the magnetic structure is longer than the Fermi wavelength; or ii) the first and second magnetic sub-lattices have a disordered non-collinear magnetic structure such that the angle between the local magnetic moment of the first and second magnetic sub-lattices is uniform in the layer and the azimuthal angle is non-uniform and/or random in the layer and the dominant current carrying sub-lattice lacks inversion symmetry; or iii) the first and second magnetic sub-lattices have a collinear magnetic structure at a current density below a first threshold current density and the dominant current carrying sub-lattice lacks inversion symmetry.
2. The method of claim 1, wherein, where: the first and second magnetic sub-lattice have a disordered non-collinear magnetic structure such that the angle between the local magnetic moment of the first and second magnetic sub-lattices is uniform in the layer and the azimuthal angle is non-uniform and/or random in the layer and the dominant current carrying sub-lattice lacks inversion symmetry, or the first and second magnetic sub-lattices have a collinear magnetic structure at a current density below a first threshold current density and the dominant current carrying sub-lattice lacks inversion symmetry: and the current-induced spin-orbit-interaction energy is at least 50% of the energy of the first non-collinear excited state.
3. The method of claim 2, wherein the magnetic layer comprises a material comprising a first atomic species, and a second p-block atomic species.
4. The method of claim 3, wherein one sub-lattice comprises atoms with high-Z: at least Ga.
5. The method of claim 1, wherein, where: the first and second magnetic sub-lattices have a disordered non-collinear magnetic structure such that the angle between the local magnetic moment of the first and second magnetic sub-lattices is uniform in the layer and the azimuthal angle is non-uniform and/or random in the layer and the dominant current carrying sub-lattice lacks inversion symmetry, or the first and second magnetic sub-lattices have a collinear magnetic structure at a current density below a first threshold current density and the dominant current carrying sub-lattice lacks inversion symmetry, the dominant sub-lattice exhibits a spin-orbit splitting energy of at least 100 meV.
6. The method of claim 1, wherein the material has a damping factor of less than or approximately equal to 0.01.
7. The method of claim 1, wherein where the first and second magnetic sub-lattices have a disordered non-collinear magnetic structure such that the angle between the local magnetic moment of the first and second magnetic sub-lattices is uniform in the layer and the azimuthal angle is non-uniform and/or random in the layer and the dominant current carrying sub-lattice lacks inversion symmetry, the probability of inter-sub-lattice scattering involving spin flip is greater than inter-sub-lattice scattering not involving spin flip.
8. The method of 1, wherein the inter-sub-lattice (neighbouring spin belonging to different sub-lattices) exchange parameter is weaker than at least one intra-sub-lattice (neighbouring spin belonging to the same sub-lattice) exchange parameter.
9. The method of claim 1, further comprising making an electrical short circuit between the pair of transverse voltage leads.
10. The method of claim 1, wherein the magnetic layer comprises a ferrimagnet.
11. The method of claim 1, wherein the magnetic layer comprises a half-metallic ferrimagnet.
12. The method of claim 1, wherein the magnetic layer exhibits a spin polarisation of at least 50%.
13. The method of claim 12, wherein the magnetic layer exhibits a spin polarisation of at least 50% at 300 Kelvin.
14. A system comprising a device for generating voltage and/or current oscillations, the device comprising: a single magnetic layer through which a current or voltage is applied in a longitudinal direction perpendicular to a thickness direction; and a pair of longitudinal and/or transverse voltage leads for measuring a respective longitudinal and/or transverse voltage; wherein the layer comprises a ferrimagnetic or anti-ferrimagnetic material having a first and second magnetic sub-lattice, wherein the first sub-lattice is a dominant sub-lattice such that the charge carriers at the Fermi energy originate predominantly from the dominant sub-lattice and the charge carriers at the Fermi energy are spin polarised; and wherein: i) the first and second magnetic sub-lattices have an ordered non-collinear magnetic structure such that the angle between the local magnetic moment of the first and second magnetic sub-lattices is uniform in the layer and an azimuthal angle of the local magnetic moment of the first magnetic sub-lattice about the direction of the local magnetic moment of the second sub-lattice varies periodically along one or more spatial directions giving a magnetic texture, and the wavelength of the magnetic structure is longer than the Fermi wavelength; or ii) the first and second magnetic sub-lattices have a disordered non-collinear magnetic structure such that the angle between the local magnetic moment of the first and second magnetic sub-lattices is uniform in the layer and the azimuthal angle is non-uniform and/or random in the layer and the dominant current carrying sub-lattice lacks inversion symmetry; or iii) the first and second magnetic sub-lattices have a collinear magnetic structure at a current density below a first threshold current density and the dominant current carrying sub-lattice lacks inversion symmetry.
15. The system of claim 14, further comprising a means for applying the voltage and/or current to the device.
16. The system of claim 14, further comprising a means for measuring the longitudinal and/or transverse voltage.
17. The system of claim 14, further comprising a means for extracting the generated voltage and/or current oscillations from the longitudinal and/or transverse voltage.
18. The system of claim 17, wherein the means for extracting the generated voltage and/or current oscillations comprises a bias tee and/or a capacitor coupled to the longitudinal and/or transverse voltage leads.
19. The system of claim 14, wherein the magnetic layer comprises a ferrimagnet, and/or a half-metallic ferrimagnet.
20. The system of claim 14, wherein the magnetic layer comprises MnRuGa, MnFeGa, or MnGa.
Description
BRIEF DESCRIPTION OF DRAWINGS
(1) In order that the invention can be well understood, embodiments will now be discussed by way of example only with reference to the accompanying drawings, in which:
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DETAILED DESCRIPTION
(19) Existing spin-transfer torque (STT) devices require at least two separate magnetic layers having a non-collinear magnetisation structure, separated by a non-magnetic spacer layer, to generate a magnetic torque and alter the magnetisation of a magnetic layer, such as spin valves (GMR) and magnetic tunnel junctions (TMR). As shown in
(20) A magnetic torque can also be generated in a single magnetic layer from another current-driven mechanism based on the spin-orbit interaction (SOI). This effect, known as spin-orbit torque (SOT), is due to a net spin-orbit effective magnetic field B.sub.SO resulting in a current-induced spin accumulation (in momentum space) that is non-collinear to the local magnetisation m of the magnetic layer. Thus, in contrast to STT, SOT does not rely on two non-collinear, independent ferromagnetic layers 110, 130.
(21) The current-induced SOI effects arise in materials (magnetic and non-magnetic) that lack inversion symmetry, such as bulk inversion asymmetry (BIA) (e.g. in zincblende crystal structures, where this is a feature of the local order and the crystal potential), or lack inversion symmetry in the macroscopic electrostatic potential of the structure, known as structural inversion asymmetry (SIA) (e.g. in two-dimensional layers and/or heterostructures). The inversion asymmetry lifts the orbital-degeneracy of the conduction electrons and generates a spin splitting (via the SOI), which is dependent on the direction of the electron wave-vector k. By analogy to the Zeeman effect, the k-dependent SO spin splitting can be considered as resulting from a k-dependent effective SO field B.sub.SO(k), whose magnitude is proportional to the strength of the SOI. The spin orientation aligns with B.sub.SO(k). For the case of SIA in a two-dimensional layer, B.sub.SO(k) points in a direction transverse to k, which itself is confined within the plane of the structure. At equilibrium (J=0), B.sub.SO(k) averaged over k at the Fermi energy is zero, because the average k is zero. However, under non-equilibrium conditions (|J|>0) the average k is non-zero and proportional to J producing a net B.sub.SO(k) pointing in a direction transverse to J. This leads to a net spatially uniform spin accumulation <δσ> (transverse accumulation in k-space) proportional to J and the strength of the SOI.
(22) The above current-induced spin accumulation occurs in both magnetic and non-magnetic materials with SOI. In the case of a magnetic material, B.sub.SO(k) is not necessarily dependent on the direction of the local magnetisation m. Although at equilibrium the electron spins tend to align with m, a non-collinear current-induced spin accumulation <δσ> can exert a torque (SOT) on m (i.e. in 3d itinerant ferromagnets through the s-d exchange interaction) that can induce magnetisation switching of the magnetic material. Candidate magnetic materials with high SOI may rely on either high Z-number atoms, or on sufficiently low crystalline symmetry (as, for example, induced by p-type hybridisation). SOT has been demonstrated to induce magnetisation switching in single layers of antiferromagnetic metals and dilute ferromagnetic semiconductors. However, the SOT effect in single ferromagnetic or ferrimagnetic layers has not been shown to induce magnetisation precession (or sustained magnetic oscillations).
(23) According to an aspect of the present invention, the functionality provided by complex magnetic layer stacks in the standard case of STT oscillators is here achieved in a single magnetic layer by making use of the unusual properties of specific ferrimagnets or antiferromagnets.
(24) The key requirements for the generation of sustained magnetic oscillations and an oscillatory conductivity (voltage and/or current) in a single ferrimagnetic or antiferromagnetic layer are that the charge carriers at or near the Fermi energy are (i) highly spin polarised, and (ii) originate from predominantly one of the magnetic sub-lattices (see below).
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(26) Electrical transport through the ferrimagnetic layer 200 can be described phenomenologically in terms of separate independent conduction channels for the electrons of majority spin (parallel to the magnetization of the dominant sub-lattice) with a conductivity σ.sub.↑, and electrons of minority spin (anti-parallel to the latter) with a conductivity σ.sub.↓, leading to a total conductivity σ=σ.sub.↑+σ.sub.↓ (where σ.sub.↑≠σ.sub.↓). The density of states (DoS) for each spin channel at the Fermi energy is not equal due to the crystallographic difference between sub-lattice A and B. As such, charge current passed through the ferrimagnetic layer 200 is highly spin polarised (similar to current in a ferromagnetic layer).
(27) Each of the sub-lattices A, B contribute to the electronic band structure and DoS, however, unlike in the case of a simple antiferromagnet, the DoS for sub-lattice A is not simply a spin-reflection of the DoS of sub-lattice B. As a result, the DoS at the Fermi energy may be partially or completely dominated by one of the two magnetic sub-lattices A, B of the ferrimagnetic layer 200. When the DoS is dominated by one of the sub-lattices A, B at the Fermi energy, the conduction band may be described by a single effective spin-polarised carrier (one spin channel). In other words, charge carriers flowing through the ferrimagnet effectively only “see” the dominant sub-lattice or behave as if only the dominant sub-lattice were present.
(28) An example of a ferrimagnetic, highly (fully) spin-polarised material, with broken inversion symmetry is Mn.sub.2Ru.sub.xGa [H. Kurt et al., Physical Review letters 112, 027201 (2014)]. Mn.sub.2Ru.sub.xGa meets the requirements for exhibiting SOT effects. The large magnetocrystalline anisotropy and the lack of local inversion symmetry existing in Mn.sub.2Ru.sub.xGa imply considerable SOT, which is demonstrated in the experimental section below.
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(30) The example material, Mn.sub.2Ru.sub.xGa, is a ferrimagnetic half-metal with a gap A in the DoS for one spin channel (spin down, in this example). The illustration shows that by varying the Ru content x, the Fermi energy E.sub.F can be tuned to lie within the gap, where the material would be fully spin polarised (i.e. all charge carriers at the Fermi energy originating from one spin band). Suitable Ru contents x lie in the range between substantially 0.4 to 0.7.
(31) Certain ferrimagnets may have a non-collinear magnetic structure and/or exhibit a magnetic texture.
(32) Although the local magnetisation m.sub.A of sub-lattice A is shown along the z-axis in
(33) In the example of
(34) The current-induced change of spin orientation is accompanied by a transfer of spin angular momentum to the dominant magnetic sub-lattice, sub-lattice B in this example. This in turn provides an opposing torque, acting on the local magnetisation of the dominant sub-lattice in question (which is proportional to its cross product with the current density j which is the x-y plane), that provides a back-action that alters the polar angle θ between m.sub.A and m.sub.B. Under steady-state conditions, since the spin orientation always follows the magnetic texture, the sub-lattice torque is spatially uniform. A general form of the current induced SOT in the local approximation is T.sub.AB=m.sub.A,B×H.sub.AB(m.sub.A,m.sub.B,j), where H.sub.A,B is the effective field that depends on the magnetisation direction and is induced by the current density j.
(35) As such, the effect of the magnetic texture in ferrimagnetic layer 300 on the spin orientation is similar to the operation principle of a STT device 100, as shown in
(36) As with a STT oscillator 100, if sufficient spin angular momentum is transferred from the spins to the dominant sub-lattice (e.g., B in this example), magnetisation precession can be induced in the ferrimagnetic layer 300. As the sub-lattice torque is spatially uniform across the layer 300, such oscillations are in phase across the layer 300. The oscillation frequency is given by the ratio v.sub.F/λ.sub.texture, where v.sub.F is the Fermi velocity of the charge carrier. Assuming a Fermi velocity for a typical metal in the range 0.1-2×10.sup.6 m/s and a magnetic texture wavelength λ.sub.texture in the range 1-1000 nm, this gives an oscillation frequency in the range 0.1 THz 2000 THz.
(37) The transfer of spin angular momentum and hence the sub-lattice torque is proportional to the current density and to the degree of spin polarisation of the current. These two parameters are interrelated, such that, the lower the spin polarisation of the current, the more current density is required to provide sufficient sub-lattice torque. High spin polarisation is thus advantageous in order to reduce the operating current density of a device. It follows that, as with STT devices, a minimum or threshold current density is required to observe any sub-lattice magnetisation dynamics. The threshold current densities required to induce magnetisation precession in ferrimagnetic layer 300 may be of the order 10.sup.4-10.sup.7 A/cm.sup.2.
(38) In an alternative embodiment, ferrimagnetic layer 300 may have a collinear magnetic structure in the ground state (i.e. when no current is applied) such that θ=180°. Where the dominant current carrying sub-lattice (present at the Fermi energy), e.g. sub-lattice B, of the ferrimagnetic layer 300 lacks inversion symmetry, current-induced transverse spin accumulation in the presence of SOI may be utilised to exert a SOT on the magnetisation of the dominant current-carrying sub-lattice B and introduce an angle θ≠180°. In this way, the current flowing through the ferrimagnetic layer 300 may transform the collinear magnetic structure into a non-collinear, non-equilibrium magnetic structure (e.g. “frozen magnon”), similar to that shown in
(39) The strength of the SOI felt by the charge carriers should be on the order of the static splitting Δ (see
(40) The threshold current densities required to induce a spin torque induced non-collinearity may be of the order 10.sup.4-10.sup.5 A/cm.sup.2.
(41) Provided that the charge current is highly spin polarised (e.g. >50%) and originating from predominantly one of the two magnetic sub-lattices A, B of the ferrimagnetic layer 300, the oscillatory magnetisation behaviour may manifest as a time-varying change in the conductivity (or resistivity) of the ferrimagnetic layer 300. For example, this may manifest through the anisotropic magnetoresistance (AMR) effect, whereby the longitudinal component of the electrical conductivity (or resistivity) depends on the relative angle θ between the net magnetisation direction M and the electrical current j. Alternatively or additionally, the oscillatory behaviour may manifest through the anomalous Hall effect, whereby the transverse component of the electrical conductivity (or resistivity) depends on the out-of-plane component (e.g. the z-component) of the magnetisation, M.sub.z. In the example ferrimagnetic layer 300 shown in
(42) The magnitude of the effect, or the depth/amplitude of the oscillations in the conductivity is determined by the change in angle θ. The degree of spin polarisation also affects the amplitude of the conductivity oscillations, since only spin polarised charge carriers contribute the oscillatory component of the conductivity and any unpolarised charge carriers will contribute to an offset signal. A ferrimagnet with 100% spin polarisation is ideal. 100% spin polarisation is expected for certain half metallic ferrimagnets. For example, the ferrimagnet Mn.sub.2Ru.sub.0.5Ga shown in the middle panel of
(43) It is also necessary to overcome the intrinsic damping (i.e. Gilbert damping) in the ferrimagnet to observe magnetisation precession. Gilbert damping is characterised by a damping factor α. Consequently, a low damping factor α is advantageous. The damping factor is a dimensionless coefficient that enters directly into the equations that govern the magnetisation dynamics (e.g. the Landau-Lifshitz-Gilbert equation). For example, damping factors of α<0.01 may be required to observe magnetisation precession. It is also necessary for the gain-bandwidth product (GBP) to be greater than 1 to observe magnetisation precession. If the damping factor α is too high, the gain band width product (GBP) will be too low, e.g. <1. Damping, net magnetic moment, spin polarisation and anisotropy are all affected by temperature. As it is expected that realistic oscillators would operate above ambient temperature, some welcome gains in terms of damping can occur, as inhomogeneity (anisotropy) driven magnon generation is suppressed at high temperatures.
(44) Sustained current controlled magnetic oscillations with tunable amplitudes and frequencies in a single antiferromagnetic and ferrimagnetic layer (such as Mn.sub.2Ru.sub.xGa) has been demonstrated theoretically via a phenomenological approach in R. E. Troncoso et al. Physical Review B, 99, 054433 (2019).
(45) The conductivity or resistivity of ferrimagnetic layer 300 may be determined using standard resistance measurements, e.g. by passing current through the layer 300 and measuring a voltage.
(46) In an embodiment, external feedback may be used to enhance the back-action provided by the current induced torques. In one example, the two sides of the Hall bar, e.g. ports 3 and 5 and/or ports 4 and 6, may be electrically short-circuited. In this way, the presence of a transverse voltage V.sub.xy will drive a charge transverse charge current between the respective ports. Oscillations in the transverse charge current will be in phase with the oscillations in the longitudinal and transverse conductivity, thus providing positive feedback.
(47) The oscillatory conductivity may also manifest as negative differential conductance. For applied current densities below a critical current density required to induce magnetisation dynamics, the current-voltage relationship may be substantially linear, in accordance with Ohm's law. At or above the critical current density, the average conductivity may exhibit a drop (i.e. increased resistance) due to increased momentum scattering associated with the magnetisation dynamics. This manifests as a turnover or region of non-linearity in the current-voltage relationship.
(48) In another embodiment, the ferrimagnetic layer 300 may have a non-collinear magnetic structure such that θ≠180°, but there is no long range order such that the azimuthal angle ϕ varies randomly across the layer 300. This is in contrast to the case of
(49) The nonlinear changes in internal scattering coefficients, would thus result in a region of negative differential conductivity, at sufficiently high current densities (leading to an appreciable change in the cone/polar angle θ). The frequency of oscillation in this case would be determined by extrinsic parameters, such as wave-guide dispersion, if the structure is forming a part of a waveguide system, or RC time-constants in the case of capacitive coupling to an antennae structure.
(50) Spin-flip scattering is a SOI driven process. As such, a necessary requirement is that the SOI felt by the charge carriers is on the order of the static splitting Δ (see
(51) Suitable ferrimagnetic materials for the oscillator 400 may include, but are not limited to MnRuGa, Mn.sub.2FeGa, Mn.sub.3-xGa.
(52) The ferrimagnetic structure may be an ordered non-collinear one (e.g. the first embodiment), an ordered collinear one (e.g. the second embodiment), or a disordered non-collinear one (e.g. the third embodiment). In the latter two cases, the presence of SOI is necessary.
(53) A condition for the observation of an oscillatory voltage and/or current in a single ferrimagnetic layer is a sufficiently small damping factor α. This ensures the system will produce oscillations, for an arbitrarily small SOT. If the damping factor is too high (e.g. >>0.01) the gain-bandwidth product (GBP) will be too low for practical uses, as the bandwidth of the oscillator will be adversely affected. GBP >1 is a necessary condition for the observation of oscillations.
(54) The invention greatly simplifies the production and integration of an oscillator in existing technology by reducing the number magnetic layers required (e.g. one layer compared to three layers in existing STT devices). In addition, the range of frequencies accessible by the proposed method greatly exceeds that achievable using existing semi-conductor and magnetic based technologies.
(55) Experimental Section: Measurements of Spin-Orbit Torque in MnRuGa
(56) In the following we show that spin-orbit torque in a single layer of the highly spin-polarized compensated ferrimagnet Mn.sub.2Ru.sub.xGa is remarkably efficient at generating spin-orbit fields μ.sub.0H.sub.eff (where μ.sub.0 is the vacuum permittivity) which approach 0.1×10.sup.−10 Tm.sup.2/A in the low-current density limit almost a thousand times the Oersted field, and one to two orders of magnitude greater than the effective fields in heavy metal/ferromagnet bilayers.
(57) To date, there has been no quantitative measurement of the damping-like (dissipative) component of the spin-orbit torque in homogeneously magnetized ferrimagnetic or antiferromagnetic single layers. In a single layer of half-metallic Mn.sub.2Ru.sub.xGa with x=0.7 (MRG) we show that both the field-like (reactive) and damping-like (dissipative) components of the torque are almost two orders of magnitude greater than those obtained in bilayer ferromagnet/heavy metal systems, or in metallic ferromagnets and semimagnetic semiconductors. From a harmonic analysis of the anomalous Hall effect, taking into account of the thermal contributions from the anomalous Nernst effect, we show that the dissipative component of the spin-orbit torque is sufficient to sustain self-oscillations in the magnetization.
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(59) The MRG (x=0.7) was grown on a single-crystal MgO (001) substrate by magnetron co-sputtering from Mn.sub.2Ga and Ru targets in a ‘Shamrock’ deposition cluster tool at a substrate temperature approximately 350 degrees C. The Ru concentration x can be varied by changing the power to the Mn.sub.2Ga target while keeping that of the Ru target constant. After deposition of the active MRG layer, the samples were covered, at room temperature, with approximately 2 nm of AlO.sub.x to prevent oxidation. The Hall bar was patterned using standard UV lithography and Argon ion milling, and electrical contacts were formed by titanium/gold patterned by lift-off, as is known in the art.
(60) The longitudinal and transverse voltages were measured using lock-in detection at the first, second and third harmonic, at a low drive frequency of approximately 1 kHz. The excitation frequency is far from the frequency of magnetisation oscillations or thermal dynamics, but provides a convenient means to separate effects that are odd or even functions of the bias current. Measurements were performed as a function of temperature and applied external magnetic field μ.sub.0H. AHE measurements are performed after saturation in an out-of-plane magnetic field by recording the first, second and third harmonics of the drive frequency as a function of the magnitude and azimuthal angle ϕ.sub.H of an applied in-plane magnetic field μ.sub.0H.
(61) Thin-film samples of MRG grown on MgO substrates by DC-magnetron sputtering from stoichiometric targets crystallise in a Heusler-like structure (space group F
(62) The coordinate system describing the magnetic state is shown in
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(64) The current induced effective fields were determined from the AHE measurements, assuming that the AHE is proportional to the z component of the magnetization of the Mn.sup.4c (dominant) sub-lattice. The low conductivity of the MRG coupled with high values of its temperature derivative (see
(65) In the following, we restrict our analysis to the effect to SOT fields on one sublattice, as the other will follow via inter-sublattice exchange with a phase lag. All SOT torques are treated as equivalent to effective external applied fields, i.e. μ.sub.0H.sub.eff. In the presence of a unit charge current density j parallel to the MRG [010] axis as shown in
μ.sub.0h.sub.SOT=m.sub.zx.sub.dle.sub.x−x.sub.fle.sub.y+m.sub.xx.sub.dle.sub.z (1)
where e.sub.x, e.sub.y, e.sub.z are unit vectors, m.sub.x and m.sub.z are the components of the unit net magnetisation vector, and x.sub.fl and x.sub.di are the coefficients of the field-like and damping-like contributions to the SOT effective field, respectively. The units of μ.sub.0h.sub.SOT, x.sub.fl and x.sub.dl are Tm.sup.2/A (also known as the Henry).
(66) In the AHE measurement, the transverse (Hall) voltage V.sub.xy varies with the out-of-plane component of the net magnetization vector m.sub.z, i.e. with cos(θ.sub.0+Δθ), where Δθ is a small change in the angle due to the SOT field. To convert determine the effective SOT fields from the AHE measurements it is therefore necessary to relate the small efficient SOT field h.sub.SOT to Δθ.
(67) The magnetic part of the free energy in a tetragonal system is written, to second order in anisotropy as:
E=K.sub.1 sin.sup.2(θ)+K.sub.2 sin.sup.4(θ)+K.sub.2′ sin.sup.4(θ)cos(4ϕ.sub.M)−μ.sub.0{right arrow over (H)}(θ.sub.H,ϕ.sub.H){right arrow over (M)}(θ,ϕ.sub.M) (2)
(68) where θ and ϕ.sub.M are the polar and azimuthal angles of the net magnetization vector, and ϕ.sub.H is the azimuthal angle of the applied field μ.sub.0H, and K.sub.1, K.sub.2 and K′.sub.2 are coefficients. K′.sub.2 is usually much weaker than K.sub.1,2 and we assume the in-plane component of the magnetization is aligned with the applied field μ.sub.0H, such that ϕ.sub.M=ϕ.sub.H. The equilibrium position of the magnetization can then be derived from the stability condition:
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(70) Although equation 3 cannot be directly solved for θ, the aim is to relate the small efficient SOT field h.sub.SOT to Δθ. We write H=H.sub.0+h.sub.SOT and θ=θ.sub.0+Δθ, and note that F(θ.sub.0, H.sub.0)=0 (the equilibrium position) as well as
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because E is linear in H. We now expand F to second order in h.sub.SOT which leads to a quadratic equation. Realising that
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me square root portion of the solution of the quadratic can be expanded to select the solution that ensures F=0 when h.sub.SOT=0. The change in angle Δθ is then:
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(74) which can be rewritten as
Δθ=Δθ.sub.1j+Δθ.sub.2j.sup.2 (7)
(75) where j is the current density and the units of Δθ.sub.1 and Δθ.sub.2 are rad m.sup.2/A and rad m.sup.4/A.sup.2, respectively, because h.sub.SOT is linear in j.
(76) To derive the expressions for the second and third harmonics of the transverse voltage V.sub.xy taking into account the effects of homogeneous heating and the SOT field through ΔT and Δθ, we write ρ=σ.sup.−1, σ.sub.xx.sup.0=σ.sub.xx.sup.0(1+δ), σ.sub.xy=σ.sub.xy.sup.0(1+β) with
(77)
δ and β are correction factors homogenous heating and can be determined from the experimental σ.sub.xx(T) and σ.sub.xy(T) data (see
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(79) Obtaining the voltage response on the second V.sub.xy.sup.2ω and third V.sub.xy.sup.3ω harmonic signals of the bias current I can be achieved by expanding equation 8 to first order in ε and β, and second order in Δθ, and expanding the powers of the sinusoidal bias current I=I.sub.ac sin ωt+I.sub.dc and projecting onto the respective harmonics, which gives:
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(81) where l takes into account a small longitudinal offset of one of the transverse Hall contacts due to misalignment during fabrication, w and t are the width and thickness of the MRG film, and σ.sub.oh is the normal Hall conductivity. Similar equations can be derived for the harmonics of the longitudinal voltage responses (V.sub.xx.sup.nω, where n is the order of the harmonic).
(82) The extracted parameters for the field and damping-like contributions to the SOT are obtained by fitting equations 9 and 10 to the experimental data using values for σ.sub.xx.sup.0, ε and β and anisotropy constants determined experimentally.
(83)
(84) All the salient features in the experimental data are reproduced in the model: the two deep minima near the +/− maximum field in the x-direction μ.sub.0H.sub.x, four maxima that correspond to the fourfold in-plane anisotropy of MRG (due to the small value of the in-plane anisotropy constant K′.sub.2), as well as a weaker central minimum around H=0. Qualitatively, the shape of the SOT can be understood by comparing equation 1 with the blue surface plots and projected 2D image plots in
(85) It is expected from the model of equation 9 that the contribution to V.sub.xy.sup.2ω from SOT scales with I.sub.de and I.sub.ac.sup.2, while the anomalous Nernst effect should be independent of I.sub.dc and scale as I.sub.ac.sup.2.
(86) It is instructive to compare the effective fields due to SOT with those recorded on conventional bilayers of a heavy metal (typically Pt, Ta or W) and a 3d ferromagnet (typically Co, Fe, CoFe or CoFeB). For bi-layers, the damping-like effective field per current density can be written: μ.sub.0H.sub.dl/j=(θ.sub.SHℏ)/(2eM.sub.st), where θ.sub.SH is the spin-Hall angle of the heavy metal, ℏ is the Planck's constant, e is the electron charge, M.sub.s the magnetisation of the ferromagnet and t its thickness. For 1 nm of CoFeB (M.sub.s˜1 MA m−.sup.1), which has a magnetic moment equivalent to that of a nearly compensated ˜30 nm thick MRG film, and θ.sub.SH=40% we obtain an effective damping-like field of 1.3×10.sup.−13 T m.sup.2/A or 0.13 pH. A fictitiously large spin-Hall angle of 400% would be needed to match the value of the determined field-like term of 15×10.sup.−13 Tm.sup.2/A in MRG and 1200% to match the determined damping-like term of 50×10.sup.−13 Tm.sup.2/A in MRG. As such, compared to the effective SOT fields in heavy metal/ferromagnet bilayers, the values determined for a 30 nm thick MRG film are up to two orders of magnitude greater and independent of the thickness of the MRG film (for fixed current density).
(87) This comparison highlights the inherent advantage of using a single ferrimagnetic layer in combination with intrinsic SOT. In a ferromagnetic bilayer, increasing the thickness of the ferromagnet beyond the spin diffusion length (typically <10 nm), does not produce any additional SOT. If the ferromagnet is 2 nm rather than 1 nm thick, the effective SOT field may be reduced to half, whereas the SOT field in single layer of MRG is unchanged with thickness. For a fixed current density, the volume of MRG can be scaled up or down without changing the SOT torque.
(88) However, the nature of the intrinsic SOT torque in MRG is staggered, acting directly on the Mn.sup.4c sub-lattice, hence a more correct comparison might be to normalise the spin Hall angle using the sub-lattice magnetisation, which is approximately ten times greater than the net magnetisation at room temperature for the 30 nm thick MRG film. Furthermore, the SOT torque is maintained even in the absolute absence of net magnetisation at the ferrimagnetic compensation temperature, thus permitting GMR and TMR based device structures to be excited by SOT even in the absence of any net magnetic moment. This enables a far more targeted control of the dynamics, and the excitation of both in-and out-of phase resonance modes.
(89) The high effective fields found in the linear response,
(90) m.sub.z is then measured (from V.sub.xy) with a constant in-plane field μ.sub.0H=0.4 T as function of the azimuthal angle ϕ.sub.H for range of current densities from 0.2 to 2.5×10.sup.6 A m.sup.−2. As the action of the SOT field depends directly on its direction relative to the direction of the magnetization vector m (θ.sub.M and ϕ.sub.M≈ϕ.sub.H), any variations that are ϕ-independent, shown in
(91) The strong observed effective SOT fields in MRG are related to its high anomalous Hall angle (see N. Thiyagarajah et al. Applied Physics Letters, 106, 122402 (2015)). The anomalous Hall angle value is unusual in the sense that MRG does not contain any elements heavier than Ru, and in any case the AHE angle does not scale with Ru content x. Furthermore the conduction electrons in MRG are predominantly d-like, while it has been suggested that Ga in the Mn-containing Heuslers lends some p character to the bands at the Fermi-level through hybridisation, increasing the spin-orbit coupling of the conduction electrons (see Y. C. Lau et al. Physical Review B, 99, 064410 (2019)). From our measurements of σ.sub.xx and σ.sub.xy, (in
(92) The above results demonstrate that, in the example material MRG, high current-induced effective fields as well as a high ratio (˜3) of the dissipative (anti-damping) to the reactive (field-like) SOT torques exists. To demonstrate that sustained oscillations of the magnetisation can be driven by the SOT we consider first the results established by Troncoso et al. (Physical Review B, 99, 054433 (2019)), noting that the effective fields will act distinctly on the magnetisation and the Neel vectors. Using the numerical values of the effective fields found in the linear, low-current regime, oscillations will emerge for current densities that provide a reactive torque which is sufficient to overcome the in-plane anisotropy ˜0.1 T for MRG, which corresponds to j>7×10.sup.6 A cm−.sup.2. The second necessary condition is that the dissipative torque must overcome the Gilbert damping α. Taking α≈0.01 we find the condition j >10×10.sup.6 A cm−.sup.2. Second, we directly compare the effective inductance created by the SOT and the self-inductance of the oscillating element. In a device structure of the shorted Hall bar type, a crude estimate of the self-inductance for a 500 nm thick MRG film with an active length of 20 μm is about 0.1 pH (where the device dimensions are chosen to enhance impedance matching to free space in a real oscillator).
(93) As such, with realistic values of the Gilbert damping, oscillations in the magnetisation can be achieved in ferrimagnets such as MRG at attainable current densities that are similar to those used existing STT devices. Such magnetic oscillations are converted to oscillations in the current and/or voltage via magnetoresistive effects, such as AMR, GMR and TMR. Alternatively or additionally, such oscillations can be directly emitted into free space using a suitable antenna.
(94) Although the above experimental results are shown for a 30 nm thick MRG with x=0.7, it will be appreciated that the results and findings are not limited to the particular sample studied, but will apply to MRG with different dimensions and Ru contents, and different ferrimagnets such as MnFeGa, or MnGa, as well as other ferrimagnetic materials not studied or reported to date.
(95) From reading the present disclosure, other variations and modifications will be apparent to the skilled person. Such variations and modifications may involve equivalent and other features, which are already known in the art, and which may be used instead of, or in addition to, features already described herein.
(96) Although the appended claims are directed to particular combinations of features, it should be understood that the scope of the disclosure of the present invention also includes any novel feature or any novel combination of features disclosed herein either explicitly or implicitly or any generalisation thereof, whether or not it relates to the same invention as presently claimed in any claim and whether or not it mitigates any or all of the same technical problems as does the present invention.
(97) Features which are described in the context of separate embodiments may also be provided in combination in a single embodiment. Conversely, various features which are, for brevity, described in the context of a single embodiment, may also be provided separately or in any suitable sub-combination.
(98) For the sake of completeness it is also stated that the term “comprising” does not exclude other elements or steps, the term “a” or “an” does not exclude a plurality, and any reference signs in the claims shall not be construed as limiting the scope of the claims.