The invention relates to a process for producing a composite comprising: a. providing a particulate material, wherein the particulate material comprises minerals having a content of at least 30% m/m of calcium, magnesium, aluminium, silicon, potassium or iron, or a combination of two or more thereof. b. providing an aggregate, c. providing a primary additive, wherein the primary additive comprises a sugar or derivative thereof, a polyol or derivative thereof, an organic acid, an organic acid salt or an inorganic acid, or any combination of two or more thereof, d. mixing the particulate material, the aggregate and the primary additive with water to form a mixture, and e. carbonating the mixture in the presence of carbon dioxide, wherein the concentration of carbon dioxide is greater than about 2 vol %.

The invention relates to a process for producing a composite comprising: a. providing a particulate material, wherein the particulate material comprises minerals having a content of at least 30% m/m of calcium, magnesium, aluminium, silicon, potassium or iron, or a combination of two or more thereof. b. providing an aggregate, c. providing a primary additive, wherein the primary additive comprises a sugar or derivative thereof, a polyol or derivative thereof, an organic acid, an organic acid salt or an inorganic acid, or any combination of two or more thereof, d. mixing the particulate material, the aggregate and the primary additive with water to form a mixture, and e. carbonating the mixture in the presence of carbon dioxide, wherein the concentration of carbon dioxide is greater than about 2 vol %.

A method of manufacturing a concrete product, includes: providing a composition including a binder, an aggregate, and water; mixing the binder, the aggregate, and the water to produce a concrete mixture; imparting a form to the concrete mixture to provide a formed intermediate having a first water-to-binder ratio; and concurrently conditioning and curing the formed intermediate by conditioning the formed intermediate while curing the formed intermediate, wherein the formed intermediate is concurrently cured and conditioned to obtain final water-to-binder ratio less than the first water-to-binder ratio.

A method for making a carbonated precast concrete product includes: obtaining a mixture including at least one binder material, an aggregate, and water; molding the mixture into a molded intermediate; demolding the molded intermediate to obtain a demolded intermediate, the demolded intermediate having a first water-to-binder ratio; conditioning the demolded intermediate to provide a conditioned article having a second water-to-binder ratio less than the first water-to-binder ratio of the demolded intermediate; moisturizing at least one surface of the conditioned article with an aqueous medium, thereby causing a weight gain of the conditioned article and providing a moisturized product, a first portion of the moisturized product having a third water-to-binder ratio greater than a fourth water-to-binder ratio of a remainder of the moisturized product; and curing the moisturized product with carbon dioxide to obtain the carbonated precast concrete product.

A method for making a carbonated precast concrete product includes: obtaining a mixture including at least one binder material, an aggregate, and water; molding the mixture into a molded intermediate; demolding the molded intermediate to obtain a demolded intermediate, the demolded intermediate having a first water-to-binder ratio; conditioning the demolded intermediate to provide a conditioned article having a second water-to-binder ratio less than the first water-to-binder ratio of the demolded intermediate; moisturizing at least one surface of the conditioned article with an aqueous medium, thereby causing a weight gain of the conditioned article and providing a moisturized product, a first portion of the moisturized product having a third water-to-binder ratio greater than a fourth water-to-binder ratio of a remainder of the moisturized product; and curing the moisturized product with carbon dioxide to obtain the carbonated precast concrete product.

A method of forming a concrete product includes directly capturing CO.sub.2 from a gas source, the capturing comprising contacting the gas source with an absorption solution having a solvent and a solute, wherein the solvent and/or the solute are capable of reacting with CO.sub.2 to form an anionic compound, adjusting the pH of the absorption solution electrochemically to less than about 7 to release the CO.sub.2 as a concentrated vapor containing CO.sub.2, collecting the concentrated vapor containing CO.sub.2, regenerating the solvent and/or the solute, and optionally collecting the regenerated solvent and/or solute; flowing the concentrated vapor containing CO.sub.2 through a gas processing unit to adjust at least one of a temperature, a relative humidity, or a flow rate of the concentrated vapor containing CO.sub.2; and contacting the concentrated vapor containing CO.sub.2 with a concrete component.

A method of forming a concrete product includes directly capturing CO.sub.2 from a gas source, the capturing comprising contacting the gas source with an absorption solution having a solvent and a solute, wherein the solvent and/or the solute are capable of reacting with CO.sub.2 to form an anionic compound, adjusting the pH of the absorption solution electrochemically to less than about 7 to release the CO.sub.2 as a concentrated vapor containing CO.sub.2, collecting the concentrated vapor containing CO.sub.2, regenerating the solvent and/or the solute, and optionally collecting the regenerated solvent and/or solute; flowing the concentrated vapor containing CO.sub.2 through a gas processing unit to adjust at least one of a temperature, a relative humidity, or a flow rate of the concentrated vapor containing CO.sub.2; and contacting the concentrated vapor containing CO.sub.2 with a concrete component.

A cement composition including a hydraulic cement material, a latent-hydraulic cement material, and a non-hydraulic cement material. Also provided is a method including combining, at a jobsite, the cement composition comprising the hydraulic cement material, the latent-hydraulic cement material, and the non-hydraulic cement material with water to provide a cement slurry, and allowing the cement slurry to harden in the presence of carbon dioxide (CO.sub.2) to provide a hardened cement.

A cement composition including a hydraulic cement material, a latent-hydraulic cement material, and a non-hydraulic cement material. Also provided is a method including combining, at a jobsite, the cement composition comprising the hydraulic cement material, the latent-hydraulic cement material, and the non-hydraulic cement material with water to provide a cement slurry, and allowing the cement slurry to harden in the presence of carbon dioxide (CO.sub.2) to provide a hardened cement.

Disclosed are composite materials comprising a porous, carbonated, calcium silicate ceramic having a microstructure comprising interconnected open pores; where the calcium silicate surface defining the pores is partially or completely coated with an amorphous silica layer, and the silica coating comprises an overlayer of calcium carbonate crystals; where the silica coating and calcium carbonate overlayer form a network that interconnects throughout the ceramic microstructure, but do not completely occlude the pores. Also disclosed are methods of forming such composite materials.