Femtosecond laser excitation tagging anemometry
09863975 ยท 2018-01-09
Assignee
Inventors
- Richard B Miles (Princeton, NJ, US)
- Arthur Dogariu (Hamilton, NJ, US)
- James B Michael (Ames, IA, US)
- Matthew R Edwards (Santa Monica, CA, US)
Cpc classification
G01S17/58
PHYSICS
G01S17/74
PHYSICS
Y02A90/10
GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
G01P5/001
PHYSICS
International classification
G01S17/58
PHYSICS
G01P5/00
PHYSICS
G01S17/74
PHYSICS
Abstract
An apparatus for the imaging of gaseous fluid motion is disclosed. The apparatus includes a sub-nanosecond pulsed laser. The sub-nanosecond pulsed laser is configured to cause a particle species to fragment and for the recombining fragments subsequently to fluoresce. The apparatus also includes a gaseous fluid comprised of particle species. The apparatus also includes a time gated camera. The time gated camera configured to capture at least one image of the fluorescence from the recombining particle fragment species displaced after a specific time lapse following the laser pulse. Additionally, a fluid velocity can be calculated from a comparison of the image of the displaced particle species to an initial reference position and the time lapse. A Femtosecond Laser Electronic Excitation Tagging (FLEET) method of using the disclosed apparatus is also disclosed.
Claims
1. An apparatus for imaging of gaseous fluid motion comprising: a gaseous fluid comprising particle species; a sub-nanosecond pulsed laser configured to cause, in a single laser pulse, the particle species to fragment and recombining fragments subsequently to fluoresce; and a time gated camera wherein the time gated camera is configured to capture at least one image of the fluorescence from the recombining fragments displaced after a specific time lapse following the single laser pulse.
2. The apparatus of claim 1, wherein a fluid velocity is calculated from a comparison of the image of the displaced fragments to an initial reference position and the time lapse.
3. The apparatus of claim 1, wherein the laser is a sub-picosecond laser.
4. The apparatus of claim 1, wherein the laser has a pulse length below 250 fs.
5. The apparatus of claim 1, wherein the pulse from the pulsed laser has an energy above 1 mJ.
6. The apparatus of claim 1, wherein the time lapse is between about 0 s to about 20 s.
7. The apparatus of claim 1, wherein the time gated camera has a time gate of between 0 s to about 5 s.
8. The apparatus of claim 1, wherein the camera is configured to capture a plurality of time delayed images of the fluorescence, wherein a time sequenced series of images of the gaseous fluid motion is produced.
9. The apparatus of claim 1, wherein the camera also captures an image of a laser beam path during the laser pulse.
10. The apparatus of claim 1, further comprising a plurality of laser beams.
11. The apparatus of claim 1, wherein the camera simultaneously images the fluorescence from different angles.
12. The apparatus of claim 1, wherein the particle species comprises nitrogen.
13. The apparatus of claim 12, wherein the gaseous fluid comprises air.
14. The apparatus of claim 12, wherein the gaseous fluid comprises products of combustion in air.
15. A Femtosecond Laser Electronic Excitation Tagging (FLEET) method comprising: identifying a gaseous fluid comprising particle species; exposing the gaseous fluid to a single sub-nanosecond laser pulse to fragment the particle species and recombining fragments subsequently to fluoresce; capturing with a time gated camera at least one image of the fluoresced recombining fragments separated in time by a specific time lapse from an instant of exposure of the particle species to the single laser pulse; determining a displacement of at least one fluoresced fragment from its location at the time of the instant of exposure of the particle species to the single laser pulse and the instant of the image capture by the camera; and using the displacement and the specific time lapse to determine at least one velocity component of the gaseous fluid.
16. The FLEET method of claim 15, wherein the image of the fluoresced particle species is captured in a spectral range from approximately 560 to 660 nm.
17. The FLEET method of claim 15, wherein two time-gated cameras are used to capture images of the fluoresced particle species.
18. The FLEET method of claim 17, wherein the velocity of the gaseous fluid is determined in two or three dimensions.
19. The FLEET method of claim 15, wherein the laser has a pulse length below 1 picosecond.
20. The FLEET method of claim 15, wherein the pulse from the pulsed laser has an energy above 1 mJ.
21. The FLEET method of claim 15, wherein the time gated camera has a delay of between about 0 s to about 20 s after the laser pulse.
22. The FLEET method of claim 15, wherein the time gated camera has a time gate of between 0 s to about 5 s.
23. The FLEET method of claim 15 further comprising the following step: capturing a plurality of time delayed images of the fluorescence.
24. The FLEET method of claim 23 further comprising the following step: organizing the plurality of images into a time sequenced series of images of a gaseous fluid motion.
25. The FLEET method of claim 15 further comprising the following steps: capturing an image at the instant of exposure of the particle species to the laser pulse (T.sub.0 image); and using the T.sub.0 image to measure the displacement of at least one fluoresced fragment.
26. The FLEET method of claim 15 further comprising the following step: exposing the gaseous fluid to a laser pulse from an array of sub-nanosecond lasers to fluoresce the particle species.
27. The FLEET method of claim 15, comprising the following step: simultaneously capturing images of the fluorescing particle species from different angles.
28. The FLEET method of claim 15, wherein the particle species comprises nitrogen.
29. The FLEET method of claim 28, wherein the gaseous fluid comprises air.
30. The FLEET method of claim 28, wherein the gaseous fluid comprises products of combustion in air.
31. The apparatus of claim 1, wherein a line is written into the fluid by the laser and a fluid velocity profile is calculated from a comparison of the image of the line to an initial reference position and the time lapse.
32. The apparatus of claim 1, wherein a pattern is written into the fluid by the laser and fluid transport properties including at least one of velocity, vorticity, shear stress and dilatation are calculated from a comparison of the image of the pattern to an initial reference pattern and the time lapse.
33. The apparatus of claim 1, wherein the laser apparatus is pulsed multiple times and multiple images are recorded to determine fluctuating properties of the gaseous fluid motion.
34. The FLEET method of claim 15, further comprising: writing a line into the fluid by the laser and calculating a fluid velocity profile from a comparison of the image of the line to an initial reference position and the time lapse.
35. The FLEET method of claim 15, further comprising: writing a pattern into the fluid by the laser and calculating fluid transport properties including at least one of velocity, vorticity, shear stress and dilatation from a comparison of the image of the pattern to an initial reference pattern and the time lapse.
36. The FLEET method of claim 15, wherein fluctuating properties of fluid motion are determined by: causing the particles species to fragment and the recombining fragments subsequently to fluoresce multiple times; and capturing multiple images of the fluoresced recombining fragments.
Description
BRIEF DESCRIPTION OF FIGURES
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DETAILED DESCRIPTION OF THE INVENTION
(14) Definitions
(15) As used herein, the acronym FLEET refers to femtosecond laser electronic excitation tagging.
(16) As used herein, the initials PMT refers to a photomultiplier tube.
(17) As used herein, the initials ICCD refers to intensified charge-coupled device.
(18) As used herein, the initials psi refers to the unit of pressure: pounds per square inch. This unit can be converted into atmospheres which are abbreviated herein atm.
(19) As used herein, the term particle species refers to an atom or molecule that is fluoresced by a sub-nanosecond laser as described in techniques and apparatus disclosed. Herein, the terms Particle species and fluoresced species are used interchangeably.
(20) Disclosed is a process that uses nitrogen in naturally occurring air or other molecular species in a gaseous flow to create a line image whose displacement provides a precise measure of the flow velocity profile. The disclosed process uses a focused, sub nanosecond pulsed laser to dissociate molecules, producing atoms or other molecular fragments which subsequently recombine, producing fluorescence. The recombination and fluorescence processes last many microseconds, leading to fluorescence that persists for times long enough for the displacement for the flow to be recorded.
(21) The energy of the laser is low, and it is not tightly focused, so a long line (centimeters in length) can be excited without producing any spark or significant change in the nature of the flow. The laser does not need to be tuned into resonance with any specific molecular transition.
(22) For the quantification of the flow, the fluorescence is imaged by a time gated camera. The delay between the laser pulse and the gate time of the camera allows the flow to evolve before the image is taken.
(23) The disclosed process enables the measurement of flow velocity and other gas properties through femtosecond molecular tagging. The sub nanosecond laser has high intensity through the focal zone, which provides a mechanism for the excitation and/or dissociation of all molecular species that are naturally occurring in the flow through multi-photon absorption, so no seeding is required and the laser does not need to be tuned in frequency. In addition, the laser has a pulse length short enough and energy low enough to avoid breakdown, so long lines can be written without perturbing the flow in any significant manner. The process is robust to high temperatures and will operate over a wide range of pressures.
(24) The recombination of the molecular fragments takes many microseconds, so the displacement of the tagged line with time can be recorded with a camera. Time gating the camera provides the capability of following the precise location of the line as a function of the time following tagging. By accurately knowing the time between tagging and observation and measuring the line displacement distance, the velocity profile of the flow is determined. The vector component of the velocity profile measured is perpendicular to the line and in the plane normal to the camera axis. By focusing multiple laser beams into the flow or by refocusing a single beam, multiple lines, crosses and grid patterns can be written, and the measurement of their displacements provides a method for the measurement of other transport properties including vorticity, shear stress, dilatation, etc.
(25) Referring to
(26) This approach measures the velocity or the velocity profile in a single laser pulse, and thus can capture details of the turbulent character of the flow.
(27) To determine three dimensional movement, a second camera can be used. With the use of two or more cameras, a second component of the velocity profile can be simultaneously acquired. Additionally, the laser can be configured to produce a cross or pattern in the air for more precise or planar measurements of velocities.
(28) For applications in air, the predominant fluorescing species is nitrogen which is formed in an upper electronic state when two nitrogen atoms combine. The fluorescence from this state is in the red to infrared portion of the spectrum and due to the time required for the atoms to recombine, it persists for 25 microseconds in ambient pressure air. Lines have a width on the order of 50 microns. By fitting the transverse line profile, the line center can be determined to better than 10 microns, so even with a few microsecond delay, accurate measurements of the velocity profile can be made.
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(30) One embodiment features an apparatus for the imaging of gaseous fluid motion comprising: a sub nanosecond pulsed laser beam which is focused into the gaseous fluid such that some of the molecular species along the laser path through the focal zone are caused to be fragmented by nonlinear absorption of laser light. A time gated camera is implemented that is capable of imaging luminosity from said gaseous medium as the atomic or molecular fragments combine and emit light, thus providing an image of the displacement of the gaseous fluid due to its motion during the time interval between the laser fragmentation and the camera imaging. In many applications the gaseous fluid contains nitrogen for which the fragments are nitrogen atoms, which recombine emitting light in the red and near infrared portion of the visible spectrum. In many applications the gaseous fluid containing nitrogen is simply air. In other applications, the gaseous fluid contains the products of combustion in air. This basic configuration can be augmented to obtain additional information or provide additional features.
(31) For instance, the embodiment can further comprise a camera that captures multiple time delayed images of the emitted light, thus providing a time sequenced series of images of the motion of the gaseous fluid. From the image or images a velocity of fluoresced particles can be calculated. It can be extrapolated that the velocity of the fluoresced particles within the gaseous fluid is indicative of the movement of the gaseous fluid itself.
(32) In some embodiments of the basic configuration the apparatus also comprises a camera that captures an immediate image of the original laser beam path and a time delayed image of the emitted light, thus providing an undisplaced reference and a displaced image of the gaseous fluid so accurate measurement of the displacement can be achieved. In this configuration, again the velocity of fluorescent particles can be calculated from the image or images.
(33) Another embodiment is similar to the above but further features an array of sub-nanosecond laser beams such that a pattern of fragmented molecules is created and a time gated camera that images said pattern, providing further information on the motion of the gaseous fluid.
(34) In yet another embodiment of the basic configuration features more than one camera that simultaneously image the displacement of the molecular fragments from different angles, thus providing the capability for three dimensional tracking of the motion of the gaseous fluid.
(35) Another approach to acquire three dimensional tracking is to add to the basic configuration a single camera that simultaneously images the displacement of the molecular fragments from different angles, thus providing the capability for three dimensional tracking of the motion of the gaseous fluid.
(36) Laser
(37) Almost any extremely short duration laser that pulses with a duration under 1 nanosecond can be used with the described techniques and apparatus. It is understood and demonstrated that pulses with durations under 1 picosecond (ps) work well with the described techniques and apparatus. It is understood and demonstrated that pulses with durations under 250 femtosecond (fs) work well with the described techniques and apparatus. Some of the examples discussed herein use a laser configured to provide a pulse with a duration of about 120 fs.
(38) For some of the examples discussed here, fluorescence was obtained using an amplified 120 fs pulse from a Spectra-Physics Mai Tai titanium-sapphire oscillator and a Coherent Hidra Ti:sapphire amplifier with pulsed chirp compression. The system outputs 120 fs, 1.2 mJ pulses centered at 810 nm at a 10 Hz repetition frequency. The laser is focused by a 50 cm planoconvex lens in air to a beam waist of 30 m, resulting in a fluorescent region with a length of 1 cm. The intensity in the focal volume is approximately 110.sup.18 W per m.sup.2. Unless specified, this is the laser that was used in the examples contained herein.
(39) Sub-nanosecond lasers are well known in the art. These extremely short duration laser pulses are generally achieved through a technique referred to as mode-locking. The basis of the technique is to induce a fixed phase relationship between the modes of the laser's resonant cavity. The laser is then said to be phase-locked or mode-locked. Interference between these modes causes the laser light to be produced as a train of pulses. Depending on the properties of the laser, these pulses may be of extremely brief duration, as short as a few femtoseconds.
(40) Fluorescing Species and Fluorescence
(41) A number of researchers have observed relatively long-lived emission from nitrogen in flowing systemscommonly referred to as the nitrogen LewisRayleigh afterglow. Studies of nitrogen afterglow have been carried out in postglow discharges, postspark discharges, and postmicrowave discharges. These various generation methods have all shown evidence of significant populations of N(.sup.4S) atoms, which undergo three-body recombination to form unstable nitrogen N.sub.2(.sup.5.sup.+.sub.g) and subsequently, a vibrationally excited nitrogen B state (v.sup.011) as described by Eqs. (1) and (2):
N(.sup.4S)+N(.sup.4S)+M.fwdarw.N.sub.2(.sup.5.sub.g.sup.+)+M (1)
N.sub.2 (.sup.5.sub.g.sup.+)+M.fwdarw.N.sub.2(B.sup.3.sub.g)+M (2)
N.sub.2(B.sup.3.sub.g.sup.1).fwdarw.N.sub.2(A.sup.3.sub.u.sup.+, )+h. (3)
(42) C. R. Stanley was the first to observe this afterglow at near-atmospheric pressure, where the first positive emission of nitrogen was observed in the range of 560 to 700 nm. These features correspond to the v=3 and v=4 bands of the first positive system of nitrogen for the transitions described by the equation 3. Emission from these bands has been observed at up to atmospheric pressure. The recombining nitrogen atoms repopulate the nitrogen B state, allowing the emission to continue for relatively long durations. Similar emission from recombining fragments of other molecular species may as well be used for other embodiments of this invention.
(43) In order to utilize molecular fluorescence for velocity determination, relatively long-lived emission from the recombination process is beneficial. Measurements indicate the initial decay of the first positive nitrogen fluorescence signal in air and determine a lifetime of approximately 4 s by fitting an exponential. This signal arises from the initial formation of excited nitrogen molecules by the laser pulse. After that initial response, a long decay with a lifetime of tens of microseconds is observed. The long decay time associated with this emission is arises primarily from the time for atomic nitrogen to recombine into molecular nitrogen, a process that leads to molecular nitrogen in an electronically excited state. Examination of the fluorescence signal with a PMT and filter combination passing light from 560 to 660 nm resulted in good agreement with the signal recorded by sequentially time delayed images taken by the camera. As shown in
(44)
(45) The spectrum in the region of interest, from about 560 to 660 nm, exhibits features of the first positive system of nitrogen similar to those observed for flowing gas discharge systems at near-atmospheric pressures in nitrogen and air by previous investigators. (C. R. Stanley, A new method for the production of active nitrogen and its application to the study of collision effects in the nitrogen molecular spectrum, Proc. Phys. Soc. A 67, 821-827 (1954).
(46) J. F. Noxon, Active nitrogen at high pressure, J. Chem. Phys. 36, 926-940 (1962).
(47) K. D. Bayes and G. B. Kistiakowsky, On the mechanism of the Lewis-Rayleigh nitrogen afterglow, J. Chem. Phys. 32, 992-1000 (1960).)
(48) Camera
(49) The collection of images of the displaced emission for FLEET does not require any specific camera, although it does require a fast-gated camera with fast and accurate timing and average or better sensitivity. The emission is not particularly bright and in general would only be quantifiable while using an intensified camera. For accurate measurements coordinated timing is also important. Sub microsecond accuracy on image capture delay and width is necessary for accurate measurements. To produce displacement images which are sharp and focused, a camera gate of about 1 s or faster is preferable for typical flow velocities. If the described technique and apparatus are to be used for obtaining multiple images of the same line, a MHz rate camera is required since the emission last only microseconds.
(50) An example of a suitable camera for use with the described technique and apparatus is the PI-MAX 512 ICCD (Princeton Instruments). The camera can be configured to capture a 512 by 512 pixel image. The camera can also be focused to give a resolution of 20-100 m/pixel, which is a suitable resolution required to measure flow phenomena. The camera was modified to achieve the requisite timing. A laser timing system was added and configured Q-switch firing. The PI-Max is just one example of a suitable camera for use with the described techniques and apparatus. Other cameras have been successfully tested with the described system.
(51) Calculating Velocity of a Fluid
(52) The fact that the velocity is directly related to distance traveled in a known amount of time makes it possible to determine the instantaneous velocity. The calculation of the velocity uses the displacement and a time delay to the center of the 1 s intensifier gate width as the time offset. The displacement of the fluorescence line at each position from the original straight line as determined by a Rayleigh scattering image results in an instantaneous velocity profile across the jet for each image. For quantitative determination of the velocity contour, at each radial location across the image a Gaussian profile can be fitted by a least-squares routine to determine the line center. The velocity can then determined by the difference between these Gaussian center fits and the Gaussian fit to the undisplaced Rayleigh scattering line image.
(53) To verify that the intensifier gate width does not impact the determination of velocity, the gate width was varied between 300 ns and 1 s and mean velocity profiles over 50 shots was determined. As shown in
(54) Mean velocity profiles at different downstream locations above the nozzle exit are shown in
(55) These images can be used to determine the statistical properties of the flow. For example,
EXAMPLES
(56) The Examples presented herein are meant for an illustrative purpose and should not read as limiting of the claims that follow.
Example 1.
(57) Small Underexpanded Jet.
(58) FLEET was first demonstrated on a vertical 1 mm diameter free jet. The velocity at the jet exit was approximately 400 m/s, and the jet was mounted on a movable stage so that different regions of the flow could be imaged. The femtosecond laser was focused through a 50 cm plano-convex lens to a beam waste of 30 m. Images were taken at camera delays between 0 and 5 s and gate widths of 300 and 1000 ns. In
(59) Images captured using FLEET provide the ability to extract velocities from the data. Such velocities have been calculated from the images shown in
Example 2.
(60) Large Sonic Jet.
(61) Velocity measurements were taken in a 6 mm vertically oriented under expanded free jet, whose flow is depicted in
(62) The centerline velocity profile measured using FLEET is plotted in