1,5-DIPHENYLPYRAZOLYL-3-OXYALKYL ACIDS AND 1-PHENYL-5-THIENYLPYRAZOLYL-3-OXYALKYL ACIDS AND THE USE THEREOF FOR CONTROL OF UNWANTED PLANT GROWTH

Abstract

The present invention relates to novel herbicidally active, substituted 1,5-diphenylpyrazolyl-3-oxyalkyl acids and 1-phenyl-5-thienylpyrazolyl-3-oxyalkyl acids and derivatives thereof according to the general formula (I) or agrochemically acceptable salts thereof, to processes for preparation thereof and to the use thereof for control of broadleaved weeds and weed grasses in crops of useful plants and for general control of broadleaved weeds and weed grasses in areas of the environment where plant growth is troublesome. The derivatives of the 1,5-diphenylpyrazolyl-3-oxyalkyl acids and 1-phenyl-5-thienylpyrazolyl-3-oxyalkyl acids especially include the esters, salts and amides thereof.

Claims

1. A compound comprising a 1,5-Diphenylpyrazolyl-3-oxyalkyl acid and/or a 1-phenyl-5-thienylpyrazolyl-3-oxyalkyl acid of formula (I), and/or an agrochemically acceptable salt thereof, ##STR00028## where A is selected from the group consisting of A1-A3, ##STR00029## R.sup.1 is selected from the group consisting of OR.sup.1a and NR.sup.9R.sup.10; where R.sup.1a is selected from the group consisting of hydrogen; methyl, ethyl which is unsubstituted or substituted by one or more substituents selected from the group consisting of halogen, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.1-C.sub.4)-trialkylsilyl, (C.sub.1-C.sub.6)-alkoxy, cyano and nitro; (C.sub.2-C.sub.6)-alkenyl, (C.sub.2-C.sub.6)-haloalkenyl; (C.sub.2-C.sub.6)-alkynyl, (C.sub.3-C.sub.6)-cycloalkyl which is unsubstituted or substituted by one or more substituents selected from the group consisting of halogen, (C.sub.1-C.sub.6)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl; (C.sub.1-C.sub.4)-alkyl-SO—(C.sub.1-C.sub.4)-alkyl, (C.sub.1-C.sub.4)-alkyl-SO.sub.2—(C.sub.1-C.sub.4)-alkyl; heterocyclyl, heteroaryl and aryl which is unsubstituted or substituted by one or more substituents selected from the group consisting of halogen, (C.sub.1-C.sub.6)-alkyl, (C.sub.1-C.sub.6)-haloalkyl; heterocyclyl-(C.sub.1-C.sub.4)-alkyl, heteroaryl-(C.sub.1-C.sub.4)-alkyl and aryl-(C.sub.1-C.sub.4)-alkyl, where the heterocyclyl, heteroaryl and aryl is unsubstituted or substituted by one or more substituents selected from the group consisting of halogen, (C.sub.1-C.sub.6)-alkyl, (C.sub.1-C.sub.6)-haloalkyl; R.sup.9 is selected from the group consisting of hydrogen, (C.sub.1-C.sub.12)-alkyl; R.sup.10 is selected from the group consisting of hydrogen; aryl, heteroaryl, heterocyclyl, which is unsubstituted or substituted by one or more substituents selected from the group consisting of halogen, (C.sub.1-C.sub.6)-alkyl, (C.sub.1-C.sub.6)-haloalkyl; (C.sub.3-C.sub.7)-cycloalkyl-(C.sub.1-C.sub.4)-alkyl, heterocyclyl-(C.sub.1-C.sub.4)-alkyl, heteroaryl-(C.sub.1-C.sub.4)-alkyl, aryl-(C.sub.1-C.sub.4)-alkyl, aryl-(C.sub.1-C.sub.4)-alkoxy; where the cycloalkyl, heterocyclyl, heteroaryl and aryl is unsubstituted or substituted by one or more substituents selected from the group consisting of halogen, (C.sub.1-C.sub.6)-alkyl, (C.sub.1-C.sub.6)-haloalkyl; (C.sub.1-C.sub.12)-alkyl; (C.sub.3-C.sub.8)-cycloalkyl, (C.sub.2-C.sub.12)-alkenyl, (C.sub.5-C.sub.8)-cycloalkenyl, (C.sub.2-C.sub.12)-alkynyl; where the abovementioned alkyl, cycloalkenyl, alkenyl, cycloalkenyl and alkynyl radicals are unsubstituted or each independently substituted by m radicals selected from the group consisting of cyano, nitro, OR.sup.5, S(O).sub.nR.sup.5, SO.sub.2NR.sup.6R.sup.7, C(O)OR.sup.8, CONR.sup.6R.sup.8, COR.sup.6, NR.sup.6R.sup.8, NR.sup.6COR.sup.8, NR.sup.6CONR.sup.8R.sup.8, NR.sup.6CO.sub.2R.sup.8, NR.sup.6SO.sub.2R.sup.8, NR.sup.6SO.sub.2NR.sup.6R.sup.8, C(R.sup.6)═NOR.sup.8; (C.sub.1-C.sub.12)-haloalkyl; S(O).sub.nR.sup.5, cyano, nitro, OR.sup.5, SO.sub.2NR.sup.6R.sup.7, C.sub.02R.sup.8, COR.sup.8, NR.sup.6R.sup.8, NR.sup.6COR.sup.8, NR.sup.6CO.sub.2R.sup.8, NR.sup.6SO.sub.2R.sup.8;  or R.sup.9 and R.sup.10 together with the nitrogen atom to which they are attached form a saturated, partially or fully unsaturated five-, six- or seven-membered ring which is optionally mono- to hexasubstituted by radicals from the group consisting of halogen, (C.sub.1-C.sub.6)-alkyl, halo-(C.sub.1-C.sub.6)-alkyl, OR.sup.5, S(O).sub.nR.sup.5, CO.sub.2R.sup.8, CONR.sup.6R.sup.8, COR.sup.6 and C(R.sup.6)═NOR.sup.8 and which, in addition to this nitrogen atom, contains r carbon atoms, o oxygen atoms, p sulfur atoms and q elements from the group consisting of NR.sup.7, CO and NCOR.sup.7 as ring atoms; R.sup.5 is (C.sub.1-C.sub.6)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.1-C.sub.6)-haloalkyl or aryl; R.sup.6 is hydrogen or R.sup.5; R.sup.7 is hydrogen, (C.sub.1-C.sub.6)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.3-C.sub.4)-alkenyl or (C.sub.3-C.sub.4)-alkynyl; R.sup.8 is hydrogen, (C.sub.1-C.sub.6)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.3-C.sub.4)-alkenyl or (C.sub.3-C.sub.4)-alkynyl; R.sup.2a is selected from the group consisting of hydrogen; methyl; R.sup.2b is hydrogen; R.sup.3 is selected from the group consisting of halogen, cyano, isocyano, NO.sub.2; (C.sub.1-C.sub.6)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.1-C.sub.6)-haloalkyl, (C.sub.1-C.sub.6)-alkylcarbonyl, (C.sub.1-C.sub.6)-haloalkylcarbonyl, (C.sub.1-C.sub.4)-alkyloxycarbonyl; (C.sub.2-C.sub.3)-alkenyl, (C.sub.2-C.sub.3)-haloalkenyl; (C.sub.2-C.sub.3)-alkynyl, (C.sub.2-C.sub.3)-haloalkynyl; (C.sub.1-C.sub.2)-alkyl-S(O).sub.n and (C.sub.1-C.sub.2)-haloalkyl-S(O).sub.n; CHO; NH.sub.2; R.sup.4 is phenyl, where the phenyl radical is unsubstituted or mono- or polysubstituted by a radical selected from the group consisting of halogen, cyano, isocyano, nitro; (C.sub.1-C.sub.6)-alkyl, (C.sub.1-C.sub.6)-haloalkyl, (C.sub.1-C.sub.3)-haloalkoxy; (C.sub.2-C.sub.3)-alkenyl, (C.sub.2-C.sub.3)-haloalkenyl, (C.sub.1-C.sub.6)-alkoxy; (C.sub.2-C.sub.3)-alkynyl, (C.sub.2-C.sub.3)-haloalkynyl, (C.sub.1-C.sub.4)-alkyl-S(O).sub.n; CHO, (C.sub.1-C.sub.4)-alkyloxycarbonyl and NH.sub.2; R.sup.12 is selected from the group consisting of halogen, cyano, isocyano, NO.sub.2; (C.sub.1-C.sub.6)-alkyl, (C.sub.1-C.sub.6)-haloalkyl, (C.sub.1-C.sub.6)-alkylcarbonyl, (C.sub.1-C.sub.6)-haloalkylcarbonyl, (C.sub.1-C.sub.4)-alkyloxycarbonyl, (C.sub.1-C.sub.6)-alkoxy, (C.sub.1-C.sub.3)-haloalkoxy, (C.sub.1-C.sub.4)-alkyl-S(O).sub.n; (C.sub.2-C.sub.3)-alkenyl, (C.sub.2-C.sub.3)-haloalkenyl; (C.sub.2-C.sub.3)-alkynyl, (C.sub.2-C.sub.3)-haloalkynyl; NH.sub.2; and where the indices are as follows: m is 0, 1 or 2; n is 0, 1 or 2; o is 0, 1 or 2; p is 0 or 1; q is 0 or 1; r is 3, 4, 5 or 6; and s is 0, 1, 2, 3, 4 or 5, excluding the following compounds: [(4-chloro-1,5-diphenyl-1H-pyrazol-3-yl)oxy]acetic acid, {[4-chloro-5-(4-methylphenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetic acid, {[4-chloro-5-(3-chlorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetic acid, ethyl [(4-chloro-1,5-diphenyl-1H-pyrazol-3-yl)oxy]acetate, ethyl {[4-chloro-5-(4-methylphenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetate, ethyl {[4-chloro-5-(3-chlorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetate, 2-(4-chloro-1,5-diphenyl-pyrazol-3-yl)oxypropanoic acid, 2-(4-bromo-1,5-diphenylpyrazol-3-yl)oxypropanoic acid.

2. The compound of the formula (I) according to claim 1 and/or an agrochemically acceptable salt thereof, where A is selected from the group consisting of A1-A3, ##STR00030## R.sup.1 is selected from the group consisting of OR.sup.1a and NR.sup.9R.sup.10; where R.sup.1a is selected from the group consisting of hydrogen; methyl, ethyl which is unsubstituted or substituted by one or more substituents selected from the group consisting of halogen, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.1-C.sub.4)-trialkylsilyl, (C.sub.1-C.sub.4)-alkoxy, cyano and nitro; (C.sub.2-C.sub.6)-alkenyl, (C.sub.2-C.sub.6)-haloalkenyl; aryl-(C.sub.1-C.sub.4)-alkyl, where the aryl is unsubstituted or substituted by one or more substituents selected from the group consisting of halogen, (C.sub.1-C.sub.4)-alkyl, (C.sub.1-C.sub.4)-haloalkyl; R.sup.9 is selected from the group consisting of hydrogen, (C.sub.1-C.sub.6)-alkyl; R.sup.10 is selected from the group consisting of hydrogen; (C.sub.3-C.sub.7)-cycloalkyl-(C.sub.1-C.sub.4)-alkyl, aryl-(C.sub.1-C.sub.4)-alkyl, aryl-(C.sub.1-C.sub.4)-alkoxy, where the cycloalkyl and aryl is unsubstituted or substituted by one or more substituents selected from the group consisting of halogen, (C.sub.1-C.sub.4)-alkyl, (C.sub.1-C.sub.4)-haloalkyl; (C.sub.1-C.sub.6)-alkyl, (C.sub.2-C.sub.6)-alkenyl, (C.sub.2-C.sub.6)-alkynyl; (C.sub.3-C.sub.8)-cycloalkyl;  where the abovementioned alkyl, alkenyl, alkynyl and cycloalkenyl radicals are unsubstituted or are each independently substituted by m radicals selected from the group consisting of Cyano, C(O)OR.sup.8; (C.sub.1-C.sub.6)-haloalkyl R.sup.8 is hydrogen, (C.sub.1-C.sub.6)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl; R.sup.2a is selected from the group consisting of hydrogen; methyl; R.sup.2b is hydrogen; R.sup.3 is selected from the group consisting of fluorine, chlorine, bromine, iodine, cyano, isocyano, NO.sub.2; (C.sub.1-C.sub.6)-alkyl, (C.sub.3-C.sub.6)-cycloalkyl, (C.sub.1-C.sub.6)-haloalkyl, (C.sub.1-C.sub.4)-alkyloxycarbonyl; (C.sub.2-C.sub.3)-alkynyl, (C.sub.2-C.sub.3)-haloalkynyl; R.sup.4 is phenyl, where the phenyl radical is unsubstituted or mono- or polysubstituted by a radical selected from the group consisting of fluorine, chlorine, bromine; methyl, ethyl; methoxy, ethoxy; R.sup.12 is selected from the group consisting of halogen, cyano, nitro; (C.sub.1-C.sub.6)-alkyl, (C.sub.1-C.sub.6)-haloalkyl, (C.sub.1-C.sub.3)-haloalkoxy; (C.sub.1-C.sub.6)-alkoxy; and where the indices are as follows: m is 0, 1 or 2; s is 0, 1, 2, 3, excluding the compounds: [(4-chloro-1,5-diphenyl-1H-pyrazol-3-yl)oxy]acetic acid, {[4-chloro-5-(4-methylphenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetic acid, {[4-chloro-5-(3-chlorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetic acid, ethyl [(4-chloro-1,5-diphenyl-1H-pyrazol-3-yl)oxy]acetate, ethyl {[4-chloro-5-(4-methylphenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetate, ethyl {[4-chloro-5-(3-chlorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetate, 2-(4-chloro-1,5-diphenyl-pyrazol-3-yl)oxypropanoic acid, 2-(4-bromo-1,5-diphenylpyrazol-3-yl)oxypropanoic acid.

3. The compound of the formula (I) according to claim 1 and/or an agrochemically acceptable salt thereof, where A is A1; ##STR00031## R.sup.1 is selected from the group consisting of OR.sup.1a and NR.sup.9R.sup.10; where R.sup.1a is selected from the group consisting of hydrogen; methyl, ethyl, trimethylsilylmethyl; 1-propenyl, 2-propenyl; benzyl, 1-phenylethyl, 2-phenylethyl, where the phenyl radical in each of the three groups mentioned is unsubstituted or substituted by halogen; R.sup.9 is hydrogen; R.sup.10 is selected from the group consisting of hydrogen; cyclopropylmethyl; benzyl, 1-phenylethyl, 2-phenylethyl, benzyloxy, where the phenyl radical in each of the four groups mentioned is unsubstituted or substituted by halogen; methyl, ethyl, propyl, 1-methylethyl, butyl, 1-methylpropyl, 2-methylpropyl, 1,1-dimethylethyl, pentyl, 1-methylbutyl, 2-methylbutyl, 3-methylbutyl, 2,2-dimethylpropyl, 1-ethylpropyl, hexyl, where the abovementioned radicals are unsubstituted or are each independently monosubstituted by a C(O)OR.sup.8 radical; cyclopropyl, cyclobutyl, cyclopentyl, where the three radicals mentioned are unsubstituted or are each independently monosubstituted by a C(O)OR.sup.8 radical; 1-propenyl, 2-propenyl, 2-methyl-2-propenyl, prop-2-yn-1-yl, but-2-yn-1-yl; R.sup.8 is hydrogen, methyl, ethyl; R.sup.2a is selected from the group consisting of hydrogen; methyl; R.sup.2b is hydrogen; R.sup.3 is selected from the group consisting of fluorine, chlorine, bromine, iodine, cyano, NO.sub.2; trifluoromethyl; ethynyl; C(O)Omethyl; R.sup.4 is phenyl, where the phenyl radical is unsubstituted or mono- or polysubstituted by a radical selected from the group consisting of fluorine, chlorine, bromine; methyl, ethyl; methoxy, ethoxy; R.sup.12 is selected from the group consisting of fluorine, chlorine, NO.sub.2; trifluoromethyl, methoxy, ethoxy; and where the indices are as follows: s 1, 2, 3, excluding the compounds: [(4-chloro-1,5-diphenyl-1H-pyrazol-3-yl)oxy]acetic acid, {[4-chloro-5-(4-methylphenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetic acid, {[4-chloro-5-(3-chlorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetic acid, ethyl [(4-chloro-1,5-diphenyl-1H-pyrazol-3-yl)oxy]acetate, ethyl {[4-chloro-5-(4-methylphenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetate, ethyl {[4-chloro-5-(3-chlorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetate, 2-(4-chloro-1,5-diphenyl-pyrazol-3-yl)oxypropanoic acid, 2-(4-bromo-1,5-diphenylpyrazol-3-yl)oxypropanoic acid.

4. The compound of formula (I) according claim 1 and/or an agrochemically acceptable salt thereof, where A is A1 ##STR00032## R.sup.1 is selected from the group consisting of OR.sup.1a and NR.sup.9R.sup.10; where R.sup.1a is selected from the group consisting of hydrogen; methyl, ethyl; 2-propenyl; R.sup.9 is hydrogen; R.sup.10 is selected from the group consisting of cyclopentyl monosubstituted by C(O)OR.sup.8; cyclopropylmethyl; CH.sub.2C(O)OR.sup.8, CH.sub.2CH.sub.2C(O)OR.sup.8; 2-propenyl, prop-2-yn-1-yl; R.sup.8 is hydrogen, methyl, ethyl; R.sup.2a is selected from the group consisting of hydrogen; methyl; R.sup.2b is hydrogen; R.sup.3 is selected from the group consisting of chlorine, bromine, iodine, cyano, NO.sub.2; R.sup.4 is phenyl, where the phenyl radical is unsubstituted or mono- or polysubstituted by a radical selected from the group consisting of fluorine, chlorine; R.sup.12 is selected from the group consisting of fluorine, chlorine; and where the indices are as follows: s is 1, 2, excluding the compounds: [(4-chloro-1,5-diphenyl-1H-pyrazol-3-yl)oxy]acetic acid, {[4-chloro-5-(4-methylphenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetic acid, {[4-chloro-5-(3-chlorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetic acid, ethyl [(4-chloro-1,5-diphenyl-1H-pyrazol-3-yl)oxy]acetate, ethyl {[4-chloro-5-(4-methylphenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetate, ethyl {[4-chloro-5-(3-chlorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}acetate, 2-(4-chloro-1,5-diphenyl-pyrazol-3-yl)oxypropanoic acid, 2-(4-bromo-1,5-diphenylpyrazol-3-yl)oxypropanoic acid.

5. A process for preparing one or more compounds of formula (Ia) and/or an agrochemically acceptable salt thereof according to claim 1 comprising reacting one or more compounds of formulae (II) and (III) to give one or more compounds of formula (IV), which are reacted with one or more compounds of formula (V) to give one or more compounds of formula (Ia), ##STR00033## in which R.sup.4, R.sup.2a, R.sup.2b, R.sup.1a, R.sup.3, and A have the definition given above, and X is chlorine, bromine or iodine.

6. A process for preparing one or more compounds of formula (Ib) and/or an agrochemically acceptable salt thereof according to claim 1 comprising reacting one or more compounds of formula (Ia) in which R.sup.4, R.sup.2a, R.sup.2b, R.sup.1a, R.sup.3, and A have the definitions given above further with one or more compounds of formula (VI) to give one or more compounds of formula (Ib). ##STR00034##

7. An agrochemical composition comprising a) at least one compound of formula (I) or an agrochemically acceptable salt thereof as defined in claim 1, and b) one or more auxiliaries and/or additives customary in crop protection.

8. The agrochemical composition comprising a) at least one compound of the formula (I) or an agrochemically acceptable salt thereof as defined in claim 1, b) one or more active agrochemical ingredients other than component a), and optionally c) one or more auxiliaries and/or additives customary in crop protection.

9. A method of controlling unwanted one or more plants or for regulating the growth of one or more plants, comprising applying an effective amount of at least one compound of the formula (I) and/or an agrochemically acceptable salt thereof, as defined in claim 1, to the plants, seed and/or an area in which the plants grow.

10. A product comprising one or more compounds of the formula (I) and/or an agrochemically acceptable salt thereof, as defined in claim 1, wherein said product is an herbicide and/or a plant growth regulator.

11. The product according to claim 10, wherein the compound of formula (I) or an agrochemically acceptable salt thereof is used for controlling harmful one or more plants and/or for regulating growth in one or more plant crops.

12. The product according to claim 11, wherein the crop plants are transgenic or nontransgenic crop plants.

Description

EXAMPLES

[0545] The present invention is illustrated in detail by the examples which follow, but these examples do not restrict the invention in any way.

A. Synthesis Examples

[0546] Methyl (2R)-2-{[4-bromo-1-(2,5-difluorophenyl)-5-(3,4-difluorophenyl)-1H-pyrazol-3-yl]oxy}propanoate (1-182): To a solution of 0.40 g (1.01 mmol) of methyl (2R)-2-{[1-(2,5-difluorophenyl)-5-(3,4-difluorophenyl)-1H-pyrazol-3-yl]oxy}propanoate in 14 ml of DMF was added 0.22 g (1.22 mmol) of N-bromosuccinimide, and the mixture was stirred at 65° C. for one hour. The solvent was removed under reduced pressure, the residue was taken up in water and extracted repeatedly with methylene chloride, the combined organic phases were dried over sodium sulfate, and the solvent was removed under reduced pressure. After purification by column chromatography on silica gel with a heptane/ethyl acetate gradient (start with heptane/ethyl acetate=95:5, to heptane/ethyl acetate=50:50 within 20 min), 0.36 g (71%) of a product with m/z (%)=473 (50) [M.sup.+], 475 (50) [M.sup.+] and a specific angle of rotation of [α]=+20° was obtained. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.57 (d, 3H), 3.69 (s, 3H), 5.15 (q, 1H), 7.18 (m, 1H), 7.36 (m, 2H), 7.50 (m, 3H).

[0547] Synthesis of the Starting Compounds:

[0548] Methyl (2R)-2-{[1-(2,5-difluorophenyl)-5-(3,4-difluorophenyl)-1H-pyrazol-3-yl]oxy}propanoate: To a solution of 0.50 g (1.54 mmol) of 1-(2,5-difluorophenyl)-5-(3,4-difluorophenyl)-1H-pyrazol-3-ol in 31 g of dimethylformamide was added 0.75 g (2.31 mmol) of caesium carbonate, the mixture was stirred at room temperature for 10 minutes, 0.23 g (1.85 mmol) of methyl (2S)-2-chloropropanoate was added, and the mixture was stirred at 80° C. for a further hour. The solvent was removed under reduced pressure, the residue was taken up in water and extracted repeatedly with methylene chloride, the combined organic phases were dried over sodium sulfate, and the solvent was removed under reduced pressure. After purification by column chromatography on silica gel with heptane/ethyl acetate (start with heptane/ethyl acetate=95:5, to heptane/ethyl acetate=50:50 within 12 min), 0.46 g (72%) of a product with m/z=395 [M.sup.+] and a specific angle of rotation of [α]=+40° was obtained. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.63 (d, 3H), 3.78 (s, 3H), 5.18 (q, 1H), 6.03 (s, 1H), 6.91 (m, 1H), 7.08 (m, 4H), 7.16 (m, 1H). [0549] b) 1-(2,5-Difluorophenyl)-5-(3,4-difluorophenyl)-1H-pyrazol-3-ol: To a solution of 4.95 g (9.64 mmol) of N′-(2,5-difluorophenyl)-3-(3,4-difluorophenyl)prop-2-yne hydrazide in 10 ml of DMF was added 0.15 g (0.77 mmol) of copper(I) iodide, and the mixture was stirred at 80° C. for one hour. After purification by column chromatography on silica gel with heptane/ethyl acetate (start with heptane/ethyl acetate=95:5, to heptane/ethyl acetate=20:80 within 15 min), 1.06 g (28%) of a product with m/z=309 [M.sup.+] was obtained. .sup.1H-NMR (400 MHz, d.sub.6-DMSO): δ=6.09 (s, 1H), 7.02 (m, 1H), 7.40 (m, 4H), 7.50 (m, 1H), 10.41 (s, 1H). [0550] c) N′-(2,5-Difluorophenyl)-3-(3,4-difluorophenyl)prop-2-yne hydrazide: To a solution of 2.14 g (11.75 mmol) of 3-(3,4-difluorophenyl)prop-2-ynoic acid in 20 ml of tetrahydrofuran were successively added 1.86 g (12.92 mmol) of (2,5-difluorophenyl)hydrazine and 5.94 g (58.75 mmol) of triethylamine. 11.22 g (17.62 mmol) of propanephosphonic anhydride (T3P, 50% solution in tetrahydrofuran) was added dropwise, and the mixture was stirred at room temperature for one hour. The reaction mixture was poured onto water and extracted repeatedly with methyl acetate, the combined organic phases were dried over magnesium sulfate, the solvent was removed under reduced pressure, and 4.97 g (80%) of an oily product (HPLC/MS purity=80%, m/z=309 [M.sup.+]), which was converted further without purification. [0551] d) 3-(3,4-Difluorophenyl)prop-2-ynoic acid: Under an argon atmosphere, the following were added successively to 5.00 g (20.83 mmol) of 1,2-difluoro-4-iodobenzene in 30 ml of dry tetrahydrofuran: 1.46 g (20.83 mmol) of propiolic acid, 0.29 g (0.42 mmol) of bis(triphenylphosphine)palladium(11) dichloride, 0.16 g (0.83 mmol) of copper(I)iodide and 7.38 g (72.92 mmol) of diisopropylamine. The mixture was stirred at room temperature for 2 hours, the reaction mixture was added to water, 15.00 ml of 2 N hydrochloric acid was added and extraction was effected repeatedly with ethyl acetate. The combined organic phases were dried over sodium sulfate and concentrated under reduced pressure. After purification by column chromatography on silica gel with heptane/ethyl acetate (start with heptane/ethyl acetate=95:5, to heptane/ethyl acetate=40:60 within 15 min), 2.89 g (76%) of a product with m/z=183 [M.sup.+] was obtained. .sup.1H-NMR (400 MHz, d.sub.6-DMSO): δ=7.56 (m, 2H), 7.86 (m, 1H), 13.95 (bs, 1H).

[0552] Methyl (2R)-2-{[4-cyano-1-(2,5-difluorophenyl)-5-(3,4-difluorophenyl)-1H-pyrazol-3-yl]oxy}propanoate (I-185): A mixture consisting of 0.18 g (0.37 mmol) of methyl (2R)-2-{[4-bromo-1-(2,5-difluorophenyl)-5-(3,4-difluorophenyl)-1H-pyrazol-3-yl]oxy}propanoate (I-182), 0.04 g (0.35 mmol) of zinc cyanide and 0.04 g (0.04 mmol) of tetrakis(triphenylphosphine)palladium in 5 ml of dimethylacetamide was heated to 180° C. in a microwave under an argon atmosphere for 40 minutes. The solvent was removed under reduced pressure, the residue was taken up in water/methylene chloride, the aqueous phase was extracted repeatedly with methylene chloride, the combined organic phases were dried over sodium sulfate, and the solvent was removed under reduced pressure. After purification by column chromatography on silica gel with a heptane/ethyl acetate gradient (start with heptane/ethyl acetate=95:5, to heptane/ethyl acetate=60:40 within 15 min), 0.11 g (67%) of a product with m/z=420 [M.sup.+] and a specific angle of rotation of [α]=+170 was obtained. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.68 (d, 3H), 3.78 (s, 3H), 5.18 (q, 1H), 7.12 (m, 6H).

[0553] Methyl 2-{[4-chloro-5-(3,5-difluorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}propanoate (I-165): A reaction mixture consisting of 150.0 mg (0.35 mmol) of methyl 2-[(4-chloro-5-iodo-1-phenyl-1H-pyrazol-3-yl)oxy]propanoate, 83.0 mg (0.53 mmol) of (3,5-difluorophenyl)boronic acid, 12.3 mg (0.02 mmol) of bis(triphenylphosphine)palladium(II) dichloride, 228.4 mg (0.70 mmol) of caesium carbonate (2.5 molar aqueous solution) and 4.4 ml of 1,2-dimethoxyethane was heated to 80° C. for 3 hours. The solvent was removed under reduced pressure, the residue was taken up in water/ethyl acetate, the aqueous phase was extracted repeatedly with ethyl acetate, the combined organic phases were dried over sodium sulfate, and the solvent was removed under reduced pressure. After purification by column chromatography on silica gel with heptane/ethyl acetate, 0.11 g (67%) of a product with m/z (%)=393 (76) [M.sup.+], 395 (24) [M.sup.+] was obtained. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.69 (d, 3H), 3.79 (s, 3H), 5.24 (q, 1H), 6.82 (m, 3H), 7.12 (m, 2H), 7.29 (m, 3H).

[0554] Synthesis of the Starting Compounds: [0555] a) Methyl 2-[(4-chloro-5-iodo-1-phenyl-1H-pyrazol-3-yl)oxy]propanoate: To a solution of 2.80 g (9.47 mmol) of methyl 2-[(5-amino-4-chloro-1-phenyl-1H-pyrazol-3-yl)oxy]propanoate in 56 ml of acetonitrile were successively added 10.14 g (37.87 mmol) of diiodomethane and 2.22 g (18.94 mmol) of isopentyl nitrite, and the mixture was heated to 50° C. for 30 minutes. The solvent was removed under reduced pressure, the residue was taken up in water/ethyl acetate, the aqueous phase was extracted repeatedly with ethyl acetate, the combined organic phases were dried over sodium sulfate, and the solvent was removed under reduced pressure. After purification by column chromatography on silica gel with heptane/ethyl acetate, 2.59 g (64%) of a yellowish solid with m/z (%)=407 (76) [M.sup.+], 409 (24) [M.sup.+] was obtained. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.65 (d, 3H), 3.75 (s, 3H), 5.17 (q, 1H), 7.41 (m, 2H), 7.45 (m, 3H). [0556] b) Methyl 2-[(5-amino-4-chloro-1-phenyl-1H-pyrazol-3-yl)oxy]propanoate: To a solution of 0.80 g (2.76 mmol) of methyl 2-[(5-amino-1-phenyl-1H-pyrazol-3-yl)oxy]propanoate in 5.0 ml of dimethylformamide was added 0.44 g (3.31 mmol) of N-chlorosuccinimide, and the mixture was stirred at room temperature for 30 minutes. The solvent was removed under reduced pressure, the residue was taken up in water/methylene chloride, the aqueous phase was extracted repeatedly with methylene chloride, the combined organic phases were dried over sodium sulfate, and the solvent was removed under reduced pressure. After purification by column chromatography on silica gel with heptane/ethyl acetate, 0.50 g (59%) of a colourless solid with m/z (%)=296 (76) [M.sup.+], 298 (24) [M.sup.+] was obtained. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.64 (d, 3H), 3.76 (s, 3H), 3.91 (bs, 2H), 5.20 (q, 1H), 7.30 (m, 1H), 7.45 (m, 4H). [0557] c) Methyl 2-[(5-amino-1-phenyl-1H-pyrazol-3-yl)oxy]propanoate: To a solution of 0.20 g (1.09 mmol) of 5-amino-1-phenyl-1H-pyrazol-3-ol in 5.0 ml of dimethylformamide was added 0.53 g (1.63 mmol) of caesium carbonate, the mixture was stirred at room temperature for 10 minutes, 0.22 g (1.30 mmol) of methyl 2-bromopropanoate was added, and the mixture was stirred at room temperature for 2 hours. The mixture was filtered, the filtrate was concentrated under reduced pressure, and the residue was stirred with dimethyl ether. This gave 0.19 g (64%) of a crystalline product with m/z=262 [M.sup.+]. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.59 (d, 3H), 3.77 (s, 3H), 3.80 (bs, 2H), 5.16 (q, 1H), 5.20 (s, 1H), 7.26 (m, 1H), 7.45 (m, 2H), 7.49 (m, 2H).

[0558] Methyl {[4-chloro-1-(2-fluorophenyl)-5-(5-fluoro-2-thienyl)-1H-pyrazol-3-yl]oxy}acetate (1-094): To a solution of 85.0 mg (0.24 mmol) of methyl {[1-(2-fluorophenyl)-5-(5-fluoro-2-thienyl)-1H-pyrazol-3-yl]oxy}acetate in 3.2 ml of dimethylformamide was added 42.0 mg (0.32 mmol) of N-chlorosuccinimide in portions, and the mixture was stirred at room temperature for 14 hours. The solvent was removed under reduced pressure, the residue was taken up in water/methylene chloride, the organic phase was washed with saturated aqueous sodium hydrogencarbonate solution and water, the combined aqueous phases were extracted repeatedly with methylene chloride, the combined organic phases were dried over sodium sulfate, and the solvent was removed under reduced pressure. This gave 78 g (67%) of a product with m/z (%)=385 (76) [M.sup.+], 387 (24) [M.sup.+]. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=3.79 (s, 3H), 4.90 (s, 2H), 6.38 (d, 2H), 6.72 (d, 2H), 7.16 (t, 1H), 7.24 (m, 1H), 7.41 (m, 2H).

[0559] Synthesis of the Starting Compounds: [0560] a) Methyl {[1-(2-fluorophenyl)-5-(5-fluoro-2-thienyl)-1H-pyrazol-3-yl]oxy}acetate: Under an argon atmosphere, the following were added successively to a solution of 0.40 g (1.06 mmol) of methyl {[1-(2-fluorophenyl)-5-iodo-1H-pyrazol-3-yl]oxy}acetate in 6.1 ml of dioxane: 37.0 mg (0.05 mmol) of bis(triphenylphosphine)palladium(II) dichloride, 0.24 g (1.06 mmol) of 2-(5-fluoro-2-thienyl)-4,4,5,5-tetramethyl-1,3,2-dioxaborolane, 0.44 g (3.19 mmol) of potassium carbonate, 0.4 ml of water, and the mixture was heated under reflux for 6 hours. The solvent was removed under reduced pressure, the residue was taken up in water/methylene chloride, the aqueous phase was extracted repeatedly with methylene chloride, the combined organic phases were dried over sodium sulfate, and the solvent was removed under reduced pressure. After purification by column chromatography on silica gel with heptane/ethyl acetate, 0.18 g (38%) of a product with m/z (%)=351 [M.sup.+] was obtained. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=3.80 (s, 3H), 4.84 (s, 2H), 6.06 (s, 1H), 6.31 (d, 2H), 6.45 (d, 2H), 7.18 (t, 1H), 7.28 (m, 1H), 7.44 (m, 2H). [0561] b) Methyl {[1-(2-fluorophenyl)-5-iodo-1H-pyrazol-3-yl]oxy}acetate To a solution of 2.69 g (8.85 mmol) of 1-(2-fluorophenyl)-5-iodo-1H-pyrazol-3-ol in 197 ml of acetonitrile was added 3.67 g (26.54 mmol) of potassium carbonate, the mixture was stirred at room temperature for 10 minutes, 1.35 g (8.85 mmol) of methyl bromoacetate was added, and the mixture was stirred under reflux for 8 hours. The mixture was filtered, the filtrate was concentrated under reduced pressure, the residue was taken up in water/methylene chloride, the aqueous phase was extracted repeatedly with methylene chloride, the combined organic phases were dried over sodium sulfate, and the solvent was removed under reduced pressure. After purification by column chromatography on silica gel with heptane/ethyl acetate, 1.81 g (54%) of a product with m/z (%)=377 [M.sup.+] was obtained. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=3.78 (s, 3H), 4.80 (s, 2H), 6.18 (s, 1H), 7.22 (m, 2H), 7.39 (m, 1H), 7.45 (m, 1H). [0562] c) 1-(2-Fluorophenyl)-5-iodo-1H-pyrazol-3-ol: To a solution of 4.70 g (11.24 mmol) of 3-{[tert-butyl(dimethyl)silyl]oxy}-1-(2-fluorophenyl)-5-iodo-1H-pyrazole in 105 ml of tetrahydrofuran was added 3.82 g (14.61 mmol) of tetra-n-butylammonium fluoride, and the mixture was stirred at room temperature for 4 hours. The solvent was removed under reduced pressure, the residue was taken up in water/ethyl acetate, the aqueous phase was extracted repeatedly with ethyl acetate, the combined organic phases were dried over sodium sulfate, and the solvent was removed under reduced pressure. After purification by column chromatography on silica gel with heptane/ethyl acetate, 2.37 g (69%) of a product with m/z (%)=305 [M.sup.+] was obtained. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=6.01 (s, 1H), 7.30 (m, 2H), 7.42 (m, 1H), 7.48 (m, 1H), 10.56 (bs, 1H). [0563] d) 3-{[tert-Butyl(dimethyl)silyl]oxy}-1-(2-fluorophenyl)-5-iodo-1H-pyrazole: Under argon, a solution of 6.00 g (20.52 mmol) of 3-{[tert-butyl(dimethyl)silyl]oxy}-1-(2-fluorophenyl)-1H-pyrazole in 98 ml of tetrahydrofuran was added to a mixture of 1.71 g (26.67 mmol) of n-butyllithium and 2.70 g (26.67 mmol) of diisopropylamine in 98 ml of tetrahydrofuran, and the mixture was stirred at −78° C. for one hour. A solution of 6.77 g (26.67 mmol) of iodine in 98 ml of tetrahydrofuran was added dropwise, and the mixture was stirred at −78° C. for a further hour. The mixture was allowed to warm up to room temperature, water was added, and extraction was effected repeatedly with ethyl acetate. The combined organic phases were dried over sodium sulfate, and the solvent was removed under reduced pressure. After purification by column chromatography on silica gel with heptane/ethyl acetate, 4.72 g (55%) of a product with m/z (%)=419 [M.sup.+] was obtained. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=0.26 (s, 6H), 0.98 (s, 9H), 6.02 (s, 1H), 7.23 (m, 2H), 7.40 (m, 2H). [0564] e) 3-{[tert-Butyl(dimethyl)silyl]oxy}-1-(2-fluorophenyl)-1H-pyrazole: To a solution of 20.00 g (112.26 mmol) of 1-(2-fluorophenyl)-1H-pyrazol-3-ol in 900 ml of dichloromethane were successively added 21.05 g (208.1 mmol) of triethylamine and 15.32 g (101.64 mmol) of tert-butyl(chloro)dimethylsilane, and the mixture was stirred at room temperature for 4 hours. The solvent was removed under reduced pressure, and 29.60 g (quant.) of a product with m/z=293 [M.sup.+] was obtained, which was converted further without purification. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=0.31 (s, 6H), 1.00 (s, 9H), 5.85 (d, 1H), 7.17 (m, 3H), 7.84 (m, 2H).

[0565] Methyl 2-{[4-bromo-5-(4-fluorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}propanoate (I-132): To a solution of 1.10 g (2.91 mmol) of methyl 2-{[5-(4-fluorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}propanoate in 16 ml of DMF was added 0.57 g (3.20 mmol) of N-bromosuccinimide, and the mixture was stirred at 70° C. for three hours. The solvent was removed under reduced pressure, the residue was taken up in water and extracted repeatedly with methylene chloride, the combined organic phases were dried over sodium sulfate, and the solvent was removed under reduced pressure. After purification by column chromatography on silica gel with heptane/ethyl acetate, 1.04 g (81%) of a product with m/z (%)=419 (50) [M.sup.+], 421 (50) [M.sup.+] was obtained. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.69 (d, 3H), 3.79 (s, 3H), 5.26 (q, 1H), 7.07 (m, 4H), 7.22 (m, 5H).

[0566] Synthesis of the starting compounds: The starting compounds were synthesized by the methods described in Example No. I-182.

2-{[4-Bromo-5-(4-fluorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}propanoic acid (I-138)

[0567] A mixture of 1.00 g (2.27 mmol) of methyl 2-{[4-bromo-5-(4-fluorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}propanoate (I-132), 0.73 g (18.25 mmol) of 2N sodium hydroxide solution and 5 ml of tetrahydrofuran was stirred at room temperature for three hours. The solvent was removed under reduced pressure, and the remaining organic phase was adjusted to pH 2 with 2 N HCl. The precipitated solids were dried at 40° C. under reduced pressure, and 0.90 g (93%) of a colourless solid with m/z (%)=405 (50) [M.sup.+], 407 (50) [M.sup.+] was obtained. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.71 (d, 3H), 5.27 (q, 1H), 7.08 (m, 4H), 7.25 (m, 5H).

Methyl N-(2-{[4-bromo-5-(4-fluorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}propanoyl)glycinate (III-056)

[0568] Under argon, the following were added successively to a solution of 0.15 g (0.35 mmol) of 2-{[4-bromo-5-(4-fluorophenyl)-1-phenyl-1H-pyrazol-3-yl]oxy}propanoic acid (I-138) in 4 ml of tetrahydrofuran: 2.13 g (1.68 mmol) of 2-methoxy-2-oxoethanaminium chloride, 1.71 g (1.68 mmol) of propanephosphonic anhydride (T3P, 50% solution in tetrahydrofuran) and 0.34 g (3.36 mmol) of triethylamine, and the mixture was stirred at 50° C. for 6 hours. The solvent was removed under reduced pressure, the residue was taken up in water and extracted repeatedly with methylene chloride, the combined organic phases were dried over sodium sulfate, and the solvent was removed under reduced pressure. After purification by column chromatography on silica gel with heptane/ethyl acetate, 0.14 g (79%) of a colourless oil with m/z (%)=478 (50) [M.sup.+], 476 (50) [M.sup.+] was obtained. .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.71 (d, 3H), 3.77 (s, 3H), 4.12 (m, 2H), 5.35 (q, 1H), 7.08 (m, 2H), 7.15 (m, 3H), 7.26 (m, 5H).

[0569] NMR data of selected examples:

[0570] The .sup.1H NMR data of selected examples of compounds of the general formula (I) are stated in two different ways, namely (a) conventional NMR evaluation and interpretation or (b) in the form of .sup.1H NMR peak lists according to the method described further down.

[0571] a) Conventional NMR Interpretation

[0572] I-094: .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=3.79 (s, 3H), 4.90 (s, 2H), 6.38 (d, 2H), 6.72 (d, 2H), 7.16 (t, 1H), 7.24 (m, 1H), 7.41 (m, 2H).

[0573] I-125: .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.70 (d, 3H), 3.79 (s, 3H), 5.23 (q, 1H), 6.88 (m, 1H), 7.0 (m, 3H), 7.17 (m, 2H), 7.27 (m, 1H), 7.40 (m, 1H).

[0574] I-132: .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.69 (d, 3H), 3.79 (s, 3H), 5.26 (q, 1H), 7.07 (m, 4H), 7.22 (m, 5H).

[0575] I-138: .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.71 (d, 3H), 5.27 (q, 1H), 7.08 (m, 4H), 7.25 (m, 5H).

[0576] I-143: .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.28 (t, 3H), 4.27 (q, 2H), 4.98 (s, 2H), 7.11 (m, 5H), 7.33 (t, 1H), 7.40 (m, 1H).

[0577] I-145: .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.69 (d, 3H), 3.79 (s, 3H), 5.26 (q, 1H), 7.08 (m, 4H), 7.25 (m, 5H).

[0578] I-165: .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.69 (d, 3H), 3.79 (s, 3H), 5.24 (q, 1H), 6.82 (m, 3H), 7.12 (m, 2H), 7.29 (m, 3H).

[0579] I-181: .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=3.81 (s, 3H), 4.91 (s, 2H), 7.00 (m, 3H), 7.13 (m, 3H).

[0580] I-182: .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.57 (d, 3H), 3.69 (s, 3H), 5.15 (q, 1H), 7.18 (m, 1H), 7.36 (m, 2H), 7.50 (m, 3H).

[0581] I-183: .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=3.81 (s, 3H), 4.91 (s, 2H), 7.07 (m, 1H), 7.13 (m, 3H), 7.21 (m, 2H).

[0582] I-184: .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.67 (d, 3H), 3.77 (s, 3H), 5.22 (q, 1H), 6.98 (m, 1H), 7.02 (m, 1H), 7.12 (m, 2H), 7.17 (t, 1H), 7.32 (m, 2H).

[0583] I-185: .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.68 (d, 3H), 3.78 (s, 3H), 5.18 (q, 1H), 7.12 (m, 6H).

[0584] III-056: .sup.1H-NMR (400 MHz, CDCl.sub.3): δ=1.71 (d, 3H), 3.77 (s, 3H), 4.12 (m, 2H), 5.35 (q, 1H), 7.08 (m, 2H), 7.15 (m, 3H), 7.26 (m, 5H).

[0585] b) NMR Peak List Method

[0586] The .sup.1H NMR data of selected examples may also be stated in the form of .sup.1H NMR peak lists. For each signal peak, first the δ value in ppm and then the signal intensity in round brackets are listed. The δ value—signal intensity number pairs for different signal peaks are listed with separation from one another by semicolons.

[0587] The peak list for one example therefore takes the form of:

[0588] δ.sub.1 (intensity.sub.1); δ.sub.2 (intensity.sub.2); . . . α.sub.i (intensity.sub.i); . . . ; δ.sub.n (intensity.sub.n)

[0589] The intensity of sharp signals correlates with the height of the signals in a printed example of an NMR spectrum in cm and shows the true ratios of the signal intensities. In the case of broad signals, several peaks or the middle of the signal and the relative intensity thereof may be shown in comparison to the most intense signal in the spectrum.

[0590] To calibrate the chemical shift of .sup.1H-NMR spectra, we use tetramethylsilane and/or the chemical shift of the solvent, particularly in the case of spectra measured in DMSO. Therefore, the tetramethylsilane peak may but need not occur in NMR peak lists.

[0591] The lists of the .sup.1H NMR peaks are similar to the conventional .sup.1H NMR printouts and thus usually contain all peaks listed in a conventional NMR interpretation.

[0592] In addition, like conventional .sup.1H NMR printouts, they may show solvent signals, signals of stereoisomers of the target compounds which are likewise provided by the invention, and/or peaks of impurities.

[0593] In the reporting of compound signals within the delta range of solvents and/or water, our lists of .sup.1H NMR peaks show the standard solvent peaks, for example peaks of DMSO in DMSO-D.sub.6 and the peak of water, which usually have a high intensity on average.

[0594] The peaks of stereoisomers of the target compounds and/or peaks of impurities usually have a lower intensity on average than the peaks of the target compounds (for example with a purity of >90%).

[0595] Such stereoisomers and/or impurities may be typical of the particular preparation process. Their peaks can thus help in identifying reproduction of our preparation process with reference to “by-product fingerprints”.

[0596] An expert calculating the peaks of the target compounds by known methods (MestreC, ACD simulation, but also with empirically evaluated expected values) can, if required, isolate the peaks of the target compounds, optionally using additional intensity filters. This isolation would be similar to the relevant peak picking in conventional 1H NMR interpretation.

[0597] Further details of .sup.1H NMR peak lists can be found in the Research Disclosure Database Number 564025.

TABLE-US-00004 I-022: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4060 (1.0); 7.4002 (1.6); 7.3929 (0.8); 7.3856 (1.8); 7.3822 (2.4); 7.3778 (1.4); 7.3706 (0.8); 7.3639 (2.0); 7.3608 (0.9); 7.3585 (0.8); 7.3502 (0.9); 7.3458 (3.0); 7.3283 (1.7); 7.3250 (1.2); 7.3188 (0.5); 7.3139 (2.6); 7.3116 (2.2); 7.3100 (2.3); 7.2988 (0.5); 7.2936 (1.4); 7.2889 (1.1); 7.2593 (32.9); 7.2236 (0.7); 7.2063 (0.9); 7.2039 (1.2); 7.0878 (0.7); 7.0850 (0.6); 7.0662 (0.7); 7.0628 (1.2); 7.0602 (0.8); 7.0415 (0.6); 7.0378 (0.6); 4.9164 (9.0); 3.8062 (16.0); 1.5424 (0.8); −0.0002 (12.9) I-054: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3511 (0.6); 7.3467 (0.7); 7.3322 (1.4); 7.3244 (2.8); 7.3202 (2.8); 7.3139 (1.8); 7.3111 (1.5); 7.3064 (2.5); 7.3039 (2.4); 7.2988 (0.8); 7.2970 (1.0); 7.2940 (1.4); 7.2922 (1.0); 7.2845 (1.2); 7.2834 (1.2); 7.2793 (3.1); 7.2745 (2.3); 7.2702 (0.9); 7.2685 (1.0); 7.2637 (1.2); 7.2622 (1.3); 7.2582 (19.1); 7.2546 (1.2); 7.1584 (0.6); 7.1566 (0.6); 7.1550 (0.7); 7.1535 (0.6); 7.1356 (0.9); 7.0253 (0.7); 7.0220 (0.6); 7.0045 (0.6); 7.0006 (1.1); 6.9969 (0.7); 6.9795 (0.6); 6.9762 (0.5); 5.2961 (1.8); 4.9226 (8.9); 3.8029 (16.0); −0.0002 (7.2) I-055: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3769 (0.6); 7.3623 (1.1); 7.3578 (1.4); 7.3433 (1.0); 7.3391 (1.2); 7.3310 (0.7); 7.3229 (0.5); 7.3107 (0.5); 7.2597 (20.0); 7.2089 (0.6); 7.2073 (0.7); 7.2056 (0.7); 7.1896 (0.9); 7.1879 (1.0); 7.1862 (1.0); 7.1487 (0.6); 7.1434 (0.6); 7.1390 (0.6); 7.1300 (0.6); 7.1246 (0.7); 7.1216 (0.7); 7.1172 (1.2); 7.1142 (0.7); 7.1029 (0.6); 7.0976 (1.3); 7.0929 (0.9); 7.0725 (0.7); 7.0558 (0.7); 7.0525 (0.6); 7.0351 (0.6); 7.0311 (1.0); 7.0274 (0.6); 7.0099 (1.0); 7.0064 (1.0); 6.9993 (0.6); 6.9956 (0.7); 5.2980 (4.1); 4.9117 (9.0); 3.8010 (16.0); 2.9549 (0.6); 2.8837 (0.5); 2.8825 (0.5); 1.5420 (2.6); −0.0002 (7.6) I-056: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.2897 (0.6); 7.2878 (0.8); 7.2826 (3.3); 7.2785 (1.1); 7.2770 (1.3); 7.2737 (0.9); 7.2689 (3.9); 7.2680 (4.0); 7.2662 (4.6); 7.2593 (62.1); 7.2518 (2.2); 7.2474 (6.0); 7.2386 (1.2); 7.2345 (2.3); 7.2307 (1.4); 7.2237 (0.6); 7.2174 (1.5); 7.1987 (0.5); 7.1342 (1.6); 7.1324 (2.9); 7.1285 (4.0); 7.1228 (1.0); 7.1156 (1.6); 7.1131 (1.2); 7.1112 (2.8); 7.1080 (2.2); 7.0752 (3.1); 7.0696 (0.9); 7.0609 (0.5); 7.0582 (1.0); 7.0536 (4.5); 7.0483 (0.9); 7.0369 (0.8); 7.0315 (2.4); 4.9188 (13.3); 4.3060 (1.7); 4.2881 (5.4); 4.2703 (5.5); 4.2525 (1.8); 4.2304 (0.5); 1.5403 (16.0); 1.3199 (7.1); 1.3021 (14.6); 1.2925 (0.8); 1.2842 (7.0); 0.0080 (0.6); −0.0002 (22.6); −0.0085 (0.6) I-057: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5182 (1.7); 7.3087 (1.0); 7.3026 (0.8); 7.2985 (1.0); 7.2970 (1.1); 7.2929 (0.8); 7.2882 (1.3); 7.2857 (3.0); 7.2808 (4.1); 7.2771 (2.0); 7.2724 (3.7); 7.2691 (3.1); 7.2660 (4.4); 7.2593 (288.4); 7.2536 (6.4); 7.2500 (4.5); 7.2456 (0.8); 7.2431 (1.4); 7.2370 (1.3); 7.2354 (1.3); 7.2265 (0.6); 7.1557 (0.6); 7.1515 (0.8); 7.1452 (2.8); 7.1410 (3.4); 7.1351 (1.3); 7.1311 (0.7); 7.1287 (1.4); 7.1241 (2.8); 7.1207 (2.3); 7.0826 (3.2); 7.0770 (1.0); 7.0683 (0.6); 7.0657 (1.0); 7.0612 (4.9); 7.0558 (1.0); 7.0443 (0.8); 7.0390 (2.5); 6.9953 (1.7); 4.9952 (16.0); 0.3308 (0.6); 0.2375 (0.6); 0.0079 (3.5); −0.0002 (130.0); −0.0085 (3.9) I-058: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3327 (0.7); 7.3289 (1.8); 7.3248 (1.5); 7.3208 (5.1); 7.3166 (5.2); 7.3101 (3.8); 7.3056 (3.4); 7.3028 (4.2); 7.3006 (3.6); 7.2942 (1.7); 7.2903 (2.2); 7.2868 (2.1); 7.2838 (1.2); 7.2818 (1.3); 7.2796 (1.8); 7.2750 (1.5); 7.2734 (1.4); 7.2683 (5.0); 7.2638 (5.2); 7.2592 (30.7); 7.2518 (1.8); 7.2491 (1.8); 7.2471 (1.7); 7.2435 (2.1); 7.1409 (1.0); 7.1392 (1.1); 7.1375 (1.2); 7.1181 (1.7); 7.1023 (0.7); 7.1006 (0.8); 7.0990 (0.7); 7.0117 (1.2); 7.0084 (1.1); 6.9909 (1.1); 6.9871 (1.8); 6.9834 (1.1); 6.9659 (1.0); 6.9627 (0.9); 4.8954 (16.0); 4.2908 (2.0); 4.2729 (6.3); 4.2551 (6.4); 4.2373 (2.1); 2.1688 (1.5); 1.5705 (3.9); 1.3044 (7.6); 1.2866 (15.5); 1.2687 (7.5); 1.2565 (0.6); −0.0002 (10.8) I-059: .sup.1H-NMR(601.6 MHz, CD3CN): δ = 7.4173 (0.4); 7.4144 (0.6); 7.4090 (0.5); 7.4059 (0.8); 7.4049 (0.8); 7.4007 (1.9); 7.3968 (1.2); 7.3954 (0.9); 7.3935 (1.1); 7.3924 (1.1); 7.3874 (2.5); 7.3847 (1.6); 7.3800 (1.0); 7.3743 (1.3); 7.3717 (0.9); 7.3492 (0.8); 7.3468 (1.1); 7.3407 (2.5); 7.3385 (5.6); 7.3354 (2.9); 7.3292 (1.9); 7.3266 (3.6); 7.3256 (3.4); 7.3213 (0.7); 7.3201 (0.8); 7.3172 (1.1); 7.3143 (0.5); 7.3116 (0.7); 7.2409 (3.8); 7.2398 (4.1); 7.2387 (4.1); 7.2265 (4.1); 7.2142 (0.9); 7.2132 (0.9); 7.1210 (1.0); 7.1194 (1.0); 7.1071 (1.0); 7.1041 (1.4); 7.1019 (1.1); 7.0900 (1.0); 7.0882 (1.0); 4.8184 (16.0); 4.1925 (2.0); 4.1806 (6.0); 4.1688 (6.1); 4.1569 (2.0); 2.0980 (6.3); 1.9225 (0.4); 1.9182 (0.5); 1.9145 (3.5); 1.9104 (6.2); 1.9062 (9.3); 1.9022 (6.5); 1.8981 (3.3); 1.2109 (7.1); 1.1990 (14.5); 1.1872 (7.1) I-060: .sup.1H-NMR(601.6 MHz, CD3CN): δ = 7.4611 (0.5); 7.4582 (0.7); 7.4511 (1.3); 7.4483 (1.9); 7.4467 (1.5); 7.4372 (3.5); 7.4242 (3.7); 7.4191 (1.0); 7.4150 (1.6); 7.4124 (2.9); 7.4096 (2.0); 7.4065 (3.0); 7.4040 (1.8); 7.3968 (1.9); 7.3943 (4.6); 7.3862 (0.8); 7.3833 (1.6); 7.3797 (1.3); 7.3410 (3.9); 7.3388 (4.2); 7.3360 (2.1); 7.3312 (1.2); 7.3278 (3.0); 7.3250 (2.4); 7.2759 (1.2); 7.2635 (1.9); 7.2621 (1.8); 7.2511 (0.8); 7.1598 (1.2); 7.1579 (1.0); 7.1454 (1.2); 7.1428 (1.6); 7.1278 (0.9); 4.8860 (16.0); 4.4421 (0.6); 4.2520 (2.0); 4.2401 (5.9); 4.2283 (5.9); 4.2165 (2.0); 4.1374 (0.4); 4.1257 (0.4); 2.1602 (655.3); 2.1329 (0.4); 2.0871 (0.5); 2.0831 (0.8); 2.0790 (1.2); 2.0749 (0.8); 2.0707 (0.4); 1.9927 (4.6); 1.9846 (10.1); 1.9804 (13.4); 1.9766 (81.7); 1.9725 (144.5); 1.9684 (199.9); 1.9642 (135.7); 1.9601 (71.1); 1.8618 (0.4); 1.8577 (0.8); 1.8536 (1.2); 1.8496 (0.8); 1.8454 (0.4); 1.3017 (1.4); 1.2717 (7.1); 1.2599 (14.8); 1.2481 (7.0); 1.1792 (0.5); 1.1673 (1.0); 1.1555 (0.5); 0.0606 (0.4) I-061: .sup.1H-NMR(300.1 MHz, CDCl3): δ = 7.4164 (0.3); 7.4114 (0.3); 7.4078 (0.5); 7.4023 (0.5); 7.3941 (1.2); 7.3829 (1.1); 7.3748 (1.9); 7.3719 (2.1); 7.3652 (2.3); 7.3613 (2.1); 7.3576 (1.6); 7.3508 (2.0); 7.3467 (2.0); 7.3447 (2.0); 7.3380 (3.2); 7.3351 (2.7); 7.3242 (1.4); 7.3164 (2.0); 7.3078 (3.2); 7.2993 (1.9); 7.2967 (1.4); 7.2883 (0.6); 7.2808 (1.1); 7.2741 (0.8); 7.2602 (3.6); 7.2124 (0.8); 7.2103 (0.8); 7.1861 (1.1); 7.1609 (0.4); 7.1591 (0.4); 7.0860 (0.7); 7.0824 (0.6); 7.0580 (0.7); 7.0534 (1.1); 7.0491 (0.7); 7.0254 (0.6); 7.0219 (0.5); 5.2451 (0.5); 5.2218 (1.6); 5.1986 (1.7); 5.1754 (0.5); 3.7711 (16.0); 2.0412 (0.9); 1.6902 (6.7); 1.6670 (6.6); 1.5789 (1.0); 1.2570 (0.6); −0.0001 (2.8) I-062: .sup.1H-NMR(300.1 MHz, CDCl3): δ = 7.2640 (0.6); 7.2493 (1.7); 7.2200 (4.6); 7.1952 (7.9); 7.1898 (8.1); 7.1777 (7.5); 7.0497 (1.4); 7.0249 (1.9); 6.9986 (0.8); 6.9475 (1.1); 6.9158 (1.6); 6.8870 (0.9); 4.8826 (9.9); 3.7244 (16.0); 3.6578 (15.8); 1.5397 (0.4); 1.1862 (0.6); 0.0002 (5.8); −0.0709 (2.0) I-063: .sup.1H-NMR(300.1 MHz, CDCl3): δ = 7.3913 (0.6); 7.3857 (0.7); 7.3649 (1.5); 7.3594 (1.9); 7.3263 (6.4); 7.3138 (6.3); 7.3073 (3.8); 7.2861 (1.8); 7.2600 (18.4); 7.2391 (0.4); 7.2246 (0.4); 7.1861 (1.0); 7.1607 (1.4); 7.1348 (0.6); 7.0591 (0.8); 7.0265 (1.3); 6.9982 (0.8); 4.9254 (9.2); 3.7975 (16.0); 3.1683 (5.1); 2.0437 (1.0); 1.5555 (6.5); 1.2822 (0.7); 1.2550 (4.4); 1.2349 (0.4); 0.8807 (0.3); 0.0696 (1.2); −0.0001 (14.4); −0.0108 (0.5) I-064: .sup.1H-NMR(300.1 MHz, CDCl3): δ = 7.6138 (0.3); 7.3225 (9.6); 7.2594 (49.0); 7.1697 (3.7); 7.0995 (2.9); 7.0707 (4.5); 7.0482 (1.9); 6.9081 (0.4); 5.2712 (0.7); 5.2470 (2.0); 5.2242 (1.9); 5.2028 (0.7); 3.7824 (16.0); 1.7600 (0.3); 1.6946 (8.0); 1.6712 (7.7); 1.6536 (0.7); 1.5499 (68.6); 1.3134 (0.4); 1.2583 (1.7); 0.8833 (0.3); 0.8586 (0.4); 0.0686 (4.2); −0.0006 (41.4) I-065: .sup.1H-NMR(300.1 MHz, CDCl3): δ = 7.2888 (0.4); 7.2713 (2.4); 7.2591 (19.5); 7.2537 (4.9); 7.2415 (6.3); 7.2347 (5.3); 7.2243 (2.9); 7.1085 (2.7); 7.0987 (1.8); 7.0942 (1.7); 7.0826 (2.0); 7.0758 (1.6); 7.0495 (2.2); 7.0207 (3.7); 6.9915 (1.7); 4.9778 (9.0); 3.8115 (16.0); 3.7362 (16.0); 2.0422 (0.6); 1.5567 (4.7); 1.2580 (0.7); 0.0106 (0.9); −0.0001 (14.4); −0.0110 (0.5) I-066: .sup.1H-NMR(300.1 MHz, CDCl3): δ = 7.3529 (1.6); 7.3352 (2.0); 7.3231 (2.6); 7.3129 (1.4); 7.3054 (2.8); 7.3002 (2.6); 7.2807 (2.6); 7.2740 (5.3); 7.2596 (44.7); 7.2331 (0.8); 7.2189 (0.4); 7.2069 (0.4); 7.1766 (2.5); 7.1697 (2.3); 7.1491 (1.9); 7.1440 (1.6); 7.0685 (0.4); 7.0591 (2.0); 7.0302 (3.4); 7.0009 (1.6); 5.5336 (0.3); 4.9415 (8.8); 3.8057 (16.0); 3.1592 (5.4); 1.5404 (12.3); 1.5124 (2.2); 1.2547 (2.6); 0.0106 (1.8); −0.0001 (35.9); −0.0110 (1.6) I-067: .sup.1H-NMR(300.1 MHz, CDCl3): δ = 7.4439 (0.4); 7.4248 (0.5); 7.4170 (0.8); 7.3992 (0.7); 7.3969 (0.7); 7.3904 (0.7); 7.3714 (0.6); 7.3061 (0.5); 7.2854 (0.6); 7.2785 (1.1); 7.2600 (12.0); 7.2516 (1.0); 7.2310 (0.7); 7.1975 (0.4); 7.1942 (0.6); 7.1890 (0.5); 7.1858 (0.6); 7.1695 (0.8); 7.1664 (1.1); 7.1583 (2.0); 7.1554 (1.4); 7.1532 (1.5); 7.1499 (0.9); 7.1413 (0.5); 7.1380 (0.6); 7.1331 (1.2); 7.1296 (1.4); 7.1279 (1.3); 7.1245 (0.8); 7.0701 (0.5); 7.0670 (0.5); 7.0618 (0.6); 7.0587 (0.6); 7.0425 (0.8); 7.0395 (0.8); 7.0342 (1.0); 7.0311 (1.0); 7.0250 (0.8); 7.0191 (0.9); 7.0158 (1.0); 7.0117 (1.0); 7.0066 (0.6); 7.0034 (0.6); 6.9949 (1.4); 6.9881 (1.8); 6.9809 (1.1); 6.9640 (0.7); 6.9569 (1.0); 6.9494 (0.6); 6.9025 (1.0); 6.8987 (0.8); 6.8779 (0.8); 6.8757 (0.8); 6.8722 (0.8); 5.2616 (0.5); 5.2383 (1.6); 5.2151 (1.6); 5.1918 (0.5); 3.7919 (16.0); 1.7023 (6.5); 1.6790 (6.4); 1.5453 (6.2); 0.0107 (0.4); −0.0001 (9.8); −0.0037 (1.6); −0.0111 (0.3) I-068: .sup.1H-NMR(300.1 MHz, CDCl3): δ = 7.3751 (0.4); 7.3550 (0.6); 7.3481 (0.9); 7.3287 (1.0); 7.3222 (0.8); 7.3024 (0.8); 7.2600 (16.6); 7.2204 (0.4); 7.1935 (1.0); 7.1726 (1.2); 7.1668 (0.8); 7.1439 (1.2); 7.1204 (1.0); 7.1149 (1.0); 7.0921 (0.5); 7.0868 (0.5); 7.0642 (1.5); 7.0354 (1.9); 7.0050 (0.9); 7.0004 (1.0); 6.9734 (0.6); 6.9678 (0.8); 6.9651 (0.7); 6.9399 (2.2); 6.9273 (0.6); 6.9100 (1.4); 6.9020 (1.2); 6.8951 (0.6); 6.8348 (1.2); 6.8313 (1.1); 6.8061 (1.1); 4.9754 (8.1); 3.8212 (16.0); 3.7329 (15.7); 1.5501 (4.4); 1.2572 (0.4); 0.0107 (0.6); −0.0001 (13.9); −0.0112 (0.5) I-069: .sup.1H-NMR(300.1 MHz, CDCl3): δ = 7.3714 (0.3); 7.3491 (0.8); 7.3309 (0.8); 7.3210 (0.8); 7.3088 (0.4); 7.3010 (0.7); 7.2602 (29.7); 7.2400 (1.2); 7.2167 (1.0); 7.2109 (0.8); 7.1892 (0.7); 7.1210 (4.2); 7.0922 (2.7); 7.0652 (0.7); 6.9931 (2.2); 6.9679 (2.1); 6.9634 (2.3); 6.9441 (0.9); 6.9021 (1.5); 6.8773 (1.0); 4.9367 (8.9); 3.8143 (16.0); 3.1835 (5.5); 2.0440 (0.9); 1.5530 (16.2); 1.2826 (0.6); 1.2549 (3.6); 1.2353 (0.3); 0.0700 (0.4); −0.0001 (21.8) I-070: .sup.1H-NMR(400.4 MHz, d.sub.6-DMSO): δ = 7.4457 (6.7); 7.4389 (7.8); 7.4292 (7.0); 7.3610 (1.9); 7.3435 (5.3); 7.3245 (4.8); 7.3061 (5.1); 7.3034 (5.7); 7.3003 (7.0); 7.2914 (5.8); 7.2857 (5.4); 7.2677 (1.1); 7.1494 (4.0); 7.1457 (6.6); 7.1255 (4.8); 4.9533 (14.0); 4.7640 (0.4); 4.2791 (0.4); 4.2199 (2.2); 4.2022 (6.9); 4.1845 (7.0); 4.1667 (2.4); 3.3849 (0.5); 3.3349 (117.7); 2.6779 (1.5); 2.6036 (0.5); 2.5588 (1.5); 2.5135 (168.7); 2.5090 (244.4); 2.5046 (207.4); 2.3361 (1.4); 2.3319 (1.2); 1.9965 (0.9); 1.2472 (0.8); 1.2323 (7.8); 1.2145 (16.0); 1.1968 (7.7); 1.1817 (0.7); 0.9624 (0.4); 0.9459 (0.4); 0.8677 (1.0); 0.8594 (0.7); 0.8502 (0.6); 0.8406 (0.6); 0.8237 (0.3) I-071: .sup.1H-NMR(400.4 MHz, d.sub.6-DMSO): δ = 7.5293 (6.5); 7.5080 (7.8); 7.3894 (2.0); 7.3849 (1.0); 7.3719 (5.6); 7.3526 (4.8); 7.3301 (9.7); 7.3088 (9.1); 7.2899 (0.8); 7.1626 (6.0); 7.1447 (4.9); 4.9501 (14.5); 4.7623 (0.7); 4.2779 (0.8); 4.2132 (2.2); 4.1955 (6.9); 4.1777 (7.0); 4.1601 (2.3); 3.3367 (64.9); 2.6755 (1.3); 2.5106 (154.6); 2.5068 (190.6); 2.5027 (133.8); 2.4574 (0.5); 2.3336 (1.3); 1.2368 (1.2); 1.2261 (7.9); 1.2083 (16.0); 1.1906 (7.6) I-072: .sup.1H-NMR(400.2 MHz, d.sub.6-DMSO): δ = 7.4958 (0.6); 7.4424 (7.8); 7.4346 (9.7); 7.4264 (8.5); 7.3025 (4.8); 7.2961 (5.3); 7.2869 (4.7); 7.2005 (8.0); 7.1929 (8.8); 7.1790 (15.0); 4.9380 (16.0); 4.7548 (0.6); 4.2687 (0.8); 4.2080 (2.6); 4.1906 (7.1); 4.1729 (7.2); 4.1553 (2.5); 3.6598 (0.6); 3.5534 (0.7); 3.5120 (0.8); 3.4784 (0.9); 3.4603 (1.2); 3.4199 (1.4); 3.3880 (2.1); 3.3250 (971.4); 3.3223 (684.4); 3.2696 (1.7); 2.6694 (5.8); 2.6004 (1.0); 2.5710 (1.3); 2.5003 (885.0); 2.4967 (826.3); 2.4405 (3.2); 2.4169 (1.1); 2.3273 (5.9); 1.2313 (1.8); 1.2213 (7.7); 1.2036 (15.4); 1.1858 (7.5) I-073: .sup.1H-NMR(400.3 MHz, d.sub.6-DMSO): δ = 7.4684 (9.8); 7.4613 (9.5); 7.4572 (7.5); 7.4456 (2.8); 7.4417 (3.0); 7.4310 (7.7); 7.4256 (3.0); 7.4190 (3.3); 7.4134 (6.4); 7.4090 (7.4); 7.4011 (1.1); 7.3218 (5.8); 7.3157 (5.4); 7.3106 (5.0); 7.3070 (5.0); 7.3032 (3.5); 7.2982 (2.8); 7.1556 (8.6); 7.1502 (3.0); 7.1383 (5.5); 7.1335 (6.3); 4.9566 (13.8); 4.2163 (2.2); 4.1986 (6.8); 4.1808 (6.8); 4.1631 (2.3); 3.3452 (15.7); 3.3352 (56.3); 2.6800 (1.5); 2.6755 (1.5); 2.5109 (202.9); 2.5066 (202.5); 2.5023 (126.4); 2.3380 (1.5); 2.3337 (1.5); 1.2393 (1.9); 1.2290 (8.0); 1.2218 (3.4); 1.2113 (16.0); 1.2043 (2.2); 1.1936 (7.4) I-074: .sup.1H-NMR(400.2 MHz, d.sub.6-DMSO): δ = 7.5517 (6.3); 7.5307 (7.9); 7.4582 (6.5); 7.4365 (7.6); 7.3490 (7.7); 7.3279 (6.5); 7.1765 (7.6); 7.1548 (6.8); 4.9517 (13.8); 4.7590 (2.1); 4.2731 (2.3); 4.2107 (2.2); 4.1930 (6.6); 4.1752 (6.7); 4.1576 (2.5); 4.1436 (0.9); 4.1259 (0.3); 3.4327 (0.4); 3.3843 (1.9); 3.3348 (292.4); 2.6735 (1.1); 2.5083 (131.3); 2.5046 (165.9); 2.5009 (127.3); 2.3314 (1.1); 1.2641 (0.6); 1.2345 (3.5); 1.2244 (8.6); 1.2066 (16.0); 1.1889 (7.9); 1.1718 (0.9); 0.8531 (0.6); 0.8357 (0.4) I-075: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4024 (0.7); 7.3917 (0.6); 7.3849 (2.0); 7.3778 (0.8); 7.3712 (1.4); 7.3668 (2.3); 7.3626 (1.4); 7.3539 (1.0); 7.3518 (0.9); 7.3495 (1.0); 7.3474 (1.0); 7.3417 (2.7); 7.3375 (2.1); 7.3266 (2.0); 7.3223 (5.4); 7.3092 (1.7); 7.3045 (4.1); 7.3019 (2.5); 7.2905 (5.6); 7.2875 (6.2); 7.2707 (3.7); 7.2662 (2.9); 7.2599 (27.3); 7.1604 (1.2); 7.1415 (1.9); 7.1227 (0.8); 7.0452 (1.2); 7.0421 (1.2); 7.0243 (1.1); 7.0209 (2.1); 7.0176 (1.3); 6.9997 (1.0); 6.9965 (1.1); 5.2970 (9.0); 4.9859 (16.0); 4.2998 (2.1); 4.2820 (6.4); 4.2641 (6.5); 4.2463 (2.1); 1.5482 (4.3); 1.3028 (7.5); 1.2955 (0.8); 1.2849 (15.2); 1.2781 (0.7); 1.2671 (7.3); −0.0002 (10.0) I-076: .sup.1H-NMR(400.3 MHz, d.sub.6-DMSO): δ = 10.8519 (0.6); 7.3806 (2.5); 7.3583 (5.7); 7.3446 (5.6); 7.3195 (5.3); 7.2973 (7.6); 7.2754 (3.7); 7.2469 (1.6); 7.2246 (6.6); 7.2113 (8.0); 7.2041 (10.0); 7.1984 (10.7); 4.9427 (14.5); 4.7619 (0.7); 4.2752 (0.8); 4.2120 (2.4); 4.1945 (7.1); 4.1766 (7.6); 4.1590 (3.7); 4.1083 (1.0); 4.0954 (1.2); 4.0842 (0.7); 3.4315 (0.6); 3.3318 (372.2); 3.2799 (1.5); 3.2247 (0.7); 3.1792 (3.4); 3.1661 (3.1); 3.1088 (0.6); 3.0815 (0.7); 3.0416 (0.8); 3.0255 (1.1); 2.9520 (1.1); 2.8550 (0.6); 2.6761 (6.7); 2.6068 (1.3); 2.5072 (1051.7); 2.3992 (1.1); 2.3746 (0.8); 2.3341 (6.7); 2.2686 (0.6); 2.2217 (0.6); 2.1319 (0.7); 1.5669 (0.7); 1.5031 (0.6); 1.4028 (0.7); 1.2668 (1.3); 1.2262 (7.8); 1.2085 (16.0); 1.1908 (9.0); 1.0907 (1.0); 0.8812 (0.6); 0.8563 (0.7); 0.8490 (0.7); −1.5794 (0.6); −3.1735 (0.6); −3.5033 (0.6); −3.6659 (0.6); −3.8138 (0.6) I-077: .sup.1H-NMR(400.2 MHz, d.sub.6-DMSO): δ = 7.5334 (6.0); 7.5121 (7.9); 7.3342 (7.8); 7.3128 (6.7); 7.2552 (1.3); 7.2493 (0.8); 7.2327 (6.1); 7.2205 (7.0); 7.2125 (8.8); 7.2073 (8.8); 7.1988 (2.0); 7.1849 (0.8); 7.1570 (0.3); 4.9418 (14.4); 4.7596 (0.4); 4.2746 (0.5); 4.2085 (2.2); 4.1908 (6.9); 4.1730 (7.0); 4.1553 (2.3); 3.3294 (39.3); 2.6732 (0.8); 2.5539 (1.4); 2.5088 (86.7); 2.5044 (111.2); 2.5001 (82.8); 2.4537 (0.8); 2.3357 (0.5); 2.3312 (0.6); 1.2690 (0.3); 1.2343 (3.4); 1.2221 (8.0); 1.2044 (16.0); 1.1866 (7.6); 0.8531 (0.6) I-078: .sup.1H-NMR(400.3 MHz, d.sub.6-DMSO): δ = 7.4489 (7.3); 7.4271 (8.8); 7.3949 (2.6); 7.3791 (4.3); 7.3733 (6.1); 7.3596 (5.4); 7.3378 (5.4); 7.3157 (7.5); 7.2940 (2.9); 7.1658 (8.3); 7.1443 (7.6); 4.9529 (16.0); 4.2139 (2.4); 4.1963 (7.2); 4.1785 (7.4); 4.1609 (2.7); 3.3662 (0.4); 3.3316 (94.9); 3.2939 (0.7); 3.1784 (0.9); 3.1658 (0.9); 2.6756 (1.6); 2.5859 (0.3); 2.5069 (264.9); 2.3340 (1.6); 1.2279 (7.7); 1.2101 (15.2); 1.1924 (8.0); 1.1509 (0.4) I-080: .sup.1H-NMR(400.4 MHz, d.sub.6-DMSO): δ = 7.6418 (0.9); 7.6268 (1.1); 7.6198 (1.9); 7.6048 (1.9); 7.5979 (1.2); 7.5828 (1.0); 7.5179 (6.2); 7.5133 (2.8); 7.5014 (2.5); 7.4965 (8.2); 7.4267 (1.0); 7.4200 (1.0); 7.3977 (1.5); 7.3939 (1.4); 7.3780 (1.0); 7.3712 (1.0); 7.3249 (7.7); 7.3203 (3.0); 7.3083 (2.2); 7.3035 (6.5); 7.2411 (0.8); 7.2214 (1.5); 7.1989 (0.8); 4.9214 (13.7); 4.1954 (2.2); 4.1777 (6.9); 4.1599 (7.0); 4.1421 (2.2); 3.3332 (182.0); 2.6809 (0.8); 2.6765 (1.2); 2.6718 (0.9); 2.5565 (0.5); 2.5298 (3.9); 2.5160 (65.0); 2.5118 (140.8); 2.5074 (199.2); 2.5030 (154.0); 2.4987 (77.5); 2.3389 (0.8); 2.3344 (1.2); 2.3300 (1.0); 1.9948 (0.8); 1.4029 (1.9); 1.2669 (0.9); 1.2380 (1.1); 1.2067 (7.8); 1.1979 (0.9); 1.1890 (16.0); 1.1803 (1.1); 1.1712 (7.5); 1.0921 (0.5); 0.9606 (0.8); 0.9440 (0.8); 0.8776 (0.4); 0.8658 (1.0); 0.8573 (0.7); 0.8444 (0.6); 0.8387 (0.9); 0.8212 (0.5) I-081: .sup.1H-NMR(400.2 MHz, d.sub.6-DMSO): δ = 7.6335 (0.9); 7.6185 (1.0); 7.6115 (1.8); 7.5966 (1.8); 7.5895 (1.0); 7.5745 (0.9); 7.4070 (1.0); 7.4000 (1.1); 7.3842 (1.3); 7.3805 (1.4); 7.3775 (1.4); 7.3738 (1.3); 7.3649 (2.4); 7.3587 (1.9); 7.3512 (3.6); 7.3426 (4.1); 7.3348 (1.5); 7.3290 (3.6); 7.3221 (0.4); 7.3001 (0.7); 7.2935 (4.2); 7.2877 (1.1); 7.2764 (1.4); 7.2712 (6.1); 7.2656 (1.1); 7.2544 (0.9); 7.2490 (2.2); 7.2323 (0.6); 7.2289 (0.7); 7.2252 (0.6); 7.2086 (1.2); 7.1897 (0.6); 7.1861 (0.6); 7.1826 (0.5); 4.9151 (12.8); 4.7822 (0.8); 4.7586 (0.3); 4.2701 (0.4); 4.1947 (2.1); 4.1769 (6.8); 4.1591 (6.8); 4.1414 (2.2); 3.4235 (0.6); 3.3745 (0.8); 3.3625 (0.4); 3.3236 (429.6); 3.2988 (0.6); 3.2936 (0.4); 3.2740 (0.8); 2.6787 (0.8); 2.6742 (1.0); 2.6697 (0.7); 2.5277 (3.2); 2.5229 (5.0); 2.5142 (62.8); 2.5097 (132.0); 2.5052 (180.0); 2.5006 (127.3); 2.4962 (58.8); 2.4611 (0.8); 2.3410 (0.4); 2.3367 (0.8); 2.3321 (1.2); 2.3275 (0.8); 1.4017 (0.7); 1.2656 (0.6); 1.2383 (0.7); 1.2325 (0.7); 1.2146 (1.0); 1.2061 (7.7); 1.1968 (0.9); 1.1884 (16.0); 1.1706 (7.6); 1.0910 (0.4) I-082: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): δ = 13.0004 (0.8); 7.5268 (1.1); 7.5227 (1.4); 7.5076 (2.3); 7.5032 (2.8); 7.4881 (1.4); 7.4838 (1.6); 7.4730 (0.7); 7.4686 (0.7); 7.4603 (0.8); 7.4540 (1.3); 7.4488 (1.2); 7.4412 (1.3); 7.4368 (1.2); 7.4337 (1.3); 7.4290 (1.0); 7.4208 (1.0); 7.4164 (0.9); 7.4047 (1.0); 7.3952 (7.5); 7.3881 (7.2); 7.3787 (6.5); 7.3721 (2.0); 7.2953 (1.7); 7.2926 (2.3); 7.2863 (1.0); 7.2798 (4.9); 7.2758 (5.2); 7.2736 (7.4); 7.2681 (3.6); 7.2649 (5.9); 7.2557 (3.9); 7.2452 (1.8); 7.2403 (2.1); 7.2369 (1.6); 7.2192 (1.3); 7.2161 (1.2); 4.8316 (0.9); 4.8209 (16.0); 4.0382 (0.6); 4.0205 (0.6); 3.3141 (10.9); 2.5231 (1.4); 2.5184 (2.0); 2.5097 (20.0); 2.5052 (40.9); 2.5006 (55.8); 2.4961 (38.8); 2.4916 (17.6); 1.9876 (2.5); 1.2360 (0.8); 1.1920 (0.7); 1.1742 (1.4); 1.1564 (0.7); 0.0080 (0.6); −0.0002 (19.0); −0.0085 (0.6) I-083: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.6410 (2.5); 7.6207 (2.9); 7.4145 (2.8); 7.3943 (2.5); 7.2592 (32.4); 7.1139 (1.5); 7.1084 (0.8); 7.1020 (1.8); 7.0967 (1.3); 7.0912 (2.5); 7.0851 (1.0); 7.0793 (2.4); 7.0025 (2.3); 6.9967 (0.8); 6.9908 (0.5); 6.9821 (2.8); 6.9653 (0.7); 6.9596 (1.6); 4.9345 (9.3); 3.8483 (0.6); 3.8148 (16.0); 3.8015 (0.8); 1.5409 (0.7); 1.2546 (0.7); 1.0706 (0.9); −0.0002 (12.2); −0.0084 (0.7) I-084: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4709 (1.1); 7.4545 (1.2); 7.4384 (0.8); 7.3819 (0.8); 7.3639 (1.8); 7.3463 (1.4); 7.2734 (1.9); 7.2595 (17.6); 7.2337 (3.1); 7.2098 (1.4); 5.2978 (0.6); 4.8440 (10.3); 3.7706 (16.0); 2.7713 (0.6); 1.5422 (1.7); 1.2429 (0.5); −0.0002 (6.2) I-085: .sup.1H-NMR(400.3 MHz, d.sub.6-DMSO): δ = 7.5852 (1.9); 7.5689 (2.7); 7.5642 (2.6); 7.5481 (2.7); 7.5264 (1.0); 7.4298 (2.2); 7.4245 (2.2); 7.4054 (3.9); 7.4001 (3.4); 7.3865 (4.8); 7.3815 (4.5); 7.3688 (7.4); 7.3531 (4.1); 7.3492 (4.8); 7.3199 (3.5); 7.3073 (2.6); 7.3022 (3.6); 7.2814 (2.5); 7.2600 (2.9); 7.2373 (1.2); 7.1615 (7.2); 7.1579 (7.4); 7.1438 (4.7); 7.1401 (4.7); 5.0105 (0.9); 4.9852 (4.0); 4.9678 (11.3); 4.2777 (0.4); 4.2562 (0.4); 4.2192 (3.7); 4.2013 (7.9); 4.1836 (7.0); 4.1660 (2.1); 3.4369 (0.6); 3.3826 (10.3); 3.3562 (50.7); 3.3419 (98.1); 3.3364 (183.0); 3.2985 (0.8); 3.0350 (0.4); 2.9853 (0.4); 2.9509 (0.4); 2.9008 (0.3); 2.8834 (0.3); 2.7341 (0.5); 2.7272 (0.5); 2.7144 (0.6); 2.6801 (3.4); 2.6757 (3.4); 2.6055 (1.4); 2.5505 (52.5); 2.5113 (502.8); 2.5067 (493.7); 2.5027 (303.6); 2.4041 (0.6); 2.3779 (0.5); 2.3382 (3.3); 2.3337 (3.3); 1.2275 (10.4); 1.2156 (8.8); 1.2097 (16.0); 1.1980 (4.0); 1.1920 (7.2); 1.1541 (0.7); 0.8615 (0.3) I-086: .sup.1H-NMR(400.2 MHz, d.sub.6-DMSO): δ = 7.5866 (0.9); 7.5702 (1.1); 7.5653 (1.7); 7.5493 (1.7); 7.5443 (1.1); 7.5281 (1.0); 7.4279 (1.0); 7.4217 (1.0); 7.4023 (1.3); 7.3983 (1.4); 7.3793 (0.9); 7.3727 (0.9); 7.2782 (1.0); 7.2736 (0.9); 7.2572 (1.7); 7.2512 (2.5); 7.2439 (0.8); 7.2348 (1.7); 7.2276 (5.5); 7.2222 (1.5); 7.2127 (5.4); 7.2071 (6.4); 7.2033 (2.9); 7.1995 (5.7); 7.1906 (1.2); 7.1836 (0.5); 7.1770 (0.6); 4.9798 (0.3); 4.9573 (10.3); 4.7572 (0.7); 4.2696 (0.9); 4.2138 (2.0); 4.1960 (6.4); 4.1783 (6.4); 4.1606 (2.3); 4.1430 (0.3); 3.3684 (0.6); 3.3623 (0.6); 3.3599 (0.6); 3.3425 (4.7); 3.3360 (1.9); 3.3181 (360.9); 3.3051 (1.6); 3.3038 (1.4); 3.3025 (1.3); 3.3012 (1.3); 3.3000 (1.3); 3.2937 (3.9); 2.6810 (1.0); 2.6765 (2.2); 2.6719 (3.0); 2.6673 (2.2); 2.6628 (1.1); 2.5662 (1.3); 2.5256 (18.4); 2.5209 (19.4); 2.5120 (161.2); 2.5075 (344.7); 2.5029 (469.2); 2.4984 (332.3); 2.4938 (151.3); 2.4799 (10.9); 2.3389 (1.0); 2.3344 (2.1); 2.3298 (2.9); 2.3253 (2.0); 1.2349 (0.7); 1.2227 (7.6); 1.2049 (16.0); 1.1872 (7.3) I-087: .sup.1H-NMR(400.4 MHz, d.sub.6-DMSO): δ = 7.6065 (0.8); 7.5903 (1.0); 7.5852 (1.7); 7.5691 (1.7); 7.5642 (1.1); 7.5480 (0.9); 7.4688 (0.6); 7.4610 (6.4); 7.4556 (2.9); 7.4485 (1.3); 7.4443 (2.4); 7.4389 (7.9); 7.4312 (2.2); 7.4251 (1.5); 7.4060 (1.0); 7.3996 (1.0); 7.3022 (0.8); 7.2970 (0.8); 7.2811 (1.5); 7.2756 (1.4); 7.2597 (0.8); 7.2547 (0.7); 7.1886 (0.8); 7.1810 (7.4); 7.1756 (2.2); 7.1641 (2.0); 7.1588 (6.4); 7.1511 (0.7); 4.9731 (9.8); 4.2754 (0.4); 4.2196 (2.0); 4.2019 (6.4); 4.1841 (6.5); 4.1664 (2.1); 3.3273 (115.4); 2.6809 (0.6); 2.6762 (0.9); 2.6717 (0.6); 2.5298 (2.9); 2.5250 (4.4); 2.5163 (49.8); 2.5119 (106.9); 2.5073 (147.4); 2.5028 (106.8); 2.4983 (50.9); 2.4621 (0.5); 2.4577 (0.5); 2.3433 (0.3); 2.3389 (0.7); 2.3343 (0.9); 2.3297 (0.7); 1.2430 (0.9); 1.2281 (7.7); 1.2104 (16.0); 1.1926 (7.3) I-088: .sup.1H-NMR(400.2 MHz, d.sub.6-DMSO): δ = 7.5608 (0.9); 7.5459 (1.0); 7.5388 (1.7); 7.5239 (1.8); 7.5168 (1.0); 7.5019 (0.9); 7.4849 (0.9); 7.4686 (1.1); 7.4637 (1.7); 7.4476 (1.8); 7.4426 (1.2); 7.4266 (2.3); 7.4224 (1.7); 7.4030 (2.7); 7.4009 (2.7); 7.3966 (2.5); 7.3804 (1.3); 7.3779 (1.4); 7.3734 (1.4); 7.2170 (1.1); 7.2108 (1.6); 7.2033 (1.0); 7.1957 (2.0); 7.1906 (2.8); 7.1745 (1.0); 7.1705 (1.3); 7.1680 (1.3); 4.9293 (12.7); 4.1977 (2.1); 4.1800 (6.7); 4.1622 (6.9); 4.1444 (2.2); 3.3772 (0.7); 3.3629 (0.3); 3.3264 (227.7); 3.2910 (0.4); 3.2883 (0.4); 3.2770 (0.6); 2.6831 (0.5); 2.6788 (0.9); 2.6742 (1.3); 2.6697 (0.9); 2.5606 (0.6); 2.5561 (0.8); 2.5515 (0.8); 2.5464 (0.7); 2.5276 (5.4); 2.5226 (8.4); 2.5142 (76.5); 2.5097 (155.6); 2.5052 (209.3); 2.5007 (149.9); 2.4962 (71.4); 2.4561 (0.7); 2.4514 (0.4); 2.3366 (0.9); 2.3321 (1.3); 2.3275 (0.9); 1.2400 (0.4); 1.2073 (7.7); 1.1896 (16.0); 1.1719 (7.5) I-089: .sup.1H-NMR(400.2 MHz, d.sub.6-DMSO): δ = 7.3952 (1.5); 7.3912 (1.7); 7.3742 (6.8); 7.3591 (4.4); 7.3554 (6.0); 7.3149 (0.3); 7.2859 (2.6); 7.2717 (4.0); 7.2638 (5.4); 7.2550 (3.1); 7.2501 (4.7); 7.2266 (5.2); 7.2045 (7.0); 7.1871 (1.7); 7.1825 (2.4); 7.0328 (2.1); 7.0112 (4.8); 7.0069 (4.2); 6.9917 (2.6); 6.9854 (3.3); 4.8806 (15.7); 4.1879 (2.4); 4.1701 (7.4); 4.1524 (7.4); 4.1347 (2.4); 3.4614 (0.9); 3.4361 (27.6); 3.3768 (0.4); 3.3704 (0.4); 3.3271 (178.3); 2.6775 (0.8); 2.6732 (0.9); 2.5488 (0.6); 2.5085 (135.6); 2.5043 (155.1); 2.5003 (105.1); 2.3352 (0.8); 2.3313 (0.9); 1.2382 (1.0); 1.2062 (8.3); 1.1884 (16.0); 1.1708 (7.7) I-090: .sup.1H-NMR(400.3 MHz, d.sub.6-DMSO): δ = 7.4603 (3.2); 7.4537 (6.8); 7.4487 (2.4); 7.4370 (4.7); 7.4323 (7.5); 7.4261 (0.9); 7.4077 (1.4); 7.4034 (1.7); 7.3910 (4.7); 7.3870 (5.6); 7.3721 (3.9); 7.3679 (4.8); 7.2576 (3.9); 7.2511 (8.1); 7.2460 (2.2); 7.2345 (4.0); 7.2298 (5.8); 7.2231 (0.6); 7.0456 (2.0); 7.0428 (1.8); 7.0266 (4.4); 7.0237 (4.8); 7.0195 (3.7); 7.0110 (1.5); 7.0045 (2.6); 6.9978 (2.7); 4.8881 (13.5); 4.1923 (2.3); 4.1814 (2.9); 4.1744 (6.7); 4.1637 (2.9); 4.1567 (6.8); 4.1390 (2.2); 4.0273 (0.3); 3.6148 (0.6); 3.5402 (0.3); 3.4429 (10.8); 3.4362 (25.5); 3.3948 (0.6); 3.3878 (0.8); 3.3800 (1.0); 3.3729 (1.5); 3.3371 (214.4); 3.3300 (520.8); 3.3160 (3.0); 3.3083 (1.5); 3.3002 (0.7); 3.2962 (1.0); 3.2797 (0.4); 3.2308 (0.4); 3.0561 (0.4); 3.0106 (0.5); 2.9816 (0.6); 2.9511 (0.6); 2.9453 (0.5); 2.6819 (4.5); 2.6778 (4.8); 2.6733 (3.2); 2.6168 (0.5); 2.5857 (0.4); 2.5132 (713.7); 2.5088 (763.9); 2.5044 (482.6); 2.5001 (194.1); 2.4792 (3.2); 2.4634 (1.4); 2.4590 (1.5); 2.4544 (1.4); 2.4192 (1.0); 2.3767 (0.4); 2.3402 (4.4); 2.3358 (4.8); 2.3312 (3.0); 1.9964 (0.8); 1.7669 (0.5); 1.2690 (0.8); 1.2456 (1.7); 1.2172 (2.9); 1.2101 (7.8); 1.1996 (6.1); 1.1924 (16.0); 1.1818 (3.4); 1.1747 (7.2); 0.8686 (0.4); 0.8613 (0.5) I-091: .sup.1H-NMR(400.3 MHz, d.sub.6-DMSO): δ = 7.3739 (7.3); 7.3583 (8.7); 7.3408 (3.4); 7.3314 (2.0); 7.2935 (1.5); 7.2749 (2.5); 7.2569 (2.4); 7.2362 (1.0); 7.1114 (2.2); 7.0910 (3.2); 7.0698 (1.6); 7.0360 (3.1); 7.0173 (4.6); 6.9953 (3.8); 6.9894 (4.7); 6.9680 (3.4); 4.9007 (16.0); 4.1981 (3.9); 4.1805 (8.2); 4.1628 (7.4); 4.1451 (2.4); 3.4607 (25.7); 3.4256 (0.4); 3.3323 (60.6); 3.3017 (0.4); 2.6821 (1.1); 2.5128 (136.3); 2.5089 (136.9); 2.4748 (1.1); 2.4697 (1.0); 2.3359 (1.0); 1.2140 (10.2); 1.1962 (16.0); 1.1785 (7.2) I-092: .sup.1H-NMR(400.2 MHz, d.sub.6-DMSO): δ = 7.3816 (1.2); 7.3774 (1.6); 7.3586 (8.0); 7.3520 (6.0); 7.3433 (8.0); 7.3397 (9.9); 7.3360 (7.4); 7.2377 (0.6); 7.2276 (3.5); 7.2239 (2.3); 7.2201 (3.1); 7.2176 (2.6); 7.2142 (2.4); 7.2108 (2.7); 7.2036 (2.4); 7.0217 (1.5); 7.0189 (1.7); 7.0027 (2.4); 7.0001 (3.1); 6.9953 (2.6); 6.9925 (2.5); 6.9836 (1.3); 6.9808 (1.7); 6.9731 (2.5); 5.7580 (1.8); 4.8805 (13.4); 4.1892 (2.1); 4.1715 (6.6); 4.1537 (6.7); 4.1360 (2.2); 3.4296 (0.4); 3.4030 (25.5); 3.3802 (2.7); 3.3701 (0.7); 3.3545 (1.7); 3.3298 (523.0); 3.2975 (0.7); 3.2934 (0.8); 3.2848 (1.2); 3.2792 (2.6); 3.2723 (0.5); 2.6769 (0.8); 2.6724 (1.1); 2.6679 (0.8); 2.5541 (1.4); 2.5258 (3.8); 2.5209 (5.9); 2.5124 (63.4); 2.5079 (131.9); 2.5034 (179.4); 2.4989 (128.1); 2.4944 (60.1); 2.4536 (1.6); 2.3349 (0.9); 2.3304 (1.2); 2.3258 (0.8); 1.2394 (1.1); 1.2075 (7.6); 1.1898 (16.0); 1.1721 (7.4) I-093: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3830 (0.5); 7.3789 (0.9); 7.3771 (0.9); 7.3712 (5.9); 7.3668 (5.6); 7.3599 (2.3); 7.3577 (2.0); 7.3532 (3.3); 7.3518 (2.8); 7.3448 (0.9); 7.3410 (1.1); 7.2799 (0.9); 7.2710 (3.8); 7.2666 (4.2); 7.2595 (24.7); 7.2554 (3.0); 7.2466 (2.8); 7.2434 (1.2); 7.2387 (1.0); 7.2354 (1.1); 7.2185 (0.7); 6.9026 (0.7); 6.8852 (0.8); 6.8786 (1.3); 6.8612 (1.3); 6.8550 (0.8); 6.8377 (0.7); 5.2973 (3.1); 4.8815 (16.0); 4.8074 (3.9); 4.3030 (2.0); 4.2852 (6.3); 4.2674 (6.5); 4.2498 (2.5); 4.2332 (1.5); 1.5462 (0.9); 1.3149 (7.8); 1.2970 (16.0); 1.2869 (2.1); 1.2792 (7.6); 1.2690 (3.9); 1.2512 (1.9); −0.0002 (10.0) I-094: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4347 (0.5); 7.4326 (0.5); 7.4283 (0.6); 7.4203 (0.5); 7.4136 (1.1); 7.4084 (0.9); 7.3949 (1.3); 7.3899 (1.0); 7.3751 (0.8); 7.3707 (0.7); 7.2598 (43.6); 7.2507 (0.9); 7.2476 (1.0); 7.2459 (1.0); 7.2291 (1.2); 7.2104 (0.7); 7.1648 (0.7); 7.1615 (0.6); 7.1440 (0.7); 7.1404 (1.2); 7.1369 (0.7); 7.1194 (0.6); 7.1162 (0.6); 6.7312 (1.4); 6.7218 (2.0); 6.7117 (1.5); 6.3895 (1.7); 6.3847 (1.7); 6.3791 (1.6); 6.3743 (1.6); 6.1771 (1.0); 4.9050 (0.5); 4.8896 (8.9); 4.8481 (1.2); 4.8039 (1.4); 3.7940 (1.5); 3.7896 (16.0); 3.7810 (2.7); 3.7746 (2.2); 2.9186 (14.2); −0.0002 (17.8); −0.0085 (0.6) I-095: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4131 (0.6); 7.4112 (0.5); 7.4004 (1.0); 7.3962 (0.7); 7.3926 (0.6); 7.3847 (0.6); 7.3804 (1.6); 7.3766 (0.8); 7.3617 (1.0); 7.3575 (0.6); 7.2594 (27.0); 7.2536 (1.1); 7.2386 (0.7); 7.2371 (0.7); 7.2338 (1.0); 7.2185 (0.9); 7.2171 (1.0); 7.2155 (1.0); 7.1518 (0.7); 7.1486 (0.6); 7.1310 (0.6); 7.1275 (1.1); 7.1240 (0.6); 7.1064 (0.6); 7.1033 (0.5); 6.7232 (1.4); 6.7140 (1.8); 6.7131 (1.8); 6.7038 (1.4); 6.3851 (1.7); 6.3803 (1.7); 6.3747 (1.6); 6.3699 (1.6); 5.2978 (0.6); 4.8889 (9.0); 4.8440 (2.8); 3.7872 (16.0); 3.7705 (5.0); −0.0002 (11.8) I-096: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5179 (0.5); 7.3913 (0.6); 7.3860 (1.0); 7.3783 (4.6); 7.3746 (5.1); 7.3684 (2.0); 7.3642 (1.7); 7.3600 (3.2); 7.3584 (2.8); 7.3512 (1.0); 7.3470 (1.1); 7.3368 (0.6); 7.2912 (0.9); 7.2811 (0.6); 7.2739 (4.4); 7.2697 (4.7); 7.2646 (2.8); 7.2590 (92.5); 7.2497 (3.9); 7.2293 (0.9); 6.9950 (0.5); 6.9132 (0.7); 6.8958 (0.8); 6.8893 (1.2); 6.8720 (1.2); 6.8658 (0.8); 6.8484 (0.7); 5.2981 (0.5); 4.9621 (16.0); 4.8889 (2.0); 2.0451 (0.8); 1.3325 (1.8); 1.2842 (3.0); 1.2767 (1.2); 1.2552 (5.7); 1.2409 (0.7); 0.8799 (0.8); 0.0079 (0.9); −0.0002 (40.4); −0.0085 (1.6) I-097: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3575 (0.9); 7.3418 (1.2); 7.3366 (1.9); 7.3225 (2.0); 7.3166 (1.4); 7.3016 (1.9); 7.2814 (1.5); 7.2755 (1.3); 7.2601 (27.9); 7.2592 (28.9); 7.2385 (1.3); 7.1043 (1.0); 7.0861 (1.7); 7.0799 (2.0); 7.0651 (0.9); 7.0589 (1.0); 7.0270 (4.7); 7.0061 (3.2); 6.9985 (2.1); 6.9276 (0.9); 6.9102 (1.0); 6.9041 (1.8); 6.8867 (1.8); 6.8803 (1.2); 6.8629 (0.9); 5.2977 (0.5); 4.8779 (16.0); 4.3029 (2.0); 4.2850 (6.0); 4.2672 (6.2); 4.2494 (2.2); 1.3148 (6.3); 1.2976 (12.6); 1.2969 (12.7); 1.2797 (6.5); 1.2791 (6.5); 0.0007 (10.2); −0.0002 (10.6) I-098: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3715 (1.0); 7.3571 (1.0); 7.3499 (1.6); 7.3354 (1.6); 7.3291 (1.7); 7.3141 (2.0); 7.3087 (1.7); 7.2941 (1.5); 7.2904 (0.8); 7.2881 (0.8); 7.2742 (1.2); 7.2591 (31.0); 7.0780 (0.6); 7.0755 (0.7); 7.0716 (0.8); 7.0692 (0.8); 7.0569 (1.1); 7.0539 (1.2); 7.0481 (1.6); 7.0357 (0.6); 7.0332 (0.7); 7.0297 (1.9); 7.0267 (2.7); 7.0237 (1.6); 7.0142 (1.2); 7.0101 (3.1); 7.0055 (3.0); 6.9901 (1.3); 6.9861 (1.2); 6.9800 (0.8); 6.9372 (0.6); 6.9335 (0.6); 6.9304 (0.7); 6.9267 (0.7); 6.9180 (0.7); 6.9146 (1.1); 6.9112 (1.2); 6.9078 (1.2); 6.9045 (0.7); 6.8958 (0.6); 6.8921 (0.6); 6.8889 (0.6); 6.8852 (0.6); 6.8178 (1.1); 6.8109 (0.9); 6.7967 (1.1); 6.7930 (1.2); 6.7900 (1.1); 6.7862 (1.0); 6.7721 (1.0); 6.7652 (0.9); 4.8831 (16.0); 4.2944 (2.0); 4.2765 (6.3); 4.2587 (6.4); 4.2409 (2.1); 1.3054 (7.5); 1.2876 (15.3); 1.2697 (7.4); −0.0002 (11.4) I-099: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 8.2827 (0.5); 8.2799 (0.5); 8.2771 (0.5); 8.2623 (0.8); 8.2592 (0.8); 8.2565 (0.6); 8.2084 (3.4); 8.2034 (1.0); 8.1912 (1.1); 8.1861 (3.6); 8.1512 (0.8); 8.1466 (1.1); 8.1418 (0.6); 7.6937 (0.6); 7.6742 (0.8); 7.6707 (0.7); 7.6360 (0.6); 7.5872 (1.0); 7.5668 (1.4); 7.5472 (0.7); 7.5188 (0.8); 7.5133 (0.6); 7.5077 (3.0); 7.5031 (1.2); 7.4905 (1.1); 7.4856 (2.7); 7.4176 (0.9); 7.4129 (0.7); 7.4101 (0.8); 7.4078 (0.7); 7.3999 (1.4); 7.3973 (1.3); 7.3846 (1.1); 7.3810 (1.4); 7.3766 (0.9); 7.3690 (0.8); 7.3647 (1.3); 7.3469 (0.8); 7.3423 (0.8); 7.2890 (0.7); 7.2599 (100.1); 7.2425 (0.6); 7.2350 (0.7); 7.2213 (1.0); 7.2150 (1.0); 7.1979 (0.5); 7.0625 (0.7); 7.0594 (0.7); 7.0416 (0.7); 7.0381 (1.2); 7.0346 (0.8); 7.0316 (0.5); 7.0282 (0.8); 7.0169 (0.7); 7.0139 (0.7); 6.9958 (0.6); 5.2986 (12.4); 5.0260 (6.6); 5.0221 (9.1); 5.0070 (0.6); 4.9412 (3.2); 3.8380 (1.2); 3.8347 (0.5); 3.8264 (4.1); 3.8202 (12.1); 3.8183 (16.0); 3.8108 (0.8); 3.7898 (1.2); 3.7746 (5.5); 3.6222 (0.5); 0.0079 (1.1); −0.0002 (36.6); −0.0085 (1.1) I-100: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3504 (1.4); 7.3481 (1.1); 7.3439 (5.5); 7.3392 (5.4); 7.3314 (3.4); 7.3298 (2.8); 7.3279 (3.5); 7.3264 (3.8); 7.3248 (3.2); 7.3226 (1.3); 7.3188 (1.1); 7.3149 (2.5); 7.3071 (1.4); 7.3025 (0.7); 7.2926 (1.1); 7.2728 (0.6); 7.2650 (3.6); 7.2587 (28.7); 7.2522 (2.4); 7.2502 (1.8); 7.2487 (1.8); 7.2475 (1.8); 7.2460 (1.6); 7.2429 (1.5); 7.2404 (2.4); 7.2353 (0.6); 6.9073 (0.6); 6.9035 (0.6); 6.9004 (0.6); 6.8967 (0.7); 6.8880 (0.7); 6.8846 (1.0); 6.8812 (1.2); 6.8778 (1.1); 6.8745 (0.7); 6.8658 (0.6); 6.8620 (0.6); 6.8589 (0.6); 6.8552 (0.6); 6.7965 (0.9); 6.7896 (0.8); 6.7753 (1.0); 6.7718 (1.1); 6.7686 (1.0); 6.7650 (0.9); 6.7507 (0.9); 6.7439 (0.8); 5.2966 (1.3); 4.8878 (14.8); 4.2952 (1.9); 4.2774 (5.9); 4.2595 (6.0); 4.2417 (2.0); 1.3060 (7.7); 1.2882 (16.0); 1.2703 (7.7); −0.0002 (10.6) I-101: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.2865 (0.8); 7.2822 (2.0); 7.2768 (1.0); 7.2693 (4.0); 7.2656 (2.0); 7.2602 (19.7); 7.2547 (1.5); 7.2509 (3.0); 7.2489 (2.4); 7.2470 (2.5); 7.2420 (0.9); 7.2379 (1.7); 7.2341 (1.0); 7.2206 (1.2); 7.1328 (2.0); 7.1288 (2.9); 7.1232 (0.7); 7.1161 (1.0); 7.1115 (2.0); 7.1085 (1.7); 7.0752 (2.1); 7.0697 (0.7); 7.0583 (0.6); 7.0534 (3.3); 7.0485 (0.7); 7.0370 (0.6); 7.0317 (1.7); 4.9414 (9.1); 4.7549 (1.2); 3.8129 (16.0); 3.7951 (1.3); 2.9544 (3.4); 2.8824 (2.9); 2.7669 (2.8); 1.5676 (1.4); −0.0002 (6.1) I-102: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5185 (0.6); 7.3767 (0.7); 7.3624 (0.9); 7.3575 (1.3); 7.3506 (0.5); 7.3436 (0.9); 7.3424 (0.8); 7.3391 (1.1); 7.3379 (1.0); 7.3314 (0.8); 7.3300 (0.5); 7.3232 (0.6); 7.3110 (0.6); 7.2695 (0.5); 7.2687 (0.6); 7.2679 (0.7); 7.2671 (0.7); 7.2663 (0.8); 7.2655 (0.9); 7.2647 (1.1); 7.2638 (1.5); 7.2596 (105.1); 7.2093 (0.8); 7.2075 (0.6); 7.2058 (0.7); 7.2043 (0.6); 7.1899 (1.0); 7.1882 (1.0); 7.1863 (1.0); 7.1853 (0.9); 7.1689 (0.5); 7.1485 (0.6); 7.1431 (0.6); 7.1391 (0.6); 7.1296 (0.6); 7.1243 (0.7); 7.1212 (0.7); 7.1176 (1.0); 7.1141 (0.6); 7.1026 (0.6); 7.0975 (1.2); 7.0928 (0.8); 7.0726 (0.7); 7.0559 (0.6); 7.0529 (0.6); 7.0352 (0.6); 7.0315 (1.0); 7.0279 (0.6); 7.0098 (0.9); 7.0064 (0.9); 7.0008 (0.5); 6.9991 (0.6); 6.9956 (1.1); 6.9938 (0.5); 4.9228 (1.0); 4.9118 (8.1); 3.8066 (2.2); 3.8014 (16.0); 2.9618 (0.8); 2.9561 (2.2); 2.9552 (2.3); 2.8845 (2.0); 2.8830 (2.0); 2.7731 (6.2); 1.5415 (8.4); 0.0079 (1.4); 0.0046 (0.6); 0.0038 (0.7); 0.0021 (1.9); −0.0002 (44.3); −0.0028 (2.2); −0.0043 (1.0); −0.0052 (0.7); −0.0060 (0.6); −0.0085 (1.3) I-104: .sup.1H-NMR(400.6 MHz, CDCl3): δ = 7.4359 (0.5); 7.4215 (0.7); 7.4159 (0.9); 7.4016 (0.9); 7.3956 (0.8); 7.3813 (0.7); 7.2972 (0.7); 7.2819 (1.1); 7.2766 (1.7); 7.2604 (28.3); 7.2410 (1.0); 7.1907 (0.7); 7.1885 (0.7); 7.1844 (0.7); 7.1822 (0.7); 7.1697 (1.1); 7.1675 (1.2); 7.1633 (1.2); 7.1612 (1.2); 7.1551 (1.5); 7.1525 (1.5); 7.1512 (1.6); 7.1488 (1.4); 7.1423 (0.8); 7.1400 (0.8); 7.1359 (1.2); 7.1334 (1.2); 7.1320 (1.2); 7.1297 (0.8); 7.0635 (0.6); 7.0613 (0.6); 7.0572 (0.7); 7.0552 (0.6); 7.0428 (1.0); 7.0407 (1.0); 7.0365 (1.1); 7.0346 (1.0); 7.0197 (1.3); 7.0156 (1.4); 7.0093 (0.8); 6.9967 (1.2); 6.9906 (1.6); 6.9857 (1.6); 6.9793 (0.8); 6.9670 (0.9); 6.9616 (1.2); 6.9559 (0.7); 6.8979 (1.1); 6.8948 (1.0); 6.8790 (1.0); 6.8748 (0.9); 5.3002 (2.3); 5.2511 (0.5); 5.2336 (1.7); 5.2162 (1.7); 5.1988 (0.5); 3.7933 (16.0); 1.7003 (6.8); 1.6829 (6.7); 1.5400 (13.2); 0.0077 (2.4); −0.0002 (30.5); −0.0085 (1.6) I-107: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 8.0573 (0.5); 7.3503 (0.5); 7.3445 (0.8); 7.3300 (0.8); 7.3256 (0.6); 7.3242 (0.6); 7.3102 (0.6); 7.2615 (26.6); 7.1267 (1.6); 7.1210 (0.6); 7.1148 (1.7); 7.1096 (1.4); 7.1037 (2.7); 7.0977 (0.7); 7.0955 (0.5); 7.0918 (2.6); 7.0884 (0.8); 7.0861 (0.6); 7.0822 (1.0); 7.0444 (0.8); 7.0418 (1.0); 7.0406 (1.2); 7.0381 (1.0); 7.0254 (0.9); 7.0230 (2.3); 7.0192 (1.5); 7.0015 (0.8); 6.9975 (0.9); 6.9953 (0.7); 6.9914 (2.6); 6.9855 (0.6); 6.9741 (0.7); 6.9710 (2.4); 6.9685 (1.8); 6.9653 (0.7); 6.9539 (0.5); 6.9482 (1.6); 4.9282 (8.3); 3.8127 (16.0); 2.9762 (4.3); 2.8980 (3.9); 2.7690 (10.4); −0.0002 (9.7) I-108: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3837 (0.5); 7.3774 (0.7); 7.3758 (0.6); 7.3632 (0.8); 7.3583 (0.6); 7.3570 (0.6); 7.3435 (0.6); 7.2628 (28.0); 7.1837 (0.6); 7.1812 (0.5); 7.1747 (0.5); 7.1625 (0.9); 7.1598 (0.8); 7.1563 (0.7); 7.1536 (0.9); 7.1349 (0.6); 7.1266 (1.6); 7.1208 (0.6); 7.1148 (1.7); 7.1093 (1.1); 7.1035 (2.3); 7.0977 (0.8); 7.0954 (0.5); 7.0918 (2.2); 7.0739 (0.9); 7.0713 (1.0); 7.0700 (1.2); 7.0675 (1.0); 7.0517 (2.2); 7.0485 (1.4); 7.0460 (0.8); 7.0305 (0.7); 7.0264 (0.6); 7.0249 (0.7); 7.0202 (0.7); 7.0119 (2.4); 7.0059 (0.7); 6.9945 (0.7); 6.9920 (2.5); 6.9889 (1.7); 6.9861 (0.7); 6.9748 (0.6); 6.9690 (1.5); 5.2991 (1.3); 5.0251 (7.9); 4.9111 (0.8); 3.8219 (16.0); 3.8069 (1.7); 3.0134 (14.3); 2.9409 (8.9); 2.0822 (9.8); −0.0002 (10.3) I-109: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 8.0119 (1.2); 7.3489 (0.6); 7.3344 (0.6); 7.2610 (55.1); 7.1087 (1.4); 7.1055 (0.6); 7.1030 (0.6); 7.0969 (1.4); 7.0932 (0.8); 7.0910 (1.3); 7.0859 (2.2); 7.0798 (0.6); 7.0739 (1.8); 7.0656 (0.5); 7.0380 (0.7); 7.0354 (0.8); 7.0341 (1.0); 7.0316 (0.8); 7.0189 (0.6); 7.0162 (0.7); 7.0150 (1.0); 7.0125 (0.8); 7.0073 (0.6); 7.0018 (0.5); 6.9971 (0.6); 6.9850 (0.7); 6.9801 (0.6); 6.9769 (2.0); 6.9710 (0.6); 6.9597 (0.6); 6.9566 (1.9); 6.9539 (1.5); 6.9507 (0.6); 6.9336 (1.3); 4.9215 (6.5); 3.8097 (12.6); 3.0090 (16.0); 2.9580 (11.9); 2.9573 (12.6); 2.8825 (10.8); 2.8810 (11.0); 2.7716 (5.0); 1.5585 (7.2); 0.0080 (0.7); −0.0002 (22.0); −0.0085 (0.6) I-110: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 8.0184 (0.8); 7.3499 (0.5); 7.3446 (0.8); 7.3301 (0.8); 7.3255 (0.6); 7.3243 (0.6); 7.3104 (0.7); 7.2607 (33.5); 7.1372 (1.6); 7.1314 (0.6); 7.1252 (1.7); 7.1199 (1.0); 7.1143 (2.3); 7.1083 (1.0); 7.1065 (0.9); 7.1024 (2.6); 7.0879 (0.7); 7.0851 (0.8); 7.0814 (0.6); 7.0789 (0.9); 7.0422 (0.9); 7.0395 (1.0); 7.0384 (1.3); 7.0358 (1.0); 7.0224 (1.0); 7.0202 (2.2); 7.0167 (1.4); 7.0148 (0.9); 7.0120 (0.5); 7.0003 (2.4); 6.9944 (1.3); 6.9884 (0.8); 6.9831 (0.8); 6.9800 (2.5); 6.9775 (1.9); 6.9742 (0.7); 6.9629 (0.6); 6.9571 (1.6); 4.9289 (8.6); 4.4776 (1.3); 3.8145 (16.0); 2.9550 (8.4); 2.8839 (7.1); 2.8825 (7.2); 2.7698 (1.2); 2.7048 (3.0); 1.5641 (1.0); −0.0002 (12.6) I-111: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.2776 (3.1); 7.2708 (1.9); 7.2677 (1.6); 7.2643 (3.9); 7.2577 (38.2); 7.2527 (5.0); 7.2487 (3.0); 7.2420 (4.0); 7.2384 (2.8); 7.2343 (5.6); 7.2328 (4.8); 7.2315 (5.0); 7.2271 (2.3); 7.2230 (0.9); 7.2168 (2.5); 7.2143 (1.4); 7.1259 (1.7); 7.1245 (1.8); 7.1222 (1.3); 7.1091 (0.9); 7.1068 (1.3); 7.1054 (1.4); 7.0835 (0.7); 7.0762 (6.4); 7.0710 (4.2); 7.0656 (1.5); 7.0597 (3.1); 7.0549 (9.5); 7.0514 (4.6); 7.0431 (0.5); 7.0381 (1.6); 7.0328 (3.9); 7.0277 (1.0); 7.0126 (0.6); 7.0103 (0.7); 7.0062 (0.5); 6.9910 (1.1); 6.9897 (1.1); 6.9846 (0.9); 6.9833 (0.9); 6.9705 (0.5); 6.9681 (0.5); 5.2962 (9.2); 5.2420 (9.9); 4.9865 (16.0); 1.5364 (4.1); −0.0002 (15.1) I-112: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3629 (1.4); 7.3566 (1.6); 7.3550 (1.0); 7.3478 (2.4); 7.3451 (1.5); 7.3384 (2.7); 7.3346 (0.9); 7.3139 (1.1); 7.3126 (1.0); 7.3095 (1.3); 7.3044 (8.2); 7.3006 (2.8); 7.2981 (5.7); 7.2928 (2.2); 7.2908 (1.7); 7.2896 (2.0); 7.2876 (3.2); 7.2824 (0.7); 7.2785 (0.8); 7.2712 (3.2); 7.2655 (2.4); 7.2567 (35.5); 7.2519 (4.1); 7.2503 (5.0); 7.2489 (5.5); 7.2468 (2.2); 7.2440 (1.1); 7.2417 (2.3); 7.2356 (5.8); 7.2320 (4.9); 7.2306 (5.6); 7.2258 (2.3); 7.2220 (1.0); 7.2159 (1.5); 7.2129 (1.2); 7.0817 (0.6); 7.0746 (4.4); 7.0724 (4.4); 7.0703 (2.2); 7.0686 (2.8); 7.0675 (3.4); 7.0620 (1.4); 7.0604 (1.1); 7.0572 (2.3); 7.0531 (7.1); 7.0521 (6.7); 7.0478 (4.4); 7.0363 (1.0); 7.0309 (2.9); 5.2951 (1.9); 5.2592 (11.4); 4.9721 (16.0); 1.5355 (5.4); −0.0002 (15.1) I-113: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.2884 (0.7); 7.2868 (1.0); 7.2813 (3.8); 7.2773 (1.2); 7.2757 (1.5); 7.2726 (0.9); 7.2675 (4.3); 7.2670 (4.5); 7.2651 (5.0); 7.2612 (3.4); 7.2586 (34.1); 7.2506 (2.7); 7.2465 (6.6); 7.2391 (2.0); 7.2350 (2.8); 7.2311 (1.8); 7.2244 (0.7); 7.2183 (1.5); 7.2174 (1.6); 7.1994 (0.6); 7.1317 (1.6); 7.1298 (3.4); 7.1258 (4.5); 7.1201 (1.1); 7.1132 (1.8); 7.1107 (1.3); 7.1087 (3.4); 7.1054 (2.7); 7.0753 (3.7); 7.0697 (1.1); 7.0610 (0.6); 7.0583 (1.1); 7.0538 (5.2); 7.0484 (1.1); 7.0370 (0.9); 7.0316 (2.9); 5.9782 (0.6); 5.9640 (1.2); 5.9520 (0.7); 5.9499 (0.7); 5.9379 (1.4); 5.9352 (0.8); 5.9237 (0.7); 5.9210 (1.5); 5.9090 (0.8); 5.9069 (0.8); 5.8948 (1.5); 5.8808 (0.8); 5.3723 (0.8); 5.3684 (2.1); 5.3648 (2.2); 5.3609 (0.8); 5.3292 (0.7); 5.3254 (1.9); 5.3217 (1.9); 5.3179 (0.7); 5.2966 (1.2); 5.2497 (0.9); 5.2465 (2.3); 5.2433 (2.2); 5.2401 (0.8); 5.2235 (0.8); 5.2203 (2.2); 5.2171 (2.2); 5.2139 (0.8); 4.9592 (16.0); 4.7282 (2.5); 4.7247 (4.0); 4.7211 (2.6); 4.7141 (2.5); 4.7106 (3.9); 4.7070 (2.4); 1.5465 (1.1); −0.0002 (12.0) I-114: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 8.0183 (0.8); 7.4156 (0.6); 7.4140 (0.7); 7.4076 (4.0); 7.4034 (3.5); 7.3967 (1.5); 7.3941 (1.3); 7.3897 (2.0); 7.3881 (1.8); 7.3811 (0.6); 7.3773 (0.7); 7.3051 (2.3); 7.3007 (2.6); 7.2965 (0.7); 7.2946 (0.8); 7.2933 (0.9); 7.2916 (0.8); 7.2892 (1.0); 7.2869 (1.0); 7.2807 (1.7); 7.2603 (32.2); 7.1938 (0.5); 7.1781 (0.5); 7.1730 (1.1); 7.1574 (1.1); 7.1526 (0.7); 7.1371 (0.6); 6.9576 (0.5); 6.9520 (1.0); 6.9467 (0.7); 6.9327 (0.5); 6.9272 (1.0); 6.9211 (1.0); 6.9186 (0.6); 6.9001 (0.9); 6.8978 (1.0); 6.8937 (0.7); 6.8914 (0.7); 6.8564 (0.8); 6.8541 (0.8); 6.8513 (0.8); 6.8491 (0.7); 6.8361 (0.7); 6.8339 (0.7); 6.8310 (0.7); 6.8288 (0.6); 4.9429 (8.7); 4.7599 (0.7); 3.8242 (16.0); 3.7970 (1.3); 2.9554 (8.2); 2.8841 (7.3); 2.8826 (7.1); 2.7699 (1.3); 1.5731 (1.0); −0.0002 (13.4) I-115: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4102 (1.3); 7.4060 (1.2); 7.3923 (0.7); 7.3908 (0.6); 7.2901 (0.8); 7.2858 (0.9); 7.2658 (0.9); 7.2594 (33.9); 4.9363 (2.9); 3.8218 (5.6); 1.5379 (16.0); 0.0691 (1.0); −0.0002 (14.1) I-116: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5185 (1.2); 7.3437 (0.8); 7.3332 (8.5); 7.3299 (3.4); 7.3279 (4.9); 7.3251 (9.3); 7.3207 (7.1); 7.3167 (9.3); 7.3078 (5.7); 7.3036 (2.8); 7.2983 (5.7); 7.2909 (2.5); 7.2854 (5.5); 7.2781 (1.3); 7.2757 (1.0); 7.2751 (1.0); 7.2742 (0.9); 7.2734 (1.0); 7.2726 (1.0); 7.2718 (1.0); 7.2710 (1.2); 7.2702 (1.3); 7.2694 (1.4); 7.2686 (1.5); 7.2678 (1.7); 7.2670 (2.0); 7.2662 (2.3); 7.2653 (2.8); 7.2637 (4.3); 7.2596 (203.6); 7.2091 (1.0); 7.1916 (0.9); 7.1841 (1.3); 7.1801 (5.1); 7.1770 (2.8); 7.1725 (3.2); 7.1699 (3.0); 7.1658 (3.3); 7.1638 (2.8); 7.1614 (2.1); 7.1589 (2.0); 7.1557 (3.8); 7.1517 (0.7); 7.1040 (0.7); 7.0968 (5.4); 7.0913 (1.6); 7.0830 (0.8); 7.0798 (1.7); 7.0757 (7.5); 7.0704 (1.8); 7.0672 (0.7); 7.0589 (1.5); 7.0534 (4.3); 6.9956 (1.4); 5.9912 (0.5); 5.3318 (1.2); 5.3142 (4.6); 5.2967 (4.6); 5.2791 (1.2); 2.0049 (3.0); 1.7453 (16.0); 1.7277 (15.8); 1.6955 (0.7); 1.6782 (0.7); 0.0080 (3.0); −0.0002 (104.2); −0.0085 (3.0); −0.0506 (0.5) I-117: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): δ = 8.3124 (4.8); 7.5517 (3.9); 7.5369 (4.1); 7.5167 (2.9); 7.4667 (2.2); 7.4465 (5.1); 7.4300 (4.8); 7.4097 (3.9); 7.3783 (3.4); 7.2860 (4.9); 7.2666 (6.2); 7.2277 (4.8); 7.2073 (4.6); 7.1880 (4.0); 7.1688 (2.9); 7.1639 (3.9); 7.0516 (4.4); 7.0348 (3.8); 5.0096 (2.9); 4.9925 (3.1); 3.3146 (10.8); 2.6694 (2.9); 2.5094 (189.0); 2.5049 (389.4); 2.5003 (530.0); 2.4957 (370.7); 2.4912 (170.7); 2.3273 (3.4); 1.9874 (2.3); 1.5249 (16.0); 1.5076 (16.0); −0.0002 (28.3) I-118: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5182 (1.0); 7.3750 (0.7); 7.3612 (0.8); 7.3553 (1.2); 7.3407 (1.3); 7.3358 (1.0); 7.3211 (1.0); 7.2763 (0.6); 7.2755 (0.6); 7.2747 (0.6); 7.2739 (0.6); 7.2731 (0.7); 7.2723 (0.7); 7.2715 (0.8); 7.2707 (0.8); 7.2699 (0.9); 7.2691 (1.0); 7.2683 (1.2); 7.2675 (1.3); 7.2667 (1.5); 7.2659 (1.7); 7.2651 (2.0); 7.2643 (2.4); 7.2635 (3.1); 7.2593 (181.8); 7.1213 (2.7); 7.1159 (1.5); 7.1095 (2.6); 7.1040 (1.7); 7.1016 (1.6); 7.0986 (4.2); 7.0952 (1.6); 7.0926 (2.2); 7.0865 (3.3); 7.0805 (0.7); 7.0781 (1.0); 7.0740 (0.7); 7.0715 (0.6); 7.0396 (1.3); 7.0370 (1.6); 7.0358 (1.8); 7.0332 (1.6); 7.0205 (1.1); 7.0167 (1.8); 7.0141 (1.6); 7.0089 (1.2); 7.0026 (1.1); 6.9993 (0.8); 6.9953 (1.2); 6.9927 (0.6); 6.9844 (3.7); 6.9789 (1.6); 6.9762 (1.0); 6.9725 (0.6); 6.9672 (1.0); 6.9641 (3.6); 6.9616 (2.8); 6.9584 (1.1); 6.9470 (0.8); 6.9413 (2.4); 4.9737 (16.0); 2.9626 (1.2); 2.8902 (1.1); 1.8551 (0.6); 0.0079 (2.3); 0.0064 (0.6); 0.0055 (0.7); 0.0047 (0.8); −0.0002 (76.6); −0.0059 (1.2); −0.0067 (1.0); −0.0085 (2.4) I-119: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5182 (0.9); 7.3707 (0.7); 7.3558 (1.1); 7.3498 (1.7); 7.3354 (1.7); 7.3296 (1.3); 7.3154 (1.4); 7.2659 (1.8); 7.2592 (171.5); 7.1462 (0.7); 7.1374 (2.9); 7.1319 (1.1); 7.1256 (3.4); 7.1199 (2.7); 7.1145 (4.8); 7.1108 (1.8); 7.1028 (4.3); 7.0986 (1.8); 7.0957 (1.8); 7.0897 (2.0); 7.0775 (0.8); 7.0751 (0.8); 7.0710 (0.8); 7.0685 (0.9); 7.0460 (1.7); 7.0422 (2.6); 7.0397 (2.2); 7.0244 (4.7); 7.0207 (3.3); 7.0029 (1.8); 6.9971 (5.6); 6.9918 (1.9); 6.9854 (0.8); 6.9769 (4.8); 6.9711 (1.5); 6.9599 (1.0); 6.9541 (3.0); 4.9821 (16.0); 4.9283 (1.0); 3.8129 (1.9); 2.0446 (0.8); 1.2585 (0.6); 0.0079 (1.9); −0.0002 (69.8); −0.0085 (2.2) I-120: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5184 (0.5); 7.3704 (0.6); 7.3555 (0.8); 7.3524 (0.6); 7.3496 (1.2); 7.3351 (1.3); 7.3305 (0.9); 7.3154 (1.0); 7.2709 (0.5); 7.2693 (0.6); 7.2685 (0.7); 7.2677 (0.8); 7.2669 (0.8); 7.2661 (1.0); 7.2652 (1.2); 7.2644 (1.4); 7.2636 (1.8); 7.2595 (92.6); 7.2530 (0.6); 7.1479 (2.5); 7.1421 (1.0); 7.1360 (2.8); 7.1306 (1.6); 7.1250 (3.6); 7.1190 (1.2); 7.1132 (4.1); 7.1095 (0.9); 7.1070 (0.9); 7.1048 (0.5); 7.0948 (1.2); 7.0920 (1.2); 7.0882 (0.9); 7.0858 (1.4); 7.0737 (0.6); 7.0712 (0.6); 7.0671 (0.6); 7.0647 (0.7); 7.0440 (1.4); 7.0414 (1.6); 7.0401 (2.0); 7.0376 (1.7); 7.0219 (3.5); 7.0185 (2.2); 7.0135 (1.1); 7.0050 (3.6); 6.9995 (2.0); 6.9956 (1.6); 6.9933 (1.5); 6.9880 (1.3); 6.9848 (3.9); 6.9822 (2.9); 6.9790 (1.2); 6.9677 (0.9); 6.9619 (2.5); 4.9819 (16.0); 3.7571 (0.5); 2.9661 (1.9); 2.8941 (1.7); 2.8926 (1.8); 1.8576 (0.6); 1.4319 (0.8); 0.0080 (1.2); 0.0048 (0.5); 0.0040 (0.6); −0.0002 (39.1); −0.0084 (1.1) I-121: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5185 (1.1); 7.4037 (0.6); 7.3890 (1.0); 7.3857 (0.7); 7.3829 (1.3); 7.3690 (1.4); 7.3639 (1.0); 7.3492 (1.2); 7.2597 (198.1); 7.1909 (0.8); 7.1884 (0.8); 7.1842 (0.8); 7.1819 (0.9); 7.1697 (1.4); 7.1670 (1.3); 7.1634 (1.2); 7.1608 (1.5); 7.1485 (0.9); 7.1393 (3.3); 7.1335 (1.1); 7.1275 (3.0); 7.1218 (2.0); 7.1162 (4.0); 7.1104 (1.2); 7.1045 (3.9); 7.0962 (0.6); 7.0783 (1.5); 7.0744 (2.2); 7.0719 (2.0); 7.0561 (3.7); 7.0529 (2.4); 7.0350 (1.3); 7.0292 (1.2); 7.0253 (1.3); 7.0171 (3.9); 7.0112 (1.2); 7.0055 (0.6); 6.9972 (4.2); 6.9942 (3.3); 6.9914 (1.4); 6.9800 (1.0); 6.9743 (2.7); 5.0798 (16.0); 4.9644 (1.4); 3.8227 (0.7); 3.0213 (0.8); 2.9521 (0.7); 2.1027 (3.4); 2.0449 (1.1); 1.2587 (0.8); 0.0080 (2.4); −0.0002 (84.0); −0.0085 (2.3) I-122: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4991 (0.7); 7.4812 (0.6); 7.4744 (1.4); 7.4595 (0.8); 7.4560 (1.4); 7.4524 (0.7); 7.4304 (1.6); 7.4269 (0.8); 7.4154 (1.4); 7.4115 (2.9); 7.3980 (0.6); 7.3936 (1.4); 7.3903 (0.9); 7.3661 (0.6); 7.3634 (0.6); 7.3458 (0.6); 7.3229 (2.4); 7.3199 (2.8); 7.3161 (1.4); 7.3076 (0.7); 7.3025 (2.3); 7.2987 (1.6); 7.2602 (14.6); 7.2272 (0.6); 7.2119 (0.6); 7.2066 (1.3); 7.1913 (1.2); 7.1860 (0.8); 7.1708 (0.7); 7.0015 (0.5); 6.9993 (0.5); 6.9870 (0.8); 6.9850 (0.8); 6.9807 (0.9); 6.9787 (0.8); 6.9580 (0.6); 6.9356 (0.9); 6.9301 (1.3); 6.9246 (0.7); 6.9120 (0.7); 6.9066 (1.1); 6.9008 (0.6); 6.8438 (0.9); 6.8401 (0.8); 6.8235 (0.8); 6.8198 (0.7); 5.2972 (0.8); 5.0502 (2.0); 5.0368 (8.8); 3.8448 (3.7); 3.8317 (16.0); 3.8173 (0.8); −0.0002 (6.2) I-123: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3660 (0.7); 7.3638 (0.5); 7.3507 (1.0); 7.3480 (0.8); 7.3451 (1.4); 7.3307 (1.6); 7.3259 (1.1); 7.3108 (1.2); 7.2917 (0.8); 7.2771 (0.9); 7.2719 (1.7); 7.2586 (40.0); 7.2524 (1.8); 7.2375 (1.2); 7.1246 (1.9); 7.1234 (1.9); 7.1137 (0.9); 7.1112 (1.0); 7.1047 (2.3); 7.0926 (1.3); 7.0898 (1.4); 7.0862 (1.2); 7.0837 (1.6); 7.0714 (0.7); 7.0690 (0.8); 7.0650 (0.9); 7.0625 (1.0); 7.0585 (3.1); 7.0528 (2.2); 7.0467 (3.3); 7.0412 (2.1); 7.0356 (6.7); 7.0322 (3.1); 7.0297 (2.8); 7.0238 (5.7); 7.0166 (4.8); 7.0131 (3.0); 7.0020 (1.5); 6.9950 (2.4); 6.9910 (1.6); 6.9846 (1.2); 6.9774 (1.4); 6.9694 (4.3); 6.9635 (1.2); 6.9574 (0.7); 6.9491 (4.5); 6.9434 (1.3); 6.9321 (0.9); 6.9264 (2.4); 5.2973 (1.9); 5.2422 (11.0); 4.9719 (16.0); 4.9277 (0.5); 3.8122 (0.9); 2.2706 (0.9); 1.5396 (2.0); 1.4318 (8.6); −0.0002 (16.0); −0.0085 (0.5) I-124: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3669 (2.2); 7.3602 (2.0); 7.3517 (3.5); 7.3486 (3.3); 7.3419 (4.1); 7.3327 (2.3); 7.3272 (2.8); 7.3232 (2.0); 7.3178 (9.4); 7.3115 (7.0); 7.3060 (2.6); 7.3009 (3.1); 7.2960 (0.7); 7.2924 (0.7); 7.2576 (39.0); 7.1135 (0.8); 7.1111 (0.9); 7.1070 (0.9); 7.1047 (0.9); 7.0923 (1.3); 7.0899 (1.5); 7.0858 (1.4); 7.0835 (1.5); 7.0712 (0.6); 7.0688 (0.7); 7.0646 (0.7); 7.0624 (0.7); 7.0250 (3.1); 7.0206 (3.1); 7.0183 (2.2); 7.0138 (2.8); 7.0085 (2.0); 7.0029 (6.1); 6.9991 (2.4); 6.9971 (1.8); 6.9909 (5.5); 6.9840 (1.7); 6.9805 (1.2); 6.9673 (1.4); 6.9634 (1.4); 6.9612 (1.4); 6.9568 (1.4); 6.9484 (4.4); 6.9424 (1.2); 6.9362 (0.7); 6.9281 (4.7); 6.9224 (1.4); 6.9111 (0.9); 6.9053 (2.4); 5.2962 (1.1); 5.2548 (13.0); 4.9502 (16.0); 4.5006 (0.5); 1.5392 (2.0); 1.4317 (3.7); 0.0701 (2.0); −0.0002 (14.8) I-127: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5184 (2.0); 7.4222 (1.1); 7.4142 (5.0); 7.4107 (5.3); 7.4046 (2.1); 7.4004 (2.2); 7.3962 (3.4); 7.3873 (1.0); 7.3831 (1.2); 7.3774 (0.6); 7.3724 (0.6); 7.3072 (3.7); 7.3029 (4.1); 7.2960 (1.6); 7.2932 (1.8); 7.2906 (2.2); 7.2884 (2.3); 7.2829 (3.2); 7.2595 (362.7); 7.2239 (1.3); 7.2102 (0.6); 7.1940 (0.8); 7.1888 (1.6); 7.1734 (1.4); 7.1681 (1.0); 7.1531 (0.9); 6.9956 (2.1); 6.9611 (0.8); 6.9554 (1.4); 6.9497 (1.1); 6.9364 (1.5); 6.9305 (1.8); 6.9257 (1.2); 6.9157 (1.5); 6.9134 (1.6); 6.9094 (1.0); 6.8927 (0.9); 6.8886 (0.7); 6.8783 (1.3); 6.8582 (1.1); 6.8553 (1.0); 5.0006 (16.0); 2.0444 (0.5); 1.5663 (1.1); 1.2587 (0.7); 0.1579 (0.5); 0.0080 (4.5); −0.0002 (152.0); −0.0085 (5.7); −0.1495 (0.5) I-128: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5183 (0.7); 7.4275 (1.1); 7.4224 (1.7); 7.4145 (6.5); 7.4109 (7.2); 7.4048 (3.1); 7.4006 (2.8); 7.3964 (4.5); 7.3948 (4.0); 7.3876 (1.5); 7.3834 (1.7); 7.3775 (0.8); 7.3731 (1.0); 7.3094 (0.8); 7.2911 (5.0); 7.2869 (5.6); 7.2818 (2.8); 7.2798 (2.8); 7.2773 (2.7); 7.2744 (3.5); 7.2724 (3.8); 7.2669 (5.6); 7.2594 (119.9); 7.1937 (1.2); 7.1782 (1.3); 7.1733 (2.3); 7.1579 (2.1); 7.1532 (1.4); 7.1378 (1.2); 6.9954 (0.7); 6.9352 (1.0); 6.9299 (2.1); 6.9248 (1.7); 6.9163 (1.4); 6.9140 (1.6); 6.9104 (1.6); 6.9053 (2.2); 6.9002 (1.9); 6.8957 (2.3); 6.8933 (2.5); 6.8894 (1.5); 6.8870 (1.4); 6.8750 (1.1); 6.8728 (1.2); 6.8687 (1.0); 6.8641 (2.1); 6.8617 (2.1); 6.8594 (1.9); 6.8569 (1.6); 6.8436 (1.7); 6.8416 (1.7); 6.8389 (1.6); 4.9914 (16.0); 2.0450 (0.8); 1.2586 (0.6); 0.0080 (1.6); −0.0002 (49.6); −0.0085 (2.2) I-129: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 10.5842 (0.5); 7.9716 (0.6); 7.9485 (0.7); 7.5190 (1.1); 7.5010 (1.3); 7.4975 (0.7); 7.4890 (0.7); 7.4822 (3.1); 7.4764 (0.9); 7.4675 (1.3); 7.4640 (2.5); 7.4605 (1.4); 7.4365 (2.6); 7.4332 (1.4); 7.4215 (2.3); 7.4177 (4.7); 7.4042 (0.8); 7.3998 (2.4); 7.3965 (1.5); 7.3672 (1.1); 7.3496 (1.2); 7.3325 (0.9); 7.3274 (3.8); 7.3245 (4.7); 7.3122 (1.1); 7.3070 (3.7); 7.3032 (2.6); 7.2600 (160.0); 7.2385 (0.9); 7.2235 (1.2); 7.2180 (1.9); 7.2103 (1.0); 7.2029 (1.9); 7.1974 (1.2); 7.1821 (1.2); 7.0335 (0.6); 7.0275 (0.7); 7.0177 (0.8); 7.0155 (0.8); 7.0092 (0.8); 6.9960 (2.0); 6.9906 (1.4); 6.9886 (1.4); 6.9761 (0.7); 6.9741 (0.7); 6.9701 (0.8); 6.9419 (1.2); 6.9366 (1.9); 6.9309 (1.1); 6.9184 (1.2); 6.9131 (1.8); 6.9073 (1.0); 6.8647 (1.5); 6.8612 (1.4); 6.8445 (1.2); 6.8410 (1.2); 6.0463 (0.5); 5.1063 (4.1); 5.0941 (16.0); 5.0017 (0.7); 4.9442 (1.0); 4.8496 (0.5); 3.7744 (0.7); 3.7639 (0.7); 3.7577 (1.8); 3.7411 (0.7); 3.6087 (0.6); 1.8751 (0.9); 1.8673 (0.8); 1.8586 (2.3); 1.8499 (0.8); 1.8420 (0.8); 0.0080 (2.2); −0.0002 (66.7); −0.0085 (2.1) I-130: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3316 (3.7); 7.3226 (5.0); 7.3158 (6.2); 7.3046 (2.9); 7.2955 (2.6); 7.2876 (1.4); 7.2825 (2.3); 7.2606 (8.2); 7.1666 (2.4); 7.1578 (2.5); 7.1536 (2.0); 7.1488 (2.0); 7.1426 (1.9); 7.0919 (2.2); 7.0705 (3.8); 7.0489 (1.8); 5.2969 (2.6); 5.2622 (0.6); 5.2448 (1.8); 5.2273 (1.8); 5.2099 (0.6); 3.7819 (16.0); 1.6914 (7.4); 1.6739 (7.3); 1.5622 (0.5); −0.0002 (3.0) I-131: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5184 (1.1); 7.3920 (0.9); 7.3878 (1.1); 7.3730 (1.7); 7.3684 (2.4); 7.3550 (1.4); 7.3494 (2.1); 7.3440 (1.1); 7.3363 (1.2); 7.3283 (1.0); 7.3234 (0.8); 7.3159 (0.9); 7.3091 (1.0); 7.2595 (207.3); 7.2122 (1.6); 7.1945 (2.0); 7.1731 (0.9); 7.1416 (1.9); 7.1369 (1.2); 7.1202 (2.2); 7.1095 (1.3); 7.0999 (1.6); 7.0957 (2.6); 7.0908 (1.3); 7.0750 (1.2); 7.0605 (1.3); 7.0571 (1.1); 7.0357 (2.0); 7.0145 (1.2); 7.0062 (1.0); 7.0023 (1.1); 6.9956 (2.3); 6.9916 (1.2); 6.9796 (0.8); 6.9708 (0.8); 4.8919 (16.0); 4.2949 (2.0); 4.2771 (6.3); 4.2592 (6.5); 4.2414 (2.3); 4.2306 (0.9); 4.0988 (0.5); 1.5367 (14.5); 1.3058 (7.5); 1.2879 (14.9); 1.2701 (7.8); 1.2543 (1.8); 0.0080 (2.5); −0.0002 (74.4); −0.0083 (3.0) I-132: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.2775 (1.0); 7.2722 (0.9); 7.2593 (47.0); 7.2421 (1.1); 7.2364 (1.2); 7.2223 (0.7); 7.1101 (0.9); 7.1062 (1.3); 7.0888 (0.9); 7.0858 (0.7); 7.0730 (0.9); 7.0513 (1.4); 7.0294 (0.7); 5.2640 (0.8); 5.2466 (0.8); 3.7878 (7.6); 1.6968 (3.2); 1.6793 (3.2); 1.5355 (16.0); 0.0079 (0.6); −0.0002 (17.6); −0.0084 (0.7) I-133: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3813 (0.8); 7.3769 (1.0); 7.3621 (1.4); 7.3577 (2.0); 7.3480 (0.7); 7.3433 (1.4); 7.3392 (1.9); 7.3287 (1.2); 7.3242 (0.7); 7.3204 (1.0); 7.3160 (0.7); 7.3083 (0.8); 7.3039 (0.8); 7.2597 (38.3); 7.2558 (2.1); 7.2066 (0.9); 7.2031 (1.2); 7.1873 (1.5); 7.1856 (1.4); 7.1837 (1.4); 7.1681 (0.7); 7.1645 (0.6); 7.1485 (0.9); 7.1432 (1.1); 7.1377 (0.9); 7.1298 (1.0); 7.1244 (1.1); 7.1214 (1.1); 7.1164 (2.3); 7.1127 (1.0); 7.1027 (0.9); 7.0968 (1.7); 7.0917 (1.4); 7.0712 (1.1); 7.0532 (1.1); 7.0498 (1.0); 7.0325 (1.0); 7.0285 (1.7); 7.0247 (1.1); 7.0096 (1.0); 7.0066 (1.5); 7.0043 (1.6); 6.9991 (1.0); 6.9955 (1.2); 6.9902 (0.8); 6.9847 (0.7); 6.9793 (0.6); 6.9740 (0.6); 6.9688 (0.5); 4.8903 (14.9); 4.8862 (1.6); 4.2919 (1.9); 4.2741 (6.0); 4.2703 (0.7); 4.2563 (6.0); 4.2525 (0.6); 4.2385 (2.0); 1.5438 (13.1); 1.5400 (0.7); 1.3038 (8.0); 1.3005 (1.0); 1.2860 (16.0); 1.2826 (1.8); 1.2682 (9.1); 1.2647 (2.6); 0.8987 (1.1); 0.8817 (4.0); 0.8640 (1.5); −0.0002 (13.9); −0.0040 (0.8) I-134: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3790 (0.5); 7.3637 (1.0); 7.3572 (1.0); 7.3484 (0.6); 7.3423 (2.0); 7.3361 (0.7); 7.3268 (1.0); 7.3209 (1.2); 7.3057 (0.6); 7.2600 (30.0); 7.1873 (0.9); 7.1820 (1.0); 7.1686 (1.0); 7.1608 (1.2); 7.1553 (1.1); 7.1505 (1.0); 7.1418 (1.0); 7.1367 (1.1); 7.1293 (1.7); 7.1257 (1.0); 7.1091 (1.3); 7.1044 (1.6); 7.0843 (1.2); 7.0504 (0.8); 7.0459 (1.1); 7.0400 (1.2); 7.0352 (1.2); 7.0311 (0.9); 7.0251 (0.8); 7.0191 (0.7); 7.0145 (0.7); 6.9554 (3.0); 6.9370 (4.0); 6.9340 (4.0); 6.9156 (2.6); 4.8743 (16.0); 4.2811 (2.0); 4.2632 (6.3); 4.2454 (6.4); 4.2275 (2.1); 1.5445 (11.0); 1.3037 (0.7); 1.2900 (7.9); 1.2722 (16.0); 1.2543 (7.9); 0.8982 (1.2); 0.8815 (3.8); 0.8638 (1.6); 0.0079 (0.5); −0.0002 (15.1); −0.0084 (0.7) I-135: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.2791 (1.0); 7.2736 (0.6); 7.2654 (1.6); 7.2594 (33.1); 7.2495 (1.1); 7.2437 (1.4); 7.2367 (1.5); 7.2317 (0.7); 7.2215 (0.6); 7.2176 (1.4); 7.2007 (0.8); 7.1971 (0.5); 7.1832 (0.7); 7.0837 (1.3); 7.0797 (2.0); 7.0778 (1.7); 7.0665 (0.7); 7.0595 (1.4); 7.0556 (2.1); 7.0508 (0.5); 7.0338 (1.0); 3.7461 (10.0); 2.9553 (0.6); 2.8833 (0.5); 2.7723 (1.4); 1.7553 (16.0); 1.5440 (1.2); 0.0080 (0.6); −0.0002 (16.8); −0.0084 (0.7) I-136: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3977 (0.9); 7.3935 (1.1); 7.3785 (1.7); 7.3744 (2.1); 7.3663 (0.7); 7.3591 (1.5); 7.3552 (1.8); 7.3518 (1.3); 7.3472 (0.9); 7.3392 (1.1); 7.3336 (1.0); 7.3311 (1.0); 7.3267 (0.8); 7.3188 (0.9); 7.3144 (0.7); 7.2597 (43.0); 7.2129 (1.3); 7.1935 (1.9); 7.1759 (0.8); 7.1506 (1.0); 7.1450 (1.7); 7.1319 (1.1); 7.1237 (2.8); 7.1190 (1.8); 7.1033 (1.8); 7.0993 (2.4); 7.0782 (1.1); 7.0597 (1.3); 7.0565 (1.2); 7.0388 (1.3); 7.0351 (2.0); 7.0314 (1.3); 7.0139 (1.9); 7.0105 (2.0); 7.0037 (1.2); 6.9996 (1.2); 6.9950 (1.0); 6.9886 (0.8); 6.9824 (0.8); 6.9780 (0.7); 6.9733 (0.5); 4.9654 (16.0); 4.1318 (1.2); 4.1140 (1.2); 2.0453 (5.5); 1.4318 (0.7); 1.2764 (1.5); 1.2585 (2.9); 1.2407 (1.4); 0.0079 (0.8); −0.0002 (22.6); −0.0083 (1.0) I-137: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3871 (0.5); 7.3718 (1.0); 7.3656 (0.9); 7.3565 (0.6); 7.3504 (1.9); 7.3442 (0.6); 7.3351 (0.9); 7.3290 (1.1); 7.3137 (0.6); 7.2607 (30.4); 7.1884 (0.9); 7.1831 (0.9); 7.1696 (0.9); 7.1643 (1.1); 7.1618 (1.1); 7.1562 (1.6); 7.1430 (0.9); 7.1349 (1.6); 7.1311 (0.9); 7.1147 (1.3); 7.1099 (1.4); 7.0900 (1.1); 7.0533 (0.8); 7.0497 (0.9); 7.0428 (1.0); 7.0393 (1.0); 7.0341 (0.8); 7.0284 (0.6); 7.0232 (0.6); 7.0179 (0.6); 6.9709 (0.5); 6.9655 (1.2); 6.9626 (2.8); 6.9442 (3.7); 6.9411 (3.5); 6.9360 (0.6); 6.9229 (2.4); 6.9198 (1.0); 5.2985 (4.2); 4.9432 (16.0); 3.7819 (0.8); 3.7783 (3.0); 3.7763 (2.0); 3.7720 (1.9); 3.7699 (1.6); 3.7679 (2.5); 3.7617 (7.5); 3.7556 (2.6); 3.7513 (1.9); 3.7470 (2.0); 3.7450 (3.1); 3.7415 (0.7); 1.8763 (3.0); 1.8685 (2.8); 1.8643 (2.0); 1.8597 (9.0); 1.8549 (2.1); 1.8508 (2.8); 1.8430 (3.0); 1.8391 (0.7); 1.4319 (0.8); −0.0002 (17.0); −0.0085 (0.7) I-138: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5182 (1.6); 7.3446 (0.8); 7.2593 (301.4); 7.2485 (9.6); 7.2465 (9.6); 7.2399 (4.8); 7.2360 (6.9); 7.2315 (7.1); 7.2273 (14.9); 7.2187 (8.3); 7.2140 (8.9); 7.2085 (2.4); 7.2024 (3.5); 7.1831 (1.1); 7.1687 (0.6); 7.1120 (6.8); 7.1079 (8.6); 7.1022 (2.5); 7.0955 (3.6); 7.0910 (6.9); 7.0877 (5.7); 7.0612 (6.7); 7.0558 (2.4); 7.0394 (10.5); 7.0231 (2.0); 7.0177 (5.3); 6.9952 (1.6); 5.2993 (1.2); 5.2821 (4.4); 5.2646 (4.5); 5.2472 (1.2); 3.8179 (1.1); 1.7194 (16.0); 1.7020 (16.0); 1.4318 (0.7); 1.2557 (1.0); 0.1462 (0.5); 0.0080 (5.0); −0.0002 (159.4); −0.0084 (5.4); −0.1498 (0.6) I-139: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 19.9731 (0.8); 7.5183 (2.5); 7.3101 (0.9); 7.2930 (1.7); 7.2879 (2.5); 7.2711 (13.4); 7.2594 (475.1); 7.2526 (17.5); 7.2436 (7.6); 7.2360 (6.9); 7.2274 (3.8); 7.2094 (2.5); 7.1355 (6.0); 7.1314 (7.6); 7.1145 (6.1); 7.1113 (5.1); 7.0781 (6.1); 7.0564 (9.6); 7.0345 (4.8); 6.9954 (2.5); 5.3315 (1.2); 5.3139 (4.4); 5.2965 (4.5); 5.2788 (1.3); 1.7459 (15.8); 1.7284 (16.0); 1.2562 (0.8); 0.1458 (0.9); 0.0079 (8.1); −0.0002 (246.6); −0.0084 (8.8); −0.0499 (0.9); −0.1499 (0.9) I-140: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5189 (0.8); 7.2600 (132.6); 7.2336 (4.5); 7.2164 (2.5); 7.1101 (2.3); 7.0932 (2.1); 7.0732 (1.7); 7.0520 (2.8); 7.0304 (1.4); 6.9960 (0.8); 2.0043 (0.9); 1.7788 (16.0); 1.2553 (0.7); 0.0079 (3.3); −0.0002 (78.0); −0.0084 (4.2) I-141: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3390 (0.7); 7.3319 (2.8); 7.3229 (3.6); 7.3156 (4.9); 7.3046 (2.2); 7.2997 (1.2); 7.2952 (2.2); 7.2877 (1.0); 7.2823 (2.0); 7.2602 (10.9); 7.1667 (1.9); 7.1576 (1.9); 7.1533 (1.4); 7.1487 (1.5); 7.1459 (1.1); 7.1423 (1.6); 7.0922 (2.0); 7.0869 (0.7); 7.0707 (3.2); 7.0661 (0.9); 7.0542 (0.6); 7.0490 (1.6); 5.2973 (1.3); 5.2446 (1.7); 5.2271 (1.7); 5.2097 (0.5); 3.7821 (16.0); 1.6915 (6.8); 1.6740 (6.8); 1.5553 (0.5); −0.0002 (4.2) I-146: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3732 (1.0); 7.3668 (0.8); 7.3580 (0.6); 7.3518 (2.0); 7.3455 (0.7); 7.3363 (0.9); 7.3304 (1.2); 7.3151 (0.6); 7.2650 (0.5); 7.2592 (51.0); 7.1808 (0.8); 7.1756 (0.9); 7.1622 (0.9); 7.1545 (1.7); 7.1488 (1.1); 7.1347 (1.8); 7.1300 (1.8); 7.1135 (1.2); 7.1087 (1.4); 7.0887 (1.1); 7.0460 (0.7); 7.0410 (0.8); 7.0354 (1.0); 7.0318 (1.0); 7.0266 (0.8); 7.0209 (0.7); 7.0157 (0.6); 7.0104 (0.6); 6.9772 (0.9); 6.9730 (0.6); 6.9673 (1.1); 6.9644 (2.9); 6.9513 (0.6); 6.9460 (3.7); 6.9429 (3.7); 6.9247 (2.6); 6.9216 (1.1); 6.9164 (0.5); 5.9521 (0.6); 5.9380 (1.2); 5.9260 (0.7); 5.9239 (0.7); 5.9118 (1.3); 5.9092 (0.8); 5.8976 (0.7); 5.8950 (1.4); 5.8829 (0.8); 5.8809 (0.8); 5.8688 (1.4); 5.8547 (0.7); 5.3471 (0.7); 5.3433 (2.0); 5.3396 (2.1); 5.3358 (0.9); 5.3042 (0.6); 5.3003 (1.7); 5.2966 (1.9); 5.2928 (0.8); 5.2365 (0.8); 5.2334 (2.1); 5.2301 (2.2); 5.2269 (0.9); 5.2104 (0.8); 5.2072 (2.0); 5.2039 (2.1); 5.2007 (0.9); 5.0015 (0.7); 4.9177 (15.3); 4.7050 (2.4); 4.7015 (4.0); 4.6981 (2.7); 4.6909 (2.6); 4.6874 (4.0); 4.6839 (2.7); 2.2705 (1.7); 1.5390 (4.2); 1.4319 (16.0); 1.2559 (0.9); 0.0080 (0.5); −0.0002 (19.1); −0.0085 (0.9) I-149: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4454 (0.5); 7.4300 (1.1); 7.4238 (1.0); 7.4146 (0.6); 7.4085 (2.0); 7.4024 (0.7); 7.3931 (1.0); 7.3869 (1.2); 7.3716 (0.6); 7.2596 (76.5); 7.2239 (1.0); 7.2190 (0.9); 7.2057 (0.9); 7.1994 (1.3); 7.1931 (0.9); 7.1770 (1.3); 7.1559 (1.5); 7.1525 (1.0); 7.1362 (1.4); 7.1312 (1.4); 7.1119 (1.2); 7.0784 (1.0); 7.0726 (1.0); 7.0678 (1.0); 7.0569 (0.7); 7.0513 (0.6); 7.0467 (0.6); 6.9957 (0.5); 6.9870 (1.5); 6.9835 (2.6); 6.9654 (3.8); 6.9619 (3.8); 6.9438 (2.3); 6.9401 (1.3); 5.9436 (0.5); 5.9293 (1.1); 5.9174 (0.7); 5.9151 (0.6); 5.9032 (1.3); 5.9009 (0.8); 5.8887 (0.8); 5.8863 (1.4); 5.8744 (0.8); 5.8721 (0.8); 5.8602 (1.4); 5.8459 (0.7); 5.3474 (0.8); 5.3437 (2.2); 5.3400 (2.2); 5.3363 (0.9); 5.3044 (0.7); 5.3007 (1.9); 5.2971 (2.0); 5.2933 (0.8); 5.2412 (0.9); 5.2382 (2.3); 5.2351 (2.2); 5.2320 (0.9); 5.2151 (0.9); 5.2121 (2.1); 5.2090 (2.1); 5.2059 (0.8); 5.0047 (16.0); 4.7072 (2.9); 4.7038 (4.7); 4.7004 (2.9); 4.6929 (3.0); 4.6895 (4.6); 4.6861 (2.8); 1.5355 (14.9); 1.4319 (1.3); 0.0078 (0.8); −0.0002 (27.7); −0.0086 (1.2) I-150: .sup.1H-NMR(300.1 MHz, d.sub.6-DMSO): δ = 7.6062 (2.4); 7.5988 (2.4); 7.5721 (2.3); 7.5649 (2.4); 7.5109 (1.6); 7.4967 (1.1); 7.4828 (3.8); 7.4756 (1.7); 7.4686 (2.2); 7.4555 (3.2); 7.4465 (3.0); 7.4401 (2.1); 7.4183 (1.8); 7.4054 (4.2); 7.4027 (4.1); 7.3983 (2.8); 7.3769 (1.9); 7.3732 (2.3); 7.2294 (1.0); 7.2230 (1.0); 7.2016 (1.8); 7.1950 (1.7); 7.1753 (0.8); 7.1669 (0.8); 4.9336 (12.6); 4.2054 (2.2); 4.1817 (6.8); 4.1580 (6.9); 4.1344 (2.2); 3.3214 (19.8); 2.5141 (10.6); 2.5085 (19.2); 2.5026 (24.1); 2.4968 (16.6); 1.9894 (0.8); 1.2348 (0.5); 1.2119 (7.8); 1.1883 (16.0); 1.1750 (1.2); 1.1646 (7.3); 1.1514 (0.4); 0.0107 (0.8); 0.0000 (15.2); −0.0110 (0.6) I-151: .sup.1H-NMR(300.3 MHz, d.sub.6-DMSO): δ = 7.6216 (4.0); 7.5923 (3.8); 7.5816 (3.3); 7.5246 (2.0); 7.4965 (4.6); 7.4691 (3.5); 7.4334 (4.1); 7.4117 (13.2); 7.3817 (3.0); 4.9452 (15.7); 4.2088 (2.5); 4.1852 (7.7); 4.1615 (7.8); 4.1379 (2.6); 3.3717 (41.8); 3.3661 (39.4); 2.5111 (5.1); 2.0832 (0.4); 1.2304 (1.2); 1.2138 (8.0); 1.1902 (16.0); 1.1666 (7.7); −0.0001 (0.4) I-152: .sup.1H-NMR(300.1 MHz, d.sub.6-DMSO): δ = 7.7620 (4.8); 7.7572 (4.5); 7.6027 (2.6); 7.5973 (2.6); 7.5672 (4.0); 7.5385 (8.3); 7.5283 (5.2); 7.5061 (0.7); 7.4997 (0.8); 7.4262 (0.9); 7.3983 (3.7); 7.3806 (8.3); 7.3586 (0.7); 7.3524 (0.6); 4.9164 (13.0); 4.1929 (2.3); 4.1692 (7.0); 4.1455 (7.1); 4.1219 (2.4); 3.3282 (74.2); 2.5100 (10.8); 2.5043 (13.2); 2.4986 (9.3); 1.2333 (1.1); 1.2086 (7.8); 1.1849 (16.0); 1.1612 (7.4); 0.0001 (5.4) I-153: .sup.1H-NMR(300.1 MHz, d.sub.6-DMSO): δ = 7.7512 (6.5); 7.7478 (6.6); 7.5704 (1.7); 7.5419 (8.8); 7.5332 (7.4); 7.5040 (1.5); 7.4986 (1.5); 7.4798 (1.4); 7.4518 (2.9); 7.4287 (3.3); 7.4230 (3.4); 7.4018 (2.1); 7.3823 (3.1); 7.3547 (1.7); 7.3481 (1.7); 7.2075 (1.7); 7.2021 (1.7); 7.1796 (3.0); 7.1520 (1.6); 4.9238 (15.8); 4.1992 (2.6); 4.1757 (7.6); 4.1521 (7.8); 4.1286 (2.8); 3.3512 (38.7); 2.5127 (4.4); 2.0834 (0.4); 1.2335 (1.7); 1.2137 (8.4); 1.1901 (16.0); 1.1665 (8.0); 0.0003 (0.6) I-154: .sup.1H-NMR(300.1 MHz, d.sub.6-DMSO): δ = 7.7772 (5.7); 7.7711 (5.5); 7.6052 (2.7); 7.5981 (2.7); 7.5709 (2.7); 7.5643 (2.8); 7.5520 (1.9); 7.5455 (1.6); 7.5242 (4.8); 7.5177 (4.6); 7.4951 (6.6); 7.4671 (2.8); 7.4343 (3.7); 7.4081 (3.4); 7.3831 (3.7); 7.3772 (3.2); 7.3539 (1.5); 7.3481 (1.4); 4.9380 (13.6); 4.2073 (2.3); 4.1836 (6.9); 4.1599 (7.0); 4.1363 (2.3); 3.3233 (22.0); 2.5089 (14.2); 2.5034 (17.3); 2.4980 (12.4); 1.2328 (0.8); 1.2144 (7.9); 1.1907 (16.0); 1.1671 (7.5); 0.0001 (7.2) I-155: .sup.1H-NMR(3OO.1 MHz, d.sub.6-DMSO): δ = 7.6142 (2.7); 7.6058 (2.8); 7.5957 (2.9); 7.5878 (3.5); 7.5855 (3.4); 7.5763 (2.8); 7.5614 (2.9); 7.5549 (4.2); 7.5346 (2.2); 7.5262 (2.5); 7.5060 (2.3); 7.4557 (1.6); 7.4274 (3.5); 7.4013 (3.4); 7.3766 (3.4); 7.3695 (3.1); 7.3604 (1.9); 7.3514 (2.0); 7.3395 (1.7); 7.3322 (2.7); 7.3236 (2.3); 7.3038 (1.2); 7.2952 (1.0); 4.9360 (13.0); 4.2077 (2.2); 4.1840 (6.8); 4.1604 (6.9); 4.1367 (2.3); 3.3199 (10.7); 2.5089 (10.6); 2.5031 (13.2); 2.4973 (9.0); 2.0757 (2.8); 1.2151 (7.8); 1.1915 (16.0); 1.1678 (7.4); −0.0001 (7.8); −0.0111 (0.3) I-156: .sup.1H-NMR(300.1 MHz, d.sub.6-DMSO): δ = 7.5759 (3.7); 7.5497 (6.4); 7.5414 (3.2); 7.5227 (2.9); 7.4206 (2.8); 7.4169 (2.6); 7.3919 (2.2); 7.3874 (2.2); 7.3776 (2.5); 7.3699 (1.5); 7.3586 (3.3); 7.3478 (5.6); 7.3370 (2.5); 7.3295 (5.0); 7.3073 (5.2); 7.2778 (6.9); 7.2482 (2.4); 4.9203 (14.1); 4.2024 (2.3); 4.1788 (7.1); 4.1551 (7.2); 4.1315 (2.4); 3.3288 (66.3); 2.5094 (9.8); 2.5039 (12.1); 2.4984 (8.8); 1.2341 (1.6); 1.2108 (8.0); 1.1872 (16.0); 1.1635 (7.6); 0.0001 (2.4) I-157: .sup.1H-NMR(300.1 MHz, d.sub.6-DMSO): δ = 7.5937 (2.5); 7.5859 (3.2); 7.5593 (3.6); 7.5544 (5.7); 7.5258 (8.1); 7.5191 (2.6); 7.5030 (3.0); 7.4968 (8.3); 7.4889 (1.3); 7.4313 (2.3); 7.4278 (2.4); 7.4238 (2.2); 7.4026 (1.6); 7.3991 (1.7); 7.3952 (1.5); 7.3320 (8.2); 7.3256 (2.7); 7.3096 (2.6); 7.3034 (6.1); 4.9243 (12.8); 4.2026 (2.2); 4.1790 (6.9); 4.1553 (7.0); 4.1316 (2.3); 3.3336 (64.1); 2.5107 (6.4); 2.5049 (8.0); 2.4992 (5.6); 2.0768 (1.4); 1.2340 (0.7); 1.2105 (7.7); 1.1868 (16.0); 1.1631 (7.4); 0.0000 (1.3) I-158: .sup.1H-NMR(300.1 MHz, d.sub.6-DMSO): δ = 7.7502 (5.8); 7.7429 (5.9); 7.6476 (3.9); 7.6192 (6.5); 7.5476 (4.1); 7.5401 (3.7); 7.5191 (2.5); 7.5117 (2.3); 7.3687 (2.8); 7.3618 (1.9); 7.3499 (4.0); 7.3394 (6.0); 7.3212 (5.2); 7.2903 (5.3); 7.2609 (7.3); 7.2315 (2.7); 5.0201 (0.4); 4.9040 (14.6); 4.1908 (2.5); 4.1672 (7.3); 4.1435 (7.5); 4.1199 (2.7); 4.0964 (0.3); 3.3330 (31.8); 2.5116 (6.2); 2.5066 (7.2); 1.2335 (1.6); 1.2083 (8.2); 1.1847 (16.0); 1.1611 (7.8); 1.1294 (0.4); 0.0003 (1.3) I-159: .sup.1H-NMR(300.1 MHz, d.sub.6-DMSO): δ = 7.7576 (5.5); 7.7502 (5.6); 7.6480 (3.6); 7.6196 (6.3); 7.5537 (4.0); 7.5461 (3.6); 7.5253 (2.5); 7.5175 (2.9); 7.5070 (6.5); 7.5008 (2.6); 7.4845 (3.4); 7.4785 (8.5); 7.3172 (8.5); 7.3108 (2.8); 7.2947 (2.8); 7.2887 (6.2); 4.9041 (12.8); 4.1888 (2.2); 4.1652 (6.9); 4.1415 (7.0); 4.1178 (2.3); 3.6856 (0.3); 3.3222 (13.8); 2.5099 (7.6); 2.5041 (9.3); 2.4984 (6.5); 2.0767 (0.4); 1.2357 (0.6); 1.2062 (7.8); 1.1826 (16.0); 1.1589 (7.4); 0.0001 (4.6) I-160: .sup.1H-NMR(300.1 MHz, d.sub.6-DMSO): δ = 7.6095 (2.5); 7.6034 (2.4); 7.5767 (2.5); 7.5709 (2.5); 7.5538 (1.6); 7.5265 (3.3); 7.5010 (3.0); 7.4685 (3.8); 7.4623 (3.2); 7.4406 (1.8); 7.4344 (1.6); 7.2690 (0.8); 7.2384 (8.9); 7.2330 (8.4); 7.2134 (16.0); 7.1843 (0.5); 7.1651 (0.4); 7.1563 (0.3); 7.1257 (0.3); 4.9655 (11.9); 4.2257 (2.2); 4.2020 (6.4); 4.1784 (6.5); 4.1547 (2.2); 3.3449 (33.4); 2.5140 (3.1); 2.5086 (3.7); 1.2300 (7.6); 1.2064 (14.3); 1.1827 (6.8); 0.0000 (0.5) I-161: .sup.1H-NMR(300.1 MHz, d.sub.6-DMSO): δ = 7.6310 (2.4); 7.6246 (2.5); 7.5980 (2.4); 7.5920 (2.5); 7.5638 (1.5); 7.5363 (3.4); 7.5112 (3.2); 7.4849 (4.2); 7.4785 (4.2); 7.4679 (6.9); 7.4607 (2.9); 7.4576 (2.6); 7.4504 (2.5); 7.4455 (3.0); 7.4384 (8.2); 7.4284 (1.1); 7.2008 (1.2); 7.1908 (8.0); 7.1837 (2.5); 7.1680 (2.6); 7.1613 (6.5); 7.1509 (0.7); 4.9686 (11.8); 4.2225 (2.1); 4.1988 (6.9); 4.1751 (7.0); 4.1514 (2.3); 3.5005 (0.3); 3.3950 (0.6); 3.3352 (356.2); 2.5090 (22.0); 2.5032 (28.0); 2.4974 (19.7); 1.2275 (8.2); 1.2038 (16.0); 1.1802 (7.4); 0.8535 (0.4); 0.0000 (9.7); −0.0111 (0.5) I-162: .sup.1H-NMR(300.1 MHz, d.sub.6-DMSO): δ = 7.6365 (1.6); 7.6176 (1.8); 7.6062 (2.6); 7.6009 (3.5); 7.5906 (5.4); 7.5724 (2.8); 7.5630 (4.3); 7.4204 (0.9); 7.3928 (3.3); 7.3732 (7.0); 7.3553 (1.8); 7.3457 (1.8); 7.3280 (2.0); 7.3185 (1.8); 7.2989 (1.2); 7.2894 (1.0); 4.9134 (12.5); 4.8877 (0.4); 4.1929 (2.2); 4.1693 (6.8); 4.1456 (6.8); 4.1220 (2.2); 3.3288 (67.9); 2.5101 (8.3); 2.5042 (10.5); 2.4984 (7.3); 1.2342 (1.5); 1.2086 (7.8); 1.1850 (16.0); 1.1613 (7.4); −0.0001 (2.0) I-163: .sup.1H-NMR(300.1 MHz, d.sub.6-DMSO): δ = 7.6120 (2.4); 7.6063 (2.4); 7.5765 (2.8); 7.5730 (2.8); 7.5522 (1.2); 7.5428 (2.0); 7.5230 (2.0); 7.5134 (1.2); 7.4936 (1.1); 7.4446 (1.5); 7.4349 (1.5); 7.4209 (3.7); 7.4143 (2.3); 7.4005 (8.4); 7.3788 (1.5); 7.3695 (1.8); 7.2229 (0.9); 7.2181 (1.0); 7.2137 (0.9); 7.1912 (1.6); 7.1658 (0.8); 7.1613 (0.8); 7.1570 (0.7); 7.1525 (0.6); 4.9291 (12.8); 4.2037 (2.3); 4.1800 (6.9); 4.1564 (7.0); 4.1327 (2.2); 3.5477 (0.5); 3.3191 (18.5); 2.5137 (8.6); 2.5082 (15.6); 2.5024 (19.4); 2.4965 (13.3); 1.2098 (7.8); 1.1861 (16.0); 1.1625 (7.3); −0.0001 (11.6); −0.0112 (0.5) I-164: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.7645 (0.6); 7.3332 (0.5); 7.3277 (0.8); 7.3131 (0.8); 7.3079 (0.7); 7.2928 (0.9); 7.2872 (0.8); 7.2701 (2.3); 7.2663 (1.2); 7.2638 (1.5); 7.2586 (26.8); 7.2515 (3.0); 7.2441 (1.1); 7.2400 (1.5); 7.2361 (1.0); 7.2231 (1.0); 7.1329 (1.8); 7.1289 (2.6); 7.1233 (0.7); 7.1162 (1.0); 7.1117 (1.9); 7.1088 (1.6); 7.0716 (0.6); 7.0692 (0.8); 7.0653 (0.8); 7.0628 (0.9); 7.0557 (0.9); 7.0518 (1.3); 7.0495 (1.0); 7.0417 (0.5); 7.0365 (0.7); 7.0330 (1.2); 7.0302 (0.9); 7.0269 (0.8); 7.0209 (0.7); 7.0034 (0.7); 6.9994 (0.7); 6.9936 (0.5); 5.2688 (1.6); 5.2513 (1.7); 3.7889 (16.0); 3.7719 (1.7); 1.6994 (6.7); 1.6868 (1.2); 1.6819 (6.7); 1.6695 (0.8); 1.5352 (2.4); −0.0002 (9.7) I-165: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.7643 (0.9); 7.3183 (0.6); 7.3018 (2.1); 7.2981 (0.9); 7.2955 (0.9); 7.2871 (1.1); 7.2833 (2.5); 7.2784 (1.0); 7.2742 (1.7); 7.2703 (1.1); 7.2587 (17.6); 7.1355 (1.8); 7.1314 (2.4); 7.1258 (0.7); 7.1189 (1.0); 7.1144 (2.0); 7.1113 (1.6); 6.8371 (0.6); 6.8219 (2.1); 6.8165 (2.5); 6.8065 (1.3); 6.7991 (3.6); 5.2968 (1.1); 5.2595 (1.6); 5.2421 (1.7); 5.2247 (0.5); 3.7853 (16.0); 3.7721 (2.7); 1.6969 (6.7); 1.6869 (1.5); 1.6794 (6.6); 1.6695 (1.3); 1.5430 (2.1); −0.0002 (6.3) I-166: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4230 (0.7); 7.4202 (0.5); 7.4180 (0.6); 7.4094 (0.5); 7.4071 (0.5); 7.4049 (0.6); 7.4023 (0.7); 7.3169 (0.9); 7.3131 (0.9); 7.2991 (0.7); 7.2948 (0.6); 7.2586 (17.3); 7.2401 (2.3); 7.2361 (1.1); 7.2345 (1.1); 7.2250 (1.2); 7.2212 (2.8); 7.2116 (1.6); 7.2091 (1.6); 7.2071 (1.8); 7.2032 (1.1); 7.1929 (1.8); 7.1903 (2.6); 7.1743 (0.9); 7.1714 (0.9); 7.1467 (2.2); 7.1427 (3.1); 7.1370 (0.7); 7.1298 (1.1); 7.1254 (1.9); 7.1224 (1.5); 7.0927 (0.7); 7.0904 (0.7); 7.0690 (1.2); 7.0475 (0.6); 7.0454 (0.6); 5.2967 (2.0); 5.2928 (0.6); 5.2753 (1.8); 5.2579 (1.8); 5.2405 (0.5); 3.7949 (16.0); 1.7042 (7.4); 1.6868 (7.3); 1.5386 (1.0); −0.0002 (9.6) I-169: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3538 (0.6); 7.3476 (0.6); 7.3323 (1.0); 7.3171 (0.6); 7.3109 (0.6); 7.2602 (28.6); 7.2514 (0.8); 7.2481 (0.6); 7.1750 (0.6); 7.1536 (0.6); 7.1481 (0.6); 7.1445 (0.5); 7.1348 (0.5); 7.1296 (0.6); 7.1233 (0.9); 7.1195 (0.5); 7.1033 (0.7); 7.0983 (0.8); 7.0783 (0.6); 7.0355 (0.5); 7.0289 (0.6); 7.0248 (0.5); 6.9246 (0.7); 5.1950 (1.6); 5.1777 (1.6); 3.7529 (16.0); 1.6837 (6.5); 1.6663 (6.4); 1.5409 (1.9); 0.0079 (0.7); −0.0002 (18.0); −0.0086 (0.9) I-176: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4057 (3.0); 7.4014 (2.7); 7.3945 (1.1); 7.3923 (1.0); 7.3878 (1.6); 7.3864 (1.4); 7.3757 (0.6); 7.3010 (1.8); 7.2966 (2.0); 7.2903 (0.6); 7.2891 (0.7); 7.2877 (0.6); 7.2851 (0.8); 7.2829 (0.8); 7.2766 (1.4); 7.2601 (32.2); 7.1584 (0.9); 7.1428 (0.8); 7.1381 (0.5); 6.9279 (0.8); 6.9226 (0.6); 6.9029 (1.3); 6.8970 (0.8); 6.8845 (0.8); 6.8822 (0.9); 6.8781 (0.6); 6.8758 (0.5); 6.8323 (0.7); 6.8301 (0.7); 6.8274 (0.6); 6.8252 (0.6); 6.8120 (0.6); 6.8099 (0.6); 6.8070 (0.6); 5.2991 (5.6); 5.2536 (1.5); 5.2362 (1.5); 3.8008 (16.0); 2.7744 (3.0); 1.7044 (6.2); 1.6870 (6.1); 1.5997 (0.9); 0.0080 (0.6); −0.0002 (18.5) I-177: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4213 (1.2); 7.4167 (1.6); 7.4078 (7.3); 7.4045 (7.9); 7.3986 (2.9); 7.3937 (2.6); 7.3897 (4.8); 7.3806 (1.2); 7.3763 (1.6); 7.3707 (0.5); 7.3666 (0.8); 7.3456 (0.7); 7.3004 (1.1); 7.2951 (5.7); 7.2909 (5.8); 7.2862 (2.2); 7.2842 (1.9); 7.2812 (1.8); 7.2782 (2.6); 7.2761 (3.1); 7.2709 (3.8); 7.2600 (22.9); 7.1810 (1.3); 7.1655 (1.2); 7.1605 (2.6); 7.1449 (2.4); 7.1401 (1.4); 7.1247 (1.3); 6.9274 (1.3); 6.9219 (2.7); 6.9167 (2.0); 6.9061 (1.5); 6.9037 (2.3); 6.8973 (3.0); 6.8922 (2.2); 6.8855 (2.2); 6.8832 (2.6); 6.8792 (1.3); 6.8769 (1.3); 6.8622 (3.2); 6.8592 (2.6); 6.8570 (2.3); 6.8416 (1.9); 6.8395 (1.8); 6.8367 (1.6); 6.8346 (1.3); 6.0115 (1.1); 5.3340 (1.2); 5.3165 (4.5); 5.3024 (0.9); 5.2990 (4.5); 5.2815 (1.2); 1.7566 (16.0); 1.7391 (15.8); 1.7038 (1.2); 1.6864 (1.2); 0.0080 (0.8); −0.0002 (29.9); −0.0085 (0.9) I-178: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4466 (0.6); 7.4404 (0.6); 7.4251 (1.1); 7.4099 (0.6); 7.4036 (0.6); 7.2615 (16.5); 7.1948 (0.7); 7.1755 (0.6); 7.1708 (1.1); 7.1660 (0.6); 7.1527 (0.8); 7.1508 (0.6); 7.1477 (0.7); 7.1405 (0.6); 7.1327 (0.6); 7.1298 (0.6); 7.1269 (0.6); 7.1233 (0.9); 7.1214 (1.1); 7.0013 (0.6); 6.9976 (0.6); 6.9826 (0.6); 5.1792 (1.6); 5.1618 (1.6); 3.7555 (16.0); 1.6871 (6.6); 1.6697 (6.5); 1.5496 (1.0); −0.0002 (10.7) I-179: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4467 (0.6); 7.4406 (0.7); 7.4253 (1.2); 7.4100 (0.7); 7.4038 (0.7); 7.2617 (13.1); 7.2161 (0.5); 7.1948 (1.0); 7.1752 (0.9); 7.1708 (1.5); 7.1663 (0.9); 7.1526 (1.1); 7.1478 (1.0); 7.1406 (0.9); 7.1325 (0.8); 7.1270 (0.9); 7.1215 (1.5); 7.1139 (0.7); 7.1083 (0.5); 6.9976 (1.0); 6.9820 (1.0); 5.1967 (0.5); 5.1793 (1.7); 5.1619 (1.7); 5.1445 (0.5); 3.7555 (16.0); 1.6871 (7.0); 1.6697 (7.0); −0.0002 (8.0) II-01: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): δ = 7.4677 (1.3); 7.4591 (5.0); 7.4564 (4.7); 7.4541 (3.9); 7.4485 (8.2); 7.4424 (10.4); 7.4331 (1.3); 7.3315 (1.2); 7.3148 (1.5); 7.3108 (2.8); 7.2965 (4.9); 7.2944 (5.1); 7.2905 (4.1); 7.2876 (5.2); 7.2785 (4.2); 7.2728 (4.3); 7.0697 (1.1); 7.0654 (1.1); 7.0482 (1.8); 7.0442 (1.9); 7.0272 (0.9); 7.0230 (1.0); 6.9311 (1.3); 6.9257 (2.1); 6.9200 (1.5); 6.9052 (1.3); 6.9000 (2.2); 6.8940 (1.6); 6.8856 (2.4); 6.8835 (2.7); 6.8808 (2.0); 6.8785 (1.7); 6.8653 (2.1); 6.8633 (2.2); 6.8605 (2.0); 4.2659 (16.0); 3.2925 (0.7); 2.6742 (1.3); 2.6695 (1.8); 2.6650 (1.3); 2.5996 (0.6); 2.5955 (0.5); 2.5587 (0.9); 2.5541 (1.8); 2.5495 (2.6); 2.5448 (2.4); 2.5401 (2.1); 2.5230 (8.0); 2.5183 (11.4); 2.5095 (107.9); 2.5051 (223.3); 2.5005 (302.9); 2.4959 (216.2); 2.4914 (102.7); 2.4636 (1.0); 2.4585 (0.5); 2.3318 (1.4); 2.3273 (1.9); 2.3227 (1.4); 0.0080 (1.2); −0.0002 (38.8); −0.0085 (1.5) II-02: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): δ = 7.4592 (6.1); 7.4490 (9.5); 7.4426 (11.3); 7.3322 (1.4); 7.3117 (3.2); 7.2961 (6.6); 7.2910 (5.1); 7.2874 (6.1); 7.2785 (4.9); 7.2727 (4.4); 7.0728 (1.2); 7.0663 (1.4); 7.0511 (2.1); 7.0467 (2.3); 7.0320 (1.1); 7.0255 (1.2); 6.9360 (1.6); 6.9306 (2.5); 6.9249 (1.8); 6.9102 (1.6); 6.9049 (2.6); 6.8991 (1.9); 6.8843 (3.1); 6.8641 (2.5); 6.8613 (2.4); 4.2979 (16.0); 3.5676 (1.2); 3.2987 (5.8); 2.6747 (3.1); 2.6701 (4.3); 2.6655 (3.1); 2.6136 (0.8); 2.5879 (0.8); 2.5492 (2.1); 2.5447 (3.9); 2.5234 (27.4); 2.5188 (38.3); 2.5100 (276.3); 2.5055 (561.0); 2.5010 (754.3); 2.4964 (546.2); 2.4919 (268.5); 2.4351 (1.1); 2.4003 (0.8); 2.3956 (0.7); 2.3905 (0.5); 2.3323 (3.6); 2.3277 (4.8); 2.3232 (3.7); 0.0080 (2.2); −0.0002 (62.8); −0.0085 (3.1) II-04: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): δ = 7.4612 (9.0); 7.4559 (6.4); 7.4531 (10.2); 7.4452 (10.4); 7.4411 (3.6); 7.4352 (1.3); 7.4201 (0.6); 7.4097 (0.8); 7.4034 (0.9); 7.3498 (1.5); 7.3333 (1.9); 7.3292 (3.3); 7.3128 (3.9); 7.3082 (3.5); 7.3047 (5.6); 7.3010 (3.6); 7.2973 (5.1); 7.2943 (4.6); 7.2914 (5.1); 7.2882 (4.6); 7.2845 (3.1); 7.2807 (4.2); 7.1042 (1.4); 7.0997 (1.4); 7.0828 (2.4); 7.0784 (2.4); 7.0636 (1.1); 7.0616 (1.2); 7.0571 (1.2); 6.9641 (1.8); 6.9587 (2.8); 6.9529 (1.9); 6.9384 (1.8); 6.9332 (2.9); 6.9272 (2.0); 6.9054 (2.9); 6.9033 (3.2); 6.9006 (2.6); 6.8984 (2.4); 6.8852 (2.6); 6.8831 (2.7); 6.8802 (2.6); 6.8782 (2.2); 6.5483 (0.7); 6.5083 (0.6); 4.6410 (16.0); 3.7305 (1.2); 3.5917 (10.8); 3.5799 (12.4); 3.5679 (11.6); 3.3549 (2.2); 2.8119 (10.1); 2.7998 (11.2); 2.7880 (9.8); 2.6740 (1.0); 2.6694 (1.5); 2.6647 (1.1); 2.5228 (4.6); 2.5182 (6.6); 2.5094 (79.9); 2.5049 (168.4); 2.5003 (230.8); 2.4958 (164.0); 2.4912 (76.9); 2.4589 (0.5); 2.4546 (0.8); 2.4497 (1.2); 2.4453 (1.1); 2.3806 (0.5); 2.3316 (1.1); 2.3271 (1.4); 2.3226 (1.1); 0.0080 (1.5); −0.0002 (47.9); −0.0085 (1.8) II-05: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): δ = 7.4597 (5.9); 7.4516 (6.9); 7.4437 (7.2); 7.4341 (1.0); 7.3407 (1.0); 7.3241 (1.3); 7.3201 (2.2); 7.3117 (0.8); 7.3013 (4.7); 7.2939 (3.6); 7.2911 (3.1); 7.2877 (2.9); 7.2843 (3.8); 7.2774 (3.0); 7.0944 (1.0); 7.0897 (1.0); 7.0730 (1.7); 7.0683 (1.7); 7.0536 (0.8); 7.0517 (0.8); 7.0471 (0.8); 6.9550 (1.2); 6.9496 (2.0); 6.9439 (1.3); 6.9293 (1.2); 6.9241 (2.0); 6.9183 (1.4); 6.9003 (2.2); 6.8975 (1.8); 6.8819 (1.8); 6.8801 (1.9); 6.8772 (1.8); 5.9152 (0.6); 5.8889 (0.8); 5.8720 (0.9); 5.8458 (0.8); 5.7527 (16.0); 5.3459 (1.4); 5.3422 (1.5); 5.3026 (1.2); 5.2990 (1.2); 5.2357 (1.5); 5.2324 (1.5); 5.2095 (1.4); 5.2063 (1.4); 4.5838 (9.4); 3.4125 (2.8); 3.4092 (2.0); 3.3976 (2.9); 2.5101 (12.4); 2.5057 (28.0); 2.5011 (39.9); 2.4966 (30.1); 2.4922 (15.6); −0.0002 (7.0) II-06: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): δ = 7.4659 (1.8); 7.4600 (8.1); 7.4515 (9.7); 7.4477 (6.6); 7.4439 (11.4); 7.4409 (5.1); 7.4343 (2.1); 7.4096 (0.8); 7.4050 (0.8); 7.3970 (0.9); 7.3921 (0.9); 7.3381 (1.5); 7.3216 (1.8); 7.3175 (3.3); 7.3091 (1.1); 7.2992 (6.8); 7.2912 (5.2); 7.2893 (4.9); 7.2859 (4.2); 7.2817 (5.7); 7.2751 (5.0); 7.2689 (1.4); 7.0922 (1.2); 7.0903 (1.4); 7.0839 (1.4); 7.0689 (2.4); 7.0627 (2.5); 7.0496 (1.2); 7.0477 (1.3); 7.0432 (1.3); 7.0413 (1.3); 6.9524 (1.8); 6.9469 (2.8); 6.9412 (2.0); 6.9266 (1.8); 6.9213 (3.0); 6.9155 (2.1); 6.8948 (2.8); 6.8928 (3.2); 6.8900 (2.7); 6.8880 (2.6); 6.8746 (2.6); 6.8726 (2.8); 6.8697 (2.7); 6.8677 (2.4); 5.7531 (16.0); 4.5178 (12.9); 2.7229 (3.9); 2.7043 (4.8); 2.6853 (4.3); 2.6749 (0.6); 2.6702 (0.6); 2.5236 (1.0); 2.5189 (1.5); 2.5102 (22.4); 2.5057 (48.9); 2.5011 (69.0); 2.4965 (50.9); 2.4920 (26.2); 1.5622 (2.0); 1.5434 (3.6); 1.5246 (3.8); 1.5060 (2.3); 1.4874 (0.7); 0.8847 (7.7); 0.8661 (16.0); 0.8474 (7.2); −0.0002 (12.8); −0.0085 (0.6) II-07: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): δ = 7.6913 (1.0); 7.6823 (1.3); 7.6792 (1.0); 7.6728 (1.3); 7.6672 (1.2); 7.6036 (1.4); 7.5635 (1.6); 7.4630 (3.1); 7.4581 (2.1); 7.4551 (3.3); 7.4524 (2.0); 7.4469 (3.2); 7.4419 (1.1); 7.4296 (0.7); 7.4233 (2.1); 7.4137 (2.7); 7.4068 (2.9); 7.3572 (0.6); 7.3407 (0.7); 7.3366 (1.2); 7.3202 (1.3); 7.3159 (1.0); 7.3088 (1.9); 7.3018 (1.9); 7.2983 (1.6); 7.2947 (1.4); 7.2928 (1.6); 7.2885 (1.0); 7.2848 (1.4); 7.0949 (0.8); 7.0904 (0.8); 6.9767 (0.6); 6.9713 (0.9); 6.9654 (0.6); 6.9511 (0.6); 6.9458 (1.0); 6.9399 (0.6); 6.9103 (0.9); 6.9083 (1.0); 6.9055 (0.9); 6.9034 (0.8); 6.8902 (0.8); 6.8881 (0.9); 6.8852 (0.8); 6.8831 (0.7); 6.5494 (2.3); 6.5093 (2.1); 4.7574 (4.4); 3.5677 (3.8); 3.3165 (0.8); 3.2439 (0.6); 2.5232 (1.4); 2.5185 (2.0); 2.5098 (25.7); 2.5053 (54.0); 2.5007 (74.1); 2.4961 (53.5); 2.4916 (25.8); 2.4766 (2.5); 2.4565 (1.8); 1.4641 (1.6); 1.4454 (2.7); 1.4266 (2.8); 1.4080 (1.7); 1.2353 (0.9); 0.8610 (7.7); 0.8427 (16.0); 0.8242 (6.9); −0.0002 (8.7) II-08: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): δ = 7.6397 (1.8); 7.6343 (1.6); 7.6203 (2.3); 7.6159 (2.0); 7.4867 (2.0); 7.4678 (1.0); 7.4610 (4.1); 7.4519 (5.4); 7.4448 (7.4); 7.4351 (1.0); 7.4203 (0.6); 7.4112 (0.7); 7.4066 (0.6); 7.3979 (2.4); 7.3879 (1.8); 7.3823 (3.8); 7.3797 (3.7); 7.3697 (0.9); 7.3657 (0.7); 7.3378 (0.9); 7.3214 (1.2); 7.3171 (1.9); 7.3082 (0.6); 7.3008 (2.9); 7.2985 (3.6); 7.2927 (2.0); 7.2895 (3.0); 7.2856 (2.1); 7.2807 (3.4); 7.2744 (2.6); 7.0896 (0.7); 7.0876 (0.8); 7.0832 (0.8); 7.0812 (0.8); 7.0682 (1.2); 7.0662 (1.3); 7.0618 (1.3); 7.0599 (1.3); 7.0471 (0.6); 7.0450 (0.7); 7.0406 (0.6); 7.0386 (0.6); 6.9515 (1.0); 6.9460 (1.5); 6.9403 (1.0); 6.9257 (1.0); 6.9204 (1.6); 6.9145 (1.1); 6.8868 (1.5); 6.8847 (1.7); 6.8818 (1.4); 6.8798 (1.3); 6.8665 (1.4); 6.8644 (1.4); 6.8615 (1.4); 6.8594 (1.2); 6.5233 (3.3); 6.4833 (3.1); 4.4480 (8.9); 2.8181 (1.9); 2.8000 (5.9); 2.7819 (6.0); 2.7638 (2.0); 2.6701 (0.5); 2.5235 (1.3); 2.5189 (2.0); 2.5101 (30.5); 2.5056 (65.0); 2.5010 (89.4); 2.4964 (63.7); 2.4919 (30.1); 2.4388 (32.4); 2.3279 (0.6); 1.2344 (1.0); 1.1270 (7.5); 1.1089 (16.0); 1.0908 (7.2); −0.0002 (11.7) II-09: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): δ = 7.4605 (1.5); 7.4514 (1.8); 7.4443 (2.2); 7.3167 (0.7); 7.3005 (1.0); 7.2975 (1.3); 7.2886 (1.1); 7.2848 (0.7); 7.2800 (1.2); 7.2736 (0.8); 6.9426 (0.5); 6.9170 (0.5); 6.8864 (0.6); 6.8843 (0.6); 6.8815 (0.5); 6.8662 (0.5); 4.4522 (1.4); 3.3124 (3.9); 2.5228 (1.5); 2.5181 (2.1); 2.5093 (26.2); 2.5048 (54.8); 2.5002 (74.9); 2.4957 (53.0); 2.4911 (24.7); 1.2204 (16.0); −0.0002 (11.8) II-10: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): δ = 7.4582 (1.7); 7.4495 (2.0); 7.4421 (2.4); 7.4003 (0.6); 7.3293 (0.6); 7.3110 (1.7); 7.2918 (2.4); 7.2820 (0.9); 7.2751 (1.1); 7.2711 (1.0); 7.2387 (1.7); 7.2264 (1.0); 7.2196 (1.0); 7.0634 (0.5); 7.0589 (0.5); 6.9355 (0.6); 6.9103 (0.6); 6.8877 (0.7); 6.8672 (0.6); 4.4795 (1.5); 3.3118 (16.0); 2.9714 (0.6); 2.9534 (1.2); 2.9470 (0.7); 2.9322 (1.1); 2.8076 (1.0); 2.7866 (1.1); 2.7687 (0.6); 2.6740 (0.8); 2.6694 (1.1); 2.6648 (0.9); 2.5229 (3.4); 2.5181 (4.9); 2.5094 (65.6); 2.5049 (138.2); 2.5003 (189.2); 2.4958 (135.0); 2.4913 (63.8); 2.4507 (1.1); 2.4457 (0.7); 2.3317 (0.8); 2.3271 (1.1); 2.3225 (0.8); 0.0079 (0.6); −0.0002 (20.9); −0.0085 (0.8) II-11: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): δ = 7.4678 (1.1); 7.4612 (4.0); 7.4522 (5.1); 7.4450 (6.2); 7.4353 (1.1); 7.3381 (0.8); 7.3217 (0.9); 7.3175 (1.7); 7.3076 (0.6); 7.3010 (2.6); 7.2977 (3.6); 7.2920 (1.9); 7.2892 (2.9); 7.2850 (2.2); 7.2805 (3.5); 7.2739 (2.6); 7.0904 (0.6); 7.0884 (0.7); 7.0838 (0.7); 7.0820 (0.8); 7.0688 (1.1); 7.0670 (1.2); 7.0624 (1.3); 7.0608 (1.3); 7.0478 (0.6); 7.0458 (0.7); 7.0413 (0.7); 7.0394 (0.6); 6.9539 (0.9); 6.9484 (1.5); 6.9427 (1.0); 6.9281 (1.0); 6.9227 (1.5); 6.9169 (1.1); 6.8870 (1.4); 6.8849 (1.6); 6.8821 (1.4); 6.8800 (1.4); 6.8667 (1.3); 6.8647 (1.4); 6.8618 (1.4); 6.8597 (1.3); 5.7530 (16.0); 4.4682 (8.4); 2.9324 (2.6); 2.9191 (3.8); 2.9050 (3.1); 2.5188 (0.7); 2.5101 (11.8); 2.5055 (26.3); 2.5009 (37.8); 2.4964 (28.5); 2.4918 (15.1); 1.6250 (0.6); 1.5973 (3.0); 1.5847 (2.5); 1.5700 (1.3); 1.5030 (1.4); 1.4914 (1.5); −0.0002 (8.6) II-12: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): δ = 7.4608 (6.4); 7.4524 (7.3); 7.4485 (4.8); 7.4447 (8.3); 7.3453 (1.1); 7.3289 (1.3); 7.3246 (2.4); 7.3082 (2.8); 7.3024 (4.6); 7.2986 (2.7); 7.2945 (3.7); 7.2923 (3.4); 7.2885 (3.7); 7.2855 (3.7); 7.2783 (3.3); 7.0970 (1.0); 7.0907 (1.0); 7.0758 (1.8); 7.0698 (1.8); 7.0544 (0.9); 7.0501 (0.8); 6.9567 (1.3); 6.9512 (2.1); 6.9455 (1.4); 6.9309 (1.3); 6.9258 (2.1); 6.9198 (1.4); 6.8999 (2.1); 6.8979 (2.3); 6.8950 (1.9); 6.8796 (1.9); 6.8776 (2.0); 6.8748 (1.9); 6.8726 (1.7); 4.5654 (4.1); 3.5675 (4.6); 3.3120 (16.0); 3.1682 (0.6); 2.7559 (1.9); 2.7373 (2.2); 2.7180 (2.0); 2.6740 (1.4); 2.6694 (2.0); 2.6647 (1.4); 2.5988 (0.8); 2.5228 (5.9); 2.5181 (8.6); 2.5094 (116.8); 2.5049 (246.0); 2.5003 (336.5); 2.4957 (238.9); 2.4912 (112.9); 2.4397 (0.6); 2.4123 (0.5); 2.3317 (1.4); 2.3270 (2.0); 2.3225 (1.5); 1.5031 (1.1); 1.4842 (0.8); 1.2483 (9.4); 0.8748 (1.9); 0.8580 (6.5); 0.8404 (2.3); 0.0080 (1.9); −0.0002 (58.5); −0.0085 (2.3) II-13: .sup.1H-NMR(400.0 MHz, d.sub.6-DMSO): δ = 7.4584 (8.7); 7.4500 (10.1); 7.4461 (6.9); 7.4423 (11.6); 7.4389 (4.9); 7.4341 (4.5); 7.4302 (5.0); 7.4133 (7.0); 7.3981 (1.0); 7.3930 (0.9); 7.3769 (2.5); 7.3729 (3.4); 7.3682 (1.5); 7.3558 (8.0); 7.3517 (3.4); 7.3407 (2.5); 7.3373 (4.7); 7.3260 (2.4); 7.3221 (4.0); 7.3184 (4.0); 7.3141 (4.1); 7.3047 (4.2); 7.2969 (8.7); 7.2933 (6.1); 7.2891 (6.0); 7.2868 (5.7); 7.2834 (4.8); 7.2798 (5.4); 7.2769 (5.3); 7.2728 (4.9); 7.0902 (1.3); 7.0882 (1.5); 7.0838 (1.5); 7.0819 (1.5); 7.0687 (2.3); 7.0668 (2.5); 7.0624 (2.5); 7.0476 (1.2); 7.0455 (1.3); 7.0411 (1.3); 7.0392 (1.2); 6.9493 (1.8); 6.9438 (2.9); 6.9381 (2.0); 6.9235 (1.9); 6.9183 (3.1); 6.9124 (2.1); 6.8967 (3.0); 6.8947 (3.4); 6.8918 (2.7); 6.8897 (2.5); 6.8764 (2.7); 6.8744 (2.9); 6.8716 (2.7); 6.8695 (2.4); 5.7530 (16.0); 4.5278 (14.7); 3.9323 (14.6); 2.5231 (0.9); 2.5184 (1.4); 2.5096 (30.8); 2.5051 (67.2); 2.5005 (93.6); 2.4960 (68.4); 2.4914 (33.5); 2.4359 (0.5); 2.3319 (0.6); 2.3274 (0.7); 2.3227 (0.6); −0.0002 (12.0); −0.0085 (0.5) II-14: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4021 (0.6); 7.3954 (3.7); 7.3906 (3.8); 7.3829 (2.3); 7.3779 (2.3); 7.3706 (0.6); 7.3669 (0.8); 7.2821 (2.2); 7.2775 (2.5); 7.2692 (1.7); 7.2618 (22.2); 7.2581 (2.4); 7.1197 (0.5); 7.1039 (0.6); 7.0991 (1.2); 7.0833 (1.2); 7.0786 (0.8); 7.0628 (0.7); 6.9710 (0.6); 6.9654 (1.0); 6.9598 (0.7); 6.9454 (0.6); 6.9399 (1.0); 6.9342 (0.7); 6.8362 (0.6); 6.8298 (0.6); 6.8209 (1.3); 6.8170 (1.9); 6.8110 (1.1); 6.8091 (0.8); 6.7998 (1.0); 6.7966 (1.3); 6.7904 (0.5); 5.2979 (11.6); 4.8230 (7.5); 3.0865 (2.1); 3.0682 (7.0); 3.0499 (7.2); 3.0316 (2.2); 1.2574 (7.5); 1.2392 (16.0); 1.2208 (7.2); −0.0002 (8.9) III-001: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3870 (1.0); 7.3827 (1.2); 7.3678 (2.0); 7.3637 (2.3); 7.3531 (1.1); 7.3493 (2.3); 7.3393 (5.0); 7.3364 (5.7); 7.3310 (2.8); 7.3211 (5.4); 7.3074 (2.5); 7.3004 (1.8); 7.2887 (1.7); 7.2830 (5.2); 7.2787 (4.7); 7.2741 (2.2); 7.2686 (1.5); 7.2592 (20.6); 7.1839 (1.4); 7.1649 (2.1); 7.1462 (0.9); 7.0343 (1.3); 7.0312 (1.2); 7.0135 (1.3); 7.0098 (2.1); 7.0061 (1.3); 6.9885 (1.1); 6.9854 (1.0); 6.7256 (0.7); 5.2952 (11.6); 4.8957 (3.1); 4.8718 (16.0); 4.8652 (3.6); 4.8618 (2.6); 3.9428 (3.6); 3.9276 (3.5); 1.7660 (11.9); 1.5854 (0.8); 1.2557 (0.8); −0.0002 (6.8) III-002: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3748 (0.7); 7.3705 (0.9); 7.3555 (1.5); 7.3517 (2.1); 7.3375 (4.2); 7.3356 (4.7); 7.3327 (3.0); 7.3301 (2.3); 7.3236 (1.9); 7.3197 (3.8); 7.3176 (3.4); 7.3089 (1.2); 7.3057 (1.7); 7.3005 (1.2); 7.2967 (1.1); 7.2881 (0.8); 7.2838 (1.1); 7.2774 (3.6); 7.2732 (3.6); 7.2688 (1.7); 7.2604 (15.8); 7.2530 (1.7); 7.1828 (0.9); 7.1812 (1.0); 7.1620 (1.4); 7.1442 (0.6); 7.1427 (0.6); 7.0377 (0.9); 7.0345 (0.9); 7.0169 (0.9); 7.0130 (1.5); 7.0094 (1.0); 6.9918 (0.8); 6.9886 (0.8); 6.6878 (0.6); 5.2956 (16.0); 4.8041 (11.3); 2.8234 (0.7); 2.8141 (1.0); 2.8055 (1.0); 2.7962 (0.8); 2.0419 (0.6); 1.6016 (0.5); 1.2572 (0.9); 0.8631 (0.8); 0.8491 (1.8); 0.8454 (2.8); 0.8426 (1.3); 0.8317 (2.6); 0.8276 (2.1); 0.8247 (1.2); 0.8143 (0.9); 0.6284 (0.9); 0.6184 (1.8); 0.6153 (2.0); 0.6113 (2.0); 0.6099 (2.0); 0.6057 (2.0); 0.6020 (1.8); 0.5883 (0.7); −0.0002 (5.3) III-003: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3866 (1.2); 7.3823 (1.4); 7.3742 (0.6); 7.3672 (2.2); 7.3630 (2.5); 7.3541 (1.4); 7.3504 (1.8); 7.3486 (1.9); 7.3423 (4.0); 7.3400 (5.4); 7.3372 (6.3); 7.3317 (3.3); 7.3296 (1.8); 7.3259 (2.7); 7.3219 (5.7); 7.3196 (5.1); 7.3141 (1.4); 7.3121 (1.5); 7.3103 (1.8); 7.3082 (2.8); 7.3064 (2.0); 7.3021 (1.8); 7.2989 (1.5); 7.2898 (2.0); 7.2836 (5.7); 7.2793 (5.3); 7.2747 (2.4); 7.2694 (1.6); 7.2663 (2.4); 7.2592 (37.8); 7.1877 (1.2); 7.1860 (1.4); 7.1844 (1.4); 7.1650 (2.0); 7.1491 (0.8); 7.1474 (0.9); 7.1458 (0.9); 7.1444 (0.8); 7.0377 (1.4); 7.0345 (1.3); 7.0169 (1.4); 7.0131 (2.2); 7.0094 (1.4); 6.9919 (1.2); 6.9887 (1.1); 6.7103 (0.6); 5.9472 (0.6); 5.9336 (1.3); 5.9213 (0.8); 5.9078 (1.4); 5.9043 (0.8); 5.8941 (0.8); 5.8906 (1.5); 5.8783 (0.9); 5.8772 (0.9); 5.8649 (1.5); 5.8512 (0.7); 5.2963 (9.6); 5.2791 (0.9); 5.2749 (2.1); 5.2717 (2.2); 5.2674 (1.1); 5.2362 (0.8); 5.2320 (1.8); 5.2287 (1.9); 5.2245 (1.0); 5.1885 (1.1); 5.1849 (2.5); 5.1816 (2.4); 5.1780 (1.0); 5.1628 (1.0); 5.1592 (2.3); 5.1558 (2.2); 5.1522 (0.9); 4.8601 (16.0); 4.0348 (1.4); 4.0309 (2.4); 4.0269 (1.6); 4.0202 (2.5); 4.0167 (4.0); 4.0131 (2.4); 4.0065 (1.4); 4.0025 (2.2); 3.9986 (1.2); 1.5654 (5.0); 0.0079 (0.6); −0.0002 (18.2); −0.0085 (0.7) III-004: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3122 (0.9); 7.3081 (1.2); 7.3068 (1.4); 7.3024 (0.9); 7.2981 (0.7); 7.2956 (0.8); 7.2920 (3.2); 7.2905 (4.9); 7.2866 (5.4); 7.2843 (3.0); 7.2810 (1.9); 7.2758 (2.8); 7.2719 (7.8); 7.2700 (5.6); 7.2667 (3.3); 7.2641 (6.6); 7.2625 (5.7); 7.2596 (38.6); 7.2510 (4.7); 7.2464 (2.1); 7.2449 (2.1); 7.2270 (0.6); 7.1570 (4.2); 7.1529 (5.2); 7.1472 (1.4); 7.1406 (2.2); 7.1379 (1.7); 7.1360 (4.2); 7.1326 (3.4); 7.0974 (0.5); 7.0902 (4.5); 7.0847 (1.3); 7.0761 (0.7); 7.0733 (1.4); 7.0688 (6.3); 7.0635 (1.4); 7.0608 (0.6); 7.0521 (1.2); 7.0466 (3.5); 6.6980 (0.6); 5.9491 (0.6); 5.9354 (1.3); 5.9232 (0.8); 5.9219 (0.8); 5.9096 (1.5); 5.9062 (0.8); 5.8960 (0.8); 5.8925 (1.6); 5.8803 (0.9); 5.8789 (0.9); 5.8667 (1.6); 5.8531 (0.8); 5.2970 (7.6); 5.2791 (0.9); 5.2748 (2.1); 5.2716 (2.2); 5.2673 (1.0); 5.2361 (0.8); 5.2318 (1.9); 5.2286 (1.9); 5.2243 (0.9); 5.1882 (1.0); 5.1846 (2.5); 5.1812 (2.4); 5.1776 (0.9); 5.1625 (0.9); 5.1589 (2.3); 5.1555 (2.2); 5.1519 (0.9); 4.8824 (16.0); 4.0374 (1.2); 4.0334 (2.1); 4.0295 (1.4); 4.0228 (2.2); 4.0192 (3.7); 4.0155 (2.2); 4.0089 (1.3); 4.0049 (2.1); 4.0009 (1.2); −0.0002 (16.4) III-005: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3116 (0.6); 7.3075 (0.8); 7.3062 (1.0); 7.3018 (0.6); 7.2977 (0.6); 7.2950 (0.6); 7.2909 (4.3); 7.2899 (4.4); 7.2859 (2.1); 7.2837 (1.8); 7.2778 (3.0); 7.2750 (2.3); 7.2713 (4.7); 7.2690 (4.8); 7.2654 (1.8); 7.2635 (1.6); 7.2603 (20.1); 7.2570 (3.0); 7.2555 (3.4); 7.2508 (0.8); 7.2483 (0.5); 7.2449 (1.3); 7.2436 (1.3); 7.1614 (2.9); 7.1574 (3.6); 7.1516 (1.0); 7.1449 (1.5); 7.1422 (1.1); 7.1403 (2.9); 7.1370 (2.2); 7.0926 (3.1); 7.0871 (0.9); 7.0783 (0.5); 7.0757 (1.0); 7.0711 (4.3); 7.0658 (0.9); 7.0544 (0.9); 7.0490 (2.4); 5.2965 (16.0); 4.8572 (10.2); 3.2647 (2.2); 3.2505 (2.5); 3.2471 (2.5); 3.2328 (2.2); 1.0479 (0.5); 1.0280 (0.9); 1.0080 (0.6); 0.5572 (0.8); 0.5454 (1.9); 0.5423 (2.4); 0.5400 (1.3); 0.5372 (1.0); 0.5309 (1.1); 0.5252 (2.3); 0.5222 (1.9); 0.5109 (0.9); 0.2743 (0.9); 0.2628 (2.6); 0.2604 (2.2); 0.2508 (1.9); 0.2480 (2.6); 0.2363 (0.6); −0.0002 (8.0) III-006: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3125 (0.6); 7.3084 (0.8); 7.3069 (0.9); 7.3025 (0.6); 7.2958 (0.7); 7.2907 (3.2); 7.2885 (3.0); 7.2842 (1.8); 7.2754 (3.4); 7.2722 (4.7); 7.2704 (3.6); 7.2661 (3.8); 7.2636 (3.3); 7.2596 (29.3); 7.2530 (3.3); 7.2476 (1.3); 7.2459 (1.4); 7.1591 (2.8); 7.1549 (3.2); 7.1492 (0.9); 7.1427 (1.4); 7.1399 (1.1); 7.1381 (2.7); 7.1347 (2.2); 7.0918 (2.9); 7.0863 (0.9); 7.0749 (0.9); 7.0704 (4.0); 7.0651 (1.0); 7.0537 (0.8); 7.0483 (2.3); 5.2972 (16.0); 4.8798 (10.2); 4.1930 (2.8); 4.1866 (2.9); 4.1793 (2.8); 4.1729 (2.8); 2.2746 (2.3); 2.2682 (4.9); 2.2618 (2.2); −0.0002 (11.6) III-007: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3056 (0.5); 7.3041 (0.6); 7.2895 (1.4); 7.2879 (2.2); 7.2848 (2.2); 7.2816 (1.2); 7.2794 (0.9); 7.2717 (2.2); 7.2694 (3.2); 7.2676 (2.5); 7.2625 (3.1); 7.2599 (19.0); 7.2559 (1.7); 7.2495 (2.3); 7.2440 (0.9); 7.2424 (1.0); 7.1546 (1.9); 7.1505 (2.3); 7.1449 (0.6); 7.1382 (1.0); 7.1355 (0.7); 7.1336 (1.9); 7.1302 (1.5); 7.0905 (2.0); 7.0849 (0.6); 7.0735 (0.6); 7.0690 (2.8); 7.0637 (0.6); 7.0523 (0.6); 7.0469 (1.6); 5.2970 (3.7); 4.8574 (7.0); 3.2283 (1.7); 3.2118 (2.5); 3.1960 (1.7); 1.8661 (0.7); 1.8493 (0.9); 1.8325 (0.8); 1.5713 (2.6); 0.9560 (16.0); 0.9513 (1.2); 0.9392 (15.4); 0.9343 (0.8); −0.0002 (7.5) III-008: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5185 (0.7); 7.3843 (0.9); 7.3692 (1.1); 7.3636 (1.6); 7.3490 (1.9); 7.3444 (1.3); 7.3293 (1.4); 7.2596 (116.5); 7.1371 (3.4); 7.1314 (1.9); 7.1252 (4.3); 7.1198 (2.5); 7.1142 (5.1); 7.1114 (2.3); 7.1084 (3.2); 7.1023 (6.2); 7.0939 (0.7); 7.0901 (1.0); 7.0877 (1.0); 7.0837 (1.0); 7.0812 (0.9); 7.0364 (1.9); 7.0326 (2.7); 7.0301 (2.2); 7.0139 (4.1); 7.0111 (3.2); 7.0077 (2.2); 6.9994 (4.9); 6.9955 (1.5); 6.9935 (1.8); 6.9905 (2.0); 6.9872 (2.1); 6.9792 (6.0); 6.9766 (4.1); 6.9734 (1.7); 6.9620 (1.3); 6.9563 (3.4); 6.6799 (0.7); 5.9590 (0.6); 5.9454 (1.4); 5.9330 (1.0); 5.9196 (1.5); 5.9161 (0.8); 5.9060 (0.8); 5.9024 (1.6); 5.8891 (1.0); 5.8767 (1.6); 5.8630 (0.8); 5.2906 (1.0); 5.2863 (2.2); 5.2831 (2.2); 5.2788 (1.0); 5.2476 (0.9); 5.2433 (2.0); 5.2402 (2.0); 5.2358 (0.9); 5.1969 (1.1); 5.1933 (2.5); 5.1899 (2.3); 5.1864 (1.0); 5.1711 (1.0); 5.1675 (2.3); 5.1642 (2.2); 5.1605 (0.9); 4.8613 (16.0); 4.0433 (1.3); 4.0393 (2.2); 4.0352 (1.4); 4.0251 (4.0); 4.0150 (1.5); 4.0109 (2.2); 1.5454 (4.1); 0.0080 (1.5); −0.0002 (43.8); −0.0085 (1.6) III-009: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5187 (0.5); 7.3846 (0.8); 7.3698 (1.2); 7.3640 (1.6); 7.3496 (1.8); 7.3447 (1.3); 7.3297 (1.3); 7.2599 (86.0); 7.1351 (3.4); 7.1299 (1.9); 7.1234 (4.3); 7.1179 (2.4); 7.1122 (5.8); 7.1091 (2.3); 7.1060 (2.8); 7.1005 (4.9); 7.0907 (0.9); 7.0881 (0.8); 7.0841 (0.8); 7.0817 (0.8); 7.0356 (1.7); 7.0318 (2.6); 7.0293 (2.1); 7.0131 (4.3); 7.0103 (3.1); 6.9975 (4.8); 6.9914 (2.7); 6.9856 (2.0); 6.9804 (2.5); 6.9773 (5.3); 6.9716 (1.6); 6.9602 (1.1); 6.9546 (3.2); 6.5958 (0.7); 5.2982 (0.6); 4.8225 (15.7); 3.4107 (1.8); 3.3931 (3.7); 3.3781 (3.6); 3.3605 (1.8); 1.6093 (0.8); 1.5909 (2.0); 1.5849 (0.9); 1.5727 (3.1); 1.5669 (1.8); 1.5505 (5.6); 1.5363 (1.3); 1.4439 (0.7); 1.4257 (2.0); 1.4066 (2.6); 1.3872 (2.6); 1.3692 (1.6); 1.3509 (0.6); 0.9602 (7.7); 0.9419 (16.0); 0.9236 (6.5); 0.0080 (1.0); −0.0002 (31.8); −0.0085 (1.0) III-010: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3737 (1.0); 7.3586 (1.5); 7.3533 (1.9); 7.3383 (2.7); 7.3337 (2.2); 7.3271 (4.7); 7.3239 (7.9); 7.3224 (6.9); 7.3176 (7.5); 7.3134 (5.0); 7.3114 (7.1); 7.3094 (6.9); 7.3030 (2.0); 7.2969 (1.9); 7.2930 (3.3); 7.2902 (2.5); 7.2865 (2.4); 7.2828 (1.6); 7.2781 (1.1); 7.2747 (1.4); 7.2713 (1.7); 7.2583 (44.3); 7.1235 (1.1); 7.1213 (1.3); 7.1169 (1.4); 7.1137 (3.9); 7.1078 (1.6); 7.1018 (4.8); 7.0962 (4.0); 7.0934 (3.0); 7.0907 (5.2); 7.0847 (1.9); 7.0788 (5.5); 7.0749 (1.4); 7.0724 (1.2); 7.0168 (2.0); 7.0130 (2.7); 7.0105 (2.3); 7.0035 (1.0); 6.9951 (7.2); 6.9913 (4.3); 6.9846 (2.2); 6.9816 (1.7); 6.9778 (2.1); 6.9749 (5.7); 6.9724 (4.3); 6.9690 (3.0); 6.9640 (2.1); 6.9624 (1.9); 6.9580 (2.4); 6.9521 (3.5); 6.9438 (0.6); 6.9008 (0.9); 5.2962 (6.9); 4.8965 (16.0); 4.5951 (6.8); 4.5802 (6.7); 1.5591 (3.8); 0.0079 (0.7); −0.0002 (17.1); −0.0085 (0.6) III-011: .sup.1H-NMR(400.0MHz, CDCl3): δ = 7.3826 (0.7); 7.3676 (1.1); 7.3620 (1.6); 7.3474 (1.7); 7.3420 (1.2); 7.3275 (1.3); 7.2605 (46.3); 7.1299 (3.6); 7.1245 (2.0); 7.1181 (3.3); 7.1127 (2.4); 7.1102 (2.2); 7.1073 (5.9); 7.1043 (2.1); 7.1013 (3.0); 7.0953 (4.4); 7.0891 (0.9); 7.0868 (1.2); 7.0827 (0.9); 7.0803 (0.8); 7.0312 (1.7); 7.0275 (2.5); 7.0249 (2.0); 7.0085 (4.0); 7.0059 (3.4); 7.0022 (1.9); 6.9979 (5.1); 6.9920 (1.5); 6.9859 (2.1); 6.9775 (5.5); 6.9720 (1.6); 6.9606 (1.1); 6.9548 (3.2); 6.6633 (0.8); 5.2982 (4.4); 4.8063 (16.0); 2.8459 (0.6); 2.8373 (1.0); 2.8280 (1.4); 2.8194 (1.4); 2.8101 (1.1); 2.8014 (0.6); 1.5620 (3.0); 1.4319 (0.5); 0.8758 (1.0); 0.8616 (2.6); 0.8583 (4.0); 0.8554 (1.9); 0.8445 (3.6); 0.8405 (3.0); 0.8375 (1.7); 0.8270 (1.3); 0.6308 (1.3); 0.6208 (2.6); 0.6176 (2.9); 0.6139 (2.8); 0.6119 (2.8); 0.6080 (2.9); 0.6044 (2.6); 0.5906 (0.9); 0.0079 (0.5); −0.0002 (18.7); −0.0085 (0.6) III-012: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3866 (0.9); 7.3850 (0.8); 7.3719 (1.3); 7.3681 (1.2); 7.3660 (1.7); 7.3515 (1.9); 7.3467 (1.4); 7.3317 (1.4); 7.2603 (53.4); 7.1415 (3.5); 7.1356 (1.8); 7.1344 (1.7); 7.1296 (4.2); 7.1245 (3.1); 7.1186 (5.0); 7.1128 (3.3); 7.1103 (3.1); 7.1068 (6.2); 7.0984 (0.9); 7.0919 (1.0); 7.0895 (1.0); 7.0854 (1.0); 7.0830 (1.0); 7.0406 (2.0); 7.0380 (2.5); 7.0369 (2.8); 7.0343 (2.3); 7.0180 (4.3); 7.0154 (3.4); 7.0129 (2.0); 7.0080 (1.5); 6.9994 (5.2); 6.9960 (2.5); 6.9935 (2.4); 6.9895 (2.0); 6.9856 (1.7); 6.9821 (2.1); 6.9792 (5.6); 6.9767 (4.3); 6.9734 (1.8); 6.9681 (0.7); 6.9621 (1.4); 6.9563 (3.5); 6.7201 (0.8); 5.2981 (2.3); 4.8349 (16.0); 4.8229 (0.6); 3.2716 (3.6); 3.2573 (4.2); 3.2540 (4.2); 3.2398 (3.7); 1.5602 (3.2); 1.0563 (0.8); 1.0542 (0.8); 1.0484 (0.8); 1.0443 (0.6); 1.0364 (1.5); 1.0284 (0.6); 1.0242 (0.8); 1.0184 (0.8); 1.0164 (1.0); 1.0043 (0.5); 0.5677 (1.3); 0.5559 (3.2); 0.5529 (3.8); 0.5506 (2.2); 0.5478 (1.7); 0.5414 (1.8); 0.5357 (3.7); 0.5328 (3.1); 0.5214 (1.6); 0.2840 (1.5); 0.2724 (4.2); 0.2701 (3.6); 0.2604 (3.4); 0.2577 (4.3); 0.2460 (1.1); 0.0080 (0.8); −0.0002 (21.5); −0.0085 (0.8) III-013: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3687 (0.6); 7.3631 (0.8); 7.3487 (0.9); 7.3433 (0.7); 7.3286 (0.7); 7.2601 (18.6); 7.1347 (1.6); 7.1293 (1.1); 7.1229 (2.1); 7.1176 (1.2); 7.1120 (2.6); 7.1080 (1.1); 7.1042 (1.3); 7.1004 (2.6); 7.0344 (0.8); 7.0309 (1.3); 7.0282 (1.0); 7.0117 (2.0); 7.0094 (1.6); 7.0051 (1.1); 7.0018 (0.6); 6.9966 (2.4); 6.9885 (1.0); 6.9845 (1.0); 6.9820 (0.9); 6.9764 (2.8); 6.9711 (0.8); 6.9595 (0.5); 6.9538 (1.6); 5.2975 (1.5); 4.8347 (8.3); 3.2365 (2.0); 3.2203 (3.3); 3.2044 (2.0); 1.8734 (0.8); 1.8566 (1.1); 1.8398 (0.9); 1.5647 (1.4); 0.9700 (16.0); 0.9532 (15.4); −0.0002 (7.2) III-014: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5184 (1.4); 7.3726 (0.6); 7.3626 (0.6); 7.3480 (0.7); 7.3418 (0.9); 7.3281 (1.1); 7.3226 (1.0); 7.3076 (1.0); 7.2868 (1.1); 7.2595 (250.5); 7.2092 (0.9); 7.1048 (1.2); 7.0983 (1.3); 7.0942 (1.2); 7.0832 (1.6); 7.0795 (1.4); 7.0770 (1.6); 7.0320 (1.0); 7.0127 (1.0); 6.9955 (2.0); 6.9731 (2.0); 6.9525 (2.0); 6.9303 (1.1); 5.2653 (0.6); 5.1635 (0.6); 5.0152 (2.3); 4.9941 (2.0); 4.0569 (0.8); 4.0424 (0.8); 3.9668 (0.7); 3.9543 (0.7); 3.0239 (3.7); 2.9833 (3.3); 1.5331 (16.0); 0.0080 (4.1); −0.0002 (102.1); −0.0085 (3.9) III-015: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3800 (1.3); 7.3652 (1.2); 7.3594 (2.4); 7.3447 (2.0); 7.3388 (1.7); 7.3250 (1.4); 7.2599 (47.4); 7.1604 (0.5); 7.1521 (3.4); 7.1463 (1.5); 7.1402 (3.7); 7.1347 (2.5); 7.1292 (5.3); 7.1233 (2.5); 7.1212 (2.3); 7.1173 (4.7); 7.1091 (2.2); 7.1066 (2.1); 7.1028 (1.9); 7.1002 (2.0); 7.0880 (1.0); 7.0855 (1.0); 7.0816 (1.1); 7.0791 (1.0); 7.0431 (1.8); 7.0393 (3.0); 7.0367 (2.6); 7.0325 (2.1); 7.0284 (2.3); 7.0262 (2.1); 7.0221 (3.5); 7.0203 (3.8); 7.0175 (1.9); 7.0118 (5.2); 7.0058 (2.8); 7.0029 (2.1); 6.9992 (1.8); 6.9946 (2.1); 6.9916 (5.5); 6.9890 (4.2); 6.9859 (1.8); 6.9805 (0.8); 6.9745 (1.4); 6.9687 (3.4); 6.6717 (0.7); 5.9486 (0.6); 5.9349 (1.3); 5.9227 (0.8); 5.9213 (0.8); 5.9091 (1.5); 5.9057 (0.8); 5.8954 (0.8); 5.8920 (1.6); 5.8798 (1.0); 5.8784 (0.9); 5.8662 (1.6); 5.8525 (0.8); 5.2975 (1.8); 5.2763 (1.0); 5.2720 (2.2); 5.2688 (2.3); 5.2645 (1.0); 5.2333 (0.9); 5.2291 (1.9); 5.2259 (2.0); 5.2216 (1.0); 5.1912 (1.1); 5.1876 (2.5); 5.1842 (2.4); 5.1807 (1.0); 5.1655 (1.0); 5.1618 (2.3); 5.1585 (2.3); 5.1549 (0.9); 4.8668 (16.0); 4.0373 (1.4); 4.0334 (2.4); 4.0294 (1.6); 4.0226 (2.6); 4.0191 (4.1); 4.0155 (2.5); 4.0088 (1.6); 4.0048 (2.3); 4.0009 (1.4); 1.5587 (2.9); 0.0079 (0.7); −0.0002 (19.0); −0.0085 (0.8) III-016: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3818 (1.1); 7.3668 (1.0); 7.3613 (2.2); 7.3464 (1.9); 7.3406 (1.5); 7.3267 (1.3); 7.2600 (35.0); 7.1544 (3.1); 7.1487 (1.2); 7.1425 (3.3); 7.1372 (2.1); 7.1317 (5.0); 7.1256 (2.3); 7.1233 (2.0); 7.1198 (4.4); 7.1111 (1.8); 7.1085 (1.7); 7.1046 (1.6); 7.1023 (1.8); 7.0900 (0.8); 7.0875 (0.8); 7.0835 (0.9); 7.0811 (0.8); 7.0453 (1.5); 7.0417 (2.7); 7.0391 (2.2); 7.0341 (1.6); 7.0300 (1.9); 7.0233 (3.6); 7.0201 (1.9); 7.0115 (5.3); 7.0058 (2.5); 7.0001 (1.6); 6.9944 (1.6); 6.9913 (5.0); 6.9858 (1.5); 6.9743 (1.1); 6.9687 (3.2); 6.7735 (0.7); 5.2975 (6.7); 4.9274 (0.8); 4.8645 (16.0); 4.1932 (4.3); 4.1868 (4.4); 4.1795 (4.3); 4.1731 (4.2); 3.8121 (1.4); 2.2781 (2.6); 2.2717 (5.4); 2.2652 (2.6); 1.5585 (2.7); −0.0002 (13.7) III-017: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3821 (0.8); 7.3672 (0.7); 7.3615 (1.5); 7.3470 (1.3); 7.3409 (1.1); 7.3272 (0.9); 7.2606 (19.7); 7.1540 (2.2); 7.1482 (0.9); 7.1421 (2.4); 7.1366 (1.6); 7.1311 (3.5); 7.1252 (1.7); 7.1230 (1.5); 7.1192 (3.1); 7.1108 (1.4); 7.1083 (1.3); 7.1044 (1.3); 7.1020 (1.3); 7.0898 (0.6); 7.0873 (0.6); 7.0833 (0.7); 7.0808 (0.6); 7.0460 (1.1); 7.0423 (2.0); 7.0397 (1.7); 7.0361 (1.4); 7.0321 (1.4); 7.0299 (1.2); 7.0260 (2.3); 7.0233 (2.0); 7.0204 (1.2); 7.0100 (3.6); 7.0067 (1.4); 7.0056 (1.5); 7.0044 (1.5); 6.9983 (0.8); 6.9927 (1.2); 6.9899 (3.6); 6.9874 (2.7); 6.9842 (1.2); 6.9728 (0.9); 6.9671 (2.3); 6.7110 (0.5); 5.2974 (16.0); 4.8486 (10.5); 4.1364 (0.8); 4.1303 (2.2); 4.1240 (2.6); 4.1171 (2.6); 4.1108 (2.2); 4.1047 (0.8); 3.8119 (0.8); 1.8344 (0.7); 1.8294 (6.1); 1.8233 (12.3); 1.8171 (6.0); 1.5722 (0.7); −0.0002 (7.9) III-018: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3783 (1.1); 7.3632 (1.0); 7.3578 (2.2); 7.3432 (1.8); 7.3372 (1.4); 7.3232 (1.2); 7.2604 (37.6); 7.1450 (3.0); 7.1394 (1.2); 7.1332 (3.2); 7.1277 (2.6); 7.1224 (5.1); 7.1162 (1.5); 7.1104 (4.4); 7.1057 (1.8); 7.1018 (1.9); 7.0994 (1.7); 7.0870 (0.7); 7.0846 (0.7); 7.0806 (0.8); 7.0782 (0.8); 7.0378 (1.4); 7.0342 (2.6); 7.0315 (2.2); 7.0277 (1.7); 7.0236 (1.8); 7.0215 (1.6); 7.0177 (3.3); 7.0152 (2.9); 7.0104 (4.8); 7.0043 (2.6); 6.9983 (2.0); 6.9933 (2.2); 6.9900 (4.9); 6.9879 (3.9); 6.9846 (1.5); 6.9731 (1.0); 6.9674 (3.0); 6.6448 (0.8); 5.2977 (5.6); 4.8113 (16.0); 2.8352 (0.6); 2.8265 (1.0); 2.8173 (1.4); 2.8086 (1.4); 2.7994 (1.1); 2.7907 (0.6); 1.5653 (4.7); 1.2577 (0.5); 0.8712 (1.0); 0.8570 (2.6); 0.8536 (3.8); 0.8508 (1.9); 0.8398 (3.6); 0.8358 (2.9); 0.8329 (1.7); 0.8224 (1.2); 0.6268 (1.3); 0.6167 (2.6); 0.6136 (2.9); 0.6098 (2.8); 0.6080 (2.8); 0.6040 (2.8); 0.6004 (2.6); 0.5865 (0.9); −0.0002 (14.7) III-019: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3766 (1.0); 7.3613 (1.0); 7.3559 (2.0); 7.3413 (1.8); 7.3354 (1.3); 7.3212 (1.2); 7.2607 (31.4); 7.1496 (2.8); 7.1442 (1.1); 7.1378 (3.0); 7.1325 (2.0); 7.1269 (4.7); 7.1203 (2.1); 7.1152 (4.5); 7.1054 (1.9); 7.1028 (2.0); 7.0987 (2.0); 7.0964 (2.2); 7.0842 (1.1); 7.0818 (1.2); 7.0777 (1.1); 7.0754 (1.1); 7.0426 (1.3); 7.0391 (2.5); 7.0366 (2.0); 7.0322 (1.5); 7.0280 (1.7); 7.0260 (1.5); 7.0204 (2.9); 7.0170 (1.6); 7.0080 (5.2); 7.0023 (2.4); 6.9978 (1.2); 6.9875 (4.4); 6.9856 (3.8); 6.9823 (1.4); 6.9707 (1.0); 6.9651 (2.9); 5.2977 (6.5); 4.8244 (15.2); 4.1832 (2.2); 4.1654 (6.8); 4.1475 (6.9); 4.1296 (2.3); 3.6791 (1.6); 3.6637 (4.0); 3.6484 (4.2); 3.6329 (1.6); 2.6151 (3.6); 2.6097 (0.7); 2.5997 (5.7); 2.5904 (0.6); 2.5846 (3.4); 1.5715 (2.5); 1.2793 (7.7); 1.2615 (16.0); 1.2436 (7.6); −0.0002 (12.3) III-020: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3711 (0.7); 7.3606 (7.3); 7.3572 (3.1); 7.3552 (4.0); 7.3524 (7.7); 7.3496 (4.2); 7.3469 (3.4); 7.3442 (7.9); 7.3401 (2.6); 7.3327 (4.3); 7.3273 (1.8); 7.3197 (4.2); 7.3153 (2.3); 7.3104 (4.8); 7.3030 (1.9); 7.2975 (4.5); 7.2900 (0.7); 7.2635 (33.4); 7.2140 (1.0); 7.2023 (4.3); 7.1993 (2.4); 7.1950 (3.0); 7.1921 (2.9); 7.1879 (3.0); 7.1859 (2.7); 7.1810 (1.9); 7.1779 (3.3); 7.1229 (0.5); 7.1156 (4.6); 7.1101 (1.4); 7.1018 (0.7); 7.0985 (1.5); 7.0943 (6.9); 7.0894 (1.6); 7.0778 (1.2); 7.0724 (3.7); 6.5837 (1.0); 5.9140 (0.6); 5.9003 (1.4); 5.8880 (0.9); 5.8746 (1.6); 5.8712 (0.9); 5.8608 (0.8); 5.8574 (1.7); 5.8450 (1.0); 5.8317 (1.7); 5.8180 (0.8); 5.3784 (1.1); 5.3615 (3.6); 5.3445 (3.6); 5.3275 (1.2); 5.2342 (1.0); 5.2301 (2.3); 5.2267 (2.6); 5.2226 (1.1); 5.1913 (0.9); 5.1872 (2.1); 5.1838 (2.2); 5.1797 (0.9); 5.1691 (1.0); 5.1656 (2.7); 5.1622 (2.6); 5.1588 (1.0); 5.1435 (1.0); 5.1399 (2.5); 5.1365 (2.5); 5.1331 (1.0); 3.9879 (1.5); 3.9840 (2.7); 3.9801 (1.7); 3.9734 (2.8); 3.9697 (4.8); 3.9660 (2.9); 3.9593 (1.7); 3.9554 (2.7); 3.9515 (1.6); 1.7097 (15.9); 1.6927 (16.0); 1.6645 (0.8); 1.6476 (0.8); 1.4323 (2.7); 0.9952 (0.5); 0.9913 (0.6); −0.0002 (14.3) III-021: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3629 (0.7); 7.3570 (3.0); 7.3543 (1.5); 7.3485 (3.3); 7.3439 (1.9); 7.3406 (3.8); 7.3363 (2.7); 7.3305 (1.2); 7.3231 (1.9); 7.3187 (1.2); 7.3137 (2.2); 7.3063 (1.0); 7.3009 (2.1); 7.2639 (20.6); 7.2003 (2.0); 7.1976 (1.1); 7.1917 (1.6); 7.1863 (1.3); 7.1832 (1.3); 7.1791 (0.9); 7.1759 (1.5); 7.1121 (2.0); 7.1067 (0.7); 7.0950 (0.8); 7.0908 (3.0); 7.0858 (0.9); 7.0742 (0.6); 7.0689 (1.7); 5.3017 (4.2); 5.2988 (1.8); 5.2816 (1.6); 3.6867 (16.0); 3.6294 (0.8); 3.6247 (1.2); 3.6099 (1.7); 3.5953 (1.3); 2.5996 (1.8); 2.5843 (3.2); 2.5689 (1.6); 1.6809 (6.5); 1.6730 (0.8); 1.6639 (6.4); 1.6561 (0.6); 1.4323 (1.4); −0.0002 (8.3) III-022: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3810 (1.2); 7.3662 (1.0); 7.3604 (2.3); 7.3457 (1.9); 7.3398 (1.6); 7.3261 (1.3); 7.2605 (37.7); 7.1610 (3.3); 7.1552 (1.2); 7.1491 (3.5); 7.1437 (2.2); 7.1381 (4.7); 7.1320 (1.5); 7.1262 (5.1); 7.1218 (1.1); 7.1191 (1.2); 7.1069 (1.5); 7.1044 (1.6); 7.1006 (1.6); 7.0981 (1.7); 7.0858 (0.7); 7.0834 (0.8); 7.0794 (0.8); 7.0769 (0.8); 7.0411 (1.6); 7.0374 (2.8); 7.0347 (2.4); 7.0306 (2.0); 7.0266 (2.2); 7.0243 (1.8); 7.0204 (7.5); 7.0148 (2.3); 7.0068 (1.8); 7.0031 (2.7); 7.0001 (6.3); 6.9974 (4.8); 6.9945 (1.7); 6.9830 (1.2); 6.9773 (3.3); 6.6686 (0.6); 5.9450 (0.6); 5.9312 (1.3); 5.9191 (0.8); 5.9176 (0.8); 5.9055 (1.5); 5.9021 (0.8); 5.8917 (0.8); 5.8883 (1.6); 5.8762 (0.9); 5.8746 (0.9); 5.8626 (1.6); 5.8488 (0.8); 5.2978 (10.2); 5.2728 (0.9); 5.2686 (2.1); 5.2653 (2.3); 5.2611 (1.0); 5.2299 (0.8); 5.2257 (1.9); 5.2224 (2.0); 5.2181 (0.9); 5.1903 (0.9); 5.1867 (2.5); 5.1833 (2.4); 5.1797 (0.9); 5.1645 (0.9); 5.1610 (2.3); 5.1576 (2.2); 5.1540 (0.8); 4.8669 (16.0); 4.0364 (1.2); 4.0324 (2.2); 4.0285 (1.4); 4.0218 (2.2); 4.0181 (3.8); 4.0144 (2.2); 4.0077 (1.3); 4.0038 (2.1); 3.9999 (1.2); 1.5879 (1.1); 1.4318 (0.9); −0.0002 (15.2) III-023: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3623 (0.7); 7.3475 (0.6); 7.2605 (10.0); 7.1634 (1.0); 7.1516 (1.0); 7.1462 (0.7); 7.1407 (1.4); 7.1289 (1.5); 7.1000 (0.5); 7.0396 (0.8); 7.0370 (0.7); 7.0320 (0.6); 7.0280 (0.7); 7.0204 (2.3); 7.0083 (0.7); 7.0000 (1.8); 6.9773 (1.0); 5.2980 (16.0); 4.8645 (5.0); 4.1933 (1.4); 4.1869 (1.4); 4.1796 (1.4); 4.1732 (1.3); 2.2780 (0.9); 2.2716 (1.9); 2.2652 (0.9); 1.5728 (0.5); −0.0002 (4.1) III-024: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3795 (0.5); 7.3589 (1.0); 7.3443 (0.8); 7.3383 (0.7); 7.3243 (0.6); 7.2610 (17.9); 7.1541 (1.4); 7.1485 (0.5); 7.1423 (1.5); 7.1369 (1.0); 7.1313 (2.1); 7.1250 (1.0); 7.1194 (2.2); 7.1060 (0.7); 7.1035 (0.7); 7.0996 (0.7); 7.0972 (0.7); 7.0358 (0.7); 7.0320 (1.2); 7.0294 (1.1); 7.0259 (0.9); 7.0215 (1.1); 7.0191 (2.6); 7.0157 (1.6); 7.0131 (1.8); 7.0018 (1.3); 6.9986 (2.7); 6.9963 (2.3); 6.9928 (1.0); 6.9760 (1.4); 5.2982 (16.0); 4.8113 (7.1); 2.8143 (0.6); 2.8058 (0.6); 1.5740 (1.3); 0.8564 (1.1); 0.8532 (1.7); 0.8502 (0.8); 0.8393 (1.6); 0.8353 (1.3); 0.8323 (0.7); 0.8218 (0.6); 0.6289 (0.6); 0.6189 (1.2); 0.6158 (1.3); 0.6120 (1.2); 0.6100 (1.2); 0.6061 (1.3); 0.6026 (1.1); −0.0002 (7.2) III-025: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3833 (1.2); 7.3685 (1.0); 7.3628 (2.3); 7.3482 (1.9); 7.3422 (1.6); 7.3283 (1.3); 7.2608 (36.5); 7.1653 (3.3); 7.1596 (1.2); 7.1534 (3.5); 7.1480 (2.2); 7.1425 (4.7); 7.1364 (1.5); 7.1306 (5.0); 7.1275 (1.3); 7.1234 (1.2); 7.1212 (1.2); 7.1087 (1.5); 7.1062 (1.7); 7.1023 (1.6); 7.0998 (1.8); 7.0876 (0.8); 7.0851 (0.8); 7.0811 (0.8); 7.0787 (0.8); 7.0451 (1.5); 7.0413 (2.8); 7.0387 (2.4); 7.0357 (2.0); 7.0317 (2.0); 7.0293 (2.0); 7.0254 (3.5); 7.0202 (5.9); 7.0141 (1.8); 7.0120 (2.0); 7.0083 (1.9); 7.0057 (1.8); 6.9999 (5.5); 6.9975 (4.2); 6.9943 (1.6); 6.9829 (1.2); 6.9772 (3.3); 6.6928 (0.7); 5.2979 (16.0); 4.8422 (15.8); 3.2639 (3.5); 3.2495 (4.0); 3.2463 (4.0); 3.2320 (3.5); 1.5787 (2.7); 1.0458 (0.8); 1.0438 (0.8); 1.0380 (0.7); 1.0339 (0.5); 1.0259 (1.4); 1.0180 (0.6); 1.0137 (0.7); 1.0080 (0.8); 1.0060 (0.9); 0.5591 (1.2); 0.5473 (3.0); 0.5442 (3.6); 0.5420 (2.0); 0.5392 (1.6); 0.5328 (1.6); 0.5272 (3.4); 0.5242 (2.9); 0.5128 (1.4); 0.2732 (1.4); 0.2616 (4.0); 0.2496 (3.1); 0.2468 (4.1); 0.2349 (1.0); 0.0701 (0.8); −0.0002 (14.8) III-026: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3791 (0.6); 7.3642 (0.5); 7.3586 (1.1); 7.3438 (1.0); 7.3379 (0.8); 7.3241 (0.6); 7.2614 (16.9); 7.1596 (1.6); 7.1539 (0.7); 7.1477 (1.8); 7.1423 (1.2); 7.1367 (2.3); 7.1306 (0.9); 7.1250 (2.6); 7.1191 (0.8); 7.1166 (1.0); 7.1043 (1.1); 7.1018 (1.2); 7.0979 (1.2); 7.0955 (1.3); 7.0832 (0.7); 7.0808 (0.7); 7.0768 (0.7); 7.0744 (0.6); 7.0429 (0.8); 7.0392 (1.4); 7.0366 (1.2); 7.0323 (1.0); 7.0282 (1.1); 7.0261 (1.2); 7.0179 (2.9); 7.0120 (0.9); 7.0083 (1.0); 7.0053 (1.0); 7.0010 (1.3); 6.9977 (3.1); 6.9920 (0.9); 6.9806 (0.7); 6.9749 (1.6); 5.2983 (4.1); 4.8241 (8.1); 3.6958 (16.0); 3.6787 (1.0); 3.6633 (2.3); 3.6480 (2.3); 3.6325 (1.0); 2.6318 (1.9); 2.6164 (2.9); 2.6012 (1.8); 1.5819 (2.0); −0.0002 (6.8) III-027: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3797 (0.6); 7.3649 (0.6); 7.3592 (1.1); 7.3444 (0.9); 7.3383 (0.6); 7.3246 (0.6); 7.2609 (19.2); 7.1705 (1.7); 7.1649 (0.6); 7.1587 (1.8); 7.1533 (1.1); 7.1477 (2.3); 7.1416 (0.8); 7.1359 (2.2); 7.1256 (0.6); 7.1230 (0.6); 7.1191 (0.6); 7.1166 (0.7); 7.1044 (1.1); 7.1017 (1.2); 7.0983 (1.0); 7.0955 (1.2); 7.0833 (0.6); 7.0808 (0.5); 7.0768 (0.5); 7.0469 (0.8); 7.0431 (1.3); 7.0405 (1.1); 7.0333 (0.8); 7.0291 (1.3); 7.0270 (1.6); 7.0235 (2.4); 7.0200 (2.6); 7.0141 (0.8); 7.0091 (1.0); 7.0028 (1.4); 6.9996 (3.0); 6.9940 (0.8); 6.9826 (0.6); 6.9769 (1.6); 5.2981 (4.6); 4.8950 (7.8); 4.1775 (3.6); 4.1639 (3.6); 3.7892 (16.0); 1.5695 (2.2); −0.0002 (7.7) III-028: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5194 (0.7); 7.5156 (0.9); 7.5127 (1.1); 7.5093 (0.7); 7.5007 (0.8); 7.4942 (2.9); 7.4881 (1.0); 7.4791 (1.5); 7.4756 (2.8); 7.4721 (1.5); 7.4514 (0.7); 7.4461 (3.2); 7.4427 (1.7); 7.4310 (2.9); 7.4272 (5.7); 7.4227 (1.6); 7.4137 (1.1); 7.4093 (3.0); 7.4061 (1.8); 7.3639 (0.7); 7.3593 (0.7); 7.3463 (0.7); 7.3412 (0.6); 7.3308 (0.9); 7.3257 (4.6); 7.3226 (5.6); 7.3189 (2.7); 7.3104 (1.4); 7.3053 (5.0); 7.3015 (3.4); 7.2606 (65.6); 7.2496 (1.7); 7.2484 (1.7); 7.2438 (3.0); 7.2287 (2.4); 7.2234 (1.9); 7.2092 (1.2); 7.2077 (1.2); 7.0346 (1.1); 7.0324 (1.3); 7.0283 (1.5); 7.0261 (1.5); 7.0138 (2.4); 7.0115 (2.7); 7.0074 (2.6); 7.0056 (2.7); 6.9966 (1.1); 6.9932 (1.2); 6.9910 (1.2); 6.9870 (1.2); 6.9847 (1.1); 6.9403 (1.4); 6.9350 (2.2); 6.9293 (1.5); 6.9168 (1.2); 6.9117 (2.0); 6.9072 (3.6); 6.9052 (3.7); 6.9023 (1.6); 6.8998 (1.4); 6.8869 (1.7); 6.8855 (1.8); 6.8821 (1.4); 5.9884 (0.9); 5.2981 (10.6); 4.9142 (1.7); 4.9026 (16.0); 4.7268 (1.1); 2.8681 (0.7); 2.8592 (1.2); 2.8501 (1.6); 2.8411 (1.6); 2.8320 (1.2); 2.8231 (0.8); 2.0433 (0.6); 1.5631 (4.3); 1.2584 (0.6); 0.8814 (1.2); 0.8757 (0.6); 0.8669 (2.6); 0.8640 (4.2); 0.8610 (2.3); 0.8501 (3.8); 0.8461 (3.1); 0.8430 (2.0); 0.8370 (0.7); 0.8326 (1.6); 0.6537 (1.4); 0.6438 (3.0); 0.6405 (3.3); 0.6349 (3.2); 0.6309 (3.3); 0.6272 (2.9); 0.6134 (1.3); 0.0079 (0.8); −0.0002 (26.2); −0.0085 (1.0) III-029: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5124 (0.5); 7.5090 (0.5); 7.4907 (1.4); 7.4845 (0.5); 7.4757 (0.8); 7.4722 (1.4); 7.4686 (0.8); 7.4446 (1.6); 7.4411 (0.9); 7.4296 (1.5); 7.4258 (2.9); 7.4212 (0.8); 7.4123 (0.8); 7.4078 (1.8); 7.4045 (1.2); 7.3558 (0.6); 7.3402 (0.6); 7.3349 (2.3); 7.3318 (2.8); 7.3281 (1.3); 7.3196 (0.8); 7.3145 (2.4); 7.3107 (1.7); 7.2610 (20.9); 7.2555 (0.7); 7.2513 (0.6); 7.2485 (0.8); 7.2428 (1.3); 7.2276 (1.2); 7.2222 (0.9); 7.2072 (0.7); 7.0340 (0.6); 7.0319 (0.6); 7.0278 (0.6); 7.0257 (0.6); 7.0135 (0.8); 7.0112 (0.9); 7.0072 (1.0); 7.0050 (0.9); 6.9865 (0.5); 6.9610 (0.7); 6.9556 (1.1); 6.9500 (0.6); 6.9375 (0.7); 6.9323 (1.0); 6.9267 (0.7); 6.9137 (0.9); 6.9120 (1.0); 6.9088 (0.8); 6.9068 (0.7); 6.8933 (0.8); 6.8920 (0.8); 6.8884 (0.7); 6.8869 (0.6); 5.2979 (9.4); 4.9951 (0.9); 4.9831 (7.6); 4.8328 (0.6); 4.1905 (3.8); 4.1766 (3.8); 4.1669 (0.5); 3.7927 (16.0); 3.7800 (1.5); −0.0002 (8.5) III-030: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5037 (1.4); 7.5004 (0.8); 7.4916 (0.8); 7.4852 (3.0); 7.4792 (1.1); 7.4701 (1.6); 7.4666 (2.9); 7.4631 (1.6); 7.4415 (0.8); 7.4363 (3.3); 7.4328 (1.8); 7.4212 (3.1); 7.4174 (5.8); 7.4129 (1.6); 7.4038 (1.2); 7.3994 (3.2); 7.3962 (1.9); 7.3448 (10.8); 7.3442 (10.8); 7.3378 (5.2); 7.3331 (13.0); 7.3248 (2.0); 7.3177 (2.1); 7.3139 (2.4); 7.3089 (6.3); 7.3058 (6.6); 7.3006 (5.1); 7.2933 (3.0); 7.2884 (6.5); 7.2847 (4.7); 7.2792 (2.8); 7.2737 (1.6); 7.2684 (1.9); 7.2587 (55.0); 7.2478 (2.6); 7.2420 (3.7); 7.2326 (1.7); 7.2269 (3.1); 7.2216 (2.2); 7.2134 (1.0); 7.2070 (1.7); 7.1927 (0.5); 7.0357 (0.9); 7.0334 (1.0); 7.0294 (1.0); 7.0272 (1.0); 7.0150 (1.7); 7.0127 (1.9); 7.0088 (1.7); 7.0066 (1.8); 6.9943 (1.3); 6.9921 (1.1); 6.9880 (1.1); 6.9858 (1.0); 6.9451 (0.6); 6.9345 (1.3); 6.9290 (2.2); 6.9235 (1.5); 6.9109 (1.2); 6.9059 (2.1); 6.8988 (2.8); 6.8961 (2.6); 6.8932 (1.6); 6.8908 (1.4); 6.8778 (1.8); 6.8764 (1.8); 6.8730 (1.5); 6.8712 (1.3); 5.9808 (1.3); 5.2961 (16.0); 4.9904 (2.1); 4.9819 (15.6); 4.8250 (1.6); 4.7655 (0.6); 4.6005 (7.1); 4.5854 (7.0); 4.5689 (0.9); 4.5540 (0.8); 1.5619 (3.4); 0.0080 (0.8); −0.0002 (22.3); −0.0085 (0.8) III-031: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5362 (0.6); 7.5167 (1.4); 7.5132 (1.2); 7.5098 (0.7); 7.5013 (0.8); 7.4988 (0.7); 7.4948 (3.0); 7.4887 (1.1); 7.4797 (1.6); 7.4762 (2.9); 7.4727 (1.6); 7.4529 (0.7); 7.4490 (2.8); 7.4476 (3.2); 7.4441 (1.8); 7.4325 (3.0); 7.4287 (5.9); 7.4240 (1.6); 7.4152 (1.2); 7.4108 (3.2); 7.4076 (1.9); 7.3713 (0.9); 7.3681 (1.0); 7.3647 (0.6); 7.3603 (0.8); 7.3553 (0.7); 7.3508 (1.1); 7.3469 (0.9); 7.3421 (0.8); 7.3353 (0.9); 7.3302 (4.8); 7.3271 (5.9); 7.3248 (2.6); 7.3233 (2.9); 7.3148 (1.5); 7.3097 (5.1); 7.3060 (3.6); 7.2665 (2.1); 7.2600 (90.9); 7.2520 (2.8); 7.2462 (3.2); 7.2350 (1.1); 7.2310 (2.6); 7.2256 (1.8); 7.2201 (0.6); 7.2153 (0.8); 7.2110 (1.6); 7.2012 (0.7); 7.0368 (1.4); 7.0346 (1.6); 7.0305 (1.6); 7.0283 (1.7); 7.0159 (2.4); 7.0138 (2.7); 7.0098 (2.6); 7.0077 (2.5); 6.9957 (1.8); 6.9932 (1.3); 6.9892 (1.4); 6.9869 (1.4); 6.9497 (1.4); 6.9444 (2.4); 6.9390 (1.6); 6.9263 (1.3); 6.9213 (2.2); 6.9141 (2.8); 6.9115 (2.6); 6.9085 (1.6); 6.9062 (1.4); 6.8932 (1.6); 6.8918 (1.7); 6.8884 (1.4); 6.0755 (0.5); 6.0122 (1.0); 5.9580 (0.7); 5.9441 (1.5); 5.9321 (0.9); 5.9304 (0.9); 5.9184 (1.7); 5.9151 (1.0); 5.9045 (1.0); 5.9012 (1.9); 5.8892 (1.1); 5.8875 (1.2); 5.8754 (1.9); 5.8616 (0.9); 5.3045 (1.0); 5.3003 (2.5); 5.2978 (3.5); 5.2931 (1.2); 5.2615 (1.0); 5.2573 (2.2); 5.2543 (2.3); 5.2501 (1.2); 5.2208 (0.5); 5.2154 (1.2); 5.2119 (2.6); 5.2087 (2.6); 5.2052 (1.2); 5.1950 (0.5); 5.1897 (1.1); 5.1862 (2.4); 5.1830 (2.3); 5.1795 (1.0); 5.1735 (0.5); 4.9628 (2.6); 4.9512 (16.0); 4.7881 (1.8); 4.7298 (0.6); 4.0499 (1.6); 4.0459 (2.4); 4.0418 (1.8); 4.0357 (3.0); 4.0317 (4.5); 4.0278 (2.7); 4.0214 (1.9); 4.0174 (2.6); 4.0136 (1.6); 4.0008 (0.7); 1.5559 (5.7); 0.0080 (1.2); −0.0002 (38.0); −0.0085 (1.4) III-035: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4378 (0.8); 7.4325 (1.4); 7.4250 (6.7); 7.4212 (7.1); 7.4150 (2.8); 7.4111 (2.5); 7.4069 (4.4); 7.4053 (3.9); 7.3981 (1.3); 7.3939 (1.5); 7.3879 (0.6); 7.3836 (0.7); 7.3186 (0.6); 7.3113 (4.7); 7.3071 (5.2); 7.3020 (2.0); 7.3002 (1.9); 7.2976 (1.8); 7.2948 (2.4); 7.2925 (2.6); 7.2871 (3.5); 7.2601 (36.3); 7.2271 (1.0); 7.2109 (1.0); 7.2067 (2.1); 7.1919 (1.7); 7.1905 (1.8); 7.1874 (1.3); 7.1724 (1.0); 7.1705 (1.0); 6.9607 (0.8); 6.9554 (2.0); 6.9506 (1.8); 6.9473 (1.5); 6.9447 (1.7); 6.9409 (0.8); 6.9380 (0.9); 6.9362 (0.9); 6.9309 (2.0); 6.9268 (3.7); 6.9241 (3.9); 6.9202 (1.7); 6.9175 (3.5); 6.9145 (2.3); 6.9101 (1.5); 6.9060 (1.1); 6.9037 (1.4); 6.8974 (2.5); 6.8951 (1.8); 6.8924 (1.7); 6.8901 (1.3); 6.7097 (0.7); 5.2973 (7.6); 4.8608 (16.0); 3.2684 (3.6); 3.2541 (4.2); 3.2509 (4.2); 3.2366 (3.6); 1.5736 (3.6); 1.0504 (0.8); 1.0484 (0.8); 1.0425 (0.7); 1.0385 (0.6); 1.0361 (0.5); 1.0305 (1.4); 1.0225 (0.6); 1.0183 (0.8); 1.0125 (0.8); 1.0105 (0.9); 0.5610 (1.2); 0.5491 (3.2); 0.5462 (3.7); 0.5440 (2.3); 0.5411 (1.7); 0.5347 (1.8); 0.5291 (3.6); 0.5261 (3.1); 0.5147 (1.4); 0.2767 (1.4); 0.2651 (4.2); 0.2531 (3.4); 0.2503 (4.3); 0.2384 (1.0); −0.0002 (14.4); −0.0084 (0.6) III-038: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 8.9430 (1.5); 7.4486 (0.7); 7.4444 (0.8); 7.4322 (3.8); 7.4281 (4.7); 7.4193 (7.5); 7.4170 (12.4); 7.4148 (14.1); 7.4095 (9.7); 7.4031 (4.9); 7.3991 (6.9); 7.3974 (6.3); 7.3891 (2.5); 7.3852 (3.2); 7.3742 (4.3); 7.3655 (7.3); 7.3573 (3.9); 7.3514 (7.5); 7.3478 (6.9); 7.3404 (1.8); 7.2726 (1.2); 7.2655 (6.8); 7.2609 (10.1); 7.2581 (49.7); 7.2517 (3.4); 7.2484 (4.1); 7.2466 (4.4); 7.2415 (5.0); 7.2110 (1.1); 7.1904 (2.2); 7.1746 (2.2); 7.1702 (1.6); 7.1541 (1.2); 6.9328 (1.1); 6.9286 (1.4); 6.9267 (1.5); 6.9060 (3.6); 6.9000 (2.0); 6.8939 (1.7); 6.8875 (1.8); 6.8854 (1.8); 6.8754 (1.9); 6.8655 (3.0); 6.8639 (2.9); 6.8450 (2.1); 6.8412 (2.1); 5.2951 (16.0); 4.9969 (13.2); 4.9029 (5.9); 4.7024 (2.2); 1.5851 (0.9); 0.0079 (0.6); −0.0002 (20.3); −0.0085 (0.8) III-039: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4141 (1.2); 7.3996 (1.1); 7.3936 (2.4); 7.3790 (1.9); 7.3728 (1.7); 7.3593 (1.4); 7.2611 (47.7); 7.2040 (1.0); 7.2015 (1.1); 7.1977 (1.1); 7.1952 (1.1); 7.1829 (1.8); 7.1803 (2.0); 7.1767 (1.9); 7.1740 (2.0); 7.1624 (4.1); 7.1594 (1.8); 7.1567 (1.8); 7.1509 (3.9); 7.1453 (2.6); 7.1397 (5.2); 7.1338 (1.7); 7.1280 (5.0); 7.1197 (0.6); 7.0759 (1.8); 7.0721 (3.0); 7.0695 (2.6); 7.0641 (1.9); 7.0600 (2.3); 7.0560 (2.6); 7.0535 (4.3); 7.0412 (2.0); 7.0357 (6.6); 7.0302 (2.3); 7.0242 (0.9); 7.0158 (5.6); 7.0129 (4.2); 7.0102 (1.9); 7.0045 (0.6); 6.9987 (1.3); 6.9930 (3.6); 6.9289 (0.9); 5.2984 (1.2); 5.0248 (0.5); 4.8993 (16.0); 3.8220 (1.0); 3.4083 (1.8); 3.3907 (3.3); 3.3756 (3.3); 3.3577 (1.8); 1.6204 (1.7); 1.6028 (2.6); 1.5955 (1.5); 1.5844 (2.4); 1.5740 (2.6); 1.3826 (1.5); 1.3733 (3.8); 1.3644 (5.3); 1.3549 (6.6); 1.3460 (3.1); 1.3372 (1.7); 0.9288 (3.6); 0.9244 (2.1); 0.9113 (11.0); 0.9052 (2.4); 0.8971 (2.0); 0.8934 (3.0); 0.0080 (0.6); −0.0002 (19.1); −0.0085 (0.7) III-040: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4161 (1.3); 7.4017 (1.1); 7.3956 (2.4); 7.3908 (0.5); 7.3811 (1.9); 7.3747 (1.7); 7.3615 (1.4); 7.2611 (46.2); 7.2054 (1.0); 7.2029 (1.1); 7.1990 (1.1); 7.1965 (1.2); 7.1843 (1.8); 7.1816 (1.9); 7.1781 (1.8); 7.1754 (2.2); 7.1666 (3.7); 7.1632 (1.8); 7.1608 (2.3); 7.1549 (4.4); 7.1494 (2.8); 7.1437 (5.2); 7.1378 (1.8); 7.1320 (4.9); 7.1237 (0.8); 7.0801 (2.0); 7.0762 (3.2); 7.0737 (2.9); 7.0678 (2.4); 7.0638 (3.0); 7.0602 (3.3); 7.0574 (5.3); 7.0455 (2.9); 7.0375 (6.6); 7.0316 (2.3); 7.0259 (1.2); 7.0200 (2.2); 7.0176 (5.8); 7.0145 (4.3); 7.0118 (2.1); 7.0061 (0.8); 7.0004 (1.5); 6.9947 (3.6); 6.9863 (0.5); 5.2985 (3.1); 4.9118 (16.0); 3.2784 (3.6); 3.2642 (4.2); 3.2607 (4.4); 3.2466 (3.8); 1.5731 (2.4); 1.0671 (0.8); 1.0651 (0.8); 1.0592 (0.8); 1.0551 (0.6); 1.0528 (0.6); 1.0472 (1.6); 1.0392 (0.7); 1.0350 (0.8); 1.0292 (0.9); 1.0272 (1.0); 1.0151 (0.6); 0.5872 (1.2); 0.5753 (3.2); 0.5724 (4.0); 0.5700 (2.4); 0.5673 (1.8); 0.5608 (2.0); 0.5552 (3.8); 0.5523 (3.3); 0.5408 (1.7); 0.2972 (1.4); 0.2855 (4.3); 0.2832 (3.7); 0.2735 (3.5); 0.2708 (4.5); 0.2590 (1.3); 0.0080 (0.6); −0.0002 (19.7); −0.0084 (0.9) III-041: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4129 (1.2); 7.3984 (1.1); 7.3923 (2.3); 7.3778 (1.8); 7.3715 (1.6); 7.3582 (1.3); 7.2610 (53.3); 7.2035 (0.9); 7.2009 (1.1); 7.1972 (1.0); 7.1946 (1.1); 7.1824 (1.7); 7.1798 (1.8); 7.1762 (1.7); 7.1735 (1.8); 7.1611 (1.1); 7.1569 (3.5); 7.1513 (1.7); 7.1452 (3.5); 7.1397 (2.4); 7.1339 (4.8); 7.1281 (1.6); 7.1256 (1.4); 7.1223 (4.7); 7.1140 (0.6); 7.0721 (1.8); 7.0683 (2.9); 7.0657 (2.5); 7.0601 (1.9); 7.0561 (2.3); 7.0522 (2.6); 7.0496 (4.2); 7.0439 (1.1); 7.0355 (5.6); 7.0301 (2.4); 7.0278 (1.6); 7.0240 (1.0); 7.0181 (2.1); 7.0156 (5.5); 7.0126 (4.1); 7.0099 (2.1); 7.0041 (1.1); 6.9985 (2.1); 6.9927 (4.2); 6.9845 (1.0); 5.2986 (5.9); 4.8865 (16.0); 2.8649 (0.7); 2.8561 (1.1); 2.8469 (1.5); 2.8380 (1.6); 2.8288 (1.1); 2.8200 (0.7); 1.5641 (3.4); 1.2585 (0.5); 0.8827 (1.1); 0.8683 (2.8); 0.8654 (4.2); 0.8623 (2.0); 0.8514 (3.8); 0.8475 (3.1); 0.8444 (1.8); 0.8338 (1.3); 0.6509 (1.3); 0.6409 (2.9); 0.6377 (3.2); 0.6341 (2.9); 0.6319 (3.0); 0.6281 (3.2); 0.6246 (2.7); 0.6107 (1.0); 0.0080 (0.7); −0.0002 (22.6); −0.0085 (0.8) III-042: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4159 (1.1); 7.4010 (1.1); 7.3953 (2.2); 7.3911 (0.6); 7.3808 (1.8); 7.3744 (1.4); 7.3608 (1.4); 7.2612 (28.4); 7.2056 (1.0); 7.2032 (1.1); 7.1992 (1.1); 7.1969 (1.1); 7.1845 (1.7); 7.1819 (1.8); 7.1783 (1.8); 7.1757 (1.9); 7.1636 (3.8); 7.1577 (2.0); 7.1521 (3.6); 7.1467 (2.5); 7.1410 (4.8); 7.1351 (1.8); 7.1293 (4.8); 7.1210 (1.0); 7.0948 (1.1); 7.0788 (2.1); 7.0752 (3.2); 7.0726 (2.6); 7.0660 (2.0); 7.0619 (2.4); 7.0592 (3.1); 7.0559 (4.6); 7.0432 (2.1); 7.0377 (6.1); 7.0323 (2.3); 7.0263 (1.0); 7.0178 (5.1); 7.0151 (3.9); 7.0124 (1.9); 7.0066 (0.7); 7.0008 (1.3); 6.9952 (3.3); 5.2984 (5.3); 4.9386 (16.0); 4.2016 (4.4); 4.1953 (4.7); 4.1880 (4.6); 4.1816 (4.5); 3.8217 (0.7); 2.2867 (2.5); 2.2803 (5.2); 2.2739 (2.7); 2.0433 (0.6); 1.5721 (1.6); −0.0002 (12.3); −0.0085 (0.6) III-043: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4140 (1.2); 7.3995 (1.1); 7.3935 (2.3); 7.3890 (0.5); 7.3790 (1.8); 7.3726 (1.5); 7.3592 (1.3); 7.2613 (35.5); 7.2037 (1.0); 7.2011 (1.1); 7.1973 (1.0); 7.1948 (1.1); 7.1826 (1.7); 7.1799 (1.8); 7.1764 (1.8); 7.1736 (2.0); 7.1647 (3.5); 7.1615 (1.7); 7.1590 (2.1); 7.1529 (4.2); 7.1475 (2.5); 7.1418 (5.0); 7.1359 (1.6); 7.1301 (4.7); 7.1219 (0.6); 7.0767 (1.8); 7.0728 (2.8); 7.0703 (2.4); 7.0641 (1.8); 7.0600 (2.4); 7.0571 (2.8); 7.0538 (4.8); 7.0462 (1.0); 7.0409 (2.3); 7.0379 (6.2); 7.0319 (2.5); 7.0264 (1.1); 7.0181 (5.7); 7.0151 (4.3); 7.0124 (2.2); 7.0066 (1.1); 7.0009 (1.9); 6.9952 (4.0); 6.9869 (0.9); 5.9558 (0.6); 5.9419 (1.4); 5.9300 (0.8); 5.9282 (0.8); 5.9162 (1.6); 5.9128 (0.9); 5.9023 (0.9); 5.8990 (1.6); 5.8870 (0.9); 5.8853 (0.9); 5.8732 (1.7); 5.8594 (0.8); 5.3015 (1.3); 5.2981 (7.6); 5.2945 (2.6); 5.2903 (1.1); 5.2588 (0.9); 5.2546 (2.0); 5.2515 (2.0); 5.2473 (0.9); 5.2154 (1.1); 5.2119 (2.6); 5.2087 (2.4); 5.2052 (1.0); 5.1897 (1.0); 5.1861 (2.4); 5.1829 (2.3); 5.1794 (0.9); 4.9349 (16.0); 4.0468 (1.4); 4.0431 (2.3); 4.0391 (1.5); 4.0325 (2.7); 4.0288 (4.4); 4.0251 (2.6); 4.0185 (1.6); 4.0145 (2.3); 4.0107 (1.3); 1.5850 (1.2); −0.0002 (14.3); −0.0085 (0.6) III-045: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5181 (1.5); 7.3032 (1.2); 7.2976 (1.7); 7.2931 (1.2); 7.2831 (7.3); 7.2816 (6.9); 7.2777 (4.5); 7.2750 (3.8); 7.2699 (6.4); 7.2592 (256.6); 7.2500 (5.6); 7.2477 (5.8); 7.2440 (1.8); 7.2381 (2.3); 7.2365 (2.1); 7.2223 (0.5); 7.2187 (0.7); 7.2092 (0.6); 7.1748 (0.6); 7.1471 (4.5); 7.1430 (5.4); 7.1373 (1.6); 7.1307 (2.4); 7.1261 (4.4); 7.1227 (3.6); 7.0952 (0.6); 7.0881 (4.6); 7.0826 (1.4); 7.0711 (1.7); 7.0666 (6.7); 7.0614 (1.6); 7.0499 (1.3); 7.0445 (3.6); 6.9952 (1.4); 6.7413 (0.8); 5.9268 (0.6); 5.9133 (1.3); 5.9007 (0.9); 5.8875 (1.5); 5.8839 (0.8); 5.8740 (0.8); 5.8703 (1.6); 5.8577 (1.1); 5.8446 (1.6); 5.8311 (0.8); 5.3280 (1.0); 5.3109 (3.2); 5.2938 (3.3); 5.2768 (1.0); 5.2406 (1.0); 5.2363 (2.3); 5.2330 (2.4); 5.2287 (1.0); 5.1977 (0.9); 5.1933 (2.0); 5.1900 (2.1); 5.1858 (0.9); 5.1558 (1.1); 5.1522 (2.7); 5.1487 (2.6); 5.1451 (1.0); 5.1300 (1.0); 5.1264 (2.5); 5.1230 (2.4); 5.1193 (1.0); 3.9914 (0.8); 3.9872 (1.5); 3.9813 (1.7); 3.9772 (2.0); 3.9727 (2.6); 3.9674 (2.8); 3.9633 (2.0); 3.9592 (1.6); 3.9533 (1.5); 3.9490 (0.8); 1.7140 (16.0); 1.6970 (15.9); 1.5575 (6.2); 0.0080 (3.4); −0.0002 (99.9); −0.0085 (3.4) III-046: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5182 (0.7); 7.3013 (0.6); 7.2961 (0.8); 7.2877 (0.8); 7.2814 (3.6); 7.2798 (3.4); 7.2759 (2.3); 7.2733 (2.1); 7.2684 (3.4); 7.2593 (131.7); 7.2519 (4.6); 7.2475 (2.7); 7.2464 (2.7); 7.2415 (0.7); 7.2355 (1.1); 7.1457 (2.2); 7.1415 (2.7); 7.1359 (0.8); 7.1291 (1.2); 7.1246 (2.2); 7.1213 (1.8); 7.0879 (2.2); 7.0824 (0.7); 7.0709 (0.8); 7.0662 (3.3); 7.0612 (0.8); 7.0497 (0.6); 7.0443 (1.7); 6.9953 (0.7); 5.2764 (1.6); 5.2594 (1.6); 3.3302 (0.6); 3.3124 (1.2); 3.3002 (1.3); 3.2974 (1.2); 3.2857 (1.2); 3.2802 (0.6); 3.2680 (0.6); 1.6990 (7.7); 1.6820 (7.6); 1.6004 (1.2); 1.5823 (2.5); 1.5641 (2.8); 1.5389 (16.0); 0.9486 (4.0); 0.9302 (8.2); 0.9116 (3.5); 0.0080 (1.7); −0.0002 (49.5); −0.0084 (1.7) III-047: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3029 (0.7); 7.2988 (1.0); 7.2975 (1.0); 7.2932 (0.9); 7.2873 (3.0); 7.2813 (4.2); 7.2774 (2.2); 7.2744 (4.1); 7.2650 (6.0); 7.2594 (82.3); 7.2528 (5.6); 7.2491 (2.2); 7.2448 (0.7); 7.2427 (0.7); 7.2368 (1.4); 7.2354 (1.3); 7.1528 (3.0); 7.1487 (3.7); 7.1431 (1.0); 7.1363 (1.6); 7.1318 (2.9); 7.1285 (2.4); 7.0901 (3.0); 7.0846 (0.9); 7.0759 (0.6); 7.0731 (1.1); 7.0686 (4.4); 7.0633 (1.1); 7.0519 (0.8); 7.0465 (2.3); 6.7700 (0.6); 5.2980 (0.6); 5.2809 (2.1); 5.2639 (2.1); 5.2469 (0.6); 3.2195 (1.6); 3.2173 (1.6); 3.2027 (2.8); 3.1875 (1.6); 1.7060 (10.3); 1.6890 (10.1); 1.5458 (16.0); 1.0121 (0.6); 1.0098 (0.5); 0.9921 (1.0); 0.9799 (0.5); 0.9744 (0.6); 0.9721 (0.6); 0.5169 (0.8); 0.5116 (2.0); 0.5087 (2.6); 0.5060 (1.5); 0.4961 (1.0); 0.4915 (2.3); 0.4886 (2.1); 0.4837 (0.8); 0.2395 (0.9); 0.2331 (1.2); 0.2307 (1.3); 0.2275 (1.8); 0.2238 (2.0); 0.2184 (1.7); 0.2121 (1.2); 0.2060 (0.8); 0.0079 (1.1); −0.0002 (31.3); −0.0085 (1.0) III-048: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.2782 (1.2); 7.2741 (0.8); 7.2715 (0.8); 7.2595 (48.7); 7.2465 (0.7); 7.2441 (0.8); 7.1435 (0.7); 7.1393 (0.8); 7.1224 (0.7); 7.1192 (0.6); 7.0878 (0.7); 7.0661 (1.0); 7.0443 (0.5); 1.7046 (2.3); 1.6876 (2.2); 1.5377 (16.0); 0.9226 (3.6); 0.9059 (3.5); 0.0079 (0.7); −0.0002 (19.6); −0.0085 (0.8) III-049: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5182 (0.7); 7.3099 (1.3); 7.3044 (1.9); 7.3000 (1.2); 7.2882 (5.9); 7.2819 (6.1); 7.2763 (3.0); 7.2733 (4.0); 7.2690 (10.6); 7.2593 (120.4); 7.2527 (4.8); 7.2465 (5.8); 7.2337 (0.6); 7.2288 (0.6); 7.2250 (0.7); 7.1562 (4.7); 7.1520 (5.9); 7.1464 (1.7); 7.1398 (2.4); 7.1352 (4.5); 7.1318 (3.8); 7.0970 (0.6); 7.0899 (4.5); 7.0844 (1.5); 7.0677 (7.5); 7.0632 (1.8); 7.0517 (1.3); 7.0463 (3.7); 6.9952 (0.7); 6.7242 (1.0); 5.9218 (0.6); 5.9082 (1.3); 5.8948 (1.1); 5.8824 (1.5); 5.8788 (0.9); 5.8687 (0.8); 5.8652 (1.6); 5.8519 (1.2); 5.8395 (1.6); 5.8259 (0.8); 5.3246 (1.1); 5.3076 (3.5); 5.2906 (3.5); 5.2736 (1.1); 5.2346 (1.0); 5.2303 (2.5); 5.2270 (2.4); 5.2227 (1.1); 5.1917 (0.9); 5.1874 (2.2); 5.1840 (2.1); 5.1832 (2.0); 5.1798 (1.0); 5.1490 (2.7); 5.1456 (2.6); 5.1420 (1.1); 5.1232 (2.5); 5.1198 (2.4); 5.1163 (1.0); 3.9846 (1.9); 3.9801 (2.1); 3.9753 (2.2); 3.9703 (3.5); 3.9659 (3.5); 3.9615 (2.2); 3.9562 (2.0); 3.9519 (1.9); 3.9477 (0.8); 1.7111 (16.0); 1.6941 (15.8); 1.5438 (11.2); 0.0080 (1.6); −0.0002 (45.9); −0.0085 (1.8) III-050: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.5182 (0.7); 7.3083 (1.7); 7.3027 (1.6); 7.2982 (1.1); 7.2940 (1.0); 7.2863 (5.1); 7.2804 (5.4); 7.2751 (2.6); 7.2715 (3.5); 7.2676 (10.4); 7.2594 (124.2); 7.2545 (6.3); 7.2510 (3.3); 7.2452 (4.7); 7.2421 (2.4); 7.2227 (0.7); 7.1547 (4.2); 7.1506 (5.4); 7.1449 (1.5); 7.1382 (2.3); 7.1336 (4.2); 7.1303 (3.5); 7.0968 (0.6); 7.0897 (4.3); 7.0842 (1.4); 7.0755 (0.8); 7.0727 (1.5); 7.0682 (6.4); 7.0630 (1.6); 7.0515 (1.2); 7.0461 (3.4); 6.9954 (0.7); 6.6541 (0.8); 5.2893 (0.9); 5.2723 (3.1); 5.2553 (3.1); 5.2383 (0.9); 3.3270 (1.2); 3.3174 (1.2); 3.3093 (2.3); 3.3026 (1.5); 3.2997 (2.3); 3.2942 (2.2); 3.2849 (2.4); 3.2765 (1.1); 3.2673 (1.2); 1.6956 (15.0); 1.6786 (14.9); 1.6152 (0.6); 1.5968 (2.5); 1.5787 (5.1); 1.5604 (6.1); 1.5466 (5.9); 1.5426 (6.2); 1.5243 (0.9); 0.9427 (7.9); 0.9243 (16.0); 0.9057 (6.9); 0.0080 (1.6); −0.0002 (45.1); −0.0085 (1.5) III-051: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.2870 (1.5); 7.2817 (1.0); 7.2733 (1.8); 7.2695 (2.4); 7.2678 (2.2); 7.2594 (66.9); 7.2437 (0.7); 7.1620 (1.0); 7.1580 (1.3); 7.1455 (0.6); 7.1410 (1.0); 7.1377 (0.8); 7.0922 (1.0); 7.0706 (1.6); 7.0486 (0.8); 5.2774 (0.7); 5.2604 (0.8); 3.2163 (0.8); 3.2020 (1.0); 3.1990 (1.0); 3.1847 (0.9); 1.7023 (3.6); 1.6853 (3.6); 1.5378 (16.0); 0.5081 (0.7); 0.5053 (0.9); 0.5027 (0.6); 0.4881 (0.8); 0.4852 (0.7); 0.2234 (0.7); 0.2196 (0.7); 0.2141 (0.6); 0.0080 (0.9); −0.0002 (25.2); −0.0084 (1.0) III-052: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3059 (0.9); 7.3017 (1.2); 7.3004 (1.3); 7.2960 (0.9); 7.2918 (0.8); 7.2842 (4.3); 7.2784 (4.4); 7.2730 (2.2); 7.2694 (3.1); 7.2655 (9.4); 7.2637 (7.7); 7.2595 (64.8); 7.2529 (3.9); 7.2488 (2.2); 7.2465 (1.7); 7.2431 (4.1); 7.2410 (2.3); 7.2213 (0.6); 7.1523 (3.7); 7.1481 (4.5); 7.1425 (1.3); 7.1358 (2.0); 7.1312 (3.7); 7.1279 (3.0); 7.0892 (3.8); 7.0837 (1.2); 7.0749 (0.8); 7.0722 (1.3); 7.0677 (5.5); 7.0625 (1.4); 7.0510 (1.1); 7.0456 (2.9); 6.6798 (0.7); 5.2943 (0.8); 5.2773 (2.6); 5.2603 (2.6); 5.2433 (0.8); 3.2352 (0.6); 3.2189 (1.0); 3.2022 (1.8); 3.1857 (2.2); 3.1694 (1.2); 3.1499 (1.4); 3.1351 (1.8); 3.1330 (1.7); 3.1180 (1.7); 3.1019 (0.8); 3.0998 (0.8); 3.0850 (0.7); 1.8452 (0.7); 1.8283 (1.4); 1.8115 (1.8); 1.7947 (1.5); 1.7780 (0.8); 1.7011 (12.6); 1.6840 (12.6); 1.5563 (2.4); 0.9167 (16.0); 0.9149 (15.6); 0.9000 (15.5); 0.8982 (15.0); 0.0079 (0.8); −0.0002 (23.7); −0.0085 (0.9) III-058: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3094 (0.6); 7.3045 (0.7); 7.2874 (3.7); 7.2817 (1.9); 7.2735 (2.9); 7.2690 (4.1); 7.2595 (62.6); 7.2542 (3.4); 7.2517 (3.4); 7.2478 (1.1); 7.2445 (0.7); 7.2413 (1.2); 7.1648 (2.2); 7.1608 (2.9); 7.1552 (1.1); 7.1482 (1.5); 7.1437 (2.5); 7.1405 (2.1); 7.0883 (2.1); 7.0828 (0.7); 7.0712 (0.8); 7.0667 (3.2); 7.0616 (0.8); 7.0501 (0.8); 7.0447 (1.7); 5.3521 (1.5); 5.3351 (1.5); 5.2981 (1.5); 4.1430 (1.7); 4.1293 (2.0); 4.1190 (1.9); 4.1057 (1.8); 3.7752 (2.5); 3.7680 (16.0); 1.7188 (7.2); 1.7017 (7.3); 1.6799 (0.8); 1.5424 (9.5); 0.0080 (0.7); −0.0002 (23.2); −0.0085 (0.9) III-059: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.2989 (1.0); 7.2938 (1.0); 7.2909 (1.6); 7.2807 (3.2); 7.2776 (4.2); 7.2673 (3.8); 7.2600 (66.7); 7.2516 (3.5); 7.2476 (3.4); 7.2450 (3.0); 7.2348 (1.4); 7.2313 (1.6); 7.2158 (0.6); 7.1569 (1.7); 7.1529 (2.1); 7.1456 (1.9); 7.1414 (2.7); 7.1358 (2.1); 7.1326 (1.4); 7.1289 (1.1); 7.1244 (1.9); 7.1212 (1.5); 7.0870 (2.7); 7.0825 (1.1); 7.0656 (4.6); 7.0444 (2.3); 7.0361 (0.6); 7.0253 (0.7); 5.2978 (3.2); 5.2467 (1.2); 5.2298 (1.4); 5.2142 (1.6); 5.1973 (1.4); 4.3949 (0.7); 4.3779 (0.8); 3.6839 (1.7); 3.6745 (1.5); 3.6659 (16.0); 3.6614 (13.9); 2.8912 (0.7); 2.8847 (0.7); 2.8696 (0.8); 2.2657 (0.6); 2.2543 (0.5); 2.2486 (0.8); 2.2317 (0.7); 2.2260 (0.5); 2.0075 (0.5); 1.9977 (1.2); 1.9860 (0.9); 1.9815 (1.6); 1.9656 (1.3); 1.9558 (0.8); 1.9448 (1.1); 1.9309 (0.7); 1.9146 (0.6); 1.8564 (0.8); 1.8371 (0.7); 1.8301 (0.5); 1.8236 (0.6); 1.7699 (0.6); 1.7530 (0.5); 1.7360 (0.7); 1.7204 (0.7); 1.7051 (0.6); 1.6867 (6.4); 1.6791 (5.4); 1.6696 (6.3); 1.6621 (5.4); 1.6484 (0.8); 1.6414 (0.6); 1.5600 (14.0); 0.0080 (0.8); −0.0002 (23.2); −0.0085 (0.8) III-063: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3021 (0.5); 7.2857 (2.3); 7.2795 (1.3); 7.2719 (2.2); 7.2675 (2.9); 7.2660 (2.8); 7.2593 (23.0); 7.2501 (1.7); 7.2453 (0.9); 7.2434 (0.9); 7.1572 (1.4); 7.1528 (1.5); 7.1472 (0.6); 7.1409 (0.9); 7.1363 (1.4); 7.1329 (1.2); 7.0883 (1.2); 7.0712 (0.5); 7.0665 (1.9); 7.0448 (1.0); 5.2854 (0.6); 5.2819 (0.6); 5.2424 (0.6); 5.2388 (0.5); 5.1413 (0.7); 5.1378 (0.7); 5.1155 (0.7); 5.1120 (0.6); 3.9979 (0.5); 3.9938 (0.8); 3.9897 (0.6); 3.9835 (0.8); 3.9798 (1.3); 3.9761 (0.8); 3.9700 (0.6); 3.9658 (0.8); 1.7663 (16.0); 1.5476 (6.4); −0.0002 (8.0) III-066: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4567 (0.6); 7.4530 (0.7); 7.4443 (0.7); 7.4390 (1.2); 7.4345 (1.3); 7.4220 (1.2); 7.4205 (1.2); 7.4182 (1.2); 7.4132 (1.0); 7.4044 (0.9); 7.3998 (1.8); 7.3953 (1.2); 7.3798 (2.2); 7.3764 (1.9); 7.3616 (1.7); 7.3573 (1.3); 7.2609 (29.4); 7.2601 (28.7); 7.2400 (2.5); 7.2386 (2.5); 7.2199 (1.2); 7.2064 (1.1); 7.2011 (1.1); 7.1879 (1.1); 7.1815 (1.6); 7.1751 (1.3); 7.1710 (1.2); 7.1621 (1.1); 7.1568 (1.2); 7.1501 (1.9); 7.1296 (1.6); 7.1255 (1.8); 7.1051 (2.7); 7.0837 (1.7); 7.0805 (2.6); 7.0593 (1.4); 7.0563 (1.3); 7.0460 (1.0); 7.0419 (1.4); 7.0366 (1.5); 7.0315 (1.4); 7.0265 (1.1); 7.0206 (1.1); 7.0154 (1.2); 7.0104 (1.1); 6.9968 (0.9); 6.9810 (0.8); 5.9546 (0.5); 5.9409 (1.0); 5.9278 (0.9); 5.9151 (1.2); 5.9120 (0.8); 5.9010 (0.8); 5.8980 (1.3); 5.8848 (1.0); 5.8722 (1.3); 5.8583 (0.6); 5.2979 (4.2); 5.2554 (1.9); 5.2515 (1.9); 5.2483 (0.9); 5.2124 (2.3); 5.2089 (2.1); 5.1866 (2.1); 5.1832 (2.0); 4.9068 (16.0); 4.7635 (0.8); 4.0409 (2.5); 4.0373 (1.7); 4.0267 (4.6); 4.0161 (1.7); 4.0125 (2.4); 1.5684 (7.0); 1.2557 (0.5); −0.0002 (10.8); −0.0009 (10.1); −0.0083 (0.5) III-068: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.3990 (0.8); 7.3930 (0.8); 7.3776 (1.4); 7.3616 (1.0); 7.3561 (1.0); 7.3405 (0.7); 7.3108 (0.8); 7.2595 (56.5); 7.2116 (0.6); 7.1876 (0.9); 7.1825 (0.9); 7.1695 (1.3); 7.1627 (1.2); 7.1558 (1.0); 7.1495 (1.4); 7.1373 (0.9); 7.1251 (1.2); 7.1043 (0.8); 7.0424 (0.9); 7.0365 (1.0); 7.0314 (0.9); 7.0152 (0.8); 6.9953 (0.9); 6.9866 (1.8); 6.9677 (2.6); 6.9466 (1.6); 6.6319 (0.5); 5.9223 (0.5); 5.8968 (0.6); 5.8798 (0.7); 5.8670 (0.6); 5.8539 (0.6); 5.2631 (1.2); 5.2202 (1.1); 5.1851 (1.2); 5.1821 (1.3); 5.1565 (1.2); 4.8347 (8.3); 4.0253 (1.5); 4.0110 (2.6); 3.9969 (1.5); 1.5380 (16.0); −0.0002 (21.3) III-069: .sup.1H-NMR(400.0 MHz, CDCl3): δ = 7.4723 (0.6); 7.4569 (1.2); 7.4507 (1.1); 7.4414 (0.7); 7.4354 (2.3); 7.4293 (0.8); 7.4199 (1.1); 7.4138 (1.3); 7.3984 (0.6); 7.2612 (32.0); 7.2350 (1.0); 7.2298 (1.0); 7.2168 (1.0); 7.2105 (1.6); 7.2043 (1.2); 7.1937 (1.2); 7.1914 (1.2); 7.1860 (1.1); 7.1727 (1.7); 7.1695 (1.1); 7.1531 (1.6); 7.1482 (1.7); 7.1287 (1.4); 7.0892 (0.8); 7.0852 (1.1); 7.0796 (1.2); 7.0751 (1.2); 7.0701 (0.9); 7.0637 (0.8); 7.0584 (0.8); 7.0536 (0.8); 7.0101 (3.0); 6.9918 (4.4); 6.9885 (4.4); 6.9703 (3.0); 5.9519 (0.6); 5.9381 (1.3); 5.9259 (0.8); 5.9123 (1.5); 5.9090 (0.8); 5.8985 (0.8); 5.8952 (1.6); 5.8817 (1.0); 5.8694 (1.6); 5.8556 (0.7); 5.3019 (1.0); 5.2979 (3.3); 5.2949 (2.3); 5.2907 (1.0); 5.2590 (0.8); 5.2549 (1.9); 5.2519 (1.9); 5.2477 (0.9); 5.2151 (1.1); 5.2117 (2.5); 5.2085 (2.3); 5.2051 (1.0); 5.1894 (1.0); 5.1859 (2.3); 5.1827 (2.2); 5.1793 (0.9); 4.8934 (16.0); 4.0443 (1.4); 4.0405 (2.3); 4.0367 (1.6); 4.0300 (2.7); 4.0263 (4.3); 4.0226 (2.6); 4.0160 (1.6); 4.0121 (2.3); 4.0083 (1.3); 1.5740 (7.8); −0.0002 (11.3)

B. Formulation Examples

[0598] a) A dusting product is obtained by mixing 10 parts by weight of a compound of the formula (I) and/or salts thereof and 90 parts by weight of talc as inert substance and comminuting the mixture in an impact mill.

[0599] b) A readily water-dispersible, wettable powder is obtained by mixing 25 parts by weight of a compound of the formula (I) and/or salts thereof, 64 parts by weight of kaolin-containing quartz as inert substance, 10 parts by weight of potassium lignosulfonate and 1 part by weight of sodium oleoylmethyltaurate as wetting agent and dispersant and grinding in a pinned-disc mill.

[0600] c) A readily water-dispersible dispersion concentrate is obtained by mixing 20 parts by weight of a compound of the formula (I) and/or salts thereof with 6 parts by weight of alkylphenol polyglycol ether (®Triton X 207), 3 parts by weight of isotridecanol polyglycol ether (8 EO) and 71 parts by weight of paraffinic mineral oil (boiling range e.g. about 255 to more than 277° C.) and grinding to a fineness of below 5 microns in an attrition ball mill.

[0601] d) An emulsifiable concentrate is obtained from 15 parts by weight of a compound of the formula (I) and/or salts thereof, 75 parts by weight of cyclohexanone as solvent and 10 parts by weight of oxethylated nonylphenol as emulsifier.

[0602] e) Water-dispersible granules are obtained by mixing

[0603] 75 parts by weight of a compound of the formula (I) and/or salts thereof,

[0604] 10 parts by weight of calcium lignosulfonate,

[0605] 5 parts by weight of sodium lauryl sulfate,

[0606] 3 parts by weight of polyvinyl alcohol and

[0607] 7 parts by weight of kaolin,

[0608] grinding the mixture in a pinned-disc mill, and granulating the powder in a fluidized bed by spray application of water as a granulating liquid.

[0609] f) Water-dispersible granules are also obtained by homogenizing and precomminuting, in a colloid mill,

[0610] 25 parts by weight of a compound of the formula (I) and/or salts thereof,

[0611] 5 parts by weight of sodium 2,2′-dinaphthylmethane-6,6′-disulfonate,

[0612] 2 parts by weight of sodium oleoylmethyltaurate,

[0613] 1 part by weight of polyvinyl alcohol,

[0614] 17 parts by weight of calcium carbonate and

[0615] 50 parts by weight of water,

[0616] then grinding the mixture in a bead mill and atomizing and drying the resulting suspension in a spray tower by means of a one-phase nozzle.

C. Biological Examples

[0617] 1. Pre-Emergence Herbicidal Action and Crop Plant Compatibility

[0618] Seeds of mono- and dicotyledonous weed plants are placed in plastic pots in sandy loam soil (doubly sown with one species each of mono- or dicotyledonous weed plants per pot) and covered with soil. The compounds of the invention, formulated in the form of wettable powders (WP) or as emulsion concentrates (EC), are then applied onto the surface of the covering soil as aqueous suspension or emulsion with addition of 0.5% additive at a water application rate equivalent to 600 litres per hectare. After the treatment, the pots are placed in a greenhouse and kept under good growth conditions for the trial plants. After about 3 weeks, the effect of the preparations is scored visually in comparison with untreated controls as percentages. For example, 100% activity=the plants have died, 0% activity=like control plants.

[0619] In Tables 4.1-4.15 and 5.1-5.16 below, the following abbreviations are used:

TABLE-US-00005 ALOMY: Alopecurus myosuroides AMARE: Amaranthus retroflexus AVEFA: Avena fatua CYPES: Cyperus esculentus ECHCG: Echinochloa crus-galli HORMU: Hordeum murinum LOLRI: Lolium rigidum MATIN: Matricaria inodora PHBPU: Pharbitis purpurea POLCO: Polygonum convolvulus SETVI: Setaria viridis STEME: Stellaria media VERPE: Veronica persica VIOTR: Viola tricolor

[0620] Tables 4.1-4.15 below show the effects of selected compounds of the general formula (I) according to Tables 1 to 3 on various harmful plants at an application rate corresponding to 1280 or 320 g/ha, which have been obtained by the aforementioned experimental method.

TABLE-US-00006 TABLE 4.1 Pre-emergence action at 1280 g/ha against ALOMY in % Ex. Dosage No. [g/ha] ALOMY I-002 1280 80 I-007 1280 80 I-008 1280 100 I-056 1280 90 I-057 1280 90 I-061 1280 90 I-067 1280 90 I-070 1280 90 I-072 1280 80

TABLE-US-00007 TABLE 4.2 Pre-emergence action at 1280 g/ha against CYPES in % Ex. Dosage No. [g/ha] CYPES I-003 1280 100 I-006 1280 100 I-012 1280 100 I-021 1280 100 I-022 1280 100 I-056 1280 90 I-061 1280 90 I-067 1280 90 I-070 1280 80

TABLE-US-00008 TABLE 4.3 Pre-emergence action at 1280 g/ha against ECHCG in % Ex. Dosage No. [g/ha] ECHCG I-011 1280 80 I-022 1280 80 I-054 1280 90 I-055 1280 100 I-057 1280 80 I-061 1280 90 I-067 1280 80 I-069 1280 80 I-070 1280 90 I-076 1280 90 I-079 1280 90 I-081 1280 90 I-085 1280 100 I-093 1280 100 I-097 1280 100 I-098 1280 100 I-100 1280 100 I-101 1280 100 I-102 1280 100 I-107 1280 100 I-111 1280 100 I-114 1280 90 I-120 1280 90 I-121 1280 100 I-122 1280 100 I-125 1280 100 I-130 1280 100 I-131 1280 100 I-133 1280 90 I-134 1280 100 I-136 1280 100 I-137 1280 100 I-138 1280 100 I-139 1280 100 I-140 1280 90 I-141 1280 100 I-142 1280 100 I-145 1280 100 I-164 1280 100 I-167 1280 100 I-168 1280 90 I-169 1280 100 I-171 1280 90 II-04 1280 100 III-001 1280 90 III-003 1280 100 III-004 1280 100 III-005 1280 100 III-006 1280 100 III-015 1280 100 III-016 1280 100 III-022 1280 100 III-023 1280 90 III-024 1280 90 III-027 1280 100 III-033 1280 90 III-053 1280 100 III-058 1280 90 III-067 1280 100 III-068 1280 100 III-069 1280 100

TABLE-US-00009 TABLE 4.4 Pre-emergence action at 1280 g/ha against SETVI in % Ex. Dosage No. [g/ha] SETVI I-008 1280 90 I-015 1280 90 I-022 1280 100 I-025 1280 80 I-036 1280 80 I-054 1280 90 I-055 1280 100 I-056 1280 100 I-057 1280 90 I-061 1280 100 I-063 1280 100 I-067 1280 100 I-069 1280 90 I-070 1280 90 I-072 1280 80 I-076 1280 100 I-078 1280 100 I-079 1280 100 I-081 1280 100 I-085 1280 100 I-086 1280 90 I-088 1280 90 I-091 1280 90 I-092 1280 100 I-093 1280 100 I-094 1280 100 I-095 1280 100 I-097 1280 100 I-098 1280 90 I-100 1280 100 I-101 1280 100 I-102 1280 100 I-107 1280 90 I-108 1280 100 I-111 1280 90 I-114 1280 100 I-118 1280 90 I-119 1280 100 I-120 1280 100 I-121 1280 100 I-123 1280 90 I-124 1280 100 I-125 1280 100 I-126 1280 100 I-127 1280 100 I-129 1280 100 I-130 1280 100 I-131 1280 100 I-132 1280 100 I-133 1280 100 I-134 1280 100 I-136 1280 100 I-137 1280 100 I-138 1280 100 I-139 1280 100 I-140 1280 100 I-141 1280 100 I-142 1280 100 I-143 1280 100 I-144 1280 100 I-145 1280 100 I-156 1280 90 I-164 1280 100 I-165 1280 100 I-166 1280 90 I-167 1280 100 I-169 1280 100 I-170 1280 100 I-171 1280 100 III-001 1280 100 III-003 1280 100 III-004 1280 100 III-005 1280 100 III-006 1280 100 III-015 1280 100 III-016 1280 100 III-017 1280 100 III-018 1280 90 III-019 1280 100 III-022 1280 100 III-023 1280 100 III-024 1280 100 III-026 1280 90 III-027 1280 90 III-033 1280 100 III-053 1280 100 III-054 1280 90 III-056 1280 90 III-058 1280 90 III-066 1280 90 III-067 1280 100 III-068 1280 100 III-069 1280 100

TABLE-US-00010 TABLE 4.5 Pre-emergence action at 1280 g/ha against AMARE in % Ex. Dosage No. [g/ha] AMARE I-002 1280 100 I-003 1280 100 I-004 1280 90 I-006 1280 100 I-007 1280 100 I-008 1280 100 I-011 1280 90 I-012 1280 100 I-015 1280 90 I-016 1280 100 I-021 1280 100 I-022 1280 100 I-023 1280 90 I-025 1280 90 I-026 1280 80 I-036 1280 80 I-046 1280 90 I-051 1280 90 I-054 1280 100 I-055 1280 100 I-056 1280 100 I-057 1280 100 I-061 1280 100 I-063 1280 80 I-066 1280 100 I-067 1280 100 I-069 1280 90 I-070 1280 100 I-072 1280 90 I-076 1280 100 I-078 1280 90 I-079 1280 100 I-081 1280 100 I-085 1280 100 I-086 1280 100 I-088 1280 90 I-091 1280 100 I-092 1280 100 I-093 1280 100 I-094 1280 100 I-095 1280 100 I-097 1280 100 I-098 1280 100 I-099 1280 90 I-100 1280 100 I-101 1280 90 I-102 1280 100 I-107 1280 90 I-108 1280 90 I-112 1280 100 I-114 1280 100 I-118 1280 100 I-119 1280 100 I-120 1280 100 I-121 1280 90 I-122 1280 100 I-123 1280 100 I-125 1280 100 I-126 1280 100 I-127 1280 100 I-128 1280 100 I-129 1280 100 I-130 1280 100 I-131 1280 100 I-132 1280 100 I-133 1280 100 I-134 1280 100 I-136 1280 100 I-137 1280 100 I-138 1280 100 I-139 1280 100 I-140 1280 90 I-141 1280 100 I-142 1280 100 I-143 1280 100 I-144 1280 100 I-145 1280 90 I-155 1280 90 I-156 1280 100 I-164 1280 100 I-165 1280 100 I-166 1280 90 I-167 1280 100 I-168 1280 100 I-169 1280 100 I-170 1280 100 I-171 1280 100 II-04 1280 100 II-06 1280 90 II-07 1280 90 II-09 1280 90 II-13 1280 100 II-14 1280 100 III-003 1280 100 III-004 1280 100 III-005 1280 90 III-006 1280 90 III-015 1280 100 III-016 1280 100 III-017 1280 100 III-018 1280 90 III-019 1280 90 III-022 1280 90 III-023 1280 90 III-024 1280 100 III-026 1280 90 III-027 1280 100 III-029 1280 90 III-033 1280 90 III-053 1280 90 III-054 1280 90 III-056 1280 100 III-058 1280 100 III-066 1280 90 III-067 1280 100 III-068 1280 90 III-069 1280 90

TABLE-US-00011 TABLE 4.6 Pre-emergence action at 320 g/ha against AMARE in % Ex. No. Dosage [g/ha] AMARE I-002 320 100 I-003 320 100 I-006 320 80 I-007 320 80 I-008 320 100 I-012 320 100 I-014 320 100 I-015 320 90 I-021 320 100 I-022 320 100 I-023 320 90 I-025 320 90 I-046 320 90 I-047 320 90 I-054 320 100 I-054 320 100 I-055 320 100 I-056 320 80 I-057 320 100 I-057 320 90 I-061 320 90 I-064 320 100 I-067 320 90 I-069 320 90 I-070 320 100 I-072 320 80 I-079 320 80 I-081 320 80 I-082 320 90 I-100 320 100 I-101 320 90 I-102 320 90 I-125 320 100 I-130 320 100 I-137 320 90 I-139 320 100 I-141 320 90 I-165 320 90 III-003 320 100 III-004 320 80 III-006 320 90 HI-069 320 100

TABLE-US-00012 TABLE 4.7 Pre-emergence action at 1280 g/ha against MATIN in % Ex. No. Dosage [g/ha] MATIN I-002 1280 100 I-003 1280 100 I-008 1280 90 I-012 1280 100 I-015 1280 90 I-016 1280 90 I-021 1280 90 I-022 1280 90 I-023 1280 100 I-026 1280 90 I-046 1280 90 I-048 1280 80 I-056 1280 90 I-057 1280 100 I-061 1280 90 I-067 1280 90 I-069 1280 90 I-070 1280 90 I-072 1280 80

TABLE-US-00013 TABLE 4.8 Pre-emergence action at 1280 g/ha against AVEFA in % Ex. No. Dosage [g/ha] AVEFA I-056 1280 80 I-057 1280 80 I-067 1280 80

TABLE-US-00014 TABLE 4.9 Pre-emergence action at 1280 g/ha against PHBPU in % Ex. No. Dosage [g/ha] PHBPU I-003 1280 80 I-015 1280 100 I-057 1280 90 I-061 1280 90 I-069 1280 80 I-070 1280 90 I-072 1280 90

TABLE-US-00015 TABLE 4.10 Pre-emergence action at 320 g/ha against POLCO in % Ex. No. Dosage [g/ha] POLCO I-001 320 90 I-008 320 80 I-054 320 100 I-055 320 90 I-056 320 80 I-057 320 90 I-064 320 100 I-070 320 80 I-072 320 90 I-075 320 80 I-079 320 80 I-081 320 100 I-082 320 80 I-101 320 100 I-102 320 100 I-125 320 100 I-130 320 90 I-137 320 100 I-139 320 90 III-003 320 100 III-006 320 90 III-015 320 90 III-069 320 90 320 90

TABLE-US-00016 TABLE 4.11 Pre-emergence action at 1280 g/ha against STEME in % Ex. No. Dosage [g/ha] STEME I-002 1280 100 I-003 1280 100 I-006 1280 100 I-007 1280 90 I-008 1280 100 I-015 1280 90 I-016 1280 80 I-020 1280 80 I-021 1280 90 I-022 1280 90 I-054 1280 100 I-055 1280 100 I-056 1280 100 I-057 1280 100 I-061 1280 100 I-063 1280 80 I-067 1280 90 I-069 1280 90 I-070 1280 90 I-072 1280 90 I-076 1280 100 I-079 1280 100 I-081 1280 100 I-086 1280 90 I-088 1280 100 I-092 1280 100 I-093 1280 100 I-094 1280 100 I-095 1280 100 I-097 1280 100 I-098 1280 100 I-100 1280 100 I-101 1280 100 I-102 1280 90 I-107 1280 100 I-109 1280 100 I-111 1280 100 I-112 1280 100 I-114 1280 100 I-119 1280 100 I-120 1280 100 I-121 1280 100 I-123 1280 100 I-124 1280 100 I-125 1280 100 I-126 1280 100 I-127 1280 100 I-128 1280 90 I-129 1280 100 I-130 1280 100 I-132 1280 100 I-133 1280 100 I-134 1280 100 I-135 1280 100 I-136 1280 100 I-137 1280 100 I-138 1280 100 I-139 1280 100 I-140 1280 100 I-141 1280 90 I-142 1280 100 I-143 1280 90 I-145 1280 100 I-150 1280 100 I-155 1280 100 I-156 1280 100 I-164 1280 100 I-165 1280 100 I-166 1280 90 I-167 1280 100 I-168 1280 100 I-169 1280 100 I-170 1280 100 I-171 1280 100 II-04 1280 100 II-06 1280 90 II-07 1280 90 II-09 1280 100 II-13 1280 90 III-001 1280 100 III-003 1280 100 III-004 1280 100 III-005 1280 100 III-006 1280 100 III-008 1280 100 III-015 1280 100 III-016 1280 100 III-017 1280 100 III-018 1280 100 III-019 1280 100 III-022 1280 100 III-023 1280 100 III-024 1280 100 III-025 1280 100 III-027 1280 100 III-033 1280 100 III-053 1280 100 III-056 1280 100 III-058 1280 100 III-066 1280 90 III-067 1280 90 III-068 1280 90 III-069 1280 90

TABLE-US-00017 TABLE 4.12 Pre-emergence action at 320 g/ha against STEME in % Ex. No. Dosage [g/ha] STEME I-002 320 80 I-054 320 100 I-055 320 100 I-057 320 80 I-061 320 90 I-064 320 90 I-070 320 80 I-075 320 80 I-081 320 80 I-100 320 90 I-102 320 90 I-125 320 90 I-130 320 90 I-137 320 90 I-139 320 100 I-141 320 80 III-003 320 100 III-069 320 100

TABLE-US-00018 TABLE 4.13 Pre-emergence action at 1280 g/ha against VIOTR in % Ex. No. Dosage [g/ha] VIOTR I-021 1280 90 I-022 1280 90 I-046 1280 90 I-051 1280 90 I-056 1280 80 I-057 1280 100 I-061 1280 90 I-063 1280 100 I-066 1280 90 I-067 1280 100 I-069 1280 100 I-070 1280 90 I-072 1280 80

TABLE-US-00019 TABLE 4.14 Pre-emergence action at 320 g/ha against VERPE in % Ex. No. Dosage [g/ha] VERPE I-002 320 100 I-003 320 100 I-008 320 90 I-014 320 100 I-015 320 90 I-021 320 90 I-022 320 100 I-023 320 90 I-025 320 80 I-047 320 90 I-054 320 100 I-055 320 90 I-057 320 90 I-081 320 80 I-082 320 80 I-100 320 100 I-102 320 80 I-125 320 90 I-130 320 100 I-137 320 90 I-139 320 100 I-165 320 100 III-003 320 100 III-004 320 100 III-006 320 90 III-015 320 90 III-069 320 100

TABLE-US-00020 TABLE 4.15 Pre-emergence action at 320 g/ha against HORMU in % Ex. No. Dosage [g/ha] HORMU I-056 320 80 I-064 320 90 I-125 320 90 I-130 320 100 I-139 320 90 III-069 320 90

[0621] As the results show, inventive compounds, for example compound nos. I-002, I-003, I-008, I-021, I-022, I-056, I-057, I-061, I-067, I-069, I-070, I-072, I-121, I-125, I-138, I-139, II-013, III-003, III-022, III-027, III-053, III-069 and other compounds from tables 4.1-4.15, show good herbicidal efficacy against harmful plants in the case of pre-emergence treatment. For example, compounds no. I-008, I-056, I-057, I-061, I-067, I-070 and I-072 applied by the pre-emergence method have very good action (80% to 100% herbicidal action) against harmful plants such as Alopecurus myosuroides, Amaranthus retroflexus, Matricaria inodora, Polygonum convolvulus, Setaria viridis and Stellaria media at an application rate of 1.28 kg of active substance or less per hectare.

[0622] 2. Post-Emergence Herbicidal Action and Crop Plant Compatibility

[0623] Seeds of mono- and dicotyledonous weed plants are placed in plastic pots in sandy loam soil (twin sowing with one species each of mono- or dicotyledonous weed plants per pot), covered with soil and cultivated in a greenhouse under controlled growth conditions. 2 to 3 weeks after sowing, the test plants are treated at the one-leaf stage. The compounds of the invention, formulated in the form of wettable powders (WP) or as emulsion concentrates (EC), are applied to the green parts of the plants as aqueous suspension or emulsion with addition of 0.5% additive at a water application rate equivalent to 600 litres per hectare. After the test plants have been kept in the greenhouse under optimum growth conditions for about 3 weeks, the activity of the preparations is rated visually in comparison to untreated controls. For example, 100% activity=the plants have died, 0% activity=like control plants.

[0624] Tables 5.1-5.16 below show the effects of selected compounds of the general formula (I) according to Tables 1 to 3 on various harmful plants at an application rate corresponding to 1280 or 320 g/ha, which have been obtained by the aforementioned experimental method.

TABLE-US-00021 TABLE 5.1 Post-emergence action at 1280 g/ha against ALOMY in % Ex. No. Dosage [g/ha] ALOMY I-002 1280 80 I-006 1280 80 I-021 1280 80 I-022 1280 80 I-046 1280 80 I-051 1280 80 I-056 1280 90 I-057 1280 90 I-061 1280 90 I-067 1280 100 I-070 1280 80 I-072 1280 80

TABLE-US-00022 TABLE 5.2 Post-emergence action at 1280 g/ha against AVEFA in % Ex. No. Dosage [g/ha] AVEFA I-009 1280 80 I-012 1280 80 I-022 1280 80 I-025 1280 80 I-036 1280 80 I-051 1280 80 I-056 1280 90 I-057 1280 90

TABLE-US-00023 TABLE 5.3 Post-emergence action at 1280 g/ha against ECHCG in % Ex. No. Dosage [g/ha] ECHCG I-002 1280 80 I-003 1280 80 I-016 1280 80 I-021 1280 80 I-022 1280 80 I-054 1280 90 I-055 1280 100 I-061 1280 80 I-067 1280 90 I-070 1280 80 I-072 1280 80 I-079 1280 100 I-081 1280 90 I-093 1280 100 I-097 1280 100 I-098 1280 100 I-100 1280 90 I-107 1280 90 I-120 1280 90 I-123 1280 90 I-125 1280 90 I-126 1280 90 I-130 1280 100 I-136 1280 100 I-137 1280 100 I-141 1280 100 I-143 1280 100 I-164 1280 90 I-167 1280 90 I-169 1280 90 I-171 1280 100 III-003 1280 100 III-019 1280 90 III-022 1280 90 III-027 1280 90 III-053 1280 100

TABLE-US-00024 TABLE 5.4 Post-emergence action at 1280 g/ha against LOLRI in % Ex. No. Dosage [g/ha] LOLRI I-057 1280 80 I-067 1280 90 I-130 1280 90 I-171 1280 100

TABLE-US-00025 TABLE 5.5 Post-emergence action at 1280 g/ha against SETVI in % Ex. No. Dosage [g/ha] SETVI I-002 1280 80 I-006 1280 90 I-009 1280 80 I-016 1280 80 I-022 1280 80 I-054 1280 100 I-056 1280 80 I-061 1280 80 I-063 1280 80 I-072 1280 80 I-079 1280 100 I-081 1280 90 I-089 1280 100 I-097 1280 90 I-098 1280 90 I-125 1280 90 I-126 1280 90 I-137 1280 90 I-145 1280 90 I-164 1280 100 I-165 1280 90 I-169 1280 90 I-171 1280 100 III-001 1280 100 III-003 1280 100 III-019 1280 90 III-022 1280 100 III-023 1280 100 III-026 1280 100 III-027 1280 100 III-033 1280 100 III-053 1280 100 III-054 1280 100 III-058 1280 100 III-066 1280 100 III-067 1280 100 III-068 1280 90

TABLE-US-00026 TABLE 5.6 Post-emergence action at 1280 g/ha against AMARE in % Ex. Dosage No. [g/ha] AMARE I-002 1280 90 I-003 1280 80 I-004 1280 80 I-005 1280 80 I-006 1280 100 I-007 1280 80 I-008 1280 80 I-009 1280 80 I-012 1280 80 I-015 1280 80 I-016 1280 80 I-021 1280 80 I-022 1280 80 I-023 1280 80 I-025 1280 80 I-026 1280 80 I-027 1280 80 I-038 1280 90 I-046 1280 80 I-054 1280 100 I-055 1280 90 I-056 1280 80 I-057 1280 80 I-061 1280 80 I-069 1280 90 I-070 1280 80 I-072 1280 80 I-076 1280 100 I-078 1280 100 I-079 1280 100 I-081 1280 100 I-085 1280 100 I-086 1280 100 I-088 1280 100 I-089 1280 100 I-091 1280 100 I-092 1280 100 I-093 1280 100 I-094 1280 100 I-095 1280 100 I-098 1280 100 I-099 1280 90 I-100 1280 90 I-101 1280 100 I-102 1280 90 I-107 1280 100 I-109 1280 100 I-111 1280 100 I-114 1280 100 I-119 1280 100 I-123 1280 90 I-125 1280 90 I-126 1280 100 I-127 1280 90 I-128 1280 90 I-129 1280 100 I-130 1280 90 I-133 1280 90 I-134 1280 90 I-136 1280 90 I-137 1280 90 I-141 1280 90 I-143 1280 100 I-156 1280 100 I-164 1280 100 I-165 1280 100 I-166 1280 100 I-169 1280 100 I-170 1280 90 I-171 1280 90 III-001 1280 100 III-003 1280 100 III-004 1280 100 III-006 1280 100 III-016 1280 90 III-017 1280 100 III-018 1280 100 III-019 1280 100 III-022 1280 90 III-025 1280 90 III-026 1280 90 III-027 1280 90 III-033 1280 90 III-058 1280 90

TABLE-US-00027 TABLE 5.7 Post-emergence action at 320 g/ha against AMARE in % Ex. Dosage No. [g/ha] AMARE I-002 320 80 I-005 320 80 I-008 320 80 I-012 320 80 I-014 320 80 I-015 320 80 I-021 320 80 I-022 320 80 I-025 320 80 I-047 320 80 I-054 320 90 I-055 320 90 I-056 320 80 I-057 320 80 I-061 320 80 I-079 320 80 I-081 320 90 I-082 320 80 I-100 320 80 I-101 320 80 I-102 320 80 I-125 320 90 I-130 320 90 I-137 320 80 I-139 320 90 I-141 320 90 III-003 320 80 III-004 320 80 III-006 320 80 III-015 320 80 III-069 320 90

TABLE-US-00028 TABLE 5.8 Post-emergence action at 1280 g/ha against MATIN in % Ex. Dosage No. [g/ha] MATIN I-002 1280 80 I-003 1280 80 I-006 1280 80 I-008 1280 90 I-011 1280 90 I-015 1280 90 I-021 1280 80 I-022 1280 80 I-023 1280 80 I-025 1280 80 I-036 1280 80 I-038 1280 80 I-046 1280 80 I-051 1280 90 I-054 1280 100 I-055 1280 100 I-056 1280 80 I-057 1280 90 I-063 1280 80 I-066 1280 80 I-067 1280 80 I-070 1280 80 I-072 1280 80 I-076 1280 90 I-079 1280 100 I-081 1280 100 I-085 1280 90 I-088 1280 90 I-093 1280 100 I-095 1280 100 I-097 1280 100 I-098 1280 90 I-100 1280 90 I-101 1280 90 I-102 1280 100 I-107 1280 100 I-111 1280 90 I-114 1280 90 I-119 1280 90 I-120 1280 90 I-121 1280 90 I-123 1280 90 I-124 1280 90 I-125 1280 90 I-127 1280 90 I-129 1280 100 I-130 1280 90 I-131 1280 90 I-132 1280 90 I-133 1280 90 I-136 1280 90 I-137 1280 90 I-139 1280 90 I-141 1280 90 I-142 1280 90 I-143 1280 100 I-145 1280 90 I-156 1280 90 I-164 1280 100 I-165 1280 100 I-166 1280 100 I-168 1280 90 I-169 1280 90 I-171 1280 90 II-13 1280 100 III-019 1280 90 III-026 1280 90 III-027 1280 100 III-053 1280 90 III-056 1280 90 III-058 1280 100 III-067 1280 90 III-068 1280 90

TABLE-US-00029 TABLE 5.9 Post-emergence action at 320 g/ha against MATIN in % Ex. Dosage No. [g/ha] MATIN I-003 320 80 I-008 320 90 I-011 320 90 I-015 320 90 I-022 320 80 I-036 320 80 I-047 320 80 I-051 320 90 I-054 320 90 I-056 320 80 I-057 320 80 I-064 320 80 I-066 320 80 I-075 320 80 I-079 320 80 I-081 320 80 I-082 320 80 I-100 320 80 I-101 320 90 I-102 320 80 I-125 320 80 I-130 320 90 I-137 320 80 I-139 320 80 I-141 320 80 III-069 320 80

TABLE-US-00030 TABLE 5.10 Post-emergence action at 320 g/ha against PHBPU in % Ex. Dosage No. [g/ha] PHBPU I-002 320 80 I-003 320 80 I-004 320 80 I-005 320 80 I-006 320 80 I-012 320 80 I-014 320 80 I-015 320 80 I-016 320 80 I-021 320 80 I-023 320 80 I-026 320 90 I-029 320 80 I-036 320 80 I-038 320 80 I-046 320 80 I-047 320 80 I-051 320 80 I-054 320 100 I-055 320 80 I-056 320 80 I-057 320 90 I-061 320 80 I-064 320 80 I-066 320 90 I-069 320 80 I-070 320 90 I-075 320 90 I-079 320 90 I-081 320 90 I-082 320 90 I-100 320 90 I-101 320 90 I-102 320 90 I-125 320 80 I-137 320 90 I-165 320 80 III-003 320 80 III-004 320 80 III-006 320 80 III-015 320 80

TABLE-US-00031 TABLE 5.11 Post-emergence action at 320 g/ha against POLCO in % Ex. Dosage No. [g/ha] POLCO I-004 320 80 I-008 320 80 I-011 320 80 I-014 320 80 I-022 320 80 I-051 320 80 I-054 320 80 I-055 320 80 I-056 320 80 I-057 320 80 I-061 320 80 I-064 320 80 I-075 320 80 I-079 320 80 I-081 320 80 I-100 320 90 I-125 320 80 I-130 320 90 I-137 320 90 I-139 320 90 I-165 320 80 III-004 320 80 III-015 320 80 III-069 320 80

TABLE-US-00032 TABLE 5.12 Post-emergence action at 1280 g/ha against STEME in % Ex. Dosage No. [g/ha] STEME I-002 1280 90 I-003 1280 80 I-006 1280 80 I-008 1280 90 I-011 1280 80 I-012 1280 80 I-016 1280 80 I-021 1280 80 I-022 1280 80 I-023 1280 80 I-036 1280 80 I-046 1280 80 I-051 1280 80 I-054 1280 100 I-055 1280 100 I-056 1280 90 I-057 1280 90 I-061 1280 80 I-067 1280 90 I-069 1280 80 I-070 1280 90 I-072 1280 80 I-079 1280 100 I-081 1280 100 I-085 1280 100 I-088 1280 100 I-093 1280 100 I-097 1280 100 I-098 1280 90 I-100 1280 90 I-102 1280 100 I-107 1280 90 I-109 1280 90 I-111 1280 90 I-119 1280 90 I-121 1280 100 I-125 1280 90 I-126 1280 100 I-130 1280 100 I-131 1280 90 I-132 1280 100 I-133 1280 100 I-134 1280 100 I-136 1280 100 I-137 1280 100 I-138 1280 100 I-139 1280 90 I-140 1280 100 I-141 1280 90 I-142 1280 100 I-143 1280 100 I-145 1280 100 I-150 1280 100 I-164 1280 100 I-165 1280 100 I-167 1280 100 I-168 1280 100 I-169 1280 100 I-170 1280 100 I-171 1280 100 II-04 1280 100 II-06 1280 100 II-08 1280 90 II-09 1280 100 III-008 1280 100 III-022 1280 100 III-025 1280 100 III-027 1280 90 III-053 1280 100 III-058 1280 100 III-067 1280 100

TABLE-US-00033 TABLE 5.13 Post-emergence action at 320 g/ha against STEME in % Ex. Dosage No. [g/ha] STEME I-002 320 80 I-003 320 80 I-008 320 90 I-012 320 80 I-014 320 80 I-021 320 80 I-022 320 80 I-023 320 80 I-036 320 80 I-046 320 80 I-047 320 80 I-054 320 90 I-055 320 80 I-057 320 80 I-064 320 90 I-067 320 80 I-081 320 80 I-100 320 80 I-130 320 90 I-137 320 90 I-139 320 80 I-141 320 90 III-069 320 90

TABLE-US-00034 TABLE 5.14 Post-emergence action at 320 g/ha against VIOTR in % Ex. Dosage No. [g/ha] VIOTR I-005 320 80 I-012 320 80 I-023 320 80 I-025 320 80 I-026 320 80 I-036 320 80 I-046 320 80 I-047 320 90 I-051 320 90 I-054 320 90 I-055 320 100 I-061 320 80 I-063 320 90 I-064 320 100 I-066 320 80 I-067 320 80 I-075 320 100 I-079 320 100 I-081 320 100 I-082 320 100 I-100 320 100 I-101 320 100 I-102 320 90 I-125 320 90 I-130 320 90 I-137 320 80 I-139 320 80 I-141 320 90 I-165 320 80 III-006 320 80 III-015 320 80

TABLE-US-00035 TABLE 5.15 Post-emergence action at 320 g/ha against VERPE in % Ex. Dosage No. [g/ha] VERPE I-002 320 80 I-007 320 90 I-008 320 90 I-011 320 80 I-015 320 90 I-022 320 80 I-025 320 80 I-029 320 80 I-036 320 80 I-038 320 80 I-046 320 80 I-047 320 80 I-048 320 80 I-051 320 80 I-054 320 80 I-055 320 80 I-056 320 90 I-057 320 80 I-075 320 80 I-079 320 80 I-081 320 80 I-082 320 80 I-100 320 90 I-101 320 80 I-102 320 80 I-125 320 80 I-130 320 90 I-137 320 90 I-165 320 80 III-003 320 80 III-006 320 80 III-015 320 90 III-069 320 90

TABLE-US-00036 TABLE 5.16 Post-emergence action at 320 g/ha against HORMU in % Ex. Dosage No. [g/ha] HORMU I-055 320 80 I-057 320 80 I-064 320 90 I-067 320 80 I-075 320 80 I-125 320 90 I-130 320 80 I-137 320 80 I-139 320 80 I-141 320 80 III-069 320 80

[0625] As the results from Tables 5.1-5.16 show, compounds of the invention have good herbicidal post-emergence efficacy against a broad spectrum of weed grasses and weeds.

[0626] As the results show, compounds of the invention, for example compound Nos. I-002, I-003, I-006, I-014, 1-021, 1-054, 1-072, 11-04, 111-058 and other compounds from Tables 5.1-5.16, when applied post-emergence, have very good herbicidal efficacy against harmful plants. For example, compounds Nos. I-002, I-006, I-022, I-056 and I-072 applied by the post-emergence method have very good herbicidal action (80% to 100% herbicidal action) against harmful plants such as Alopecurus myosuroides, Amaranthus retroflexus, Matricaria inodora, Setaria viridis, Pharbitis purpurea and Stellaria media at an application rate of 1.28 kg of active substance or less per hectare.