SWITCHABLE RADIATION SOURCE
20190013109 ยท 2019-01-10
Assignee
Inventors
Cpc classification
International classification
Abstract
A switchable radiation source device includes a primary source assembly that emits primary radiation, and a target assembly in which, upon irradiation of the target assembly by the primary radiation, secondary radiation or radioactivity is produced. An alignment, proximity or exposure of the primary source assembly to the target assembly is adjustable to control irradiation of the target assembly by the primary radiation and thereby control the production of secondary radiation or radioactivity.
Claims
1. A switchable radiation source device comprising: a primary source assembly that emits primary radiation; and a target assembly in which, upon irradiation of the target assembly by the primary radiation, secondary radiation or radioactivity is produced; wherein an alignment, proximity or exposure of the primary source assembly to the target assembly is adjustable to control irradiation of the target assembly by the primary radiation and thereby control the production of secondary radiation or radioactivity.
2. The switchable radiation source of claim 1, wherein: the primary source assembly comprises at least one planar source tile; the target assembly comprises at least one planar target tile; and alignment of the source tile and target tile is adjustable by movement of the source tile or target tile.
3. The switchable radiation source of claim 1, wherein: the primary source assembly comprises at least one planar source tile; the target assembly comprises at least one planar target tile; and proximity of the source tile and target tile is adjustable by movement of the source tile or target tile.
4. The switchable radiation source of claim 1, wherein: the primary source assembly comprises a first planar array of separated multiple source tiles; the target assembly comprises a second planar array of separated multiple target tiles; and alignment of the source tiles and target tiles is adjustable by movement of at least one of the first planar array and second planar array.
5. The switchable radiation source of claim 4, wherein the first planar array is a rectangular array having rows in which interstitial blank cells are placed between the source tiles.
6. The switchable radiation source of claim 1, further comprising a shielding shell, wherein: the primary source assembly comprises a shell that at least partially encloses the target assembly; and the shielding shell is movable by rotation or translation between the primary source assembly and target assembly.
7. The switchable radiation source of claim 6, wherein the shielding shell is shaped as a spherical portion that at least partially encloses the target assembly, and the shielding shell is movable by relative rotation between the primary source assembly and target assembly.
8. The switchable radiation source of claim 7, wherein: the primary source assembly comprises an outer hemispherical shell; the shielding shell comprises an intermediate hemispherical shell between the outer hemispherical shell and the target assembly; and the target assembly comprises an at least partially spherical core concentric with the outer hemispherical shell and intermediate hemispherical shell.
9. The switchable radiation source of claim 1, further comprising a shielding plate, wherein: the primary source assembly has a planar shape; the target assembly has a planar shape parallel to and spaced from the primary source; and the shielding plate is movable between the primary source assembly and the target assembly to adjust exposure of the primary source assembly to the target assembly and thereby control the production of secondary radiation or radioactivity.
10. The switchable radiation source of claim 9, wherein the primary source assembly has a forward active side and a rear inactive side, and wherein the forward active side faces the target assembly.
11. The switchable radiation source of claim 1, wherein the primary source assembly emits primary radiation by natural radioactive decay.
12. The switchable radiation source device of claim 1, wherein the primary source assembly comprises an alpha particle emitter.
13. The switchable radiation source device of claim 12, wherein the secondary radiation or radioactivity causes ejection of one or more neutrons.
14. The switchable radiation source device of claim 13, wherein the target assembly comprises a stable isotope and irradiation of the target assembly by the primary radiation creates a compound nucleus and the one or more neutrons.
15. The switchable radiation source device of claim 1, wherein the target assembly comprises a circular arrangement of multiple target panels, and the primary source assembly comprises a source panel relative to which the circular arrangement of multiple target panels is rotatable.
16. The switchable radiation source device of claim 15, wherein the multiple target panels comprise different respective target materials.
17. The switchable radiation source device of claim 15, wherein the target assembly comprises an annular base ring upon which the multiple target panels are mounted in the circular arrangement.
18. The switchable radiation source device of claim 17, wherein the switchable radiation source device is operated by rotary movement of the annular base ring relative to the source panel to at least partially align a selected target panel with the source panel.
19. The switchable radiation source device of claim 16, wherein the source panel comprises an alpha-emitting radioactive isotope.
20. The switchable radiation source device of claim 19, wherein the secondary radiation or radioactivity causes ejection of one or more neutrons and the energy of the one or more neutrons varies according to the different respective target materials.
Description
BRIEF DESCRIPTION OF THE DRAWINGS
[0020] The previous summary and the following detailed descriptions are to be read in view of the drawings, which illustrate particular exemplary embodiments and features as briefly described below. The summary and detailed descriptions, however, are not limited to only those embodiments and features explicitly illustrated.
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DETAILED DESCRIPTIONS
[0043] These descriptions are presented with sufficient details to provide an understanding of one or more particular embodiments of broader inventive subject matters. These descriptions expound upon and exemplify particular features of those particular embodiments without limiting the inventive subject matters to the explicitly described embodiments and features. Considerations in view of these descriptions will likely give rise to additional and similar embodiments and features without departing from the scope of the inventive subject matters. Although the term step may be expressly used or implied relating to features of processes or methods, no implication is made of any particular order or sequence among such expressed or implied steps unless an order or sequence is explicitly stated.
[0044] Any dimensions expressed or implied in the drawings and these descriptions are provided for exemplary purposes. Thus, not all embodiments within the scope of the drawings and these descriptions are made according to such exemplary dimensions. The drawings are not made necessarily to scale. Thus, not all embodiments within the scope of the drawings and these descriptions are made according to the apparent scale of the drawings with regard to relative dimensions in the drawings. However, for each drawing, at least one embodiment is made according to the apparent relative scale of the drawing.
[0045] In at least one embodiment, Alpha-capture reactions are used in source generation applications. A reaction is produced by having an alpha emitting isotope bombard a stable isotope, creating a compound nucleus between an alpha particle and the target nucleus. The compound nucleus will be in an excited state, and emit gammas, neutrons, and or protons depending on the target material. Target materials are specifically chosen that will emit the desired type of radiation after alpha-capture; the energy of the radiation may also vary by changing the target material. The amount of each type of radiation produced depends on the energy of the alpha particle and the target material. A thin sheet of non-metallic shielding material may be used to screen or block alpha particles from hitting the target, thus acting as an attenuator or a switch for the source generator. The non-metallic material may be moved by an actuator operated by or switched according to an electric signal.
[0046] The device may be scaled to allow for different intensities of radiation. Increasing the activity of the alpha source will result in more radiation produced by the target material through alpha capture reactions.
[0047] These descriptions detail an approach to experimental validation of previous alpha-capture cross section values and comparison to the analytical values approximated by using Hauser-Feshbach calculations. These values are then compared to analytical validated cross sections found in the NON-SMOKER database, which contains statistical model results for a range of nuclei. These cross sections are dependent on the energy of the alpha particle. This energy will vary due to different alpha sources being used. The activity of the alpha source will depend on the geometry used and the alpha flux needed for irradiation. Due to the alpha-capture cross section of the target materials being energy dependent on the alpha particle, reaction rates will be calculated for each independent source. The energy of the gammas, neutrons, and protons are dependent on the energy of the alpha particle, binding energy of the stable target, and electron structure of the stable target.
[0048] Alpha-capture cross sections for X(,)Y are evaluated experimentally using multiple alpha sources and foil targets. The different alpha sources and materials are listed in Table 1. An alpha source geometry example is provided in
[0049] Within Equation 1, compound nucleus values are used to analytically obtain the capture cross section. The summation occurs over the angular momentum values of the alpha particle, ranging from zero to n, which is the maximum angular momentum quantum number. The change in angular momentum, denoted as 1, of the alpha particle from the ground state. The intrinsic spin of the alpha particle, denoted by s.sub.1, interacting with the target nucleus as the angular momentum changes through the summation, which is constant. The wavelength of the alpha particle is . The wave number just after the alpha particle enters the target nucleus is K. The compound nucleus radius of the alpha particle and the target is R. R and K remain constant throughout the summation. Equation 1 is generally true for any target atom, but has been used specifically for finding alpha-capture cross sections.
[0050] The alpha-capture cross section obtained from NON-SMOKER database was used as the microscopic capture cross section in Equation 2 to determine the expected activation of the foil targets. The flux used in Equation 2 varies depending on the activity of the alpha sources. The decay constant in Equation 2 is the decay constant of the newly formed compound nucleus after alpha capture, and t is the activation time. Equation 2 was integrated over time to determine the expected counts from alpha-activation. Using an activation time of 24 hours, the integral of Equation 2 predicts the number of counts emitted from the reaction.
[0051] Experimental Cross Sections and Theoretical Yields of Target Materials:
[0052] Analytical validation has been done and cross sections have been obtained from the NON-SMOKER database. Values for cross sections for multiple proposed foil target materials were found (see Appendix 1 of U.S. Provisional Patent Application 62/529,583).
[0053] Alpha Sources and Target Materials:
[0054] Multiple isotopes for the alpha source may be implemented based upon the desired emission rates of different particles. The nuclear properties of the alpha sources are listed in Table 1. Alpha particle energies and their half-lives are included in Table 1.
TABLE-US-00001 TABLE 1 Alpha source properties Alpha Energy Half-life Alpha (Mev) (years) .sup.148Gd 3.182 71.1 .sup.210Po 5.3044 0.379112329 .sup.226Ra 4.7844 1600 .sup.228Th 5.423 1.9116 .sup.229Th 4.5845 7880 .sup.231Pa 5.013 32760 .sup.232U 5.3203 68.9 .sup.236Pu 5.7675 2.858 .sup.239Pu 5.156 24110 .sup.240Pu 5.1685 6561 .sup.241Am 5.4857 432.6 .sup.243Am 5.276 7364 .sup.242Cm 6.1127 0.446027397 .sup.243Cm 5.785 29.1 .sup.244Cm 5.8048 18.1 .sup.245Cm 5.362 8423 .sup.246Cm 5.386 4706 .sup.247Cm 4.87 15600000 .sup.248Cm 5.078 348000 .sup.249Cf 5.813 351 .sup.250Cf 6.0304 13.08 .sup.254Es 6.429 0.755342466
[0055] Target materials were chosen specifically for their transmutation products after absorbing an alpha particle. Equation 3 demonstrates an X(,)W reaction, Equation 4 demonstrates an X(a,n)W reaction, and Equation 5 demonstrates an X(a,p)W reaction. Table 2 lists the Initial material and the products produced. Table 3 and Table 4 contain nuclear properties of the target materials and the corresponding products.
+.sub.y.sup.zX.fwdarw..sub.y+2.sup.z+4W+(Equation 3)
+.sub.y.sup.zX.fwdarw..sub.y+2.sup.z+3W+n (Equation 4)
+.sub.y.sup.zX.fwdarw..sub.y+1.sup.z+3W+p (Equation 5)
[0056] In Equation 3, a is the alpha particle, y is the atomic number of the target material, z is the atomic mass of the target material, and is the photon emission from the reaction. X is the target material and W is the product of X after transmutation.
TABLE-US-00002 TABLE 2 Target materials and corresponding products Target Product Product (X) Product (, ) (, n) (, p) .sup.39K .sup.43Sc .sup.42Sc .sup.42Ca .sup.40K .sup.44Sc .sup.43Sc .sup.43Ca .sup.40Ca .sup.44Ti .sup.43Ti .sup.43Sc .sup.47Ti .sup.51Cr .sup.50Cr .sup.50V .sup.58Ni .sup.62Zn .sup.61Zn .sup.61Cu .sup.63Cu .sup.67Ga .sup.66Ga .sup.66Zn .sup.79Br .sup.83Rb .sup.82Rb .sup.82Kr .sup.48Ca .sup.52Ti .sup.51Ti .sup.51Sc
TABLE-US-00003 TABLE 3 Target material properties Target atomic (X) abundance weight .sup.39K 0.932581 38.96370649 .sup.40K 0.9 39.96399817 .sup.40Ca 0.96941 39.9626 .sup.47Ti 0.0744 46.95175879 .sup.58Ni 0.680769 57.93534241 .sup.63Cu 0.6915 62.92959772 .sup.79Br 0.5069 78.91833758 .sup.48Ca 0.00187 47.95252277
TABLE-US-00004 TABLE 4 Product nuclear properties Decay Constant gamma energy emission Product (W) Half-life (s) (s.sup.1) (Mev) rate .sup.42Sc 0.6813 1.02E+00 1524 0.000075 .sup.43Sc 14007.6 4.95E05 372.9 0.225 .sup.44Sc 14292 4.85E05 1157 0.999 .sup.51Sc 12.4 5.59E02 1437.3 0.52 .sup.42Ca stable 0 N/A N/A .sup.43Ca stable 0 N/A N/A .sup.44Ti 1.87E+09 3.71E10 78.3 0.964 .sup.51Ti 345.6 2.01E03 320.076 0.93 .sup.52Ti 102 6.80E03 124.45 0.917 .sup.53Ti 0.509 1.36E+00 2288 0.044 .sup.50V stable 0 N/A N/A .sup.50Cr stable 0 N/A N/A .sup.51Cr 2.39E+06 2.90E07 320 0.09 .sup.61Cu 12020.4 5.77E05 282.956 0.122 .sup.61Zn 89.1 7.78E03 475 0.165 .sup.62Zn 33192 2.09E05 596 0.26 .sup.66Zn stable 0 N/A N/A .sup.66Ga 34164 2.03E05 1039 0.37 .sup.67Ga 281759.04 2.46E06 93, 184, 300 0.38 .sup.82Kr stable 0 N/A N/A .sup.82Rb 75.45 9.19E03 776.5 0.1508 .sup.83Rb 7.45E+06 9.31E08 520 0.45
[0057] Device Geometry:
[0058] A switchable radioisotope source device can utilize alpha particles to irradiate stable target materials to emit photons, neutrons, and or protons. Depending on the need of the consumer and the application, the size and strength of the switchable isotope source device may be changed. The probability of producing each particle and product may be found in the preceding under Experimental Cross Sections and Theoretical Yields of Target Materials and in Appendix 1 of U.S. Provisional Patent Application 62/529,583, and are dependent on the alpha particle energy. Specific activities of the produced products may be between 1000 and 10000 Bq/g.
[0059]
[0060] As shown in
[0061] In at least one example according to
[0062] Switchable Source Device:
[0063]
[0064] In
[0065]
[0066]
[0067] While a square tile geometry is illustrated, other shapes that overlap into alignment and stagger out of alignment are within the scope of these descriptions. For example, other rectangular shapes other than squares may be used, and triangular, hexagonal, and other shapes may be used.
[0068] In
[0069] Spherical source:
[0070]
[0071] In the particularly illustrated design of
[0072] Plate with shielding:
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[0074] Expected Activities and Products:
[0075] The activities of activated foils were calculated using Mathcad 15 by utilizing coupled differential equations. The alpha-capture cross sections for each of the foil materials were interpolated for an energy of 5.48 MeV. Activities of activated foils were calculated for 1 Ci, 0.1 Ci, and 10 mCi sources of .sup.241Am. Based on the results, the activated material for spectroscopy is obtained using a 1 Ci .sup.241Am on nickel and copper foil targets. Potassium was disregarded due to it being a very reactive metal. These calculations are to show proof of concept for the switchable radioisotope and are to be used as a template to calculate product activities.
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[0077] Similar calculations as those for which the results are shown in
[0078] Nomenclature Listing:
[0079] a=isotope abundance
[0080] A.sub.t=activity
[0081] AW=atomic weight
[0082] l=angular momentum change
[0083] =decay constant
[0084] =alpha particle wavelength
[0085] K=Wave number inside target nuclear surface
[0086] l=angular momentum of alpha particle
[0087] m=mass
[0088] n=maximum angular momentum of alpha particle
[0089] N.sub.a=Avogadro's number
[0090] R=compound nuclear radius
[0091] s.sub.l=intrinsic spin of alpha particle
[0092] =flux
[0093] A reaction in the above or other embodiments as described below is produced by having an alpha emitting isotope bombard a stable isotope, creating a compound nucleus and the ejection of a neutron. Radiations such as gammas and or neutrons are then emitted depending on the target material. Target materials are specifically chosen that will emit the desired type of neutron energy after alpha-capture; the scattering angle of the radiation may also vary by changing the target material. The amount of each type of radiation produced depends on the energy of the alpha particle and the target material. A rotary device may be used to place targets in front of or away from alpha particles, thus acting as a switch for the neutron source generator. The rotary device may be moved through an electric signal or mechanically.
[0094] Alpha-capture cross sections for .sup.27Al(,n).sup.30P are evaluated experimentally using a 90 Ci .sup.241Am alpha source and foil targets. The .sup.241Am alpha source information is provided in
[0095] Cross sections found within ENDF were integrated over energy, then averaged to find the average interaction rate for each material depending on the starting energy of the alpha particle. This may be seen in Equation 6. The averaged cross section obtained from Equation 6 was used as the microscopic capture cross section in Equation 7 to determine the expected activation of the foil targets. The flux used in Equation 7 varies depending on the activity of the .sup.241Am source. The decay constant in Equation 7 is the decay constant of the newly formed compound nucleus after alpha capture, and t is the activation time. Equation 7 was integrated over time to determine the expected counts from alpha-activation. Using an activation time of 24 hours, the integral of Equation 7 predicts the number of counts incident on the NaI detector. Equation 8 is used to determine the neutron production rate from the foil and the expected count rate on the .sup.3He neutron detector.
[0096] Stopping power charts for each target material was used in combination with Srim & Trim to find the range of alpha particles in various target materials. This allowed the optimal target thickness to be determined. An example of a stopping power chart is provided in
[0097] Expected Neutron Production:
[0098] Calculating the neutron production rate for a foil target included the change in alpha energy as it moves through the foil target, secondary energy of the neutrons, angle of scattering, and energy dependent cross sections. Stopping power was used to determine the target thickness for the highest production rate. Simulations in SRIM were run to show the path alpha particles travel as they enter a .sup.27Al target, as seen in
[0099] For the simulation, one hundred thousand individual particles were run. Values for .sup.27Al were integrated and averaged to account for the change in energy of the alpha particle as it moves through the .sup.27Al target. Stopping power figures shown in
[0100] Experimental Cross Sections and Theoretical Yields:
[0101] Analytical validation has been done and cross sections have been obtained from the ENDF database. Values for cross sections for the proposed foil targets were determined. The cross sections were integrated then averaged to find expected interaction rates used in calculations.
[0102] Alpha Sources and Target Materials:
[0103] Multiple isotopes for the alpha source may be implemented based upon the desired emission rates of neutrons and their respective energy. The nuclear properties of the alpha sources are listed in Table 1 in the preceding. Alpha particle energies and their half-lives are included in the table.
[0104] Target materials were chosen specifically for their transmutation products after absorbing an alpha particle. Equation 9 demonstrates an X(,n)W reaction. Table 5 lists the initial material, the products produced, and the kinetic energy and scattering angle of the produced products. Table 6 and Table 7 contain nuclear properties of the target materials and the corresponding products.
+.sub.y.sup.zX.sub.y+2.sup.z+3W+n (Equation 9)
[0105] In Equation 9, a is the alpha particle, y is the atomic number of the target material, z is the atomic mass of the target material, and n is the neutron emission from the reaction. X is the target material and W is the product of X after transmutation.
TABLE-US-00005 TABLE 5 Target materials and corresponding products Target Product (X) (, n) .sup.9Be .sup.12C .sup.10Be .sup.13C .sup.19F .sup.22Na .sup.22Ne .sup.25Mg .sup.23Na .sup.26Al .sup.25Mg .sup.28Si .sup.27Al .sup.30P .sup.29Si .sup.32S .sup.41K .sup.44Sc .sup.45Sc .sup.48V .sup.48Ti .sup.51Cr .sup.51V .sup.54Mn
TABLE-US-00006 TABLE 6 Target material properties Target (X) abundance atomic weight .sup.9Be 1 9.01218207 .sup.10Be N/A 10.01353469 .sup.19F 1 18.9984031629 .sup.22Ne 0.0925 21.991385109 .sup.23Na 1 22.989769282 .sup.25Mg 0.1 24.98583696 .sup.27Al 1 26.98153841 .sup.29Si 0.04685 28.9764946652 .sup.41K 0.067302 40.961825258 .sup.45Sc 1 44.9559075 .sup.48Ti 0.7372 47.94794093 .sup.51V 0.9975 50.9439569
TABLE-US-00007 TABLE 7 Product nuclear properties gamma energy emission Product (W) Half-life (s) Decay (s) (Mev) rate .sup.12C Stable 0 N/A N/A .sup.13C Stable 0 N/A N/A .sup.22Na 82050365 8.45E09 1274 0.9994 .sup.25Mg Stable 0 N/A N/A .sup.26Al 2.26E+13 3.07E14 1808 0.9976 .sup.28Si Stable 0 N/A N/A .sup.30P 149.9 4.62E03 2235 0.00059 .sup.32S Stable 0 N/A N/A .sup.44Sc 14292 4.85E05 1157 0.999 .sup.48V 1.38E+06 5.02E07 983.5 0.9998 .sup.51Cr 2.39E+06 2.90E07 320 0.0919 .sup.54Mn 2.70E+07 2.57E08 834.8 0.9998
[0106] Device Geometry:
[0107] Above descriptions of particular embodiments of switchable source devices and the corresponding drawings are to be taken as cumulative with further embodiments. For example, a rotary switchable source device 500 according to at least one other embodiment is shown in
[0108] In
[0109] The rotary device 500 will allow for multiple neutron energies and fluxes depending on the target materials. The neutron flux generated by the target materials may be changed by changing the size and thickness of the targets, increasing the distance between the source and the target materials, and the strength of the source. The geometry of the rotary device and the materials may vary in size depending on the application.
[0110] Expected Activities and Products:
[0111] The activities of activated foils were calculated using Mathcad 15 by utilizing coupled differential equations. The alpha-capture cross sections for each of the foil materials were interpolated for an energy of 5.48 MeV. Activities of activated foils and neutron production rates were calculated for 1 Ci, 0.1 Ci, and 10 mCi sources of .sup.241Am. Each foil had a mass of 1 g.
[0112]
[0113] Similar calculations as those for which the results are shown in
[0114] Particular embodiments and features have been described with reference to the drawings. It is to be understood that these descriptions are not limited to any single embodiment or any particular set of features, and that similar embodiments and features may arise or modifications and additions may be made without departing from the scope of these descriptions and the spirit of the appended claims.