INTELLIGENT MULTI-POLLUTANT ULTRA-LOW EMISSION SYSTEM AND GLOBAL OPTIMIZATION METHOD THEREOF
20210319373 · 2021-10-14
Inventors
- XIANG GAO (HANGZHOU, ZHEJIANG PROVINCE, CN)
- CHENGHANG ZHENG (HANGZHOU, ZHEJIANG PROVINCE, CN)
- YUEQI HUANG (HANGZHOU, ZHEJIANG PROVINCE, CN)
- YISHAN GUO (HANGZHOU, ZHEJIANG PROVINCE, CN)
- YONGXIN ZHANG (HANGZHOU, ZHEJIANG PROVINCE, CN)
- WEIGUO WENG (HANGZHOU, ZHEJIANG PROVINCE, CN)
- WEIHONG WU (HANGZHOU, ZHEJIANG PROVINCE, CN)
- RUIYANG QU (HANGZHOU, ZHEJIANG PROVINCE, CN)
- SHAOJUN LIU (HANGZHOU, ZHEJIANG PROVINCE, CN)
- HAITAO ZHAO (HANGZHOU, ZHEJIANG PROVINCE, CN)
Cpc classification
B01D53/60
PERFORMING OPERATIONS; TRANSPORTING
B01D53/8665
PERFORMING OPERATIONS; TRANSPORTING
B01D2257/602
PERFORMING OPERATIONS; TRANSPORTING
B01D53/64
PERFORMING OPERATIONS; TRANSPORTING
B01D53/501
PERFORMING OPERATIONS; TRANSPORTING
G06F30/18
PHYSICS
B01D2257/404
PERFORMING OPERATIONS; TRANSPORTING
G06Q10/0631
PHYSICS
International classification
G06Q10/06
PHYSICS
B01D53/60
PERFORMING OPERATIONS; TRANSPORTING
B01D53/64
PERFORMING OPERATIONS; TRANSPORTING
Abstract
The invention relates to an intelligent multi-pollutant ultra-low emission system and a global optimization method thereof. The intelligent multi-pollutant ultra-low emission system comprises a device layer, a sensing layer, a control layer and an optimization layer from bottom to top. The global optimization method comprises: obtaining an accurate description multiple pollutants in the generation, migration, transformation and removal process in multiple devices by means of accurate modeling of a multi-device multi-pollutant simultaneous removal process of the ultra-low emission system; accurately evaluating multi-pollutant emission reduction costs under different loads, coal qualities, pollutant concentrations and operating parameters through a global operating cost evaluation method of the ultra-low emission system; realizing minute-level planning and optimization of emission reductions of a global pollutant emission reduction device under different emission targets through a multi-pollutant, multi-target and multi-condition global operating optimization method; and guaranteeing reliable emission reduction and margin control of the pollutants through an advanced control method for reliable up-to-standard ultra-low emission of the pollutants.
Claims
1. An intelligent multi-pollutant ultra-low emission system, comprising a device layer, a sensing layer, a control layer and an optimization layer from bottom to top, wherein the device layer comprises multiple key devices of the ultra-low emission system, including a desulfurization device, a denitration device and precipitators, and realizes efficient removal of pollutants through a series of physical and chemical reactions; the sensing layer is an information hub of the intelligent multi-pollutant ultra-low emission system and is used for acquiring, preprocessing, integrating, storing and issuing information by means of a pollutant online detection device, a distributed control system and other sensing and communication systems; the control layer is an intermediate layer for controlling key manipulated variables according to real-time operating conditions and optimized parameter settings to guarantee stable up-to-standard operation and optimal regulation of the system; the optimization layer is a key layer for realizing efficient simultaneous removal of multiple pollutants in the intelligent multi-pollutant ultra-low emission system, fulfills optimization of global set points by establishing an optimization model, a prediction model and a cost evaluation model, and has the functions of balancing emission reductions of all devices and optimizing global material and energy distributions of the ultra-low emission system; in the ultra-low emission system, a control information flow flows from top to bottom, and a feedback information flow flows from bottom to top.
2. The intelligent multi-pollutant ultra-low emission system according to claim 1, wherein information flows in the sensing layer, the control layer and the optimization layer adopt different time scales which are t, t* and t**, respectively, wherein, t represents a real-time scale mainly used for online monitoring and local control, t* represents a second scale (also referred to as control scale) mainly used for reception and feedback of second-level signals of the control layer, and t** represents a minute scale or a superior scale (also referred to as a global scale) mainly used for instruction optimization and allocation of the optimization layer.
3. A global optimization method of an intelligent multi-pollutant ultra-low emission system, comprising obtaining an accurate description of multiple pollutants in a generation, migration, transformation and removal of in multiple devices by means of accurate modeling of a multi-device multi-pollutant simultaneous removal process of an ultra-low emission system; accurately evaluating multi-pollutant emission reduction costs under different loads, coal qualities, pollutant concentrations and operating parameters through a global operating cost evaluation method of the ultra-low emission system; realizing minute-level planning and optimization of emission reductions of a global pollutant emission reduction device under different emission targets through a multi-pollutant, multi-target and multi-condition global operating optimization method; and guaranteeing reliable emission reduction and margin control of the pollutants through an advanced control method for reliable up-to-standard ultra-low emission of the pollutants.
4. The global optimization method of an intelligent multi-pollutant ultra-low emission system according to claim 3, wherein accurate modeling of the multi-device multi-pollutant simultaneous removal process of the ultra-low emission system includes accurate prediction of a multi-pollutant generation process, accurate modeling of a multi-pollutant simultaneous removal process of a desulfurization system, accurate modeling of a multi-pollutant simultaneous removal and transformation process of a denitration system, and accurate modeling of a multi-pollutant removal process of a precipitation system; accurate prediction of the multi-pollutant generation process: a boiler operating database and a multi-pollutant outlet concentration database under different conditions and variable coal qualities are established by acquiring long-term operating data of a boiler and a continuous emission monitoring system and combining coal quality detection data and test reports of the multiple pollutants including NO.sub.x, SO.sub.2, SO.sub.3, PM and Hg; and a model for describing a corresponding relationship of boiler parameters and coal quality parameters with the concentrations of the multiple pollutants at a boiler outlet under different coal qualities and loads is established based on the boiler operating database and the multi-pollutant outlet concentration database through a data modeling method; accurate modeling of the multi-pollutant simultaneous removal process of the desulfurization system: based on a generation, migration and transformation mechanism of the multiple pollutant as well as a removal mechanism of the multiple pollutants in the desulfurization system, a corresponding relationship of inlet SO.sub.2 concentration, inlet flue gas temperature, liquid-gas ratio, slurry density and pH with outlet SO.sub.2 concentration of the desulfurization system, a corresponding relationship of inlet SO.sub.3 concentration, inlet SO.sub.2 concentration, inlet dust content, inlet flue gas temperature, liquid-gas ratio and flue gas velocity with outlet SO.sub.3 concentration of the desulfurization system, and a corresponding relationship of inlet Hg concentration, inlet dust content, load, flue gas velocity and inlet flue gas temperature with outlet Hg concentration are established by combining coal qualities, boiler operating parameters, inlet flue gas parameters of the desulfurization system, and operating parameter historical data of the desulfurization system, and then, a model for accurately describing the multi-pollutant simultaneous removal process of the desulfurization system is obtained; accurate modeling of the multi-pollutant simultaneous removal and transformation process of the denitration system: based on an operating mechanism of an SCR denitration system, a corresponding relationship of inlet NO.sub.x, concentration, flue gas parameters, reaction condition and reducer supply with outlet NO.sub.x, concentration of the denitration system a corresponding relationship of inlet SO.sub.2 concentration, flue gas parameters, reaction condition and reducer supply with SO.sub.2-to-SO.sub.3 transformation rate in the denitration system, and a corresponding relationship of inlet Hg concentration, flue gas parameters, reaction condition and reducer supply with transformation ratio of particulate mercury, mercury oxides and elementary mercury in the denitration system are established by combining inlet flue gas parameters, online detection results of the CEMS and operating parameter historical data of the denitration system, and then, a model for accurately describing the multi-pollutant simultaneous removal and transformation process of the denitration system under different conditions and operating parameters is obtained based on these corresponding relationships; accurate modeling of the multi-pollutant removal process of the precipitation system: based on a particulate matter removal mechanism of an electrostatic precipitation system, a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, operating voltage and outlet particulate matter concentration of a dry electric precipitator, a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, theoretical SO.sub.3 concentration of the denitration system, operating voltage and outlet SO.sub.3 concentration of the dry electric precipitator, a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, theoretical Hg concentration of the denitration system and outlet Hg concentration of the dry electric precipitator, a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, circulating water quantity, operating voltage and outlet particulate matter concentration of a wet electric precipitator, a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, inlet NO.sub.x concentration, circulating water quantity, circulating water pH, operating voltage and outlet NO.sub.x concentration of the wet electric precipitator, a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, inlet SO.sub.2 concentration, circulating water quantity, circulating water pH, operating voltage and outlet SO.sub.2 concentration of the wet electric precipitator, a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, inlet SO.sub.3 concentration, circulating water quantity, circulating water pH, operating voltage and outlet SO.sub.3 concentration of the wet electric precipitator, and a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, inlet Hg concentration, circulating water quantity, circulating water pH, operating voltage and outlet Hg concentration of the wet electric precipitator are established by combining coal quality, boiler operating parameters, inlet flue gas parameters of the electrostatic precipitation system, and historical operating data; then, a model for accurately describing the multi-pollutant simultaneous removal process of the precipitation system is obtained.
5. The global optimization method of an intelligent multi-pollutant ultra-low emission system according to claim 4, wherein accurate prediction of the multi-pollutant generation process refers to accurate prediction of the concentration of the multiple pollutants, including NO.sub.x, SO.sub.2, SO.sub.3, PM and Hg at a boiler outlet according to real-time boiler operating data and periodically-updated coal quality reports; a boiler model is established through the following steps: S101: collecting boiler parameters, coal quality parameters and a boiler outlet test report; S102: collecting long-term operating historical data including boiler coal feed, flue gas, water, and boiler outlet pollutant concentrations detected by the CEMS; S103: marking out typical boiler load intervals according to the test report and online operating data, and obtaining corresponding datasets of boiler operating parameters, coal qualities and outlet pollutant concentrations in the typical boiler load intervals; S104: for pollutants, data of which is monitored online by the CEMS, obtaining a corresponding relationship of the boiler operating data and coal quality parameters with outlet pollutant concentrations through a data modeling method, based on the datasets; S105: for pollutants, data of which is not monitored online by the CEMS, obtaining a corresponding relationship of the boiler operating data and the coal quality parameters with outlet pollutant concentrations through a data modeling method according to coal quality data and the test report, based on the datasets; and S106: combining the model obtained in S104 and the model obtain in S105 to obtain the multi-pollutant concentration prediction model of the boiler.
6. The global optimization method of an intelligent multi-pollutant ultra-low emission system according to claim 4, wherein the model for accurately describing the multi-pollutant simultaneous removal process of the desulfurization system is obtained specifically through the following steps: S201: collecting design parameters and test reports of all devices of the desulfurization system; S202: collecting online operating historical data of the desulfurization system, including boiler load, inlet flue gas parameters, flue gas rate, pH, liquid-gas ratio, slurry density, and inlet concentration and outlet concentrations; S203: marking out typical load intervals and pollutant concentration intervals according to data distribution, and obtaining corresponding datasets of boiler loads, coal qualities and outlet pollutant concentrations in the typical boiler load intervals and the pollutant concentration intervals; S204: based on the datasets, establishing an SO.sub.2 removal mechanism model in the typical boiler load intervals and in the pollutant concentration intervals according to an SO.sub.2 removal mechanism of a desulfurization tower, and correcting the model according to historical data to obtain corresponding relationships of inlet SO.sub.2 concentration, inlet flue gas parameters, liquid-gas ratio, slurry density and pH with outlet SO.sub.2 concentration in the typical boiler load intervals and the pollutant concentration intervals; S205: based on the datasets, obtaining corresponding relationships of inlet SO.sub.3 concentration, inlet SO.sub.2 concentration, inlet dust content, inlet flue gas temperature, liquid-gas ratio and flue gas velocity with outlet SO.sub.3 concentration of the desulfurization system and corresponding relationships of inlet Hg concentration, inlet dust content, load, flue gas velocity and inlet flue gas temperature with outlet Hg concentration, in the typical boiler load intervals and the pollutant concentration intervals through a data modeling method according to results of the test reports; and S206: based on these corresponding relationships, obtaining the model for accurately describing the multi-pollutant simultaneous removal and transformation process of the desulfurization system under different conditions and operating parameters; the model for accurately describing the multi-pollutant simultaneous removal and transformation process of the denitration system is established specifically through the following steps: S301: collecting design parameters of a denitration device, catalyst parameters, a catalyst test report, and a reducer test report; S302: collecting historical data having an influence on online operation of the denitration device, including boiler load, operating temperature, flue gas rate, reducer supply, and inlet and outlet pollutant concentrations detected by the CEMS; S303: marking out typical load intervals and a pollutant concentration intervals according to data distribution, and obtaining corresponding datasets of boiler load, coal quality and outlet pollutant concentration in the typical boiler load intervals and the pollutant concentration intervals; S304: based on the datasets, establishing a mechanism model of the denitration device in the typical boiler load intervals and the pollutant concentration intervals according to an NO.sub.x removal mechanism of the denitration system, and correcting the model according to the historical data to obtain corresponding relationships of inlet NO.sub.x concentration, flue gas parameter, reaction condition and reducer supply with the outlet NO.sub.x concentration of the denitration device, in the typical boiler load intervals and the pollutant concentration intervals; S305: based on the datasets, obtaining corresponding relationships of inlet SO.sub.2 concentration, flue gas parameters, reaction condition and reducer supply with the SO.sub.2-to-SO.sub.3 transformation rate in the denitration device, and corresponding relationships of inlet Hg concentration, flue gas parameters, reaction condition and reducer supply with the transformation rate of particulate mercury, mercury oxides and elementary mercury in the denitration system, in the typical boiler load intervals and the pollutant concentration intervals according to results in the test reports through a data modeling method; and S306: based on these corresponding relationships, obtaining the model for accurately describing the multi-pollutant simultaneous removal and transformation process of the denitration system under different conditions and operating parameters; the model for accurately describing the multi-pollutant simultaneous removal process of the precipitation system is established specifically through the following steps: S401: collecting design parameters and test reports of electrostatic precipitators; S402: collecting historical data having an influence on online operation of the electrostatic precipitators, including boiler load, operating temperature, flue gas rate, secondary voltage, secondary current, and inlet and outlet pollutant concentrations detected by the CEMS; S403: marking out typical load intervals and pollutant concentration intervals according to data distribution, and obtaining corresponding datasets of boiler load, coal quality and outlet pollutant concentration in the typical boiler load intervals and the pollutant concentration intervals; S404: based on the datasets, establishing PM removal mechanism models of the electrostatic precipitators in the typical boiler load intervals and the pollutant concentration intervals according to a PM removal mechanism of the electrostatic precipitators, and correcting the models by means of the historical data to obtain corresponding relationships of inlet PM concentration, flue gas parameter and operating voltage with the outlet PM concentration of the electrostatic precipitators, in the typical boiler intervals and the pollutant concentration intervals; S405: based on the datasets, obtaining corresponding relationships of inlet SO.sub.3 concentration, inlet PM concentration, boiler load, operating temperature, flue gas rate operating voltage and outlet SO3 concentration and corresponding relationships of inlet Hg concentration, inlet PM concentration, boiler load, operating temperature, flue gas rate, operating voltage and outlet Hg concentration in the typical boiler load interval and the pollutant concentration interval through a data modeling method according to results of the test report; and S406: based on these corresponding relationships, obtaining the model for accurately describing the multi-pollutant simultaneous removal and transformation process of the precipitation system under different conditions and operating parameters.
7. The global optimization method of an intelligent multi-pollutant ultra-low emission system according to claim 6, wherein by means of accurate modeling of the multi-pollutant removal and transformation process of the denitration system, real-time description of a dynamic transformation process of NO.sub.x, SO.sub.2, SO.sub.3 and Hg and accurate prediction of the concentration are realized; during accurate modeling of the multi-pollutant simultaneous removal process of the desulfurization system, inlet flue gas parameters include inlet flue gas temperature, inlet SO.sub.2 concentration, inlet SO.sub.3 concentration, inlet particulate matter concentration and inlet Hg concentration, and outlet flue gas parameters include outlet flue gas temperature, outlet SO2 concentration, outlet SO3 concentration, outlet particulate matter concentration and outlet Hg concentration; the established mechanism models are corrected by coherent combination.
8. The global optimization method of an intelligent multi-pollutant ultra-low emission system according to claim 3, wherein the global operating cost evaluation method of the ultra-low emission system specifically includes operating costs and fixed costs of all pollutant emission reduction systems; regarding to a limestone-gypsum wet desulphurization system, a total operating cost and a fixed cost are expressed as:
COST.sub.WFGD=COST.sub.bf+COST.sub.sa+COST.sub.scp+COST.sub.oab+COST.sub.CaCo.sub.
COST.sub.WFGD_fix=COST.sub.WwFGD_d+COST.sub.WFGD_r+COST.sub.WFGD_m wherein, power consumption of booster fans COST.sub.bf, power consumption of oxidization blowers COST.sub.sa, power consumption of slurry circulating pumps COST.sub.scp, power consumption of slurry agitators COST.sub.oab, a limestone slurry cost COST.sub.CaCO.sub.
V=m×q×V.sub.tc wherein, V.sub.tc is the amount of flue gas generated by coal per unit, and m is coal quality; the process water consumption is calculated as follows:
COST.sub.SCR=COST.sub.SCR_idf+COST.sub.sb+COST.sub.adf COST.sub.NH.sub.
COST.sub.SCR_fix=COST.sub.SCR_d+COST.sub.SCR_r+COST.sub.SCR_m the operating cost includes energy consumption and material consumption, and the energy consumption includes power consumption of induced draft fans, power consumption of soot blowers and power consumption of dilution fans, which are respectively calculated as follows:
COST.sub.ESP=COST.sub.ESP_idf+COST.sub.ESP_e
COST.sub.EST_fix=COST.sub.ESP_d COST.sub.ESP_r+COST.sub.ESP_m
COST.sub.WESP=COST.sub.WESP_idf+COST.sub.WESP_e+COST.sub.WESP_w+COST.sub.Na+COST.sub.WC
COST.sub.WESP_fix=COST.sub.WESP_d+COST.sub.WESP_r+COST.sub.WESP_m the operating costs include power consumption, power consumption of a dry electrostatic precipitator includes power consumption of induced draft fans and power consumption of power supplies, which are respectively calculated as follows:
9. The global optimization method of an intelligent multi-pollutant ultra-low emission system according to claim 3, wherein based on accurate modeling of the multi-device multi-pollutant simultaneous removal process and global operating cost evaluation, the multi-pollutant, multi-target and multi-condition global operating optimization method is applied to a typical intelligent multi-pollutant ultra-low emission system constituted by an SCR denitration system, a dry electrostatic precipitation system, a wet flue gas desulphurization system and a wet electrostatic precipitation system to realize minute-level planning and optimization of emission reductions of a global pollutant emission reduction device under different emission targets through sub-disciplinary decomposition of different pollutants and global and local swarm intelligence algorithms by means of a simultaneous removal effect of the devices on the pollutants and a mutual inter-coupling and competition relationship of the pollutants.
10. The global optimization method of an intelligent multi-pollutant ultra-low emission system according to claim 9, wherein a disperse policy decision method based on a collaborative optimization algorithm is used as a solution to multi-model optimization of the operation of the complicated intelligent multi-pollutant ultra-low emission system; according to the collaborative optimization algorithm, expected values of coupling variables are transmitted from a system level to discipline levels at first, and under the condition of meeting corresponding constraints, the discipline levels are separately optimized to make optimization results closest to the expected values provided by the system level; then, the optimization results are transmitted to the system level; after receiving the optimization results of the discipline levels, the system level coordinates the coupling variables and generates new expected values of the coupling variables; the new expected values are transmitted to the discipline levels again; a feasible solution that makes the coupling variables consistent and meets optimization targets is finally obtained through repeated iterations between the system level and the discipline levels.
11. The global optimization method of an intelligent multi-pollutant ultra-low emission system according to claim 9, wherein according to the advanced control method for reliable up-to-standard ultra-low emission of the pollutants, dynamic property response models of manipulated variables and disturbance parameters of pollutant removal devices to pollutant removal are established based on real-time data, and under the condition of set emission reduction values of the devices for global optimization, control variables of the pollutant removal devices are optimized and controlled in real time through a model prediction and control method; the dynamic property response models are updated online to better adapt to large-delay, non-linearity and variable-load characteristics of the system, and even if system parameters change, margin control of pollutant emission can be realized, and pollutant removal costs are further reduced when the system varies.
12. The global optimization method of an intelligent multi-pollutant ultra-low emission system according to claim 11, wherein nine pollutant-removal dynamic property response models for load increase, load decrease and load maintaining under high, medium and small load conditions are established, and in different load change stages, different dynamic property response models are used to calculate control variables of the pollutant removal devices to better conform to actual changes of the system; online updating of the models refer to parameter substitutions of the models every a certain period of time in case of not meeting dynamic response properties, and the period of time varies according to different properties of the desulfurization system, the denitration system and the precipitation system; the model of the denitration system will be updated every one hour, the model of the desulfurization system will be updated every one day, and the model of the precipitation system will be updated every ten minutes.
Description
BRIEF DESCRIPTION OF THE SEVERAL VIEWS OF THE DRAWINGS
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DETAILED DESCRIPTION OF THE INVENTION
[0112] The present invention is further explained below in conjunction with the accompanying drawings and specific embodiments, but the protection scope of the invention is not limited to the following description.
[0113] Referring to
[0114] Referring to
[0115] The sensing layer of the intelligent multi-pollutant ultra-low emission system mainly comprises a physical sensing system and a network structure (including a bottom layer, an intermediate layer and an upper layer). The physical sensing layer mainly comprises a flue gas online monitoring system, a local detection and feedback system for DCS key elements (such as analog signals fed back by pump motors and switch quantity signals fed back by valves), and a measurement system included in the DCS system (liquid level, pH and liquid density detectors). The bottom layer of the network structure is an upgraded DCS control layer originally possessed by an enterprise and is a basic control network segment. The intermediate layer of the network structure is a data acquisition and processing layer of the intelligent multi-pollutant ultra-low emission system and is configured with an operation server, a database server, a WEB server, an application server and the like. The upper layer of the network structure is an enterprise management layer, is an office network segment based on an original intranet of an enterprise and allows users to have access to the intelligent multi-pollutant ultra-low emission system easily by visiting a website. The sensing layer is an information hinge of the intelligent multi-pollutant ultra-low emission system, communicates with the original DCS system of the intelligent multi-pollutant ultra-low emission system in real time through an OPC service, and is used for acquiring, preprocessing, integrating, storing and issuing information by means of a pollutant online detection device, a distributed control system and other sensing and communication systems.
[0116] The control layer of the intelligent multi-pollutant ultra-low emission system is an important intermediate layer for controlling key manipulated variables according to real-time operating conditions and optimized parameter settings to guarantee stable up-to-standard operation and optimal regulation of the system. Advanced control methods including optimizing control logics, optimizing manipulated variables and controlling target optimization values are established by studying the operating characteristics and key influence factors of all the key devices to realize advanced control of the pollutant removal process of the intelligent multi-pollutant ultra-low emission system, promote rational allocation of energy and resources and improve the pollutant control level.
[0117] The optimization layer is a key layer for realizing efficient simultaneous removal of multiple pollutants in the intelligent multi-pollutant ultra-low emission system, fulfills the optimization of global set points by establishing an optimization model, a prediction model and a cost evaluation model, and has the functions of balancing emission reductions of all the devices and optimizing global material and energy distributions of the ultra-low emission system. Referring to of all pollutant emission reduction devices are obtained according to a predicted global optimization setting vector value
output by the optimization model; the cost evaluation model evaluates the operation of the ultra-low emission system and obtains a specific cost vector
according to
and √{square root over (sp.sub.p.sup.y)}; the optimization model optimizes
through by establishing an optimization algorithm.
[0118] Referring to
[0119] According to the present invention, a boiler performance database, an environmentally-friendly device performance database, a system operating database, and a raw material (coal quality, absorbent, or the like) database are established by acquiring key parameters of the key devices of the system and a boiler and establishing the cost evaluation model and the pollutant prediction model to generate secondary parameters of the system such as energy consumption and target rates. The boiler performance database and a coal quality database are used to predict the concentration of multiple pollutants at a boiler outlet. The device performance database, an absorbent characteristic database and the system operating database are used to predict the concentration of multiple pollutants on the cross-section of inlets/outlets of the environmentally-friendly devices.
[0120] Referring to
[0121] Accurate modeling of the multi-device multi-pollutant simultaneous removal process of the ultra-low emission system includes accurate prediction of a multi-pollutant generation process, accurate modeling of a multi-pollutant simultaneous removal process of a desulfurization system, accurate modeling of a multi-pollutant simultaneous removal and transformation process of a denitration system, and accurate modeling of a multi-pollutant removal process of a precipitation system.
[0122] Accurate prediction of the multi-pollutant generation process: a boiler operating database and a multi-pollutant outlet concentration database under different conditions and variable coal qualities are established by acquiring long-term operating data of a boiler and a pollutant continuous emission monitoring system (CEMS) and combining coal quality detection data and test reports of multiple pollutants including NO.sub.x, SO.sub.2, SO.sub.3, PM and Hg; and a model for describing a corresponding relationship of boiler parameters and coal quality parameters with the concentrations of the multiple pollutants at a boiler outlet under different coal qualities and loads is established based on the boiler operating database and the multi-pollutant outlet concentration database.
[0123] Accurate modeling of the multi-pollutant simultaneous removal process of the desulfurization system: based on the generation, migration and transformation mechanism of the multiple pollutant as well as the removal mechanism of the multiple pollutants in the desulfurization system, a corresponding relationship of inlet SO.sub.2 concentration, inlet flue gas temperature, liquid-gas ratio, slurry density and pH with outlet SO.sub.2 concentration of the desulfurization system, a corresponding relationship of inlet SO.sub.3 concentration, inlet SO.sub.2concentration, inlet dust content, inlet flue gas temperature, liquid-gas ratio and flue gas velocity with outlet SO.sub.3 concentration of the desulfurization system, and a corresponding relationship of inlet Hg concentration, inlet dust content, load, flue gas velocity and inlet flue gas temperature with outlet Hg concentration are established according to coal quality, boiler operating parameters and inlet flue gas parameters of the desulfurization system, and then a model for accurately describing the multi-pollutant simultaneous removal process of the desulfurization system is obtained.
[0124] Accurate modeling of the multi-pollutant simultaneous removal and transformation process of the denitration system: based on the operating mechanism of an SCR denitration system, a corresponding relationship of inlet NO.sub.x concentration, flue gas parameters, reaction condition and reducer supply with outlet NO.sub.x concentration of the denitration system, a corresponding relationship of inlet SO.sub.2 concentration, flue gas parameters, reaction condition and reducer supply with SO.sub.2-to-SO.sub.3 transformation rate in the denitration system, and a corresponding relationship of inlet Hg concentration, flue gas parameters, reaction condition and reducer supply with transformation ratio of particulate mercury (Hg.sup.P), mercury oxides (Hg.sup.2+ and Hg.sup.+) and elementary mercury)(Hg.sup.0) in the denitration system are established by combining inlet flue gas parameters, online detection results of the CEMS and operating parameter historical data of the denitration system; then, a model for accurately describing the multi-pollutant simultaneous removal and transformation process of the denitration system under different conditions and operating parameters is obtained based on these corresponding relationships.
[0125] Accurate modeling of the multi-pollutant removal process of the precipitation system: based on the particulate matter removal mechanism of an electrostatic precipitation system, a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, operating voltage and outlet particulate matter concentration of a dry electric precipitator, a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, theoretical SO.sub.3 concentration of the denitration system, operating voltage and outlet SO.sub.3 concentration of the dry electric precipitator, a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, theoretical Hg concentration of the denitration system and outlet Hg concentration of the dry electric precipitator, a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, circulating water quantity, operating voltage and outlet particulate matter concentration of a wet electric precipitator, a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, inlet NO.sub.x concentration, circulating water quantity, circulating water pH, operating voltage and outlet NO.sub.x concentration of the wet electric precipitator, a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, inlet SO.sub.2 concentration, circulating water quantity, circulating water pH, operating voltage and outlet SO.sub.2 concentration of the wet electric precipitator, a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, inlet SO.sub.3 concentration, circulating water quantity, circulating water pH, operating voltage and outlet SO.sub.3 concentration of the wet electric precipitator, and a corresponding relationship of coal quality, load, flue gas temperature, flue gas rate, inlet Hg concentration, circulating water quantity, circulating water pH, operating voltage and outlet Hg concentration of the wet electric precipitator are established by combining coal quality, boiler operating parameters, inlet flue gas parameters of the electrostatic precipitation system, and historical operating data; then, a model for accurately describing the multi-pollutant simultaneous removal process of the precipitation system is obtained.
[0126] Preferably, accurate prediction of the multi-pollutant generation process refers to accurate prediction of the concentration of multiple pollutants, including NO.sub.x, SO.sub.2, SO.sub.3, PM and Hg at the boiler outlet according to real-time boiler operating data and periodically-updated coal quality reports.
[0127] A boiler model is established through the following steps:
[0128] S101: collecting boiler parameters, coal quality parameters and a boiler outlet test report;
[0129] S102: collecting long-term operating historical data including boiler coal feed, flue gas, water, and boiler outlet pollutant concentrations detected by the CEMS;
[0130] S103: marking out typical boiler load intervals (100%, 75%, 50%, etc.) according to the test report and online operating data, and obtaining a corresponding datasets of boiler operating parameters, coal qualities and outlet pollutant concentrations in the typical boiler load intervals;
[0131] S104: for pollutants, data of which is monitored online by the CEMS, obtaining a corresponding relationship of the boiler operating data and coal quality parameters with outlet pollutant concentrations through a data modeling method (a neural network algorithm is adopted in this embodiment), based on the datasets;
[0132] S105: for pollutants, data of which is not monitored online by the CEMS, obtaining a corresponding relationship of the boiler operating data and the coal quality parameters with outlet pollutant concentrations through a data modeling method (a neural network algorithm is adopted in this embodiment) according to coal quality data and the test report, based on the datasets; and
[0133] S106: combining the model obtained in S104 and the model obtain in S105 to obtain a boiler-side multi-pollutant concentration prediction model.
[0134] Preferably, the model for accurately describing the multi-pollutant simultaneous removal process of the desulfurization system is obtained specifically through the following steps:
[0135] S201: collecting design parameters and test reports of all devices of the desulfurization system;
[0136] S202: collecting online operating historical data of the desulfurization system, including boiler load, inlet flue gas parameters, flue gas rate, pH, liquid-gas ratio, slurry density, and inlet concentration and outlet concentrations;
[0137] S203: marking out typical load intervals and pollutant concentration intervals according to data distribution, and obtaining corresponding datasets of boiler loads, coal qualities and outlet pollutant concentrations in the typical boiler load intervals and the pollutant concentration intervals;
[0138] S204: based on the datasets, establishing an SO.sub.2 removal mechanism model in the typical boiler load intervals and the pollutant concentration intervals according to the SO.sub.2 removal mechanism of a desulfurization tower, and correcting the model according to historical data to obtain corresponding relationships of inlet SO.sub.2 concentration, inlet flue gas parameters, liquid-gas ratio, slurry density and pH with outlet SO.sub.2 concentration in the typical boiler load intervals and the pollutant concentration intervals;
[0139] S205: based on the datasets, obtaining corresponding relationships of inlet SO.sub.3 concentration, inlet SO.sub.2 concentration, inlet dust content, inlet flue gas temperature, liquid-gas ratio and flue gas velocity with outlet SO.sub.3 concentration of the desulfurization system and corresponding relationships of inlet Hg concentration, inlet dust content, load, flue gas velocity and inlet flue gas temperature with outlet Hg concentration in the typical boiler load intervals and the pollutant concentration intervals through a data modeling method according to results of the test reports; and
[0140] S206: based on these corresponding relationships, obtaining the model for accurately describing the multi-pollutant simultaneous removal and transformation process of the desulfurization system under different conditions and operating parameters.
[0141] The model for accurately describing the multi-pollutant simultaneous removal and transformation process of the denitration system is established specifically through the following steps:
[0142] S301: collecting design parameters of a denitration device, catalyst parameters, a catalyst test report, and a reducer test report;
[0143] S302: collecting historical data having an influence on online operation of the denitration device, including boiler load, operating temperature, flue gas rate, reducer supply, and inlet and outlet pollutant concentrations detected by the CEMS;
[0144] S303: marking out typical load intervals and pollutant concentration intervals according to data distribution, and obtaining corresponding datasets of boiler load, coal quality and outlet pollutant concentration in the typical boiler load intervals and the pollutant concentration intervals;
[0145] S304: based on the datasets, establishing a mechanism model of the denitration device in the typical boiler load intervals and the pollutant concentration intervals according to the NO.sub.x removal mechanism of the denitration system, and correcting the model according to the historical data to obtain corresponding relationships of inlet NO.sub.x concentration, flue gas parameter, reaction condition and reducer supply with the outlet NO.sub.x concentration of the denitration device, in the typical boiler load intervals and the pollutant concentration intervals;
[0146] S305: based on the datasets, obtaining corresponding relationships of inlet SO.sub.2 concentration, flue gas parameters, reaction condition and reducer supply with the SO.sub.2-to-SO.sub.3 transformation rate in the denitration device, and corresponding relationships of inlet Hg concentration, flue gas parameters, reaction condition and reducer supply with the transformation rate of particulate mercury, mercury oxides and elementary mercury in the denitration system, in the typical boiler load interval and the pollutant concentration intervals according to results in the test reports through a data modeling method (a neural network algorithm is adopted in this embodiment); and
[0147] S306: based on these corresponding relationships, obtaining the model for accurately describing the multi-pollutant simultaneous removal and transformation process of the denitration system under different conditions and operating parameters.
[0148] The model for accurately describing the multi-pollutant simultaneous removal process of the precipitation system is established specifically through the following steps:
[0149] S401: collecting design parameters and test reports of electrostatic precipitators;
[0150] S402: collecting historical data having an influence on online operation of the electrostatic precipitators, including boiler load, operating temperature, flue gas rate, secondary voltage, secondary current, and inlet and outlet pollutant concentrations detected by the CEMS;
[0151] S403: marking out typical load intervals and pollutant concentration intervals according to data distribution, and obtaining corresponding datasets of boiler loads, coal quality and outlet pollutant concentration in the typical boiler load intervals and the pollutant concentration intervals;
[0152] S404: based on the datasets, establishing PM removal mechanism models of the electrostatic precipitators in the typical boiler load intervals and the pollutant concentration intervals according to the PM removal mechanism of the electrostatic precipitators, and correcting the models by means of the historical data to obtain corresponding relationships of inlet PM concentration, flue gas parameter and operating voltage with the outlet PM concentration of the electrostatic precipitators, in the typical boiler intervals and the pollutant concentration intervals;
[0153] S405: based on the datasets, obtaining corresponding relationships of inlet SO.sub.3 concentration, inlet PM concentration, boiler load, operating temperature, flue gas rate operating voltage and outlet SO.sub.3 concentration and corresponding relationships of inlet Hg concentration, inlet PM concentration, boiler load, operating temperature, flue gas rate, operating voltage and outlet Hg concentration in the typical boiler load interval and the pollutant concentration interval through a data modeling method according to results of the test report; and
[0154] S406: based on these corresponding relationships, obtaining the model for accurately describing the multi-pollutant simultaneous removal and transformation process of the precipitation system under different conditions and operating parameters.
[0155] Modeling of the SO.sub.2 removal mechanism comprises:
[0156] Calculating the SO.sub.2 removal rate:
[0157] wherein, dC.sub.so.sub.
[0158] In a spray tower, the quantity of SO.sub.2 removed from flue gas is equal to the quantity of SO.sub.2 absorbed by slurry, and in case where the spray tower adopts an infinitesimal height dz, the following mass transfer equation is obtained:
[0159] Wherein, K.sub.OG is a total mass transfer coefficient of a gas phase and a liquid phase, kmol/(m.sup.2×s); a is a mass transfer area per unit volume, m.sup.2/m.sup.3; P is a total pressure, Pa; y is a molar fraction of SO.sub.2 in the gas phase, y* is an equilibrium molar fraction of SO.sub.2 in a gas film; G is a flue gas rate, kmol/(m.sup.2×s); dy is a differential of the molar fraction in the gas phase; Simplification of the desulfurization system: assume the flow rate in the vertical direction is constant and the total mass transfer coefficient is constant, an absorption height Z is obtained by integrating dz in the above equation:
[0160] Wherein, (1−y).sub.LM is the logarithmic mean values of (1−y*) and (1−y), and the SO.sub.2 absorption process in the desulfurization tower is approximate to 1; m is an average thrust of the gas film of the desulfurization tower; y.sub.1 is a molar fraction of an inlet gas phase; y.sub.2 is a molar fraction of an outlet gas phase.
[0161] The basic form of the mechanism model is:
c.sub.out=c.sub.in*exp(−NTU)
[0162] Wherein, c.sub.out and c.sub.in are respectively an inlet SO.sub.2 concentration and an outlet SO.sub.2 concentration, and NTU is the number of mass transfer elements, which refers to the difficulty level of an absorption tower to absorb SO.sub.2 and is mathematically expressed as:
[0163] Parameters having an influence on NTU include: slurry pH, Ca/S ratio and gas-liquid ratio;
[0164] The total mass transfer coefficient of a spray region is:
[0165] According to the unsteady-state penetration theory, k.sub.G is the absorptivity of the gas film, kmol/(m.sup.2.Math.s.Math.kPa); β.sub.SO.sub.
[0166] Modeling of the particulate matter removal mechanism specifically comprises:
[0167] The grade efficiency η.sub.n(d.sub.p, t) is defined as the ratio of the total amount of collected soot particles at moment t and scale d.sub.p to an initial amount:
[0168] d.sub.p.sup.− and d.sub.p.sup.+ respectively present an upper limit and a lower limit of a particle interval at scale d.sub.p, and N.sub.p(d.sub.p,t) represents the total amount of soot particles at scale d.sub.p; dd.sub.p represents a differential of scale d.sub.p, and n.sub.p(d.sub.p,t) refers to the amount of correspondingly graded soot particles at moment t and scale d.sub.p.
[0169] The following equations can be obtained by integrating the variable d.sub.p:
[0170] Λ(d.sub.p) is a deposition kernel (removal coefficient) which refers to the removal rate of particles at scale d.sub.p by slurry drops (unit: s−1) and is expressed as:
Λ(d.sub.p)=∫.sub.D.sub.
[0171] The relationship of the deposition kernel and the grade efficiency η.sub.m(d.sub.p, t) is:
η.sub.m(d.sub.p,t)≈η.sub.n(d.sub.p,t)=1−exp(−Λ(d.sub.p)×t)
[0172] The overall grade efficiency η.sub.total(t) is defined as the ratio of the total mass of particles at all scales collected at moment t to an initial mass:
[0173] Wherein, ρ.sub.p refers to the density, and n.sub.p(d.sub.p, 0) refers to the amount of correspondingly graded soot particles at the initial moment and scale d.sub.p.
[0174] Preferably, by means of accurate modeling of the multi-pollutant removal and transformation process of the denitration system, real-time description of the dynamic transformation process of NO.sub.x, SO.sub.2, SO.sub.3 and Hg and accurate prediction of the concentration are realized.
[0175] Preferably, during accurate modeling of the multi-pollutant simultaneous removal process of the desulfurization system, inlet flue gas parameters include inlet flue gas temperature, inlet SO.sub.2 concentration, inlet SO.sub.3 concentration, inlet particulate matter concentration (PM) and inlet Hg concentration, and outlet flue gas parameters include outlet flue gas temperature, outlet SO.sub.2 concentration, outlet SO.sub.3 concentration, outlet particulate matter (PM) concentration and outlet Hg concentration; the established mechanism models are corrected by coherent combination.
[0176] The form of coherent combination is as follows:
[0177] C.sub.SO.sub.
[0178] The influence of principal factors is mainly taken into consideration for the mechanism model, and the influence of secondary factors is taken into consideration for data correction.
[0179] Preferably, the global operating cost evaluation method of the ultra-low emission system specifically includes operating costs and fixed costs of all pollutant emission reduction systems.
[0180] Regarding to a limestone-gypsum wet desulphurization system, a total operating cost and a fixed cost are expressed as:
COST.sub.WFGD=COST.sub.bf+COST.sub.sa+COST.sub.scp+COST.sub.oab+COST.sub.CaCO.sub.
COST.sub.WFGD_fix=COST.sub.wFGD_d+COST.sub.WFGD_r+COST.sub.WFGD_m
[0181] Wherein, power consumption of booster fans COST.sub.bf, power consumption of oxidization blowers COST.sub.sa, power consumption of slurry circulating pumps COST.sub.scp, power consumption of slurry agitators COST.sub.oab, a limestone slurry cost COST.sub.CaCO.sub.
[0182] The operating cost of the desulfurization system includes energy consumption and material consumption, wherein the energy consumption is mainly generated by a motor of the desulfurization system and includes the power consumption of booster fans, the power consumption of oxidization blowers, the power consumption of slurry circulating pumps and the power consumption of the slurry agitators, and the costs are calculated as follows:
[0183] Wherein, q is a real-time boiler load, n.sub.bf,n.sub.sa, n.sub.scp and n.sub.oab respectively represent the number of booster fans in operation, the number of oxidization fans in operation, the number of slurry circulating pumps in operation and the number of slurry agitators in operation, U.sub.i and I.sub.i respectively represent the voltage and current of the i.sup.th facility, cosφ is a power factor and is generally 0.8, and P.sub.E is the electricity price;
[0184] a.sub.WFGD is the ratio of the resistance of the desulfurization tower to the total resistance of a second half of ultra-low emission system and is calculated as follows:
[0185] Wherein, p.sub.dt is a pressure drop of the desulfurization tower, P.sub.WESP is a pressure drop of the wet electrostatic precipitator under resistance, and p.sub.gd2 is a pressure drop of a gas duct under resistance.
[0186] Material consumption of the desulfurization system includes limestone consumption and process water consumption, a desulfurization absorber adopted by the limestone-gypsum wet desulphurization system is limestone slurry, and in accordance with material balance, the cost, namely limestone consumption, of power generation per unit is calculated as follows:
[0187] Wherein, c.sub.SO.sub.
V=m×q×V.sub.tc
[0188] Wherein, V.sub.tc is the amount of flue gas generated by coal per unit, and m is the coal quality.
[0189] The process water consumption is calculated as follows:
[0190] Wherein, M.sub.H.sub.
[0191] Because gypsum is generated as a by-product when SO.sub.2 in flue gas is removed, the gypsum, as revenue obtained in the operating process of the desulfurization system, is included in cost calculation of the limestone-gypsum wet desulfurization system, and the revenue is calculated as follows:
[0192] Wherein, M.sub.CaSO.sub.
[0193] The fixed cost of the desulfurization system includes the depreciation cost COSTWFGD_d, the repair cost COSTWFGD_r and the manual cost COSTWFGD_m which are respectively calculated as follows:
[0194] Wherein, Q is the capacity of a unit, H is annual operating hours of the unit, P.sub.WFGD_init is an initial investment cost of the desulfurization system, η.sub.WFGD is a fixed assets formation rate of the desulfurization system, Y.sub.WFGD is a depreciable life of the desulfurization system, η.sub.WFGD_r is the proportion of the repair cost of the desulfurization system to an investment cost, n.sub.wFGD is the total number of workers, and S.sub.WFGD.sub.
[0195] Regarding to the SCR denitration system, a total operating cost and a fixed cost are expressed as follows:
COST.sub.SCR=COST.sub.SCR_idf+COST.sub.sb+COST.sub.adf+COST.sub.NH.sub.
COST.sub.SCR_fix=COST.sub.SCR_d+COST.sub.SCR_r+COST.sub.SCR_m
[0196] The operating cost includes energy consumption and material consumption, and the energy consumption includes power consumption of induced draft fans, power consumption of soot blowers and power consumption of dilution fans, which are respectively calculated as follows:
[0197] Wherein, n.sub.idf, n.sub.sb and n.sub.adf are respectively the number of induced draft fans in operation, the number of soot blowers in operation and the number of dilution fans in operation, P.sub.steam is empirical steam consumption, CV.sub.s is empirical reference catalyst consumption, and CV is actual catalyst consumption;
[0198] a.sub.SCR represents the ratio of the resistance of a denitration reactor to the total resistance in the first half and is calculated as follows:
[0199] The material consumption of the denitration system includes a liquid ammonia cost and a catalyst cost, and in accordance with material balance, the liquid ammonia cost is calculated as follows:
[0200] Wherein, c.sub.No.sub.
[0201] The catalyst cost is calculated as follows:
[0202] Wherein, P.sub.c is the price of a catalyst, Q is the capacity of a unit, and h is the annual operating hours of the unit.
[0203] The fixed cost of the denitration system includes a depreciation cost COST.sub.SCR_d, a repair cost COST.sub.SCR_r and a manual cost COST.sub.SCR_m, which are respectively calculated as follows:
[0204] Wherein, P.sub.SCR_init is an initial investment cost of the denitration system, η.sub.SCR is a fixed assets formation rate of the denitration system, Y.sub.SCR is a depreciable life of the denitration system, η.sub.SCR_r is the proportion of the repair cost of the denitration system to the investment cost, n.sub.SCR is the total number of workers of the denitration system, and S.sub.SCR.sub.
[0205] Regarding to electrostatic precipitation systems, total operating costs and fixed costs of a dry electrostatic precipitation system and a wet electrostatic precipitation system are respectively expressed as follows:
COST.sub.ESP=COST.sub.ESP_idf+COST.sub.ESP_e
COST.sub.ESP_fix=COST.sub.ESP_d+COST.sub.ESP_r+COST.sub.ESP_m
COST.sub.WESP=COST.sub.WESP_idf+COST.sub.WESP_e+COST.sub.WESP_w,+COST.sub.Na+COST.sub.wc
COST.sub.WESP_fix=COST.sub.WESP_d+COST.sub.WESP_r+COST.sub.WESP_m
[0206] The operating costs include power consumption.
[0207] Power consumption of a dry electrostatic precipitator includes power consumption of induced draft fans and power consumption of power supplies, which are respectively calculated as follows:
[0208] Wherein, n.sub.e is the number of electric fields, and α.sub.ESP is the proportion of the resistance of the dry electrostatic precipitator to the total resistance in the first half and is calculated as follows:
[0209] Power consumption of a wet electrostatic precipitator includes power consumption of induced draft fans, power consumption of power supplies, a power cost and a material cost, and the power consumption of induced draft fans of the wet electrostatic precipitator is calculated as follows:
[0210] The power consumption of power supplies of the wet electrostatic precipitator is:
[0211] Compared with the dry electrostatic precipitator, the wet electrostatic precipitator has the power cost and the material cost, and the power cost mainly refers to power consumption of a water circulation system;
[0212] The material cost of the wet electrostatic precipitator includes a process water cost and an alkali consumption cost, which are calculated as follows:
[0213] The fixed costs of the dry electrostatic precipitation system and the wet electrostatic precipitation system include depreciation costs COST.sub.ESP_d and COST.sub.WESP_d, repair costs COST.sub.ESP_r and COST.sub.WESP_r, and manual costs COST.sub.ESP_m and COST.sub.WESP_m, which are respectively calculated as follows:
[0214] Wherein, P.sub.ESP_init and P.sub.WESP_init respectively represent initial investment costs of the dry electrostatic precipitation system and the wet electrostatic precipitation system, η.sub.ESP and η.sub.WESP respectively represent fixed assets formation rates of the dry electrostatic precipitation system and the wet electrostatic precipitation system, Y.sub.ESP and Y.sub.WESP respectively represent a depreciable life of the dry electrostatic precipitation system and a depreciable life of the wet electrostatic precipitation system, N.sub.ESP_r and n.sub.WESP_r respectively represent the ratio of the repair cost of the dry electrostatic precipitation system to the investment cost and the ratio of the repair cost of the wet electrostatic precipitation system to the investment cost, n.sub.ESP and n.sub.WESP respectively represent the total number of workers of the dry electrostatic precipitation system, and S.sub.ESP.sub.
[0215]
[0216] According to the invention, under high load and high pollutant concentration conditions, after pollutants are removed by the intelligent multi-pollutant ultra-low emission system, the actual concentration of NO.sub.x is 250 mg/m.sup.3, the actual concentration of PM is 15356.6 mg/m.sup.3, and the actual concentration of SO.sub.2 is 1200 mg/m.sup.3. The concentration of NO.sub.x is decreased to about 40 mg/m.sup.3 by the SCR system and is further decreased to be less than 35 mg/m.sup.3 under the simultaneous removal effect of the WFGD system. Most PM is removed by the ESP system which has a PM removal rate over 99%, the PM concentration at an outlet of the ESP system is only 12.07 mg/m.sup.3, and the PM concentration of flue gas is controlled to 1.25 mg/m.sup.3 under the removal effect of the WFGD system and the WESP system. Most SO.sub.2 is removed by the WFGD system, the SO.sub.2 concentration will be less than 20 mg/m.sup.3 after the flue gas flows through the WFGD system, and afterwards, the SO.sub.2 concentration is controlled to 12.69 mg/m.sup.3 under the simultaneous removal effect of the WESP system.
[0217] Based on accurate modeling of the multi-device multi-pollutant simultaneous removal process and global operating cost evaluation, the multi-pollutant, multi-target and multi-condition global operating optimization method is applied to the typical intelligent multi-pollutant ultra-low emission system constituted by the SCR denitration system, the dry electrostatic precipitation (ESP) system, the wet flue gas desulphurization (WFGD) system and the wet electrostatic precipitation (WESP) system to realize minute-level planning and optimization of emission reductions of a global pollutant emission reduction device under different emission targets through sub-disciplinary decomposition of different pollutants and global and local swarm intelligence algorithms by means of the simultaneous removal effect of the devices on the pollutants and the mutual inter-coupling and competition relationship of the pollutants.
[0218] NO.sub.x is not only subjected to an SCR reaction in the SCR denitration device, but also is absorbed by the desulfurization system, and main reactions are as follows:
NO.sub.2+H.sub.2O.fwdarw.HNO.sub.2+H.sup.++NO.sub.3.sup.−
NO+NO.sub.2+H.sub.2O.fwdarw.HNO.sub.2
[0219] Residual SO.sub.2 that is not removed by a limestone-gypsum wet desulphurization device can be removed along with the flowing of a washing solution when flue gas flows through the wet electrostatic precipitator. Residual PM that is not removed by the dry electrostatic precipitator and the wet electrostatic precipitator will be removed under the washing effect of slurry in the desulfurization tower.
[0220] According to the invention, a disperse policy decision method based on a collaborative optimization algorithm is used as a solution to multi-model optimization of the operation of the complicated intelligent multi-pollutant ultra-low emission system in a coal-fired power plant and has high system autonomy and good adaptability, and the models are resolved independently and have to be repeatedly coordinated to guarantee the consistency of decision results, which causes some communication costs, but the decision results are optimal because the solution process is carried out based on optimal solutions of the models.
[0221] Referring to
[0222] Referring to
[0223] System-level and discipline-level optimization problems are resolved by a particle swarm algorithm which has a high convergence rate and a wide application range.
[0224] Design variables of the discipline-level optimization problems include a coupling variable y and an uncoupling variable x, and the optimization problems are expressed as:
min J.sub.i(γ.sub.1)=Σ.sub.j=1.sup.s.sup.
s.t.g.sub.i(x.sub.i,y.sub.i)≤0
[0225] Wherein, y.sub.ij represents the j.sup.th coupling variable of the i.sup.th sub-discipline, z.sub.j* represents an expected value of the j.sup.th variable allocated to the sub-discipline by the system level, s.sub.i represents the number of coupling variables of the i.sup.th sub-discipline, n represents the number of the sub-disciplines, x.sub.i represents an uncoupling variable of the i.sup.th sub-discipline, and g.sub.i represents a constraint condition of the i.sup.th sub-discipline.
[0226] Design variables of the system-level optimization problem include a coupling variable z and an uncoupling variable w, and the optimization problem is expressed as:
minF(z,w)
s.t. Σ.sub.j=1.sup.s.sup.
[0227] Wherein, F represents a system-level target function, z.sub.j represents the j.sup.th coupling variable of the system level, y.sub.ij* represents an optimization result of the j.sup.th coupling variable of the i.sup.th sub-discipline, and ε is a relaxation factor.
[0228] By adoption of a dynamic relaxation factor, the optimization conditions can be met, and the optimal solution can be resolved at a high convergence rate. At the initial optimization stage, a large initial value is assigned to the relaxation factor to define a large feasible region to guarantee the existence of a feasible solution. With the continuation of iteration, the relaxation factor is decreased to narrow down the feasible region to further improve the consistency of the coupling variables.
[0229] If the optimal solution of the i.sup.th sub-discipline during k.sup.th iteration x.sub.i.sup.*(k), y.sub.i.sup.*(k) the maximum difference D between the sub-disciplines is defined as D=max∥y.sub.i.sup.*(k)−y.sub.j.sup.*(k)∥,i,j=1,2, . . . , n. If the optimal system-level solution during (k-1).sup.th iteration is z.sub.i.sup.*(k−1), w.sub.i.sup.*(k−1), a collaborative difference P.sub.i is defined as P.sub.i.sup.k=∥z.sub.i.sup.*(k−1)−y.sub.i.sup.*(k)∥, and the relaxation factor ε.sub.i.sup.k of the i.sup.th sub-discipline during k.sup.th iteration is ε.sub.i.sup.k=(λ.sub.i.sup.kD).sup.2+d, wherein d is a minimum positive number to guarantee the relaxation effect, and λ.sub.i.sup.k is defined as λ.sub.i.sup.k=0.5*(1−a.sup.P.sup.
[0230] Based on the RBT neural network models adopted in the pollutant removal process, the maximum iterations between the system level and the discipline level of the collaborative optimization algorithm is set to 50, the maximum iterations of the particle swarm algorithm is set to 50, and the number of particles is set to 100 to optimize the operating condition under a typical load and a typical inlet concentration.
[0231] According to the advanced control method for reliable up-to-standard ultra-low emission of the pollutants, dynamic property response models of manipulated variables and disturbance parameters of the pollutant removal devices to pollutant removal are established based on real-time data, and under the condition of set emission reduction values of the devices, control variables of the pollutant removal devices are optimized and controlled in real time through a model prediction and control method; the dynamic property response models are updated online to better adapt to large-delay, non-linearity and variable-load characteristics of the system, and even if system parameters change, margin control of pollutant emission can be realized, and pollutant removal costs are further reduced in case of changes to the system.
[0232] During global optimization, the set emission reduction values of the devices will be given to the control system, the control system will set each set value as an input variable, and the pollutant removal control effect should be close to the set values as much as possible. A dynamic property response model of manipulated variables and disturbance parameters of the pollutant removal devices to pollutant removal is established based on real-time data, and the model has nine sub-models for load increase, load decrease and load maintaining under high, medium and small load conditions, and in different load change stages, different sub-models are used to optimize and control variables of the pollutant removal devices through a model prediction control method. The dynamic property response model will be updated every period of time to ensure that operation parameters can be controlled when the removal model changes actually. Considering the properties of the desulfurization system, the model of the denitration system will be updated every one hour, the model of the desulfurization system will be updated every one, and the model the precipitation system will be updated every ten minutes.
[0233] By adoption of the above solutions, the invention can realize simultaneous removal of multiple flue gas pollutants by means of the key devices of the intelligent multi-pollutant ultra-low emission system, on the basis of existing ultra-low emission systems, improve the simultaneous removal effect of multiple pollutants such as nitrogen oxide, sulfur oxide, particulate matter and mercury, effectively improve the multi-pollutant efficient removal effect of flue gas emission reduction devices, greatly reduce operating costs, and improve the operating adaptability under different conditions.