A solid electrolyte (10) of the present disclosure includes porous silica (11) having a plurality of pores (12) interconnected mutually and an electrolyte (13) coating inner surfaces of the plurality of pores (12). The electrolyte (13) includes 1-ethyl-3-methylimidazolium bis(trifluoromethanesulfonyl)imide represented by EMI-TFSI and a lithium salt dissolved in the EMI-TFSI. A molar ratio of the EMI-TFSI to the porous silica (11) is larger than 1.5 and less than 2.0.

The present disclosure provides a method for forming a solid-state battery. The method includes stacking two or more cell units, where each cell unit is formed by substantially aligning a first electrode and a second electrode, where the first electrode includes one or more first electroactive material layers disposed on or adjacent to one or more surfaces of a releasable substrate and the second electrode includes one or more second electroactive material layers disposed on or adjacent to one or more surfaces of a current collector; disposing an electrolyte layer between exposed surfaces of the first electrode and the second electrode; and removing the releasable substrate to form the cell unit.

The present disclosure provides a method for forming a solid-state battery. The method includes stacking two or more cell units, where each cell unit is formed by substantially aligning a first electrode and a second electrode, where the first electrode includes one or more first electroactive material layers disposed on or adjacent to one or more surfaces of a releasable substrate and the second electrode includes one or more second electroactive material layers disposed on or adjacent to one or more surfaces of a current collector; disposing an electrolyte layer between exposed surfaces of the first electrode and the second electrode; and removing the releasable substrate to form the cell unit.

A method for manufacturing a lithium-ion microbattery having a capacity not exceeding 1 mAh, implementing a method for manufacturing an assembly comprising a porous electrode and a porous separator comprising a porous layer deposited on a substrate having a porosity comprised between 20% and 60% by volume, and pores with an average diameter of less than 50 nm. The separator comprises a porous inorganic layer deposited on the electrode, the porous inorganic layer having a porosity comprised between 20% and 60% by volume, and pores with an average diameter of less than 50 nm.

The present invention provides a crosslinker of formula (I) for electrolytes, and a electrolyte composition and a lithium-ion battery including the same, wherein M, R and X are as defined in the description. With the crosslinker of formula (I), not only the mechanical strength, heat resistance, ionic conductivity and electrochemical stability of the prepared electrolyte composition are improved, but also the long-term charge-discharge cycling stability of the lithium-ion battery is improved. The crosslinker has high industrial value.

The present invention provides a crosslinker of formula (I) for electrolytes, and a electrolyte composition and a lithium-ion battery including the same, wherein M, R and X are as defined in the description. With the crosslinker of formula (I), not only the mechanical strength, heat resistance, ionic conductivity and electrochemical stability of the prepared electrolyte composition are improved, but also the long-term charge-discharge cycling stability of the lithium-ion battery is improved. The crosslinker has high industrial value.

A negative electrode for a lithium secondary battery includes a negative electrode current collector and a negative electrode layer. The negative electrode layer includes a composite layer and a single lithium metal layer. The composite layer includes, as a negative electrode active material, an alloy of lithium metal and dissimilar metal. The composite layer and the single lithium metal layer are arranged in this order from the negative electrode current collector. The dissimilar metal is an element that is able to form a solid solution with the lithium metal or an element that is able to form an intermetallic compound with the lithium metal.

The present invention provides a separator formed by hydrolysis of a resin film. The resin film comprises a non-hydrolyzable organic polymer; and a hydrolyzable organic polymer being hydrolyzable by treatment with at least one of an acid aqueous solution, an alkaline aqueous solution and pure water, wherein the content of the hydrolyzable organic polymer ranges from 10 parts by weight to 70 parts by weight relative to 100 parts by weight of the resin film. The separator of the present invention has good ion conductivity and thus, is extremely suitable for use in various types of batteries.

A solid-state lithium-ion battery may include a metal layer. A solid-state lithium-ion battery may include a cathode layer disposed in the metal layer. A solid-state lithium-ion battery may include a reinforced lithiated composite electrolyte layer disposed on the cathode layer. A solid-state lithium-ion battery may include a lithiated ionomer coating layer disposed on the reinforced lithiated composite electrolyte layer. A solid-state lithium-ion battery may include an anode layer disposed on the lithiated ionomer coating layer.

A solid-state lithium-ion battery may include a metal layer. A solid-state lithium-ion battery may include a cathode layer disposed in the metal layer. A solid-state lithium-ion battery may include a reinforced lithiated composite electrolyte layer disposed on the cathode layer. A solid-state lithium-ion battery may include a lithiated ionomer coating layer disposed on the reinforced lithiated composite electrolyte layer. A solid-state lithium-ion battery may include an anode layer disposed on the lithiated ionomer coating layer.