Ultrafast photomagnetic recording in a dielectric medium using anisotropic ions effective gilber damping
10037777 ยท 2018-07-31
Assignee
Inventors
Cpc classification
G11B5/676
PHYSICS
G11B7/24
PHYSICS
G11B2005/0021
PHYSICS
G11B5/658
PHYSICS
International classification
G11B11/00
PHYSICS
Abstract
A recording medium comprising a dielectric magnetic layer, the dielectric magnetic layer comprising anisotropic ions having a difference in a single ion contribution to magnetic anisotropy (?K/ion) between a ground state and an excited state of said anisotropic ions equal to at least 0.1 cm.sup.?1 (0.0124 meV/ion) at 20? C. (68? F.), wherein the effective Gilbert damping (?) of said dielectric magnetic layer is equal to at least 0.01.
Claims
1. A recording medium comprising at least one dielectric magnetic recording layer, the dielectric magnetic recording layer comprising anisotropic ions having a difference in a single ion contribution to magnetic anisotropy (?K/ion) between a ground state and an excited state of said anisotropic ions equal to at least 0.1 cm.sup.?1 (0.0124 meV/ion) at 20? C. (68? F.), wherein the effective Gilbert damping (?) of said dielectric magnetic recording layer is equal to at least 0.01.
2. The recording medium of claim 1, wherein the dielectric magnetic recording layer has an amorphous structure comprising 3d, 4d, 5d or 4f transition metal ions as the anisotropic ions.
3. The recording medium of claim 1, wherein the dielectric magnetic recording layer has a crystalline structure selected from a group comprising: ferrite (garnet, spinel, ortho- and hexaferrite, ferric borates, magnetite), perovskite, corundum, wurzite, zincblende, Heusler, cubic, hexagonal, tetragonal; wherein the dielectric magnetic recording layer is comprising 3d, 4d, 5d or 4f transition metal ions as the anisotropic ions.
4. The recording medium of claim 1, wherein the anisotropic ions are ions with non-zero spin and orbital degeneracy in their ground level, selected from a group comprising 3d ions Mn.sup.2+, Mn.sup.3+, Cr.sup.2+, Cr.sup.3+, Fe.sup.2+, Co.sup.2+, Co.sup.3+, Ni.sup.2+, Ni.sup.3+, 4d ions Ru.sup.3+, Ru.sup.4+ and 5d ions Ir.sup.3+, Ir.sup.4+, 4f ions Ce.sup.3+, Tb.sup.3+.
5. The recording medium of claim 1, wherein the dielectric magnetic recording layer further comprises additional elements selected from a group comprising: Ga, Ge, In, Sn, Sb, Ti, Bi.
6. The recording medium of claim 1, wherein the dielectric magnetic recording layer is provided on a substrate which is selected from a group comprising: GGG, MgO, Si, GaAs, SiC, GaN, SiO2, Al2O3 or glass.
7. The recording medium of claim 1, comprising a plurality of dielectric magnetic recording layers made of different materials.
8. The recording medium of claim 1, comprising a plurality of dielectric magnetic recording layers separated by non-magnetic or metallic spacer layers.
9. The recording medium of claim 1, wherein the dielectric magnetic recording layer has a thickness of not more than 10 ?m.
10. A method for ultrafast photomagnetic recording comprising: providing a recording medium comprising at least one dielectric magnetic recording layer, the dielectric magnetic recording layer comprising anisotropic ions having a difference in a single ion contribution to magnetic anisotropy (?K/ion) between a ground state and an excited state of said anisotropic ions equal to at least 0.1 cm.sup.?1 (0.0124 meV/ion) at 20? C. (68? F.), wherein the effective Gilbert damping (?) of said dielectric magnetic recording layer is equal to at least 0.01; illuminating said dielectric magnetic recording layer by a light pulses that have a pulse duration equal to not more than 100 ps; tuning a wavelength and a polarization of the light pulses to cause optical resonances excitation of said anisotropic ions, thereby inducing transitions to the excited states of said anisotropic ions of said dielectric magnetic recording layer.
11. A system for ultrafast photomagnetic recording comprising: a recording medium comprising a dielectric magnetic recording layer, the dielectric magnetic recording layer comprising anisotropic ions having a difference in a single ion contribution to magnetic anisotropy (?K/ion) between a ground state and an excited state of said anisotropic ions equal to at least 0.1 cm.sup.?1 (0.0124 meV/ion) at 20? C. (68? F.), wherein the effective Gilbert damping (?) of said dielectric magnetic recording layer is equal to at least 0.01; a light source for emitting light pulses that have a pulse duration equal to not more than 100 ps; a polarizer for polarizing light output from said light source; a light guide for directing the polarized light to the recording medium to cause optical resonances excitation of said anisotropic ions, thereby inducing transitions to the excited states of said anisotropic ions of said dielectric magnetic recording layer.
12. The system of claim 11 embedded in a hard disk drive (HDD).
13. The system of claim 11 embedded in a random-access memory (RAM) chip.
14. The system of claim 11, further comprising a near-field transducer for coupling the light from the light guide to the recording medium.
15. The system of claim 11, wherein the light source is a diode laser, Vertical-Cavity Surface-Emitting-Laser (VCSEL), a quantum well, a quantum dot based laser or a sub-wavelength plasmonic nanoparticle laser.
16. The system of claim 11, wherein the light source comprises two light sources connected in series, configured to emit different light wavelengths, wherein the wavelength of the first light source is tuned to the anisotropic ions resonances in the dielectric magnetic recording layer, whereas wavelength of the second light source is different from the wavelength of the first light source and detuned from the ions resonances.
17. The system of claim 11, further comprising a magnetic tunnel junction magnetically coupled to the dielectric recording layer and means for reading a resistance of the magnetic tunnel junction to effect bit state reading.
Description
BRIEF DESCRIPTION OF DRAWINGS
(1) The present disclosure is accompanied by drawings, in which:
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NOTATION AND NOMENCLATURE
(14) Terms such as processing or creating or transferring or executing or determining or detecting or obtaining or selecting or calculating or generating or the like, refer to the action and processes of a computer system that manipulates and transforms data represented as physical (electronic) quantities within the computer's registers and memories into other data similarly represented as physical quantities within the memories or registers or other such information storage.
(15) As used herein, the term example means serving as a non-limiting example, instance, or illustration. As utilized herein, the terms for example and e.g. introduce a list of one or more non-limiting examples, instances, or illustrations.
(16) As used herein, the term ultrafast means femtosecond and picosecond time scale.
(17) As used herein, the term ultrashort laser pulse means pulses with durations of femtoseconds or picoseconds
DETAILED DESCRIPTION
(18) This disclosure relates to a method for performing ultrafast magnetic recording in an all-optical manner, using only single laser pulses and employing a dielectric recording medium, under no external magnetic field required for the magnetization switching. The method is based on a novel physical mechanism and it offers vast speed and energy-efficiency improvements over state-of-the-art.
(19) This disclosure also relates generally to a magnetic recording system based on the presented method. The system can be employed in a Hard Disk Drive (HDD) or a magnetic Random Access Memory (RAM). As such, the presented method and system significantly simplify magnetic recording as they remove the need for a use of magnetic coils, which are typically used for a bit writing operation in modem HDDs and suffer from limited operation speed.
(20) The photomagnetic effect, as typically reported in the scientific literature, is not an ultrafast phenomenon, but rather relates to slow, light-induced domain wall motion or the changes of magnetic permeability under continuous-wave (CW) laser illumination on the timescale of seconds. It will be shown in this disclosure how the magnitude of the effect can be enhanced, thus allowing ultrafast photo-magnetic recording, by using ultrashort laser pulses for the excitation, instead of a CW laser. Since such ultrashort laser pulses have orders of magnitude larger peak power and the pulse energy is concentrated only in a very brief moment of time, this makes the excitation both ultrastrong and ultrafast. Then one can achieve a significantly larger concentration of excited ions in comparison to CW-laser excitation (before the ions relaxation can have its effect) and thus also achieve much larger amplitude of the light-induced anisotropy field. The change of magnetic anisotropy is then sufficient to trigger ultrafast magnetization switching.
(21) The ultrafast photomagnetic effect, which is employed for the recording here, is a general effect which can be engineered in various dielectric materials. Thus, the all-optical recording as described herein can be also performed for other dielectric materials besides YIG:Co presented as an example only.
(22) The general requirements for the materials engineering of photomagnetic recording medium useful for the presented method and system are: dielectric (for the nonthermal dynamics), large Gilbert damping ?>0.01 (to stop the excited magnetization motion at the final state after switching), the material is hosting strongly anisotropic, light sensitive ions; wherein the ions possess an optical resonance which can be excited by tuning the laser pulse wavelength and polarization, thus inducing transition from the ground to the excited state of the ions; wherein the ground and excited states have different contribution to the single ion magnetic anisotropy (?K/ion>0.1 cm.sup.?1 or 0.0124 meV/ion at 20? C. (68? F.), i.e. at a room temperature).
(23) By tuning the laser light wavelength, polarization and intensity one can excite optical transitions of these ions, change their electronic configuration and consequently also their contribution, to the magnetic anisotropy, thus manipulating the energetically-preferred magnetization direction.
(24) In general, the dielectric magnetic medium can be amorphous in structure, as well as crystalline (single or polycrystalline). Examples of suitable materials are ferrites (garnet, spinel, ortho- and hexaferrites, ferric borates, magnetite), perovskites, Heusler compounds, spin glasses or transition metal oxides. The anisotropic ions with strong contribution to single ion anisotropy are typically 3d, 4d, 5d or 4f transition metal ions, especially ions with non-zero spin and orbital degeneracy in their ground level. Examples of appropriate ions are 3d ions Mn.sup.2+, Mn.sup.3+, Cr.sup.2 +, Cr.sup.3+, Fe.sup.2+, Co.sup.2+, Co.sup.3+, Ni.sup.2+, Ni.sup.3+, 4d ions Ru.sup.3+, Ru.sup.4+ and 5d ions Ir.sup.3+, Ir.sup.4+, 4f ions Ce.sup.3+, Tb.sup.3+.
(25) A particular instance of a suitable material is silicone-doped garnet YIG:Si (due to the Fe.sup.2+ ions), cobalt-doped garnet YIG:Co (Co.sup.2+ and Co.sup.3+ ions) or cobalt spinel CoFe.sub.2O.sub.4 (Co.sup.2+ ions). The dielectric recording medium properties can also be modified by the use of other ionsfor instance, the YIG:Co system magnetic and optical properties can by fine-tuned by doping with Ge.sup.4+, Ti.sup.4+ and Bi.sup.3+ ions. The disclosed method can also be used in antiferromagnetic materials (two magnetic sublattices with equal and opposite magnetic moments, yielding zero net magnetization).
(26) As an example, the all-optical recording will be demonstrated in a cobalt-substituted yttrium iron garnet (YIG:Co), which is an optically transparent dielectric with a cubic lattice and ferrimagnetic ordering due to two antiferromagnetically coupled spin sublattices of Fe.sup.3+ in both tetrahedral and octahedral sites. The Co ions substitute Fe ions and are responsible for a strong magnetocrystalline and photo-induced magnetic anisotropy as well as for a very large Gilbert damping ?=0.2.
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(28) The magnetization switching results were obtained on YIG:Co film d=7.5 ?m thick with composition Y.sub.2CaFe.sub.3.9Co.sub.0.1GeO.sub.12. The single-crystal YIG:Co garnet film was grown by liquid-phase epitaxy on GGGgadolinium gallium garnet Gd.sub.3Ga.sub.5O.sub.12 (001)-oriented substrates of 400 ?m thickness. The saturation magnetization at room temperature was 4? MS=90 G and the N?el temperature was 445 K.
(29) In an unperturbed state at room temperature, the equilibrium orientation of the magnetization is defined by cubic (K.sub.t=8.4?10.sup.3 erg cm.sup.?3) and uniaxial (K.sub.U=?2.5?10.sup.3erg cm.sup.31 3) anisotropy, which favor orientation of the magnetization along one of the body diagonals of the cubic cell (<111> -type of axes) and perpendicular to the [001] axis, respectively. For easier distinction between different magnetic domains, a garnet film is used with a miscut of 4? towards the [001] axis. The large stripe-like domains have magnetizations along M.sup.(L)+ near the [1-11] and M.sup.(L)? near the [11-1] axes and the small labyrinth-like domains have magnetizations along M.sup.(S)+ near the [111] and M.sup.(S)? the [1-1-1] axes [1].
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(32) Taking the difference between the images underlines the photo-magnetic changes and is used for detailed analysis. Light can lift the degeneracy between the domains by generating photo-induced magnetic anisotropy. In this case, pumping the initial pattern of magnetic domains with a single laser pulse polarized along the [100] axis (?=0?) turns large white domains (M.sup.(L)+) into large black ones (M.sup.(L)?). Simultaneously, small black domains (M.sup.(S)?) turn into small white ones (M.sup.(S)?). The domain pattern stays remarkably unperturbed, only the contrast reverses. The initial state can be restored by pumping with a single laser pulse polarized along the [010] axis (?=90?). The recorded domains are stable due to the non-zero coercivity of the garnet film at room temperature, as shown in
(33) The minimum pump fluence required for the magnetic recording in YIG:Co is very sensitive to the wavelength of the pump pulse. The switched area estimated from the magneto-optical images is plotted as a function of the pump fluence for different pump wavelengths, as shown in
(34) The wavelength was varied in the range between 1150 nm and 1450 nm (1.08-0.86 eV), where the light resonantly excites electronic d-d transitions in Co-ions (Reference [2]). In the YIG:Co film, a resonant pumping of the transitions in Co.sup.3+ and Co.sup.2+ ions at the tetrahedral sites at 1305 nm is accompanied by absorption of about 12% (?=0.12) of light energy. The spectral dependence in
(35) The inventors have observed that the ultrafast photomagnetic recording is spectrally tunable by selective pumping of different Co sublattices. Changing the pump wavelength within near infrared range and linear polarization of femtosecond laser pulses along [110] or [100] directions resonantly pumps the optical transitions in Co ions, as shown in
(36) To quantify the dynamics of the laser-induced changes, the inventors have studied the time-delay between the pump and probe pulses. It is seen that the recorded domain emerges with the characteristic time ? of about 20 ps and gets stabilized after about 60 ps (Reference [1]). In reality in YIG:Co film, the life-time of the photo-induced anisotropy at room temperature is also of the order of 60 ps (Reference [6]) and the damping is indeed very large, yielding ?=0.2 from FMR measurements. From the orientation of the linear polarization of the pump light which results in the recording it can be concluded that the photo-induced anisotropy originates from optical excitation of Co ions at tetrahedral sites (Reference [6]). Note that the amplitude of the spin precession induced by light is also at maximum when the linear polarization of light is along the [100] or the [010] axes thus supporting the above described mechanism.
(37) Additionally, the inventors found find that the threshold laser fluence required for the photomagnetic recording decreases with the thickness of garnet films, minimizing the heat load, as shown in
(38) As to why the cold photomagnetic recording is so extremely efficient, a simple answer follows from the argument that this method directly reduces the energy bather for switching. Other recording methods are based on either overcoming the energy barrier (as with applied field and spin-transfer torque) or trying to modify the barrier indirectly, as in the case of strong heating in HAMR, which is used to temporarily lower the coercivity, or the thermally-induced all-optical switching in the metallic systems. The photomagnetic recording approach is unique in the respect that the strongly anisotropic dopant Co ions, which are responsible for the magnetic anisotropy of YIG:Co, are resonantly excited by the laser pulses. Then the bulk of the light energy absorbed for the switching goes directly into the dopant Co ions for the modification of the energy barrier and thus extremely little energy is wastedthe dielectric matrix itself absorbs below few % of the incoming energy. The inventors have determined that the possibility of such resonant excitation is a unique feature of magnetic dielectrics, where any thermal effects are vastly limited in comparison to all-optical switching in metals.
(39) The recording medium can be provided on a substrate flamed by various materials, such as GGG, MgO, Si, GaAs, SIC, GaN, SiO.sub.2, Al.sub.2O.sub.3 or glass.
EXAMPLE EMBODIMENTS
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(41) In a typical HDD, the magnetic bits are recorded by applying the magnetic field pulses generated by the electrical current pulses running through the recording coil (writer) within the disk head. However, such approach is limited in terms of speed and maximum achievable magnetic field amplitude. For the high-density recording media used in the Heat Assisted Magnetic Recording (HAMR) HDDs, the disk head cannot produce sufficiently high magnetic field to switch the bits, making the thermal assist necessary to temporarily decrease the medium coercivity. The thermal assist is due to the sub-wavelength focusing of laser light on the selected bits within the recording medium by the means of a near-field transducer. However, this approach is still limited to the switching by magnetic field pulses, and thus limited in terms of speed.
(42) It will be shown in the following description how one can remove the coils from the HDD head and employ only laser light pulses for the all-optical recording in a magnetic dielectric material, provided the material fulfills the specified requirements. Additionally, the system enables minimum heat load on the dielectric recording medium under all-optical writing operations, as opposed to the thermally-driven all-optical switching in metallic systems, which require strong heating close to the Curie temperature for the laser-induced reversal.
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(45) Another embodiment of the recording system presented herein may further comprise a near-field transducer instead of the lens 44 for the focusing of the laser light below the optical diffraction limit, in order to switch nanometer-sized bits.
(46) In general, the recording medium may not only be a rotating disk as in HDD, but also an array of discrete memory cells as in a random access memory (RAM) or solid state drives (SSD). As the routing of laser pulses over chips presents logic-level restoration issues, a simpler approach is to employ a miniaturized light source integrated with the memory cell.
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(48) The light source 51 can be a simple miniaturized solid state source, such as a diode laser, Vertical-Cavity Surface-Emitting-Laser (VCSEL), a quantum well or a quantum dot based laser. A suitable light source can also be a sub-wavelength plasmonic nanoparticle laser with coupling of the near field plasmmonic mode to the far field optical mode, yielding photon emission into the recording layer 54. Depending on the particular type and dimensions of the laser source, the laser emission might not be direcional, thus requiring an external collimator 52 to efficiently couple the laser emission to the recording layer 54. This is especially relevant for the sub-wavelength laser sources.
(49) The memory cell comprises terminals for electrical communication with the memory controller. The write/read operation is achieved using a write pulse 49 and a read pulse 50. The write pulse has a larger magnitude than the read pulse and. thus represents the injection of larger current into the laser gain medium, producing a higher light emission intensity. The intensity of laser 51 emission under the write pulse 49 injection is sufficient to trigger the switching of the dielectric recording layer 54. However, the intensity of laser 54 emission under the read pulse 50 is lower and only sufficient to aquire a read signal 57 on the photodetector 56 for the magnetooptical reading operation, without triggering switching of the recording layer.
(50) In
(51) Additionally, a variation of the system embodiment presented in
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(53) While the invention presented herein has been depicted, described, and has been defined with reference to particular preferred embodiments, such references and examples of implementation in the foregoing specification do not imply any limitation on the invention. It will, however, be evident that various modifications and changes may be made thereto without departing from the broader scope of the technical concept. The presented preferred embodiments are exemplary only, and are not exhaustive of the scope of the technical concept presented herein. Accordingly, the scope of protection is not limited to the preferred embodiments described in the specification, but is only limited by the claims that follow.
REFERENCES
(54) [1] A. Stupakiewicz, K. Szerenos, D. Afanasiev, A. Kirilyuk, A. V. Kimel, Ultrafast nonthermal photo-magnetic recording in a transparent medium, Nature 542, 71 (2017). [2] Z. ?im?a, Optical and magnetooptical properties of Co-doped YIG films. Czech. J Phys. B 34, 78-87 (1984). [3] M. Savoini, R. Medapalli, B. Koene, A. R. Khorsand, L. Le Guyader, L. Du?, M. Finazzi, A. Tsukamoto, A. Itoh, F. bolting, A. Kirilyuk, A. V. Kimel, Th. Rasing, Highly efficient all-optical switching of magnetization in GdFeCo microstructures by interference-enhanced. absorption of light. Phys. Rev. B 86, 140404(R) (2012). [4] A. Hylick, R. Sohan, A. Rice, B. Jones, An Analysis of Hard Drive Energy Consumption, Proceedings of MASCOTS. IEEE Comp. Soc. 103-112 (2008). [5] K. L. Wang, J. G. Alzate, Amiri, P. Khalili, Low-power non-volatile spintronic memory: STT-RAM and beyond. J. Phys. D: Appl. Phys. 46, 074003 (2013). [6] F. Atoneche, A. M. Kalashnikova, A. V. Kimel, A. Stupakiewicz, A. Maziewski, A. Kirilyuk, Th. Rasing, Large ultrafast photoinduced magnetic anisotropy in a cobalt-substituted yttrium iron garnet. Phys. Rev. B 81, 214440 (2010).