Disclosed are an R-T-B-based permanent magnet material, a preparation method therefor and the use thereof. The R-T-B-based permanent magnet material comprises R, B, M, Fe, Co, X and inevitable impurities, wherein: (1) R is a rare earth element, and the R includes at least Nd and RH, M being one or more of Ti, Zr and Nb, and X including Cu, “Al and/or Ga”; and (2) in percentage by weight, R: 30.5-32.0 wt%, B: 0.95-0.99 wt%, M: 0.3-0.6 wt%, X: 0.8-1.8 wt%, and Cu: 0.35-0.50 wt%, and the balance is Fe, Co and inevitable impurities. According to the present invention, under the condition of 0.3-0.6 wt% of a high melting point metal, a permanent magnet material with an excellent magnet performance and a good squareness is obtained.

A method for manufacturing an R-T-B based sintered magnet according the present disclosure comprises: a step for preparing a coarse ground powder which is made from an alloy for R-T-B based sintered magnets and which has an average particle size of 10-500 μm; a step for obtaining a fine powder having an average particle size of 2.0-4.5 μm, by feeding the coarse ground powder to a jet mill device that has a grinding chamber filled with inert gas and grinding the coarse ground powder; and a step for producing a sintered body of the fine powder, wherein the inert gas has been humidified, and the oxygen content of the R-T-B based sintered magnet is 1000-3500 ppm by mass.

The present disclosure is directed at methods of preparing rare earth-based permanent magnets having improved coercivity and remanence, the method comprising one or more steps comprising: (a) homogenizing a first population of particles of a first GBM alloy with a second population of particles of a second core alloy to form a composite alloy preform, the first GBM alloy being substantially represented by the formula: AC.sub.bR.sub.xCo.sub.yCu.sub.dM.sub.z, the second core alloy being substantially represented by the formula G.sub.2Fe.sub.14B, where AC, R, M, G, b, x, y, and z are defined; (b) heating the composite alloy preform particles to form a population of mixed alloy particles; (c) compressing the mixed alloy particles, under a magnetic field of a suitable strength to align the magnetic particles with a common direction of magnetization and inert atmosphere, to form a green body; (d) sintering the green body; and (e) annealing the sintered body. Particular embodiments include magnets comprising neodymium-iron-boron core alloys, including Nd.sub.2Fe.sub.14B.

An R-T-B based permanent magnet in which R is a rare earth element, T is Fe and Co, and B is boron. R at least includes Dy. The R-T-B based permanent magnet includes M, and M is at least one or more elements selected from the group consisting of Cu, Ga, Al, Mn, Zr, Ti, Cr, Ni, Nb, Ag, Hf, Ta, W, Si, Bi, and Sn. M at least includes Cu. A total content of R is 28.0 mass % to 30.2 mass %, a content of Dy is 1.0 mass % to 6.5 mass %, a content of Cu is 0.04 mass % to 0.50 mass %, a content of Co is 0.5 mass % to 3.0 mass %, and a content of B is 0.85 mass % to 0.95 mass %.

The present disclosure is directed towards a method of manufacturing a permanent magnet such that the magnet defines a channel for allowing circulation of a coolant through the permanent magnet, or defines a channel for allowing circulation of the coolant through an interface between the permanent magnet and a substrate. Magnets made by this method may be useful for manufacturing and/or operating a machine, such as a motor, engine, or sensor.

The present invention provides a rare-earth sintered magnet that is characterized in that: R (R indicates one or more elements selected from rare-earth elements, wherein Nd is essential), T (T indicates one or more elements selected from iron-group elements, wherein Fe is essential), X (X indicates one or two elements selected from B and C, wherein B is essential), M.sup.1 (M.sup.1 indicates one or more elements selected from Al, Si, Cr, Mn, Cu, Zn, Ga, Ge, Mo, Sn, W, Pb, and Bi), 0.1 mass % or less of O, 0.05 mass % or less of N, and 0.07 mass % or less of C are contained; the average crystal grain size is 4.0 μm or less; and relational expression (1) 0.26×D+97≤Or≤0.26×D+99 is satisfied assuming that the degree of orientation is Or [%] and that the average crystal grain size is D [μm]. With this rare-earth sintered magnet, it is possible to achieve superior magnetic characteristics in which both high Br and high H.sub.cJ are achieved.

An R-T-B-based sintered magnet and a preparation method therefor. The R-T-B-based sintered magnet comprises: R, B, Ti, Ga, Al, Cu, and T. The contents thereof are as follows: R is 29.0-33%; the content of B is 0.86-0.93%; the content of Ti is 0.05-0.25%; the content of Ga is 0.3-0.5%, but not 0.5%; the content of Al is 0.6-1%, but not 0.6%; the content of Cu is 0.36-0.55%. The percentage is the mass percentage. Under the condition that no heavy rare earth is added or a small amount of heavy rare earth is added, by using a low B technology, not only the remanence performance of the R-T-B-based sintered magnet is improved, but also the coercivity and the squareness of the magnet are ensured.

Disclosed are a neodymium-iron-boron magnet material, a raw material composition, a preparation method therefor and a use thereof. The raw material composition of the neodymium-iron-boron magnet material comprises the following components in weight content: R: 28-33%; R being rare earth elements, and comprising R1 and R2, R1 being a rare earth element added during smelting, R1 comprising Nd and Dy, R2 being a rare earth element added during grain boundary diffusion, R2 comprising Tb, and the content of R2 being 0.2-1%; M: ≤0.4% but not 0, M being one or more elements among Bi, Sn, Zn, Ga, In, Au and Pb; Cu: ≤0.15% but not 0; B: 0.9-1.1%; Fe: 60-70%; but not containing Co. The neodymium-iron-boron magnet material under the condition of adding a small amount of heavy rare earth elements and not adding cobalt, can still have a relatively high coercivity and remanence, and excellent thermal stability.

The present invention relates to an R-T-B sintered magnet and a preparation method thereof. The sintered magnet includes a grain boundary region T1, a shell layer region T2 and an R.sub.2Fe.sub.14B grain region T3; at 10 μm to 60 μm from a surface of the sintered magnet toward a center thereof, an area ratio of the shell layer region T2 to the R.sub.2Fe.sub.14B grain region T3 is 0.1 to 0.3, and a thickness of the shell layer region T2 is 0.5 μm to 1.2 μm; and an average coating percent of the shell layer region T2 on the R.sub.2Fe.sub.14B grain region T3 is 80% or more. In the present invention, by optimizing a preparation process and a microstructure of a traditional rare earth permanent magnet, diffusion efficiency of heavy rare earth in the magnet is improved, such that coercivity of the magnet is greatly improved, and manufacturing cost is reduced.

Disclosed are a cerium magnet with diffused grain boundaries containing REFe2 and a preparation method therefor, wherein an original cerium magnet contains a 2-14-1 main phase, a REFe2 phase and a rare earth-rich phase, and the REFe 2 phase is a CeFe2 phase or a (Ce,RE′)Fe2 phase. The RE″ element in a rare earth diffusion source is diffused into the original cerium magnet by means of a grain boundary diffusion treatment at the melting point of the REFe2 phase, and same is then cooled directly or cooled after a tempering treatment to room temperature to obtain a final cerium magnet. The final cerium magnet contains a new 2-14-1 main phase, a new enhanced REFe2 phase and a new rare earth-rich phase, wherein the new 2-14-1 main phase is a (Ce,RE″)2Fe14B or (Ce,RE′,RE″)2Fe14B main phase, and the new enhanced REFe2 phase is a (CeRE″)Fe2 phase or a (Ce,RE′,RE″)Fe2 phase, wherein RE′ and RE″ are one or more of La, Pr, Nd, Pm, Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb, Lu and Y. The cerium magnet improves the diffusion efficiency of the element RE″ in the diffusion source, and substantially improve the coercivity thereof.