A method of curing a low Ca/Mg cement composition is described that includes providing a predetermined quantity of the low Ca/Mg cement composition in uncured form; and reacting the uncured low Ca/Mg cement composition with a reagent chemical for a time sufficient to cure said cementitious material, wherein said reagent chemical is a compound synthesized from CO.sub.2 and comprises dicarboxylic acids, tricarboxylic acids, or alpha-hydroxycarboxylic acids.

Disclosed is a magnesium-based cementitious material, preparation method and application thereof. The magnesium-based cementitious material, comprising magnesite, sandstone, and water, wherein: the magnesite is provided with CaO, SiO.sub.2, Al.sub.2O.sub.3, Fe.sub.2O.sub.3, and MgO, a mass percentage of the CaO is less than 5%, a mass percentage of SiO.sub.2 is less than 5%, a mass percentage of Al.sub.2O.sub.3 is less than 5%, a mass percentage of Fe.sub.2O.sub.3 is less than 7%, a mass percentage of MgO is between 37% and 50%; the sandstone is provided with SiO.sub.2, CaO, Al.sub.2O.sub.3, and Fe.sub.2O.sub.3, a mass percentage of SiO.sub.2 is greater than 70%. The beneficial effects of this disclosure are: the cementitious material does not contain MgCl.sub.2, which avoids the reduction of the strength of the cementitious material due to the dissolution of MgCl.sub.2 in water; the magnesium-based cementitious material of this disclosure is immiscible with water and has strong water resistance.

Disclosed is a magnesium-based cementitious material, preparation method and application thereof. The magnesium-based cementitious material, comprising magnesite, sandstone, and water, wherein: the magnesite is provided with CaO, SiO.sub.2, Al.sub.2O.sub.3, Fe.sub.2 O.sub.3, and MgO, a mass percentage of the CaO is less than 5%, a mass percentage of SiO.sub.2 is less than 5%, a mass percentage of Al.sub.2 O.sub.3 is less than 5%, a mass percentage of Fe.sub.2 O.sub.3 is less than 7%, a mass percentage of MgO is between 37% and 50%; the sandstone is provided with SiO.sub.2, CaO, Al.sub.2 O.sub.3, and Fe.sub.2O.sub.3, a mass percentage of SiO.sub.2 is greater than 70%. The beneficial effects of this disclosure are: the cementitious material does not contain MgCl.sub.2, which avoids the reduction of the strength of the cementitious material due to the dissolution of MgCl.sub.2 in water; the magnesium-based cementitious material of this disclosure is immiscible with water and has strong water resistance.

The invention provides novel methods and novel additive compositions and use thereof in a wide range of concrete production for improving properties of concrete materials, such as durability and aestheticity. The methods and compositions of the invention may be applied in a variety of cement and concrete components in the infrastructure, construction, pavement and landscaping industries.

An ozonation-based method for producing a cementitious material comprises the steps of: (1) mixing a flue gas with an ozone-containing gas to form a mixed flue gas; and introducing the mixed flue gas into an absorption tower, where the mixed flue gas undergoes dry desulfurization and denitrification by reacting with a powdered desulfurizing and denitrificating agent and becomes a treated flue gas; (2) subjecting the treated flue gas to dust removal to generate by-products; and (3) uniformly mixing raw materials that comprise the first by-product, magnesium oxide, fly ash and an additive to give a cementitious material, wherein on the basis of 100 parts by weight of the cementitious material, the first by-product is 20-60 parts by weight, magnesium oxide is 16-33 parts by weight, the fly ash is 15-35 parts by weight, and the additive is 1-15 parts by weight.

Herein discloses a method of carbonating reactive magnesia cement, which includes: (i) providing an aqueous suspension including a carbon dioxide-producing bacteria; (ii) mixing the aqueous suspension with a precursor which the carbon dioxide-producing bacteria generates carbon dioxide from for a duration to form an aqueous mixture sufficient for substantially carbonating the reactive magnesia cement; (iii) mixing the aqueous mixture with the reactive magnesia cement to form a blend; wherein a nutrient is provided in the aqueous suspension of step (i) or in the reactive magnesia cement of step (iii) to sustain the carbon dioxide-producing bacteria in the reactive magnesia cement; and (iv) curing the blend to carbonate the reactive magnesia cement. A reactive magnesia cement composite formed by the method is also disclosed.

Herein discloses a method of carbonating reactive magnesia cement, which includes: (i) providing an aqueous suspension including a carbon dioxide-producing bacteria; (ii) mixing the aqueous suspension with a precursor which the carbon dioxide-producing bacteria generates carbon dioxide from for a duration to form an aqueous mixture sufficient for substantially carbonating the reactive magnesia cement; (iii) mixing the aqueous mixture with the reactive magnesia cement to form a blend; wherein a nutrient is provided in the aqueous suspension of step (i) or in the reactive magnesia cement of step (iii) to sustain the carbon dioxide-producing bacteria in the reactive magnesia cement; and (iv) curing the blend to carbonate the reactive magnesia cement. A reactive magnesia cement composite formed by the method is also disclosed.

A downhole tool comprising a cylindrical housing, a sleeve disposed in the cylindrical housing, forming an annular space between the sleeve and the cylindrical housing, and a tool cement composition disposed in the annular space, wherein prior to setting the tool cement composition comprises a cement, sand, a silicon-containing material, a dispersant, and water, and wherein upon setting the tool cement composition provides an annular seal having a fluid leakage of less than 750 ml over 15 minutes at a pressure of 7500 psi and a temperature of 400° F.

A downhole tool comprising a cylindrical housing, a sleeve disposed in the cylindrical housing, forming an annular space between the sleeve and the cylindrical housing, and a tool cement composition disposed in the annular space, wherein prior to setting the tool cement composition comprises a cement, sand, a silicon-containing material, a dispersant, and water, and wherein upon setting the tool cement composition provides an annular seal having a fluid leakage of less than 750 ml over 15 minutes at a pressure of 7500 psi and a temperature of 400° F.

A downhole tool comprising a cylindrical housing, a sleeve disposed in the cylindrical housing, forming an annular space between the sleeve and the cylindrical housing, and a tool cement composition disposed in the annular space, wherein prior to setting the tool cement composition comprises a cement, sand, a silicon-containing material, a dispersant, and water, and wherein upon setting the tool cement composition provides an annular seal having a fluid leakage of less than 750 ml over 15 minutes at a pressure of 7500 psi and a temperature of 400° F.