DIFFRACTIVE IMAGING MAGNETO-OPTICAL SYSTEM
20220373452 · 2022-11-24
Assignee
Inventors
Cpc classification
G01R33/032
PHYSICS
G01N21/1717
PHYSICS
G01R33/0017
PHYSICS
International classification
Abstract
A system for imaging, including a source of coherent light; a polarization state generator for generating polarized optical photons from the light originating in the source of coherent light; a sample environment; a polarization state analyzer for permitting photons having a desired polarization to interact with a detector; and an imaging unit for generating an image based on the interactions of the photons with the detector. The sample environment includes a plurality of electromagnets, each connected to one or more power supply components; and a controller, connected to the electromagnets and including software for generating and controlling a desired magnetic field created by each of the electromagnets in concert with each other.
Claims
1. A system for imaging, comprising: a source of coherent light; a polarization state generator for generating polarized optical photons from the light originating in the source of coherent light; a sample environment, comprising a plurality of electromagnets, each connected to one or more power supply components via one or more electronic circuits for supplying voltage to the plurality of electromagnets to generate a desired magnetic field; and a controller, connected to the electromagnets and including software for generating and controlling the desired magnetic field created by each of the plurality of electromagnets in concert with each other; a polarization state analyzer for permitting photons having a desired polarization to interact with a detector; and an imaging unit for generating an image based on the interactions of the photons with the detector; wherein the sample environment creates a multi-pole complex magnetic field having variable shape, variable amplitude, and variable frequency.
2. (canceled)
3. (canceled)
4. (canceled)
5. The system of claim 1, wherein the sample environment creates a rotated magnetic field.
6. The system of claim 5, wherein the rotated magnetic field has a magnetic flux density of 0.5 T and a frequency of up to 60 KHz.
7. The system of claim 1, wherein the sample environment further comprises a sample holder positioned such that the plurality of electromagnets surround the sample holder.
8. The system of claim 1, wherein each of the plurality of electromagnets are held within a magnet holder and located in a magnet housing positioned to surround a sample holder in the sample environment.
9. The system of claim 8, wherein the magnet housing is rotatable around the sample holder.
10. The system of claim 8, wherein the magnet housing has an octagonal shape or an annular shape.
11. (canceled)
12. The system of claim 1, further comprising one or more filtering optics positioned between the polarization state generator and the sample environment.
13. The system of claim 1, further comprising one or more collimating optics positioned between the polarization state generator and the sample environment.
14. The system of claim 1, further comprising one or more alignment mirrors positioned between the polarization state generator and the sample environment.
15. The system of claim 1, wherein the sample environment is a cryo-free environment.
16. The system of claim 1, wherein the polarization state analyzer is reconfigurable between a plurality of modes.
17. The system of claim 16, wherein the plurality of modes of the polarization state analyzer comprises an imaging mode and a diffraction mode.
18. (canceled)
19. A method of creating Neel type skyrmion domains in a sample, comprising: placing the sample in a sample environment, the sample environment comprising: a sample holder; and a plurality of electromagnets arranged to surround the sample holder; and applying a rotated magnetic field generated by the plurality of electromagnets to the sample to induce bubble skyrmionic polarization dipole textures in the sample.
20. The method of claim 19, wherein the sample environment further comprises: one or more power supply components connected to each of the plurality of electromagnets; one or more electronic circuits to bridge the one or more power supply components to the electromagnets; wherein the electronic circuits supply voltage pulses to the electromagnets to generate the rotated magnetic field; and a controller, connected to the electromagnets and including software for controlling the magnetic field.
21. The method of claim 19, wherein the sample environment is a cryo-free environment.
22. The method of claim 19, wherein the rotated magnetic field has a magnetic flux density of 0.5 T and a frequency of up to 60 KHz.
23. The method of claim 19, wherein the sample comprises a uniaxial centrosymmetric ferromagnetic thin-film material.
24. The method of claim 23, wherein the sample comprises Y.sub.3Fe.sub.5O.sub.12.
25. A system for imaging, comprising: a source of coherent light; a polarization state generator for generating polarized optical photons from the light originating in the source of coherent light; a sample environment, comprising a sample holder; a plurality of electromagnets, each connected to one or more power supply components, each of the plurality of electromagnets are held within a magnet holder and located in a magnet housing positioned to surround the sample holder, the magnet housing is rotatable around the sample holder; and a controller, connected to the electromagnets and including software for generating and controlling a desired magnetic field created by each of the electromagnets in concert with each other; a polarization state analyzer for permitting photons having a desired polarization to interact with a detector; and an imaging unit for generating an image based on the interactions of the photons with the detector.
Description
BRIEF DESCRIPTION OF DRAWINGS:
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DETAILED DESCRIPTION
[0037] Accordingly, embodiments of the present technology are directed to a programmable multi-pole magnet device that can be applied in magneto-electronic devices, magnetic microscopy and magnetic imaging microscopes, diffraction microscopy, super-resolution birefringent diffractive imaging (“Sr-BDP”) (which generates contrast via computer processing of polarized light scattered differently by tissues with different birefringences, and enables tissue and cell imaging in-vivo without staining or abusive contrast agents), synchrotron imaging and spectroscopy, biomedical research on drug delivery, space research and engineering, and device testing and reconfiguration. Some embodiments achieve the same results at room temperature that Faraday and Kerr microscopes achieve, but without the need for the bulky cooling chambers of Faraday and Kerr microscopes.
[0038] In some embodiments, the programmable multi-pole magnet device includes an arrangement of electro-magnets on electro-magnet holders that are used to induce magnetism and to control the configuration of magnetization in materials such as thin films, heterostructures and bulk crystals. In some embodiments, the components that comprise the magnet device are: electro-magnet holders, an arrangement of electromagnets attached to electro-magnet holders, power supply, electronic circuit, a microcontroller, and a control system for the device control. Generally speaking, these components are structured, in some embodiments, such that the microcontroller controls the electronic circuit that allows the delivery of voltage pulses with variable shape, amplitude, and frequency from the power source to the individual electro-magnets. In some embodiments, the microcontroller controls the electronic circuit that permits control of the supply voltage in a programmable way, while the electronic circuit bridges the power supply with individual electro-magnets, thus supplying them with voltage to generate a reproducible complex configuration of the magnetization on the material. Preferably, this architecture allows the system to supply a multi-pole complex magnetic field configuration with variable shape, amplitude, and frequency to the sample material.
[0039] In some embodiments, the programmable multi-pole magnet device is a CDIMOM 10 that is capable of both generating complex topologies of magnetic textured polarization and also imaging these textures, as shown in
[0040] Preferably, the polarization state generator block 11 creates tunable polarized (elliptical, horizontal, circular left/right, 45-degrees, etc.) optical photons. In some embodiments, the polarization state analyzer block 13 includes a detector 18, one or more polarization optics 19, and a microscope 20, as shown in
[0041] Some embodiments of the present technology comprise a compact CDIMOM 10 for sub-optical wavelength characterization (imaging and diffraction) of magnetic polarization. Some embodiments of the present technology include a programmable multi-pole magnetic setup that is capable of inducing bubble skyrmionic magnetic polarization dipole texture at room temperature in magnetic materials. Some embodiments include a method for inducing and imaging highly mobile topological magnetic spin textures in epitaxial magnetic films, for example, Y.sub.3Fe.sub.5O.sub.12 (“YIG”) thin films, permalloy, FePt, CoPd, and other films.
[0042] The embodiment shown in
[0043] Embodiments of the present technology are useful for academia, industry, and research laboratories that study complex magnetic materials for potential applications in elements of electronics, study magnetic materials and magnetic effects for application in medicine and biology, and perform fundamental research. The present technology is also useful for the space industry, where parts are exposed to varying magnetic fields, both during the design and testing cycles and during the quality control process. Other applications include engineering new magnetic domain textures and polarized coherent diffraction patterns to detect them in magneto-electronic devices, magnetic microscopy and magnetic imaging microscopes, diffraction microscopy, Sr-BDI, synchrotron imaging and spectroscopy, biomedical research on drug delivery, space research and engineering, and device testing and reconfiguration. The system can be integrated into synchrotron, microscopy, neutron, and magneto-electric instruments such as those used for device testing and for monitoring modifications of samples in real time.
[0044] The directional dependence of the index of refraction contains a wealth of information about anisotropic optical properties in magnetic, semiconducting, and insulating materials. Some embodiments of a CDIMOM according to the present technology provide a high-resolution lens-less technique that uses birefringence as a contrast mechanism to map the index of refraction and magnetic topological texture distribution in optically anisotropic materials.
[0045] In one embodiment, a CDIMOM based on optical birefringence was applied to a YIG film using polarized light from a helium neon laser. In other embodiments, this approach is applied to imaging with diffraction-limited resolution, including with the use of brilliant X-ray sources. Applications of this imaging technique are in electronic devices, for example, in which both charge and spin carry information as in multiferroic materials and photonic materials such as light modulators and optical storage.
[0046] Some embodiments of the present technology are directed to a Polarimetric Coherent Diffractive Imaging system. In anisotropic (magnetic, ferroelectric, semiconducting) materials with lower than cubic symmetry, the index of refraction, dielectric and susceptibility constant generally depends on the polarization and propagation direction of the traversing light. Properties of materials related to dichroism, depolarization, and birefringent can be reconstructed using iterative phase retrieval algorithms. An exemplary embodiment of the bottle-neck of this experimental setup is the presence of an analyzer 13 and a polarizer 11 in the scattering geometry of the experiment, with the sample 22 mounted between them as shown in
[0047] Some embodiments of the present technology are directed to a Birefringent Coherent Diffractive Imaging system. In magnetic materials with lower than cubic symmetry, the index of refraction generally depends on the polarization and propagation direction of the traversing light. This anisotropy is due to the directional dependence of material properties and the broken symmetry in the optical axes of these materials. The analysis of the propagation of light shows that uniaxial materials are characterized by two indices of refraction, one parallel to the optical axis n.sub.e, and two degenerate indices of refraction in the plane perpendicular to the optical axis n.sub.0. This phenomenon is known as Birefringence. The index of refraction for intermediate propagation directions interpolates smoothly between these two limiting values and is predictable from the laws of light propagation in optically anisotropic media. However, the limiting values themselves as well as their difference (birefringence) depend on material composition, crystallography, and symmetry. Capturing microscopic (local) 3-dimensional variations of the birefringence on a nanometer scale is challenging due to the limited resolution of lens based optical microscopy. In another embodiment of the present technology, a method is provided to overcome this limitation by using birefringence as a contrast mechanism for imaging the variability of optical properties in materials with nanometer resolution. A wide variety of materials including magnetic, liquid crystals, polymers and other soft matter show birefringence due to anisotropically distributed bonds. In condensed matter systems with magnetic, ferroelectric, and even multiferroic properties, birefringence can be manifested as electro- and magneto-optical phenomena which can play key roles in photonic technology enabling light modulators, optical data storage, sensors, and numerous spectroscopic techniques.
[0048] In some embodiments, the CDIMOM 10 of
[0049] In some embodiments, a Fienup hybrid input output (“HIO”) algorithm was used to reconstruct the birefringent density maps and light illumination probe. The square-root values of the integrated diffraction intensities are used as constraints in reciprocal space. In some embodiments, reconstructions are performed by starting from an array of random numbers and running 400 iterations of the HIO algorithm. It was noted on average after 300 iterations of the HIO algorithm, that the algorithm was circling around a solution region, so the final 100 iterations of the HIO algorithm were collected and averaged to produce a smoother and high quality reconstruction. The real space constraint reflecting the illumination region is generated from the pinhole scattering measurement with the aid of the Marchesini shrink wrap algorithm. In some embodiments, the real space constraint reflecting the illumination region is determined from an optical microscopic image of the pinhole aperture.
[0050] When light propagates through an optical media the polarization can change as a result of a change in the amplitude (dichroism) or phase shift (birefringence) of the electric vector. It is possible to determine the anisotropic properties of media determined from these two optical features. In some embodiments, Quantitative Birefringent Density Maps Δn (r) were obtaining by scaling the reconstructed phases Δϕ (r) by the calculated scaling factor. Some embodiments assume that the optical axis has a component that is uniaxial, planar oriented, and perpendicular to the propagation direction. Two directions of differential absorption are found and the intensity of the two distinct polarization direction of the transmitted beam in the sample is expressed in terms of the absorption coefficient along the ordinary direction α.sub.o and extraordinary direction α.sub.e:
II.sub.o=I.sub.0 exp[αod], l.sub.e=I.sub.0 exp[α.sub.ed] (1)
where I.sub.o and I.sub.e are transmitted intensities along the ordinary and extraordinary directions, respectively, and d is the thickness of the sample. Since the arbitrarily polarization states of photons β that enter the sample suffer a retardation and if the embodiment is well aligned with the principal axis of the component, then the Jones matrix J, corresponding to that of a retarder with real refractive index n.sub.1 and n.sub.2, is obtainable. Some embodiments account for the complex absorption in both principle directions, by introducing the correction: n.sub.1=n.sub.e+ik.sub.e and n.sub.2=n.sub.o+ik.sub.o. To determine the relationship between the complex part of the index of refraction k.sub.i and the absorption coefficients α.sub.i, embodiments having the sample illuminated with a vertically polarized photon beam corresponding to the quantum mechanical vector state represented in Jones notation is used.
[0051] In some embodiments, to characterize the quality of the reconstructed magnetic textures in the drawing figures, the concept of the phase retrieval transfer function (“PRTF”) is used. The PRTF defined as the ratio of the reconstructed diffraction amplitude (the absolute value of the Fourier transform of the reconstruction) to the measured diffraction amplitude as a function of momentum transfer. PRTF is a success metrics used to assess the fidelity and quality of the reconstruction. From PRTF one can judge on the range of frequencies over which the reconstructed information can be trusted with given confidence. There are a number of contributions that compromise the reconstruction, such as camera noise, mechanical instability of the equipment, and light source stability over the measurements time.
[0052] In some embodiments, given a reconstructed complex image S (r) obtained by phase retrieval starting from random phases, and its Fourier transform A (Q)=|A| exp {iϕ (Q)}, the PRTF is defined as:
PRTF(Q)=|A(Q))|/|I(Q)|I (2)
where I (Q) is the measured diffraction intensity, and denotes averaging over many independent reconstructions. The diffraction phases are averaged over constant frequency contours to produce the PRTF, which takes a value of 1 where the iterative algorithm consistently produced perfect convergence and a value near 0 where the algorithm continually failed to converge.
[0053] Some embodiments of the present technology are directed to systems and methods for the creation of Neel type skyrmion in uniaxial centrosymmetric ferromagnetic thin-film materials at room temperature. Some embodiments include a CDIMOM 10 tested on an optically transparent YIG thin film sample 22 in transmission scattering geometry. As shown in
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[0055] In some embodiments, the results are modeled through the following formulas. In the uniaxial ferromagnetic film with perpendicular easy axis, the basic Hamiltonian of the system is:
.sub.J=∫[K.sub.u(m.sub.1.sup.2+m.sub.2.sup.2)+J(∇m.sub.i).sup.2]dV, i=1, 2, 3 (3)
where K.sub.u represents the uniaxial energy coefficient, and J is the exchange energy constant. The demagnetic field energy is written as:
.sub.d=∫1/2∫H.sub.d.Math.mdV (4)
where H.sub.d is the stray field that is determined by the long-range interaction among the magnetic moments:
where r=|r−r′|. The Zeeman energy from the external applied field is .sub.ext=−∫H.sub.ext.Math.MdV. Thus, the total energy of the system is
=
.sub.J+
.sub.d+
.sub.ext. The temporal evolution of the magnetization configuration is obtained by solving the Landau-Lifshitz-Gilbert (“LLG”) equation:
where
is the effective magnetic field, and μ.sub.0 is the permeability of vacuum.
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[0059] Although the technology has been described and illustrated with respect to exemplary embodiments thereof, it should be understood by those skilled in the art that the foregoing and various other changes, omissions, and additions may be made there and thereto, without departing from the spirit and scope of the present technology.